Articles | Volume 19, issue 5
Atmos. Chem. Phys., 19, 2947–2964, 2019
https://doi.org/10.5194/acp-19-2947-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Atmos. Chem. Phys., 19, 2947–2964, 2019
https://doi.org/10.5194/acp-19-2947-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article 07 Mar 2019
Research article | 07 Mar 2019
Fine dust emissions from active sands at coastal Oceano Dunes, California
Yue Huang et al.
Related authors
Akinori Ito, Adeyemi A. Adebiyi, Yue Huang, and Jasper F. Kok
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-134, https://doi.org/10.5194/acp-2021-134, 2021
Preprint under review for ACP
Short summary
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We improve the simulated dust properties with datasets that leverage measurements of size-resolved dust concentration and particle shape. The improved simulation suggests much less atmospheric radiative heating over the major source regions, compared to the default simulation. The less intensified atmospheric heating due to mineral dust could substantially modify vertical temperature profile in Earth system models, and thus has important implications for the projection of dust feedback.
Jasper F. Kok, Adeyemi A. Adebiyi, Samuel Albani, Yves Balkanski, Ramiro Checa-Garcia, Mian Chin, Peter R. Colarco, Douglas S. Hamilton, Yue Huang, Akinori Ito, Martina Klose, Longlei Li, Natalie M. Mahowald, Ron L. Miller, Vincenzo Obiso, Carlos Pérez García-Pando, Adriana Rocha-Lima, and Jessica S. Wan
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-4, https://doi.org/10.5194/acp-2021-4, 2021
Preprint under review for ACP
Short summary
Short summary
The many impacts of dust on the Earth system depend on dust mineralogy, which varies between dust source regions. We constrain the contribution of the world's main dust source regions by integrating dust observations with global model simulations. We find that Asian dust contributes more, and that North African dust contributes less, than models account for. We obtain a data set of each source region's contribution to the dust cycle that can be used to constrain dust impacts on the Earth system.
Jasper F. Kok, Adeyemi A. Adebiyi, Samuel Albani, Yves Balkanski, Ramiro Checa-Garcia, Mian Chin, Peter R. Colarco, Douglas Stephen Hamilton, Yue Huang, Akinori Ito, Martina Klose, Danny M. Leung, Longlei Li, Natalie M. Mahowald, Ron L. Miller, Vincenzo Obiso, Carlos Pérez García-Pando, Adriana Rocha-Lima, Jessica S. Wan, and Chloe A. Whicker
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-1131, https://doi.org/10.5194/acp-2020-1131, 2020
Preprint under review for ACP
Short summary
Short summary
Desert dust interacts with virtually every component of the Earth system, including the climate system. We develop a new methodology to represent the global dust cycle that integrates observational constraints on the properties and abundance of desert dust with global atmospheric model simulations. We show that the resulting representation of the global dust cycle is more accurate than can be obtained from a large number of current climate global atmospheric models.
Akinori Ito, Adeyemi A. Adebiyi, Yue Huang, and Jasper F. Kok
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-134, https://doi.org/10.5194/acp-2021-134, 2021
Preprint under review for ACP
Short summary
Short summary
We improve the simulated dust properties with datasets that leverage measurements of size-resolved dust concentration and particle shape. The improved simulation suggests much less atmospheric radiative heating over the major source regions, compared to the default simulation. The less intensified atmospheric heating due to mineral dust could substantially modify vertical temperature profile in Earth system models, and thus has important implications for the projection of dust feedback.
Jasper F. Kok, Adeyemi A. Adebiyi, Samuel Albani, Yves Balkanski, Ramiro Checa-Garcia, Mian Chin, Peter R. Colarco, Douglas S. Hamilton, Yue Huang, Akinori Ito, Martina Klose, Longlei Li, Natalie M. Mahowald, Ron L. Miller, Vincenzo Obiso, Carlos Pérez García-Pando, Adriana Rocha-Lima, and Jessica S. Wan
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-4, https://doi.org/10.5194/acp-2021-4, 2021
Preprint under review for ACP
Short summary
Short summary
The many impacts of dust on the Earth system depend on dust mineralogy, which varies between dust source regions. We constrain the contribution of the world's main dust source regions by integrating dust observations with global model simulations. We find that Asian dust contributes more, and that North African dust contributes less, than models account for. We obtain a data set of each source region's contribution to the dust cycle that can be used to constrain dust impacts on the Earth system.
Jasper F. Kok, Adeyemi A. Adebiyi, Samuel Albani, Yves Balkanski, Ramiro Checa-Garcia, Mian Chin, Peter R. Colarco, Douglas Stephen Hamilton, Yue Huang, Akinori Ito, Martina Klose, Danny M. Leung, Longlei Li, Natalie M. Mahowald, Ron L. Miller, Vincenzo Obiso, Carlos Pérez García-Pando, Adriana Rocha-Lima, Jessica S. Wan, and Chloe A. Whicker
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-1131, https://doi.org/10.5194/acp-2020-1131, 2020
Preprint under review for ACP
Short summary
Short summary
Desert dust interacts with virtually every component of the Earth system, including the climate system. We develop a new methodology to represent the global dust cycle that integrates observational constraints on the properties and abundance of desert dust with global atmospheric model simulations. We show that the resulting representation of the global dust cycle is more accurate than can be obtained from a large number of current climate global atmospheric models.
Longlei Li, Natalie M. Mahowald, Ron L. Miller, Carlos Pérez García-Pando, Martina Klose, Douglas S. Hamilton, Maria Gonçalves Ageitos, Paul Ginoux, Yves Balkanski, Robert O. Green, Olga Kalashnikova, Jasper F. Kok, Vincenzo Obiso, David Paynter, and David R. Thompson
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-547, https://doi.org/10.5194/acp-2020-547, 2020
Revised manuscript accepted for ACP
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For the first time, this study quantifies the range of dust direct radiative effect due to uncertainty in the soil mineral abundance using all currently available information. We show that the majority of the estimated direct radiative effect range is due to uncertainty in the simulated mass fractions of iron oxides and thus their soil abundance which is independent of the model employed. We, therefore, prove the necessity of considering mineralogy for understanding dust-climate interactions.
Adeyemi A. Adebiyi, Jasper F. Kok, Yang Wang, Akinori Ito, David A. Ridley, Pierre Nabat, and Chun Zhao
Atmos. Chem. Phys., 20, 829–863, https://doi.org/10.5194/acp-20-829-2020, https://doi.org/10.5194/acp-20-829-2020, 2020
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Although atmospheric dust particles produce significant impacts on the Earth system, most climate models still have difficulty representing the basic processes that affect these particles. In this study, we present new constraints on dust properties that consistently outperform the conventional climate models, when compared to independent measurements. As a result, our constraints can be used to improve climate models or serve as an alternative in constraining dust impacts on the Earth system.
Douglas S. Hamilton, Rachel A. Scanza, Yan Feng, Joseph Guinness, Jasper F. Kok, Longlei Li, Xiaohong Liu, Sagar D. Rathod, Jessica S. Wan, Mingxuan Wu, and Natalie M. Mahowald
Geosci. Model Dev., 12, 3835–3862, https://doi.org/10.5194/gmd-12-3835-2019, https://doi.org/10.5194/gmd-12-3835-2019, 2019
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MIMI v1.0 was designed for use within Earth system models to simulate the 3-D emission, atmospheric processing, and deposition of iron and its soluble fraction. Understanding the iron cycle is important due to its role as an essential micronutrient for ocean phytoplankton; its supply limits primary productivity in many of the world's oceans. Human activity has perturbed the iron cycle, and MIMI is capable of diagnosing many of these impacts; hence, it is important for future climate studies.
Stelios Myriokefalitakis, Akinori Ito, Maria Kanakidou, Athanasios Nenes, Maarten C. Krol, Natalie M. Mahowald, Rachel A. Scanza, Douglas S. Hamilton, Matthew S. Johnson, Nicholas Meskhidze, Jasper F. Kok, Cecile Guieu, Alex R. Baker, Timothy D. Jickells, Manmohan M. Sarin, Srinivas Bikkina, Rachel Shelley, Andrew Bowie, Morgane M. G. Perron, and Robert A. Duce
Biogeosciences, 15, 6659–6684, https://doi.org/10.5194/bg-15-6659-2018, https://doi.org/10.5194/bg-15-6659-2018, 2018
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The first atmospheric iron (Fe) deposition model intercomparison is presented in this study, as a result of the deliberations of the United Nations Joint Group of Experts on the Scientific Aspects of Marine Environmental Protection (GESAMP; http://www.gesamp.org/) Working Group 38. We conclude that model diversity over remote oceans reflects uncertainty in the Fe content parameterizations of dust aerosols, combustion aerosol emissions and the size distribution of transported aerosol Fe.
David A. Ridley, Colette L. Heald, Jasper F. Kok, and Chun Zhao
Atmos. Chem. Phys., 16, 15097–15117, https://doi.org/10.5194/acp-16-15097-2016, https://doi.org/10.5194/acp-16-15097-2016, 2016
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Mineral dust aerosol affects climate through interaction with radiation and clouds, human health through contribution to particulate matter, and ecosystem health through nutrient transport and deposition. In this study, we use satellite and in situ retrievals to derive an observational estimate of the global dust AOD with which evaluate modeled dust AOD. Differences in the seasonality and regional distribution of dust AOD between observations and models are highlighted.
Y. Zhang, N. Mahowald, R. A. Scanza, E. Journet, K. Desboeufs, S. Albani, J. F. Kok, G. Zhuang, Y. Chen, D. D. Cohen, A. Paytan, M. D. Patey, E. P. Achterberg, J. P. Engelbrecht, and K. W. Fomba
Biogeosciences, 12, 5771–5792, https://doi.org/10.5194/bg-12-5771-2015, https://doi.org/10.5194/bg-12-5771-2015, 2015
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A new technique to determine a size-fractionated global soil elemental emission inventory based on a global soil and mineralogical data set is introduced. Spatial variability of mineral dust elemental fractions (8 elements, e.g., Ca, Fe, Al) is identified on a global scale, particularly for Ca. The Ca/Al ratio ranged between 0.1 and 5.0 and is confirmed as an indicator of dust source regions by a global dust model. Total and soluble dust element fluxes into different ocean basins are estimated.
R. A. Scanza, N. Mahowald, S. Ghan, C. S. Zender, J. F. Kok, X. Liu, Y. Zhang, and S. Albani
Atmos. Chem. Phys., 15, 537–561, https://doi.org/10.5194/acp-15-537-2015, https://doi.org/10.5194/acp-15-537-2015, 2015
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The main purpose of this study was to build a framework in the Community Atmosphere Models version 4 and 5 within the Community Earth System Model to simulate dust aerosols as their component minerals. With this framework, we investigate the direct radiative forcing that results from the mineral speciation. We find that adding mineralogy results in a small positive forcing at the top of the atmosphere, while simulations without mineralogy have a small negative forcing.
J. F. Kok, N. M. Mahowald, G. Fratini, J. A. Gillies, M. Ishizuka, J. F. Leys, M. Mikami, M.-S. Park, S.-U. Park, R. S. Van Pelt, and T. M. Zobeck
Atmos. Chem. Phys., 14, 13023–13041, https://doi.org/10.5194/acp-14-13023-2014, https://doi.org/10.5194/acp-14-13023-2014, 2014
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We developed an improved model for the emission of dust particulates ("aerosols") emitted by wind erosion from the world's deserts. The implementation of our improved dust emission model into a climate model improves its agreement against measurements. We furthermore find that dust emissions are substantially more sensitive to the soil state than most current climate models account for.
