Articles | Volume 23, issue 2
https://doi.org/10.5194/acp-23-1769-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-1769-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
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01 Feb 2023
Research article | Highlight paper |
| 01 Feb 2023
| 01 Feb 2023
Projected increases in wildfires may challenge regulatory curtailment of PM2.5 over the eastern US by 2050
Chandan Sarangi
CORRESPONDING AUTHOR
Department of Civil Engineering, Indian Institute of Technology Madras, Chennai, India
Center for Atmospheric and Climate Sciences, Indian Institute of Technology Madras, Chennai,
India
Pacific Northwest National Laboratory, Richland, WA 99352, USA
Yun Qian
CORRESPONDING AUTHOR
Pacific Northwest National Laboratory, Richland, WA 99352, USA
L. Ruby Leung
Pacific Northwest National Laboratory, Richland, WA 99352, USA
Yang Zhang
Department of Civil and Environmental Engineering, Northeastern
University, Boston, MA 30332, USA
Yufei Zou
Pacific Northwest National Laboratory, Richland, WA 99352, USA
Yuhang Wang
School of Earth and Atmospheric Sciences, Georgia Institute of
Technology, Atlanta, GA 02115, USA
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Jianfeng Li, Andrew Geiss, Zhe Feng, L. Ruby Leung, Yun Qian, and Wenjun Cui
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-112, https://doi.org/10.5194/essd-2024-112, 2024
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Huilin Huang, Yun Qian, Gautam Bisht, Jiali Wang, Tirthankar Chakraborty, Dalei Hao, Jianfeng Li, Travis Thurber, Balwinder Singh, Zhao Yang, Ye Liu, Pengfei Xue, William Sacks, Ethan Coon, and Robert Hetland
EGUsphere, https://doi.org/10.5194/egusphere-2024-1555, https://doi.org/10.5194/egusphere-2024-1555, 2024
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We integrate E3SM land model (ELM) with the WRF Model through the Lightweight Infrastructure for Land Atmosphere Coupling (LILAC) – Earth System Modeling Framework (ESMF). This framework includes a top-level driver, LILAC, for variable communication between WRF and ELM, and ESMF caps for ELM initialization, execution, and finalization. The LILAC-ESMF framework maintains the integrity of the ELM’s source code structure and facilitates the transfer of future developments in LSMs to WRF-ELM.
Tapio Schneider, L. Ruby Leung, and Robert C. J. Wills
Atmos. Chem. Phys., 24, 7041–7062, https://doi.org/10.5194/acp-24-7041-2024, https://doi.org/10.5194/acp-24-7041-2024, 2024
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Climate models are crucial for predicting climate change in detail. This paper proposes a balanced approach to improving their accuracy by combining traditional process-based methods with modern artificial intelligence (AI) techniques while maximizing the resolution to allow for ensemble simulations. The authors propose using AI to learn from both observational and simulated data while incorporating existing physical knowledge to reduce data demands and improve climate prediction reliability.
Lingcheng Li, Gautam Bisht, Dalei Hao, and L. Ruby Leung
Earth Syst. Sci. Data, 16, 2007–2032, https://doi.org/10.5194/essd-16-2007-2024, https://doi.org/10.5194/essd-16-2007-2024, 2024
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This study fills a gap to meet the emerging needs of kilometer-scale Earth system modeling by developing global 1 km land surface parameters for land use, vegetation, soil, and topography. Our demonstration simulations highlight the substantial impacts of these parameters on spatial variability and information loss in water and energy simulations. Using advanced explainable machine learning methods, we identified influential factors driving spatial variability and information loss.
Bryce E. Harrop, Jian Lu, L. Ruby Leung, William K. M. Lau, Kyu-Myong Kim, Brian Medeiros, Brian J. Soden, Gabriel A. Vecchi, Bosong Zhang, and Balwinder Singh
Geosci. Model Dev., 17, 3111–3135, https://doi.org/10.5194/gmd-17-3111-2024, https://doi.org/10.5194/gmd-17-3111-2024, 2024
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Weiming Ma, Hailong Wang, Gang Chen, Yun Qian, Ian Baxter, Yiling Huo, and Mark W. Seefeldt
Atmos. Chem. Phys., 24, 4451–4472, https://doi.org/10.5194/acp-24-4451-2024, https://doi.org/10.5194/acp-24-4451-2024, 2024
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Extreme warming events with surface temperature going above 0°C can occur in the high-Arctic winter. Although reanalysis data show that these events were short-lived and occurred rarely during 1980–2021, they have become more frequent, stronger, and longer lasting latterly. A dipole pattern, comprising high- and low-pressure systems, is found to be the key in driving them. These findings have implications for the recent changes in sea ice, hydrological cycle, and ecosystem over the Arctic.
Pengfei Shi, L. Ruby Leung, Bin Wang, Kai Zhang, Samson M. Hagos, and Shixuan Zhang
Geosci. Model Dev., 17, 3025–3040, https://doi.org/10.5194/gmd-17-3025-2024, https://doi.org/10.5194/gmd-17-3025-2024, 2024
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Improving climate predictions have profound socio-economic impacts. This study introduces a new weakly coupled land data assimilation (WCLDA) system for a coupled climate model. We demonstrate improved simulation of soil moisture and temperature in many global regions and throughout the soil layers. Furthermore, significant improvements are also found in reproducing the time evolution of the 2012 US Midwest drought. The WCLDA system provides the groundwork for future predictability studies.
Lingbo Li, Hong-Yi Li, Guta Abeshu, Jinyun Tang, L. Ruby Leung, Chang Liao, Zeli Tan, Hanqin Tian, Peter Thornton, and Xiaojuan Yang
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-43, https://doi.org/10.5194/essd-2024-43, 2024
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We have developed a new map that reveals how organic carbon from soil leaches into headwater streams over the contiguous United States. We use advanced artificial intelligence techniques and a massive amount of data, including observations at over 2,500 gauges and a wealth of climate and environmental information. The map is a critical step in understanding and predicting how carbon moves through our environment, hence a useful tool for tackling climate challenges.
Yawen Liu, Yun Qian, Philip J. Rasch, Kai Zhang, Lai-yung Ruby Leung, Yuhang Wang, Minghuai Wang, Hailong Wang, Xin Huang, and Xiu-Qun Yang
Atmos. Chem. Phys., 24, 3115–3128, https://doi.org/10.5194/acp-24-3115-2024, https://doi.org/10.5194/acp-24-3115-2024, 2024
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Fire management has long been a challenge. Here we report that spring-peak fire activity over southern Mexico and Central America (SMCA) has a distinct quasi-biennial signal by measuring multiple fire metrics. This signal is initially driven by quasi-biennial variability in precipitation and is further amplified by positive feedback of fire–precipitation interaction at short timescales. This work highlights the importance of fire–climate interactions in shaping fires on an interannual scale.
Donghui Xu, Gautam Bisht, Zeli Tan, Chang Liao, Tian Zhou, Hong-Yi Li, and L. Ruby Leung
Geosci. Model Dev., 17, 1197–1215, https://doi.org/10.5194/gmd-17-1197-2024, https://doi.org/10.5194/gmd-17-1197-2024, 2024
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We aim to disentangle the hydrological and hydraulic controls on streamflow variability in a fully coupled earth system model. We found that calibrating only one process (i.e., traditional calibration procedure) will result in unrealistic parameter values and poor performance of the water cycle, while the simulated streamflow is improved. To address this issue, we further proposed a two-step calibration procedure to reconcile the impacts from hydrological and hydraulic processes on streamflow.
Yuying Zhang, Shaocheng Xie, Yi Qin, Wuyin Lin, Jean-Christophe Golaz, Xue Zheng, Po-Lun Ma, Yun Qian, Qi Tang, Christopher R. Terai, and Meng Zhang
Geosci. Model Dev., 17, 169–189, https://doi.org/10.5194/gmd-17-169-2024, https://doi.org/10.5194/gmd-17-169-2024, 2024
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We performed systematic evaluation of clouds simulated in the Energy
Exascale Earth System Model (E3SMv2) to document model performance and understand what updates in E3SMv2 have caused changes in clouds from E3SMv1 to E3SMv2. We find that stratocumulus clouds along the subtropical west coast of continents are dramatically improved, primarily due to the retuning done in CLUBB. This study offers additional insights into clouds simulated in E3SMv2 and will benefit future E3SM developments.
Exascale Earth System Model (E3SMv2) to document model performance and understand what updates in E3SMv2 have caused changes in clouds from E3SMv1 to E3SMv2. We find that stratocumulus clouds along the subtropical west coast of continents are dramatically improved, primarily due to the retuning done in CLUBB. This study offers additional insights into clouds simulated in E3SMv2 and will benefit future E3SM developments.
Calvin Howes, Pablo E. Saide, Hugh Coe, Amie Dobracki, Steffen Freitag, Jim M. Haywood, Steven G. Howell, Siddhant Gupta, Janek Uin, Mary Kacarab, Chongai Kuang, L. Ruby Leung, Athanasios Nenes, Greg M. McFarquhar, James Podolske, Jens Redemann, Arthur J. Sedlacek, Kenneth L. Thornhill, Jenny P. S. Wong, Robert Wood, Huihui Wu, Yang Zhang, Jianhao Zhang, and Paquita Zuidema
Atmos. Chem. Phys., 23, 13911–13940, https://doi.org/10.5194/acp-23-13911-2023, https://doi.org/10.5194/acp-23-13911-2023, 2023
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To better understand smoke properties and its interactions with clouds, we compare the WRF-CAM5 model with observations from ORACLES, CLARIFY, and LASIC field campaigns in the southeastern Atlantic in August 2017. The model transports and mixes smoke well but does not fully capture some important processes. These include smoke chemical and physical aging over 4–12 days, smoke removal by rain, sulfate particle formation, aerosol activation into cloud droplets, and boundary layer turbulence.
Dongyu Feng, Zeli Tan, Donghui Xu, and L. Ruby Leung
Hydrol. Earth Syst. Sci., 27, 3911–3934, https://doi.org/10.5194/hess-27-3911-2023, https://doi.org/10.5194/hess-27-3911-2023, 2023
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This study assesses the flood risks concurrently induced by river flooding and coastal storm surge along the coast of the contiguous United States using statistical and numerical models. We reveal a few hotspots of such risks, the critical spatial variabilities within a river basin and over the whole US coast, and the uncertainties of the risk assessment. We highlight the importance of weighing different risk measures to avoid underestimating or exaggerating the compound flood impacts.
Chupeng Zhang, Shangfei Hai, Yang Gao, Yuhang Wang, Shaoqing Zhang, Lifang Sheng, Bin Zhao, Shuxiao Wang, Jingkun Jiang, Xin Huang, Xiaojing Shen, Junying Sun, Aura Lupascu, Manish Shrivastava, Jerome D. Fast, Wenxuan Cheng, Xiuwen Guo, Ming Chu, Nan Ma, Juan Hong, Qiaoqiao Wang, Xiaohong Yao, and Huiwang Gao
Atmos. Chem. Phys., 23, 10713–10730, https://doi.org/10.5194/acp-23-10713-2023, https://doi.org/10.5194/acp-23-10713-2023, 2023
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New particle formation is an important source of atmospheric particles, exerting critical influences on global climate. Numerical models are vital tools to understanding atmospheric particle evolution, which, however, suffer from large biases in simulating particle numbers. Here we improve the model chemical processes governing particle sizes and compositions. The improved model reveals substantial contributions of newly formed particles to climate through effects on cloud condensation nuclei.
Zhenxin Liu, Yuanhao Chen, Yuhang Wang, Cheng Liu, Shuhua Liu, and Hong Liao
Geosci. Model Dev., 16, 4385–4403, https://doi.org/10.5194/gmd-16-4385-2023, https://doi.org/10.5194/gmd-16-4385-2023, 2023
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The heterogeneous layout of urban buildings leads to the complex wind field in and over the urban canopy. Large discrepancies between the observations and the current simulations result from misunderstanding the character of the wind field. The Inhomogeneous Wind Scheme in Urban Street (IWSUS) was developed to simulate the heterogeneity of the wind speed in a typical street and then improve the simulated energy budget in the lower atmospheric layer over the urban canopy.
Lingcheng Li, Yilin Fang, Zhonghua Zheng, Mingjie Shi, Marcos Longo, Charles D. Koven, Jennifer A. Holm, Rosie A. Fisher, Nate G. McDowell, Jeffrey Chambers, and L. Ruby Leung
Geosci. Model Dev., 16, 4017–4040, https://doi.org/10.5194/gmd-16-4017-2023, https://doi.org/10.5194/gmd-16-4017-2023, 2023
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Accurately modeling plant coexistence in vegetation demographic models like ELM-FATES is challenging. This study proposes a repeatable method that uses machine-learning-based surrogate models to optimize plant trait parameters in ELM-FATES. Our approach significantly improves plant coexistence modeling, thus reducing errors. It has important implications for modeling ecosystem dynamics in response to climate change.
Qi Tang, Jean-Christophe Golaz, Luke P. Van Roekel, Mark A. Taylor, Wuyin Lin, Benjamin R. Hillman, Paul A. Ullrich, Andrew M. Bradley, Oksana Guba, Jonathan D. Wolfe, Tian Zhou, Kai Zhang, Xue Zheng, Yunyan Zhang, Meng Zhang, Mingxuan Wu, Hailong Wang, Cheng Tao, Balwinder Singh, Alan M. Rhoades, Yi Qin, Hong-Yi Li, Yan Feng, Yuying Zhang, Chengzhu Zhang, Charles S. Zender, Shaocheng Xie, Erika L. Roesler, Andrew F. Roberts, Azamat Mametjanov, Mathew E. Maltrud, Noel D. Keen, Robert L. Jacob, Christiane Jablonowski, Owen K. Hughes, Ryan M. Forsyth, Alan V. Di Vittorio, Peter M. Caldwell, Gautam Bisht, Renata B. McCoy, L. Ruby Leung, and David C. Bader
Geosci. Model Dev., 16, 3953–3995, https://doi.org/10.5194/gmd-16-3953-2023, https://doi.org/10.5194/gmd-16-3953-2023, 2023
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High-resolution simulations are superior to low-resolution ones in capturing regional climate changes and climate extremes. However, uniformly reducing the grid size of a global Earth system model is too computationally expensive. We provide an overview of the fully coupled regionally refined model (RRM) of E3SMv2 and document a first-of-its-kind set of climate production simulations using RRM at an economic cost. The key to this success is our innovative hybrid time step method.
Koichi Sakaguchi, L. Ruby Leung, Colin M. Zarzycki, Jihyeon Jang, Seth McGinnis, Bryce E. Harrop, William C. Skamarock, Andrew Gettelman, Chun Zhao, William J. Gutowski, Stephen Leak, and Linda Mearns
Geosci. Model Dev., 16, 3029–3081, https://doi.org/10.5194/gmd-16-3029-2023, https://doi.org/10.5194/gmd-16-3029-2023, 2023
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We document details of the regional climate downscaling dataset produced by a global variable-resolution model. The experiment is unique in that it follows a standard protocol designed for coordinated experiments of regional models. We found negligible influence of post-processing on statistical analysis, importance of simulation quality outside of the target region, and computational challenges that our model code faced due to rapidly changing super computer systems.
Zhe Feng, Joseph Hardin, Hannah C. Barnes, Jianfeng Li, L. Ruby Leung, Adam Varble, and Zhixiao Zhang
Geosci. Model Dev., 16, 2753–2776, https://doi.org/10.5194/gmd-16-2753-2023, https://doi.org/10.5194/gmd-16-2753-2023, 2023
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PyFLEXTRKR is a flexible atmospheric feature tracking framework with specific capabilities to track convective clouds from a variety of observations and model simulations. The package has a collection of multi-object identification algorithms and has been optimized for large datasets. This paper describes the algorithms and demonstrates applications for tracking deep convective cells and mesoscale convective systems from observations and model simulations at a wide range of scales.
Zeyu Xue, Paul Ullrich, and Lai-Yung Ruby Leung
Hydrol. Earth Syst. Sci., 27, 1909–1927, https://doi.org/10.5194/hess-27-1909-2023, https://doi.org/10.5194/hess-27-1909-2023, 2023
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We examine the sensitivity and robustness of conclusions drawn from the PGW method over the NEUS by conducting multiple PGW experiments and varying the perturbation spatial scales and choice of perturbed meteorological variables to provide a guideline for this increasingly popular regional modeling method. Overall, we recommend PGW experiments be performed with perturbations to temperature or the combination of temperature and wind at the gridpoint scale, depending on the research question.
Dalei Hao, Gautam Bisht, Karl Rittger, Timbo Stillinger, Edward Bair, Yu Gu, and L. Ruby Leung
The Cryosphere, 17, 673–697, https://doi.org/10.5194/tc-17-673-2023, https://doi.org/10.5194/tc-17-673-2023, 2023
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We comprehensively evaluated the snow simulations in E3SM land model over the western United States in terms of spatial patterns, temporal correlations, interannual variabilities, elevation gradients, and change with forest cover of snow properties and snow phenology. Our study underscores the need for diagnosing model biases and improving the model representations of snow properties and snow phenology in mountainous areas for more credible simulation and future projection of mountain snowpack.
