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ACP | Articles | Volume 20, issue 8
Atmos. Chem. Phys., 20, 4593–4605, 2020
https://doi.org/10.5194/acp-20-4593-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.

Special issue: Multiphase chemistry of secondary aerosol formation under...

Atmos. Chem. Phys., 20, 4593–4605, 2020
https://doi.org/10.5194/acp-20-4593-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.

Research article 21 Apr 2020

Research article | 21 Apr 2020

The evolutionary behavior of chromophoric brown carbon during ozone aging of fine particles from biomass burning

Xingjun Fan et al.

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Andreae, M. O. and Gelencsér, A.: Black carbon or brown carbon? The nature of light-absorbing carbonaceous aerosols, Atmos. Chem. Phys., 6, 3131–3148, https://doi.org/10.5194/acp-6-3131-2006, 2006. 
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Bond, T. C.: A technology-based global inventory of black and organic carbon emissions from combustion, J. Geophys. Res., 109, D14203, https://doi.org/10.1029/2003jd003697, 2004. 
Chang, J. L. and Thompson, J. E.: Characterization of colored products formed during irradiation of aqueous solutions containing H2O2 and phenolic compounds, Atmos. Environ., 44, 541–551, https://doi.org/10.1016/j.atmosenv.2009.10.042, 2010. 
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A particle-phase O3 oxidation of biomass burning (BB) smoke particles was conducted to investigate the evolution of brown carbon (BrC) therein. The O3 aging induced the decomposition of chromophores and fluorophores. EEM–PARAFAC showed a predominant decomposition of protein-like substances and a gradual increase proportion of humic-like substances for BB BrC during O3 aging. The dynamic spectral behavior of chromophores and functional groups within BrC was further explored by 2D-COS.
A particle-phase O3 oxidation of biomass burning (BB) smoke particles was conducted to...
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