Articles | Volume 18, issue 16
https://doi.org/10.5194/acp-18-12491-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-12491-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
29 Aug 2018
Research article |
| 29 Aug 2018
| 29 Aug 2018
How reliable are CMIP5 models in simulating dust optical depth?
Atmospheric and Oceanic Sciences Program, Princeton University, Princeton, New Jersey 08544, USA
NOAA Geophysical Fluid Dynamics Laboratory, Princeton, New Jersey
08540, USA
Paul Ginoux
NOAA Geophysical Fluid Dynamics Laboratory, Princeton, New Jersey
08540, USA
Related authors
Brian Harr, Bing Pu, and Qinjian Jin
Atmos. Chem. Phys., 24, 8625–8651, https://doi.org/10.5194/acp-24-8625-2024, https://doi.org/10.5194/acp-24-8625-2024, 2024
Short summary
Short summary
We found that the formation of the extreme trans-Atlantic African dust event in June 2015 was associated with a brief surge in dust emissions over western North Africa and extreme circulation patterns, including intensified easterly jets, which facilitated the westward transport of dust. The dust plume modified radiative flux along its transport pathway but had minor impacts on air quality in the US due to the record-high Caribbean low-level jet advecting part of the plume to the Pacific.
Jacob Z. Tindan, Qinjian Jin, and Bing Pu
Atmos. Chem. Phys., 23, 5435–5466, https://doi.org/10.5194/acp-23-5435-2023, https://doi.org/10.5194/acp-23-5435-2023, 2023
Short summary
Short summary
We use the Infrared Atmospheric Sounder Interferometer (IASI) retrievals of dust variables (dust optical depth and dust layer height) and surface observations to understand the day- and nighttime variations in dust aerosols over the dust belt. Our results show that daytime dust aerosols are significantly different from nighttime, and such day–night variations are influenced by meteorological factors such as wind speed, precipitation, and turbulent motions within the atmospheric boundary layer.
Bing Pu, Paul Ginoux, Huan Guo, N. Christina Hsu, John Kimball, Beatrice Marticorena, Sergey Malyshev, Vaishali Naik, Norman T. O'Neill, Carlos Pérez García-Pando, Juliette Paireau, Joseph M. Prospero, Elena Shevliakova, and Ming Zhao
Atmos. Chem. Phys., 20, 55–81, https://doi.org/10.5194/acp-20-55-2020, https://doi.org/10.5194/acp-20-55-2020, 2020
Short summary
Short summary
Dust emission initiates when surface wind velocities exceed a threshold depending on soil and surface characteristics and varying spatially and temporally. Climate models widely use wind erosion thresholds. The climatological monthly global distribution of the wind erosion threshold, Vthreshold, is retrieved using satellite and reanalysis products and improves the simulation of dust frequency, magnitude, and the seasonal cycle in the Geophysical Fluid Dynamics Laboratory land–atmosphere model.
Bing Pu and Paul Ginoux
Atmos. Chem. Phys., 18, 4201–4215, https://doi.org/10.5194/acp-18-4201-2018, https://doi.org/10.5194/acp-18-4201-2018, 2018
Short summary
Short summary
Fine dust (< 2.5 microns) is an important component of the total PM2.5 mass in the western and central US in spring and summer and has positive trends. However, the causes of the trends have not been thoroughly discussed by previous studies. This work identified key local factors controlling the variations in fine dust in the US and found that the increase in fine dust in the central Great Plains in summer is associated with increasing atmospheric stability.
Bing Pu and Paul Ginoux
Atmos. Chem. Phys., 16, 13431–13448, https://doi.org/10.5194/acp-16-13431-2016, https://doi.org/10.5194/acp-16-13431-2016, 2016
Short summary
Short summary
Dust aerosols play an important role in the climate system. Strong dust storms also have severe social and health impacts. The 2015 severe dust storm in Syria raised concerns as to whether dust activities will increase in the region. The first step toward answering this question is to understand the dust activities driven by the natural climate variability. This work found that the Pacific Decadal Oscillation plays a dominant role in springtime dust activities in Syria in the recent decade.
Adolfo González-Romero, Cristina González-Flórez, Agnesh Panta, Jesús Yus-Díez, Patricia Córdoba, Andres Alastuey, Natalia Moreno, Melani Hernández-Chiriboga, Konrad Kandler, Martina Klose, Roger N. Clark, Bethany L. Ehlmann, Rebecca N. Greenberger, Abigail M. Keebler, Phil Brodrick, Robert Green, Paul Ginoux, Xavier Querol, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 9155–9176, https://doi.org/10.5194/acp-24-9155-2024, https://doi.org/10.5194/acp-24-9155-2024, 2024
Short summary
Short summary
In this research, we studied the dust-emitting properties of crusts and aeolian ripples from the Mojave Desert. These properties are key to understanding the effect of dust upon climate. We found two different playa lakes according to the groundwater regime, which implies differences in crusts' cohesion state and mineralogy, which can affect the dust emission potential and properties. We also compare them with Moroccan Sahara crusts and Icelandic top sediments.
Brian Harr, Bing Pu, and Qinjian Jin
Atmos. Chem. Phys., 24, 8625–8651, https://doi.org/10.5194/acp-24-8625-2024, https://doi.org/10.5194/acp-24-8625-2024, 2024
Short summary
Short summary
We found that the formation of the extreme trans-Atlantic African dust event in June 2015 was associated with a brief surge in dust emissions over western North Africa and extreme circulation patterns, including intensified easterly jets, which facilitated the westward transport of dust. The dust plume modified radiative flux along its transport pathway but had minor impacts on air quality in the US due to the record-high Caribbean low-level jet advecting part of the plume to the Pacific.