C. Zhao, S. Chen, L. R. Leung, Y. Qian, J. F. Kok, R. A. Zaveri, and J. Huang
Atmos. Chem. Phys., 13, 10733–10753, https://doi.org/10.5194/acp-13-10733-2013, https://doi.org/10.5194/acp-13-10733-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Dominant synoptic patterns associated with the decay process of PM2.5 pollution episodes around Beijing
Validation of aerosol backscatter profiles from Raman lidar and ceilometer using balloon-borne measurements
Impacts of coagulation on the appearance time method for new particle growth rate evaluation and their corrections
PM2.5 surface concentrations in southern West African urban areas based on sun photometer and satellite observations
Observations on aerosol optical properties and scavenging during cloud events
Assessing the vertical structure of Arctic aerosols using balloon-borne measurements
An overview of the ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) project: aerosol–cloud–radiation interactions in the southeast Atlantic basin
Measurement report: aerosol hygroscopic properties extended to 600 nm in the urban environment
Spatiotemporal variation and trends in equivalent black carbon in the Helsinki metropolitan area in Finland
Characteristics of sub-10 nm particle emissions from in-use commercial aircraft observed at Narita International Airport
The CLoud–Aerosol–Radiation Interaction and Forcing: Year 2017 (CLARIFY-2017) measurement campaign
Measurement report: quantifying source contribution of fossil fuels and biomass-burning black carbon aerosol in the southeastern margin of the Tibetan Plateau
The electrical activity of Saharan dust as perceived from surface electric field observations
Long-term measurement of sub-3 nm particles and their precursor gases in the boreal forest
Variability in the mass absorption cross section of black carbon (BC) aerosols is driven by BC internal mixing state at a central European background site (Melpitz, Germany) in winter
Optical and hygroscopic properties of black carbon influenced by particle microphysics at the top of the anthropogenically polluted boundary layer
Measurement report: Properties of aerosol and gases in the vertical profile during the LAPSE-RATE campaign
Aircraft vertical profiles during summertime regional and Saharan dust scenarios over the north-western Mediterranean basin: aerosol optical and physical properties
African dust particles over the western Caribbean – Part I: Impact on air quality over the Yucatán Peninsula
Direct measurements of black carbon fluxes in central Beijing using the eddy covariance method
Measurements to determine the mixing state of black carbon emitted from the 2017–2018 California wildfires and urban Los Angeles
What can we learn about urban air quality with regard to the first outbreak of the COVID-19 pandemic? A case study from central Europe
Measurement report: Source and mixing state of black carbon aerosol in the North China Plain: implications for radiative effect
The potential role of organics in new particle formation and initial growth in the remote tropical upper troposphere
Impacts of long-range transport of aerosols on marine-boundary-layer clouds in the eastern North Atlantic
Influence of vegetation on occurrence and time distributions of regional new aerosol particle formation and growth
Quantifying bioaerosol concentrations in dust clouds through online UV-LIF and mass spectrometry measurements at the Cape Verde Atmospheric Observatory
New particle formation at urban and high-altitude remote sites in the south-eastern Iberian Peninsula
Characterization of submicron organic particles in Beijing during summertime: comparison between SP-AMS and HR-AMS
The characterization of Taklamakan dust properties using a multiwavelength Raman polarization lidar in Kashi, China
From a polar to a marine environment: has the changing Arctic led to a shift in aerosol light scattering properties?
Atmospheric new particle formation characteristics in the Arctic as measured at Mount Zeppelin, Svalbard, from 2016 to 2018
Rapid evolution of aerosol particles and their optical properties downwind of wildfires in the western US
Distinct aerosol effects on cloud-to-ground lightning in the plateau and basin regions of Sichuan, Southwest China
Spatial and temporal representativeness of point measurements for nitrogen dioxide pollution levels in cities
Vertical variability of the properties of highly aged biomass burning aerosol transported over the southeast Atlantic during CLARIFY-2017
Large contribution of organics to condensational growth and formation of cloud condensation nuclei (CCN) in the remote marine boundary layer
ENSO Effect on Interannual Variability of Spring Aerosols over East Asia
Decennial time trends and diurnal patterns of particle number concentrations in a central European city between 2008 and 2018
Roles of climate variability on the rapid increases of early winter haze pollution in North China after 2010
Drivers of cloud droplet number variability in the summertime in the southeastern United States
Roll vortices induce new particle formation bursts in the planetary boundary layer
Deposition of light-absorbing particles in glacier snow of the Sunderdhunga Valley, the southern forefront of Central Himalaya
Large-scale ion generation for precipitation of atmospheric aerosols
Aerosol light absorption and the role of extremely low volatility organic compounds
Size-resolved particle number emissions in Beijing determined from measured particle size distributions
Effects of marine fuel sulfur restrictions on particle number concentrations and size distributions in ship plumes at the Baltic Sea
Daytime aerosol optical depth above low-level clouds is similar to that in adjacent clear skies at the same heights: airborne observation above the southeast Atlantic
Absorption closure in highly aged biomass burning smoke
Aerosol pollution maps and trends over Germany with hourly data at four rural background stations from 2009 to 2018
Xiaoyan Wang, Renhe Zhang, Yanke Tan, and Wei Yu
Atmos. Chem. Phys., 21, 2491–2508, https://doi.org/10.5194/acp-21-2491-2021, https://doi.org/10.5194/acp-21-2491-2021, 2021
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The physical mechanisms of synoptic patterns affecting the decay process of air pollution episodes are investigated in this work. Three dominant circulation patterns are identified, which usually decrease the ambient PM2.5 concentrations by 27%–41% after they arrive around Beijing. Emission reductions led to a 4.3–5.7 μg (m3 yr-1)-1 decrease in PM2.5 concentrations around Beijing during 2014 to 2020.
Simone Brunamonti, Giovanni Martucci, Gonzague Romanens, Yann Poltera, Frank G. Wienhold, Maxime Hervo, Alexander Haefele, and Francisco Navas-Guzmán
Atmos. Chem. Phys., 21, 2267–2285, https://doi.org/10.5194/acp-21-2267-2021, https://doi.org/10.5194/acp-21-2267-2021, 2021
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Lidar (light detection and ranging) is a class of remote-sensing instruments that are widely used for the monitoring of aerosol properties in the lower levels of the atmosphere, yet their measurements are affected by several sources of uncertainty. Here we present the first comparison of two lidar systems against a fully independent instrument carried by meteorological balloons. We show that both lidars achieve a good agreement with the high-precision balloon measurements up to 6 km altitude.
Runlong Cai, Chenxi Li, Xu-Cheng He, Chenjuan Deng, Yiqun Lu, Rujing Yin, Chao Yan, Lin Wang, Jingkun Jiang, Markku Kulmala, and Juha Kangasluoma
Atmos. Chem. Phys., 21, 2287–2304, https://doi.org/10.5194/acp-21-2287-2021, https://doi.org/10.5194/acp-21-2287-2021, 2021
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Growth rate determines the survival probability of atmospheric new particles and hence their impacts. We clarify the impacts of coagulation on the values retrieved by the appearance time method, which is widely used for growth rate evaluation. A new formula with coagulation correction is proposed based on derivation and tested using both models and atmospheric data. We show that the sub-3 nm particle growth rate in polluted environments may be overestimated without the coagulation correction.
Jean-François Léon, Aristide Barthélémy Akpo, Mouhamadou Bedou, Julien Djossou, Marleine Bodjrenou, Véronique Yoboué, and Cathy Liousse
Atmos. Chem. Phys., 21, 1815–1834, https://doi.org/10.5194/acp-21-1815-2021, https://doi.org/10.5194/acp-21-1815-2021, 2021
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We have investigated the aerosol optical depth (AOD) and its relation to PM2.5 surface concentrations in southern West Africa based on in situ observations (2015–2017 period) and MODIS satellite data (2003–2019). MODIS AODs are validated using a regional network of handheld and automatic sun photometers. Satellite-derived PM2.5 shows an increasing trend during the short dry period that is possibly linked to the increase in anthropogenic emission over this area.
Antti Ruuskanen, Sami Romakkaniemi, Harri Kokkola, Antti Arola, Santtu Mikkonen, Harri Portin, Annele Virtanen, Kari E. J. Lehtinen, Mika Komppula, and Ari Leskinen
Atmos. Chem. Phys., 21, 1683–1695, https://doi.org/10.5194/acp-21-1683-2021, https://doi.org/10.5194/acp-21-1683-2021, 2021
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The study focuses mainly on cloud-scavenging efficiency of absorbing particulate matter (mainly black carbon) but additionally covers cloud-scavenging efficiency of scattering particles and statistics of cloud condensation nuclei. The main findings give insight into how black carbon is distributed in different particle sizes and the sensitivity to cloud scavenged. The main findings are useful for large-scale modelling for evaluating cloud scavenging.
Jessie M. Creamean, Gijs de Boer, Hagen Telg, Fan Mei, Darielle Dexheimer, Matthew D. Shupe, Amy Solomon, and Allison McComiskey
Atmos. Chem. Phys., 21, 1737–1757, https://doi.org/10.5194/acp-21-1737-2021, https://doi.org/10.5194/acp-21-1737-2021, 2021
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Arctic clouds play a role in modulating sea ice extent. Importantly, aerosols facilitate cloud formation, and thus it is crucial to understand the interactions between aerosols and clouds. Vertical measurements of aerosols and clouds are needed to tackle this issue. We present results from balloon-borne measurements of aerosols and clouds over the course of 2 years in northern Alaska. These data shed light onto the vertical distributions of aerosols relative to clouds spanning multiple seasons.
Jens Redemann, Robert Wood, Paquita Zuidema, Sarah J. Doherty, Bernadette Luna, Samuel E. LeBlanc, Michael S. Diamond, Yohei Shinozuka, Ian Y. Chang, Rei Ueyama, Leonhard Pfister, Ju-Mee Ryoo, Amie N. Dobracki, Arlindo M. da Silva, Karla M. Longo, Meloë S. Kacenelenbogen, Connor J. Flynn, Kristina Pistone, Nichola M. Knox, Stuart J. Piketh, James M. Haywood, Paola Formenti, Marc Mallet, Philip Stier, Andrew S. Ackerman, Susanne E. Bauer, Ann M. Fridlind, Gregory R. Carmichael, Pablo E. Saide, Gonzalo A. Ferrada, Steven G. Howell, Steffen Freitag, Brian Cairns, Brent N. Holben, Kirk D. Knobelspiesse, Simone Tanelli, Tristan S. L'Ecuyer, Andrew M. Dzambo, Ousmane O. Sy, Greg M. McFarquhar, Michael R. Poellot, Siddhant Gupta, Joseph R. O'Brien, Athanasios Nenes, Mary Kacarab, Jenny P. S. Wong, Jennifer D. Small-Griswold, Kenneth L. Thornhill, David Noone, James R. Podolske, K. Sebastian Schmidt, Peter Pilewskie, Hong Chen, Sabrina P. Cochrane, Arthur J. Sedlacek, Timothy J. Lang, Eric Stith, Michal Segal-Rozenhaimer, Richard A. Ferrare, Sharon P. Burton, Chris A. Hostetler, David J. Diner, Felix C. Seidel, Steven E. Platnick, Jeffrey S. Myers, Kerry G. Meyer, Douglas A. Spangenberg, Hal Maring, and Lan Gao
Atmos. Chem. Phys., 21, 1507–1563, https://doi.org/10.5194/acp-21-1507-2021, https://doi.org/10.5194/acp-21-1507-2021, 2021
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Southern Africa produces significant biomass burning emissions whose impacts on regional and global climate are poorly understood. ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) is a 5-year NASA investigation designed to study the key processes that determine these climate impacts. The main purpose of this paper is to familiarize the broader scientific community with the ORACLES project, the dataset it produced, and the most important initial findings.
