Articles | Volume 17, issue 11
Atmos. Chem. Phys., 17, 6679–6691, 2017
https://doi.org/10.5194/acp-17-6679-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 17, 6679–6691, 2017
https://doi.org/10.5194/acp-17-6679-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
07 Jun 2017
Research article
| 07 Jun 2017
Continuous vertical aerosol profiling with a multi-wavelength Raman polarization lidar over the Pearl River Delta, China
Birgit Heese et al.
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Athena Augusta Floutsi, Holger Baars, Ronny Engelmann, Dietrich Althausen, Albert Ansmann, Stephanie Bohlmann, Birgit Heese, Julian Hofer, Thomas Kanitz, Moritz Haarig, Kevin Ohneiser, Martin Radenz, Patric Seifert, Annett Skupin, Zhenping Yin, Sabur F. Abdullaev, Mika Komppula, Maria Filioglou, Elina Giannakaki, Iwona S. Stachlewska, Lucja Janicka, Daniele Bortoli, Eleni Marinou, Vassilis Amiridis, Anna Gialitaki, Rodanthi-Elisavet Mamouri, Boris Barja, and Ulla Wandinger
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2022-306, https://doi.org/10.5194/amt-2022-306, 2022
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DeLiAn is a collection of lidar-derived aerosol intensive optical properties for several aerosol types, namely the particle linear depolarization ratio, the extinction-to-backscatter ratio (lidar ratio), and the Ångström exponent. The data collection is based on globally distributed, long-term, ground-based, multiwavelength, Raman and polarisation lidar measurements and currently covers two wavelengths, 355 and 532 nm, for 13 aerosol categories ranging from basic aerosol types to mixtures.
Birgit Heese, Athena Augusta Floutsi, Holger Baars, Dietrich Althausen, Julian Hofer, Alina Herzog, Silke Mewes, Martin Radenz, and Yoav Y. Schechner
Atmos. Chem. Phys., 22, 1633–1648, https://doi.org/10.5194/acp-22-1633-2022, https://doi.org/10.5194/acp-22-1633-2022, 2022
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The aerosol distribution over Haifa, Israel, was measured for 2 years by a laser-based vertically resolved measurement technique called lidar. From these data, the aerosol types and their percentages of the observed aerosol mixtures were identified in terms of their size and shape. We found mostly desert dust from the surrounding deserts and sea salt from the close-by Mediterranean Sea. But aerosols from anthropogenic and industrial pollution from local and far away sources were also detected.
Holger Baars, Alina Herzog, Birgit Heese, Kevin Ohneiser, Karsten Hanbuch, Julian Hofer, Zhenping Yin, Ronny Engelmann, and Ulla Wandinger
Atmos. Meas. Tech., 13, 6007–6024, https://doi.org/10.5194/amt-13-6007-2020, https://doi.org/10.5194/amt-13-6007-2020, 2020
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A first validation for the European satellite Aeolus is presented. Aeolus is the first satellite that can actively measure horizontal wind profiles from space.
Radiosonde launches on board the German research vessel Polarstern have been utilized to validate Aeolus observations over the Atlantic Ocean, a region where almost no other reference measurements are available. It is shown that Aeolus is able to measure accurately atmospheric winds and thus may significantly improve weather forecasts.
Holger Baars, Albert Ansmann, Kevin Ohneiser, Moritz Haarig, Ronny Engelmann, Dietrich Althausen, Ingrid Hanssen, Michael Gausa, Aleksander Pietruczuk, Artur Szkop, Iwona S. Stachlewska, Dongxiang Wang, Jens Reichardt, Annett Skupin, Ina Mattis, Thomas Trickl, Hannes Vogelmann, Francisco Navas-Guzmán, Alexander Haefele, Karen Acheson, Albert A. Ruth, Boyan Tatarov, Detlef Müller, Qiaoyun Hu, Thierry Podvin, Philippe Goloub, Igor Veselovskii, Christophe Pietras, Martial Haeffelin, Patrick Fréville, Michaël Sicard, Adolfo Comerón, Alfonso Javier Fernández García, Francisco Molero Menéndez, Carmen Córdoba-Jabonero, Juan Luis Guerrero-Rascado, Lucas Alados-Arboledas, Daniele Bortoli, Maria João Costa, Davide Dionisi, Gian Luigi Liberti, Xuan Wang, Alessia Sannino, Nikolaos Papagiannopoulos, Antonella Boselli, Lucia Mona, Giuseppe D'Amico, Salvatore Romano, Maria Rita Perrone, Livio Belegante, Doina Nicolae, Ivan Grigorov, Anna Gialitaki, Vassilis Amiridis, Ourania Soupiona, Alexandros Papayannis, Rodanthi-Elisaveth Mamouri, Argyro Nisantzi, Birgit Heese, Julian Hofer, Yoav Y. Schechner, Ulla Wandinger, and Gelsomina Pappalardo
Atmos. Chem. Phys., 19, 15183–15198, https://doi.org/10.5194/acp-19-15183-2019, https://doi.org/10.5194/acp-19-15183-2019, 2019
Daniel Moran-Zuloaga, Florian Ditas, David Walter, Jorge Saturno, Joel Brito, Samara Carbone, Xuguang Chi, Isabella Hrabě de Angelis, Holger Baars, Ricardo H. M. Godoi, Birgit Heese, Bruna A. Holanda, Jošt V. Lavrič, Scot T. Martin, Jing Ming, Mira L. Pöhlker, Nina Ruckteschler, Hang Su, Yaqiang Wang, Qiaoqiao Wang, Zhibin Wang, Bettina Weber, Stefan Wolff, Paulo Artaxo, Ulrich Pöschl, Meinrat O. Andreae, and Christopher Pöhlker
Atmos. Chem. Phys., 18, 10055–10088, https://doi.org/10.5194/acp-18-10055-2018, https://doi.org/10.5194/acp-18-10055-2018, 2018
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This study presents multiple years of aerosol coarse mode observations at the remote ATTO site in the Amazon Basin. The results are discussed in light of the frequent and episodic long-range transport of Saharan dust plumes in the early wet season as well as the persistent background bioaerosol cycling in the rain forest ecosystem. This work provides a solid basis for future studies on the dynamic coarse mode aerosol cycling and its biogeochemical relevance in the Amazon.
Ronny Engelmann, Thomas Kanitz, Holger Baars, Birgit Heese, Dietrich Althausen, Annett Skupin, Ulla Wandinger, Mika Komppula, Iwona S. Stachlewska, Vassilis Amiridis, Eleni Marinou, Ina Mattis, Holger Linné, and Albert Ansmann
Atmos. Meas. Tech., 9, 1767–1784, https://doi.org/10.5194/amt-9-1767-2016, https://doi.org/10.5194/amt-9-1767-2016, 2016
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The atmospheric science community demands for autonomous and quality-assured vertically resolved measurements of aerosol and cloud properties. For this purpose, a portable lidar called Polly
was developed at TROPOS in 2003. This lidar type was continuously improved with gained experience from EARLINET, worldwide field campaigns, and institute collaborations within the last 10 years. We present recent changes to the setup of our portable multiwavelength Raman and polarization lidar PollyXT.
Holger Baars, Thomas Kanitz, Ronny Engelmann, Dietrich Althausen, Birgit Heese, Mika Komppula, Jana Preißler, Matthias Tesche, Albert Ansmann, Ulla Wandinger, Jae-Hyun Lim, Joon Young Ahn, Iwona S. Stachlewska, Vassilis Amiridis, Eleni Marinou, Patric Seifert, Julian Hofer, Annett Skupin, Florian Schneider, Stephanie Bohlmann, Andreas Foth, Sebastian Bley, Anne Pfüller, Eleni Giannakaki, Heikki Lihavainen, Yrjö Viisanen, Rakesh Kumar Hooda, Sérgio Nepomuceno Pereira, Daniele Bortoli, Frank Wagner, Ina Mattis, Lucja Janicka, Krzysztof M. Markowicz, Peggy Achtert, Paulo Artaxo, Theotonio Pauliquevis, Rodrigo A. F. Souza, Ved Prakesh Sharma, Pieter Gideon van Zyl, Johan Paul Beukes, Junying Sun, Erich G. Rohwer, Ruru Deng, Rodanthi-Elisavet Mamouri, and Felix Zamorano
Atmos. Chem. Phys., 16, 5111–5137, https://doi.org/10.5194/acp-16-5111-2016, https://doi.org/10.5194/acp-16-5111-2016, 2016
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The findings from more than 10 years of global aerosol lidar measurements with Polly systems are summarized, and a data set of optical properties for specific aerosol types is given. An automated data retrieval algorithm for continuous Polly lidar observations is presented and discussed by means of a Saharan dust advection event in Leipzig, Germany. Finally, a statistic on the vertical aerosol distribution including the seasonal variability at PollyNET locations around the globe is presented.
E. Jäkel, B. Mey, R. Levy, X. Gu, T. Yu, Z. Li, D. Althausen, B. Heese, and M. Wendisch
Atmos. Meas. Tech., 8, 5237–5249, https://doi.org/10.5194/amt-8-5237-2015, https://doi.org/10.5194/amt-8-5237-2015, 2015
Ulla Wandinger, Athena Augusta Floutsi, Holger Baars, Moritz Haarig, Albert Ansmann, Anja Hünerbein, Nicole Docter, David Donovan, Gerd-Jan van Zadelhoff, Shannon Mason, and Jason Cole
EGUsphere, https://doi.org/10.5194/egusphere-2022-1241, https://doi.org/10.5194/egusphere-2022-1241, 2022
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
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We introduce an aerosol classification model that has been developed for the Earth Clouds, Aerosols and Radiation Explorer (EarthCARE). The model provides a consistent description of microphysical, optical, and radiative properties of common aerosol types such as dust, sea salt, pollution, and smoke. It is used for aerosol classification and assessment of radiation effects based on the synergy of active and passive observations with lidar, imager, and radiometer of the multi-instrument platform.
Athena Augusta Floutsi, Holger Baars, Ronny Engelmann, Dietrich Althausen, Albert Ansmann, Stephanie Bohlmann, Birgit Heese, Julian Hofer, Thomas Kanitz, Moritz Haarig, Kevin Ohneiser, Martin Radenz, Patric Seifert, Annett Skupin, Zhenping Yin, Sabur F. Abdullaev, Mika Komppula, Maria Filioglou, Elina Giannakaki, Iwona S. Stachlewska, Lucja Janicka, Daniele Bortoli, Eleni Marinou, Vassilis Amiridis, Anna Gialitaki, Rodanthi-Elisavet Mamouri, Boris Barja, and Ulla Wandinger
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2022-306, https://doi.org/10.5194/amt-2022-306, 2022
Preprint under review for AMT
Short summary
Short summary
DeLiAn is a collection of lidar-derived aerosol intensive optical properties for several aerosol types, namely the particle linear depolarization ratio, the extinction-to-backscatter ratio (lidar ratio), and the Ångström exponent. The data collection is based on globally distributed, long-term, ground-based, multiwavelength, Raman and polarisation lidar measurements and currently covers two wavelengths, 355 and 532 nm, for 13 aerosol categories ranging from basic aerosol types to mixtures.
Albert Ansmann, Kevin Ohneiser, Alexandra Chudnovsky, Daniel A. Knopf, Edwin W. Eloranta, Diego Villanueva, Patric Seifert, Martin Radenz, Boris Barja, Félix Zamorano, Cristofer Jimenez, Ronny Engelmann, Holger Baars, Hannes Griesche, Julian Hofer, Dietrich Althausen, and Ulla Wandinger
Atmos. Chem. Phys., 22, 11701–11726, https://doi.org/10.5194/acp-22-11701-2022, https://doi.org/10.5194/acp-22-11701-2022, 2022
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For the first time we present a systematic study on the impact of wildfire smoke on ozone depletion in the Arctic (2020) and Antarctic stratosphere (2020, 2021). Two major fire events in Siberia and Australia were responsible for the observed record-breaking stratospheric smoke pollution. Our analyses were based on lidar observations of smoke parameters (Polarstern, Punta Arenas) and NDACC Arctic and Antarctic ozone profiles as well as on Antarctic OMI satellite observations of column ozone.
Xianda Gong, Martin Radenz, Heike Wex, Patric Seifert, Farnoush Ataei, Silvia Henning, Holger Baars, Boris Barja, Albert Ansmann, and Frank Stratmann
Atmos. Chem. Phys., 22, 10505–10525, https://doi.org/10.5194/acp-22-10505-2022, https://doi.org/10.5194/acp-22-10505-2022, 2022
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The sources of ice-nucleating particles (INPs) are poorly understood in the Southern Hemisphere (SH). We studied INPs in the boundary layer in the southern Patagonia region. No seasonal cycle of INP concentrations was observed. The majority of INPs are biogenic particles, likely from local continental sources. The INP concentrations are higher when strong precipitation occurs. While previous studies focused on marine INP sources in SH, we point out the importance of continental sources of INPs.
Bernd Heinold, Holger Baars, Boris Barja, Matthew Christensen, Anne Kubin, Kevin Ohneiser, Kerstin Schepanski, Nick Schutgens, Fabian Senf, Roland Schrödner, Diego Villanueva, and Ina Tegen
Atmos. Chem. Phys., 22, 9969–9985, https://doi.org/10.5194/acp-22-9969-2022, https://doi.org/10.5194/acp-22-9969-2022, 2022
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The extreme 2019–2020 Australian wildfires produced massive smoke plumes lofted into the lower stratosphere by pyrocumulonimbus convection. Most climate models do not adequately simulate the injection height of such intense fires. By combining aerosol-climate modeling with prescribed pyroconvective smoke injection and lidar observations, this study shows the importance of the representation of the most extreme wildfire events for estimating the atmospheric energy budget.
Konstantinos Michailidis, Maria-Elissavet Koukouli, Dimitris Balis, Pepijn Veefkind, Martin de Graaf, Lucia Mona, Nikolaos Papagianopoulos, Gesolmina Pappalardo, Ioanna Tsikoudi, Vassilis Amiridis, Eleni Marinou, Anna Gialitaki, Rodanthi-Elissavet Mamouri, Argyro Nisantzi, Daniele Bortoli, Maria João Costa, Vanda Salgueiro, Alexandros Papayannis, Maria Mylonaki, Lucas Alados-Arboledas, Salvatore Romano, Maria Rita Perrone, and Holger Baars
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-412, https://doi.org/10.5194/acp-2022-412, 2022
Preprint under review for ACP
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Modern satellite-born sensors have the ability to derive accurate geometrical features of lofted aerosol layers on a continental scale, such as the S5P/TROPOMI instrument. Comparisons with ground-based correlative measurements constitute a key component in the validation of the more recent-in-existence satellite aerosol products. Three days with sufficient dust and smoke aerosol load over the Mediterranean are used to illustrate the performance of the TROPOMI ALH product.
Antonis Gkikas, Anna Gialitaki, Ioannis Binietoglou, Eleni Marinou, Maria Tsichla, Nikolaos Siomos, Peristera Paschou, Anna Kampouri, Kalliopi Artemis Voudouri, Emmanouil Proestakis, Maria Mylonaki, Christina-Anna Papanikolaou, Konstantinos Michailidis, Holger Baars, Anne Grete Straume, Dimitris Balis, Alexandros Papayannis, Tomasso Parrinello, and Vassilis Amiridis
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2022-205, https://doi.org/10.5194/amt-2022-205, 2022
Revised manuscript under review for AMT
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We perform an assessment analysis of Aeolus L2A backscatter coefficient retrievals against reference observations acquired at three Greek lidar stations (Athens, Thessaloniki, Antikythera) of the PANACEA network. Overall, 46 cases are analyzed whereas emphasis is given of specific aerosol scenarios in the vicinity of the Antikythera island (SW Greece). All key Cal/Val aspects and recommendations as well as the ongoing related activities are thoroughly discussed.