Dalei Hao, Gautam Bisht, Karl Rittger, Edward Bair, Cenlin He, Huilin Huang, Cheng Dang, Timbo Stillinger, Yu Gu, Hailong Wang, Yun Qian, and L. Ruby Leung
Geosci. Model Dev., 16, 75–94, https://doi.org/10.5194/gmd-16-75-2023, https://doi.org/10.5194/gmd-16-75-2023, 2023
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Snow with the highest albedo of land surface plays a vital role in Earth’s surface energy budget and water cycle. This study accounts for the impacts of snow grain shape and mixing state of light-absorbing particles with snow on snow albedo in the E3SM land model. The findings advance our understanding of the role of snow grain shape and mixing state of LAP–snow in land surface processes and offer guidance for improving snow simulations and radiative forcing estimates in Earth system models.
Huilin Huang, Yun Qian, Ye Liu, Cenlin He, Jianyu Zheng, Zhibo Zhang, and Antonis Gkikas
Atmos. Chem. Phys., 22, 15469–15488, https://doi.org/10.5194/acp-22-15469-2022, https://doi.org/10.5194/acp-22-15469-2022, 2022
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Using a clustering method developed in the field of artificial neural networks, we identify four typical dust transport patterns across the Sierra Nevada, associated with the mesoscale and regional-scale wind circulations. Our results highlight the connection between dust transport and dominant weather patterns, which can be used to understand dust transport in a changing climate.
Dongyu Feng, Zeli Tan, Darren Engwirda, Chang Liao, Donghui Xu, Gautam Bisht, Tian Zhou, Hong-Yi Li, and L. Ruby Leung
Hydrol. Earth Syst. Sci., 26, 5473–5491, https://doi.org/10.5194/hess-26-5473-2022, https://doi.org/10.5194/hess-26-5473-2022, 2022
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Sea level rise, storm surge and river discharge can cause coastal backwater effects in downstream sections of rivers, creating critical flood risks. This study simulates the backwater effects using a large-scale river model on a coastal-refined computational mesh. By decomposing the backwater drivers, we revealed their relative importance and long-term variations. Our analysis highlights the increasing strength of backwater effects due to sea level rise and more frequent storm surge.
Yilin Fang, L. Ruby Leung, Charles D. Koven, Gautam Bisht, Matteo Detto, Yanyan Cheng, Nate McDowell, Helene Muller-Landau, S. Joseph Wright, and Jeffrey Q. Chambers
Geosci. Model Dev., 15, 7879–7901, https://doi.org/10.5194/gmd-15-7879-2022, https://doi.org/10.5194/gmd-15-7879-2022, 2022
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We develop a model that integrates an Earth system model with a three-dimensional hydrology model to explicitly resolve hillslope topography and water flow underneath the land surface to understand how local-scale hydrologic processes modulate vegetation along water availability gradients. Our coupled model can be used to improve the understanding of the diverse impact of local heterogeneity and water flux on nutrient availability and plant communities.
Zhenqi Xu, Wei Feng, Yicheng Wang, Haoran Ye, Yuhang Wang, Hong Liao, and Mingjie Xie
Atmos. Chem. Phys., 22, 13739–13752, https://doi.org/10.5194/acp-22-13739-2022, https://doi.org/10.5194/acp-22-13739-2022, 2022
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This work uses a solvent (DMF) that can efficiently dissolve low-volatility OC to examine BrC absorption and sources, which will benefit future investigations on the physicochemical properties of large organic molecules. The study results also shed light on potential sources for methanol-insoluble OC. These results highlight the importance of testing different solvents to investigate the structures and light absorption of low-volatility BrC.
Youngseob Kim, Lya Lugon, Alice Maison, Thibaud Sarica, Yelva Roustan, Myrto Valari, Yang Zhang, Michel André, and Karine Sartelet
Geosci. Model Dev., 15, 7371–7396, https://doi.org/10.5194/gmd-15-7371-2022, https://doi.org/10.5194/gmd-15-7371-2022, 2022
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This paper presents the latest version of the street-network model MUNICH, v2.0. The description of MUNICH v1.0, which models gas-phase pollutants in a street network, was published in GMD in 2018. Since then, major modifications have been made to MUNICH. The comprehensive aerosol model SSH-aerosol is now coupled to MUNICH to simulate primary and secondary aerosol concentrations. New parameterisations have also been introduced. Test cases are defined to illustrate the new model functionalities.
Meng Huang, Po-Lun Ma, Nathaniel W. Chaney, Dalei Hao, Gautam Bisht, Megan D. Fowler, Vincent E. Larson, and L. Ruby Leung
Geosci. Model Dev., 15, 6371–6384, https://doi.org/10.5194/gmd-15-6371-2022, https://doi.org/10.5194/gmd-15-6371-2022, 2022
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The land surface in one grid cell may be diverse in character. This study uses an explicit way to account for that subgrid diversity in a state-of-the-art Earth system model (ESM) and explores its implications for the overlying atmosphere. We find that the shallow clouds are increased significantly with the land surface diversity. Our work highlights the importance of accurately representing the land surface and its interaction with the atmosphere in next-generation ESMs.
Yilin Fang, L. Ruby Leung, Ryan Knox, Charlie Koven, and Ben Bond-Lamberty
Geosci. Model Dev., 15, 6385–6398, https://doi.org/10.5194/gmd-15-6385-2022, https://doi.org/10.5194/gmd-15-6385-2022, 2022
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Accounting for water movement in the soil and water transport within the plant is important for plant growth in Earth system modeling. We implemented different numerical approaches for a plant hydrodynamic model and compared their impacts on the simulated aboveground biomass (AGB) at single points and globally. We found care should be taken when discretizing the number of soil layers for numerical simulations as it can significantly affect AGB if accuracy and computational costs are of concern.
Sol Kim, L. Ruby Leung, Bin Guan, and John C. H. Chiang
Geosci. Model Dev., 15, 5461–5480, https://doi.org/10.5194/gmd-15-5461-2022, https://doi.org/10.5194/gmd-15-5461-2022, 2022
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The Energy Exascale Earth System Model (E3SM) project is a state-of-the-science Earth system model developed by the US Department of Energy (DOE). Understanding how the water cycle behaves in this model is of particular importance to the DOE’s mission. Atmospheric rivers (ARs) – which are crucial to the global water cycle – move vast amounts of water vapor through the sky and produce rain and snow. We find that this model reliably represents atmospheric rivers around the world.
Lingcheng Li, Gautam Bisht, and L. Ruby Leung
Geosci. Model Dev., 15, 5489–5510, https://doi.org/10.5194/gmd-15-5489-2022, https://doi.org/10.5194/gmd-15-5489-2022, 2022
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Land surface heterogeneity plays a critical role in the terrestrial water, energy, and biogeochemical cycles. Our study systematically quantified the effects of four dominant heterogeneity sources on water and energy partitioning via Sobol' indices. We found that atmospheric forcing and land use land cover are the most dominant heterogeneity sources in determining spatial variability of water and energy partitioning. Our findings can help prioritize the future development of land surface models.
Kai Zhang, Wentao Zhang, Hui Wan, Philip J. Rasch, Steven J. Ghan, Richard C. Easter, Xiangjun Shi, Yong Wang, Hailong Wang, Po-Lun Ma, Shixuan Zhang, Jian Sun, Susannah M. Burrows, Manish Shrivastava, Balwinder Singh, Yun Qian, Xiaohong Liu, Jean-Christophe Golaz, Qi Tang, Xue Zheng, Shaocheng Xie, Wuyin Lin, Yan Feng, Minghuai Wang, Jin-Ho Yoon, and L. Ruby Leung
Atmos. Chem. Phys., 22, 9129–9160, https://doi.org/10.5194/acp-22-9129-2022, https://doi.org/10.5194/acp-22-9129-2022, 2022
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Here we analyze the effective aerosol forcing simulated by E3SM version 1 using both century-long free-running and short nudged simulations. The aerosol forcing in E3SMv1 is relatively large compared to other models, mainly due to the large indirect aerosol effect. Aerosol-induced changes in liquid and ice cloud properties in E3SMv1 have a strong correlation. The aerosol forcing estimates in E3SMv1 are sensitive to the parameterization changes in both liquid and ice cloud processes.
Donghui Xu, Gautam Bisht, Khachik Sargsyan, Chang Liao, and L. Ruby Leung
Geosci. Model Dev., 15, 5021–5043, https://doi.org/10.5194/gmd-15-5021-2022, https://doi.org/10.5194/gmd-15-5021-2022, 2022
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The runoff outputs in Earth system model simulations involve high uncertainty, which needs to be constrained by parameter calibration. In this work, we used a surrogate-assisted Bayesian framework to efficiently calibrate the runoff-generation processes in the Energy Exascale Earth System Model v1 at a global scale. The model performance was improved compared to the default parameter after calibration, and the associated parametric uncertainty was significantly constrained.
Yun Lin, Jiwen Fan, Pengfei Li, Lai-yung Ruby Leung, Paul J. DeMott, Lexie Goldberger, Jennifer Comstock, Ying Liu, Jong-Hoon Jeong, and Jason Tomlinson
Atmos. Chem. Phys., 22, 6749–6771, https://doi.org/10.5194/acp-22-6749-2022, https://doi.org/10.5194/acp-22-6749-2022, 2022
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How sea spray aerosols may affect cloud and precipitation over the region by acting as ice-nucleating particles (INPs) is unknown. We explored the effects of INPs from marine aerosols on orographic cloud and precipitation for an atmospheric river event observed during the 2015 ACAPEX field campaign. The marine INPs enhance the formation of ice and snow, leading to less shallow warm clouds but more mixed-phase and deep clouds. This work suggests models need to consider the impacts of marine INPs.
Pinya Wang, Yang Yang, Huimin Li, Lei Chen, Ruijun Dang, Daokai Xue, Baojie Li, Jianping Tang, L. Ruby Leung, and Hong Liao
Atmos. Chem. Phys., 22, 4705–4719, https://doi.org/10.5194/acp-22-4705-2022, https://doi.org/10.5194/acp-22-4705-2022, 2022
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China is now suffering from both severe ozone (O3) pollution and heat events. We highlight that North China Plain is the hot spot of the co-occurrences of extremes in O3 and high temperatures in China. Such coupled extremes exhibit an increasing trend during 2014–2019 and will continue to increase until the middle of this century. And the coupled extremes impose more severe health impacts to human than O3 pollution occurring alone because of elevated O3 levels and temperatures.
Po-Lun Ma, Bryce E. Harrop, Vincent E. Larson, Richard B. Neale, Andrew Gettelman, Hugh Morrison, Hailong Wang, Kai Zhang, Stephen A. Klein, Mark D. Zelinka, Yuying Zhang, Yun Qian, Jin-Ho Yoon, Christopher R. Jones, Meng Huang, Sheng-Lun Tai, Balwinder Singh, Peter A. Bogenschutz, Xue Zheng, Wuyin Lin, Johannes Quaas, Hélène Chepfer, Michael A. Brunke, Xubin Zeng, Johannes Mülmenstädt, Samson Hagos, Zhibo Zhang, Hua Song, Xiaohong Liu, Michael S. Pritchard, Hui Wan, Jingyu Wang, Qi Tang, Peter M. Caldwell, Jiwen Fan, Larry K. Berg, Jerome D. Fast, Mark A. Taylor, Jean-Christophe Golaz, Shaocheng Xie, Philip J. Rasch, and L. Ruby Leung
Geosci. Model Dev., 15, 2881–2916, https://doi.org/10.5194/gmd-15-2881-2022, https://doi.org/10.5194/gmd-15-2881-2022, 2022
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An alternative set of parameters for E3SM Atmospheric Model version 1 has been developed based on a tuning strategy that focuses on clouds. When clouds in every regime are improved, other aspects of the model are also improved, even though they are not the direct targets for calibration. The recalibrated model shows a lower sensitivity to anthropogenic aerosols and surface warming, suggesting potential improvements to the simulated climate in the past and future.
Chandan Sarangi, TC Chakraborty, Sachchidanand Tripathi, Mithun Krishnan, Ross Morrison, Jonathan Evans, and Lina M. Mercado
Atmos. Chem. Phys., 22, 3615–3629, https://doi.org/10.5194/acp-22-3615-2022, https://doi.org/10.5194/acp-22-3615-2022, 2022
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Transpiration fluxes by vegetation are reduced under heat stress to conserve water. However, in situ observations over northern India show that the strength of the inverse association between transpiration and atmospheric vapor pressure deficit is weakening in the presence of heavy aerosol loading. This finding not only implicates the significant role of aerosols in modifying the evaporative fraction (EF) but also warrants an in-depth analysis of the aerosol–plant–temperature–EF continuum.
Sally S.-C. Wang, Yun Qian, L. Ruby Leung, and Yang Zhang
Atmos. Chem. Phys., 22, 3445–3468, https://doi.org/10.5194/acp-22-3445-2022, https://doi.org/10.5194/acp-22-3445-2022, 2022
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This study develops an interpretable machine learning (ML) model predicting monthly PM2.5 fire emission over the contiguous US at 0.25° resolution and compares the prediction skills of the ML and process-based models. The comparison facilitates attributions of model biases and better understanding of the strengths and uncertainties in the two types of models at regional scales, for informing future model development and their applications in fire emission projection.
Guta Wakbulcho Abeshu, Hong-Yi Li, Zhenduo Zhu, Zeli Tan, and L. Ruby Leung
Earth Syst. Sci. Data, 14, 929–942, https://doi.org/10.5194/essd-14-929-2022, https://doi.org/10.5194/essd-14-929-2022, 2022
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Existing riverbed sediment particle size data are sparsely available at individual sites. We develop a continuous map of median riverbed sediment particle size over the contiguous US corresponding to millions of river segments based on the existing observations and machine learning methods. This map is useful for research in large-scale river sediment using model- and data-driven approaches, teaching environmental and earth system sciences, planning and managing floodplain zones, etc.
Hong-Yi Li, Zeli Tan, Hongbo Ma, Zhenduo Zhu, Guta Wakbulcho Abeshu, Senlin Zhu, Sagy Cohen, Tian Zhou, Donghui Xu, and L. Ruby Leung
Hydrol. Earth Syst. Sci., 26, 665–688, https://doi.org/10.5194/hess-26-665-2022, https://doi.org/10.5194/hess-26-665-2022, 2022
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We introduce a new multi-process river sediment module for Earth system models. Application and validation over the contiguous US indicate a satisfactory model performance over large river systems, including those heavily regulated by reservoirs. This new sediment module enables future modeling of the transportation and transformation of carbon and nutrients carried by the fine sediment along the river–ocean continuum to close the global carbon and nutrient cycles.
Ye Liu, Yun Qian, and Larry K. Berg
Wind Energ. Sci., 7, 37–51, https://doi.org/10.5194/wes-7-37-2022, https://doi.org/10.5194/wes-7-37-2022, 2022
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Uncertainties in initial conditions (ICs) decrease the accuracy of wind speed forecasts. We find that IC uncertainties can alter wind speed by modulating the weather system. IC uncertainties in local thermal gradient and large-scale circulation jointly contribute to wind speed forecast uncertainties. Wind forecast accuracy in the Columbia River Basin is confined by initial uncertainties in a few specific regions, providing useful information for more intense measurement and modeling studies.
Ruili Wu, Christopher W. Tessum, Yang Zhang, Chaopeng Hong, Yixuan Zheng, Xinyin Qin, Shigan Liu, and Qiang Zhang
Geosci. Model Dev., 14, 7621–7638, https://doi.org/10.5194/gmd-14-7621-2021, https://doi.org/10.5194/gmd-14-7621-2021, 2021
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Reduced-complexity air quality models are less computationally intensive and easier to use. We developed a reduced-complexity air quality Intervention Model for Air Pollution over China (InMAP-China) to rapidly predict the air quality and estimate the health impacts of emission sources in China. We believe that this work will be of great interest to a broad audience, including environmentalists in China and scientists in relevant fields at both national and local institutes.
Claudia Tebaldi, Kalyn Dorheim, Michael Wehner, and Ruby Leung
Earth Syst. Dynam., 12, 1427–1501, https://doi.org/10.5194/esd-12-1427-2021, https://doi.org/10.5194/esd-12-1427-2021, 2021
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We address the question of how large an initial condition ensemble of climate model simulations should be if we are concerned with accurately projecting future changes in temperature and precipitation extremes. We find that for most cases (and both models considered), an ensemble of 20–25 members is sufficient for many extreme metrics, spatial scales and time horizons. This may leave computational resources to tackle other uncertainties in climate model simulations with our ensembles.
Kai Wang, Yang Zhang, Shaocai Yu, David C. Wong, Jonathan Pleim, Rohit Mathur, James T. Kelly, and Michelle Bell
Geosci. Model Dev., 14, 7189–7221, https://doi.org/10.5194/gmd-14-7189-2021, https://doi.org/10.5194/gmd-14-7189-2021, 2021
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The two-way coupled WRF-CMAQ model accounting for complex chemistry–meteorology feedbacks has been applied to the long-term predictions of regional meteorology and air quality over the US. The model results show superior performance and importance of chemistry–meteorology feedbacks when compared to the offline coupled WRF and CMAQ simulations, which suggests that feedbacks should be considered along with other factors in developing future model applications to inform policy making.