Chuanyang Shen, Gang Zhao, Weilun Zhao, Ping Tian, and Chunsheng Zhao
Atmos. Chem. Phys., 21, 1375–1388, https://doi.org/10.5194/acp-21-1375-2021, https://doi.org/10.5194/acp-21-1375-2021, 2021
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Submicron particles larger than 300 nm dominate the aerosol light extinction and mass concentration in the urban environment. Aerosol hygroscopic properties extended to 600 nm were investigated at an urban site. Our results find that there exists a large fraction of a less hygroscopic group above 300 nm, and the hygroscopicity in this size range is enhanced significantly with the development of pollution levels. The hygroscopicity variation contributes greatly to the low visibility.
Krista Luoma, Jarkko V. Niemi, Minna Aurela, Pak Lun Fung, Aku Helin, Tareq Hussein, Leena Kangas, Anu Kousa, Topi Rönkkö, Hilkka Timonen, Aki Virkkula, and Tuukka Petäjä
Atmos. Chem. Phys., 21, 1173–1189, https://doi.org/10.5194/acp-21-1173-2021, https://doi.org/10.5194/acp-21-1173-2021, 2021
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This study combined black carbon measurements from 15 Finnish sites that represented different environments (traffic, detached housing area, urban background, and regional background). The seasonal and diurnal variations in the black carbon concentration were associated with local emissions from traffic and residential wood burning. The study observed decreasing trends in the black carbon concentration and associated them with decreases in traffic emissions.
Nobuyuki Takegawa, Yoshiko Murashima, Akihiro Fushimi, Kentaro Misawa, Yuji Fujitani, Katsumi Saitoh, and Hiromu Sakurai
Atmos. Chem. Phys., 21, 1085–1104, https://doi.org/10.5194/acp-21-1085-2021, https://doi.org/10.5194/acp-21-1085-2021, 2021
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The characterization of particle emissions from aircraft is important for the assessment of the aviation impacts on climate and human health. We conducted field observations of aerosols near a runway at Narita International Airport in February 2018. We investigated particle number emissions from in-use commercial aircraft under real-world operating conditions, and we found the significance of sub-10 nm size ranges in take-off plumes for both total and non-volatile particles.
Jim M. Haywood, Steven J. Abel, Paul A. Barrett, Nicolas Bellouin, Alan Blyth, Keith N. Bower, Melissa Brooks, Ken Carslaw, Haochi Che, Hugh Coe, Michael I. Cotterell, Ian Crawford, Zhiqiang Cui, Nicholas Davies, Beth Dingley, Paul Field, Paola Formenti, Hamish Gordon, Martin de Graaf, Ross Herbert, Ben Johnson, Anthony C. Jones, Justin M. Langridge, Florent Malavelle, Daniel G. Partridge, Fanny Peers, Jens Redemann, Philip Stier, Kate Szpek, Jonathan W. Taylor, Duncan Watson-Parris, Robert Wood, Huihui Wu, and Paquita Zuidema
Atmos. Chem. Phys., 21, 1049–1084, https://doi.org/10.5194/acp-21-1049-2021, https://doi.org/10.5194/acp-21-1049-2021, 2021
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Every year, the seasonal cycle of biomass burning from agricultural practices in Africa creates a huge plume of smoke that travels many thousands of kilometres over the Atlantic Ocean. This study provides an overview of a measurement campaign called the cloud–aerosol–radiation interaction and forcing for year 2017 (CLARIFY-2017) and documents the rationale, deployment strategy, observations, and key results from the campaign which utilized the heavily equipped FAAM atmospheric research aircraft.
Huikun Liu, Qiyuan Wang, Li Xing, Yong Zhang, Ting Zhang, Weikang Ran, and Junji Cao
Atmos. Chem. Phys., 21, 973–987, https://doi.org/10.5194/acp-21-973-2021, https://doi.org/10.5194/acp-21-973-2021, 2021
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We conducted black carbon (BC) source apportionment on the southeastern Tibetan Plateau (TP) by an improved aethalometer model with the site-dependent Ångström exponent and BC mass absorption cross section (MAC). The result shows that the biomass-burning BC on the TP is slightly higher than fossil fuel BC, mainly from cross-border transportation instead of the local region, and the BC radiative effect is lower than that in the southwestern Himalaya but higher than that on the northeastern TP.
Vasiliki Daskalopoulou, Sotirios A. Mallios, Zbigniew Ulanowski, George Hloupis, Anna Gialitaki, Ioanna Tsikoudi, Konstantinos Tassis, and Vassilis Amiridis
Atmos. Chem. Phys., 21, 927–949, https://doi.org/10.5194/acp-21-927-2021, https://doi.org/10.5194/acp-21-927-2021, 2021
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This research highlights the detection of charged Saharan dust in Greece and provides indications of charge separation in the plumes through the first-ever co-located ground electric field measurements and sophisticated lidar observations. We provide a robust methodology for the extraction of a fair-weather proxy field used to assess the effect of lofted dust particles to the electric field and insert a realistic modelling aspect to the charge accumulation areas within electrically active dust.
Juha Sulo, Nina Sarnela, Jenni Kontkanen, Lauri Ahonen, Pauli Paasonen, Tiia Laurila, Tuija Jokinen, Juha Kangasluoma, Heikki Junninen, Mikko Sipilä, Tuukka Petäjä, Markku Kulmala, and Katrianne Lehtipalo
Atmos. Chem. Phys., 21, 695–715, https://doi.org/10.5194/acp-21-695-2021, https://doi.org/10.5194/acp-21-695-2021, 2021
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In this study, we analyzed over 5 years of sub-3 nm particle concentrations and their precursor vapors, identifying atmoshperic vapors important to the formation of these particles in the boreal forest. We also observed seasonal differences in both particle and precursor vapor concentrations and the formation pathways of these particles. Our results confirm the importance of organic vapors in atmospheric aerosol formation and highlight key seasonal differences that require further study.
Jinfeng Yuan, Robin Lewis Modini, Marco Zanatta, Andreas B. Herber, Thomas Müller, Birgit Wehner, Laurent Poulain, Thomas Tuch, Urs Baltensperger, and Martin Gysel-Beer
Atmos. Chem. Phys., 21, 635–655, https://doi.org/10.5194/acp-21-635-2021, https://doi.org/10.5194/acp-21-635-2021, 2021
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Black carbon (BC) aerosols contribute substantially to climate warming due to their unique light absorption capabilities. We performed field measurements at a central European background site in winter and found that variability in the absorption efficiency of BC particles is driven mainly by their internal mixing state. Our results suggest that, at this site, knowing the BC mixing state is sufficient to describe BC light absorption enhancements due to the lensing effect in good approximation.
Shuo Ding, Dantong Liu, Kang Hu, Delong Zhao, Ping Tian, Fei Wang, Ruijie Li, Yichen Chen, Hui He, Mengyu Huang, and Deping Ding
Atmos. Chem. Phys., 21, 681–694, https://doi.org/10.5194/acp-21-681-2021, https://doi.org/10.5194/acp-21-681-2021, 2021
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In this study, we for the first time characterized the detailed black carbon (BC) microphysics at a mountain site located at the top of the planetary boundary layer (PBL) influenced by surface emission over the North China Plain. We investigated the optical and hygroscopic properties of BC at this level as influenced by microphysical properties. Such information will constrain the impacts of BC in influencing the PBL dynamics and low-level cloud formation over anthropogenically polluted regions.
David Brus, Jani Gustafsson, Ville Vakkari, Osku Kemppinen, Gijs de Boer, and Anne Hirsikko
Atmos. Chem. Phys., 21, 517–533, https://doi.org/10.5194/acp-21-517-2021, https://doi.org/10.5194/acp-21-517-2021, 2021
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This paper summarizes Finnish Meteorological Institute and Kansas State University unmanned aerial vehicle measurements during the summer 2018 Lower Atmospheric Process Studies at Elevation – a Remotely-piloted Aircraft Team Experiment (LAPSE-RATE) campaign in the San Luis Valley, providing an overview of the rotorcraft deployed, payloads, scientific goals and flight strategies and presenting observations of atmospheric thermodynamics and aerosol and gas parameters in the vertical column.
Jesús Yus-Díez, Marina Ealo, Marco Pandolfi, Noemí Perez, Gloria Titos, Griša Močnik, Xavier Querol, and Andrés Alastuey
Atmos. Chem. Phys., 21, 431–455, https://doi.org/10.5194/acp-21-431-2021, https://doi.org/10.5194/acp-21-431-2021, 2021
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Here we describe the vertical profiles of extensive (scattering and absorption) and intensive (e.g. albedo and asymmetry parameter) aerosol optical properties from coupling ground-based measurements from two sites in north-eastern Spain and airborne measurements performed with an aircraft. We analyse different aerosol layers along the vertical profile for a regional pollution episode and a Saharan dust intrusion. The results show a change with height depending on the different measured layers.
Carolina Ramírez-Romero, Alejandro Jaramillo, María F. Córdoba, Graciela B. Raga, Javier Miranda, Harry Alvarez-Ospina, Daniel Rosas, Talib Amador, Jong Sung Kim, Jacqueline Yakobi-Hancock, Darrel Baumgardner, and Luis A. Ladino
Atmos. Chem. Phys., 21, 239–253, https://doi.org/10.5194/acp-21-239-2021, https://doi.org/10.5194/acp-21-239-2021, 2021
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Field measurements were conducted to confirm the arrival of African dust on the Yucatàn Peninsula. Aerosol particles were monitored at ground level by different online and off-line sensors. Several particulate matter peaks were observed with a relative increase in their levels of up to 500 % with respect to background conditions. Based on the chemical composition, back trajectories, vertical profiles, reanalysis, and satellite images, it was found that the peaks are linked to African dust.
Rutambhara Joshi, Dantong Liu, Eiko Nemitz, Ben Langford, Neil Mullinger, Freya Squires, James Lee, Yunfei Wu, Xiaole Pan, Pingqing Fu, Simone Kotthaus, Sue Grimmond, Qiang Zhang, Ruili Wu, Oliver Wild, Michael Flynn, Hugh Coe, and James Allan
Atmos. Chem. Phys., 21, 147–162, https://doi.org/10.5194/acp-21-147-2021, https://doi.org/10.5194/acp-21-147-2021, 2021
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Black carbon (BC) is a component of particulate matter which has significant effects on climate and human health. Sources of BC include biomass burning, transport, industry and domestic cooking and heating. In this study, we measured BC emissions in Beijing, finding a dominance of traffic emissions over all other sources. The quantitative method presented here has benefits for revising widely used emissions inventories and for understanding BC sources with impacts on air quality and climate.
Joseph Ko, Trevor Krasowsky, and George Ban-Weiss
Atmos. Chem. Phys., 20, 15635–15664, https://doi.org/10.5194/acp-20-15635-2020, https://doi.org/10.5194/acp-20-15635-2020, 2020
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Black carbon (BC) is the second strongest climate forcing pollutant in the atmosphere, after carbon dioxide. Here, we seek to understand how BC microphysical properties vary with atmospheric contexts, as these properties can influence its radiative forcing. Consistent with previous studies, we found that biomass burning BC had thicker coatings and larger core diameters than fossil fuel BC. We also present evidence to show that atmospheric aging also increases BC coating thickness.