Kevin Ohneiser, Albert Ansmann, Bernd Kaifler, Alexandra Chudnovsky, Boris Barja, Daniel A. Knopf, Natalie Kaifler, Holger Baars, Patric Seifert, Diego Villanueva, Cristofer Jimenez, Martin Radenz, Ronny Engelmann, Igor Veselovskii, and Félix Zamorano
Atmos. Chem. Phys., 22, 7417–7442, https://doi.org/10.5194/acp-22-7417-2022, https://doi.org/10.5194/acp-22-7417-2022, 2022
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We present and discuss 2 years of long-term lidar observations of the largest stratospheric perturbation by wildfire smoke ever observed. The smoke originated from the record-breaking Australian fires in 2019–2020 and affects climate conditions and even the ozone layer in the Southern Hemisphere. The obvious link between dense smoke occurrence in the stratosphere and strong ozone depletion found in the Arctic and in the Antarctic in 2020 can be regarded as a new aspect of climate change.
Michael Weger, Holger Baars, Henriette Gebauer, Maik Merkel, Alfred Wiedensohler, and Bernd Heinold
Geosci. Model Dev., 15, 3315–3345, https://doi.org/10.5194/gmd-15-3315-2022, https://doi.org/10.5194/gmd-15-3315-2022, 2022
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Numerical models are an important tool to assess the air quality in cities,
as they can provide near-continouos data in time and space. In this paper,
air pollution for an entire city is simulated at a high spatial resolution of 40 m.
At this spatial scale, the effects of buildings on the atmosphere,
like channeling or blocking of the air flow, are directly represented by diffuse obstacles in the used model CAIRDIO. For model validation, measurements from air-monitoring sites are used.
Xiaoxia Shang, Holger Baars, Iwona S. Stachlewska, Ina Mattis, and Mika Komppula
Atmos. Chem. Phys., 22, 3931–3944, https://doi.org/10.5194/acp-22-3931-2022, https://doi.org/10.5194/acp-22-3931-2022, 2022
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This study reports pollen observations at four lidar stations (Hohenpeißenberg, Germany; Kuopio, Finland; Leipzig, Germany; and Warsaw, Poland) during the intensive observation campaign organized in May 2020. A novel simple method for the characterization of the pure pollen is proposed, based on lidar measurements. It was applied to evaluate the pollen depolarization ratio and for the aerosol classifications.
Birgit Heese, Athena Augusta Floutsi, Holger Baars, Dietrich Althausen, Julian Hofer, Alina Herzog, Silke Mewes, Martin Radenz, and Yoav Y. Schechner
Atmos. Chem. Phys., 22, 1633–1648, https://doi.org/10.5194/acp-22-1633-2022, https://doi.org/10.5194/acp-22-1633-2022, 2022
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The aerosol distribution over Haifa, Israel, was measured for 2 years by a laser-based vertically resolved measurement technique called lidar. From these data, the aerosol types and their percentages of the observed aerosol mixtures were identified in terms of their size and shape. We found mostly desert dust from the surrounding deserts and sea salt from the close-by Mediterranean Sea. But aerosols from anthropogenic and industrial pollution from local and far away sources were also detected.
Jerónimo Escribano, Enza Di Tomaso, Oriol Jorba, Martina Klose, Maria Gonçalves Ageitos, Francesca Macchia, Vassilis Amiridis, Holger Baars, Eleni Marinou, Emmanouil Proestakis, Claudia Urbanneck, Dietrich Althausen, Johannes Bühl, Rodanthi-Elisavet Mamouri, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 22, 535–560, https://doi.org/10.5194/acp-22-535-2022, https://doi.org/10.5194/acp-22-535-2022, 2022
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We explore the benefits and consistency in adding lidar dust observations in a dust optical depth assimilation. We show that adding lidar data to a dust optical depth assimilation has valuable benefits and the dust analysis improves. We discuss the impact of the narrow satellite footprint of the lidar dust observations on the assimilation.
Frithjof Ehlers, Thomas Flament, Alain Dabas, Dimitri Trapon, Adrien Lacour, Holger Baars, and Anne Grete Straume-Lindner
Atmos. Meas. Tech., 15, 185–203, https://doi.org/10.5194/amt-15-185-2022, https://doi.org/10.5194/amt-15-185-2022, 2022
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The Aeolus satellite observes the Earth and can vertically detect any kind of particles (aerosols or clouds) in the atmosphere below it. These observations are typically very noisy, which needs to be accounted for. This work dampens the noise in Aeolus' aerosol and cloud data, which are provided publicly by the ESA, so that the scientific community can make better use of it. This makes the data potentially more useful for weather prediction and climate research.
Moritz Haarig, Albert Ansmann, Ronny Engelmann, Holger Baars, Carlos Toledano, Benjamin Torres, Dietrich Althausen, Martin Radenz, and Ulla Wandinger
Atmos. Chem. Phys., 22, 355–369, https://doi.org/10.5194/acp-22-355-2022, https://doi.org/10.5194/acp-22-355-2022, 2022
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The irregular shape of dust particles makes it difficult to treat them correctly in optical models. Atmospheric measurements of dust optical properties are therefore of great importance. The present study increases the space of observed parameters from 355 and 532 nm towards 1064 nm, which is of special importance for large dust particles. The lidar ratio influenced by mineralogy and the depolarization ratio influenced by shape are measured for the first time at all three wavelengths.
Martin Radenz, Johannes Bühl, Patric Seifert, Holger Baars, Ronny Engelmann, Boris Barja González, Rodanthi-Elisabeth Mamouri, Félix Zamorano, and Albert Ansmann
Atmos. Chem. Phys., 21, 17969–17994, https://doi.org/10.5194/acp-21-17969-2021, https://doi.org/10.5194/acp-21-17969-2021, 2021
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This study brings together long-term ground-based remote-sensing observations of mixed-phase clouds at three key locations of aerosol–cloud interactions in the Northern and Southern Hemisphere midlatitudes. The findings contribute several new aspects on the nature of the excess of supercooled liquid clouds in the Southern Hemisphere, such as a long-term lidar-based estimate of ice-nucleating particle profiles as well as the effects of boundary layer coupling and gravity waves on ice formation.
Sebastian Düsing, Albert Ansmann, Holger Baars, Joel C. Corbin, Cyrielle Denjean, Martin Gysel-Beer, Thomas Müller, Laurent Poulain, Holger Siebert, Gerald Spindler, Thomas Tuch, Birgit Wehner, and Alfred Wiedensohler
Atmos. Chem. Phys., 21, 16745–16773, https://doi.org/10.5194/acp-21-16745-2021, https://doi.org/10.5194/acp-21-16745-2021, 2021
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The work deals with optical properties of aerosol particles in dried and atmospheric states. Based on two measurement campaigns in the rural background of central Europe, different measurement approaches were compared with each other, such as modeling based on Mie theory and direct in situ or remote sensing measurements. Among others, it was shown that the aerosol extinction-to-backscatter ratio is relative humidity dependent, and refinement with respect to the model input parameters is needed.
Kevin Ohneiser, Albert Ansmann, Alexandra Chudnovsky, Ronny Engelmann, Christoph Ritter, Igor Veselovskii, Holger Baars, Henriette Gebauer, Hannes Griesche, Martin Radenz, Julian Hofer, Dietrich Althausen, Sandro Dahlke, and Marion Maturilli
Atmos. Chem. Phys., 21, 15783–15808, https://doi.org/10.5194/acp-21-15783-2021, https://doi.org/10.5194/acp-21-15783-2021, 2021
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The highlight of the lidar measurements during the 1-year MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition of the German icebreaker Polarstern (October 2019–October 2020) was the detection of a persistent, 10 km deep Siberian wildfire smoke layer in the upper troposphere and lower stratosphere (UTLS) from about 7–8 km to 17–18 km height that could potentially have impacted the record-breaking ozone depletion over the Arctic in the spring of 2020.
Mariana Adam, Iwona S. Stachlewska, Lucia Mona, Nikolaos Papagiannopoulos, Juan Antonio Bravo-Aranda, Michaël Sicard, Doina N. Nicolae, Livio Belegante, Lucja Janicka, Dominika Szczepanik, Maria Mylonaki, Christina-Anna Papanikolaou, Nikolaos Siomos, Kalliopi Artemis Voudouri, Luca Alados-Arboledas, Arnoud Apituley, Ina Mattis, Anatoli Chaikovsky, Constantino Muñoz-Porcar, Aleksander Pietruczuk, Daniele Bortoli, Holger Baars, Ivan Grigorov, and Zahary Peshev
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-759, https://doi.org/10.5194/acp-2021-759, 2021
Revised manuscript not accepted
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Results over 10 years of biomass burning events measured by EARLINET are analysed by means of the intensive parameters, based on the methodology described in Part I. Smoke type is characterized for each of the four geographical regions based on continental smoke origin. Relationships between intensive parameters or colour ratios are shown. The smoke is labelled in average as aged smoke.
Ronny Engelmann, Albert Ansmann, Kevin Ohneiser, Hannes Griesche, Martin Radenz, Julian Hofer, Dietrich Althausen, Sandro Dahlke, Marion Maturilli, Igor Veselovskii, Cristofer Jimenez, Robert Wiesen, Holger Baars, Johannes Bühl, Henriette Gebauer, Moritz Haarig, Patric Seifert, Ulla Wandinger, and Andreas Macke
Atmos. Chem. Phys., 21, 13397–13423, https://doi.org/10.5194/acp-21-13397-2021, https://doi.org/10.5194/acp-21-13397-2021, 2021
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A Raman lidar was operated aboard the icebreaker Polarstern during MOSAiC and monitored aerosol and cloud layers in the central Arctic up to 30 km height. The article provides an overview of the spectrum of aerosol profiling observations and shows aerosol–cloud interaction studies for liquid-water and ice clouds. A highlight was the detection of a 10 km deep wildfire smoke layer over the North Pole up to 17 km height from the fire season of 2019, which persisted over the whole winter period.
Carmen Córdoba-Jabonero, Albert Ansmann, Cristofer Jiménez, Holger Baars, María-Ángeles López-Cayuela, and Ronny Engelmann
Atmos. Meas. Tech., 14, 5225–5239, https://doi.org/10.5194/amt-14-5225-2021, https://doi.org/10.5194/amt-14-5225-2021, 2021
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An experimental assessment of a polarized micro-pulse lidar (P-MPL) in comparison to reference lidars is presented regarding the retrieval of aerosol optical properties. The evaluation is focused on both the optimally determined overlap function and volume linear depolarization ratio. A P-MPL overlap must be regularly estimated to derive suitable aerosol products (backscatter, extinction, and particle depolarization ratio). This methodology can be easily applied to other P-MPL systems.
Albert Ansmann, Kevin Ohneiser, Rodanthi-Elisavet Mamouri, Daniel A. Knopf, Igor Veselovskii, Holger Baars, Ronny Engelmann, Andreas Foth, Cristofer Jimenez, Patric Seifert, and Boris Barja
Atmos. Chem. Phys., 21, 9779–9807, https://doi.org/10.5194/acp-21-9779-2021, https://doi.org/10.5194/acp-21-9779-2021, 2021
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We present retrievals of tropospheric and stratospheric height profiles of particle mass, volume, surface area concentration of wildfire smoke layers, and related cloud condensation nuclei (CCN) and ice-nucleating particle (INP) concentrations. The new analysis scheme is applied to ground-based lidar observations of stratospheric Australian smoke over southern South America and to spaceborne lidar observations of tropospheric North American smoke.
Maria Kezoudi, Matthias Tesche, Helen Smith, Alexandra Tsekeri, Holger Baars, Maximilian Dollner, Víctor Estellés, Johannes Bühl, Bernadett Weinzierl, Zbigniew Ulanowski, Detlef Müller, and Vassilis Amiridis
Atmos. Chem. Phys., 21, 6781–6797, https://doi.org/10.5194/acp-21-6781-2021, https://doi.org/10.5194/acp-21-6781-2021, 2021
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Mineral dust concentrations in the diameter range from 0.4 to 14.0 μm were measured with the balloon-borne UCASS optical particle counter. Launches were coordinated with ground-based remote-sensing and airborne in situ measurements during a Saharan dust outbreak over Cyprus. Particle number concentrations reached 50 cm−3 for the diameter range 0.8–13.9 μm. Comparisons with aircraft data show reasonable agreement in magnitude and shape of the particle size distribution.
Ville Vakkari, Holger Baars, Stephanie Bohlmann, Johannes Bühl, Mika Komppula, Rodanthi-Elisavet Mamouri, and Ewan James O'Connor
Atmos. Chem. Phys., 21, 5807–5820, https://doi.org/10.5194/acp-21-5807-2021, https://doi.org/10.5194/acp-21-5807-2021, 2021
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The depolarization ratio is a valuable parameter for aerosol categorization from remote sensing measurements. Here, we introduce particle depolarization ratio measurements at the 1565 nm wavelength, which is substantially longer than previously utilized wavelengths and enhances our capabilities to study the wavelength dependency of the particle depolarization ratio.
Martin Radenz, Patric Seifert, Holger Baars, Athena Augusta Floutsi, Zhenping Yin, and Johannes Bühl
Atmos. Chem. Phys., 21, 3015–3033, https://doi.org/10.5194/acp-21-3015-2021, https://doi.org/10.5194/acp-21-3015-2021, 2021
Maria Mylonaki, Elina Giannakaki, Alexandros Papayannis, Christina-Anna Papanikolaou, Mika Komppula, Doina Nicolae, Nikolaos Papagiannopoulos, Aldo Amodeo, Holger Baars, and Ourania Soupiona
Atmos. Chem. Phys., 21, 2211–2227, https://doi.org/10.5194/acp-21-2211-2021, https://doi.org/10.5194/acp-21-2211-2021, 2021
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We introduce an automated aerosol type classification method, SCAN. The output of SCAN is compared with two aerosol classification methods: (1) the Mahalanobis distance automatic aerosol type classification and (2) a neural network aerosol typing algorithm. A total of 97 free tropospheric aerosol layers from four EARLINET stations in the period 2014–2018 were classified.
Anna Gialitaki, Alexandra Tsekeri, Vassilis Amiridis, Romain Ceolato, Lucas Paulien, Anna Kampouri, Antonis Gkikas, Stavros Solomos, Eleni Marinou, Moritz Haarig, Holger Baars, Albert Ansmann, Tatyana Lapyonok, Anton Lopatin, Oleg Dubovik, Silke Groß, Martin Wirth, Maria Tsichla, Ioanna Tsikoudi, and Dimitris Balis
Atmos. Chem. Phys., 20, 14005–14021, https://doi.org/10.5194/acp-20-14005-2020, https://doi.org/10.5194/acp-20-14005-2020, 2020
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Stratospheric smoke particles are found to significantly depolarize incident light, while this effect is also accompanied by a strong spectral dependence. We utilize scattering simulations to show that this behaviour can be attributed to the near-spherical shape of the particles. We also examine whether an extension of the current AERONET scattering model to include the near-spherical shapes could be of benefit to the AERONET retrieval for stratospheric smoke associated with enhanced PLDR.
Holger Baars, Alina Herzog, Birgit Heese, Kevin Ohneiser, Karsten Hanbuch, Julian Hofer, Zhenping Yin, Ronny Engelmann, and Ulla Wandinger
Atmos. Meas. Tech., 13, 6007–6024, https://doi.org/10.5194/amt-13-6007-2020, https://doi.org/10.5194/amt-13-6007-2020, 2020
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A first validation for the European satellite Aeolus is presented. Aeolus is the first satellite that can actively measure horizontal wind profiles from space.