Dalei Hao, Gautam Bisht, Yu Gu, Wei-Liang Lee, Kuo-Nan Liou, and L. Ruby Leung
Geosci. Model Dev., 14, 6273–6289, https://doi.org/10.5194/gmd-14-6273-2021, https://doi.org/10.5194/gmd-14-6273-2021, 2021
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Topography exerts significant influence on the incoming solar radiation at the land surface. This study incorporated a well-validated sub-grid topographic parameterization in E3SM land model (ELM) version 1.0. The results demonstrate that sub-grid topography has non-negligible effects on surface energy budget, snow cover, and surface temperature over the Tibetan Plateau and that the ELM simulations are sensitive to season, elevation, and spatial scale.
Syuichi Itahashi, Rohit Mathur, Christian Hogrefe, Sergey L. Napelenok, and Yang Zhang
Geosci. Model Dev., 14, 5751–5768, https://doi.org/10.5194/gmd-14-5751-2021, https://doi.org/10.5194/gmd-14-5751-2021, 2021
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The Community Multiscale Air Quality (CMAQ) modeling system extended for hemispheric-scale applications (H-CMAQ) incorporated the satellite-constrained degassing SO2 emissions from 50 volcanos across the Northern Hemisphere. The impact on tropospheric sulfate aerosol (SO42−) is assessed for 2010. Although the considered volcanic emissions occurred at or below the middle of free troposphere (500 hPa), SO42− enhancements of more than 10 % were detected up to the top of free troposphere (250 hPa).
Chao Qin, Yafeng Gou, Yuhang Wang, Yuhao Mao, Hong Liao, Qin'geng Wang, and Mingjie Xie
Atmos. Chem. Phys., 21, 12141–12153, https://doi.org/10.5194/acp-21-12141-2021, https://doi.org/10.5194/acp-21-12141-2021, 2021
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In this study, we found that the aqueous solution in aerosols is an important absorbing phase for gaseous polyols in the atmosphere, indicating that the dissolution in aerosol liquid water should not be ignored when investigating gas–particle partitioning of water-soluble organics. The exponential increase in effective partitioning coefficients of polyol tracers with sulfate ion concentrations could be attributed to organic–inorganic interactions in the particle phase.
Jianfeng Li, Yuhang Wang, Ruixiong Zhang, Charles Smeltzer, Andrew Weinheimer, Jay Herman, K. Folkert Boersma, Edward A. Celarier, Russell W. Long, James J. Szykman, Ruben Delgado, Anne M. Thompson, Travis N. Knepp, Lok N. Lamsal, Scott J. Janz, Matthew G. Kowalewski, Xiong Liu, and Caroline R. Nowlan
Atmos. Chem. Phys., 21, 11133–11160, https://doi.org/10.5194/acp-21-11133-2021, https://doi.org/10.5194/acp-21-11133-2021, 2021
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Comprehensive evaluations of simulated diurnal cycles of NO2 and NOy concentrations, vertical profiles, and tropospheric vertical column densities at two different resolutions with various measurements during the DISCOVER-AQ 2011 campaign show potential distribution biases of NOx emissions in the National Emissions Inventory 2011 at both 36 and 4 km resolutions, providing another possible explanation for the overestimation of model results.
Yongkang Xue, Tandong Yao, Aaron A. Boone, Ismaila Diallo, Ye Liu, Xubin Zeng, William K. M. Lau, Shiori Sugimoto, Qi Tang, Xiaoduo Pan, Peter J. van Oevelen, Daniel Klocke, Myung-Seo Koo, Tomonori Sato, Zhaohui Lin, Yuhei Takaya, Constantin Ardilouze, Stefano Materia, Subodh K. Saha, Retish Senan, Tetsu Nakamura, Hailan Wang, Jing Yang, Hongliang Zhang, Mei Zhao, Xin-Zhong Liang, J. David Neelin, Frederic Vitart, Xin Li, Ping Zhao, Chunxiang Shi, Weidong Guo, Jianping Tang, Miao Yu, Yun Qian, Samuel S. P. Shen, Yang Zhang, Kun Yang, Ruby Leung, Yuan Qiu, Daniele Peano, Xin Qi, Yanling Zhan, Michael A. Brunke, Sin Chan Chou, Michael Ek, Tianyi Fan, Hong Guan, Hai Lin, Shunlin Liang, Helin Wei, Shaocheng Xie, Haoran Xu, Weiping Li, Xueli Shi, Paulo Nobre, Yan Pan, Yi Qin, Jeff Dozier, Craig R. Ferguson, Gianpaolo Balsamo, Qing Bao, Jinming Feng, Jinkyu Hong, Songyou Hong, Huilin Huang, Duoying Ji, Zhenming Ji, Shichang Kang, Yanluan Lin, Weiguang Liu, Ryan Muncaster, Patricia de Rosnay, Hiroshi G. Takahashi, Guiling Wang, Shuyu Wang, Weicai Wang, Xu Zhou, and Yuejian Zhu
Geosci. Model Dev., 14, 4465–4494, https://doi.org/10.5194/gmd-14-4465-2021, https://doi.org/10.5194/gmd-14-4465-2021, 2021
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The subseasonal prediction of extreme hydroclimate events such as droughts/floods has remained stubbornly low for years. This paper presents a new international initiative which, for the first time, introduces spring land surface temperature anomalies over high mountains to improve precipitation prediction through remote effects of land–atmosphere interactions. More than 40 institutions worldwide are participating in this effort. The experimental protocol and preliminary results are presented.
Xiaoyang Chen, Yang Zhang, Kai Wang, Daniel Tong, Pius Lee, Youhua Tang, Jianping Huang, Patrick C. Campbell, Jeff Mcqueen, Havala O. T. Pye, Benjamin N. Murphy, and Daiwen Kang
Geosci. Model Dev., 14, 3969–3993, https://doi.org/10.5194/gmd-14-3969-2021, https://doi.org/10.5194/gmd-14-3969-2021, 2021
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The continuously updated National Air Quality Forecast Capability (NAQFC) provides air quality forecasts. To support the development of the next-generation NAQFC, we evaluate a prototype of GFSv15-CMAQv5.0.2. The performance and the potential improvements for the system are discussed. This study can provide a scientific basis for further development of NAQFC and help it to provide more accurate air quality forecasts to the public over the contiguous United States.
Mario Eduardo Gavidia-Calderón, Sergio Ibarra-Espinosa, Youngseob Kim, Yang Zhang, and Maria de Fatima Andrade
Geosci. Model Dev., 14, 3251–3268, https://doi.org/10.5194/gmd-14-3251-2021, https://doi.org/10.5194/gmd-14-3251-2021, 2021
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The MUNICH model was used to calculate pollutant concentrations inside the streets of São Paulo. The VEIN emission model provided the vehicular emissions and the coordinates of the streets. We used information from an air quality station to account for pollutant concentrations over the street rooftops. Results showed that when emissions are calibrated, MUNICH satisfied the performance criteria. MUNICH can be used to evaluate the impact of traffic-related air pollution on public health.
Mengying Bao, Yan-Lin Zhang, Fang Cao, Yu-Chi Lin, Yuhang Wang, Xiaoyan Liu, Wenqi Zhang, Meiyi Fan, Feng Xie, Robert Cary, Joshua Dixon, and Lihua Zhou
Atmos. Meas. Tech., 14, 4053–4068, https://doi.org/10.5194/amt-14-4053-2021, https://doi.org/10.5194/amt-14-4053-2021, 2021
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We introduce a two-wavelength method for brown C measurements with a modified Sunset carbon analyzer. We defined the enhanced concentrations and gave the possibility of providing an indicator of brown C. Compared with the strong local sources of organic and elemental C, we found that differences in EC mainly originated from regional transport. Biomass burning emissions significantly contributed to high differences in EC concentrations during the heavy biomass burning periods.
Kun Zhang, Ling Huang, Qing Li, Juntao Huo, Yusen Duan, Yuhang Wang, Elly Yaluk, Yangjun Wang, Qingyan Fu, and Li Li
Atmos. Chem. Phys., 21, 5905–5917, https://doi.org/10.5194/acp-21-5905-2021, https://doi.org/10.5194/acp-21-5905-2021, 2021
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Recently, high O3 concentrations were frequently observed in rural areas of the Yangtze River Delta (YRD) region under stagnant conditions. Using an online measurement and observation-based model, we investigated the budget of ROx radicals and the influence of isoprene chemistry on O3 formation. Our results underline that isoprene chemistry in the rural atmosphere becomes important with the participation of anthropogenic NOx.
Jianfeng Li, Zhe Feng, Yun Qian, and L. Ruby Leung
Earth Syst. Sci. Data, 13, 827–856, https://doi.org/10.5194/essd-13-827-2021, https://doi.org/10.5194/essd-13-827-2021, 2021
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Deep convection has different properties at different scales. We develop a 4 km h−1 observational data product of mesoscale convective systems and isolated deep convection in the United States from 2004–2017. We find that both types of convective systems contribute significantly to precipitation east of the Rocky Mountains but with distinct spatiotemporal characteristics. The data product will be useful for observational analyses and model evaluations of convection events at different scales.
Goutam Choudhury, Bhishma Tyagi, Naresh Krishna Vissa, Jyotsna Singh, Chandan Sarangi, Sachchida Nand Tripathi, and Matthias Tesche
Atmos. Chem. Phys., 20, 15389–15399, https://doi.org/10.5194/acp-20-15389-2020, https://doi.org/10.5194/acp-20-15389-2020, 2020
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This study uses 17 years (2001–2017) of observed rain rate, aerosol optical depth (AOD), meteorological reanalysis fields and outgoing long-wave radiation to investigate high precipitation events at the foothills of the Himalayas. Composite analysis of all data sets for high precipitation events (daily rainfall > 95th percentile) indicates clear and robust associations between high precipitation events, high aerosol loading and high moist static energy values.
Yohei Shinozuka, Pablo E. Saide, Gonzalo A. Ferrada, Sharon P. Burton, Richard Ferrare, Sarah J. Doherty, Hamish Gordon, Karla Longo, Marc Mallet, Yan Feng, Qiaoqiao Wang, Yafang Cheng, Amie Dobracki, Steffen Freitag, Steven G. Howell, Samuel LeBlanc, Connor Flynn, Michal Segal-Rosenhaimer, Kristina Pistone, James R. Podolske, Eric J. Stith, Joseph Ryan Bennett, Gregory R. Carmichael, Arlindo da Silva, Ravi Govindaraju, Ruby Leung, Yang Zhang, Leonhard Pfister, Ju-Mee Ryoo, Jens Redemann, Robert Wood, and Paquita Zuidema
Atmos. Chem. Phys., 20, 11491–11526, https://doi.org/10.5194/acp-20-11491-2020, https://doi.org/10.5194/acp-20-11491-2020, 2020
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In the southeast Atlantic, well-defined smoke plumes from Africa advect over marine boundary layer cloud decks; both are most extensive around September, when most of the smoke resides in the free troposphere. A framework is put forth for evaluating the performance of a range of global and regional atmospheric composition models against observations made during the NASA ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) airborne mission in September 2016.
Yi Ji, L. Gregory Huey, David J. Tanner, Young Ro Lee, Patrick R. Veres, J. Andrew Neuman, Yuhang Wang, and Xinming Wang
Atmos. Meas. Tech., 13, 3683–3696, https://doi.org/10.5194/amt-13-3683-2020, https://doi.org/10.5194/amt-13-3683-2020, 2020
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A common way of measuring trace gases in the atmosphere is chemical ionization mass spectrometry. One large drawback of these instruments is that they require radioactive ion sources. In this work we demonstrate a simple ion source that uses a small krypton lamp that can be used to replace a radioactive source.
Kurt C. Solander, Brent D. Newman, Alessandro Carioca de Araujo, Holly R. Barnard, Z. Carter Berry, Damien Bonal, Mario Bretfeld, Benoit Burban, Luiz Antonio Candido, Rolando Célleri, Jeffery Q. Chambers, Bradley O. Christoffersen, Matteo Detto, Wouter A. Dorigo, Brent E. Ewers, Savio José Filgueiras Ferreira, Alexander Knohl, L. Ruby Leung, Nate G. McDowell, Gretchen R. Miller, Maria Terezinha Ferreira Monteiro, Georgianne W. Moore, Robinson Negron-Juarez, Scott R. Saleska, Christian Stiegler, Javier Tomasella, and Chonggang Xu
Hydrol. Earth Syst. Sci., 24, 2303–2322, https://doi.org/10.5194/hess-24-2303-2020, https://doi.org/10.5194/hess-24-2303-2020, 2020
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We evaluate the soil moisture response in the humid tropics to El Niño during the three most recent super El Niño events. Our estimates are compared to in situ soil moisture estimates that span five continents. We find the strongest and most consistent soil moisture decreases in the Amazon and maritime southeastern Asia, while the most consistent increases occur over eastern Africa. Our results can be used to improve estimates of soil moisture in tropical ecohydrology models at multiple scales.
Yufei Zou, Yuhang Wang, Zuowei Xie, Hailong Wang, and Philip J. Rasch
Atmos. Chem. Phys., 20, 4999–5017, https://doi.org/10.5194/acp-20-4999-2020, https://doi.org/10.5194/acp-20-4999-2020, 2020
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We analyze the relationship between winter air stagnation and pollution extremes over eastern China and preceding Arctic sea ice loss based on climate modeling and dynamic diagnoses. We find significant increases in both the probability and intensity of air stagnation extremes in the modeling result driven by regional sea ice and sea surface temperature changes over the Pacific sector of the Arctic. We reveal the considerable impact of the Arctic climate change on mid-latitude weather extremes.
Syuichi Itahashi, Rohit Mathur, Christian Hogrefe, and Yang Zhang
Atmos. Chem. Phys., 20, 3373–3396, https://doi.org/10.5194/acp-20-3373-2020, https://doi.org/10.5194/acp-20-3373-2020, 2020
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The state-of-the-science Community Multiscale Air Quality model extended for hemispheric applications (H-CMAQ) is used to model the trans-Pacific transport which has been recognized as a potential source of air pollutants over the US. In Part 1, modeled ozone is evaluated with observations at surface, by ozonesonde and airplane, and by satellite across the Northern Hemisphere. In addition, a newly developed air mass characterization method to estimate stratospheric intrusion is presented.
Syuichi Itahashi, Rohit Mathur, Christian Hogrefe, Sergey L. Napelenok, and Yang Zhang
Atmos. Chem. Phys., 20, 3397–3413, https://doi.org/10.5194/acp-20-3397-2020, https://doi.org/10.5194/acp-20-3397-2020, 2020
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The state-of-the-science Community Multiscale Air Quality model extended for hemispheric applications (H-CMAQ) is used to model the trans-Pacific transport which has been recognized as a potential source of air pollutants over the US. In Part 2, the higher-order decoupled direct method (HDDM) is applied to investigate the emission impacts from east Asia and the US during April 2010. Furthermore, changes in trans-Pacific transport caused by the recent emissions are examined.
Aoxing Zhang, Yuhang Wang, Yuzhong Zhang, Rodney J. Weber, Yongjia Song, Ziming Ke, and Yufei Zou
Atmos. Chem. Phys., 20, 1901–1920, https://doi.org/10.5194/acp-20-1901-2020, https://doi.org/10.5194/acp-20-1901-2020, 2020
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Black carbon (BC) and brown carbon (BrC) are light-absorbing carbonaceous aerosols. We developed a module to simulate the emissions, atmospheric processing and direct radiative effect of BrC in the Community Earth System Model (CESM). We found that globally BrC is a significant absorber and is more centered in the tropical free troposphere compared to BC. The contribution of BrC heating to the Hadley circulation and latitudinal expansion of the tropics is comparable to BC heating.
Yufei Zou, Yuhang Wang, Yun Qian, Hanqin Tian, Jia Yang, and Ernesto Alvarado
Atmos. Chem. Phys., 20, 995–1020, https://doi.org/10.5194/acp-20-995-2020, https://doi.org/10.5194/acp-20-995-2020, 2020
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Fire is a natural phenomenon that has a long history of interactions with the environment and human activity. The complex interactions were less represented in previous fire and climate models. Here we use a new global fire model with improved modeling capability to study how fire responds and contributes to climate change. The modeling results show increased global fire activity in the future driven by climate change, which in turn modulates local and remote climate and ecosystems.
Jianfeng Li and Yuhang Wang
Atmos. Chem. Phys., 19, 15339–15352, https://doi.org/10.5194/acp-19-15339-2019, https://doi.org/10.5194/acp-19-15339-2019, 2019
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NO2 tropospheric vertical columns (TVCDs) and surface concentrations are widely used proxies for NOx emission variations. Through model and observation analyses, we find that satellite NO2 TVCDs provide much better information on anthropogenic NOx emission variations over urban than rural regions. NO2 surface observations, satellite column datasets, and EPA anthropogenic NOx emissions show consistent annual variations over urban regions of the United States with a continuous decrease after 2011.
Zhiyuan Hu, Jianping Huang, Chun Zhao, Yuanyuan Ma, Qinjian Jin, Yun Qian, L. Ruby Leung, Jianrong Bi, and Jianmin Ma
Atmos. Chem. Phys., 19, 12709–12730, https://doi.org/10.5194/acp-19-12709-2019, https://doi.org/10.5194/acp-19-12709-2019, 2019
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This study investigates aerosol chemical compositions and relative contributions to total aerosols in the western US. The results show that trans-Pacific aerosols have a maximum concentration in the boreal spring, with the greatest contribution from dust. Over western North America, the trans-Pacific aerosols dominate the column-integrated aerosol mass and number concentration. However, near the surface, aerosols mainly originated from local emissions.