Manon Gaillard, Vincent Vionnet, Matthieu Lafaysse, Marie Dumont, and Paul Ginoux
EGUsphere, https://doi.org/10.5194/egusphere-2024-1795, https://doi.org/10.5194/egusphere-2024-1795, 2024
Short summary
Short summary
This study presents an efficient method to improve large-scale snow albedo simulations by considering the spatial variability of light-absorbing particles (LAPs) like black carbon and dust. A global climatology of LAP deposition was created and used to optimize a parameter in the Crocus snow model. Testing at ten global sites improved albedo predictions by 10 % on average and over 25 % in the Arctic. This method can also enhance other snow models' predictions without complex simulations.
Qianqian Song, Paul Ginoux, María Gonçalves Ageitos, Ron L. Miller, Vincenzo Obiso, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 7421–7446, https://doi.org/10.5194/acp-24-7421-2024, https://doi.org/10.5194/acp-24-7421-2024, 2024
Short summary
Short summary
We implement and simulate the distribution of eight dust minerals in the GFDL AM4.0 model. We found that resolving the eight minerals reduces dust absorption compared to the homogeneous dust used in the standard GFDL AM4.0 model that assumes a globally uniform hematite content of 2.7 % by volume. Resolving dust mineralogy results in significant impacts on radiation, land surface temperature, surface winds, and precipitation over North Africa in summer.
Enrico Zorzetto, Paul Ginoux, Sergey Malyshev, and Elena Shevliakova
EGUsphere, https://doi.org/10.5194/egusphere-2024-1258, https://doi.org/10.5194/egusphere-2024-1258, 2024
Short summary
Short summary
Light-absorbing particles (LAPs) deposition on snow leads to a darkening of the snow surface and can thus accelerate snow melt. Understanding to what extent different types of LAPs contribute to snow melt is important both to predict changes in water availability and for improving global climate model predictions. Here we extend a recently developed snow model to account for the deposition of LAPs in the snowpack and evaluate the effect of snow darkening on accelerating snow melt.
Enrico Zorzetto, Sergey Malyshev, Paul Ginoux, and Elena Shevliakova
EGUsphere, https://doi.org/10.5194/egusphere-2024-506, https://doi.org/10.5194/egusphere-2024-506, 2024
Short summary
Short summary
We describe a new snow scheme developed for use in global climate models, which simulates the interactions of snowpack with vegetation, atmosphere, and soil. We test the new snow model over a set of sites where in-situ observations are available. We find that, when compared to a simpler snow model, this model improves predictions of seasonal snow and of soil temperature under the snowpack, important variables for simulating both the hydrological cycle and the global climate system.
Jacob Z. Tindan, Qinjian Jin, and Bing Pu
Atmos. Chem. Phys., 23, 5435–5466, https://doi.org/10.5194/acp-23-5435-2023, https://doi.org/10.5194/acp-23-5435-2023, 2023
Short summary
Short summary
We use the Infrared Atmospheric Sounder Interferometer (IASI) retrievals of dust variables (dust optical depth and dust layer height) and surface observations to understand the day- and nighttime variations in dust aerosols over the dust belt. Our results show that daytime dust aerosols are significantly different from nighttime, and such day–night variations are influenced by meteorological factors such as wind speed, precipitation, and turbulent motions within the atmospheric boundary layer.
Qirui Zhong, Nick Schutgens, Guido van der Werf, Twan van Noije, Kostas Tsigaridis, Susanne E. Bauer, Tero Mielonen, Alf Kirkevåg, Øyvind Seland, Harri Kokkola, Ramiro Checa-Garcia, David Neubauer, Zak Kipling, Hitoshi Matsui, Paul Ginoux, Toshihiko Takemura, Philippe Le Sager, Samuel Rémy, Huisheng Bian, Mian Chin, Kai Zhang, Jialei Zhu, Svetlana G. Tsyro, Gabriele Curci, Anna Protonotariou, Ben Johnson, Joyce E. Penner, Nicolas Bellouin, Ragnhild B. Skeie, and Gunnar Myhre
Atmos. Chem. Phys., 22, 11009–11032, https://doi.org/10.5194/acp-22-11009-2022, https://doi.org/10.5194/acp-22-11009-2022, 2022
Short summary
Short summary
Aerosol optical depth (AOD) errors for biomass burning aerosol (BBA) are evaluated in 18 global models against satellite datasets. Notwithstanding biases in satellite products, they allow model evaluations. We observe large and diverse model biases due to errors in BBA. Further interpretations of AOD diversities suggest large biases exist in key processes for BBA which require better constraining. These results can contribute to further model improvement and development.
Enza Di Tomaso, Jerónimo Escribano, Sara Basart, Paul Ginoux, Francesca Macchia, Francesca Barnaba, Francesco Benincasa, Pierre-Antoine Bretonnière, Arnau Buñuel, Miguel Castrillo, Emilio Cuevas, Paola Formenti, María Gonçalves, Oriol Jorba, Martina Klose, Lucia Mona, Gilbert Montané Pinto, Michail Mytilinaios, Vincenzo Obiso, Miriam Olid, Nick Schutgens, Athanasios Votsis, Ernest Werner, and Carlos Pérez García-Pando
Earth Syst. Sci. Data, 14, 2785–2816, https://doi.org/10.5194/essd-14-2785-2022, https://doi.org/10.5194/essd-14-2785-2022, 2022
Short summary
Short summary
MONARCH reanalysis of desert dust aerosols extends the existing observation-based information for mineral dust monitoring by providing 3-hourly upper-air, surface and total column key geophysical variables of the dust cycle over Northern Africa, the Middle East and Europe, at a 0.1° horizontal resolution in a rotated grid, from 2007 to 2016. This work provides evidence of the high accuracy of this data set and its suitability for air quality and health and climate service applications.