Radiosonde launches on board the German research vessel Polarstern have been utilized to validate Aeolus observations over the Atlantic Ocean, a region where almost no other reference measurements are available. It is shown that Aeolus is able to measure accurately atmospheric winds and thus may significantly improve weather forecasts.
Hannes J. Griesche, Patric Seifert, Albert Ansmann, Holger Baars, Carola Barrientos Velasco, Johannes Bühl, Ronny Engelmann, Martin Radenz, Yin Zhenping, and Andreas Macke
Atmos. Meas. Tech., 13, 5335–5358, https://doi.org/10.5194/amt-13-5335-2020, https://doi.org/10.5194/amt-13-5335-2020, 2020
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In summer 2017, the research vessel Polarstern performed cruise PS106 to the Arctic north of Svalbard. In the frame of the cruise, remote-sensing observations of the atmosphere were performed on Polarstern to continuously monitor aerosol and clouds above the vessel. In our study, we present the deployed instrumentation and applied data analysis methods and provide case studies of the aerosol and cloud observations made during the cruise. Statistics of low-cloud occurrence are presented as well.
Nikolaos Papagiannopoulos, Giuseppe D'Amico, Anna Gialitaki, Nicolae Ajtai, Lucas Alados-Arboledas, Aldo Amodeo, Vassilis Amiridis, Holger Baars, Dimitris Balis, Ioannis Binietoglou, Adolfo Comerón, Davide Dionisi, Alfredo Falconieri, Patrick Fréville, Anna Kampouri, Ina Mattis, Zoran Mijić, Francisco Molero, Alex Papayannis, Gelsomina Pappalardo, Alejandro Rodríguez-Gómez, Stavros Solomos, and Lucia Mona
Atmos. Chem. Phys., 20, 10775–10789, https://doi.org/10.5194/acp-20-10775-2020, https://doi.org/10.5194/acp-20-10775-2020, 2020
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Volcanic and desert dust particles affect human activities in manifold ways; consequently, mitigation tools are important. Their early detection and the issuance of early warnings are key elements in the initiation of operational response procedures. A methodology for the early warning of these hazards using European Aerosol Research Lidar Network (EARLINET) data is presented. The tailored product is investigated during a volcanic eruption and mineral dust advected in the eastern Mediterranean.
Julian Hofer, Albert Ansmann, Dietrich Althausen, Ronny Engelmann, Holger Baars, Khanneh Wadinga Fomba, Ulla Wandinger, Sabur F. Abdullaev, and Abduvosit N. Makhmudov
Atmos. Chem. Phys., 20, 9265–9280, https://doi.org/10.5194/acp-20-9265-2020, https://doi.org/10.5194/acp-20-9265-2020, 2020
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For the first time, a dense data set of particle extinction-to-backscatter ratios (lidar ratios), depolarization ratios, and backscatter- and extinction-related Ångström exponents for a Central Asian site are presented. The observations were performed with a continuously running multiwavelength polarization Raman lidar at Dushanbe, Tajikistan, during an 18-month campaign. The found optical properties reflect the large range of occurring aerosol mixtures.
Mariana Adam, Doina Nicolae, Livio Belegante, Iwona S. Stachlewska, Lucja Janicka, Dominika Szczepanik, Maria Mylonaki, Christiana Anna Papanikolaou, Nikos Siomos, Kalliopi Artemis Voudouri, Luca Alados-Arboledas, Juan Antonio Bravo-Aranda, Arnoud Apituley, Nikolaos Papagiannopoulos, Lucia Mona, Ina Mattis, Anatoli Chaikovsky, Michaël Sicard, Constantino Muñoz-Porcar, Aleksander Pietruczuk, Daniele Bortoli, Holger Baars, Ivan Grigorov, and Zahary Peshev
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-647, https://doi.org/10.5194/acp-2020-647, 2020
Revised manuscript not accepted
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Results over 10 years of biomass burning events measured by EARLINET are analysed by means of the intensive parameters based on the methodology described in Part I. Smoke type is characterized for each of the four geographical regions based on continental smoke origin. Relationships between intensive parameters or colour ratios are shown. The smoke is labelled in average as aged smoke. The local smoke has a smaller lidar ratio while the depolarization is smaller for long range transported smoke.
Christa Genz, Roland Schrödner, Bernd Heinold, Silvia Henning, Holger Baars, Gerald Spindler, and Ina Tegen
Atmos. Chem. Phys., 20, 8787–8806, https://doi.org/10.5194/acp-20-8787-2020, https://doi.org/10.5194/acp-20-8787-2020, 2020
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Atmospheric aerosols are the precondition for the formation of cloud droplets and thus have a large influence on cloud properties. Concentrations of cloud condensation nuclei of the period with highest aerosol concentrations over central Europe are uncertain. In this work, modeled estimates of CCN from today and the mid-1980s are compared to available in situ and remote sensing observations. A scaling factor between today and the 1980s for the CCN concentrations has been derived.
Kevin Ohneiser, Albert Ansmann, Holger Baars, Patric Seifert, Boris Barja, Cristofer Jimenez, Martin Radenz, Audrey Teisseire, Athina Floutsi, Moritz Haarig, Andreas Foth, Alexandra Chudnovsky, Ronny Engelmann, Félix Zamorano, Johannes Bühl, and Ulla Wandinger
Atmos. Chem. Phys., 20, 8003–8015, https://doi.org/10.5194/acp-20-8003-2020, https://doi.org/10.5194/acp-20-8003-2020, 2020
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Unique lidar observations of a strong perturbation in stratospheric aerosol conditions in the Southern Hemisphere caused by the extreme Australian bushfires in 2019–2020 are presented. One of the main goals of this article is to provide the CALIPSO and Aeolus spaceborne lidar science teams with basic input parameters (lidar ratios, depolarization ratios) for a trustworthy documentation of this record-breaking event.
Athena Augusta Floutsi, Holger Baars, Martin Radenz, Moritz Haarig, Zhenping Yin, Patric Seifert, Cristofer Jimenez, Ulla Wandinger, Ronny Engelmann, Boris Barja, Felix Zamorano, and Albert Ansmann
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-453, https://doi.org/10.5194/acp-2020-453, 2020
Preprint withdrawn
Montserrat Costa-Surós, Odran Sourdeval, Claudia Acquistapace, Holger Baars, Cintia Carbajal Henken, Christa Genz, Jonas Hesemann, Cristofer Jimenez, Marcel König, Jan Kretzschmar, Nils Madenach, Catrin I. Meyer, Roland Schrödner, Patric Seifert, Fabian Senf, Matthias Brueck, Guido Cioni, Jan Frederik Engels, Kerstin Fieg, Ksenia Gorges, Rieke Heinze, Pavan Kumar Siligam, Ulrike Burkhardt, Susanne Crewell, Corinna Hoose, Axel Seifert, Ina Tegen, and Johannes Quaas
Atmos. Chem. Phys., 20, 5657–5678, https://doi.org/10.5194/acp-20-5657-2020, https://doi.org/10.5194/acp-20-5657-2020, 2020
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The impact of anthropogenic aerosols on clouds is a key uncertainty in climate change. This study analyses large-domain simulations with a new high-resolution model to investigate the differences in clouds between 1985 and 2013 comparing multiple observational datasets. The differences in aerosol and in cloud droplet concentrations are clearly detectable. For other quantities, the detection and attribution proved difficult, despite a substantial impact on the Earth's energy budget.
Julian Hofer, Albert Ansmann, Dietrich Althausen, Ronny Engelmann, Holger Baars, Sabur F. Abdullaev, and Abduvosit N. Makhmudov
Atmos. Chem. Phys., 20, 4695–4711, https://doi.org/10.5194/acp-20-4695-2020, https://doi.org/10.5194/acp-20-4695-2020, 2020
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For the first time, continuous, vertically resolved long-term aerosol measurements were conducted with a state-of-the-art multiwavelength lidar over a Central Asian site. Such observations are urgently required in efforts to predict future climate and environmental conditions and to support spaceborne remote sensing (ground truth activities).
Johannes Bühl, Patric Seifert, Martin Radenz, Holger Baars, and Albert Ansmann
Atmos. Meas. Tech., 12, 6601–6617, https://doi.org/10.5194/amt-12-6601-2019, https://doi.org/10.5194/amt-12-6601-2019, 2019
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In the present paper, we present a novel remote-sensing technique for the measurement of ice crystal number concentrations in clouds. The fall velocity of ice crystals measured with values from cloud radar and a radar wind profiler is used in order to derive information about ice crystal size and number concentration. In contrast to existing methods based on the combination of lidar and cloud radar, the present method can also be used in optically thick clouds.
Holger Baars, Albert Ansmann, Kevin Ohneiser, Moritz Haarig, Ronny Engelmann, Dietrich Althausen, Ingrid Hanssen, Michael Gausa, Aleksander Pietruczuk, Artur Szkop, Iwona S. Stachlewska, Dongxiang Wang, Jens Reichardt, Annett Skupin, Ina Mattis, Thomas Trickl, Hannes Vogelmann, Francisco Navas-Guzmán, Alexander Haefele, Karen Acheson, Albert A. Ruth, Boyan Tatarov, Detlef Müller, Qiaoyun Hu, Thierry Podvin, Philippe Goloub, Igor Veselovskii, Christophe Pietras, Martial Haeffelin, Patrick Fréville, Michaël Sicard, Adolfo Comerón, Alfonso Javier Fernández García, Francisco Molero Menéndez, Carmen Córdoba-Jabonero, Juan Luis Guerrero-Rascado, Lucas Alados-Arboledas, Daniele Bortoli, Maria João Costa, Davide Dionisi, Gian Luigi Liberti, Xuan Wang, Alessia Sannino, Nikolaos Papagiannopoulos, Antonella Boselli, Lucia Mona, Giuseppe D'Amico, Salvatore Romano, Maria Rita Perrone, Livio Belegante, Doina Nicolae, Ivan Grigorov, Anna Gialitaki, Vassilis Amiridis, Ourania Soupiona, Alexandros Papayannis, Rodanthi-Elisaveth Mamouri, Argyro Nisantzi, Birgit Heese, Julian Hofer, Yoav Y. Schechner, Ulla Wandinger, and Gelsomina Pappalardo
Atmos. Chem. Phys., 19, 15183–15198, https://doi.org/10.5194/acp-19-15183-2019, https://doi.org/10.5194/acp-19-15183-2019, 2019
Rebecca M. Pauly, John E. Yorks, Dennis L. Hlavka, Matthew J. McGill, Vassilis Amiridis, Stephen P. Palm, Sharon D. Rodier, Mark A. Vaughan, Patrick A. Selmer, Andrew W. Kupchock, Holger Baars, and Anna Gialitaki
Atmos. Meas. Tech., 12, 6241–6258, https://doi.org/10.5194/amt-12-6241-2019, https://doi.org/10.5194/amt-12-6241-2019, 2019
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The Cloud Aerosol Transport System (CATS) demonstrated that direct calibration of 1064 nm lidar data from a spaceborne platform is possible. By normalizing the CATS signal to a modeled molecular backscatter profile the CATS data were calibrated, enabling the derivation of optical properties of clouds and aerosols. Comparisons of the calibrated signal with airborne lidar, ground-based lidar, and spaceborne lidar all show agreement within the estimated error bars of the respective instruments.
Zhenping Yin, Albert Ansmann, Holger Baars, Patric Seifert, Ronny Engelmann, Martin Radenz, Cristofer Jimenez, Alina Herzog, Kevin Ohneiser, Karsten Hanbuch, Luc Blarel, Philippe Goloub, Gaël Dubois, Stephane Victori, and Fabrice Maupin
Atmos. Meas. Tech., 12, 5685–5698, https://doi.org/10.5194/amt-12-5685-2019, https://doi.org/10.5194/amt-12-5685-2019, 2019
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A new shipborne Sun–sky–lunar photometer was validated through comparisons with collocated MICROTOPS II and multiwavelength Raman polarization lidar measurements during two trans-Atlantic cruises. A full diurnal cycle of mixed dust–smoke episode was captured by both the shipborne photometer and lidar. The coefficient of determination for the linear regression between MICROTOPS II and the shipborne photometer was 0.993 for AOD at 500 nm based on the entire dataset.
Emmanouil Proestakis, Vassilis Amiridis, Eleni Marinou, Ioannis Binietoglou, Albert Ansmann, Ulla Wandinger, Julian Hofer, John Yorks, Edward Nowottnick, Abduvosit Makhmudov, Alexandros Papayannis, Aleksander Pietruczuk, Anna Gialitaki, Arnoud Apituley, Artur Szkop, Constantino Muñoz Porcar, Daniele Bortoli, Davide Dionisi, Dietrich Althausen, Dimitra Mamali, Dimitris Balis, Doina Nicolae, Eleni Tetoni, Gian Luigi Liberti, Holger Baars, Ina Mattis, Iwona Sylwia Stachlewska, Kalliopi Artemis Voudouri, Lucia Mona, Maria Mylonaki, Maria Rita Perrone, Maria João Costa, Michael Sicard, Nikolaos Papagiannopoulos, Nikolaos Siomos, Pasquale Burlizzi, Rebecca Pauly, Ronny Engelmann, Sabur Abdullaev, and Gelsomina Pappalardo
Atmos. Chem. Phys., 19, 11743–11764, https://doi.org/10.5194/acp-19-11743-2019, https://doi.org/10.5194/acp-19-11743-2019, 2019
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To increase accuracy and validate satellite-based products, comparison with ground-based reference observations is required. To do this, we present evaluation activity of EARLINET for the qualitative and quantitative assessment of NASA's CATS lidar operating aboard the International Space Station (ISS) while identified discrepancies are discussed. Better understanding CATS performance and limitations provides a valuable basis for scientific studies implementing the satellite-based lidar system.
Albert Ansmann, Rodanthi-Elisavet Mamouri, Julian Hofer, Holger Baars, Dietrich Althausen, and Sabur F. Abdullaev
Atmos. Meas. Tech., 12, 4849–4865, https://doi.org/10.5194/amt-12-4849-2019, https://doi.org/10.5194/amt-12-4849-2019, 2019
Eleni Marinou, Matthias Tesche, Athanasios Nenes, Albert Ansmann, Jann Schrod, Dimitra Mamali, Alexandra Tsekeri, Michael Pikridas, Holger Baars, Ronny Engelmann, Kalliopi-Artemis Voudouri, Stavros Solomos, Jean Sciare, Silke Groß, Florian Ewald, and Vassilis Amiridis
Atmos. Chem. Phys., 19, 11315–11342, https://doi.org/10.5194/acp-19-11315-2019, https://doi.org/10.5194/acp-19-11315-2019, 2019
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We assess the feasibility of ground-based and spaceborne lidars to retrieve profiles of cloud-relevant aerosol concentrations and ice-nucleating particles. The retrieved profiles are in good agreement with airborne in situ measurements. Our methodology will be applied to satellite observations in the future so as to provide a global 3D product of cloud-relevant properties.
Andreas Foth, Thomas Kanitz, Ronny Engelmann, Holger Baars, Martin Radenz, Patric Seifert, Boris Barja, Michael Fromm, Heike Kalesse, and Albert Ansmann
Atmos. Chem. Phys., 19, 6217–6233, https://doi.org/10.5194/acp-19-6217-2019, https://doi.org/10.5194/acp-19-6217-2019, 2019
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In this study, we present the vertical aerosol distribution in the pristine region of the southern tip of South America determined by ground-based and spaceborne lidar observations. Most aerosol load is contained within the planetary boundary layer up to about 1200 m. The free troposphere is characterized by a very low aerosol concentration but a frequent occurrence of clouds. Lofted aerosol layers were rarely observed and, when present, were characterized by very low optical thicknesses.