Mingchen Ma, Yang Gao, Yuhang Wang, Shaoqing Zhang, L. Ruby Leung, Cheng Liu, Shuxiao Wang, Bin Zhao, Xing Chang, Hang Su, Tianqi Zhang, Lifang Sheng, Xiaohong Yao, and Huiwang Gao
Atmos. Chem. Phys., 19, 12195–12207, https://doi.org/10.5194/acp-19-12195-2019, https://doi.org/10.5194/acp-19-12195-2019, 2019
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Ozone pollution has become severe in China, and extremely high ozone episodes occurred in summer 2017 over the North China Plain. While meteorology impacts are clear, we find that enhanced biogenic emissions, previously ignored by the community, driven by high vapor pressure deficit, land cover change and urban landscape contribute substantially to ozone formation. This study has significant implications for ozone pollution control with more frequent heat waves and urbanization growth in future.
Stefan Rahimi, Xiaohong Liu, Chenglai Wu, William K. Lau, Hunter Brown, Mingxuan Wu, and Yun Qian
Atmos. Chem. Phys., 19, 12025–12049, https://doi.org/10.5194/acp-19-12025-2019, https://doi.org/10.5194/acp-19-12025-2019, 2019
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Light-absorbing particles impact the Earth system in a variety of ways. They can warm the atmosphere by their very presence, or they can warm the atmosphere after they deposit on snow, warm it, and warm the overlying atmosphere. This paper focuses on these two processes as they pertain to black carbon and dust's impacts on the South Asian monsoon. It will be shown that these two aerosols have a significant effect on the monsoon.
Chun Zhao, Mingyue Xu, Yu Wang, Meixin Zhang, Jianping Guo, Zhiyuan Hu, L. Ruby Leung, Michael Duda, and William Skamarock
Geosci. Model Dev., 12, 2707–2726, https://doi.org/10.5194/gmd-12-2707-2019, https://doi.org/10.5194/gmd-12-2707-2019, 2019
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Simulations at global uniform and variable resolutions share similar characteristics of precipitation and wind in the refined region. The experiments reveal the significant impacts of resolution on simulating the distribution and intensity of precipitation and updrafts. This study provides evidence supporting the use of convection-permitting global variable-resolution simulations to study extreme precipitation.
Run Liu, Lu Mao, Shaw Chen Liu, Yuanhang Zhang, Hong Liao, Huopo Chen, and Yuhang Wang
Atmos. Chem. Phys., 19, 8563–8568, https://doi.org/10.5194/acp-19-8563-2019, https://doi.org/10.5194/acp-19-8563-2019, 2019
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The recent paper by Shen et al. (2018; referred to hereafter as SHEN) made a sweeping statement on the winter haze pollution in Beijing by claiming an
Insignificant effect of climate change on winter haze in Beijing. We argue that the paper contains three serious flaws. Any one of the three flaws can nullify the claim of SHEN.
Chandan Sarangi, Yun Qian, Karl Rittger, Kathryn J. Bormann, Ying Liu, Hailong Wang, Hui Wan, Guangxing Lin, and Thomas H. Painter
Atmos. Chem. Phys., 19, 7105–7128, https://doi.org/10.5194/acp-19-7105-2019, https://doi.org/10.5194/acp-19-7105-2019, 2019
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Radiative forcing induced by deposition of light-absorbing particles (LAPs) on snow is an important surface forcing. Here, we have used high-resolution WRF-Chem (coupled with online snow–LAP–radiation model) simulations for 2013–2014 to estimate the spatial variation in LAP-induced snow albedo darkening effect in high-mountain Asia. Significant improvement in simulated LAP–snow properties with use of a higher spatial resolution for the same model configuration is illustrated over this region.
Lei Sun, Likun Xue, Yuhang Wang, Longlei Li, Jintai Lin, Ruijing Ni, Yingying Yan, Lulu Chen, Juan Li, Qingzhu Zhang, and Wenxing Wang
Atmos. Chem. Phys., 19, 1455–1469, https://doi.org/10.5194/acp-19-1455-2019, https://doi.org/10.5194/acp-19-1455-2019, 2019
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We quantified the detailed impacts of meteorology and anthropogenic emissions on surface O3 increase in central eastern China between 2003 and 2015 using GEOS-Chem. The emission change plays a more important role than the meteorological change, while the regions with a larger O3 increase are more sensitive to meteorology. NMVOC emission change dominated the O3 increase in eastern CEC, while NOx emission change led to an O3 increase in western and central CEC and O3 decrease in urban areas.
Junxi Zhang, Yang Gao, L. Ruby Leung, Kun Luo, Huan Liu, Jean-Francois Lamarque, Jianren Fan, Xiaohong Yao, Huiwang Gao, and Tatsuya Nagashima
Atmos. Chem. Phys., 19, 887–900, https://doi.org/10.5194/acp-19-887-2019, https://doi.org/10.5194/acp-19-887-2019, 2019
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ACCMIP simulations were used to study NOy deposition over East Asia in the future. Both dry and wet NOy deposition show significant decreases in the 2100s under RCP4.5 and RCP8.5 due to large anthropogenic emission reduction. The changes in climate only significantly affect the wet deposition primarily linked to changes in precipitation. Over the coastal seas of China, weaker transport of NOy from land due to emission reduction infers a larger impact from shipping and lightning emissions.
Ge Zhang, Yang Gao, Wenju Cai, L. Ruby Leung, Shuxiao Wang, Bin Zhao, Minghuai Wang, Huayao Shan, Xiaohong Yao, and Huiwang Gao
Atmos. Chem. Phys., 19, 565–576, https://doi.org/10.5194/acp-19-565-2019, https://doi.org/10.5194/acp-19-565-2019, 2019
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Based on observed data, this study reveals a distinct seesaw feature of abnormally high and low PM2.5 concentrations in December 2015 and January 2016 over North China. The mechanism of the seesaw pattern was found to be linked to a super El Niño and the Arctic Oscillation (AO). During the mature phase of El Niño in December 2015, the weakened East Asian winter monsoon favors strong haze formation; however, the circulation pattern was reversed in the next month due to the phase change of the AO.
Jiahui Zhang, Dao-Yi Gong, Rui Mao, Jing Yang, Ziyin Zhang, and Yun Qian
Atmos. Chem. Phys., 18, 16775–16791, https://doi.org/10.5194/acp-18-16775-2018, https://doi.org/10.5194/acp-18-16775-2018, 2018
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The Chinese Spring Festival (also known as the Chinese New Year or Lunar New Year) is the most important festival in China. This paper reports that during the Chinese Spring Festival, the precipitation over southern China has been significantly reduced. The precipitation reduction is due to anomalous northerly winds. We suppose that anomalous atmospheric circulation is likely related to the human activity during holidays. It is an interesting phenomenon.
Cenlin He, Mark G. Flanner, Fei Chen, Michael Barlage, Kuo-Nan Liou, Shichang Kang, Jing Ming, and Yun Qian
Atmos. Chem. Phys., 18, 11507–11527, https://doi.org/10.5194/acp-18-11507-2018, https://doi.org/10.5194/acp-18-11507-2018, 2018
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Snow albedo plays a key role in the Earth and climate system. It can be affected by impurities and snow properties. This study implements new parameterizations into a widely used snow model to account for effects of snow shape and black carbon–snow mixing state on snow albedo reduction in the Tibetan Plateau. This study points toward an imperative need for extensive measurements and improved model characterization of snow grain shape and aerosol–snow mixing state in Tibet and elsewhere.
Junxi Zhang, Yang Gao, Kun Luo, L. Ruby Leung, Yang Zhang, Kai Wang, and Jianren Fan
Atmos. Chem. Phys., 18, 9861–9877, https://doi.org/10.5194/acp-18-9861-2018, https://doi.org/10.5194/acp-18-9861-2018, 2018
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We used a regional model to investigate the impact of atmosphere with high temperature and low wind speed on ozone concentration. When these compound events (heat waves and stagnant weather) occur simultaneously, a striking ozone enhancement is revealed. This type of compound event is projected to increase more dominantly compared to single events in the future over the US, Europe, and China, implying the importance of reducing emissions in order to alleviate the impact from the compound events.
Ruixiong Zhang, Yuhang Wang, Charles Smeltzer, Hang Qu, William Koshak, and K. Folkert Boersma
Atmos. Meas. Tech., 11, 3955–3967, https://doi.org/10.5194/amt-11-3955-2018, https://doi.org/10.5194/amt-11-3955-2018, 2018
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This study focuses on how to improve OMI NO2 retrievals for trend analysis. We retrieve OMI tropospheric NO2 vertical column densities (VCDs) and obtain the NO2 seasonal trends over the United States, which are compared with coincident in situ surface NO2 measurements from the Air Quality System network. We find that three procedures are essential in comparing both datasets, including the ocean trend removal, the albedo update, and the lightning filter.
Christine A. Shields, Jonathan J. Rutz, Lai-Yung Leung, F. Martin Ralph, Michael Wehner, Brian Kawzenuk, Juan M. Lora, Elizabeth McClenny, Tashiana Osborne, Ashley E. Payne, Paul Ullrich, Alexander Gershunov, Naomi Goldenson, Bin Guan, Yun Qian, Alexandre M. Ramos, Chandan Sarangi, Scott Sellars, Irina Gorodetskaya, Karthik Kashinath, Vitaliy Kurlin, Kelly Mahoney, Grzegorz Muszynski, Roger Pierce, Aneesh C. Subramanian, Ricardo Tome, Duane Waliser, Daniel Walton, Gary Wick, Anna Wilson, David Lavers, Prabhat, Allison Collow, Harinarayan Krishnan, Gudrun Magnusdottir, and Phu Nguyen
Geosci. Model Dev., 11, 2455–2474, https://doi.org/10.5194/gmd-11-2455-2018, https://doi.org/10.5194/gmd-11-2455-2018, 2018
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ARTMIP (Atmospheric River Tracking Method Intercomparison Project) is a community effort with the explicit goal of understanding the uncertainties, and the implications of those uncertainties, in atmospheric river science solely due to detection algorithm. ARTMIP strives to quantify these differences and provide guidance on appropriate algorithmic choices for the science question posed. Project goals, experimental design, and preliminary results are provided.
Kai Zhang, Philip J. Rasch, Mark A. Taylor, Hui Wan, Ruby Leung, Po-Lun Ma, Jean-Christophe Golaz, Jon Wolfe, Wuyin Lin, Balwinder Singh, Susannah Burrows, Jin-Ho Yoon, Hailong Wang, Yun Qian, Qi Tang, Peter Caldwell, and Shaocheng Xie
Geosci. Model Dev., 11, 1971–1988, https://doi.org/10.5194/gmd-11-1971-2018, https://doi.org/10.5194/gmd-11-1971-2018, 2018
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The conservation of total water is an important numerical feature for global Earth system models. Even small conservation problems in the water budget can lead to systematic errors in century-long simulations for sea level rise projection. This study quantifies and reduces various sources of water conservation error in the atmosphere component of the Energy Exascale Earth System Model.
Hewen Niu, Shichang Kang, Hailong Wang, Rudong Zhang, Xixi Lu, Yun Qian, Rukumesh Paudyal, Shijin Wang, Xiaofei Shi, and Xingguo Yan
Atmos. Chem. Phys., 18, 6441–6460, https://doi.org/10.5194/acp-18-6441-2018, https://doi.org/10.5194/acp-18-6441-2018, 2018
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Deposition of light-absorbing carbonaceous aerosol on the surface of glaciers can greatly alter the energy fluxes of glaciers. Two years of continuous observations of carbonaceous aerosols in a glacierized region are analyzed. We mainly studied the light absorption properties of carbonaceous aerosol and have employed a global aerosol–climate model to estimate source attributions of atmospheric black carbon.
Longtao Wu, Yu Gu, Jonathan H. Jiang, Hui Su, Nanpeng Yu, Chun Zhao, Yun Qian, Bin Zhao, Kuo-Nan Liou, and Yong-Sang Choi
Atmos. Chem. Phys., 18, 5529–5547, https://doi.org/10.5194/acp-18-5529-2018, https://doi.org/10.5194/acp-18-5529-2018, 2018
Jianzhong Xu, Qi Zhang, Jinsen Shi, Xinlei Ge, Conghui Xie, Junfeng Wang, Shichang Kang, Ruixiong Zhang, and Yuhang Wang
Atmos. Chem. Phys., 18, 427–443, https://doi.org/10.5194/acp-18-427-2018, https://doi.org/10.5194/acp-18-427-2018, 2018
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This manuscript presents results from a comprehensive field study using an HR-AMS coupled with a suite of other instruments in central Tibetan Plateau. The study discusses the chemical composition, sources, and processes of submicron aerosol during the transition from pre-monsoon to monsoon. Organic aerosol was overall highly oxidized during the entire study with higher O / C ratios during the pre-monsoon period. Sensitivity of air pollution transport with synoptic process was also evaluated.
Yawen Liu, Kai Zhang, Yun Qian, Yuhang Wang, Yufei Zou, Yongjia Song, Hui Wan, Xiaohong Liu, and Xiu-Qun Yang
Atmos. Chem. Phys., 18, 31–47, https://doi.org/10.5194/acp-18-31-2018, https://doi.org/10.5194/acp-18-31-2018, 2018
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Fire aerosols have large impact on weather and climate through their effect on clouds and radiation, but it is difficult to quantify. Here we investigated the short-term effective radiative forcing of fire aerosols using the nudged hindcast ensemble simulations from global aerosol-climate model. Results show large effects of fire aerosols on both liquid and ice cloud and large ensemble spread of regional mean shortwave cloud radiative forcing over southern Mexico and the central US.
Kai Duan, Ge Sun, Steven G. McNulty, Peter V. Caldwell, Erika C. Cohen, Shanlei Sun, Heather D. Aldridge, Decheng Zhou, Liangxia Zhang, and Yang Zhang
Hydrol. Earth Syst. Sci., 21, 5517–5529, https://doi.org/10.5194/hess-21-5517-2017, https://doi.org/10.5194/hess-21-5517-2017, 2017
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We examined the potential roles of major climatic variables (including precipitation, air temperature, solar radiation, specific humidity, and wind speed) in altering annual runoff, which is an important indicator of freshwater supply, in the United States through the 21st century. Increasing temperature, precipitation, and humidity are recognized as three major climatic factors that drive runoff to change in different directions across the country.
Randal D. Koster, Alan K. Betts, Paul A. Dirmeyer, Marc Bierkens, Katrina E. Bennett, Stephen J. Déry, Jason P. Evans, Rong Fu, Felipe Hernandez, L. Ruby Leung, Xu Liang, Muhammad Masood, Hubert Savenije, Guiling Wang, and Xing Yuan
Hydrol. Earth Syst. Sci., 21, 3777–3798, https://doi.org/10.5194/hess-21-3777-2017, https://doi.org/10.5194/hess-21-3777-2017, 2017
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Large-scale hydrological variability can affect society in profound ways; floods and droughts, for example, often cause major damage and hardship. A recent gathering of hydrologists at a symposium to honor the career of Professor Eric Wood motivates the present survey of recent research on this variability. The surveyed literature and the illustrative examples provided in the paper show that research into hydrological variability continues to be strong, vibrant, and multifaceted.
Yang Yang, Hailong Wang, Steven J. Smith, Richard Easter, Po-Lun Ma, Yun Qian, Hongbin Yu, Can Li, and Philip J. Rasch
Atmos. Chem. Phys., 17, 8903–8922, https://doi.org/10.5194/acp-17-8903-2017, https://doi.org/10.5194/acp-17-8903-2017, 2017
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Sulfate has significant impacts on air quality and climate. Local sulfate pollution could result from remote influences, making domestic mitigation efforts inefficient. Using CESM with a sulfur source-tagging technique, we found that, over regions with relatively low emissions, sulfate concentrations are primarily attributed to non-local sources and sulfate indirect radiative forcing over the Southern Hemisphere is more sensitive to emission perturbation than the polluted Northern Hemisphere.
Chaopeng Hong, Qiang Zhang, Yang Zhang, Youhua Tang, Daniel Tong, and Kebin He
Geosci. Model Dev., 10, 2447–2470, https://doi.org/10.5194/gmd-10-2447-2017, https://doi.org/10.5194/gmd-10-2447-2017, 2017
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A regional coupled climate–chemistry modeling system using the dynamical downscaling technique was established and evaluated. The modeling system performed well for both the climatological and the short-term air quality applications over east Asia. Regional models outperformed global models in regional climate and air quality predictions. The coupled modeling system improved the model performance, although some biases remained in the aerosol–cloud–radiation variables.
Khairunnisa Yahya, Timothy Glotfelty, Kai Wang, Yang Zhang, and Athanasios Nenes
Geosci. Model Dev., 10, 2333–2363, https://doi.org/10.5194/gmd-10-2333-2017, https://doi.org/10.5194/gmd-10-2333-2017, 2017
Shi Zhong, Yun Qian, Chun Zhao, Ruby Leung, Hailong Wang, Ben Yang, Jiwen Fan, Huiping Yan, Xiu-Qun Yang, and Dongqing Liu
Atmos. Chem. Phys., 17, 5439–5457, https://doi.org/10.5194/acp-17-5439-2017, https://doi.org/10.5194/acp-17-5439-2017, 2017
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An online climate–chemistry coupled model (WRF-Chem) is integrated for 5 years at cloud-permitting scale to quantify the impacts of urbanization-induced changes in land cover and pollutants emission on regional climate in the Yangtze River Delta region in eastern China. Urbanization over this region increases the frequency of extreme precipitation and heat wave in summer. The results could help China government in making policies in mitigating the environmental impact of urbanization.