Sujung Go, Alexei Lyapustin, Gregory L. Schuster, Myungje Choi, Paul Ginoux, Mian Chin, Olga Kalashnikova, Oleg Dubovik, Jhoon Kim, Arlindo da Silva, Brent Holben, and Jeffrey S. Reid
Atmos. Chem. Phys., 22, 1395–1423, https://doi.org/10.5194/acp-22-1395-2022, https://doi.org/10.5194/acp-22-1395-2022, 2022
Short summary
Short summary
This paper presents a retrieval algorithm of iron-oxide species (hematite, goethite) content in the atmosphere from DSCOVR EPIC observations. Our results display variations within the published range of hematite and goethite over the main dust-source regions but show significant seasonal and spatial variability. This implies a single-viewing satellite instrument with UV–visible channels may provide essential information on shortwave dust direct radiative effects for climate modeling.
Maria Sand, Bjørn H. Samset, Gunnar Myhre, Jonas Gliß, Susanne E. Bauer, Huisheng Bian, Mian Chin, Ramiro Checa-Garcia, Paul Ginoux, Zak Kipling, Alf Kirkevåg, Harri Kokkola, Philippe Le Sager, Marianne T. Lund, Hitoshi Matsui, Twan van Noije, Dirk J. L. Olivié, Samuel Remy, Michael Schulz, Philip Stier, Camilla W. Stjern, Toshihiko Takemura, Kostas Tsigaridis, Svetlana G. Tsyro, and Duncan Watson-Parris
Atmos. Chem. Phys., 21, 15929–15947, https://doi.org/10.5194/acp-21-15929-2021, https://doi.org/10.5194/acp-21-15929-2021, 2021
Short summary
Short summary
Absorption of shortwave radiation by aerosols can modify precipitation and clouds but is poorly constrained in models. A total of 15 different aerosol models from AeroCom phase III have reported total aerosol absorption, and for the first time, 11 of these models have reported in a consistent experiment the contributions to absorption from black carbon, dust, and organic aerosol. Here, we document the model diversity in aerosol absorption.
Martina Klose, Oriol Jorba, María Gonçalves Ageitos, Jeronimo Escribano, Matthew L. Dawson, Vincenzo Obiso, Enza Di Tomaso, Sara Basart, Gilbert Montané Pinto, Francesca Macchia, Paul Ginoux, Juan Guerschman, Catherine Prigent, Yue Huang, Jasper F. Kok, Ron L. Miller, and Carlos Pérez García-Pando
Geosci. Model Dev., 14, 6403–6444, https://doi.org/10.5194/gmd-14-6403-2021, https://doi.org/10.5194/gmd-14-6403-2021, 2021
Short summary
Short summary
Mineral soil dust is a major atmospheric airborne particle type. We present and evaluate MONARCH, a model used for regional and global dust-weather prediction. An important feature of the model is that it allows different approximations to represent dust, ranging from more simplified to more complex treatments. Using these different treatments, MONARCH can help us better understand impacts of dust in the Earth system, such as its interactions with radiation.
Qianqian Song, Zhibo Zhang, Hongbin Yu, Paul Ginoux, and Jerry Shen
Atmos. Chem. Phys., 21, 13369–13395, https://doi.org/10.5194/acp-21-13369-2021, https://doi.org/10.5194/acp-21-13369-2021, 2021
Short summary
Short summary
We present a satellite-derived global dust climatological record over the last two decades, including the monthly mean visible dust optical depth (DAOD) and vertical distribution of dust extinction coefficient at a 2º × 5º spatial resolution derived from CALIOP and MODIS. In addition, the CALIOP climatological dataset also includes dust vertical extinction profiles. Based on these two datasets, we carried out a comprehensive comparative study of the spatial and temporal climatology of dust.
Jun Meng, Randall V. Martin, Paul Ginoux, Melanie Hammer, Melissa P. Sulprizio, David A. Ridley, and Aaron van Donkelaar
Geosci. Model Dev., 14, 4249–4260, https://doi.org/10.5194/gmd-14-4249-2021, https://doi.org/10.5194/gmd-14-4249-2021, 2021
Short summary
Short summary
Dust emissions in models, for example, GEOS-Chem, have a strong nonlinear dependence on meteorology, which means dust emission strengths calculated from different resolution meteorological fields are different. Offline high-resolution dust emissions with an optimized global dust strength, presented in this work, can be implemented into GEOS-Chem as offline emission inventory so that it could promote model development by harmonizing dust emissions across simulations of different resolutions.
Yan Yu and Paul Ginoux
Atmos. Chem. Phys., 21, 8511–8530, https://doi.org/10.5194/acp-21-8511-2021, https://doi.org/10.5194/acp-21-8511-2021, 2021
Short summary
Short summary
Despite Australian dust’s critical role in the regional climate and surrounding marine ecosystems, the controlling factors of its spatiotemporal variations are not fully understood. This study establishes the connection between large-scale climate variability and regional dust emission, leading to a better understanding of the spatiotemporal variation in dust activity and improved prediction of dust's climate and ecological influences.