Michael Weger, Bernd Heinold, Christa Engler, Ulrich Schumann, Axel Seifert, Romy Fößig, Christiane Voigt, Holger Baars, Ulrich Blahak, Stephan Borrmann, Corinna Hoose, Stefan Kaufmann, Martina Krämer, Patric Seifert, Fabian Senf, Johannes Schneider, and Ina Tegen
Atmos. Chem. Phys., 18, 17545–17572, https://doi.org/10.5194/acp-18-17545-2018, https://doi.org/10.5194/acp-18-17545-2018, 2018
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The impact of desert dust on cloud formation is investigated for a major Saharan dust event over Europe by interactive regional dust modeling. Dust particles are very efficient ice-nucleating particles promoting the formation of ice crystals in clouds. The simulations show that the observed extensive cirrus development was likely related to the above-average dust load. The interactive dust–cloud feedback in the model significantly improves the agreement with aircraft and satellite observations.
Nikolaos Papagiannopoulos, Lucia Mona, Aldo Amodeo, Giuseppe D'Amico, Pilar Gumà Claramunt, Gelsomina Pappalardo, Lucas Alados-Arboledas, Juan Luís Guerrero-Rascado, Vassilis Amiridis, Panagiotis Kokkalis, Arnoud Apituley, Holger Baars, Anja Schwarz, Ulla Wandinger, Ioannis Binietoglou, Doina Nicolae, Daniele Bortoli, Adolfo Comerón, Alejandro Rodríguez-Gómez, Michaël Sicard, Alex Papayannis, and Matthias Wiegner
Atmos. Chem. Phys., 18, 15879–15901, https://doi.org/10.5194/acp-18-15879-2018, https://doi.org/10.5194/acp-18-15879-2018, 2018
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A stand-alone automatic method for typing observations of the European Aerosol Research Lidar Network (EARLINET) is presented. The method compares the observations to model distributions that were constructed using EARLINET pre-classified data. The algorithm’s versatility and adaptability makes it suitable for network-wide typing studies.
Albert Ansmann, Holger Baars, Alexandra Chudnovsky, Ina Mattis, Igor Veselovskii, Moritz Haarig, Patric Seifert, Ronny Engelmann, and Ulla Wandinger
Atmos. Chem. Phys., 18, 11831–11845, https://doi.org/10.5194/acp-18-11831-2018, https://doi.org/10.5194/acp-18-11831-2018, 2018
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Extremely large light extinction coefficients of 500 Mm-1, about 20 times higher than after the Pinatubo volcanic eruptions in 1991, were observed by EARLINET lidars in the stratosphere over central Europe from 21 to 22 August, 2017. This paper provides an overview based on ground-based (lidar, AERONET) and satellite (MODIS, OMI) remote sensing.
Moritz Haarig, Albert Ansmann, Holger Baars, Cristofer Jimenez, Igor Veselovskii, Ronny Engelmann, and Dietrich Althausen
Atmos. Chem. Phys., 18, 11847–11861, https://doi.org/10.5194/acp-18-11847-2018, https://doi.org/10.5194/acp-18-11847-2018, 2018
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The worldwide only triple-wavelength polarization/Raman lidar was used to measure optical, microphysical, and morphological properties of aged Canadian wildfire smoke occurring in the troposphere and stratosphere over Leipzig, Germany, in August 2017. A strong contrast between the tropospheric and stratospheric smoke properties was found.
Carmen Córdoba-Jabonero, Michaël Sicard, Albert Ansmann, Ana del Águila, and Holger Baars
Atmos. Meas. Tech., 11, 4775–4795, https://doi.org/10.5194/amt-11-4775-2018, https://doi.org/10.5194/amt-11-4775-2018, 2018
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The high potential of the MPLNET polarized Micro-Pulse LiDAR (P-MPL) is demonstrated in synergy with the POLIPHON (POlarization-LIdar PHOtometer Networking) method to retrieve the vertical separation of both the optical and mass features of the dust, smoke and pollen components mixed with other aerosols. This synergetic procedure can be easily applied to the worldwide MPLNET lidar systems and to space-borne lidars: the ongoing NASA CALIPSO/CALIOP and the forthcoming ESA EarthCARE/ATLID.
Daniel Moran-Zuloaga, Florian Ditas, David Walter, Jorge Saturno, Joel Brito, Samara Carbone, Xuguang Chi, Isabella Hrabě de Angelis, Holger Baars, Ricardo H. M. Godoi, Birgit Heese, Bruna A. Holanda, Jošt V. Lavrič, Scot T. Martin, Jing Ming, Mira L. Pöhlker, Nina Ruckteschler, Hang Su, Yaqiang Wang, Qiaoqiao Wang, Zhibin Wang, Bettina Weber, Stefan Wolff, Paulo Artaxo, Ulrich Pöschl, Meinrat O. Andreae, and Christopher Pöhlker
Atmos. Chem. Phys., 18, 10055–10088, https://doi.org/10.5194/acp-18-10055-2018, https://doi.org/10.5194/acp-18-10055-2018, 2018
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This study presents multiple years of aerosol coarse mode observations at the remote ATTO site in the Amazon Basin. The results are discussed in light of the frequent and episodic long-range transport of Saharan dust plumes in the early wet season as well as the persistent background bioaerosol cycling in the rain forest ecosystem. This work provides a solid basis for future studies on the dynamic coarse mode aerosol cycling and its biogeochemical relevance in the Amazon.
Stephanie Bohlmann, Holger Baars, Martin Radenz, Ronny Engelmann, and Andreas Macke
Atmos. Chem. Phys., 18, 9661–9679, https://doi.org/10.5194/acp-18-9661-2018, https://doi.org/10.5194/acp-18-9661-2018, 2018
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Lidar measurements of two expeditions across the Atlantic Ocean aboard the research vessel Polarstern are presented. In addition to Saharan dust layers and complex dust–smoke mixtures, pure marine conditions with enhanced particle depolarisation ratios on top of the marine boundary layer could be observed. A statistical analysis shows latitudinal differences in the optical properties within the marine boundary layer and illustrates the potential of these properties for aerosol classification.
Barbara Altstädter, Andreas Platis, Michael Jähn, Holger Baars, Janine Lückerath, Andreas Held, Astrid Lampert, Jens Bange, Markus Hermann, and Birgit Wehner
Atmos. Chem. Phys., 18, 8249–8264, https://doi.org/10.5194/acp-18-8249-2018, https://doi.org/10.5194/acp-18-8249-2018, 2018
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This article describes the appearance of ultrafine aerosol particles (size < 12 nm) within the atmospheric boundary layer under cloudy conditions. New particle formation (NPF) was observed with the ALADINA unmanned aerial system in relation to increased turbulence near the inversion layer. Fast mixing processes and rapid dilution of surrounding air led to an insufficient particle growth rate, seen in sporadic clusters at ground. These events might not have been classified as NPF by surface data.
Dimitra Mamali, Eleni Marinou, Jean Sciare, Michael Pikridas, Panagiotis Kokkalis, Michael Kottas, Ioannis Binietoglou, Alexandra Tsekeri, Christos Keleshis, Ronny Engelmann, Holger Baars, Albert Ansmann, Vassilis Amiridis, Herman Russchenberg, and George Biskos
Atmos. Meas. Tech., 11, 2897–2910, https://doi.org/10.5194/amt-11-2897-2018, https://doi.org/10.5194/amt-11-2897-2018, 2018
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The paper's scope is to evaluate the performance of in situ atmospheric aerosol instrumentation on board unmanned aerial vehicles (UAVs) and the performance of algorithms used to calculate the aerosol mass from remote sensing instruments by comparing the two independent techniques to each other. Our results indicate that UAV-based aerosol measurements (using specific in situ and remote sensing instrumentation) can provide reliable ways to determine the aerosol mass throughout the atmosphere.
Livio Belegante, Juan Antonio Bravo-Aranda, Volker Freudenthaler, Doina Nicolae, Anca Nemuc, Dragos Ene, Lucas Alados-Arboledas, Aldo Amodeo, Gelsomina Pappalardo, Giuseppe D'Amico, Francesco Amato, Ronny Engelmann, Holger Baars, Ulla Wandinger, Alexandros Papayannis, Panos Kokkalis, and Sérgio N. Pereira
Atmos. Meas. Tech., 11, 1119–1141, https://doi.org/10.5194/amt-11-1119-2018, https://doi.org/10.5194/amt-11-1119-2018, 2018
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This paper presents different depolarization calibration procedures used to improve the quality of the depolarization data. The results illustrate a significant improvement of the depolarization lidar products for all the selected EARLINET lidar instruments. The calibrated volume and particle depolarization profiles at 532 nm show values that fall within a range that is accepted in the literature. The depolarization accuracy estimate at 532 nm is better than ±0.03 for all cases.
Sebastian Düsing, Birgit Wehner, Patric Seifert, Albert Ansmann, Holger Baars, Florian Ditas, Silvia Henning, Nan Ma, Laurent Poulain, Holger Siebert, Alfred Wiedensohler, and Andreas Macke
Atmos. Chem. Phys., 18, 1263–1290, https://doi.org/10.5194/acp-18-1263-2018, https://doi.org/10.5194/acp-18-1263-2018, 2018
Alexandra Tsekeri, Anton Lopatin, Vassilis Amiridis, Eleni Marinou, Julia Igloffstein, Nikolaos Siomos, Stavros Solomos, Panagiotis Kokkalis, Ronny Engelmann, Holger Baars, Myrto Gratsea, Panagiotis I. Raptis, Ioannis Binietoglou, Nikolaos Mihalopoulos, Nikolaos Kalivitis, Giorgos Kouvarakis, Nikolaos Bartsotas, George Kallos, Sara Basart, Dirk Schuettemeyer, Ulla Wandinger, Albert Ansmann, Anatoli P. Chaikovsky, and Oleg Dubovik
Atmos. Meas. Tech., 10, 4995–5016, https://doi.org/10.5194/amt-10-4995-2017, https://doi.org/10.5194/amt-10-4995-2017, 2017
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The Generalized Aerosol Retrieval from Radiometer and Lidar Combined data algorithm (GARRLiC) and the LIdar-Radiometer Inversion Code (LIRIC) provide the opportunity to study the aerosol vertical distribution by combining ground-based lidar and sun-photometric measurements. Here, we utilize the capabilities of both algorithms for the characterization of Saharan dust and marine particles, along with their mixtures, in the south-eastern Mediterranean.
Albert Ansmann, Franziska Rittmeister, Ronny Engelmann, Sara Basart, Oriol Jorba, Christos Spyrou, Samuel Remy, Annett Skupin, Holger Baars, Patric Seifert, Fabian Senf, and Thomas Kanitz
Atmos. Chem. Phys., 17, 14987–15006, https://doi.org/10.5194/acp-17-14987-2017, https://doi.org/10.5194/acp-17-14987-2017, 2017
Julian Hofer, Dietrich Althausen, Sabur F. Abdullaev, Abduvosit N. Makhmudov, Bakhron I. Nazarov, Georg Schettler, Ronny Engelmann, Holger Baars, K. Wadinga Fomba, Konrad Müller, Bernd Heinold, Konrad Kandler, and Albert Ansmann
Atmos. Chem. Phys., 17, 14559–14577, https://doi.org/10.5194/acp-17-14559-2017, https://doi.org/10.5194/acp-17-14559-2017, 2017
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The Central Asian Dust Experiment provides unprecedented data on vertically resolved aerosol optical properties over Central Asia from continuous 18-month polarization Raman lidar observations in Dushanbe, Tajikistan. Central Asia is affected by climate change (e.g. glacier retreat) but in a large part missing vertically resolved aerosol measurements, which would help to better understand transport of dust and pollution aerosol across Central Asia and their influence on climate and health.
Moritz Haarig, Albert Ansmann, Josef Gasteiger, Konrad Kandler, Dietrich Althausen, Holger Baars, Martin Radenz, and David A. Farrell
Atmos. Chem. Phys., 17, 14199–14217, https://doi.org/10.5194/acp-17-14199-2017, https://doi.org/10.5194/acp-17-14199-2017, 2017
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The depolarization ratio and the backscatter coefficient of marine particles are correlated with the relative humidity. The measurements were performed under atmospheric conditions with a multi-wavelength lidar system in pure marine conditions over Barbados in February 2014. For RH < 50 % the sea salt particles have a cubic-like shape resulting in an enhanced depolarization ratio of up to 0.15. This agrees with model results of cubic sea salt. The extinction enhancement f(RH) factor was derived.
Maria Filioglou, Anna Nikandrova, Sami Niemelä, Holger Baars, Tero Mielonen, Ari Leskinen, David Brus, Sami Romakkaniemi, Elina Giannakaki, and Mika Komppula
Atmos. Meas. Tech., 10, 4303–4316, https://doi.org/10.5194/amt-10-4303-2017, https://doi.org/10.5194/amt-10-4303-2017, 2017
Franziska Rittmeister, Albert Ansmann, Ronny Engelmann, Annett Skupin, Holger Baars, Thomas Kanitz, and Stefan Kinne
Atmos. Chem. Phys., 17, 12963–12983, https://doi.org/10.5194/acp-17-12963-2017, https://doi.org/10.5194/acp-17-12963-2017, 2017
Moritz Haarig, Albert Ansmann, Dietrich Althausen, André Klepel, Silke Groß, Volker Freudenthaler, Carlos Toledano, Rodanthi-Elisavet Mamouri, David A. Farrell, Damien A. Prescod, Eleni Marinou, Sharon P. Burton, Josef Gasteiger, Ronny Engelmann, and Holger Baars
Atmos. Chem. Phys., 17, 10767–10794, https://doi.org/10.5194/acp-17-10767-2017, https://doi.org/10.5194/acp-17-10767-2017, 2017
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Our measurements performed with a lidar on Barbados give a vertical profile of Saharan dust, which was transported over 5000 km across the Atlantic. The new triple-wavelength depolarization technique reveals more information about the shape and size of dust, which will improve our understanding of the aging process of dust in the atmosphere and its representation in dust models. Changing properties of dust particles influence the solar radiation and the cloud properties and thus our climate.
Holger Baars, Patric Seifert, Ronny Engelmann, and Ulla Wandinger
Atmos. Meas. Tech., 10, 3175–3201, https://doi.org/10.5194/amt-10-3175-2017, https://doi.org/10.5194/amt-10-3175-2017, 2017
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A novel technique for multiwavelength lidars is introduced to derive information on the particle type in the tropospheric profile in analogy to the Cloudnet target classification. Four different aerosol classes and several cloud classes are defined. The technique is based on absolute calibrated lidar signals in temporally high resolution and thus is also well suited for aerosol–cloud-interaction studies. The approach was applied on a 2-month data set of the HOPE campaign in western Germany.
Pablo Ortiz-Amezcua, Juan Luis Guerrero-Rascado, María José Granados-Muñoz, José Antonio Benavent-Oltra, Christine Böckmann, Stefanos Samaras, Iwona S. Stachlewska, Łucja Janicka, Holger Baars, Stephanie Bohlmann, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 17, 5931–5946, https://doi.org/10.5194/acp-17-5931-2017, https://doi.org/10.5194/acp-17-5931-2017, 2017
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Strong events of biomass burning aerosol transported from North American forest fires were detected during July 2013 at three European stations from EARLINET. Satellite observations and models were used to estimate the smoke sources and transport paths. Using lidar techniques and regularization algorithms, the aerosol layers were optically and microphysically characterized, finding some common features among the events, concerning the similar aging processes undergone by the particles.