Xiangyu Luo, Hong-Yi Li, L. Ruby Leung, Teklu K. Tesfa, Augusto Getirana, Fabrice Papa, and Laura L. Hess
Geosci. Model Dev., 10, 1233–1259, https://doi.org/10.5194/gmd-10-1233-2017, https://doi.org/10.5194/gmd-10-1233-2017, 2017
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This study shows that alleviating vegetation-caused biases in DEM data, refining channel cross-sectional geometry and Manning roughness coefficients, as well as accounting for backwater effects can effectively improve the modeling of streamflow, river stages and flood extent in the Amazon Basin. The obtained understanding could be helpful to hydrological modeling in basins with evident inundation, which has important implications for improving land–atmosphere interactions in Earth system models.
Ruixiong Zhang, Yuhang Wang, Qiusheng He, Laiguo Chen, Yuzhong Zhang, Hang Qu, Charles Smeltzer, Jianfeng Li, Leonardo M. A. Alvarado, Mihalis Vrekoussis, Andreas Richter, Folkard Wittrock, and John P. Burrows
Atmos. Chem. Phys., 17, 3083–3095, https://doi.org/10.5194/acp-17-3083-2017, https://doi.org/10.5194/acp-17-3083-2017, 2017
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We use short-lived reactive aromatics as proxies to diagnose transport of pollutants to Tibet. In situ observations of short-lived reactive aromatics across the Tibetan Plateau are analyzed using a regional chemistry and transport model. Our results suggest that the cut-off low system is a major pathway for long-range transport of pollutants such as black carbon. The modeling analysis reveals that even the state-of-the-science reanalysis cannot simulate this cut-off system accurately.
Teklu K. Tesfa and Lai-Yung Ruby Leung
Geosci. Model Dev., 10, 873–888, https://doi.org/10.5194/gmd-10-873-2017, https://doi.org/10.5194/gmd-10-873-2017, 2017
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Motivated by the significant topographic influence on land surface processes, this study explored two methods to discretize watersheds into two types of subgrid structures to capture spatial heterogeneity for land surface models. Adopting geomorphologic concepts in watershed discretization yields improved capability in capturing subgrid topographic heterogeneity, which also allowed climatic and land cover variability to be better represented with a nominal increase in computational requirements.
Jiwen Fan, L. Ruby Leung, Daniel Rosenfeld, and Paul J. DeMott
Atmos. Chem. Phys., 17, 1017–1035, https://doi.org/10.5194/acp-17-1017-2017, https://doi.org/10.5194/acp-17-1017-2017, 2017
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How orographic mixed-phase clouds respond to changes in cloud condensation nuclei (CCN) and ice nucleating particles (INPs) is highly uncertain. We conducted this study to improve understanding of these processes. We found a new mechanism through which CCN can invigorate orographic mixed-phase clouds and drastically intensify snow precipitation when CCN concentrations are high. Our findings have very important implications for orographic precipitation in polluted regions.
Provat K. Saha, Andrey Khlystov, Khairunnisa Yahya, Yang Zhang, Lu Xu, Nga L. Ng, and Andrew P. Grieshop
Atmos. Chem. Phys., 17, 501–520, https://doi.org/10.5194/acp-17-501-2017, https://doi.org/10.5194/acp-17-501-2017, 2017
Yiquan Jiang, Zheng Lu, Xiaohong Liu, Yun Qian, Kai Zhang, Yuhang Wang, and Xiu-Qun Yang
Atmos. Chem. Phys., 16, 14805–14824, https://doi.org/10.5194/acp-16-14805-2016, https://doi.org/10.5194/acp-16-14805-2016, 2016
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Aerosols from open fires could significantly perturb the global radiation balance and induce climate change. In this study, the CAM5 global climate model is used to investigate the spatial and seasonal characteristics of radiative effects due to fire aerosol–radiation interactions, fire aerosol-cloud interactions and fire aerosol-surface albedo interactions, including radiative effects from all fire aerosols, fire black carbon and fire particulate organic matter.
Reindert J. Haarsma, Malcolm J. Roberts, Pier Luigi Vidale, Catherine A. Senior, Alessio Bellucci, Qing Bao, Ping Chang, Susanna Corti, Neven S. Fučkar, Virginie Guemas, Jost von Hardenberg, Wilco Hazeleger, Chihiro Kodama, Torben Koenigk, L. Ruby Leung, Jian Lu, Jing-Jia Luo, Jiafu Mao, Matthew S. Mizielinski, Ryo Mizuta, Paulo Nobre, Masaki Satoh, Enrico Scoccimarro, Tido Semmler, Justin Small, and Jin-Song von Storch
Geosci. Model Dev., 9, 4185–4208, https://doi.org/10.5194/gmd-9-4185-2016, https://doi.org/10.5194/gmd-9-4185-2016, 2016
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Recent progress in computing power has enabled climate models to simulate more processes in detail and on a smaller scale. Here we present a common protocol for these high-resolution runs that will foster the analysis and understanding of the impact of model resolution on the simulated climate. These runs will also serve as a more reliable source for assessing climate risks that are associated with small-scale weather phenomena such as tropical cyclones.
Dasa Gu, Yuhang Wang, Ran Yin, Yuzhong Zhang, and Charles Smeltzer
Atmos. Meas. Tech., 9, 5193–5201, https://doi.org/10.5194/amt-9-5193-2016, https://doi.org/10.5194/amt-9-5193-2016, 2016
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We show in this study that the non-linearity of NOx chemistry implies that the local derivative (of a first-order Taylor expansion) is better suited in the inverse modelling of NOx emissions over eastern China. We used single-grid-cell-based perturbation sensitivity calculation. The method leads to smaller NOx emission over highly polluted regions and higher NOx emission over rural regions. There are also more consistent results from using two different satellite instruments.
Tianjun Zhou, Andrew G. Turner, James L. Kinter, Bin Wang, Yun Qian, Xiaolong Chen, Bo Wu, Bin Wang, Bo Liu, Liwei Zou, and Bian He
Geosci. Model Dev., 9, 3589–3604, https://doi.org/10.5194/gmd-9-3589-2016, https://doi.org/10.5194/gmd-9-3589-2016, 2016
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This paper tells why to launch the Global Monsoons Model Inter-comparison Project (GMMIP) and how to achieve its scientific goals on monsoon variability. It addresses the scientific questions to be answered, describes three tiered experiments comprehensively and proposes a basic analysis framework to guide future research. It will help the monsoon research communities to understand the objectives of the GMMIP and the modelling groups involved in the GMMIP conduct the experiments successfully.
Kai Duan, Ge Sun, Steven G. McNulty, Peter V. Caldwell, Erika C. Cohen, Shanlei Sun, Heather D. Aldridge, Decheng Zhou, Liangxia Zhang, and Yang Zhang
Hydrol. Earth Syst. Sci. Discuss., https://doi.org/10.5194/hess-2016-493, https://doi.org/10.5194/hess-2016-493, 2016
Revised manuscript not accepted
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This study examines the potential shift of the relative roles of changing precipitation and temperature in controlling freshwater availability in the USA. The influence of temperature is projected to outweigh that of precipitation in a continued warming future in the 21st century, although precipitation has been the primary control in recent decades. The vast croplands and grasslands across the central and forests in the northwestern regions might be particularly vulnerable to climate change.
Chun Zhao, Maoyi Huang, Jerome D. Fast, Larry K. Berg, Yun Qian, Alex Guenther, Dasa Gu, Manish Shrivastava, Ying Liu, Stacy Walters, Gabriele Pfister, Jiming Jin, John E. Shilling, and Carsten Warneke
Geosci. Model Dev., 9, 1959–1976, https://doi.org/10.5194/gmd-9-1959-2016, https://doi.org/10.5194/gmd-9-1959-2016, 2016
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In this study, the latest version of MEGAN is coupled within CLM4 in WRF-Chem. In this implementation, MEGAN shares a consistent vegetation map with CLM4. This improved modeling framework is used to investigate the impact of two land surface schemes on BVOCs and examine the sensitivity of BVOCs to vegetation distributions in California. This study indicates that more effort is needed to obtain the most appropriate and accurate land cover data sets for climate and air quality models.
Bin Zhao, Kuo-Nan Liou, Yu Gu, Cenlin He, Wee-Liang Lee, Xing Chang, Qinbin Li, Shuxiao Wang, Hsien-Liang R. Tseng, Lai-Yung R. Leung, and Jiming Hao
Atmos. Chem. Phys., 16, 5841–5852, https://doi.org/10.5194/acp-16-5841-2016, https://doi.org/10.5194/acp-16-5841-2016, 2016
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We examine the impact of buildings on surface solar fluxes in Beijing by accounting for their 3-D structures. We find that inclusion of buildings changes surface solar fluxes by within ±1 W m−2, ±1–10 W m−2, and up to ±100 W m−2 at grid resolutions of 4 km, 800 m, and 90 m, respectively. We can resolve pairs of positive-negative flux deviations on different sides of buildings at ≤ 800 m resolutions. We should treat building-effect on solar fluxes differently in models with different resolutions.
Zhiyuan Hu, Chun Zhao, Jianping Huang, L. Ruby Leung, Yun Qian, Hongbin Yu, Lei Huang, and Olga V. Kalashnikova
Geosci. Model Dev., 9, 1725–1746, https://doi.org/10.5194/gmd-9-1725-2016, https://doi.org/10.5194/gmd-9-1725-2016, 2016
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This study conducts the simulation of WRF-Chem with the quasi-global configuration for 2010–2014, and evaluates the simulation with multiple observation datasets for the first time. This study demonstrates that the WRF-Chem quasi-global simulation can be used for investigating trans-Pacific transport of aerosols and providing reasonable inflow chemical boundaries for the western USA to further understand the impact of transported pollutants on the regional air quality and climate.
Shanlei Sun, Ge Sun, Erika Cohen, Steven G. McNulty, Peter V. Caldwell, Kai Duan, and Yang Zhang
Hydrol. Earth Syst. Sci., 20, 935–952, https://doi.org/10.5194/hess-20-935-2016, https://doi.org/10.5194/hess-20-935-2016, 2016
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This study links an ecohydrological model with WRF (Weather Research and Forecasting Model) dynamically downscaled climate projections of the HadCM3 model under the IPCC SRES A2 emission scenario. Water yield and ecosystem productivity response to climate change were highly variable with an increasing trend across the 82 773 watersheds. Results are useful for policy-makers and land managers in formulating appropriate watershed-specific strategies for sustaining water and carbon sources.
Khairunnisa Yahya, Kai Wang, Patrick Campbell, Timothy Glotfelty, Jian He, and Yang Zhang
Geosci. Model Dev., 9, 671–695, https://doi.org/10.5194/gmd-9-671-2016, https://doi.org/10.5194/gmd-9-671-2016, 2016
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The Weather Research and Forecasting model with Chemistry (WRF/Chem) v3.6.1 is evaluated for its first decadal application during 2001 to 2010 using the Representative Concentration Pathway 8.5 emissions. The model evaluation shows acceptable performance for long-term climatological simulations of most meteorological variables and chemical concentrations. Larger biases exist for aerosol-cloud-radiation variables, which future model improvement should focus on.
Kai Zhang, Chun Zhao, Hui Wan, Yun Qian, Richard C. Easter, Steven J. Ghan, Koichi Sakaguchi, and Xiaohong Liu
Geosci. Model Dev., 9, 607–632, https://doi.org/10.5194/gmd-9-607-2016, https://doi.org/10.5194/gmd-9-607-2016, 2016
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A sub-grid treatment based on Weibull distribution is introduced to CAM5 to take into account the impact of unresolved variability of surface wind speed on sea salt and dust emissions. Simulations show that sub-grid wind variability has relatively small impacts on the global mean sea salt emissions, but considerable influence on dust emissions. Dry convective eddies and mesoscale flows associated with complex topography are the major causes of dust emission enhancement.
J. He, Y. Zhang, S. Tilmes, L. Emmons, J.-F. Lamarque, T. Glotfelty, A. Hodzic, and F. Vitt
Geosci. Model Dev., 8, 3999–4025, https://doi.org/10.5194/gmd-8-3999-2015, https://doi.org/10.5194/gmd-8-3999-2015, 2015
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The global simulations with CB05_GE and MOZART-4x predict similar chemical profiles for major gases compared to aircraft measurements, with better agreement for the NOy profile by CB05_GE. The SOA concentrations of SOA at four sites in CONUS and organic carbon over the IMPROVE sites are better predicted by MOZART-4x. The two simulations result in a global average difference of 0.5W m-2 in simulated shortwave cloud radiative forcing, with up to 13.6W m-2 over subtropical regions.
R. Zhang, H. Wang, D. A. Hegg, Y. Qian, S. J. Doherty, C. Dang, P.-L. Ma, P. J. Rasch, and Q. Fu
Atmos. Chem. Phys., 15, 12805–12822, https://doi.org/10.5194/acp-15-12805-2015, https://doi.org/10.5194/acp-15-12805-2015, 2015
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We use a global climate model with an explicit source tagging technique to quantify contributions of emissions from various geographical regions and sectors to BC in North America. Model results are evaluated against measurements of near-surface and in-snow BC. We found strong spatial variations of BC and its radiative forcing that can be quantitatively attributed to the various source origins, and also identified a significant source of BC in snow that is likely missing in most climate models.
J. He, R. He, and Y. Zhang
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmdd-8-9965-2015, https://doi.org/10.5194/gmdd-8-9965-2015, 2015
Revised manuscript not accepted
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WRF/Chem simulations are performed to understand the impacts of cumulus parameterizations and air-sea interactions on coastal air quality. The use of different cumulus parameterizations gives different vertical mixing and wet scavenging. The use of different air-sea interaction treatments also gives different predictions of O3 and PM2.5 by up to 17.3 ppb and 7.9 μg m-3, respectively. WRF/Chem-ROMS improves model predictions, illustrating the benefits and needs of using coupled atmospheric-ocean
C. He, K.-N. Liou, Y. Takano, R. Zhang, M. Levy Zamora, P. Yang, Q. Li, and L. R. Leung
Atmos. Chem. Phys., 15, 11967–11980, https://doi.org/10.5194/acp-15-11967-2015, https://doi.org/10.5194/acp-15-11967-2015, 2015
K. Yahya, K. Wang, Y. Zhang, and T. E. Kleindienst
Geosci. Model Dev., 8, 2095–2117, https://doi.org/10.5194/gmd-8-2095-2015, https://doi.org/10.5194/gmd-8-2095-2015, 2015
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The application of WRF/Chem to North America shows that it can reproduce most observations and their variation trends from 2006 to 2010. The inclusion of chemical feedbacks reduces biases in meteorological predictions in 2010 but increases errors in comparison to WRF. The net changes in meteorology from 2006 to 2010 are mostly influenced by changes in meteorology and those of ozone and fine particles are influenced by changes in emissions and chemical BCONs, and to a lesser extent meteorology.
R. Zhang, H. Wang, Y. Qian, P. J. Rasch, R. C. Easter, P.-L. Ma, B. Singh, J. Huang, and Q. Fu
Atmos. Chem. Phys., 15, 6205–6223, https://doi.org/10.5194/acp-15-6205-2015, https://doi.org/10.5194/acp-15-6205-2015, 2015
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We use the CAM5 model with a novel source-tagging technique to characterize the fate of BC particles emitted from various geographical regions and sectors and their transport pathways to the Himalayas and Tibetan Plateau (HTP). We show a comprehensive picture of the seasonal and regional dependence of BC source attributions, and find strong seasonal and spatial variations in BC-in-snow radiative forcing in the HTP that can be quantitatively attributed to the various regional/sectoral sources.
W.-L. Lee, Y. Gu, K. N. Liou, L. R. Leung, and H.-H. Hsu
Atmos. Chem. Phys., 15, 5405–5413, https://doi.org/10.5194/acp-15-5405-2015, https://doi.org/10.5194/acp-15-5405-2015, 2015
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This paper investigates 3-D mountain effects on solar flux distributions and their impact on surface hydrology over the western United States, specifically the Rocky Mountains and the Sierra Nevada, using the global CCSM4 (CAM4/CLM4) with a 0.23°×0.31° resolution for simulations over 6 years. We show that deviations in the net surface fluxes are not only affected by 3-D mountains but also influenced by feedbacks of cloud and snow in association with the long-term simulations.
Y. Fang, C. Liu, and L. R. Leung
Geosci. Model Dev., 8, 781–789, https://doi.org/10.5194/gmd-8-781-2015, https://doi.org/10.5194/gmd-8-781-2015, 2015
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1. A gradient projection method was used to reduce the computation time of carbon-nitrogen spin-up processes in CLM4.
2. Point-scale simulations showed that the cyclic stability of total carbon for some cases differs from that of the periodic atmospheric forcing, and some cases even showed instability.
3. The instability issue is resolved after the hydrology scheme in CLM4 is replaced with a flow model for variably saturated porous media.