Longlei Li, Natalie M. Mahowald, Ron L. Miller, Carlos Pérez García-Pando, Martina Klose, Douglas S. Hamilton, Maria Gonçalves Ageitos, Paul Ginoux, Yves Balkanski, Robert O. Green, Olga Kalashnikova, Jasper F. Kok, Vincenzo Obiso, David Paynter, and David R. Thompson
Atmos. Chem. Phys., 21, 3973–4005, https://doi.org/10.5194/acp-21-3973-2021, https://doi.org/10.5194/acp-21-3973-2021, 2021
Short summary
Short summary
For the first time, this study quantifies the range of the dust direct radiative effect due to uncertainty in the soil mineral abundance using all currently available information. We show that the majority of the estimated direct radiative effect range is due to uncertainty in the simulated mass fractions of iron oxides and thus their soil abundance, which is independent of the model employed. We therefore prove the necessity of considering mineralogy for understanding dust–climate interactions.
Jonas Gliß, Augustin Mortier, Michael Schulz, Elisabeth Andrews, Yves Balkanski, Susanne E. Bauer, Anna M. K. Benedictow, Huisheng Bian, Ramiro Checa-Garcia, Mian Chin, Paul Ginoux, Jan J. Griesfeller, Andreas Heckel, Zak Kipling, Alf Kirkevåg, Harri Kokkola, Paolo Laj, Philippe Le Sager, Marianne Tronstad Lund, Cathrine Lund Myhre, Hitoshi Matsui, Gunnar Myhre, David Neubauer, Twan van Noije, Peter North, Dirk J. L. Olivié, Samuel Rémy, Larisa Sogacheva, Toshihiko Takemura, Kostas Tsigaridis, and Svetlana G. Tsyro
Atmos. Chem. Phys., 21, 87–128, https://doi.org/10.5194/acp-21-87-2021, https://doi.org/10.5194/acp-21-87-2021, 2021
Short summary
Short summary
Simulated aerosol optical properties as well as the aerosol life cycle are investigated for 14 global models participating in the AeroCom initiative. Considerable diversity is found in the simulated aerosol species emissions and lifetimes, also resulting in a large diversity in the simulated aerosol mass, composition, and optical properties. A comparison with observations suggests that, on average, current models underestimate the direct effect of aerosol on the atmosphere radiation budget.
Augustin Mortier, Jonas Gliß, Michael Schulz, Wenche Aas, Elisabeth Andrews, Huisheng Bian, Mian Chin, Paul Ginoux, Jenny Hand, Brent Holben, Hua Zhang, Zak Kipling, Alf Kirkevåg, Paolo Laj, Thibault Lurton, Gunnar Myhre, David Neubauer, Dirk Olivié, Knut von Salzen, Ragnhild Bieltvedt Skeie, Toshihiko Takemura, and Simone Tilmes
Atmos. Chem. Phys., 20, 13355–13378, https://doi.org/10.5194/acp-20-13355-2020, https://doi.org/10.5194/acp-20-13355-2020, 2020
Short summary
Short summary
We present a multiparameter analysis of the aerosol trends over the last 2 decades in the different regions of the world. In most of the regions, ground-based observations show a decrease in aerosol content in both the total atmospheric column and at the surface. The use of climate models, assessed against these observations, reveals however an increase in the total aerosol load, which is not seen with the sole use of observation due to partial coverage in space and time.
Bing Pu, Paul Ginoux, Huan Guo, N. Christina Hsu, John Kimball, Beatrice Marticorena, Sergey Malyshev, Vaishali Naik, Norman T. O'Neill, Carlos Pérez García-Pando, Juliette Paireau, Joseph M. Prospero, Elena Shevliakova, and Ming Zhao
Atmos. Chem. Phys., 20, 55–81, https://doi.org/10.5194/acp-20-55-2020, https://doi.org/10.5194/acp-20-55-2020, 2020
Short summary
Short summary
Dust emission initiates when surface wind velocities exceed a threshold depending on soil and surface characteristics and varying spatially and temporally. Climate models widely use wind erosion thresholds. The climatological monthly global distribution of the wind erosion threshold, Vthreshold, is retrieved using satellite and reanalysis products and improves the simulation of dust frequency, magnitude, and the seasonal cycle in the Geophysical Fluid Dynamics Laboratory land–atmosphere model.
Fabien Paulot, David Paynter, Paul Ginoux, Vaishali Naik, and Larry W. Horowitz
Atmos. Chem. Phys., 18, 13265–13281, https://doi.org/10.5194/acp-18-13265-2018, https://doi.org/10.5194/acp-18-13265-2018, 2018
Short summary
Short summary
Observations show that the sunlight reflected to space by particles has decreased over the US and Europe, increased over India, and not changed over China from 2001 to 2015. These changes are attributed to different types of particles, namely sulfate over the US and Europe, and black carbon, sulfate, and nitrate over China and India. Our results suggest that the recent shift in human emissions from the US and Europe to Asia has altered their impact on the Earth's outgoing energy.
Jordan L. Schnell, Vaishali Naik, Larry W. Horowitz, Fabien Paulot, Jingqiu Mao, Paul Ginoux, Ming Zhao, and Kirpa Ram
Atmos. Chem. Phys., 18, 10157–10175, https://doi.org/10.5194/acp-18-10157-2018, https://doi.org/10.5194/acp-18-10157-2018, 2018
Short summary
Short summary
We evaluate the ability of a developmental version of the NOAA GFDL Atmospheric Model, version 4 to simulate observed wintertime pollution and its relationship to weather over Northern India, one of the most densely populated and polluted regions in world. We also compare two emission inventories and find that the newest version dramatically improves our simulation. Observed and modeled pollution is the highest within the Indo-Gangetic Plain, where it is closely related to near-surface weather.