Andreas Macke, Patric Seifert, Holger Baars, Christian Barthlott, Christoph Beekmans, Andreas Behrendt, Birger Bohn, Matthias Brueck, Johannes Bühl, Susanne Crewell, Thomas Damian, Hartwig Deneke, Sebastian Düsing, Andreas Foth, Paolo Di Girolamo, Eva Hammann, Rieke Heinze, Anne Hirsikko, John Kalisch, Norbert Kalthoff, Stefan Kinne, Martin Kohler, Ulrich Löhnert, Bomidi Lakshmi Madhavan, Vera Maurer, Shravan Kumar Muppa, Jan Schween, Ilya Serikov, Holger Siebert, Clemens Simmer, Florian Späth, Sandra Steinke, Katja Träumner, Silke Trömel, Birgit Wehner, Andreas Wieser, Volker Wulfmeyer, and Xinxin Xie
Atmos. Chem. Phys., 17, 4887–4914, https://doi.org/10.5194/acp-17-4887-2017, https://doi.org/10.5194/acp-17-4887-2017, 2017
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This article provides an overview of the instrumental setup and the main results obtained during the two HD(CP)2 Observational Prototype Experiments HOPE-Jülich and HOPE-Melpitz conducted in Germany in April–May and Sept 2013, respectively. Goal of the field experiments was to provide high-resolution observational datasets for both, improving the understaning of boundary layer and cloud processes, as well as for the evaluation of the new ICON model that is run at 156 m horizontal resolution.
Jann Schrod, Daniel Weber, Jaqueline Drücke, Christos Keleshis, Michael Pikridas, Martin Ebert, Bojan Cvetković, Slobodan Nickovic, Eleni Marinou, Holger Baars, Albert Ansmann, Mihalis Vrekoussis, Nikos Mihalopoulos, Jean Sciare, Joachim Curtius, and Heinz G. Bingemer
Atmos. Chem. Phys., 17, 4817–4835, https://doi.org/10.5194/acp-17-4817-2017, https://doi.org/10.5194/acp-17-4817-2017, 2017
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In this paper we present data of ice-nucleating particles (INPs) from a 1-month campaign in the Eastern Mediterranean using unmanned aircraft systems (UASs, drones) and offline sampling with subsequent laboratory analysis. To our knowledge, this is the first time INPs were measured onboard a UAS. We find that INP concentrations were 1 magnitude higher aloft than at the ground, highlighting that surface-based measurement of INP may only be of limited significance for the situation at cloud level.
Diego A. Gouveia, Boris Barja, Henrique M. J. Barbosa, Patric Seifert, Holger Baars, Theotonio Pauliquevis, and Paulo Artaxo
Atmos. Chem. Phys., 17, 3619–3636, https://doi.org/10.5194/acp-17-3619-2017, https://doi.org/10.5194/acp-17-3619-2017, 2017
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We derive the first comprehensive statistics of cirrus clouds over a tropical rain forest. Monthly frequency of occurrence can be as high as 88 %. The diurnal cycle follows that of precipitation, and frequently cirrus is found in the tropopause layer. The mean values of cloud top, base, thickness, optical depth and lidar ratio were 14.3 km, 12.9 km, 1.4 km, 0.25, and 23 sr respectively. The high fraction (42 %) of subvisible clouds may contaminate satellite measurements to an unknown extent.
Ina Mattis, Giuseppe D'Amico, Holger Baars, Aldo Amodeo, Fabio Madonna, and Marco Iarlori
Atmos. Meas. Tech., 9, 3009–3029, https://doi.org/10.5194/amt-9-3009-2016, https://doi.org/10.5194/amt-9-3009-2016, 2016
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We present an automated software tool for the retrieval of profiles of optical particle properties from lidar signals. This tool is one of the modules of the Single Calculus Chain of the European Aerosol Research Lidar Network (EARLINET). It allows for the analysis of the data of many different lidar systems of EARLINET in an automated, unsupervised way.
Ronny Engelmann, Thomas Kanitz, Holger Baars, Birgit Heese, Dietrich Althausen, Annett Skupin, Ulla Wandinger, Mika Komppula, Iwona S. Stachlewska, Vassilis Amiridis, Eleni Marinou, Ina Mattis, Holger Linné, and Albert Ansmann
Atmos. Meas. Tech., 9, 1767–1784, https://doi.org/10.5194/amt-9-1767-2016, https://doi.org/10.5194/amt-9-1767-2016, 2016
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The atmospheric science community demands for autonomous and quality-assured vertically resolved measurements of aerosol and cloud properties. For this purpose, a portable lidar called Polly
was developed at TROPOS in 2003. This lidar type was continuously improved with gained experience from EARLINET, worldwide field campaigns, and institute collaborations within the last 10 years. We present recent changes to the setup of our portable multiwavelength Raman and polarization lidar PollyXT.
Holger Baars, Thomas Kanitz, Ronny Engelmann, Dietrich Althausen, Birgit Heese, Mika Komppula, Jana Preißler, Matthias Tesche, Albert Ansmann, Ulla Wandinger, Jae-Hyun Lim, Joon Young Ahn, Iwona S. Stachlewska, Vassilis Amiridis, Eleni Marinou, Patric Seifert, Julian Hofer, Annett Skupin, Florian Schneider, Stephanie Bohlmann, Andreas Foth, Sebastian Bley, Anne Pfüller, Eleni Giannakaki, Heikki Lihavainen, Yrjö Viisanen, Rakesh Kumar Hooda, Sérgio Nepomuceno Pereira, Daniele Bortoli, Frank Wagner, Ina Mattis, Lucja Janicka, Krzysztof M. Markowicz, Peggy Achtert, Paulo Artaxo, Theotonio Pauliquevis, Rodrigo A. F. Souza, Ved Prakesh Sharma, Pieter Gideon van Zyl, Johan Paul Beukes, Junying Sun, Erich G. Rohwer, Ruru Deng, Rodanthi-Elisavet Mamouri, and Felix Zamorano
Atmos. Chem. Phys., 16, 5111–5137, https://doi.org/10.5194/acp-16-5111-2016, https://doi.org/10.5194/acp-16-5111-2016, 2016
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The findings from more than 10 years of global aerosol lidar measurements with Polly systems are summarized, and a data set of optical properties for specific aerosol types is given. An automated data retrieval algorithm for continuous Polly lidar observations is presented and discussed by means of a Saharan dust advection event in Leipzig, Germany. Finally, a statistic on the vertical aerosol distribution including the seasonal variability at PollyNET locations around the globe is presented.
Ulla Wandinger, Volker Freudenthaler, Holger Baars, Aldo Amodeo, Ronny Engelmann, Ina Mattis, Silke Groß, Gelsomina Pappalardo, Aldo Giunta, Giuseppe D'Amico, Anatoli Chaikovsky, Fiodor Osipenko, Alexander Slesar, Doina Nicolae, Livio Belegante, Camelia Talianu, Ilya Serikov, Holger Linné, Friedhelm Jansen, Arnoud Apituley, Keith M. Wilson, Martin de Graaf, Thomas Trickl, Helmut Giehl, Mariana Adam, Adolfo Comerón, Constantino Muñoz-Porcar, Francesc Rocadenbosch, Michaël Sicard, Sergio Tomás, Diego Lange, Dhiraj Kumar, Manuel Pujadas, Francisco Molero, Alfonso J. Fernández, Lucas Alados-Arboledas, Juan Antonio Bravo-Aranda, Francisco Navas-Guzmán, Juan Luis Guerrero-Rascado, María José Granados-Muñoz, Jana Preißler, Frank Wagner, Michael Gausa, Ivan Grigorov, Dimitar Stoyanov, Marco Iarlori, Vincenco Rizi, Nicola Spinelli, Antonella Boselli, Xuan Wang, Teresa Lo Feudo, Maria Rita Perrone, Ferdinando De Tomasi, and Pasquale Burlizzi
Atmos. Meas. Tech., 9, 1001–1023, https://doi.org/10.5194/amt-9-1001-2016, https://doi.org/10.5194/amt-9-1001-2016, 2016
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We introduce the quality-assurance efforts of the European Aerosol Research Lidar Network (EARLINET) at instrument level. Within several campaigns, 21 EARLINET systems from 18 EARLINET stations were intercompared. A comprehensive strategy for campaign setup and data evaluation was established. The intercomparisons have reinforced our confidence in the EARLINET data quality and allowed us to draw conclusions on necessary system improvements and to identify major challenges for our future work.
Nikolaos Papagiannopoulos, Lucia Mona, Lucas Alados-Arboledas, Vassilis Amiridis, Holger Baars, Ioannis Binietoglou, Daniele Bortoli, Giuseppe D'Amico, Aldo Giunta, Juan Luis Guerrero-Rascado, Anja Schwarz, Sergio Pereira, Nicola Spinelli, Ulla Wandinger, Xuan Wang, and Gelsomina Pappalardo
Atmos. Chem. Phys., 16, 2341–2357, https://doi.org/10.5194/acp-16-2341-2016, https://doi.org/10.5194/acp-16-2341-2016, 2016
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Satellite-derived products must undergo data evaluation with reference data sets in order to identify any possible reasons of discrepancy or to assess their representativity. In that direction, data coming from CALIPSO satellite were compared with observations from the ground. We identified a CALIPSO underestimation that could be linked to an assumption in the satellites' algorithms. The proposed correction improves the performance and could enhance aerosol modeling.
L. Belegante, J. A. Bravo-Aranda, V. Freudenthaler, D. Nicolae, A. Nemuc, L. Alados-Arboledas, A. Amodeo, G. Pappalardo, G. D’Amico, R. Engelmann, H. Baars, U. Wandinger, A. Papayannis, P. Kokkalis, and S. N. Pereira
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2015-337, https://doi.org/10.5194/amt-2015-337, 2016
Revised manuscript has not been submitted
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This study aims to present techniques developed to calibrate the lidar depolarization channels.
The experimental approach of the paper is designed to present how calibration procedures are implemented. Most of the literature is focused on the theoretical perspective of the topic and practical issues usually remain an open topic. A hands on approach for the assessment of the lidar polarization sensitivity is welcomed since most of these techniques require comprehensive practical description.
E. Jäkel, B. Mey, R. Levy, X. Gu, T. Yu, Z. Li, D. Althausen, B. Heese, and M. Wendisch
Atmos. Meas. Tech., 8, 5237–5249, https://doi.org/10.5194/amt-8-5237-2015, https://doi.org/10.5194/amt-8-5237-2015, 2015
G. D'Amico, A. Amodeo, H. Baars, I. Binietoglou, V. Freudenthaler, I. Mattis, U. Wandinger, and G. Pappalardo
Atmos. Meas. Tech., 8, 4891–4916, https://doi.org/10.5194/amt-8-4891-2015, https://doi.org/10.5194/amt-8-4891-2015, 2015
M. Sicard, G. D'Amico, A. Comerón, L. Mona, L. Alados-Arboledas, A. Amodeo, H. Baars, J. M. Baldasano, L. Belegante, I. Binietoglou, J. A. Bravo-Aranda, A. J. Fernández, P. Fréville, D. García-Vizcaíno, A. Giunta, M. J. Granados-Muñoz, J. L. Guerrero-Rascado, D. Hadjimitsis, A. Haefele, M. Hervo, M. Iarlori, P. Kokkalis, D. Lange, R. E. Mamouri, I. Mattis, F. Molero, N. Montoux, A. Muñoz, C. Muñoz Porcar, F. Navas-Guzmán, D. Nicolae, A. Nisantzi, N. Papagiannopoulos, A. Papayannis, S. Pereira, J. Preißler, M. Pujadas, V. Rizi, F. Rocadenbosch, K. Sellegri, V. Simeonov, G. Tsaknakis, F. Wagner, and G. Pappalardo
Atmos. Meas. Tech., 8, 4587–4613, https://doi.org/10.5194/amt-8-4587-2015, https://doi.org/10.5194/amt-8-4587-2015, 2015
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In the framework of the ACTRIS summer 2012 measurement campaign (8 June–17 July 2012), EARLINET organized and performed a controlled exercise of feasibility to demonstrate its potential to perform operational, coordinated measurements and deliver products in near-real time. The paper describes the measurement protocol and discusses the delivery of real-time and near-real-time lidar-derived products.
I. Binietoglou, S. Basart, L. Alados-Arboledas, V. Amiridis, A. Argyrouli, H. Baars, J. M. Baldasano, D. Balis, L. Belegante, J. A. Bravo-Aranda, P. Burlizzi, V. Carrasco, A. Chaikovsky, A. Comerón, G. D'Amico, M. Filioglou, M. J. Granados-Muñoz, J. L. Guerrero-Rascado, L. Ilic, P. Kokkalis, A. Maurizi, L. Mona, F. Monti, C. Muñoz-Porcar, D. Nicolae, A. Papayannis, G. Pappalardo, G. Pejanovic, S. N. Pereira, M. R. Perrone, A. Pietruczuk, M. Posyniak, F. Rocadenbosch, A. Rodríguez-Gómez, M. Sicard, N. Siomos, A. Szkop, E. Terradellas, A. Tsekeri, A. Vukovic, U. Wandinger, and J. Wagner
Atmos. Meas. Tech., 8, 3577–3600, https://doi.org/10.5194/amt-8-3577-2015, https://doi.org/10.5194/amt-8-3577-2015, 2015
A. Foth, H. Baars, P. Di Girolamo, and B. Pospichal
Atmos. Chem. Phys., 15, 7753–7763, https://doi.org/10.5194/acp-15-7753-2015, https://doi.org/10.5194/acp-15-7753-2015, 2015
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We present a method to derive water vapour profiles from Raman lidar measurements calibrated by the integrated water vapour from a collocated microwave radiometer. These simultaneous observations provide an operational and continuous measurement of water vapour profiles. The stability of the calibration factor allows for the calibration of the lidar even in the presence of clouds. Based on this approach, water vapour profiles can be retrieved during all non-precipitating conditions.
E. Giannakaki, A. Pfüller, K. Korhonen, T. Mielonen, L. Laakso, V. Vakkari, H. Baars, R. Engelmann, J. P. Beukes, P. G. Van Zyl, M. Josipovic, P. Tiitta, K. Chiloane, S. Piketh, H. Lihavainen, K. E. J. Lehtinen, and M. Komppula
Atmos. Chem. Phys., 15, 5429–5442, https://doi.org/10.5194/acp-15-5429-2015, https://doi.org/10.5194/acp-15-5429-2015, 2015
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In this study we summarize 1 year of Raman lidar observations over South Africa. The analyses of lidar measurements presented here could assist in bridging existing gaps in the knowledge of vertical distribution of aerosols above South Africa, since limited long-term data of this type are available for this region. For the first time, we have been able to cover the full seasonal cycle on geometrical characteristics and optical properties of free tropospheric aerosol layers in the region.
B. Altstädter, A. Platis, B. Wehner, A. Scholtz, N. Wildmann, M. Hermann, R. Käthner, H. Baars, J. Bange, and A. Lampert
Atmos. Meas. Tech., 8, 1627–1639, https://doi.org/10.5194/amt-8-1627-2015, https://doi.org/10.5194/amt-8-1627-2015, 2015
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The unmanned research aircraft Carolo P360 "ALADINA" is a flexible tool for investigating the horizontal and vertical distribution of freshly formed particles in the atmospheric boundary layer (ABL) combined with measurements of turbulent fluxes derived by fast meteorological sensors. First results of a feasibility study show, among others, events of particle bursts in an internal
layer of the ABL. Comparisons with ground-based instruments and a lidar present the reliability of the new system.