B. Zheng, Q. Zhang, Y. Zhang, K. B. He, K. Wang, G. J. Zheng, F. K. Duan, Y. L. Ma, and T. Kimoto
Atmos. Chem. Phys., 15, 2031–2049, https://doi.org/10.5194/acp-15-2031-2015, https://doi.org/10.5194/acp-15-2031-2015, 2015
M. Wang, B. Xu, J. Cao, X. Tie, H. Wang, R. Zhang, Y. Qian, P. J. Rasch, S. Zhao, G. Wu, H. Zhao, D. R. Joswiak, J. Li, and Y. Xie
Atmos. Chem. Phys., 15, 1191–1204, https://doi.org/10.5194/acp-15-1191-2015, https://doi.org/10.5194/acp-15-1191-2015, 2015
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Carbonaceous aerosols recorded in a Tibetan glacier present a distinct seasonal dependence and an increasing trend after 1980, which has important implications for the accelerated glacier melting. We use a global aerosol--climate model to quantify the aerosol source--receptor relationships, showing that emissions in South Asia had the largest contribution. The emission inventories and historical fuel consumption in South Asia are consistent with our ice-core analysis and model results.
C. Zhao, Z. Hu, Y. Qian, L. Ruby Leung, J. Huang, M. Huang, J. Jin, M. G. Flanner, R. Zhang, H. Wang, H. Yan, Z. Lu, and D. G. Streets
Atmos. Chem. Phys., 14, 11475–11491, https://doi.org/10.5194/acp-14-11475-2014, https://doi.org/10.5194/acp-14-11475-2014, 2014
T. Glotfelty, Y. Zhang, P. Karamchandani, and D. G. Streets
Atmos. Chem. Phys., 14, 9379–9402, https://doi.org/10.5194/acp-14-9379-2014, https://doi.org/10.5194/acp-14-9379-2014, 2014
J. He and Y. Zhang
Atmos. Chem. Phys., 14, 9171–9200, https://doi.org/10.5194/acp-14-9171-2014, https://doi.org/10.5194/acp-14-9171-2014, 2014
H. Wan, P. J. Rasch, K. Zhang, Y. Qian, H. Yan, and C. Zhao
Geosci. Model Dev., 7, 1961–1977, https://doi.org/10.5194/gmd-7-1961-2014, https://doi.org/10.5194/gmd-7-1961-2014, 2014
B. Gantt, J. He, X. Zhang, Y. Zhang, and A. Nenes
Atmos. Chem. Phys., 14, 7485–7497, https://doi.org/10.5194/acp-14-7485-2014, https://doi.org/10.5194/acp-14-7485-2014, 2014
F. Yan, E. Winijkul, D. G. Streets, Z. Lu, T. C. Bond, and Y. Zhang
Atmos. Chem. Phys., 14, 5709–5733, https://doi.org/10.5194/acp-14-5709-2014, https://doi.org/10.5194/acp-14-5709-2014, 2014
M. Li, Q. Zhang, D. G. Streets, K. B. He, Y. F. Cheng, L. K. Emmons, H. Huo, S. C. Kang, Z. Lu, M. Shao, H. Su, X. Yu, and Y. Zhang
Atmos. Chem. Phys., 14, 5617–5638, https://doi.org/10.5194/acp-14-5617-2014, https://doi.org/10.5194/acp-14-5617-2014, 2014
T. K. Tesfa, H.-Y. Li, L. R. Leung, M. Huang, Y. Ke, Y. Sun, and Y. Liu
Geosci. Model Dev., 7, 947–963, https://doi.org/10.5194/gmd-7-947-2014, https://doi.org/10.5194/gmd-7-947-2014, 2014
L. T. Wang, Z. Wei, J. Yang, Y. Zhang, F. F. Zhang, J. Su, C. C. Meng, and Q. Zhang
Atmos. Chem. Phys., 14, 3151–3173, https://doi.org/10.5194/acp-14-3151-2014, https://doi.org/10.5194/acp-14-3151-2014, 2014
A. Baklanov, K. Schlünzen, P. Suppan, J. Baldasano, D. Brunner, S. Aksoyoglu, G. Carmichael, J. Douros, J. Flemming, R. Forkel, S. Galmarini, M. Gauss, G. Grell, M. Hirtl, S. Joffre, O. Jorba, E. Kaas, M. Kaasik, G. Kallos, X. Kong, U. Korsholm, A. Kurganskiy, J. Kushta, U. Lohmann, A. Mahura, A. Manders-Groot, A. Maurizi, N. Moussiopoulos, S. T. Rao, N. Savage, C. Seigneur, R. S. Sokhi, E. Solazzo, S. Solomos, B. Sørensen, G. Tsegas, E. Vignati, B. Vogel, and Y. Zhang
Atmos. Chem. Phys., 14, 317–398, https://doi.org/10.5194/acp-14-317-2014, https://doi.org/10.5194/acp-14-317-2014, 2014
J. Fan, L. R. Leung, P. J. DeMott, J. M. Comstock, B. Singh, D. Rosenfeld, J. M. Tomlinson, A. White, K. A. Prather, P. Minnis, J. K. Ayers, and Q. Min
Atmos. Chem. Phys., 14, 81–101, https://doi.org/10.5194/acp-14-81-2014, https://doi.org/10.5194/acp-14-81-2014, 2014
Y. Sun, Z. Hou, M. Huang, F. Tian, and L. Ruby Leung
Hydrol. Earth Syst. Sci., 17, 4995–5011, https://doi.org/10.5194/hess-17-4995-2013, https://doi.org/10.5194/hess-17-4995-2013, 2013
K. N. Liou, Y. Gu, L. R. Leung, W. L. Lee, and R. G. Fovell
Atmos. Chem. Phys., 13, 11709–11721, https://doi.org/10.5194/acp-13-11709-2013, https://doi.org/10.5194/acp-13-11709-2013, 2013
N. Voisin, L. Liu, M. Hejazi, T. Tesfa, H. Li, M. Huang, Y. Liu, and L. R. Leung
Hydrol. Earth Syst. Sci., 17, 4555–4575, https://doi.org/10.5194/hess-17-4555-2013, https://doi.org/10.5194/hess-17-4555-2013, 2013
Y. Fang, M. Huang, C. Liu, H. Li, and L. R. Leung
Geosci. Model Dev., 6, 1977–1988, https://doi.org/10.5194/gmd-6-1977-2013, https://doi.org/10.5194/gmd-6-1977-2013, 2013
C. Zhao, X. Liu, Y. Qian, J. Yoon, Z. Hou, G. Lin, S. McFarlane, H. Wang, B. Yang, P.-L. Ma, H. Yan, and J. Bao
Atmos. Chem. Phys., 13, 10969–10987, https://doi.org/10.5194/acp-13-10969-2013, https://doi.org/10.5194/acp-13-10969-2013, 2013
C. Zhao, S. Chen, L. R. Leung, Y. Qian, J. F. Kok, R. A. Zaveri, and J. Huang
Atmos. Chem. Phys., 13, 10733–10753, https://doi.org/10.5194/acp-13-10733-2013, https://doi.org/10.5194/acp-13-10733-2013, 2013
N. Voisin, H. Li, D. Ward, M. Huang, M. Wigmosta, and L. R. Leung
Hydrol. Earth Syst. Sci., 17, 3605–3622, https://doi.org/10.5194/hess-17-3605-2013, https://doi.org/10.5194/hess-17-3605-2013, 2013
Y. Ke, L. R. Leung, M. Huang, and H. Li
Geosci. Model Dev., 6, 1609–1622, https://doi.org/10.5194/gmd-6-1609-2013, https://doi.org/10.5194/gmd-6-1609-2013, 2013
Y. Zhang, K. Sartelet, S.-Y. Wu, and C. Seigneur
Atmos. Chem. Phys., 13, 6807–6843, https://doi.org/10.5194/acp-13-6807-2013, https://doi.org/10.5194/acp-13-6807-2013, 2013
Y. Zhang, K. Sartelet, S. Zhu, W. Wang, S.-Y. Wu, X. Zhang, K. Wang, P. Tran, C. Seigneur, and Z.-F. Wang
Atmos. Chem. Phys., 13, 6845–6875, https://doi.org/10.5194/acp-13-6845-2013, https://doi.org/10.5194/acp-13-6845-2013, 2013
H. Wan, P. J. Rasch, K. Zhang, J. Kazil, and L. R. Leung
Geosci. Model Dev., 6, 861–874, https://doi.org/10.5194/gmd-6-861-2013, https://doi.org/10.5194/gmd-6-861-2013, 2013
H. Wang, R. C. Easter, P. J. Rasch, M. Wang, X. Liu, S. J. Ghan, Y. Qian, J.-H. Yoon, P.-L. Ma, and V. Vinoj
Geosci. Model Dev., 6, 765–782, https://doi.org/10.5194/gmd-6-765-2013, https://doi.org/10.5194/gmd-6-765-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Steady-state mixing state of black carbon aerosols from a particle-resolved model
Distinctive dust weather intensities in North China resulted from two types of atmospheric circulation anomalies
Biomass burning emission analysis based on MODIS aerosol optical depth and AeroCom multi-model simulations: implications for model constraints and emission inventories
Quasi-weekly oscillation of regional PM2.5 transport over China driven by the synoptic-scale disturbance of the East Asian winter monsoon circulation
Solar radiation estimation in West Africa: impact of dust conditions during the 2021 dry season
Gaps in our understanding of ice-nucleating particle sources exposed by global simulation of the UK Earth System Model
The role of interfacial tension in the size-dependent phase separation of atmospheric aerosol particles
Warming effects of reduced sulfur emissions from shipping
The key role of atmospheric absorption in the Asian summer monsoon response to dust emissions in CMIP6 models
Multi-model effective radiative forcing of the 2020 sulfur cap for shipping
Representation of iron aerosol size distributions of anthropogenic emissions is critical in evaluating atmospheric soluble iron input to the ocean
High-resolution air quality maps for Bucharest using Mixed-Effects Modeling Framework
Revealing dominant patterns of aerosol regimes in the lower troposphere and their evolution from preindustrial times to the future in global climate model simulations
Improving estimation of a record-breaking east Asian dust storm emission with lagged aerosol Ångström exponent observations
Impact of biomass burning aerosols (BBA) on the tropical African climate in an ocean–atmosphere–aerosol coupled climate model
Retrieval of refractive index and water content for the coating materials of aged black carbon aerosol based on optical properties: a theoretical analysis
Predicting hygroscopic growth of organosulfur aerosol particles using COSMOtherm
Dust aerosol from the Aralkum Desert influences the radiation budget and atmospheric dynamics of Central Asia
Global modeling of aerosol nucleation with a semi-explicit chemical mechanism for highly oxygenated organic molecules (HOMs)
Synergistic effects of the winter North Atlantic Oscillation (NAO) and El Niño–Southern Oscillation (ENSO) on dust activities in North China during the following spring
Aerosol composition, air quality, and boundary layer dynamics in the urban background of Stuttgart in winter
Measurement report: Source attribution and estimation of black carbon levels in an urban hotspot of the central Po Valley – an integrated approach combining high-resolution dispersion modelling and micro-aethalometers
Construction and Application of a Pollen Emissions Model based on Phenology and Random Forests
Microphysical modelling of aerosol scavenging by different types of clouds: description and validation of the approach
Insights into the sources of ultrafine particle numbers at six European urban sites obtained by investigating COVID-19 lockdowns
In-plume and out-of-plume analysis of aerosol–cloud interactions derived from the 2014–2015 Holuhraun volcanic eruption
Impacts of atmospheric circulation patterns and cloud inhibition on aerosol radiative effect and boundary layer structure during winter air pollution in Sichuan Basin, China
The effectiveness of solar radiation management for marine cloud brightening geoengineering by fine sea spray in worldwide different climatic regions
Accounting for Black Carbon Aging Process in a Two-way Coupled Meteorology – Air Quality Model
Investigating the sign of stratocumulus adjustments to aerosols in the ICON global storm-resolving model
A model study investigating the sensitivity of aerosol forcing to the volatilities of semi-volatile organic compounds
Characterization of Brown Carbon absorption in different European environments through source contribution analysis
Spatial and temporal evolution of future atmospheric reactive nitrogen deposition in China under different climate change mitigation strategies
The impact of uncertainty in black carbon's refractive index on simulated optical depth and radiative forcing
Decomposing the effective radiative forcing of anthropogenic aerosols based on CMIP6 Earth system models
Modeling impacts of dust mineralogy on fast climate response
Uncertainties in laboratory-measured shortwave refractive indices of mineral dust aerosols and derived optical properties: a theoretical assessment
Diagnosing uncertainties in global biomass burning emission inventories and their impact on modeled air pollutants
Role of atmospheric aerosols in severe winter fog over the Indo-Gangetic Plain of India: a case study
Long-term variability in black carbon emissions constrained by gap-filled absorption aerosol optical depth and associated premature mortality in China
Intercomparison of aerosol optical depths from four reanalyses and their multi-reanalysis consensus
Global aviation contrail climate effects from 2019 to 2021
Rapid iodine oxoacid nucleation enhanced by dimethylamine in broad marine regions
Simulations of the impact of cloud condensation nuclei and ice-nucleating particles perturbations on the microphysics and radar reflectivity factor of stratiform mixed-phase clouds
Aerosols in the central Arctic cryosphere: satellite and model integrated insights during Arctic spring and summer
Observationally constrained regional variations of shortwave absorption by iron oxides emphasize the cooling effect of dust
Droplet collection efficiencies inferred from satellite retrievals constrain effective radiative forcing of aerosol–cloud interactions
Global aerosol-type classification using a new hybrid algorithm and Aerosol Robotic Network data
Tropospheric aerosols over the western North Atlantic Ocean during the winter and summer campaigns of ACTIVATE 2020: Life cycle, transport, and distribution
Simulated phase state and viscosity of secondary organic aerosols over China
Zhouyang Zhang, Jiandong Wang, Jiaping Wang, Nicole Riemer, Chao Liu, Yuzhi Jin, Zeyuan Tian, Jing Cai, Yueyue Cheng, Ganzhen Chen, Bin Wang, Shuxiao Wang, and Aijun Ding
Atmos. Chem. Phys., 25, 1869–1881, https://doi.org/10.5194/acp-25-1869-2025, https://doi.org/10.5194/acp-25-1869-2025, 2025
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Black carbon (BC) exerts notable warming effects. We use a particle-resolved model to investigate the long-term behavior of the BC mixing state, revealing its compositions, coating thickness distribution, and optical properties all stabilize with a characteristic time of less than 1 d. This study can effectively simplify the description of the BC mixing state, which facilitates the precise assessment of the optical properties of BC aerosols in global and chemical transport models.
Qianyi Huo, Zhicong Yin, Xiaoqing Ma, and Huijun Wang
Atmos. Chem. Phys., 25, 1711–1724, https://doi.org/10.5194/acp-25-1711-2025, https://doi.org/10.5194/acp-25-1711-2025, 2025
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Dust days during the spring seasons of 2015–2023 in North China were classified into Mongolian cyclone and cold high types depending on the presence of the Mongolian cyclone. The Mongolian cyclone type led to more frequent and severe dust weather, indicated by PM10 concentrations. To comprehensively forecast the two types of dust weather, a common predictor was established based on 500 hPa anomalous circulation systems, offering insights for dust weather forecasting and climate prediction.
Mariya Petrenko, Ralph Kahn, Mian Chin, Susanne E. Bauer, Tommi Bergman, Huisheng Bian, Gabriele Curci, Ben Johnson, Johannes W. Kaiser, Zak Kipling, Harri Kokkola, Xiaohong Liu, Keren Mezuman, Tero Mielonen, Gunnar Myhre, Xiaohua Pan, Anna Protonotariou, Samuel Remy, Ragnhild Bieltvedt Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Hailong Wang, Duncan Watson-Parris, and Kai Zhang
Atmos. Chem. Phys., 25, 1545–1567, https://doi.org/10.5194/acp-25-1545-2025, https://doi.org/10.5194/acp-25-1545-2025, 2025
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We compared smoke plume simulations from 11 global models to each other and to satellite smoke amount observations aimed at constraining smoke source strength. In regions where plumes are thick and background aerosol is low, models and satellites compare well. However, the input emission inventory tends to underestimate in many places, and particle property and loss rate assumptions vary enormously among models, causing uncertainties that require systematic in situ measurements to resolve.
Yongqing Bai, Tianliang Zhao, Kai Meng, Yue Zhou, Jie Xiong, Xiaoyun Sun, Lijuan Shen, Yanyu Yue, Yan Zhu, Weiyang Hu, and Jingyan Yao
Atmos. Chem. Phys., 25, 1273–1287, https://doi.org/10.5194/acp-25-1273-2025, https://doi.org/10.5194/acp-25-1273-2025, 2025
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We proposed a composite statistical method to identify the quasi-weekly oscillation (QWO) of regional PM2.5 transport over China in winter from 2015 to 2019. The QWO of regional PM2.5 transport is constrained by synoptic-scale disturbances of the East Asian winter monsoon circulation with the periodic activities of the Siberian high, providing a new insight into the understanding of regional pollutant transport with meteorological drivers in atmospheric environment changes.
Léo Clauzel, Sandrine Anquetin, Christophe Lavaysse, Gilles Bergametti, Christel Bouet, Guillaume Siour, Rémy Lapere, Béatrice Marticorena, and Jennie Thomas
Atmos. Chem. Phys., 25, 997–1021, https://doi.org/10.5194/acp-25-997-2025, https://doi.org/10.5194/acp-25-997-2025, 2025
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Solar energy production in West Africa is set to rise and needs accurate solar radiation estimates which are affected by desert dust. This work analyses a March 2021 dust event using a modelling strategy incorporating desert dust. Results show that considering desert dust cuts errors in solar radiation estimates by 75 % and reduces surface solar radiation by 18 %. This highlights the importance of incorporating dust aerosols into solar forecasting for better accuracy.