Bing Pu and Paul Ginoux
Atmos. Chem. Phys., 18, 4201–4215, https://doi.org/10.5194/acp-18-4201-2018, https://doi.org/10.5194/acp-18-4201-2018, 2018
Short summary
Short summary
Fine dust (< 2.5 microns) is an important component of the total PM2.5 mass in the western and central US in spring and summer and has positive trends. However, the causes of the trends have not been thoroughly discussed by previous studies. This work identified key local factors controlling the variations in fine dust in the US and found that the increase in fine dust in the central Great Plains in summer is associated with increasing atmospheric stability.
Ilissa B. Ocko and Paul A. Ginoux
Atmos. Chem. Phys., 17, 4451–4475, https://doi.org/10.5194/acp-17-4451-2017, https://doi.org/10.5194/acp-17-4451-2017, 2017
Short summary
Short summary
Human-made liquid and solid particles (aerosols) are abundant in the atmosphere and play a central role in climate change. Computer models are essential tools for understanding how aerosols impact the climate, but it is critical to evaluate a model's performance by comparing with observations. Here we analyze aerosol properties in two world-renowned models by comparing with ground-based and satellite instrument data. We find that comparisons with all available data is valuable and essential.
Bing Pu and Paul Ginoux
Atmos. Chem. Phys., 16, 13431–13448, https://doi.org/10.5194/acp-16-13431-2016, https://doi.org/10.5194/acp-16-13431-2016, 2016
Short summary
Short summary
Dust aerosols play an important role in the climate system. Strong dust storms also have severe social and health impacts. The 2015 severe dust storm in Syria raised concerns as to whether dust activities will increase in the region. The first step toward answering this question is to understand the dust activities driven by the natural climate variability. This work found that the Pacific Decadal Oscillation plays a dominant role in springtime dust activities in Syria in the recent decade.
F. Paulot, P. Ginoux, W. F. Cooke, L. J. Donner, S. Fan, M.-Y. Lin, J. Mao, V. Naik, and L. W. Horowitz
Atmos. Chem. Phys., 16, 1459–1477, https://doi.org/10.5194/acp-16-1459-2016, https://doi.org/10.5194/acp-16-1459-2016, 2016
Short summary
Short summary
We characterize the sensitivity of NO3 optical depth (OD) to both the sources of its precursors (NH3 and HNO3) and to its surface sinks. Uncertainties in the heterogeneous chemistry of HNO3 and the near-surface volatilization of NH4NO3 can cause up to 25 % difference in the global NO3 OD. Simulated NO3 OD increases little (< 30 %) in response to changes in emissions (2010 to 2050). Better constraints on the tropical flux of NH3 into the free troposphere are needed to improve estimates of NO3 OD.
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Measurement report: Source attribution and estimation of black carbon levels in an urban hotspot of the central Po Valley – an integrated approach combining high-resolution dispersion modelling and micro-aethalometers
Microphysical modelling of aerosol scavenging by different types of clouds: description and validation of the approach
Insights into the sources of ultrafine particle numbers at six European urban sites obtained by investigating COVID-19 lockdowns
In-plume and out-of-plume analysis of aerosol–cloud interactions derived from the 2014–2015 Holuhraun volcanic eruption
Impacts of atmospheric circulation patterns and cloud inhibition on aerosol radiative effect and boundary layer structure during winter air pollution in Sichuan Basin, China
Investigating the sign of stratocumulus adjustments to aerosols in the ICON global storm-resolving model
A model study investigating the sensitivity of aerosol forcing to the volatilities of semi-volatile organic compounds
Decomposing the effective radiative forcing of anthropogenic aerosols based on CMIP6 Earth system models
Modeling impacts of dust mineralogy on fast climate response
Uncertainties in laboratory-measured shortwave refractive indices of mineral dust aerosols and derived optical properties: a theoretical assessment
Diagnosing uncertainties in global biomass burning emission inventories and their impact on modeled air pollutants
Role of atmospheric aerosols in severe winter fog over the Indo-Gangetic Plain of India: a case study
Long-term variability in black carbon emissions constrained by gap-filled absorption aerosol optical depth and associated premature mortality in China
Intercomparison of aerosol optical depths from four reanalyses and their multi-reanalysis consensus
Global aviation contrail climate effects from 2019 to 2021
Rapid iodine oxoacid nucleation enhanced by dimethylamine in broad marine regions
Simulations of the impact of cloud condensation nuclei and ice-nucleating particles perturbations on the microphysics and radar reflectivity factor of stratiform mixed-phase clouds
Aerosols in the central Arctic cryosphere: satellite and model integrated insights during Arctic spring and summer
Observationally constrained regional variations of shortwave absorption by iron oxides emphasize the cooling effect of dust
Droplet collection efficiencies inferred from satellite retrievals constrain effective radiative forcing of aerosol–cloud interactions
Predicting Hygroscopic Growth of Organosulfur Aerosol Particles Using COSMOtherm
Global aerosol-type classification using a new hybrid algorithm and Aerosol Robotic Network data
Simulated phase state and viscosity of secondary organic aerosols over China
Comparing the simulated influence of biomass burning plumes on low-level clouds over the southeastern Atlantic under varying smoke conditions
Improved simulations of biomass burning aerosol optical properties and lifetimes in the NASA GEOS Model during the ORACLES-I campaign
Retrieval of refractive index and water content for the coating materials of aged black carbon aerosol based on optical properties: a theoretical analysis