Imre Salma, Máté Vörösmarty, András Zénó Gyöngyösi, Wanda Thén, and Tamás Weidinger
Atmos. Chem. Phys., 20, 15725–15742, https://doi.org/10.5194/acp-20-15725-2020, https://doi.org/10.5194/acp-20-15725-2020, 2020
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Motor vehicle road traffic in Budapest was reduced by approximately 50% of its ordinary level due to COVID-19. In parallel, concentrations of most criteria air pollutants declined by 30–60%. Change rates of NO and NO2 with relative change in traffic intensity were the largest, total particle number concentration showed considerable dependency, while particulate matter mass concentrations did not appear to be related to urban traffic. Concentrations of O3 showed an increasing tendency.
Qiyuan Wang, Li Li, Jiamao Zhou, Jianhuai Ye, Wenting Dai, Huikun Liu, Yong Zhang, Renjian Zhang, Jie Tian, Yang Chen, Yunfei Wu, Weikang Ran, and Junji Cao
Atmos. Chem. Phys., 20, 15427–15442, https://doi.org/10.5194/acp-20-15427-2020, https://doi.org/10.5194/acp-20-15427-2020, 2020
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Recently, China has promulgated a series of regulations to reduce air pollutants. The decreased black carbon (BC) and co-emitted pollutants could affect the interactions between BC and other aerosols, which in turn results in changes in BC. Herein, we re-assessed the characteristics of BC of a representative pollution site in northern China in the final year of the Chinese
Action Plan for the Prevention and Control of Air Pollution.
Agnieszka Kupc, Christina J. Williamson, Anna L. Hodshire, Jan Kazil, Eric Ray, T. Paul Bui, Maximilian Dollner, Karl D. Froyd, Kathryn McKain, Andrew Rollins, Gregory P. Schill, Alexander Thames, Bernadett B. Weinzierl, Jeffrey R. Pierce, and Charles A. Brock
Atmos. Chem. Phys., 20, 15037–15060, https://doi.org/10.5194/acp-20-15037-2020, https://doi.org/10.5194/acp-20-15037-2020, 2020
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Tropical upper troposphere over the Atlantic and Pacific oceans is a major source region of new particles. These particles are associated with the outflow from deep convection. We investigate the processes that govern the formation of these particles and their initial growth and show that none of the formation schemes commonly used in global models are consistent with observations. Using newer schemes indicates that organic compounds are likely important as nucleating and initial growth agents.
Yuan Wang, Xiaojian Zheng, Xiquan Dong, Baike Xi, Peng Wu, Timothy Logan, and Yuk L. Yung
Atmos. Chem. Phys., 20, 14741–14755, https://doi.org/10.5194/acp-20-14741-2020, https://doi.org/10.5194/acp-20-14741-2020, 2020
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A recent aircraft field campaign near the Azores in the summer of 2017 provides ample observations of aerosols and clouds with detailed vertical information. This study utilizes those observational data in combination with the aerosol-aware large-eddy simulations and aerosol reanalysis data to examine the significance of the long-range-transported aerosol effect on marine-boundary-layer clouds. It is the first time that the ACE-ENA aircraft campaign data are used for this topic.
Imre Salma, Wanda Thén, Pasi Aalto, Veli-Matti Kerminen, Anikó Kern, Zoltán Barcza, Tuukka Petäjä, and Markku Kulmala
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-862, https://doi.org/10.5194/acp-2020-862, 2020
Revised manuscript accepted for ACP
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The distribution of monthly mean nucleation frequency possessed a characteristic pattern. Its shape was compared to those of environmental variables including vegetation-derived properties. The spring maximum in the occurrence frequency often overlapped with the positive T anomaly. The link between the heat stress and the occurrence minimum in summer could not be proved, while association between the occurrence frequency and vegetation growth dynamics was clearly identified in spring.
Douglas Morrison, Ian Crawford, Nicholas Marsden, Michael Flynn, Katie Read, Luis Neves, Virginia Foot, Paul Kaye, Warren Stanley, Hugh Coe, David Topping, and Martin Gallagher
Atmos. Chem. Phys., 20, 14473–14490, https://doi.org/10.5194/acp-20-14473-2020, https://doi.org/10.5194/acp-20-14473-2020, 2020
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We provide conservative estimates of the concentrations of bacteria within transatlantic dust clouds, originating from the African continent. We observe significant seasonal differences in the overall concentrations of particles but no seasonal variation in the ratio between bacteria and dust. With bacteria contributing to ice formation at warmer temperatures than dust, our observations should improve the accuracy of climate models.
Juan Andrés Casquero-Vera, Hassan Lyamani, Lubna Dada, Simo Hakala, Pauli Paasonen, Roberto Román, Roberto Fraile, Tuukka Petäjä, Francisco José Olmo-Reyes, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 20, 14253–14271, https://doi.org/10.5194/acp-20-14253-2020, https://doi.org/10.5194/acp-20-14253-2020, 2020
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New particle formation was investigated at two stations located close to each other but at different altitudes: urban and high-altitude sites. Results show that sulfuric acid is able to explain a minimal fraction contribution to the observed growth rates and point to the availability of volatile organic compounds as the main factor controlling NPF events at both sites. A closer analysis of the NPF events that were observed at high-altitude sites during a Saharan dust episode was carried out.
Junfeng Wang, Jianhuai Ye, Dantong Liu, Yangzhou Wu, Jian Zhao, Weiqi Xu, Conghui Xie, Fuzhen Shen, Jie Zhang, Paul E. Ohno, Yiming Qin, Xiuyong Zhao, Scot T. Martin, Alex K. Y. Lee, Pingqing Fu, Daniel J. Jacob, Qi Zhang, Yele Sun, Mindong Chen, and Xinlei Ge
Atmos. Chem. Phys., 20, 14091–14102, https://doi.org/10.5194/acp-20-14091-2020, https://doi.org/10.5194/acp-20-14091-2020, 2020
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We compared the organics in total submicron matter and those coated on BC cores during summertime in Beijing and found large differences between them. Traffic-related OA was associated significantly with BC, while cooking-related OA did not coat BC. In addition, a factor likely originated from primary biomass burning OA was only identified in BC-containing particles. Such a unique BBOA requires further field and laboratory studies to verify its presence and elucidate its properties and impacts.
Qiaoyun Hu, Haofei Wang, Philippe Goloub, Zhengqiang Li, Igor Veselovskii, Thierry Podvin, Kaitao Li, and Mikhail Korenskiy
Atmos. Chem. Phys., 20, 13817–13834, https://doi.org/10.5194/acp-20-13817-2020, https://doi.org/10.5194/acp-20-13817-2020, 2020
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This study presents the characteristics of Taklamakan dust particles derived from lidar measurements collected in the dust aerosol observation field campaign. It provides comprehensive parameters for Taklamakan dust properties and vertical distributions of Taklamakan dust. This paper also points out the importance of polluted dust which was frequently observed in the field campaign. The results contribute to improving knowledge about dust and reducing uncertainties in the climatic model.
Dominic Heslin-Rees, Maria Burgos, Hans-Christen Hansson, Radovan Krejci, Johan Ström, Peter Tunved, and Paul Zieger
Atmos. Chem. Phys., 20, 13671–13686, https://doi.org/10.5194/acp-20-13671-2020, https://doi.org/10.5194/acp-20-13671-2020, 2020
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Aerosol particles are one important key player in the Arctic climate. Using long-term measurements of particle light scattering from an observatory on Svalbard, this study investigates the reasons behind an observed shift towards larger particles seen in the last 2 decades. We find that increases in sea spray are the most likely cause. Air masses from the south-west have increased significantly, suggestive of a potential mechanism, whilst the retreat in sea ice has a marginal influence.
Haebum Lee, Kwangyul Lee, Chris Rene Lunder, Radovan Krejci, Wenche Aas, Jiyeon Park, Ki-Tae Park, Bang Yong Lee, Young Jun Yoon, and Kihong Park
Atmos. Chem. Phys., 20, 13425–13441, https://doi.org/10.5194/acp-20-13425-2020, https://doi.org/10.5194/acp-20-13425-2020, 2020
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New particle formation (NPF) contributes to enhance the number of particles in the ambient atmosphere, affecting local air quality and cloud condensation nuclei (CCN) concentration. This study investigated NPF characteristics in the Arctic and showed that although formation and growth rates of nanoparticles were much lower than those in continental areas, NPF occurrence frequency was comparable and marine biogenic sources played important roles in production of condensing vapors for NPF.
Lawrence I. Kleinman, Arthur J. Sedlacek III, Kouji Adachi, Peter R. Buseck, Sonya Collier, Manvendra K. Dubey, Anna L. Hodshire, Ernie Lewis, Timothy B. Onasch, Jeffery R. Pierce, John Shilling, Stephen R. Springston, Jian Wang, Qi Zhang, Shan Zhou, and Robert J. Yokelson
Atmos. Chem. Phys., 20, 13319–13341, https://doi.org/10.5194/acp-20-13319-2020, https://doi.org/10.5194/acp-20-13319-2020, 2020
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Aerosols from wildfires affect the Earth's temperature by absorbing light or reflecting it back into space. This study investigates time-dependent chemical, microphysical, and optical properties of aerosols generated by wildfires in the Pacific Northwest, USA. Wildfire smoke plumes were traversed by an instrumented aircraft at locations near the fire and up to 3.5 h travel time downwind. Although there was no net aerosol production, aerosol particles grew and became more efficient scatters.
Pengguo Zhao, Zhanqing Li, Hui Xiao, Fang Wu, Youtong Zheng, Maureen C. Cribb, Xiaoai Jin, and Yunjun Zhou
Atmos. Chem. Phys., 20, 13379–13397, https://doi.org/10.5194/acp-20-13379-2020, https://doi.org/10.5194/acp-20-13379-2020, 2020
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We discussed the different aerosol effects on lightning in plateau and basin regions of Sichuan, southwestern China. In the plateau area, the aerosol concentration is low, and aerosols (via microphysical effects) inhibit the process of warm rain and stimulate convection and lightning activity. In the basin region, however, aerosols tend to show a significant radiative effect (reducing the solar radiation reaching the surface by absorbing and scattering) and inhibit the lightning.
Ying Zhu, Jia Chen, Xiao Bi, Gerrit Kuhlmann, Ka Lok Chan, Florian Dietrich, Dominik Brunner, Sheng Ye, and Mark Wenig
Atmos. Chem. Phys., 20, 13241–13251, https://doi.org/10.5194/acp-20-13241-2020, https://doi.org/10.5194/acp-20-13241-2020, 2020
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Average NO2 concentration of on-street mobile measurements (MMs) near the monitoring stations (MSs) was found to be considerably higher than the MSs data. The common measurement height (H) and distance (D) of the MSs result in 27 % lower average concentrations in total than the concentration of our MMs. Another 21 % difference remained after correcting the influence of the measuring H and D. This result makes our city-wide measurements for capturing the full range of concentrations necessary.
