Articles | Volume 24, issue 18
https://doi.org/10.5194/acp-24-10815-2024
https://doi.org/10.5194/acp-24-10815-2024
Research article
 | 
26 Sep 2024
Research article |  | 26 Sep 2024

Two distinct ship emission profiles for organic-sulfate source apportionment of PM in sulfur emission control areas

Kirsten N. Fossum, Chunshui Lin, Niall O'Sullivan, Lu Lei, Stig Hellebust, Darius Ceburnis, Aqeel Afzal, Anja Tremper, David Green, Srishti Jain, Steigvilė Byčenkienė, Colin O'Dowd, John Wenger, and Jurgita Ovadnevaite

Related authors

Marine Organic Aerosols at Mace Head: Effects from Phytoplankton and Source Region Variability
Emmanuel Chevassus, Kirsten N. Fossum, Darius Ceburnis, Lu Lei, Chunshui Lin, Wei Xu, Colin D. O’ Dowd, and Jurgita Ovadnevaite
EGUsphere, https://doi.org/10.5194/egusphere-2024-2890,https://doi.org/10.5194/egusphere-2024-2890, 2024
Short summary

Related subject area

Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
The critical role of aqueous-phase processes in aromatic-derived nitrogen-containing organic aerosol formation in cities with different energy consumption patterns
Yi-Jia Ma, Yu Xu, Ting Yang, Lin Gui, Hong-Wei Xiao, Hao Xiao, and Hua-Yun Xiao
Atmos. Chem. Phys., 25, 2763–2780, https://doi.org/10.5194/acp-25-2763-2025,https://doi.org/10.5194/acp-25-2763-2025, 2025
Short summary
Characterization of atmospheric water-soluble brown carbon in the Athabasca oil sands region, Canada
Dane Blanchard, Mark Gordon, Duc Huy Dang, Paul Andrew Makar, and Julian Aherne
Atmos. Chem. Phys., 25, 2423–2442, https://doi.org/10.5194/acp-25-2423-2025,https://doi.org/10.5194/acp-25-2423-2025, 2025
Short summary
Sensitivity of aerosol and cloud properties to coupling strength of marine boundary layer clouds over the northwest Atlantic
Kira Zeider, Kayla McCauley, Sanja Dmitrovic, Leong Wai Siu, Yonghoon Choi, Ewan C. Crosbie, Joshua P. DiGangi, Glenn S. Diskin, Simon Kirschler, John B. Nowak, Michael A. Shook, Kenneth L. Thornhill, Christiane Voigt, Edward L. Winstead, Luke D. Ziemba, Paquita Zuidema, and Armin Sorooshian
Atmos. Chem. Phys., 25, 2407–2422, https://doi.org/10.5194/acp-25-2407-2025,https://doi.org/10.5194/acp-25-2407-2025, 2025
Short summary
Burning conditions and transportation pathways determine biomass-burning aerosol properties in the Ascension Island marine boundary layer
Amie Dobracki, Ernie R. Lewis, Arthur J. Sedlacek III, Tyler Tatro, Maria A. Zawadowicz, and Paquita Zuidema
Atmos. Chem. Phys., 25, 2333–2363, https://doi.org/10.5194/acp-25-2333-2025,https://doi.org/10.5194/acp-25-2333-2025, 2025
Short summary
Observations of high-time-resolution and size-resolved aerosol chemical composition and microphysics in the central Arctic: implications for climate-relevant particle properties
Benjamin Heutte, Nora Bergner, Hélène Angot, Jakob B. Pernov, Lubna Dada, Jessica A. Mirrielees, Ivo Beck, Andrea Baccarini, Matthew Boyer, Jessie M. Creamean, Kaspar R. Daellenbach, Imad El Haddad, Markus M. Frey, Silvia Henning, Tiia Laurila, Vaios Moschos, Tuukka Petäjä, Kerri A. Pratt, Lauriane L. J. Quéléver, Matthew D. Shupe, Paul Zieger, Tuija Jokinen, and Julia Schmale
Atmos. Chem. Phys., 25, 2207–2241, https://doi.org/10.5194/acp-25-2207-2025,https://doi.org/10.5194/acp-25-2207-2025, 2025
Short summary

Cited articles

Agrawal, H., Eden, R., Zhang, X., Fine, P. M., Katzenstein, A., Miller, J. W., Ospital, J., Teffera, S., and Cocker III, D. R.: Primary Particulate Matter from Ocean-Going Engines in the Southern California Air Basin, Environ. Sci. Technol., 43, 5398–5402, https://doi.org/10.1021/es8035016, 2009. 
Anders, L., Schade, J., Rosewig, E. I., Kroeger-Badge, T., Irsig, R., Jeong, S., Bendl, J., Saraji-Bozorgzad, M., Huang, J.-H., Zhang, F.-Y., Wang, C. C., Adam, T., Sklorz, M., Etzien, U., Buchholz, B., Czech, H., Streibel, T., Passig, J., and Zimmermann, R.: Detection of Ship Emissions from Distillate Fuel Operation via Single-Particle Profiling of Polycyclic Aromatic Hydrocarbons, Environmental Science: Atmospheres, 3, 1134–1144, https://doi.org/10.1039/D3EA00056G, 2023. 
Anderson, M., Salo, K., Hallquist, Å. M., and Fridell, E.: Characterization of particles from a marine engine operating at low loads, Atmos. Environ., 101, 65–71, https://doi.org/10.1016/j.atmosenv.2014.11.009, 2015. 
Canonaco, F., Crippa, M., Slowik, J. G., Baltensperger, U., and Prévôt, A. S. H.: SoFi, an IGOR-based interface for the efficient use of the generalized multilinear engine (ME-2) for the source apportionment: ME-2 application to aerosol mass spectrometer data, Atmos. Meas. Tech., 6, 3649–3661, https://doi.org/10.5194/amt-6-3649-2013, 2013. 
Download
Short summary
The chemical composition and sources of submicron aerosol in the Dublin Port area were investigated over a month-long campaign. Two distinct types of ship emissions were identified and characterised: sulfate-rich plumes from the use of heavy fuel oil with scrubbers and organic-rich plumes from the use of low-sulfur fuels. The latter were more frequent, emitting double the particle number and having a typical V / Ni ratio for ship emission.
Share
Altmetrics
Final-revised paper
Preprint