T. Kanitz, A. Ansmann, A. Foth, P. Seifert, U. Wandinger, R. Engelmann, H. Baars, D. Althausen, C. Casiccia, and F. Zamorano
Atmos. Meas. Tech., 7, 2061–2072, https://doi.org/10.5194/amt-7-2061-2014, https://doi.org/10.5194/amt-7-2061-2014, 2014
K. Korhonen, E. Giannakaki, T. Mielonen, A. Pfüller, L. Laakso, V. Vakkari, H. Baars, R. Engelmann, J. P. Beukes, P. G. Van Zyl, A. Ramandh, L. Ntsangwane, M. Josipovic, P. Tiitta, G. Fourie, I. Ngwana, K. Chiloane, and M. Komppula
Atmos. Chem. Phys., 14, 4263–4278, https://doi.org/10.5194/acp-14-4263-2014, https://doi.org/10.5194/acp-14-4263-2014, 2014
A. Skupin, A. Ansmann, R. Engelmann, H. Baars, and T. Müller
Atmos. Meas. Tech., 7, 701–712, https://doi.org/10.5194/amt-7-701-2014, https://doi.org/10.5194/amt-7-701-2014, 2014
Related subject area
Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Vertical profiles of cloud condensation nuclei number concentration and its empirical estimate from aerosol optical properties over the North China Plain
Measurement report: The Urmia playa as a source of airborne dust and ice-nucleating particles – Part 1: Correlation between soils and airborne samples
Constraining the particle-scale diversity of black carbon light absorption using a unified framework
Survival probability of new atmospheric particles: closure between theory and measurements from 1.4 to 100 nm
Predicting atmospheric background number concentration of ice-nucleating particles in the Arctic
Different effects of anthropogenic emissions and aging processes on the mixing state of soot particles in the nucleation and accumulation modes
Fluorescence characteristics, absorption properties, and radiative effects of water-soluble organic carbon in seasonal snow across northeastern China
Measurement report: Size distributions of urban aerosols down to 1 nm from long-term measurements
Rapid reappearance of air pollution after cold air outbreaks in northern and eastern China
On the relation between apparent ion and total particle growth rates in the boreal forest and related chamber experiments
Assessment of NAAPS-RA performance in Maritime Southeast Asia during CAMP2Ex
Comparison of particle number size distribution trends in ground measurements and climate models
Aerosol size distribution changes in FIREX-AQ biomass burning plumes: the impact of plume concentration on coagulation and OA condensation/evaporation
Impact of water uptake and mixing state on submicron particle deposition in the human respiratory tract (HRT) based on explicit hygroscopicity measurements at HRT-like conditions
Parameterizations of size distribution and refractive index of biomass burning organic aerosol with black carbon content
Newly identified climatically and environmentally significant high-latitude dust sources
Airborne observations during KORUS-AQ show that aerosol optical depths are more spatially self-consistent than aerosol intensive properties
Using aircraft measurements to characterize subgrid-scale variability of aerosol properties near the Atmospheric Radiation Measurement Southern Great Plains site
Measurement report: A multi-year study on the impacts of Chinese New Year celebrations on air quality in Beijing, China
An Evaluation of Biomass Burning Aerosol Mass, Extinction, and Size Distribution in GEOS using Observations from CAMP2Ex
Mixing state of black carbon at different atmospheres in north and southwest China
Columnar and surface urban aerosol in the Moscow megacity according to measurements and simulations with the COSMO-ART model
Vertical aerosol particle exchange in the marine boundary layer estimated from helicopter-borne measurements in the Azores region
Circum-Antarctic abundance and properties of CCN and INPs
The ice-nucleating activity of African mineral dust in the Caribbean boundary layer
Biomass burning and marine aerosol processing over the southeast Atlantic Ocean: a TEM single-particle analysis
Measurement report: Atmopsheric new particle formation in a peri-urban site in Lille, Northern France
Volatility parameterization of ambient organic aerosols at a rural site of the North China Plain
Light absorption by brown carbon over the South-East Atlantic Ocean
Particle size distribution and particulate matter concentrations during synoptic and convective dust events in West Texas
Measurement of light-absorbing particles in surface snow of central and western Himalayan glaciers: spatial variability, radiative impacts, and potential source regions
Seasonal variations in fire conditions are important drivers in the trend of aerosol optical properties over the south-eastern Atlantic
Black carbon aerosol reductions during COVID-19 confinement quantified by aircraft measurements over Europe
Diurnal evolution of negative atmospheric ions above the boreal forest: from ground level to the free troposphere
Absorption enhancement of black carbon particles in a Mediterranean city and countryside: effect of particulate matter chemistry, ageing and trend analysis
Measurement Report: Increasing trend of atmospheric ion concentrations in the boreal forest
Aerosol activation characteristics and prediction at the central European ACTRIS research station Melpitz, Germany
Characterizing the hygroscopicity of growing particles in the Canadian Arctic summer
Measurement report: Distinct size dependence and diurnal variation in organic aerosol hygroscopicity, volatility, and cloud condensation nuclei activity at a rural site in the Pearl River Delta (PRD) region, China
Measurement report: Atmospheric new particle formation in a coastal agricultural site explained with binPMF analysis of nitrate CI-APi-TOF spectra
Characteristics and evolution of brown carbon in western United States wildfires
Reduced surface fine dust under droughts over the southeastern United States during summertime: observations and CMIP6 model simulations
Strong light scattering of highly oxygenated organic aerosols impacts significantly on visibility degradation
Measurement report: Spectral and statistical analysis of aerosol hygroscopic growth from multi-wavelength lidar measurements in Barcelona, Spain
The diurnal and seasonal variability of ice-nucleating particles at the High Altitude Station Jungfraujoch (3580 m a.s.l.), Switzerland
The impact of large-scale circulation on daily fine particulate matter (PM2.5) over major populated regions of China in winter
New particle formation in coastal New Zealand with a focus on open-ocean air masses
Measurement report: Vertical profiling of particle size distributions over Lhasa, Tibet – tethered balloon-based in situ measurements and source apportionment
Seasonal Significance of New Particle Formation Impacts on Cloud Condensation Nuclei at a Mountaintop Location
Long- and short-term temporal variability in cloud condensation nuclei spectra over a wide supersaturation range in the Southern Great Plains site
Rui Zhang, Yuying Wang, Zhanqing Li, Zhibin Wang, Russell R. Dickerson, Xinrong Ren, Hao He, Fei Wang, Ying Gao, Xi Chen, Jialu Xu, Yafang Cheng, and Hang Su
Atmos. Chem. Phys., 22, 14879–14891, https://doi.org/10.5194/acp-22-14879-2022, https://doi.org/10.5194/acp-22-14879-2022, 2022
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Factors of cloud condensation nuclei number concentration (NCCN) profiles determined in the North China Plain include air mass sources, temperature structure, anthropogenic emissions, and terrain distribution. Cloud condensation nuclei (CCN) spectra suggest that the ability of aerosol activation into CCN is stronger in southeasterly than in northwesterly air masses and stronger in the free atmosphere than near the surface. A good method to parameterize NCCN from aerosol optical data is found.
Nikou Hamzehpour, Claudia Marcolli, Sara Pashai, Kristian Klumpp, and Thomas Peter
Atmos. Chem. Phys., 22, 14905–14930, https://doi.org/10.5194/acp-22-14905-2022, https://doi.org/10.5194/acp-22-14905-2022, 2022
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Playa surfaces in Iran that emerged through Lake Urmia (LU) desiccation have become a relevant dust source of regional relevance. Here, we identify highly erodible LU playa surfaces and determine their physicochemical properties and mineralogical composition and perform emulsion-freezing experiments with them. We find high ice nucleation activities (up to 250 K) that correlate positively with organic matter and clay content and negatively with pH, salinity, K-feldspars, and quartz.
Payton Beeler and Rajan K. Chakrabarty
Atmos. Chem. Phys., 22, 14825–14836, https://doi.org/10.5194/acp-22-14825-2022, https://doi.org/10.5194/acp-22-14825-2022, 2022
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Understanding and parameterizing the influences of black carbon (BC) particle morphology and compositional heterogeneity on its light absorption represent a fundamental problem. We develop scaling laws using a single unifying parameter that effectively encompasses large-scale diversity observed in BC light absorption on a per-particle basis. The laws help reconcile the disparities between field observations and model predictions. Our framework is packaged in an open-source Python application.
Runlong Cai, Chenjuan Deng, Dominik Stolzenburg, Chenxi Li, Junchen Guo, Veli-Matti Kerminen, Jingkun Jiang, Markku Kulmala, and Juha Kangasluoma
Atmos. Chem. Phys., 22, 14571–14587, https://doi.org/10.5194/acp-22-14571-2022, https://doi.org/10.5194/acp-22-14571-2022, 2022
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The survival probability of new particles is the key parameter governing their influences on the atmosphere and climate, yet the knowledge of particle survival in the atmosphere is rather limited. We propose methods to compute the size-resolved particle survival probability and validate them using simulations and measurements from diverse environments. Using these methods, we could explain particle survival from the cluster size to the cloud condensation nuclei size.
Guangyu Li, Jörg Wieder, Julie T. Pasquier, Jan Henneberger, and Zamin A. Kanji
Atmos. Chem. Phys., 22, 14441–14454, https://doi.org/10.5194/acp-22-14441-2022, https://doi.org/10.5194/acp-22-14441-2022, 2022
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The concentration of ice-nucleating particles (INPs) is atmospherically relevant for primary ice formation in clouds. In this work, from 12 weeks of field measurement data in the Arctic, we developed a new parameterization to predict INP concentrations applicable for pristine background conditions based only on temperature. The INP parameterization could improve the cloud microphysical representation in climate models, aiding in Arctic climate predictions.
Yuying Wang, Rong Hu, Qiuyan Wang, Zhanqing Li, Maureen Cribb, Yele Sun, Xiaorui Song, Yi Shang, Yixuan Wu, Xin Huang, and Yuxiang Wang
Atmos. Chem. Phys., 22, 14133–14146, https://doi.org/10.5194/acp-22-14133-2022, https://doi.org/10.5194/acp-22-14133-2022, 2022
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The mixing state of size-resolved soot particles and their influencing factors were investigated. The results suggest anthropogenic emissions and aging processes have diverse impacts on the mixing state of soot particles in different modes. Considering that the mixing state of soot particles is crucial to model aerosol absorption, this finding is important to study particle growth and the warming effect of black carbon aerosols.
Xiaoying Niu, Wei Pu, Pingqing Fu, Yang Chen, Yuxuan Xing, Dongyou Wu, Ziqi Chen, Tenglong Shi, Yue Zhou, Hui Wen, and Xin Wang
Atmos. Chem. Phys., 22, 14075–14094, https://doi.org/10.5194/acp-22-14075-2022, https://doi.org/10.5194/acp-22-14075-2022, 2022
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In this study, we do the first investigation of WSOC in seasonal snow of northeastern China. The results revealed the regional-specific compositions and sources of WSOC due to different natural environments and anthropogenic activities. The abundant concentrations of WSOC and its absorption properties contributed to a crucial impact on the snow albedo and radiative effect. We established that our study could raise awareness of carbon cycling processes, hydrological processes, and climate change.
Chenjuan Deng, Yiran Li, Chao Yan, Jin Wu, Runlong Cai, Dongbin Wang, Yongchun Liu, Juha Kangasluoma, Veli-Matti Kerminen, Markku Kulmala, and Jingkun Jiang
Atmos. Chem. Phys., 22, 13569–13580, https://doi.org/10.5194/acp-22-13569-2022, https://doi.org/10.5194/acp-22-13569-2022, 2022
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The size distributions of urban atmospheric particles convey important information on their origins and impacts. This study investigates the characteristics of typical particle size distributions and key gaseous precursors in the long term in urban Beijing. A fitting function is proposed to represent and help interpret size distribution including particles and gaseous precursors. In addition to NPF (new particle formation) as the major source, vehicles can emit sub-3 nm particles as well
Qian Liu, Guixing Chen, Lifang Sheng, and Toshiki Iwasaki
Atmos. Chem. Phys., 22, 13371–13388, https://doi.org/10.5194/acp-22-13371-2022, https://doi.org/10.5194/acp-22-13371-2022, 2022
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Air pollution can be cleaned up quickly by a cold air outbreak (CAO) but reappears after a CAO. By quantifying the CAO properties, we find the coldness and depth of the cold air mass are key factors affecting the rapid (slow) reappearance of air pollution through modulating the atmospheric boundary layer height and stability. We also find that the spatial pattern of CAO in high-latitude Eurasia a few days ahead can be recognized as a precursor for the reappearance of air pollution.
Loïc Gonzalez Carracedo, Katrianne Lehtipalo, Lauri R. Ahonen, Nina Sarnela, Sebastian Holm, Juha Kangasluoma, Markku Kulmala, Paul M. Winkler, and Dominik Stolzenburg
Atmos. Chem. Phys., 22, 13153–13166, https://doi.org/10.5194/acp-22-13153-2022, https://doi.org/10.5194/acp-22-13153-2022, 2022
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Fast nanoparticle growth is essential for the survival of new aerosol particles in the atmosphere and hence their contribution to the climate. We show that using naturally charged ions for growth calculations can cause a significant error. During the diurnal cycle, the importance of ion-induced and neutral nucleation varies, causing the ion population to have a slower measurable apparent growth. Results suggest that data from ion spectrometers need to be considered with great care below 3 nm.
Eva-Lou Edwards, Jeffrey S. Reid, Peng Xian, Sharon P. Burton, Anthony L. Cook, Ewan C. Crosbie, Marta A. Fenn, Richard A. Ferrare, Sean W. Freeman, John W. Hair, David B. Harper, Chris A. Hostetler, Claire E. Robinson, Amy Jo Scarino, Michael A. Shook, G. Alexander Sokolowsky, Susan C. van den Heever, Edward L. Winstead, Sarah Woods, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 22, 12961–12983, https://doi.org/10.5194/acp-22-12961-2022, https://doi.org/10.5194/acp-22-12961-2022, 2022
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This study compares NAAPS-RA model simulations of aerosol optical thickness (AOT) and extinction to those retrieved with a high spectral resolution lidar near the Philippines. Agreement for AOT was good, and extinction agreement was strongest below 1500 m. Substituting dropsonde relative humidities into NAAPS-RA did not drastically improve agreement, and we discuss potential reasons why. Accurately modeling future conditions in this region is crucial due to its susceptibility to climate change.
Ville Leinonen, Harri Kokkola, Taina Yli-Juuti, Tero Mielonen, Thomas Kühn, Tuomo Nieminen, Simo Heikkinen, Tuuli Miinalainen, Tommi Bergman, Ken Carslaw, Stefano Decesari, Markus Fiebig, Tareq Hussein, Niku Kivekäs, Radovan Krejci, Markku Kulmala, Ari Leskinen, Andreas Massling, Nikos Mihalopoulos, Jane P. Mulcahy, Steffen M. Noe, Twan van Noije, Fiona M. O'Connor, Colin O'Dowd, Dirk Olivie, Jakob B. Pernov, Tuukka Petäjä, Øyvind Seland, Michael Schulz, Catherine E. Scott, Henrik Skov, Erik Swietlicki, Thomas Tuch, Alfred Wiedensohler, Annele Virtanen, and Santtu Mikkonen
Atmos. Chem. Phys., 22, 12873–12905, https://doi.org/10.5194/acp-22-12873-2022, https://doi.org/10.5194/acp-22-12873-2022, 2022
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We provide the first extensive comparison of detailed aerosol size distribution trends between in situ observations from Europe and five different earth system models. We investigated aerosol modes (nucleation, Aitken, and accumulation) separately and were able to show the differences between measured and modeled trends and especially their seasonal patterns. The differences in model results are likely due to complex effects of several processes instead of certain specific model features.