Revealing dominant patterns of aerosols regimes in the lower troposphere and their evolution from preindustrial times to the future in global climate model simulations
Synergistic effects of previous winter NAO and ENSO on the spring dust activities in North China
Sharp increase in Saharan dust intrusions over the western Euro-Mediterranean in February–March 2020–2022 and associated atmospheric circulation
Temporal and spatial variations in dust activity in Australia based on remote sensing and reanalysis datasets
Sensitivity of global direct aerosol shortwave radiative forcing to uncertainties in aerosol optical properties
Molecular-level study on the role of methanesulfonic acid in iodine oxoacid nucleation
Improving estimation of a record breaking East Asian dust storm emission with lagged aerosol Ångström Exponent observations
Regional to global distributions, trends, and drivers of biogenic volatile organic compound emission from 2001 to 2020
Impacts of ice-nucleating particles on cirrus clouds and radiation derived from global model simulations with MADE3 in EMAC
Seasonal characteristics of emission, distribution, and radiative effect of marine organic aerosols over the western Pacific Ocean: an investigation with a coupled regional climate aerosol model
Fire–precipitation interactions amplify the quasi-biennial variability in fires over southern Mexico and Central America
Improved estimates of smoke exposure during Australia fire seasons: importance of quantifying plume injection heights
New particle formation induced by anthropogenic–biogenic interactions on the southeastern Tibetan Plateau
Investigation of observed dust trends over the Middle East region in NASA Goddard Earth Observing System (GEOS) model simulations
Impact of Biomass Burning Aerosols (BBA) on the tropical African climate in an ocean-atmosphere-aerosols coupled climate model
A new process-based and scale-aware desert dust emission scheme for global climate models – Part II: Evaluation in the Community Earth System Model version 2 (CESM2)
How well do Earth system models reproduce the observed aerosol response to rapid emission reductions? A COVID-19 case study
Global modeling of aerosol nucleation with an explicit chemical mechanism for highly oxygenated organic molecules (HOMs)
Observationally constrained analysis of sulfur cycle in the marine atmosphere with NASA ATom measurements and AeroCom model simulations
Impact of acidity and surface-modulated acid dissociation on cloud response to organic aerosol
The contribution of residential wood combustion to the PM2.5 concentrations in the Helsinki metropolitan area
Analysis of atmospheric particle growth based on vapor concentrations measured at the high-altitude GAW station Chacaltaya in the Bolivian Andes
Expanding the simulation of East Asian super dust storms: physical transport mechanisms impacting the western Pacific
Aerosol composition, air quality, and boundary layer dynamics in the urban background of Stuttgart in winter
Giorgio Veratti, Alessandro Bigi, Michele Stortini, Sergio Teggi, and Grazia Ghermandi
Atmos. Chem. Phys., 24, 10475–10512, https://doi.org/10.5194/acp-24-10475-2024, https://doi.org/10.5194/acp-24-10475-2024, 2024
Short summary
Short summary
In a study of two consecutive winter seasons, we used measurements and modelling tools to identify the levels and sources of black carbon pollution in a medium-sized urban area of the Po Valley, Italy. Our findings show that biomass burning and traffic-related emissions (especially from Euro 4 diesel cars) significantly contribute to BC concentrations. This research offers crucial insights for policymakers and urban planners aiming to improve air quality in cities.
Pascal Lemaitre, Arnaud Quérel, Alexis Dépée, Alice Guerra Devigne, Marie Monier, Thibault Hiron, Chloé Soto Minguez, Daniel Hardy, and Andrea Flossmann
Atmos. Chem. Phys., 24, 9713–9732, https://doi.org/10.5194/acp-24-9713-2024, https://doi.org/10.5194/acp-24-9713-2024, 2024
Short summary
Short summary
A new in-cloud scavenging scheme is proposed. It is based on a microphysical model of cloud formation and may be applied to long-distance atmospheric transport models (> 100 km) and climatic models. This model is applied to the two most extreme precipitating cloud types in terms of both relative humidity and vertical extension: cumulonimbus and stratus.
Alex Rowell, James Brean, David C. S. Beddows, Tuukka Petäjä, Máté Vörösmarty, Imre Salma, Jarkko V. Niemi, Hanna E. Manninen, Dominik van Pinxteren, Thomas Tuch, Kay Weinhold, Zongbo Shi, and Roy M. Harrison
Atmos. Chem. Phys., 24, 9515–9531, https://doi.org/10.5194/acp-24-9515-2024, https://doi.org/10.5194/acp-24-9515-2024, 2024
Short summary
Short summary
Different sources of airborne particles in the atmospheres of four European cities were distinguished by recognising their particle size distributions using a statistical procedure, positive matrix factorisation. The various sources responded differently to the changes in emissions associated with COVID-19 lockdowns, and the reasons are investigated. While traffic emissions generally decreased, particles formed from reactions of atmospheric gases decreased in some cities but increased in others.
Amy H. Peace, Ying Chen, George Jordan, Daniel G. Partridge, Florent Malavelle, Eliza Duncan, and Jim M. Haywood
Atmos. Chem. Phys., 24, 9533–9553, https://doi.org/10.5194/acp-24-9533-2024, https://doi.org/10.5194/acp-24-9533-2024, 2024
Short summary
Short summary
Natural aerosols from volcanic eruptions can help us understand how anthropogenic aerosols modify climate. We use observations and model simulations of the 2014–2015 Holuhraun eruption plume to examine aerosol–cloud interactions in September 2014. We find a shift to clouds with smaller, more numerous cloud droplets in the first 2 weeks of the eruption. In the third week, the background meteorology and previous conditions experienced by air masses modulate the aerosol perturbation to clouds.