Huihui Wu, Jonathan W. Taylor, Kate Szpek, Justin M. Langridge, Paul I. Williams, Michael Flynn, James D. Allan, Steven J. Abel, Joseph Pitt, Michael I. Cotterell, Cathryn Fox, Nicholas W. Davies, Jim Haywood, and Hugh Coe
Atmos. Chem. Phys., 20, 12697–12719, https://doi.org/10.5194/acp-20-12697-2020, https://doi.org/10.5194/acp-20-12697-2020, 2020
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Airborne measurements of highly aged biomass burning aerosols (BBAs) over the remote southeast Atlantic provide unique aerosol parameters for climate models. Our observations demonstrate the persistence of strongly absorbing BBAs across wide regions of the South Atlantic. We also found significant vertical variation in the single-scattering albedo of these BBAs, as a function of relative chemical composition and size. Aerosol properties in the marine BL are suggested to be separated from the FT.
Guangjie Zheng, Chongai Kuang, Janek Uin, Thomas Watson, and Jian Wang
Atmos. Chem. Phys., 20, 12515–12525, https://doi.org/10.5194/acp-20-12515-2020, https://doi.org/10.5194/acp-20-12515-2020, 2020
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Condensational growth of Aitken-mode particles is a major source of cloud condensation nuclei in the remote marine boundary layer. It has been long thought that over remote oceans, condensation growth is dominated by sulfate that derives from ocean-emitted dimethyl sulfide. In this study, we present the first long-term observational evidence that, contrary to conventional thinking, organics play an even more important role than sulfate in particle growth over remote oceans throughout the year.
Anbao Zhu, Haiming Xu, Jiechun Deng, Jing Ma, and Shuhui Li
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-859, https://doi.org/10.5194/acp-2020-859, 2020
Revised manuscript accepted for ACP
Santtu Mikkonen, Zoltán Németh, Veronika Varga, Tamás Weidinger, Ville Leinonen, Taina Yli-Juuti, and Imre Salma
Atmos. Chem. Phys., 20, 12247–12263, https://doi.org/10.5194/acp-20-12247-2020, https://doi.org/10.5194/acp-20-12247-2020, 2020
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We determined decennial statistical time trends and diurnal statistical patterns of atmospheric particle number concentrations in various relevant size fractions in the city centre of Budapest in an interval of 2008–2018. The mean overall decrease rate of particles in different size fractions was approximately −5 % scaled for the 10-year measurement interval. The decline can be interpreted as a consequence of the decreased anthropogenic emissions in the city.
Yijia Zhang, Zhicong Yin, and Huijun Wang
Atmos. Chem. Phys., 20, 12211–12221, https://doi.org/10.5194/acp-20-12211-2020, https://doi.org/10.5194/acp-20-12211-2020, 2020
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Haze events in early winter in North China exhibited rapid growth after 2010, which was completely different from the slow decline observed before 2010. However, global warming and anthropogenic emissions could not explain this trend reversal well, which was puzzling. Our study found that four climate factors, exhibiting completely opposite trends before and after 2010, effectively drove the trend reversal of the haze pollution in North China.
Aikaterini Bougiatioti, Athanasios Nenes, Jack J. Lin, Charles A. Brock, Joost A. de Gouw, Jin Liao, Ann M. Middlebrook, and André Welti
Atmos. Chem. Phys., 20, 12163–12176, https://doi.org/10.5194/acp-20-12163-2020, https://doi.org/10.5194/acp-20-12163-2020, 2020
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The number concentration of droplets in clouds in the summertime in the southeastern United States is influenced by aerosol variations but limited by the strong competition for supersaturated water vapor. Concurrent variations in vertical velocity magnify the response of cloud droplet number to aerosol increases by up to a factor of 5. Omitting the covariance of vertical velocity with aerosol number may therefore bias estimates of the cloud albedo effect from aerosols.
Janne Lampilahti, Hanna Elina Manninen, Katri Leino, Riikka Väänänen, Antti Manninen, Stephany Buenrostro Mazon, Tuomo Nieminen, Matti Leskinen, Joonas Enroth, Marja Bister, Sergej Zilitinkevich, Juha Kangasluoma, Heikki Järvinen, Veli-Matti Kerminen, Tuukka Petäjä, and Markku Kulmala
Atmos. Chem. Phys., 20, 11841–11854, https://doi.org/10.5194/acp-20-11841-2020, https://doi.org/10.5194/acp-20-11841-2020, 2020
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In this work, by using co-located airborne and ground-based measurements, we show that counter-rotating horizontal circulations in the planetary boundary layer (roll vortices) frequently enhance regional new particle formation or induce localized bursts of new particle formation. These observations can be explained by the ability of the rolls to efficiently lift low-volatile vapors emitted from the surface to the top of the boundary layer where new particle formation is more favorable.
Jonas Svensson, Johan Ström, Henri Honkonen, Eija Asmi, Nathaniel B. Dkhar, Shresth Tayal, Ved P. Sharma, Rakesh Hooda, Matti Leppäranta, Hans-Werner Jacobi, Heikki Lihavainen, and Antti Hyvärinen
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-1059, https://doi.org/10.5194/acp-2020-1059, 2020
Revised manuscript accepted for ACP
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Light-absorbing particles specifically affect snow melt in the Himalaya. Through measurements of the constituents in glacier snow pits from Indian Himalaya our investigations show that different snow layers display striking similarities. These similarities can be characterized by a deposition constant. Our results further indicate that mineral dust can be responsible for the majority of light absorption in the snow in this part of the Himalaya.
Shaoxiang Ma, He Cheng, Jiacheng Li, Maoyuan Xu, Dawei Liu, and Kostya Ostrikov
Atmos. Chem. Phys., 20, 11717–11727, https://doi.org/10.5194/acp-20-11717-2020, https://doi.org/10.5194/acp-20-11717-2020, 2020
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Our work suggests that a large corona discharge system is an efficient and possibly economically sustainable way to increase the ion density in the open air and control the precipitation of atmospheric aerosols. Once the system is installed on a mountaintop, it will generate lots of charged nuclei, which may trigger water precipitation or fog elimination within a certain region in the downwind directions.
Antonios Tasoglou, Evangelos Louvaris, Kalliopi Florou, Aikaterini Liangou, Eleni Karnezi, Christos Kaltsonoudis, Ningxin Wang, and Spyros N. Pandis
Atmos. Chem. Phys., 20, 11625–11637, https://doi.org/10.5194/acp-20-11625-2020, https://doi.org/10.5194/acp-20-11625-2020, 2020
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A month-long set of summertime measurements in a remote area in the Mediterranean is used to quantify aerosol absorption. The measured light absorption was two or more times higher than that of fresh black carbon. The absorption enhancement due to the coating of black carbon cores by other aerosol components could explain only part of this absorption enhancement. The rest was due to brown carbon, mostly in the form of extremely low volatility organic compounds.
Jenni Kontkanen, Chenjuan Deng, Yueyun Fu, Lubna Dada, Ying Zhou, Jing Cai, Kaspar R. Daellenbach, Simo Hakala, Tom V. Kokkonen, Zhuohui Lin, Yongchun Liu, Yonghong Wang, Chao Yan, Tuukka Petäjä, Jingkun Jiang, Markku Kulmala, and Pauli Paasonen
Atmos. Chem. Phys., 20, 11329–11348, https://doi.org/10.5194/acp-20-11329-2020, https://doi.org/10.5194/acp-20-11329-2020, 2020
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To estimate the impacts of atmospheric aerosol particles on air quality, knowledge of size distributions of particles emitted from anthropogenic sources is needed. We introduce a new method for determining size-resolved particle number emissions from measured particle size distributions. We apply our method to data measured in Beijing, China. We find that particle number emissions at our site are dominated by emissions of particles smaller than 30 nm, originating mainly from traffic.
Sami Seppälä, Joel Kuula, Antti-Pekka Hyvärinen, Sanna Saarikoski, Topi Rönkkö, Jorma Keskinen, Jukka-Pekka Jalkanen, and Hilkka Timonen
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-946, https://doi.org/10.5194/acp-2020-946, 2020
Revised manuscript accepted for ACP
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Effects of fuel sulfur content restrictions implemented by the International Maritime Organization at the Baltic Sea, in July 2010 and January 2015, on the particle properties of ship exhaust plumes and ambient aerosol were studied. The restrictions reduced the particle number concentrations and median particle size in plumes and number concentrations in the ambient aerosol. These changes may improve human health in coastal areas and decrease the cooling effect of the exhaust emissions of ships.
Yohei Shinozuka, Meloë S. Kacenelenbogen, Sharon P. Burton, Steven G. Howell, Paquita Zuidema, Richard A. Ferrare, Samuel E. LeBlanc, Kristina Pistone, Stephen Broccardo, Jens Redemann, K. Sebastian Schmidt, Sabrina P. Cochrane, Marta Fenn, Steffen Freitag, Amie Dobracki, Michal Segal-Rosenheimer, and Connor J. Flynn
Atmos. Chem. Phys., 20, 11275–11285, https://doi.org/10.5194/acp-20-11275-2020, https://doi.org/10.5194/acp-20-11275-2020, 2020
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To help satellite retrieval of aerosols and studies of their radiative effects, we demonstrate that daytime aerosol optical depth over low-level clouds is similar to that in neighboring clear skies at the same heights. Based on recent airborne lidar and sun photometer observations above the southeast Atlantic, the mean AOD difference at 532 nm is between 0 and -0.01, when comparing the cloudy and clear sides of cloud edges, with each up to 20 km wide.
Jonathan W. Taylor, Huihui Wu, Kate Szpek, Keith Bower, Ian Crawford, Michael J. Flynn, Paul I. Williams, James Dorsey, Justin M. Langridge, Michael I. Cotterell, Cathryn Fox, Nicholas W. Davies, Jim M. Haywood, and Hugh Coe
Atmos. Chem. Phys., 20, 11201–11221, https://doi.org/10.5194/acp-20-11201-2020, https://doi.org/10.5194/acp-20-11201-2020, 2020
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Every year, huge plumes of smoke hundreds of miles wide travel over the south Atlantic Ocean from fires in central and southern Africa. These plumes absorb the sun’s energy and warm the climate. We used airborne optical instrumentation to determine how absorbing the smoke was as well as the relative importance of black and brown carbon. We also tested different ways of simulating these properties that could be used in a climate model.
Jost Heintzenberg, Wolfram Birmili, Bryan Hellack, Gerald Spindler, Thomas Tuch, and Alfred Wiedensohler
Atmos. Chem. Phys., 20, 10967–10984, https://doi.org/10.5194/acp-20-10967-2020, https://doi.org/10.5194/acp-20-10967-2020, 2020
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A total of 10 years of hourly aerosol and gas data at four rural German stations have been combined with hourly back trajectories to the stations and inventories of the European Emissions Database for Global Atmospheric Research (EDGAR), yielding emission maps and trends over Germany for PM10, particle number concentrations, and equivalent black carbon (eBC). The maps reflect aerosol emissions modified with atmospheric processes during transport between sources and receptor sites.
Cited articles
Alfaro, S. C. and Gomes, L.: Modeling mineral aerosol production by wind
erosion: Emission intensities and aerosol size distributions in source areas,
J. Geophys. Res.-Atmos., 106, 18075–18084, https://doi.org/10.1029/2000JD900339, 2001.
Andreas, E. L., Claffey, K. J., Jordan, R. E., Fairall, C. W., Guest, P. S.,
Persson, P. O. G., and Grachev, A. A.: Evaluations of the von Kármán
constant in the atmospheric surface layer, J. Fluid Mech., 559, 117–149,
https://doi.org/10.1017/S0022112006000164, 2006.
Ashkenazy, Y., Yizhaq, H., and Tsoar, H.: Sand dune mobility under climate
change in the Kalahari and Australian deserts, Clim. Change, 112, 901–923,
https://doi.org/10.1007/s10584-011-0264-9, 2012.