Ross J. Herbert, Alberto Sanchez-Marroquin, Daniel P. Grosvenor, Kirsty J. Pringle, Stephen R. Arnold, Benjamin J. Murray, and Kenneth S. Carslaw
Atmos. Chem. Phys., 25, 291–325, https://doi.org/10.5194/acp-25-291-2025, https://doi.org/10.5194/acp-25-291-2025, 2025
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Aerosol particles that help form ice in clouds vary in number and type around the world and with time. However, in many weather and climate models cloud ice is not linked to aerosols that are known to nucleate ice. Here we report the first steps towards representing ice-nucleating particles within the UK Earth System Model. We conclude that in addition to ice nucleation by sea spray and mineral components of soil dust, we also need to represent ice nucleation by the organic components of soils.
Ryan Schmedding and Andreas Zuend
Atmos. Chem. Phys., 25, 327–346, https://doi.org/10.5194/acp-25-327-2025, https://doi.org/10.5194/acp-25-327-2025, 2025
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Four different approaches for computing the interfacial tension between liquid phases in aerosol particles were tested for particles with diameters from 10 nm to more than 5 μm. Antonov's rule led to the strongest reductions in the onset relative humidity of liquid–liquid phase separation and reproduced measured interfacial tensions for highly immiscible systems. A modified form of the Butler equation was able to best reproduce measured interfacial tensions in more miscible systems.
Masaru Yoshioka, Daniel P. Grosvenor, Ben B. B. Booth, Colin P. Morice, and Ken S. Carslaw
Atmos. Chem. Phys., 24, 13681–13692, https://doi.org/10.5194/acp-24-13681-2024, https://doi.org/10.5194/acp-24-13681-2024, 2024
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A 2020 regulation has reduced sulfur emissions from shipping by about 80 %, leading to a decrease in atmospheric aerosols that have a cooling effect primarily by affecting cloud properties and amounts. Our climate model simulations predict a global temperature increase of 0.04 K over the next 3 decades as a result, which could contribute to surpassing the Paris Agreement's 1.5 °C target. Reduced aerosols may have also contributed to the recent temperature spikes.
Alcide Zhao, Laura J. Wilcox, and Claire L. Ryder
Atmos. Chem. Phys., 24, 13385–13402, https://doi.org/10.5194/acp-24-13385-2024, https://doi.org/10.5194/acp-24-13385-2024, 2024
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Climate models include desert dust aerosols, which cause atmospheric heating and can change circulation patterns. We assess the effect of dust on the Indian and east Asian summer monsoons through multi-model experiments isolating the effect of dust in current climate models for the first time. Dust atmospheric heating results in a southward shift of western Pacific equatorial rainfall and an enhanced Indian summer monsoon. This shows the importance of accurate dust representation in models.
Ragnhild Bieltvedt Skeie, Rachael Byrom, Øivind Hodnebrog, Caroline Jouan, and Gunnar Myhre
Atmos. Chem. Phys., 24, 13361–13370, https://doi.org/10.5194/acp-24-13361-2024, https://doi.org/10.5194/acp-24-13361-2024, 2024
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In 2020, new regulations by the International Maritime Organization regarding sulfur emissions came into force, reducing emissions of SO2 from the shipping sector by approximately 80 %. In this study, we use multiple models to calculate how much the Earth energy balance changed due to the emission reduction or the so-called effective radiative forcing. The calculated effective radiative forcing is weak, comparable to the effect of the increase in CO2 over the last 2 to 3 years.
Mingxu Liu, Hitoshi Matsui, Douglas S. Hamilton, Sagar D. Rathod, Kara D. Lamb, and Natalie M. Mahowald
Atmos. Chem. Phys., 24, 13115–13127, https://doi.org/10.5194/acp-24-13115-2024, https://doi.org/10.5194/acp-24-13115-2024, 2024
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Atmospheric aerosol deposition provides bioavailable iron to promote marine primary production, yet the estimates of its fluxes remain highly uncertain. This study, by performing global aerosol simulations, demonstrates that iron-containing particle size upon emission is a critical factor in regulating soluble iron input to open oceans. Further observational constraints on this are needed to reduce modeling uncertainties.
Camelia Talianu, Jeni Vasilescu, Doina Nicolae, Alexandru Ilie, Andrei Dandocsi, Anca Nemuc, and Livio Belegante
EGUsphere, https://doi.org/10.5194/egusphere-2024-2930, https://doi.org/10.5194/egusphere-2024-2930, 2024
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Bucharest, Romania's capital, has successfully used mobile measurements and mixed-effects LUR models to derive seasonal maps of near-surface PM10, NO2, and UFP. The data was collected during two intensive campaigns, covering high-traffic streets, residential, industrial, and commercial districts. The model's performance was evaluated, demonstrating its potential for high-resolution mapping in other cities with well-characterized urban structures and diverse in situ monitoring stations.
Jingmin Li, Mattia Righi, Johannes Hendricks, Christof G. Beer, Ulrike Burkhardt, and Anja Schmidt
Atmos. Chem. Phys., 24, 12727–12747, https://doi.org/10.5194/acp-24-12727-2024, https://doi.org/10.5194/acp-24-12727-2024, 2024
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Aiming to understand underlying patterns and trends in aerosols, we characterize the spatial patterns and long-term evolution of lower tropospheric aerosols by clustering multiple aerosol properties from preindustrial times to the year 2050 under three Shared
Socioeconomic Pathway scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Socioeconomic Pathway scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Yueming Cheng, Tie Dai, Junji Cao, Daisuke Goto, Jianbing Jin, Teruyuki Nakajima, and Guangyu Shi
Atmos. Chem. Phys., 24, 12643–12659, https://doi.org/10.5194/acp-24-12643-2024, https://doi.org/10.5194/acp-24-12643-2024, 2024
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In March 2021, east Asia experienced an outbreak of severe dust storms after an absence of 1.5 decades. Here, we innovatively used the time-lagged ground-based aerosol size information with the fixed-lag ensemble Kalman smoother to optimize dust emission and reproduce the dust storm. This work is valuable for not only the quantification of health damage, aviation risks, and profound impacts on the Earth's system but also revealing the climatic driving force and the process of desertification.
Marc Mallet, Aurore Voldoire, Fabien Solmon, Pierre Nabat, Thomas Drugé, and Romain Roehrig
Atmos. Chem. Phys., 24, 12509–12535, https://doi.org/10.5194/acp-24-12509-2024, https://doi.org/10.5194/acp-24-12509-2024, 2024
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This study investigates the interactions between smoke aerosols and climate in tropical Africa using a coupled ocean–atmosphere–aerosol climate model. The work shows that smoke plumes have a significant impact by increasing the low-cloud fraction, decreasing the ocean and continental surface temperature and reducing the precipitation of coastal western Africa. It also highlights the role of the ocean temperature response and its feedbacks for the September–November season.
Jia Liu, Cancan Zhu, Donghui Zhou, and Jinbao Han
Atmos. Chem. Phys., 24, 12341–12354, https://doi.org/10.5194/acp-24-12341-2024, https://doi.org/10.5194/acp-24-12341-2024, 2024
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The hydrophilic coatings of aged black carbon (BC) particles absorb moisture during the hygroscopic growth process, but it is difficult to characterize how much water is absorbed under different relative humidities (RHs). In this study, we propose a method to obtain the water content in the coatings based on the equivalent complex refractive index retrieved from optical properties. This method is verified from a theoretical perspective, and it performs well for thickly coated BC at high RHs.
Zijun Li, Angela Buchholz, and Noora Hyttinen
Atmos. Chem. Phys., 24, 11717–11725, https://doi.org/10.5194/acp-24-11717-2024, https://doi.org/10.5194/acp-24-11717-2024, 2024
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Evaluating organosulfur (OS) hygroscopicity is important for assessing aerosol–cloud climate interactions in the post-fossil-fuel future, when SO2 emissions decrease and OS compounds become increasingly important. Here a state-of-the-art quantum-chemistry-based method was used to predict the hygroscopic growth factors (HGFs) of a group of atmospherically relevant OS compounds and their mixtures with (NH4)2SO4. A good agreement was observed between their model-estimated and experimental HGFs.
Jamie R. Banks, Bernd Heinold, and Kerstin Schepanski
Atmos. Chem. Phys., 24, 11451–11475, https://doi.org/10.5194/acp-24-11451-2024, https://doi.org/10.5194/acp-24-11451-2024, 2024
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The Aralkum is a new desert in Central Asia formed by the desiccation of the Aral Sea. This has created a source of atmospheric dust, with implications for the balance of solar and thermal radiation. Simulating these effects using a dust transport model, we find that Aralkum dust adds radiative cooling effects to the surface and atmosphere on average but also adds heating events. Increases in surface pressure due to Aralkum dust strengthen the Siberian High and weaken the summer Asian heat low.
Xinyue Shao, Minghuai Wang, Xinyi Dong, Yaman Liu, Wenxiang Shen, Stephen R. Arnold, Leighton A. Regayre, Meinrat O. Andreae, Mira L. Pöhlker, Duseong S. Jo, Man Yue, and Ken S. Carslaw
Atmos. Chem. Phys., 24, 11365–11389, https://doi.org/10.5194/acp-24-11365-2024, https://doi.org/10.5194/acp-24-11365-2024, 2024
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Highly oxygenated organic molecules (HOMs) play an important role in atmospheric new particle formation (NPF). By semi-explicitly coupling the chemical mechanism of HOMs and a comprehensive nucleation scheme in a global climate model, the updated model shows better agreement with measurements of nucleation rate, growth rate, and NPF event frequency. Our results reveal that HOM-driven NPF leads to a considerable increase in particle and cloud condensation nuclei burden globally.
Falei Xu, Shuang Wang, Yan Li, and Juan Feng
Atmos. Chem. Phys., 24, 10689–10705, https://doi.org/10.5194/acp-24-10689-2024, https://doi.org/10.5194/acp-24-10689-2024, 2024
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This study examines how the winter North Atlantic Oscillation (NAO) and El Niño–Southern Oscillation (ENSO) affect dust activities in North China during the following spring. The results show that the NAO and ENSO, particularly in their negative phases, greatly influence dust activities. When both are negative, their combined effect on dust activities is even greater. This research highlights the importance of these climate patterns in predicting spring dust activities in North China.
Hengheng Zhang, Wei Huang, Xiaoli Shen, Ramakrishna Ramisetty, Junwei Song, Olga Kiseleva, Christopher Claus Holst, Basit Khan, Thomas Leisner, and Harald Saathoff
Atmos. Chem. Phys., 24, 10617–10637, https://doi.org/10.5194/acp-24-10617-2024, https://doi.org/10.5194/acp-24-10617-2024, 2024
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Our study unravels how stagnant winter conditions elevate aerosol levels in Stuttgart. Cloud cover at night plays a pivotal role, impacting morning air quality. Validating a key model, our findings aid accurate air quality predictions, crucial for effective pollution mitigation in urban areas.
Giorgio Veratti, Alessandro Bigi, Michele Stortini, Sergio Teggi, and Grazia Ghermandi
Atmos. Chem. Phys., 24, 10475–10512, https://doi.org/10.5194/acp-24-10475-2024, https://doi.org/10.5194/acp-24-10475-2024, 2024
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In a study of two consecutive winter seasons, we used measurements and modelling tools to identify the levels and sources of black carbon pollution in a medium-sized urban area of the Po Valley, Italy. Our findings show that biomass burning and traffic-related emissions (especially from Euro 4 diesel cars) significantly contribute to BC concentrations. This research offers crucial insights for policymakers and urban planners aiming to improve air quality in cities.
Jiangtao Li, Xingqin An, Zhaobin Sun, Caihua Ye, Qing Hou, Yuxin Zhao, and Zhe Liu
EGUsphere, https://doi.org/10.5194/egusphere-2024-2000, https://doi.org/10.5194/egusphere-2024-2000, 2024
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Climate change and pollution have intensified pollen allergies. We developed a pollen emissions model using phenology and random forests. Key factors affecting annual pollen emissions include temperature, relative humidity, and sunshine hours. Pollen dispersal starts around August 10, peaks around August 30, and ends by September 25, lasting about 45 days. Over time, annual pollen emissions exhibit significant fluctuations and a downward trend.
Pascal Lemaitre, Arnaud Quérel, Alexis Dépée, Alice Guerra Devigne, Marie Monier, Thibault Hiron, Chloé Soto Minguez, Daniel Hardy, and Andrea Flossmann
Atmos. Chem. Phys., 24, 9713–9732, https://doi.org/10.5194/acp-24-9713-2024, https://doi.org/10.5194/acp-24-9713-2024, 2024
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A new in-cloud scavenging scheme is proposed. It is based on a microphysical model of cloud formation and may be applied to long-distance atmospheric transport models (> 100 km) and climatic models. This model is applied to the two most extreme precipitating cloud types in terms of both relative humidity and vertical extension: cumulonimbus and stratus.
Alex Rowell, James Brean, David C. S. Beddows, Tuukka Petäjä, Máté Vörösmarty, Imre Salma, Jarkko V. Niemi, Hanna E. Manninen, Dominik van Pinxteren, Thomas Tuch, Kay Weinhold, Zongbo Shi, and Roy M. Harrison
Atmos. Chem. Phys., 24, 9515–9531, https://doi.org/10.5194/acp-24-9515-2024, https://doi.org/10.5194/acp-24-9515-2024, 2024
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Different sources of airborne particles in the atmospheres of four European cities were distinguished by recognising their particle size distributions using a statistical procedure, positive matrix factorisation. The various sources responded differently to the changes in emissions associated with COVID-19 lockdowns, and the reasons are investigated. While traffic emissions generally decreased, particles formed from reactions of atmospheric gases decreased in some cities but increased in others.
Amy H. Peace, Ying Chen, George Jordan, Daniel G. Partridge, Florent Malavelle, Eliza Duncan, and Jim M. Haywood
Atmos. Chem. Phys., 24, 9533–9553, https://doi.org/10.5194/acp-24-9533-2024, https://doi.org/10.5194/acp-24-9533-2024, 2024
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Natural aerosols from volcanic eruptions can help us understand how anthropogenic aerosols modify climate. We use observations and model simulations of the 2014–2015 Holuhraun eruption plume to examine aerosol–cloud interactions in September 2014. We find a shift to clouds with smaller, more numerous cloud droplets in the first 2 weeks of the eruption. In the third week, the background meteorology and previous conditions experienced by air masses modulate the aerosol perturbation to clouds.
Hua Lu, Min Xie, Bingliang Zhuang, Danyang Ma, Bojun Liu, Yangzhihao Zhan, Tijian Wang, Shu Li, Mengmeng Li, and Kuanguang Zhu
Atmos. Chem. Phys., 24, 8963–8982, https://doi.org/10.5194/acp-24-8963-2024, https://doi.org/10.5194/acp-24-8963-2024, 2024
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To identify cloud, aerosol, and planetary boundary layer (PBL) interactions from an air quality perspective, we summarized two pollution patterns characterized by denser liquid cloud and by obvious cloud radiation interaction (CRI). Numerical simulation experiments showed CRI could cause a 50 % reduction in aerosol radiation interaction (ARI) under a low-trough system. The results emphasized the nonnegligible role of CRI and its inhibition of ARI under wet and cloudy pollution synoptic patterns.
Zhe Song, Ningning Yao, Lang Chen, Yuhai Sun, Boqiong Jiang, Pengfei Li, Daniel Rosenfeld, and Shaocai Yu
EGUsphere, https://doi.org/10.5194/egusphere-2024-2263, https://doi.org/10.5194/egusphere-2024-2263, 2024
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Our results with injected sea-salt aerosols for five open oceans show that the sea-salt aerosols with low injection amounts dominated the shortwave radiation mainly through the indirect effects. As indirect aerosol effects saturated with increasing injection rates, direct effects exceeded indirect effects. This implies that marine cloud brightening was best implemented in areas with extensive cloud cover, while the aerosol direct scattering effects remained dominant when clouds were scarce.
Yuzhi Jin, Jiandong Wang, David C. Wong, Chao Liu, Golam Sarwar, Kathleen M. Fahey, Shang Wu, Jiaping Wang, Jing Cai, Zeyuan Tian, Zhouyang Zhang, Jia Xing, Aijun Ding, and Shuxiao Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-2372, https://doi.org/10.5194/egusphere-2024-2372, 2024
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Black carbon (BC) affects climate and the environment, and its aging process alters its properties. Current models, like WRF-CMAQ, lack full account. We developed the WRF-CMAQ-BCG model to better represent BC aging by introducing Bare/Coated BC species and their conversion. Our findings show that BC mixing states have distinct spatiotemporal distribution characteristics, and BC wet deposition is dominated by Coated BC. Accounting for BC aging process improves aerosol optics simulation accuracy.