Hua Lu, Min Xie, Bingliang Zhuang, Danyang Ma, Bojun Liu, Yangzhihao Zhan, Tijian Wang, Shu Li, Mengmeng Li, and Kuanguang Zhu
Atmos. Chem. Phys., 24, 8963–8982, https://doi.org/10.5194/acp-24-8963-2024, https://doi.org/10.5194/acp-24-8963-2024, 2024
Short summary
Short summary
To identify cloud, aerosol, and planetary boundary layer (PBL) interactions from an air quality perspective, we summarized two pollution patterns characterized by denser liquid cloud and by obvious cloud radiation interaction (CRI). Numerical simulation experiments showed CRI could cause a 50 % reduction in aerosol radiation interaction (ARI) under a low-trough system. The results emphasized the nonnegligible role of CRI and its inhibition of ARI under wet and cloudy pollution synoptic patterns.
Emilie Fons, Ann Kristin Naumann, David Neubauer, Theresa Lang, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 8653–8675, https://doi.org/10.5194/acp-24-8653-2024, https://doi.org/10.5194/acp-24-8653-2024, 2024
Short summary
Short summary
Aerosols can modify the liquid water path (LWP) of stratocumulus and, thus, their radiative effect. We compare storm-resolving model and satellite data that disagree on the sign of LWP adjustments and diagnose this discrepancy with causal inference. We find that strong precipitation, the absence of wet scavenging, and cloud deepening under a weak inversion contribute to positive LWP adjustments to aerosols in the model, despite weak negative effects from cloud-top entrainment enhancement.
Muhammed Irfan, Thomas Kühn, Taina Yli-Juuti, Anton Laakso, Eemeli Holopainen, Douglas R. Worsnop, Annele Virtanen, and Harri Kokkola
Atmos. Chem. Phys., 24, 8489–8506, https://doi.org/10.5194/acp-24-8489-2024, https://doi.org/10.5194/acp-24-8489-2024, 2024
Short summary
Short summary
The study examines how the volatility of semi-volatile organic compounds affects secondary organic aerosol (SOA) formation and climate. Our simulations show that uncertainties in these volatilities influence aerosol mass and climate impacts. Accurate representation of these compounds in climate models is crucial for predicting global climate patterns.
Alkiviadis Kalisoras, Aristeidis K. Georgoulias, Dimitris Akritidis, Robert J. Allen, Vaishali Naik, Chaincy Kuo, Sophie Szopa, Pierre Nabat, Dirk Olivié, Twan van Noije, Philippe Le Sager, David Neubauer, Naga Oshima, Jane Mulcahy, Larry W. Horowitz, and Prodromos Zanis
Atmos. Chem. Phys., 24, 7837–7872, https://doi.org/10.5194/acp-24-7837-2024, https://doi.org/10.5194/acp-24-7837-2024, 2024
Short summary
Short summary
Effective radiative forcing (ERF) is a metric for estimating how human activities and natural agents change the energy flow into and out of the Earth’s climate system. We investigate the anthropogenic aerosol ERF, and we estimate the contribution of individual processes to the total ERF using simulations from Earth system models within the Coupled Model Intercomparison Project Phase 6 (CMIP6). Our findings highlight that aerosol–cloud interactions drive ERF variability during the last 150 years.
Qianqian Song, Paul Ginoux, María Gonçalves Ageitos, Ron L. Miller, Vincenzo Obiso, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 7421–7446, https://doi.org/10.5194/acp-24-7421-2024, https://doi.org/10.5194/acp-24-7421-2024, 2024
Short summary
Short summary
We implement and simulate the distribution of eight dust minerals in the GFDL AM4.0 model. We found that resolving the eight minerals reduces dust absorption compared to the homogeneous dust used in the standard GFDL AM4.0 model that assumes a globally uniform hematite content of 2.7 % by volume. Resolving dust mineralogy results in significant impacts on radiation, land surface temperature, surface winds, and precipitation over North Africa in summer.
Senyi Kong, Zheng Wang, and Lei Bi
Atmos. Chem. Phys., 24, 6911–6935, https://doi.org/10.5194/acp-24-6911-2024, https://doi.org/10.5194/acp-24-6911-2024, 2024
Short summary
Short summary
The retrieval of refractive indices of dust aerosols from laboratory optical measurements is commonly done assuming spherical particles. This paper aims to investigate the uncertainties in the shortwave refractive indices and corresponding optical properties by considering non-spherical and inhomogeneous models for dust samples. The study emphasizes the significance of using non-spherical models for simulating dust aerosols.
Wenxuan Hua, Sijia Lou, Xin Huang, Lian Xue, Ke Ding, Zilin Wang, and Aijun Ding
Atmos. Chem. Phys., 24, 6787–6807, https://doi.org/10.5194/acp-24-6787-2024, https://doi.org/10.5194/acp-24-6787-2024, 2024
Short summary
Short summary
In this study, we diagnose uncertainties in carbon monoxide and organic carbon emissions from four inventories for seven major wildfire-prone regions. Uncertainties in vegetation classification methods, fire detection products, and cloud obscuration effects lead to bias in these biomass burning (BB) emission inventories. By comparing simulations with measurements, we provide certain inventory recommendations. Our study has implications for reducing uncertainties in emissions in further studies.
Chandrakala Bharali, Mary Barth, Rajesh Kumar, Sachin D. Ghude, Vinayak Sinha, and Baerbel Sinha
Atmos. Chem. Phys., 24, 6635–6662, https://doi.org/10.5194/acp-24-6635-2024, https://doi.org/10.5194/acp-24-6635-2024, 2024
Short summary
Short summary
This study examines the role of atmospheric aerosols in winter fog over the Indo-Gangetic Plains of India using WRF-Chem. The increase in RH with aerosol–radiation feedback (ARF) is found to be important for fog formation as it promotes the growth of aerosols in the polluted environment. Aqueous-phase chemistry in the fog increases PM2.5 concentration, further affecting ARF. ARF and aqueous-phase chemistry affect the fog intensity and the timing of fog formation by ~1–2 h.