Nicole A. June, Anna L. Hodshire, Elizabeth B. Wiggins, Edward L. Winstead, Claire E. Robinson, K. Lee Thornhill, Kevin J. Sanchez, Richard H. Moore, Demetrios Pagonis, Hongyu Guo, Pedro Campuzano-Jost, Jose L. Jimenez, Matthew M. Coggon, Jonathan M. Dean-Day, T. Paul Bui, Jeff Peischl, Robert J. Yokelson, Matthew J. Alvarado, Sonia M. Kreidenweis, Shantanu H. Jathar, and Jeffrey R. Pierce
Atmos. Chem. Phys., 22, 12803–12825, https://doi.org/10.5194/acp-22-12803-2022, https://doi.org/10.5194/acp-22-12803-2022, 2022
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The evolution of organic aerosol composition and size is uncertain due to variability within and between smoke plumes. We examine the impact of plume concentration on smoke evolution from smoke plumes sampled by the NASA DC-8 during FIREX-AQ. We find that observed organic aerosol and size distribution changes are correlated to plume aerosol mass concentrations. Additionally, coagulation explains the majority of the observed growth.
Ruiqi Man, Zhijun Wu, Taomou Zong, Aristeidis Voliotis, Yanting Qiu, Johannes Größ, Dominik van Pinxteren, Limin Zeng, Hartmut Herrmann, Alfred Wiedensohler, and Min Hu
Atmos. Chem. Phys., 22, 12387–12399, https://doi.org/10.5194/acp-22-12387-2022, https://doi.org/10.5194/acp-22-12387-2022, 2022
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Regional and total deposition doses for different age groups were quantified based on explicit hygroscopicity measurements. We found that particle hygroscopic growth led to a reduction (~24 %) in the total dose. The deposition rate of hygroscopic particles was higher in the daytime, while hydrophobic particles exhibited a higher rate at night and during rush hours. The results will deepen the understanding of the impact of hygroscopicity and the mixing state on deposition patterns in the lungs.
Biao Luo, Ye Kuang, Shan Huang, Qicong Song, Weiwei Hu, Wei Li, Yuwen Peng, Duohong Chen, Dingli Yue, Bin Yuan, and Min Shao
Atmos. Chem. Phys., 22, 12401–12415, https://doi.org/10.5194/acp-22-12401-2022, https://doi.org/10.5194/acp-22-12401-2022, 2022
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We performed comprehensive analysis on biomass burning organic aerosol (BBOA) size distributions, as well as mass scattering and absorption efficiencies, with an improved method of on-line quantification of brown carbon absorptions. Both BBOA volume size distribution and retrieved refractive index depend highly on combustion conditions represented by the black carbon content, which has significant implications for BBOA climate effect simulations.
Outi Meinander, Pavla Dagsson-Waldhauserova, Pavel Amosov, Elena Aseyeva, Cliff Atkins, Alexander Baklanov, Clarissa Baldo, Sarah L. Barr, Barbara Barzycka, Liane G. Benning, Bojan Cvetkovic, Polina Enchilik, Denis Frolov, Santiago Gassó, Konrad Kandler, Nikolay Kasimov, Jan Kavan, James King, Tatyana Koroleva, Viktoria Krupskaya, Markku Kulmala, Monika Kusiak, Hanna K. Lappalainen, Michał Laska, Jerome Lasne, Marek Lewandowski, Bartłomiej Luks, James B. McQuaid, Beatrice Moroni, Benjamin Murray, Ottmar Möhler, Adam Nawrot, Slobodan Nickovic, Norman T. O’Neill, Goran Pejanovic, Olga Popovicheva, Keyvan Ranjbar, Manolis Romanias, Olga Samonova, Alberto Sanchez-Marroquin, Kerstin Schepanski, Ivan Semenkov, Anna Sharapova, Elena Shevnina, Zongbo Shi, Mikhail Sofiev, Frédéric Thevenet, Throstur Thorsteinsson, Mikhail Timofeev, Nsikanabasi Silas Umo, Andreas Uppstu, Darya Urupina, György Varga, Tomasz Werner, Olafur Arnalds, and Ana Vukovic Vimic
Atmos. Chem. Phys., 22, 11889–11930, https://doi.org/10.5194/acp-22-11889-2022, https://doi.org/10.5194/acp-22-11889-2022, 2022
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High-latitude dust (HLD) is a short-lived climate forcer, air pollutant, and nutrient source. Our results suggest a northern HLD belt at 50–58° N in Eurasia and 50–55° N in Canada and at >60° N in Eurasia and >58° N in Canada. Our addition to the previously identified global dust belt (GDB) provides crucially needed information on the extent of active HLD sources with both direct and indirect impacts on climate and environment in remote regions, which are often poorly understood and predicted.
Samuel E. LeBlanc, Michal Segal-Rozenhaimer, Jens Redemann, Connor Flynn, Roy R. Johnson, Stephen E. Dunagan, Robert Dahlgren, Jhoon Kim, Myungje Choi, Arlindo da Silva, Patricia Castellanos, Qian Tan, Luke Ziemba, Kenneth Lee Thornhill, and Meloë Kacenelenbogen
Atmos. Chem. Phys., 22, 11275–11304, https://doi.org/10.5194/acp-22-11275-2022, https://doi.org/10.5194/acp-22-11275-2022, 2022
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Airborne observations of atmospheric particles and pollution over Korea during a field campaign in May–June 2016 showed that the smallest atmospheric particles are present in the lowest 2 km of the atmosphere. The aerosol size is more spatially variable than optical thickness. We show this with remote sensing (4STAR), in situ (LARGE) observations, satellite measurements (GOCI), and modeled properties (MERRA-2), and it is contrary to the current understanding.
Jerome D. Fast, David M. Bell, Gourihar Kulkarni, Jiumeng Liu, Fan Mei, Georges Saliba, John E. Shilling, Kaitlyn Suski, Jason Tomlinson, Jian Wang, Rahul Zaveri, and Alla Zelenyuk
Atmos. Chem. Phys., 22, 11217–11238, https://doi.org/10.5194/acp-22-11217-2022, https://doi.org/10.5194/acp-22-11217-2022, 2022
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Recent aircraft measurements from the HI-SCALE campaign conducted over the Southern Great Plains (SGP) site in Oklahoma are used to quantify spatial variability of aerosol properties in terms of grid spacings typically used by weather and climate models. Surprisingly large horizontal gradients in aerosol properties were frequently observed in this rural area. This spatial variability can be used as an uncertainty range when comparing surface point measurements with model predictions.
Benjamin Foreback, Lubna Dada, Kaspar R. Daellenbach, Chao Yan, Lili Wang, Biwu Chu, Ying Zhou, Tom V. Kokkonen, Mona Kurppa, Rosaria E. Pileci, Yonghong Wang, Tommy Chan, Juha Kangasluoma, Lin Zhuohui, Yishou Guo, Chang Li, Rima Baalbaki, Joni Kujansuu, Xiaolong Fan, Zemin Feng, Pekka Rantala, Shahzad Gani, Federico Bianchi, Veli-Matti Kerminen, Tuukka Petäjä, Markku Kulmala, Yongchun Liu, and Pauli Paasonen
Atmos. Chem. Phys., 22, 11089–11104, https://doi.org/10.5194/acp-22-11089-2022, https://doi.org/10.5194/acp-22-11089-2022, 2022
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This study analyzed air quality in Beijing during the Chinese New Year over 7 years, including data from a new in-depth measurement station. This is one of few studies to look at long-term impacts, including the outcome of firework restrictions starting in 2018. Results show that firework pollution has gone down since 2016, indicating a positive result from the restrictions. Results of this study may be useful in making future decisions about the use of fireworks to improve air quality.
Allison B. Marquardt Collow, Virginie Buchard, Peter R. Colarco, Arlindo M. da Silva, Ravi Govindaraju, Edward P. Nowottnick, Sharon Burton, Richard Ferrare, Chris Hostetler, and Luke Ziemba
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-545, https://doi.org/10.5194/acp-2022-545, 2022
Revised manuscript accepted for ACP
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Biomass burning aerosol impacts aspects of the atmosphere and Earth system through radiative forcing, serving as cloud condensation nuclei, and air quality. Despite its importance, the representation of biomass burning aerosol is not always accurate in models. Field campaign observations from CAMP2Ex are used to evaluate the mass and extinction of aerosols in the GEOS model. Notable biases in the model illuminate areas of future development with GEOS and the underlying GOCART aerosol module.
Gang Zhao, Tianyi Tan, Shuya Hu, Zhuofei Du, Dongjie Shang, Zhijun Wu, Song Guo, Jing Zheng, Wenfei Zhu, Mengren Li, Limin Zeng, and Min Hu
Atmos. Chem. Phys., 22, 10861–10873, https://doi.org/10.5194/acp-22-10861-2022, https://doi.org/10.5194/acp-22-10861-2022, 2022
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Black carbon is the second strongest absorbing component in the atmosphere that exerts warming effects on climate. One critical challenge in quantifying the ambient black carbon's radiative effects is addressing the BC microphysical properties. In this study, the microphysical properties of the aged and fresh BC particles are synthetically analyzed under different atmospheres. The measurement results can be further used in models to help constrain the uncertainties of the BC radiative effects.
Natalia E. Chubarova, Heike Vogel, Elizaveta E. Androsova, Alexander A. Kirsanov, Olga B. Popovicheva, Bernhard Vogel, and Gdaliy S. Rivin
Atmos. Chem. Phys., 22, 10443–10466, https://doi.org/10.5194/acp-22-10443-2022, https://doi.org/10.5194/acp-22-10443-2022, 2022
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Effects of urban aerosol pollution in Moscow were analyzed using the COSMO-ART chemical transport model and intensive measurement campaigns. We show that urban aerosol comprises about 15–20% of columnar aerosol content, consisting mainly of fine aerosol mode. The black carbon (BC) fraction is about 5 %, depending on particle dispersion intensity (IPD). The BC fraction low value explains weak absorbing properties of the Moscow atmosphere. IPD also defines the daily cycle of urban aerosol species.
Janine Lückerath, Andreas Held, Holger Siebert, Michel Michalkow, and Birgit Wehner
Atmos. Chem. Phys., 22, 10007–10021, https://doi.org/10.5194/acp-22-10007-2022, https://doi.org/10.5194/acp-22-10007-2022, 2022
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Three different methods were applied to estimate the vertical aerosol particle flux in the marine boundary layer (MBL) and between the MBL and free troposphere. For the first time, aerosol fluxes derived from these three methods were estimated and compared using airborne aerosol measurements using data from the ACORES field campaign in the northeastern Atlantic Ocean in July 2017. The amount of fluxes was small and directed up and down for different cases, but the methods were applicable.
Christian Tatzelt, Silvia Henning, André Welti, Andrea Baccarini, Markus Hartmann, Martin Gysel-Beer, Manuela van Pinxteren, Robin L. Modini, Julia Schmale, and Frank Stratmann
Atmos. Chem. Phys., 22, 9721–9745, https://doi.org/10.5194/acp-22-9721-2022, https://doi.org/10.5194/acp-22-9721-2022, 2022
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We present the abundance and origin of cloud-relevant aerosol particles in the preindustral-like conditions of the Southern Ocean (SO) during austral summer. Cloud condensation nuclei (CCN) and ice-nucleating particles (INP) were measured during a circum-Antarctic scientific cruise with in situ instrumentation and offline filter measurements, respectively. Transport processes were found to play an equally important role as local sources for both the CCN and INP population of the SO.
Alexander D. Harrison, Daniel O'Sullivan, Michael P. Adams, Grace C. E. Porter, Edmund Blades, Cherise Brathwaite, Rebecca Chewitt-Lucas, Cassandra Gaston, Rachel Hawker, Ovid O. Krüger, Leslie Neve, Mira L. Pöhlker, Christopher Pöhlker, Ulrich Pöschl, Alberto Sanchez-Marroquin, Andrea Sealy, Peter Sealy, Mark D. Tarn, Shanice Whitehall, James B. McQuaid, Kenneth S. Carslaw, Joseph M. Prospero, and Benjamin J. Murray
Atmos. Chem. Phys., 22, 9663–9680, https://doi.org/10.5194/acp-22-9663-2022, https://doi.org/10.5194/acp-22-9663-2022, 2022
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The formation of ice in clouds fundamentally alters cloud properties; hence it is important we understand the special aerosol particles that can nucleate ice when immersed in supercooled cloud droplets. In this paper we show that African desert dust that has travelled across the Atlantic to the Caribbean nucleates ice much less well than we might have expected.
Caroline Dang, Michal Segal-Rozenhaimer, Haochi Che, Lu Zhang, Paola Formenti, Jonathan Taylor, Amie Dobracki, Sara Purdue, Pui-Shan Wong, Athanasios Nenes, Arthur Sedlacek III, Hugh Coe, Jens Redemann, Paquita Zuidema, Steven Howell, and James Haywood
Atmos. Chem. Phys., 22, 9389–9412, https://doi.org/10.5194/acp-22-9389-2022, https://doi.org/10.5194/acp-22-9389-2022, 2022
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Transmission electron microscopy was used to analyze aged African smoke particles and how the smoke interacts with the marine atmosphere. We found that the volatility of organic aerosol increases with biomass burning plume age, that black carbon is often mixed with potassium salts and that the marine atmosphere can incorporate Na and Cl into smoke particles. Marine salts are more processed when mixed with smoke plumes, and there are interesting Cl-rich yet Na-absent marine particles.
Suzanne Crumeyrolle, Jenni Kontkanen, Clémence Rose, Alejandra Velasquez Garcia, Eric Bourrianne, Maxime Catalfamo, Véronique Riffault, Emmanuel Tison, Joel Ferreira de Brito, Nicolas Visez, Nicolas Ferlay, Frédérique Auriol, and Isabelle Chiapello
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-436, https://doi.org/10.5194/acp-2022-436, 2022
Revised manuscript accepted for ACP
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Ultrafine particles (UFPs) are particles with an aerodynamic diameter of 100 nm or less, has negligible mass concentration but is the dominant contributor to the total particle number concentration. The present study aims to better understand the environmental factors favoring or inhibiting, atmospheric new particle formation (NPF) over Lille a large city North of France and to analyze the impact of such event on urban air quality using a long-term dataset (3 years).
Siman Ren, Lei Yao, Yuwei Wang, Gan Yang, Yiliang Liu, Yueyang Li, Yiqun Lu, Lihong Wang, and Lin Wang
Atmos. Chem. Phys., 22, 9283–9297, https://doi.org/10.5194/acp-22-9283-2022, https://doi.org/10.5194/acp-22-9283-2022, 2022
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We improved the empirical functions between volatility and chemical formulas of organic aerosols based on lab experiments and field observations. It was found that organic compounds in ambient aerosols can be divided into two groups according to their O / C ratios and that there should be specialized volatility parameterizations for different O / C organic compounds.
Lu Zhang, Michal Segal-Rozenhaimer, Haochi Che, Caroline Dang, Arthur J. Sedlacek III, Ernie R. Lewis, Amie Dobracki, Jenny P. S. Wong, Paola Formenti, Steven G. Howell, and Athanasios Nenes
Atmos. Chem. Phys., 22, 9199–9213, https://doi.org/10.5194/acp-22-9199-2022, https://doi.org/10.5194/acp-22-9199-2022, 2022
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Widespread biomass burning (BB) events occur annually in Africa and contribute ~ 1 / 3 of global BB emissions, which contain a large family of light-absorbing organics, known as brown carbon (BrC), whose absorption of incident radiation is difficult to estimate, leading to large uncertainties in the global radiative forcing estimation. This study quantifies the BrC absorption of aged BB particles and highlights the potential presence of absorbing iron oxides in this climatically important region.
