Articles | Volume 20, issue 8
https://doi.org/10.5194/acp-20-4593-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-20-4593-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
21 Apr 2020
Research article |
| 21 Apr 2020
| 21 Apr 2020
The evolutionary behavior of chromophoric brown carbon during ozone aging of fine particles from biomass burning
Xingjun Fan
CORRESPONDING AUTHOR
College of Resource and Environment, Anhui Science and Technology
University, Fengyang 233100, P. R. China
Anhui Province Key Laboratory of Biochar and Cropland Pollution
Prevention, Bengbu 233400, P. R. China
Tao Cao
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, P. R. China
University of Chinese Academy of Sciences, Beijing 100049, P. R. China
Xufang Yu
College of Resource and Environment, Anhui Science and Technology
University, Fengyang 233100, P. R. China
Yan Wang
College of Resource and Environment, Anhui Science and Technology
University, Fengyang 233100, P. R. China
Xin Xiao
College of Resource and Environment, Anhui Science and Technology
University, Fengyang 233100, P. R. China
Feiyue Li
College of Resource and Environment, Anhui Science and Technology
University, Fengyang 233100, P. R. China
Anhui Province Key Laboratory of Biochar and Cropland Pollution
Prevention, Bengbu 233400, P. R. China
Yue Xie
College of Resource and Environment, Anhui Science and Technology
University, Fengyang 233100, P. R. China
Wenchao Ji
College of Resource and Environment, Anhui Science and Technology
University, Fengyang 233100, P. R. China
Jianzhong Song
CORRESPONDING AUTHOR
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, P. R. China
Ping'an Peng
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, P. R. China
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Latest update: 23 Apr 2024
Short summary
A particle-phase O3 oxidation of biomass burning (BB) smoke particles was conducted to investigate the evolution of brown carbon (BrC) therein. The O3 aging induced the decomposition of chromophores and fluorophores. EEM–PARAFAC showed a predominant decomposition of protein-like substances and a gradual increase proportion of humic-like substances for BB BrC during O3 aging. The dynamic spectral behavior of chromophores and functional groups within BrC was further explored by 2D-COS.
A particle-phase O3 oxidation of biomass burning (BB) smoke particles was conducted to...
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