Atkinson, J. D., Murray, B. J., Woodhouse, M. T., Whale, T. F., Baustian, K.
J., Carslaw, K. S., Dobbie, S., O'Sullivan, D., and Malkin, T. L.: The
importance of feldspar for ice nucleation by mineral dust in mixed-phase
clouds, Nature, 498, 355–358, https://doi.org/10.1038/nature12278, 2013.
Baddock, M. C., Gill, T. E., Bullard, J. E., Acosta, M. D., and Rivera
Rivera, N. I.: Geomorphology of the Chihuahuan Desert based on potential dust
emissions, J. Maps, 7, 249–259, https://doi.org/10.4113/jom.2011.1178, 2011.
Barchyn, T. E., Hugenholtz, C. H., Li, B., Neuman, C. M., and Steven
Sanderson, R.: From particle counts to flux: Wind tunnel testing and
calibration of the “Wenglor” aeolian sediment transport sensor, Aeolian
Res., 15, 311–318, https://doi.org/10.1016/j.aeolia.2014.06.009, 2014.
Bohren, C. F. and Huffman, D. R.: Absorption and scattering of light by small
particles, 1st ed., Wiley-VCH, 503 pp., 1983.
Bowler, J. M.: Clay dunes: Their occurrence, formation and environmental
significance, Earth Sci. Rev., 9, 315–338, https://doi.org/10.1016/0012-8252(73)90001-9,
1973.
Bullard, J. E., Harrison, S. P., Baddock, M. C., Drake, N., Gill, T. E.,
McTainsh, G., and Sun, Y.: Preferential dust sources: A geomorphological
classification designed for use in global dust-cycle models, J. Geophys.
Res.-Earth, 116, F04034, https://doi.org/10.1029/2011JF002061, 2011.
Bullard, J. E., McTainsh, G. H., and Pudmenzky, C.: Factors affecting the
nature and rate of dust production from natural dune sands, Sedimentology,
54, 169–182, https://doi.org/10.1111/j.1365-3091.2006.00827.x, 2007.
Bullard, J. E., McTainsh, G. H., and Pudmenzky, C.: Aeolian abrasion and
modes of fine particle production from natural red dune sands: an
experimental study, Sedimentology, 51, 1103–1125,
https://doi.org/10.1111/j.1365-3091.2004.00662.x, 2004.
Burnett, R. T., Pope, C. A,, Ezzati, M., Olives, C., Lim, S. S., Mehta, S.,
Shin, H. H., Singh, G., Hubbell, B., Brauer, M., Anderson, H. R., Smith, K.
R., Balmes, J. R., Bruce, N. G., Kan, H., Laden, F., Prüss-Ustün, A.,
Turner, M. C., Gapstur, S. M., Diver, W. R., and Cohen, A.: An integrated
risk function for estimating the global burden of disease attributable to
ambient fine particulate matter exposure, Environ. Health Perspect., 122,
397–403, https://doi.org/10.1289/ehp.1307049, 2014.
Chou, C., Formenti, P., Maille, M., Ausset, P., Helas, G., Harrison, M., and
Osborne, S.: Size distribution, shape, and composition of mineral dust
aerosols collected during the African Monsoon Multidisciplinary Analysis
Special Observation Period 0: Dust and Biomass-Burning Experiment field
campaign in Niger, January 2006, J. Geophys. Res.-Atmos., 113, D00C10,
https://doi.org/10.1029/2008JD009897, 2008.
Combellick, R. A. and Osborne, R. H.: Sources and petrology of beach sand
from southern Monterey Bay, California, J. Sediment. Petrol., 47, 891–907,
1977.
Compton, J. S.: Origin and diagenesis of clay minerals in the Monterey
Formation, Santa Maria Basin Area, California, Clays Clay Miner., 39,
449–466, https://doi.org/10.1346/CCMN.1991.0390501, 1991.
Cooper, W. S.: Coastal dunes of California, Geol. Soc. Am. Mem., 104, 1–131,
1967.
Creamean, J. M., Suski, K. J., Rosenfeld, D., Cazorla, A., DeMott, P. J.,
Sullivan, R. C., White, A. B., Ralph, F., Minnis, P., Comstock, J. M.,
Tomlinson, J. M., and Prather, K. A.: Dust and Biological Aerosols from the
Sahara and Asia Influence Precipitation in the Western U.S., Science, 339,
1572–1578, https://doi.org/10.1126/science.1227279, 2013.
Crouvi, O., Schepanski, K., Amit, R., Gillespie, A. R., and Enzel, Y.:
Multiple dust sources in the Sahara Desert: The importance of sand dunes,
Geophys. Res. Lett., 39, L13401, https://doi.org/10.1029/2012GL052145, 2012.
DeMott, P. J., Prenni, A. J., McMeeking, G. R., Sullivan, R. C., Petters, M.
D., Tobo, Y., Niemand, M., Möhler, O., Snider, J. R., Wang, Z., and
Kreidenweis, S. M.: Integrating laboratory and field data to quantify the
immersion freezing ice nucleation activity of mineral dust particles, Atmos.
Chem. Phys., 15, 393–409, https://doi.org/10.5194/acp-15-393-2015, 2015.
Dettinger, M. D., Cayan, D. R., Meyer, M. K., and Jeton, A.: Simulated
hydrologic responses to climate variations and change in the Merced, Carson,
and American River basins, Sierra Nevada, California, 1900–2099, Clim.
Change, 62, 283–317, https://doi.org/10.1023/B:CLIM.0000013683.13346.4f, 2004.
Domingo, R. A., Southard, R. J., and Lee, K.: Laboratory System for Dust
Generation from Soils, J. Environ. Qual., 39, 1254–1261,
https://doi.org/10.2134/jeq2008.0380, 2010.
Dueker, M. E., Weathers, K. C., O'Mullan, G. D., Juhl, A. R., and Uriarte,
M.: Environmental Controls on Coastal Coarse Aerosols: Implications for
Microbial Content and Deposition in the Near-Shore Environment, Environ. Sci.
Technol., 45, 3386–3392, https://doi.org/10.1021/es1035128, 2011.
Dutta, P. K., Zhou, Z., and dos Santos, P. R.: A theoretical study of
mineralogical maturation of eolian sand, Geol. Soc. Am. Spec. Pap., 284,
203–209, 1993.
Engelstaedter, S., Tegen, I., and Washington, R.: North African dust
emissions and transport, Earth-Science Rev., 79, 73–100,
https://doi.org/10.1016/j.earscirev.2006.06.004, 2006.
Evan, A. T., Fiedler, S., Zhao, C., Menut, L., Schepanski, K., Flamant, C.,
and Doherty, O.: Derivation of an observation-based map of North African dust
emission, Aeolian Res., 16, 153–162, https://doi.org/10.1016/j.aeolia.2015.01.001, 2015.
Feng, J.-L., Zhu, L.-P., Ju, J.-T., Zhou, L.-P., Zhen, X.-L., Zhang, W., and
Shao-Peng, G.: Heavy dust fall in Beijing on April 16–17, 2006: geochemical
properties and indications of the dust provenance, Geochem. J., 42, 221–236,
https://doi.org/10.2343/geochemj.42.221, 2008.
Fryrear, D.: A field dust sampler, J. Soil Water Conserv., 41, 117–120,
1986.
Gardner, R. and Pye, K.: Nature, origin and palaeoenvironmental significance
of red coastal and desert dune sands, Prog. Phys. Geogr., 5, 514–534,
https://doi.org/10.1177/030913338100500402, 1981.
Gillette, D., Blifford Jr., I., and Fryrear, D.: The influence of wind
velocity on the size distributions of aerosols generated by the wind erosion
of soils, J. Geophys. Res., 79, 4068–4075, https://doi.org/10.1029/JC079i027p04068,
1974.
Gillette, D. A.: On the production of soil wind erosion aerosols having the
potential for long range transport, J. Rech. Atmos., 8, 734–744, 1974.
Gillette, D. A., Blifford, I. H., and Fenster, C. R.: Measurements of aerosol
size distributions and vertical fluxes of aerosols on land subject to wind
erosion, J. Appl. Meteorol. Climatol., 11, 977–987,
https://doi.org/10.1175/1520-0450(1972)011<0977:MOASDA>2.0.CO;2, 1972.
Gillies, J. A., Etyemezian, V., Nikolich, G., Glick, R., Rowland, P., Pesce,
T., and Skinner, M.: Effectiveness of an array of porous fences to reduce
sand flux: Oceano Dunes, Oceano CA, J. Wind Eng. Ind. Aerodyn., 168,
247–259, https://doi.org/10.1016/j.jweia.2017.06.015, 2017.
Gillies, J. A. and Berkofsky, L.: Eolian suspension above the saltation
layer, the concentration profile, J. Sediment. Res., 74, 176–183,
https://doi.org/10.1306/091303740176, 2004.
Ginoux, P., Chin, M., Tegen, I., Prospero, J. M., Holben, B., Dubovik, O.,
and Lin, S.-J.: Sources and distributions of dust aerosols simulated with the
GOCART model, J. Geophys. Res.-Atmos., 106, 20255–20273,
https://doi.org/10.1029/2000JD000053, 2001.
Goossens, D., Buck, B., and McLaurin, B.: Contributions to atmospheric dust
production of natural and anthropogenic emissions in a recreational area
designated for off-road vehicular activity (Nellis Dunes, Nevada, USA), J.
Arid Environ., 78, 80–99, https://doi.org/10.1016/j.jaridenv.2011.10.015, 2012.
Goossens, D. and Buck, B.: Effects of wind erosion, off-road vehicular
activity, atmospheric conditions and the proximity of a metropolitan area on
PM10 characteristics in a recreational site, Atmos. Environ., 45, 94–107,
https://doi.org/10.1016/j.atmosenv.2010.09.046, 2011.
Goossens, D., Offer, Z., and London, G.: Wind tunnel and field calibration of
five aeolian sand traps, Geomorphology, 35, 233–252,
https://doi.org/10.1016/S0169-555X(00)00041-6, 2000.
Gualtieri, A.: Modal analysis of pyroclastic rocks by combined Rietveld and
RIR methods, Powder Diffr., 11, 97–106, https://doi.org/10.1017/S0885715600009052, 1996.
Gualtieri, A. F.: Accuracy of XRPD QPA using the combined Rietveld-RIR
method, J. Appl. Crystallogr., 33, 267–278, https://doi.org/10.1107/S002188989901643X,
2000.
Hillel, D.: Environmental soil physics, 1st ed., Academic Press, San Diego,
771 pp., 1998.
Hinds, W. C.: Aerosol technology: properties, behavior, and measurement of
airborne particles, 2nd ed., Wiley-Interscience, 504 pp., 1999.
Huneeus, N., Schulz, M., Balkanski, Y., Griesfeller, J., Prospero, J., Kinne,
S., Bauer, S., Boucher, O., Chin, M., Dentener, F., Diehl, T., Easter, R.,
Fillmore, D., Ghan, S., Ginoux, P., Grini, A., Horowitz, L., Koch, D., Krol,
M. C., Landing, W., Liu, X., Mahowald, N., Miller, R., Morcrette, J.-J.,
Myhre, G., Penner, J., Perlwitz, J., Stier, P., Takemura, T., and Zender, C.
S.: Global dust model intercomparison in AeroCom phase I, Atmos. Chem. Phys.,
11, 7781–7816, https://doi.org/10.5194/acp-11-7781-2011, 2011.