Karin Ardon-Dryer and Mary C. Kelley
Atmos. Chem. Phys., 22, 9161–9173, https://doi.org/10.5194/acp-22-9161-2022, https://doi.org/10.5194/acp-22-9161-2022, 2022
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Changes in the particle size distribution and particulate matter concentrations during different dust events in West Texas were examined. Analysis based on different timescales showed that current common methods used to evaluate the impact of dust events on air quality will not capture the true impact of short (convective) dust events and, therefore, do not provide an insightful understanding of their impact on the environment and human health.
Chaman Gul, Shichang Kang, Siva Praveen Puppala, Xiaokang Wu, Cenlin He, Yangyang Xu, Inka Koch, Sher Muhammad, Rajesh Kumar, and Getachew Dubache
Atmos. Chem. Phys., 22, 8725–8737, https://doi.org/10.5194/acp-22-8725-2022, https://doi.org/10.5194/acp-22-8725-2022, 2022
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This work aims to understand concentrations, spatial variability, and potential source regions of light-absorbing impurities (black carbon aerosols, dust particles, and organic carbon) in the surface snow of central and western Himalayan glaciers and their impact on snow albedo and radiative forcing.
Haochi Che, Michal Segal-Rozenhaimer, Lu Zhang, Caroline Dang, Paquita Zuidema, Arthur J. Sedlacek III, Xiaoye Zhang, and Connor Flynn
Atmos. Chem. Phys., 22, 8767–8785, https://doi.org/10.5194/acp-22-8767-2022, https://doi.org/10.5194/acp-22-8767-2022, 2022
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A 17-month in situ study on Ascension Island found low single-scattering albedo and strong absorption enhancement of the marine boundary layer aerosols during biomass burnings on the African continent, along with apparent patterns of regular monthly variability. We further discuss the characteristics and drivers behind these changes and find that biomass burning conditions in Africa may be the main factor influencing the optical properties of marine boundary aerosols.
Ovid O. Krüger, Bruna A. Holanda, Sourangsu Chowdhury, Andrea Pozzer, David Walter, Christopher Pöhlker, Maria Dolores Andrés Hernández, John P. Burrows, Christiane Voigt, Jos Lelieveld, Johannes Quaas, Ulrich Pöschl, and Mira L. Pöhlker
Atmos. Chem. Phys., 22, 8683–8699, https://doi.org/10.5194/acp-22-8683-2022, https://doi.org/10.5194/acp-22-8683-2022, 2022
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The abrupt reduction in human activities during the first COVID-19 lockdown created unprecedented atmospheric conditions. We took the opportunity to quantify changes in black carbon (BC) as a major anthropogenic air pollutant. Therefore, we measured BC on board a research aircraft over Europe during the lockdown and compared the results to measurements from 2017. With model simulations we account for different weather conditions and find a lockdown-related decrease in BC of 41 %.
Lisa J. Beck, Siegfried Schobesberger, Heikki Junninen, Janne Lampilahti, Antti Manninen, Lubna Dada, Katri Leino, Xu-Cheng He, Iida Pullinen, Lauriane L. J. Quéléver, Anna Franck, Pyry Poutanen, Daniela Wimmer, Frans Korhonen, Mikko Sipilä, Mikael Ehn, Douglas R. Worsnop, Veli-Matti Kerminen, Tuukka Petäjä, Markku Kulmala, and Jonathan Duplissy
Atmos. Chem. Phys., 22, 8547–8577, https://doi.org/10.5194/acp-22-8547-2022, https://doi.org/10.5194/acp-22-8547-2022, 2022
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The presented article introduces an overview of atmospheric ions and their composition above the boreal forest. We provide the results of an extensive airborne measurement campaign with an air ion mass spectrometer and particle measurements, showing their diurnal evolution within the boundary layer and free troposphere. In addition, we compare the airborne dataset with the co-located data from the ground at SMEAR II station, Finland.
Jesús Yus-Díez, Marta Via, Andrés Alastuey, Angeliki Karanasiou, María Cruz Minguillón, Noemí Perez, Xavier Querol, Cristina Reche, Matic Ivančič, Martin Rigler, and Marco Pandolfi
Atmos. Chem. Phys., 22, 8439–8456, https://doi.org/10.5194/acp-22-8439-2022, https://doi.org/10.5194/acp-22-8439-2022, 2022
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This study presents the absorption enhancement of internally and externally mixed black carbon (BC) particles in a Mediterranean city and countryside. We showed the importance of secondary organic aerosols (SOAs) and particle ageing by increasing the BC absorption enhancement. We performed a trend analysis on the absorption enhancement. We found a positive trend of the absorption enhancement at the regional station in summer driven by the increase over time of the relative contribution of SOA.
Juha Sulo, Janne Lampilahti, Xuemeng Chen, Jenni Kontkanen, Tuomo Nieminen, Veli-Matti Kerminen, Tuukka Petäjä, Markku Kulmala, and Katrianne Lehtipalo
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-392, https://doi.org/10.5194/acp-2022-392, 2022
Revised manuscript accepted for ACP
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We measured atmospheric ion concentrations continuously in a boreal forest between 2005 and 2021 and observed an increasing inter-annual trend. The increase in cluster ion concentrations can be largely explained by overall decreasing level of anthropogenic aerosols in the boreal forest. This suggests that the role of ions in atmospheric new particle formation may be more important in the future.
Yuan Wang, Silvia Henning, Laurent Poulain, Chunsong Lu, Frank Stratmann, Yuying Wang, Shengjie Niu, Mira L. Pöhlker, Hartmut Herrmann, and Alfred Wiedensohler
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-427, https://doi.org/10.5194/acp-2022-427, 2022
Revised manuscript accepted for ACP
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Aerosol particle activation affects cloud, precipitation, radiation, and thus the global climate. Its long-term measurements are important but still scarce. In this study, more than 4-year measurements at a central European station were analyzed. The overall characteristics and seasonal changes of aerosol particle activation are summarized. The power-law fit between particle hygroscopicity factor and diameter was recommended for predicting CCN number concentration.
Rachel Y.-W. Chang, Jonathan P. D. Abbatt, Matthew C. Boyer, Jai Prakash Chaubey, and Douglas B. Collins
Atmos. Chem. Phys., 22, 8059–8071, https://doi.org/10.5194/acp-22-8059-2022, https://doi.org/10.5194/acp-22-8059-2022, 2022
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During summer 2016, the ability of newly formed particles to turn into droplets was measured in the Canadian Arctic. Our observations suggest that these small particles were growing by the condensation of organic vapours likely coming from the surrounding open waters. These particles grew large enough that they could form cloud droplets and therefore affect the earth’s radiation budget. These results are relevant as the Arctic summer rapidly warms with climate change.
Mingfu Cai, Shan Huang, Baoling Liang, Qibin Sun, Li Liu, Bin Yuan, Min Shao, Weiwei Hu, Wei Chen, Qicong Song, Wei Li, Yuwen Peng, Zelong Wang, Duohong Chen, Haobo Tan, Hanbin Xu, Fei Li, Xuejiao Deng, Tao Deng, Jiaren Sun, and Jun Zhao
Atmos. Chem. Phys., 22, 8117–8136, https://doi.org/10.5194/acp-22-8117-2022, https://doi.org/10.5194/acp-22-8117-2022, 2022
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This study investigated the size dependence and diurnal variation in organic aerosol hygroscopicity, volatility, and cloud condensation nuclei (CCN) activity. We found that the physical properties of OA could vary in a large range at different particle sizes and affected the number concentration of CCN (NCCN) at all supersaturations. Our results highlight the importance of evaluating the atmospheric evolution processes of OA at different size ranges and their impact on climate effects.
Miska Olin, Magdalena Okuljar, Matti P. Rissanen, Joni Kalliokoski, Jiali Shen, Lubna Dada, Markus Lampimäki, Yusheng Wu, Annalea Lohila, Jonathan Duplissy, Mikko Sipilä, Tuukka Petäjä, Markku Kulmala, and Miikka Dal Maso
Atmos. Chem. Phys., 22, 8097–8115, https://doi.org/10.5194/acp-22-8097-2022, https://doi.org/10.5194/acp-22-8097-2022, 2022
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Atmospheric new particle formation is an important source of the total particle number concentration in the atmosphere. Several parameters for predicting new particle formation events have been suggested before, but the results have been inconclusive. This study proposes an another predicting parameter, related to a specific type of highly oxidized organic molecules, especially for similar locations to the measurement site in this study, which was a coastal agricultural site in Finland.
Linghan Zeng, Jack Dibb, Eric Scheuer, Joseph M. Katich, Joshua P. Schwarz, Ilann Bourgeois, Jeff Peischl, Tom Ryerson, Carsten Warneke, Anne E. Perring, Glenn S. Diskin, Joshua P. DiGangi, John B. Nowak, Richard H. Moore, Elizabeth B. Wiggins, Demetrios Pagonis, Hongyu Guo, Pedro Campuzano-Jost, Jose L. Jimenez, Lu Xu, and Rodney J. Weber
Atmos. Chem. Phys., 22, 8009–8036, https://doi.org/10.5194/acp-22-8009-2022, https://doi.org/10.5194/acp-22-8009-2022, 2022
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Wildfires emit aerosol particles containing brown carbon material that affects visibility and global climate and is toxic. Brown carbon is poorly characterized due to measurement limitations, and its evolution in the atmosphere is not well known. We report on aircraft measurements of brown carbon from large wildfires in the western United States. We compare two methods for measuring brown carbon and study the evolution of brown carbon in the smoke as it moved away from the burning regions.
Wei Li and Yuxuan Wang
Atmos. Chem. Phys., 22, 7843–7859, https://doi.org/10.5194/acp-22-7843-2022, https://doi.org/10.5194/acp-22-7843-2022, 2022
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Fine dust is an important component of PM2.5 and can be largely modulated by droughts. In contrast to the increase in dust in the southwest USA where major dust sources are located, dust in the southeast USA is affected more by long-range transport from Africa and decreases under droughts. Both the transport and emissions of African dust are weakened when the southeast USA is under droughts, which reveals how regional-scale droughts can influence aerosol abundance through long-range transport.
Li Liu, Ye Kuang, Miaomiao Zhai, Biao Xue, Yao He, Jun Tao, Biao Luo, Wanyun Xu, Jiangchuan Tao, Changqin Yin, Fei Li, Hanbing Xu, Tao Deng, Xuejiao Deng, Haobo Tan, and Min Shao
Atmos. Chem. Phys., 22, 7713–7726, https://doi.org/10.5194/acp-22-7713-2022, https://doi.org/10.5194/acp-22-7713-2022, 2022
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Using simultaneous measurements of a humidified nephelometer system and an aerosol chemical speciation monitor in winter in Guangzhou, the strongest scattering ability of more oxidized oxygenated organic aerosol (MOOA) among aerosol components considering their dry-state scattering ability and water uptake ability was revealed, leading to large impacts of MOOA on visibility degradation. This has important implications for visibility improvement in China and aerosol radiative effect simulation.
Michaël Sicard, Daniel Camilo Fortunato dos Santos Oliveira, Constantino Muñoz-Porcar, Cristina Gil-Díaz, Adolfo Comerón, Alejandro Rodríguez-Gómez, and Federico Dios Otín
Atmos. Chem. Phys., 22, 7681–7697, https://doi.org/10.5194/acp-22-7681-2022, https://doi.org/10.5194/acp-22-7681-2022, 2022
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Atmospheric particles can absorb water vapor, and this water uptake may change their properties, e.g., their size. In the coastal region of Barcelona, Spain, we observe that (1) smaller particles absorb more water vapor, in relative terms, than larger particles and (2) the particle capacity to absorb water vapor has no annual tendency, probably because the site background is quite constant (urban + marine aerosol regime).
Cyril Brunner, Benjamin T. Brem, Martine Collaud Coen, Franz Conen, Martin Steinbacher, Martin Gysel-Beer, and Zamin A. Kanji
Atmos. Chem. Phys., 22, 7557–7573, https://doi.org/10.5194/acp-22-7557-2022, https://doi.org/10.5194/acp-22-7557-2022, 2022
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Microscopic particles called ice-nucleating particles (INPs) are essential for ice crystals to form in clouds. INPs are a tiny proportion of atmospheric aerosol, and their abundance is poorly constrained. We study how the concentration of INPs changes diurnally and seasonally at a mountaintop station in central Europe. Unsurprisingly, a diurnal cycle is only found when considering air masses that have had lower-altitude ground contact. The highest INP concentrations occur in spring.
Zixuan Jia, Ruth M. Doherty, Carlos Ordóñez, Chaofan Li, Oliver Wild, Shipra Jain, and Xiao Tang
Atmos. Chem. Phys., 22, 6471–6487, https://doi.org/10.5194/acp-22-6471-2022, https://doi.org/10.5194/acp-22-6471-2022, 2022
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This study investigates the modulation of daily PM2.5 over three major populated regions in China by regional meteorology and large-scale circulation during winter. These results demonstrate the benefits of considering the large-scale circulation for air quality studies. The novel circulation indices proposed here can explain a considerable fraction of the day-to-day variability of PM2.5 and can be combined with regional meteorology to improve our capability to predict the variability of PM2.5.
Maija Peltola, Clémence Rose, Jonathan V. Trueblood, Sally Gray, Mike Harvey, and Karine Sellegri
Atmos. Chem. Phys., 22, 6231–6254, https://doi.org/10.5194/acp-22-6231-2022, https://doi.org/10.5194/acp-22-6231-2022, 2022
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Despite the importance of marine aerosol measurements for constraining climate models, these measurements are scarce. We measured the aerosol particle number size distribution in coastal New Zealand over a total period of 10 months. This paper analyses the aerosol properties at the site, with a special focus on new particle formation and marine air masses. New particle formation was observed frequently, but in marine air masses it did not follow traditional event criteria.
Liang Ran, Zhaoze Deng, Yunfei Wu, Jiwei Li, Zhixuan Bai, Ye Lu, Deqing Zhuoga, and Jianchun Bian
Atmos. Chem. Phys., 22, 6217–6229, https://doi.org/10.5194/acp-22-6217-2022, https://doi.org/10.5194/acp-22-6217-2022, 2022
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The Tibetan Plateau (TP), the highest plateau in the world, plays a crucial role in regional and global climate. To examine the fingerprint left by human activities on the originally remote atmosphere, size distributions of particles from the ground to about 800 m were measured for the first time in summer 2020 in Lhasa, one of a few urbanized cities on TP. Potential sources of particles at different heights were explored. The contribution of emissions from religious activities was highlighted.
Noah S. Hirshorn, Lauren M. Zuromski, Christopher Rapp, Ian McCubbin, Fangqun Yu, and A. Gannet Hallar
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-338, https://doi.org/10.5194/acp-2022-338, 2022
Revised manuscript accepted for ACP
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New particle formation (NPF) is a source of atmospheric aerosol number concentration that can impact climate by growing to larger sizes and under proper conditions, forming cloud condensation nuclei (CCN). Using novel methods, we find that at Storm Peak Laboratory, a remote mountaintop site in Colorado, NPF is observed to enhance CCN concentrations in the spring by a factor of 1.54 and in the winter by a factor of 1.36 which can occur on a regional scale having important climate implications.
Russell J. Perkins, Peter J. Marinescu, Ezra J. T. Levin, Don R. Collins, and Sonia M. Kreidenweis
Atmos. Chem. Phys., 22, 6197–6215, https://doi.org/10.5194/acp-22-6197-2022, https://doi.org/10.5194/acp-22-6197-2022, 2022
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We used 5 years (2009–2013) of aerosol and cloud condensation nuclei (CCN) data from a total of seven instruments housed at the Southern Great Plains site, which were merged into a quality-controlled, continuous dataset of CCN spectra at ~45 min resolution. The data cover all seasons, are representative of a rural, agricultural mid-continental site, and are useful for model initialization and validation. Our analysis of this dataset focuses on seasonal and hourly variability.
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