Emilie Fons, Ann Kristin Naumann, David Neubauer, Theresa Lang, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 8653–8675, https://doi.org/10.5194/acp-24-8653-2024, https://doi.org/10.5194/acp-24-8653-2024, 2024
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Aerosols can modify the liquid water path (LWP) of stratocumulus and, thus, their radiative effect. We compare storm-resolving model and satellite data that disagree on the sign of LWP adjustments and diagnose this discrepancy with causal inference. We find that strong precipitation, the absence of wet scavenging, and cloud deepening under a weak inversion contribute to positive LWP adjustments to aerosols in the model, despite weak negative effects from cloud-top entrainment enhancement.
Muhammed Irfan, Thomas Kühn, Taina Yli-Juuti, Anton Laakso, Eemeli Holopainen, Douglas R. Worsnop, Annele Virtanen, and Harri Kokkola
Atmos. Chem. Phys., 24, 8489–8506, https://doi.org/10.5194/acp-24-8489-2024, https://doi.org/10.5194/acp-24-8489-2024, 2024
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The study examines how the volatility of semi-volatile organic compounds affects secondary organic aerosol (SOA) formation and climate. Our simulations show that uncertainties in these volatilities influence aerosol mass and climate impacts. Accurate representation of these compounds in climate models is crucial for predicting global climate patterns.
Hector Navarro-Barboza, Jordi Rovira, Vincenzo Obiso, Andrea Pozzer, Marta Via, Andres Alastuey, Xavier Querol, Noemi Perez, Marjan Savadkoohi, Gang Chen, Jesus Yus-Díez, Matic Ivancic, Martin Rigler, Konstantinos Eleftheriadis, Stergios Vratolis, Olga Zografou, Maria Gini, Benjamin Chazeau, Nicolas Marchand, Andre Prevot, Kaspar Dallenbach, Mikael Ehn, Krista Luoma, Tuukka Petäjä, Anna Tobler, Jaroslaw Necki, Minna Aurela, Hilkka Timonen, Jarkko Niemi, Olivier Favez, Jean-Eudes Petit, Jean-Philippe Putaud, Christoph Hueglin, Nicolas Pascal, Aurelien Chauvigné, Sebastien Conil, Marco Pandolfi, and Oriol Jorba
EGUsphere, https://doi.org/10.5194/egusphere-2024-2086, https://doi.org/10.5194/egusphere-2024-2086, 2024
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Brown carbon (BrC) absorbs UV and visible light, affecting climate. Our study investigates BrC's imaginary refractive index (k ) using data from 12 European sites. Residential emissions are a major OA source in winter, while secondary organic aerosols (SOA) dominate in summer. We derived source-specific k values, enhancing model accuracy. This research improves understanding of BrC's climate role, emphasizing the need for source-specific constraints in atmospheric models.
Mingrui Ma, Jiachen Cao, Dan Tong, Bo Zheng, and Yu Zhao
EGUsphere, https://doi.org/10.5194/egusphere-2024-1769, https://doi.org/10.5194/egusphere-2024-1769, 2024
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We combined two global climate change pathways and three national emission control scenarios to analyze the future evolution of Nr deposition till 2060s in China with air quality modeling. We demonstrate China’s clean air and carbon neutrality policies would overcome the adverse effect of climate change and efficiently reduce Nr deposition. The outflow of Nr fluxes from mainland China to West Pacific would also be clearly reduced from continuous stringent emission controls.
Ruth A. R. Digby, Knut von Salzen, Adam H. Monahan, Nathan P. Gillett, and Jiangnan Li
EGUsphere, https://doi.org/10.5194/egusphere-2024-1796, https://doi.org/10.5194/egusphere-2024-1796, 2024
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The refractive index of black carbon (BCRI), which determines how much energy black carbon absorbs and scatters, is difficult to measure and different climate models use different values. We show that varying the BCRI across commonly used values can increase absorbing aerosol optical depth by 42 % and the warming effect from interactions between black carbon and radiation by 47 %, an appreciable fraction of the overall spread between models reported in recent literature assessments.
Alkiviadis Kalisoras, Aristeidis K. Georgoulias, Dimitris Akritidis, Robert J. Allen, Vaishali Naik, Chaincy Kuo, Sophie Szopa, Pierre Nabat, Dirk Olivié, Twan van Noije, Philippe Le Sager, David Neubauer, Naga Oshima, Jane Mulcahy, Larry W. Horowitz, and Prodromos Zanis
Atmos. Chem. Phys., 24, 7837–7872, https://doi.org/10.5194/acp-24-7837-2024, https://doi.org/10.5194/acp-24-7837-2024, 2024
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Effective radiative forcing (ERF) is a metric for estimating how human activities and natural agents change the energy flow into and out of the Earth’s climate system. We investigate the anthropogenic aerosol ERF, and we estimate the contribution of individual processes to the total ERF using simulations from Earth system models within the Coupled Model Intercomparison Project Phase 6 (CMIP6). Our findings highlight that aerosol–cloud interactions drive ERF variability during the last 150 years.
Qianqian Song, Paul Ginoux, María Gonçalves Ageitos, Ron L. Miller, Vincenzo Obiso, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 7421–7446, https://doi.org/10.5194/acp-24-7421-2024, https://doi.org/10.5194/acp-24-7421-2024, 2024
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We implement and simulate the distribution of eight dust minerals in the GFDL AM4.0 model. We found that resolving the eight minerals reduces dust absorption compared to the homogeneous dust used in the standard GFDL AM4.0 model that assumes a globally uniform hematite content of 2.7 % by volume. Resolving dust mineralogy results in significant impacts on radiation, land surface temperature, surface winds, and precipitation over North Africa in summer.
Senyi Kong, Zheng Wang, and Lei Bi
Atmos. Chem. Phys., 24, 6911–6935, https://doi.org/10.5194/acp-24-6911-2024, https://doi.org/10.5194/acp-24-6911-2024, 2024
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The retrieval of refractive indices of dust aerosols from laboratory optical measurements is commonly done assuming spherical particles. This paper aims to investigate the uncertainties in the shortwave refractive indices and corresponding optical properties by considering non-spherical and inhomogeneous models for dust samples. The study emphasizes the significance of using non-spherical models for simulating dust aerosols.
Wenxuan Hua, Sijia Lou, Xin Huang, Lian Xue, Ke Ding, Zilin Wang, and Aijun Ding
Atmos. Chem. Phys., 24, 6787–6807, https://doi.org/10.5194/acp-24-6787-2024, https://doi.org/10.5194/acp-24-6787-2024, 2024
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In this study, we diagnose uncertainties in carbon monoxide and organic carbon emissions from four inventories for seven major wildfire-prone regions. Uncertainties in vegetation classification methods, fire detection products, and cloud obscuration effects lead to bias in these biomass burning (BB) emission inventories. By comparing simulations with measurements, we provide certain inventory recommendations. Our study has implications for reducing uncertainties in emissions in further studies.
Chandrakala Bharali, Mary Barth, Rajesh Kumar, Sachin D. Ghude, Vinayak Sinha, and Baerbel Sinha
Atmos. Chem. Phys., 24, 6635–6662, https://doi.org/10.5194/acp-24-6635-2024, https://doi.org/10.5194/acp-24-6635-2024, 2024
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This study examines the role of atmospheric aerosols in winter fog over the Indo-Gangetic Plains of India using WRF-Chem. The increase in RH with aerosol–radiation feedback (ARF) is found to be important for fog formation as it promotes the growth of aerosols in the polluted environment. Aqueous-phase chemistry in the fog increases PM2.5 concentration, further affecting ARF. ARF and aqueous-phase chemistry affect the fog intensity and the timing of fog formation by ~1–2 h.
Wenxin Zhao, Yu Zhao, Yu Zheng, Dong Chen, Jinyuan Xin, Kaitao Li, Huizheng Che, Zhengqiang Li, Mingrui Ma, and Yun Hang
Atmos. Chem. Phys., 24, 6593–6612, https://doi.org/10.5194/acp-24-6593-2024, https://doi.org/10.5194/acp-24-6593-2024, 2024
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We evaluate the long-term (2000–2020) variabilities of aerosol absorption optical depth, black carbon emissions, and associated health risks in China with an integrated framework that combines multiple observations and modeling techniques. We demonstrate the remarkable emission abatement resulting from the implementation of national pollution controls and show how human activities affected the emissions with a spatiotemporal heterogeneity, thus supporting differentiated policy-making by region.
Peng Xian, Jeffrey S. Reid, Melanie Ades, Angela Benedetti, Peter R. Colarco, Arlindo da Silva, Tom F. Eck, Johannes Flemming, Edward J. Hyer, Zak Kipling, Samuel Rémy, Tsuyoshi Thomas Sekiyama, Taichu Tanaka, Keiya Yumimoto, and Jianglong Zhang
Atmos. Chem. Phys., 24, 6385–6411, https://doi.org/10.5194/acp-24-6385-2024, https://doi.org/10.5194/acp-24-6385-2024, 2024
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The study compares and evaluates monthly AOD of four reanalyses (RA) and their consensus (i.e., ensemble mean). The basic verification characteristics of these RA versus both AERONET and MODIS retrievals are presented. The study discusses the strength of each RA and identifies regions where divergence and challenges are prominent. The RA consensus usually performs very well on a global scale in terms of how well it matches the observational data, making it a good choice for various applications.
Roger Teoh, Zebediah Engberg, Ulrich Schumann, Christiane Voigt, Marc Shapiro, Susanne Rohs, and Marc E. J. Stettler
Atmos. Chem. Phys., 24, 6071–6093, https://doi.org/10.5194/acp-24-6071-2024, https://doi.org/10.5194/acp-24-6071-2024, 2024
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The radiative forcing (RF) due to aviation contrails is comparable to that caused by CO2. We estimate that global contrail net RF in 2019 was 62.1 mW m−2. This is ~1/2 the previous best estimate for 2018. Contrail RF varies regionally due to differences in conditions required for persistent contrails. COVID-19 reduced contrail RF by 54% in 2020 relative to 2019. Globally, 2 % of all flights account for 80 % of the annual contrail energy forcing, suggesting a opportunity to mitigate contrail RF.
Haotian Zu, Biwu Chu, Yiqun Lu, Ling Liu, and Xiuhui Zhang
Atmos. Chem. Phys., 24, 5823–5835, https://doi.org/10.5194/acp-24-5823-2024, https://doi.org/10.5194/acp-24-5823-2024, 2024
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The nucleation of iodic acid (HIO3) and iodous acid (HIO2) was proven to be critical in marine areas. However, HIO3–HIO2 nucleation cannot effectively derive the rapid nucleation in some polluted coasts. We find a significant enhancement of dimethylamine (DMA) on the HIO3–HIO2 nucleation in marine and polar regions with abundant DMA sources, which may establish reasonable connections between the HIO3–HIO2 nucleation and the rapid formation of new particles in polluted marine and polar regions.
Junghwa Lee, Patric Seifert, Tempei Hashino, Maximilian Maahn, Fabian Senf, and Oswald Knoth
Atmos. Chem. Phys., 24, 5737–5756, https://doi.org/10.5194/acp-24-5737-2024, https://doi.org/10.5194/acp-24-5737-2024, 2024
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Spectral bin model simulations of an idealized supercooled stratiform cloud were performed with the AMPS model for variable CCN and INP concentrations. We performed radar forward simulations with PAMTRA to transfer the simulations into radar observational space. The derived radar reflectivity factors were compared to observational studies of stratiform mixed-phase clouds. These studies report a similar response of the radar reflectivity factor to aerosol perturbations as we found in our study.
Basudev Swain, Marco Vountas, Aishwarya Singh, Nidhi L. Anchan, Adrien Deroubaix, Luca Lelli, Yanick Ziegler, Sachin S. Gunthe, Hartmut Bösch, and John P. Burrows
Atmos. Chem. Phys., 24, 5671–5693, https://doi.org/10.5194/acp-24-5671-2024, https://doi.org/10.5194/acp-24-5671-2024, 2024
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Arctic amplification (AA) accelerates the warming of the central Arctic cryosphere and affects aerosol dynamics. Limited observations hinder a comprehensive analysis. This study uses AEROSNOW aerosol optical density (AOD) data and GEOS-Chem simulations to assess AOD variability. Discrepancies highlight the need for improved observational integration into models to refine our understanding of aerosol effects on cloud microphysics, ice nucleation, and radiative forcing under evolving AA.
Vincenzo Obiso, María Gonçalves Ageitos, Carlos Pérez García-Pando, Jan P. Perlwitz, Gregory L. Schuster, Susanne E. Bauer, Claudia Di Biagio, Paola Formenti, Kostas Tsigaridis, and Ron L. Miller
Atmos. Chem. Phys., 24, 5337–5367, https://doi.org/10.5194/acp-24-5337-2024, https://doi.org/10.5194/acp-24-5337-2024, 2024
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We calculate the dust direct radiative effect (DRE) in an Earth system model accounting for regionally varying soil mineralogy through a new observationally constrained method. Linking dust absorption at solar wavelengths to the varying amount of specific minerals (i.e., iron oxides) improves the modeled range of dust single scattering albedo compared to observations and increases the global cooling by dust. Our results may contribute to improved estimates of the dust DRE and its climate impact.
Charlotte M. Beall, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Adam Varble, Kentaroh Suzuki, and Takuro Michibata
Atmos. Chem. Phys., 24, 5287–5302, https://doi.org/10.5194/acp-24-5287-2024, https://doi.org/10.5194/acp-24-5287-2024, 2024
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Single-layer warm liquid clouds cover nearly one-third of the Earth's surface, and uncertainties regarding the impact of aerosols on their radiative properties pose a significant challenge to climate prediction. Here, we demonstrate how satellite observations can be used to constrain Earth system model estimates of the radiative forcing from the interactions of aerosols with clouds due to warm rain processes.
Xiaoli Wei, Qian Cui, Leiming Ma, Feng Zhang, Wenwen Li, and Peng Liu
Atmos. Chem. Phys., 24, 5025–5045, https://doi.org/10.5194/acp-24-5025-2024, https://doi.org/10.5194/acp-24-5025-2024, 2024
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A new aerosol-type classification algorithm has been proposed. It includes an optical database built by Mie scattering and a complex refractive index working as a baseline to identify different aerosol types. The new algorithm shows high accuracy and efficiency. Hence, a global map of aerosol types was generated to characterize aerosol types across the five continents. It will help improve the accuracy of aerosol inversion and determine the sources of aerosol pollution.
Hongyu Liu, Bo Zhang, Richard H. Moore, Luke D. Ziemba, Richard A. Ferrare, Hyundeok Choi, Armin Sorooshian, David Painemal, Hailong Wang, Michael A. Shook, Amy Jo Scarino, Johnathan W. Hair, Ewan C. Crosbie, Marta A. Fenn, Taylor J. Shingler, Chris A. Hostetler, Gao Chen, Mary M. Kleb, Gan Luo, Fangqun Yu, Jason L. Tackett, Mark A. Vaughan, Yongxiang Hu, Glenn S. Diskin, John B. Nowak, Joshua P. DiGangi, Yonghoon Choi, Christoph A. Keller, and Matthew S. Johnson
EGUsphere, https://doi.org/10.5194/egusphere-2024-1127, https://doi.org/10.5194/egusphere-2024-1127, 2024
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We use the GEOS-Chem model to simulate aerosols over the western North Atlantic Ocean (WNAO) during the winter and summer campaigns of ACTIVATE 2020. Model results are evaluated against in situ and remote sensing measurements from two aircraft as well as ground-based and satellite observations. The improved understanding of the aerosol life cycle, composition, transport pathways, and distribution has important implications for characterizing aerosol-cloud-meteorology interactions over the WNAO.
Zhiqiang Zhang, Ying Li, Haiyan Ran, Junling An, Yu Qu, Wei Zhou, Weiqi Xu, Weiwei Hu, Hongbin Xie, Zifa Wang, Yele Sun, and Manabu Shiraiwa
Atmos. Chem. Phys., 24, 4809–4826, https://doi.org/10.5194/acp-24-4809-2024, https://doi.org/10.5194/acp-24-4809-2024, 2024
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Secondary organic aerosols (SOAs) can exist in liquid, semi-solid, or amorphous solid states, which are rarely accounted for in current chemical transport models. We predict the phase state of SOA particles over China and find that in northwestern China SOA particles are mostly highly viscous or glassy solid. Our results indicate that the particle phase state should be considered in SOA formation in chemical transport models for more accurate prediction of SOA mass concentrations.
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Executive editor
Wildfires enhance surface PM2.5 concentration and thus adversely affect air quality and human health. Based on online-coupled fire-climate-ecosystem model simulations, this paper projects a nearly 2-fold increase in wildfire-induced summer-mean surface PM2.5 by the mid-21st century over North America. The projected enhancement is substantial even in the less-densely forested eastern US - as already manifested in the poor air quality as observed in June 2023 due to Canadian wildfires -, which is attributed to the transport of smoke from North America as well as positive climatic feedback of smoke on PM2.5. Thus, future regulatory controls on PM2.5 in North America, particularly in the eastern US where anthropogenic emissions are falling, should consider the effect of future increases in wildfires.
Wildfires enhance surface PM2.5 concentration and thus adversely affect air quality and human...
Short summary
We show that for air quality, the densely populated eastern US may see even larger impacts of wildfires due to long-distance smoke transport and associated positive climatic impacts, partially compensating the improvements from regulations on anthropogenic emissions. This study highlights the tension between natural and anthropogenic contributions and the non-local nature of air pollution that complicate regulatory strategies for improving future regional air quality for human health.
We show that for air quality, the densely populated eastern US may see even larger impacts of...
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