ISO: Determination of particle size distribution: single particle light
interaction methods, part 1: Light scattering aerosol spectrometer, ISO
21501-1, 2009.
Ito, A. and Kok, J. F.: Do dust emissions from sparsely vegetated regions
dominate atmospheric iron supply to the Southern Ocean?, J. Geophys.
Res.-Atmos., 122, 3987–4002, https://doi.org/10.1002/2016JD025939, 2017.
James, W. C., Mack, G. H., and Suttner, L. J.: Relative alteration of
microcline and sodic plagioclase in semi-arid and humid climates, J.
Sediment. Petrol., 51, 151–163, 1981.
Jari, M.: Effects of grinding and chemical factors on the generation and
composition of the till fine fraction: an experimental study, J. Geochemical
Explor., 54, 49–62, https://doi.org/10.1016/0375-6742(95)00008-D, 1995.
Jerolmack, D. J. and Brzinski, T. A.: Equivalence of abrupt grain-size
transitions in alluvial rivers and eolian sand seas: A hypothesis, Geology,
38, 719–722, https://doi.org/10.1130/G30922.1, 2010.
Jerolmack, D. J., Reitz, M. D., and Martin, R. L.: Sorting out abrasion in a
gypsum dune field, J. Geophys. Res. Earth Surf., 116, F02003,
https://doi.org/10.1029/2010JF001821, 2011.
Kandler, K., Benker, N., Bundke, U., Cuevas, E., Ebert, M., Knippertz, P.,
Rodríguez, S., Schütz, L., and Weinbruch, S.: Chemical composition
and complex refractive index of Saharan Mineral Dust at Izaña, Tenerife
(Spain) derived by electron microscopy, Atmos. Environ., 41, 8058–8074,
https://doi.org/10.1016/j.atmosenv.2007.06.047, 2007.
Kasper-Zubillaga, J. J., Zolezzi-Ruíz, H., Carranza-Edwards, A.,
Girón-García, P., Ortiz-Zamora, G., and Palma, M.: Sedimentological,
modal analysis and geochemical studies of desert and coastal dunes, Altar
Desert, NW Mexico, Earth Surf. Process. Landforms, 32, 489–508,
https://doi.org/10.1002/esp.1402, 2007.
Katra, I. and Yizhaq, H.: Intensity and degree of segregation in bimodal and
multimodal grain size distributions, Aeolian Res., 27, 23–34,
https://doi.org/10.1016/j.aeolia.2017.05.002, 2017.
Kind, R. J.: One-dimensional aeolian suspension above beds of loose
particles – A new concentration-profile equation, Atmos. Environ., 26A,
927–931, https://doi.org/10.1016/0960-1686(92)90250-O, 1992.
Klose, M. and Shao, Y.: Stochastic parameterization of dust emission and
application to convective atmospheric conditions, Atmos. Chem. Phys., 12,
7309–7320, https://doi.org/10.5194/acp-12-7309-2012, 2012.
Klute, E. A.: Methods of Soil Analysis. Part 1. Physical and Mineralogical
Methods, 2nd ed., edited by: Dinauer, R. C., American Society of Agronomy,
Inc., Soil Science Society of America, Inc., Madison, Wisconsin USA, 1358
pp., 1986.
Kok, J. F.: A scaling theory for the size distribution of emitted dust
aerosols suggests climate models underestimate the size of the global dust
cycle, P. Natl. Acad. Sci. USA, 108, 1016–1021, https://doi.org/10.1073/pnas.1014798108,
2011.
Kok, J. F., Parteli, E. J. R., Michaels, T. I., and Karam, D. B.: The physics
of wind-blown sand and dust, Reports Prog. Phys., 75,
https://doi.org/10.1088/0034-4885/75/10/106901, 2012.
Kok, J. F., Mahowald, N. M., Fratini, G., Gillies, J. A., Ishizuka, M., Leys,
J. F., Mikami, M., Park, M. S., Park, S. U., Van Pelt, R. S., and Zobeck, T.
M.: An improved dust emission model – Part 1: Model description and
comparison against measurements, Atmos. Chem. Phys., 14, 13023–13041,
https://doi.org/10.5194/acp-14-13023-2014, 2014a.
Kok, J. F., Albani, S., Mahowald, N. M., and Ward, D. S.: An improved dust
emission model – Part 2: Evaluation in the Community Earth System Model,
with implications for the use of dust source functions, Atmos. Chem. Phys.,
14, 13043–13061, https://doi.org/10.5194/acp-14-13043-2014, 2014b.
Kok, J. F., Ridley, D. A., Zhou, Q., Miller, R. L., Zhao, C., Heald, C. L.,
Ward, D. S., Albani, S., and Haustein, K.: Smaller desert dust cooling effect
estimated from analysis of dust size and abundance, Nat. Geosci., 10,
274–278, https://doi.org/10.1038/ngeo2912, 2017.
Kok, J. F., Ward, D. S., Mahowald, N. M., and Evan, A. T.: Global and
regional importance of the direct dust-climate feedback, Nat. Commun., 9,
241, https://doi.org/10.1038/s41467-017-02620-y, 2018.
Kuenen, P. H.: Experimental abrasion 4: Eolian Action, J. Geol., 68,
427–449, https://doi.org/10.1086/626675, 1960.
Kuenen, P. H.: Origin of quartz silt, J. Sediment. Res., 39, 1631–1633,
https://doi.org/10.1306/74D71ED3-2B21-11D7-8648000102C1865D, 1969.
Liang, T., Chamecki, M., and Yu, X.: Sea salt aerosol deposition in the
coastal zone: A large eddy simulation study, Atmos. Res., 180, 119–127,
https://doi.org/10.1016/j.atmosres.2016.05.019, 2016.
Liu, H., Peters, G., and Foken, T.: New equations for sonic temperature
variance and buoyancy heat flux with an omnidirectional sonic anemometer,
Boundary-Layer Meteorol., 100, 459–468, https://doi.org/10.1023/A:1019207031397, 2001.
Mahowald, N., Albani, S., Kok, J. F., Engelstaeder, S., Scanza, R., Ward, D.
S., and Flanner, M. G.: The size distribution of desert dust aerosols and its
impact on the Earth system, Aeolian Res., 15, 53–71,
https://doi.org/10.1016/j.aeolia.2013.09.002, 2014.
Marticorena, B. and Bergametti, G.: Modeling the atmospheric dust cycle: 1.
Design of a soil-derived dust emission scheme, J. Geophys. Res.-Atmos., 100,
16415–16430, https://doi.org/10.1029/95JD00690, 1995.
Martin, R. L. and Kok, J. F.: Wind-invariant saltation heights imply linear
scaling of aeolian saltation flux with shear stress, Sci. Adv., 3, e1602569,
https://doi.org/10.1126/sciadv.1602569, 2017.
Martin, R. L. and Kok, J. F.: Distinct Thresholds for the Initiation and
Cessation of Aeolian Saltation From Field Measurements, J. Geophys. Res.
Earth Surf., 123, 1546–1565, https://doi.org/10.1029/2017JF004416, 2018.
Martin, R. L., Kok, J. F., Hugenholtz, C. H., Barchyn, T. E., Chamecki, M.,
and Ellis, J. T.: High-frequency measurements of aeolian saltation flux:
Field-based methodology and applications, Aeolian Res., 30, 97–114,
https://doi.org/10.1016/j.aeolia.2017.12.003, 2018.
Mätzler, C.: MATLAB Functions for Mie Scattering and Absorption, IAP Res. Rep., version
2, 1–24, https://doi.org/10.1039/b811392k, 2002.
McConnell, C. L., Highwood, E. J., Coe, H., Formenti, P., Anderson, B.,
Osborne, S., Nava, S., Desboeufs, K., Chen, G., and Harrison, M. A. J.:
Seasonal variations of the physical and optical characteristics of Saharan
dust: Results from the Dust Outflow and Deposition to the Ocean (DODO)
experiment, J. Geophys. Res.-Atmos., 113, D14S05, https://doi.org/10.1029/2007JD009606,
2008.
McKee, E. D.: Ancient sandstones considered to be eolian, US Geol. Surv.
Prof. Pap., 1052, 189–238, 1979.
McKee, E. D.: Eolian Sand Bodies of the World, in: Eolian Sediments and
Processes, edited by: Brookfield, M. E. and Ahlbrandt, T. S., 1st edn.,
Developments in Sedimentology, 38, 1–25, Elsevier, New York,
https://doi.org/10.1016/S0070-4571(08)70785-4, 1983.
Miller, R. L., Cakmur, R. V., Perlwitz, J., Geogdzhayev, I. V., Ginoux, P.,
Koch, D., Kohfeld, K. E., Prigent, C., Ruedy, R., Schmidt, G. A., and Tegen,
I.: Mineral dust aerosols in the NASA Goddard Institute for Space Sciences
ModelE atmospheric general circulation model, J. Geophys. Res.-Atmos., 111,
D06208, https://doi.org/10.1029/2005JD005796, 2006.
Miller, R. L., Tegen, I., and Perlwitz, J.: Surface radiative forcing by soil
dust aerosols and the hydrologic cycle, J. Geophys. Res.-Atmos., 109, D04203,
https://doi.org/10.1029/2003JD004085, 2004.
Moreno, T., Gibbons, W., Jones, T., and Richards, R.: The geology of ambient
aerosols: characterising urban and rural/coastal silicate PM10−2.5 and
PM2.5 using high-volume cascade collection and scanning electron
microscopy, Atmos. Environ., 37, 4265–4276,
https://doi.org/10.1016/S1352-2310(03)00534-X, 2003.
Muhs, D. R.: Mineralogical maturity in dunefields of North America, Africa
and Australia, Geomorphology, 59, 247–269,
https://doi.org/10.1016/j.geomorph.2003.07.020, 2004.
Muhs, D. R., Stafford, T. W., Swinehart, J. B., Cowherd, S. D., Mahan, S. A.,
Bush, C. A., Madole, R. F., and Maat, P. B.: Late Holocene eolian activity in
the mineralogically mature Nebraska Sand Hills, Quat. Res., 48, 162–176,
https://doi.org/10.1006/qres.1997.1913, 1997.
Murray, B. J., O'Sullivan, D., Atkinson, J. D., and Webb, M. E.: Ice
nucleation by particles immersed in supercooled cloud droplets, Chem. Soc.
Rev., 41, 6519, https://doi.org/10.1039/c2cs35200a, 2012.
Nesbitt, H. W., Fedo, C. M., and Young, G. M.: Quartz and Feldspar Stability,
Steady and Non-Steady-State Weathering, and Petrogenesis of Siliciclastic
Sands and Muds, J. Geol., 105, 173–192, https://doi.org/10.1086/515908, 1997.
Nousiainen, T. and Kandler, K.: Light scattering by atmospheric mineral dust
particles, Light Scatt. Rev. 9, 3–52, 2015.
O'Dowd, C. D. and de Leeuw, G.: Marine aerosol production: a review of the
current knowledge, Philos. Trans. R. Soc. A Math. Phys. Eng. Sci., 365, 1856,
1753–1774, https://doi.org/10.1098/rsta.2007.2043, 2007.
O'Hara-Dhand, K., Taylor, R. L. S., Smalley, I. J., Krinsley, D. H., and
Vita-Finzi, C.: Loess and dust on Earth and Mars: particle generation by
impact mechanisms, Cent. Eur. J. Geosci., 2, 45–51,
https://doi.org/10.2478/v10085-010-0001-z, 2010.
Okada, K., Heintzenberg, J., Kai, K., and Qin, Y.: Shape of atmospheric
mineral particles collected in three Chinese arid-regions, Geophys. Res.
Lett., 28, 3123–3126, https://doi.org/10.1029/2000GL012798, 2001.
Orme, A. R.: Late Quaternary Deposits Near Point Sal, South Central
California: A Time Frame For Coastal-Dune Emplacement, Soc. Sediment. Geol.
Spec. Publ., 48, 310–315, https://doi.org/10.2110/pec.92.48.0309, 1992.
Osborne, S. R., Johnson, B. T., Haywood, J. M., Baran, A. J., Harrison, M. A.
J., and McConnell, C. L.: Physical and optical properties of mineral dust
aerosol during the Dust and Biomass-burning Experiment, J. Geophys.
Res.-Atmos., 113, D00C03, https://doi.org/10.1029/2007JD009551, 2008.
Ouren, B. D. S., Haas, C., Melcher, C. P., Stewart, S. C., Ponds, P. D.,
Secton, N. R., Burris, L., Fancher, T., and Bowen, Z. H.: Environmental
effects of off-highway vehicles on bureau of land management lands: a
literature synthesis, annotated bibliographies, extensive bibliographies, and
internet resources, U.S. Geol. Surv. Open-File Rep. 2007-1353, available at:
https://pubs.usgs.gov/of/2007/1353/report.pdf (last access:
27 February 2019), 2007.
Price, H. C., Baustian, K. J., McQuaid, J. B., Blyth, A., Bower, K. N.,
Choularton, T., Cotton, R. J., Cui, Z., Field, P. R., Gallagher, M., Hawker,
R., Merrington, A., Miltenberger, A., Neely, R. R., Parker, S. T., Rosenberg,
P. D., Taylor, J. W., Trembath, J., Vergara-Temprado, J., Whale, T. F.,
Wilson, T. W., Young, G., and Murray, B. J.: Atmospheric ice-nucleating
particles in the dusty tropical Atlantic, J. Geophys. Res.-Atmos., 123,
2175–2193, https://doi.org/10.1002/2017JD027560, 2018.
Prospero, J. M., Ginoux, P., Torres, O., Nicholson, S. E., and Gill, T. E.:
Environmental characterization of global sources of atmospheric soil dust
identified with the NIMBUS 7 Total Ozone Mapping Spectrometer (TOMS)
absorbing aerosol product, Rev. Geophys., 40, 1002, https://doi.org/10.1029/2000RG000095,
2002.
Pye, K. and Sperling, C. H. B.: Experimental investigation of silt formation
by static breakage processes: the effect of temperature, moisture and salt on
quartz dune sand and granitic regolith, Sedimentology, 30, 49–62,
https://doi.org/10.1111/j.1365-3091.1983.tb00649.x, 1983.
Pye, K. and Tsoar, H.: Aeolian sand and sand dunes, 1st ed., Springer, Berlin
Heidelberg, 457 pp., 2009.
Ramanathan, V., Crutzen, P. J., Kiehl, J. T., and Rosenfeld, D.: Aerosols,
climate, and the hydrological cycle, Science, 294, 2119–2124,
https://doi.org/10.1126/science.1064034, 2001.
Rosenberg, P. D., Dean, A. R., Williams, P. I., Dorsey, J. R., Minikin, A.,
Pickering, M. A., and Petzold, A.: Particle sizing calibration with
refractive index correction for light scattering optical particle counters
and impacts upon PCASP and CDP data collected during the Fennec campaign,
Atmos. Meas. Tech., 5, 1147–1163, https://doi.org/10.5194/amt-5-1147-2012,
2012.
Rosenberg, P. D., Parker, D. J., Ryder, C. L., Marsham, J. H.,
Garcia-Carrersa, L., Dorsey, J. R., Brooks, I. M., Dean, A. R., Crosier, J.,
McQuaid, J. B., and Washington, R.: Quantifying particle size and turbulent
scale dependence of dust flux in the Sahara using aircraft measurements, J.
Geophys. Res.-Atmos., 119, 7577–7598, https://doi.org/10.1002/2013JD021255, 2014.
Ryder, C. L., Highwood, E. J., Rosenberg, P. D., Trembath, J., Brooke, J. K.,
Bart, M., Dean, A., Crosier, J., Dorsey, J., Brindley, H., Banks, J.,
Marsham, J. H., McQuaid, J. B., Sodemann, H., and Washington, R.: Optical
properties of Saharan dust aerosol and contribution from the coarse mode as
measured during the Fennec 2011 aircraft campaign, Atmos. Chem. Phys., 13,
303–325, https://doi.org/10.5194/acp-13-303-2013, 2013.
Ryder, C. L., Marenco, F., Brooke, J. K., Estelles, V., Cotton, R., Formenti,
P., McQuaid, J. B., Price, H. C., Liu, D., Ausset, P., Rosenberg, P. D.,
Taylor, J. W., Choularton, T., Bower, K., Coe, H., Gallagher, M., Crosier,
J., Lloyd, G., Highwood, E. J., and Murray, B. J.: Coarse-mode mineral dust
size distributions, composition and optical properties from AER-D aircraft
measurements over the tropical eastern Atlantic, Atmos. Chem. Phys., 18,
17225–17257, https://doi.org/10.5194/acp-18-17225-2018, 2018.
Shao, Y.: Physics and modelling of wind erosion, 2nd ed., edited by: Shao,
Y., Springer, the Netherlands, 452 pp., 2008.
Shao, Y., Raupach, M. R., and Findlater, P. A.: Effect of saltation
bombardment on the entrainment of dust by wind, J. Geophys. Res.-Atmos., 98,
12719–12726, https://doi.org/10.1029/93JD00396, 1993.
Shao, Y., Ishizuka, M., Mikami, M., and Leys, J. F.: Parameterization of
size-resolved dust emission and validation with measurements, J. Geophys.
Res.-Atmos., 116, D08203, https://doi.org/10.1029/2010JD014527, 2011.
Sommariva, M., Gateshki, M., Gertenbach, J. A., Bolze, J., König, U.,
Vasile, B. Ş., and Surdu, V. A.: Characterizing nanoparticles with a
laboratory diffractometer: From small-angle to total X-ray scattering, Powder
Diff., 29, S47–S53, https://doi.org/10.1017/S0885715614001043, 2014.
Sow, M., Alfaro, S. C., Rajot, J. L., and Marticorena, B.: Size resolved dust
emission fluxes measured in Niger during 3 dust storms of the AMMA
experiment, Atmos. Chem. Phys., 9, 3881–3891,
https://doi.org/10.5194/acp-9-3881-2009, 2009.
Sterk, G., Jacobs, A. F. G., and Van Boxel, J. H.: The effect of turbulent
flow structures on saltation sand transport in the atmospheric boundary
layer, Earth Surf. Process. Landf., 23, 877–887,
https://doi.org/10.1002/(SICI)1096-9837(199810)23:10<877::AID-ESP905>3.0.CO;2-R, 1998.
Stull, R. B.: An introduction to boundary layer meteorology, 1st ed.,
Springer Netherlands, 666 pp., 1988.
Sweeney, M. R., Zlotnik, V. A., Joeckel, R. M., and Stout, J. E.: Geomorphic
and hydrologic controls of dust emissions during drought from Yellow Lake
playa, West Texas, USA, J. Arid Environ., 133, 37–46,
https://doi.org/10.1016/j.jaridenv.2016.05.007, 2016.
Swet, N. and Katra, I.: Reduction in soil aggregation in response to dust
emission processes, Geomorphology, 268, 177–183,
https://doi.org/10.1016/j.geomorph.2016.06.002, 2016.
Tegen, I., Harrison, S. P., Kohfeld, K., Prentice, C. I., Coe, M., and
Heimann, M.: Impact of vegetation and preferential source areas on global
dust aerosol: Results from a model study, J. Geophys. Res.-Atmos.,
107, AAC 14-1–AAC 14-27, https://doi.org/10.1029/2001JD000963, 2002.
Tiessen, H., Hauffe, H. K., and Mermut, A. R.: Deposition of Harmattan dust
and its influence on base saturation of soils in northern Ghana, Geoderma,
49, 285–299, https://doi.org/10.1016/0016-7061(91)90081-4, 1991.
Vaughan, M.: Air Board Approves Historic Order for State Parks to Reduce Dust
from Oceano Dunes, The Tribune (San Luis Obispo, California), 30 April,
available at:
https://www.sanluisobispo.com/news/local/environment/article210047754.html
(last access: 27 February 2019), 2018.
von der Weiden, S.-L., Drewnick, F., and Borrmann, S.: Particle Loss
Calculator – a new software tool for the assessment of the performance of
aerosol inlet systems, Atmos. Meas. Tech., 2, 479–494,
https://doi.org/10.5194/amt-2-479-2009, 2009.
Webb, N. P., Strong, C. L., Chappell, A., Marx, S. K., and McTainsh, G. H.:
Soil organic carbon enrichment of dust emissions: magnitude, mechanisms and
its implications for the carbon cycle, Earth Surf. Process. Landforms, 38,
1662–1671, https://doi.org/10.1002/esp.3404, 2013.
Weinzierl, B., Petzold, A., Esselborn, M., Wirth, M., Rasp, K., Kandler, K.,
Schütz, L., Koepke, P., and Fiebig, M.: Airborne measurements of dust
layer properties, particle size distribution and mixing state of Saharan dust
during SAMUM 2006, Tellus, 61, 96–117, https://doi.org/10.1111/j.1600-0889.2008.00392.x,
2009.
Whalley, W. B., Smith, B. J., McAlister, J. J., and Edwards, A. J.: Aeolian
abrasion of quartz particles and the production of silt-size fragments:
preliminary results, Geol. Soc. London, Spec. Publ., 35, 129–138,
https://doi.org/10.1144/GSL.SP.1987.035.01.09, 1987.
Wright, J.: Making loess-sized quartz silt: data from laboratory simulations
and implications for sediment transport pathways and the formation of
“desert” loess deposits associated with the Sahara, Quat. Int., 76–77,
7–19, https://doi.org/10.1016/S1040-6182(00)00085-9, 2001.
Wright, J., Smith, B., and Whalley, B.: Mechanisms of loess-sized quartz silt
production and their relative effectiveness: Laboratory simulations,
Geomorphology, 23, 15–34, https://doi.org/10.1016/S0169-555X(97)00084-6,
1998.
Yizhaq, H., Ashkenazy, Y., and Tsoar, H.: Sand dune dynamics and climate
change: A modeling approach, J. Geophys. Res.-Earth, 114, F01023,
https://doi.org/10.1029/2008JF001138, 2009.
Zender, C. S., Bian, H., and Newman, D.: Mineral Dust Entrainment and
Deposition (DEAD) model: Description and 1990s dust climatology, J. Geophys.
Res., 108, 4416, https://doi.org/10.1029/2002JD002775, 2003.
Zobeck, T. M. and Van Pelt, R. S.: Wind-induced dust generation and transport
mechanics on a bare agricultural field, J. Hazard. Mater., 132, 26–38,
https://doi.org/10.1016/j.jhazmat.2005.11.090, 2006.
Short summary
This paper provides important insights on dust emission from sand dunes, which cover a large fraction of arid lands; produces the first in situ measurements for size-resolved dust emission from active sands that could improve the representation of dust cycle in climate models and remote sensing techniques; and shows that dust from active sands is likely significantly finer than thought, implying a greater effect of dust emission from active sands on downwind climate, hydrology, and human health.
This paper provides important insights on dust emission from sand dunes, which cover a large...
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