Wenxin Zhao, Yu Zhao, Yu Zheng, Dong Chen, Jinyuan Xin, Kaitao Li, Huizheng Che, Zhengqiang Li, Mingrui Ma, and Yun Hang
Atmos. Chem. Phys., 24, 6593–6612, https://doi.org/10.5194/acp-24-6593-2024, https://doi.org/10.5194/acp-24-6593-2024, 2024
Short summary
Short summary
We evaluate the long-term (2000–2020) variabilities of aerosol absorption optical depth, black carbon emissions, and associated health risks in China with an integrated framework that combines multiple observations and modeling techniques. We demonstrate the remarkable emission abatement resulting from the implementation of national pollution controls and show how human activities affected the emissions with a spatiotemporal heterogeneity, thus supporting differentiated policy-making by region.
Peng Xian, Jeffrey S. Reid, Melanie Ades, Angela Benedetti, Peter R. Colarco, Arlindo da Silva, Tom F. Eck, Johannes Flemming, Edward J. Hyer, Zak Kipling, Samuel Rémy, Tsuyoshi Thomas Sekiyama, Taichu Tanaka, Keiya Yumimoto, and Jianglong Zhang
Atmos. Chem. Phys., 24, 6385–6411, https://doi.org/10.5194/acp-24-6385-2024, https://doi.org/10.5194/acp-24-6385-2024, 2024
Short summary
Short summary
The study compares and evaluates monthly AOD of four reanalyses (RA) and their consensus (i.e., ensemble mean). The basic verification characteristics of these RA versus both AERONET and MODIS retrievals are presented. The study discusses the strength of each RA and identifies regions where divergence and challenges are prominent. The RA consensus usually performs very well on a global scale in terms of how well it matches the observational data, making it a good choice for various applications.
Roger Teoh, Zebediah Engberg, Ulrich Schumann, Christiane Voigt, Marc Shapiro, Susanne Rohs, and Marc E. J. Stettler
Atmos. Chem. Phys., 24, 6071–6093, https://doi.org/10.5194/acp-24-6071-2024, https://doi.org/10.5194/acp-24-6071-2024, 2024
Short summary
Short summary
The radiative forcing (RF) due to aviation contrails is comparable to that caused by CO2. We estimate that global contrail net RF in 2019 was 62.1 mW m−2. This is ~1/2 the previous best estimate for 2018. Contrail RF varies regionally due to differences in conditions required for persistent contrails. COVID-19 reduced contrail RF by 54% in 2020 relative to 2019. Globally, 2 % of all flights account for 80 % of the annual contrail energy forcing, suggesting a opportunity to mitigate contrail RF.
Haotian Zu, Biwu Chu, Yiqun Lu, Ling Liu, and Xiuhui Zhang
Atmos. Chem. Phys., 24, 5823–5835, https://doi.org/10.5194/acp-24-5823-2024, https://doi.org/10.5194/acp-24-5823-2024, 2024
Short summary
Short summary
The nucleation of iodic acid (HIO3) and iodous acid (HIO2) was proven to be critical in marine areas. However, HIO3–HIO2 nucleation cannot effectively derive the rapid nucleation in some polluted coasts. We find a significant enhancement of dimethylamine (DMA) on the HIO3–HIO2 nucleation in marine and polar regions with abundant DMA sources, which may establish reasonable connections between the HIO3–HIO2 nucleation and the rapid formation of new particles in polluted marine and polar regions.
Junghwa Lee, Patric Seifert, Tempei Hashino, Maximilian Maahn, Fabian Senf, and Oswald Knoth
Atmos. Chem. Phys., 24, 5737–5756, https://doi.org/10.5194/acp-24-5737-2024, https://doi.org/10.5194/acp-24-5737-2024, 2024
Short summary
Short summary
Spectral bin model simulations of an idealized supercooled stratiform cloud were performed with the AMPS model for variable CCN and INP concentrations. We performed radar forward simulations with PAMTRA to transfer the simulations into radar observational space. The derived radar reflectivity factors were compared to observational studies of stratiform mixed-phase clouds. These studies report a similar response of the radar reflectivity factor to aerosol perturbations as we found in our study.
Basudev Swain, Marco Vountas, Aishwarya Singh, Nidhi L. Anchan, Adrien Deroubaix, Luca Lelli, Yanick Ziegler, Sachin S. Gunthe, Hartmut Bösch, and John P. Burrows
Atmos. Chem. Phys., 24, 5671–5693, https://doi.org/10.5194/acp-24-5671-2024, https://doi.org/10.5194/acp-24-5671-2024, 2024
Short summary
Short summary
Arctic amplification (AA) accelerates the warming of the central Arctic cryosphere and affects aerosol dynamics. Limited observations hinder a comprehensive analysis. This study uses AEROSNOW aerosol optical density (AOD) data and GEOS-Chem simulations to assess AOD variability. Discrepancies highlight the need for improved observational integration into models to refine our understanding of aerosol effects on cloud microphysics, ice nucleation, and radiative forcing under evolving AA.
Vincenzo Obiso, María Gonçalves Ageitos, Carlos Pérez García-Pando, Jan P. Perlwitz, Gregory L. Schuster, Susanne E. Bauer, Claudia Di Biagio, Paola Formenti, Kostas Tsigaridis, and Ron L. Miller
Atmos. Chem. Phys., 24, 5337–5367, https://doi.org/10.5194/acp-24-5337-2024, https://doi.org/10.5194/acp-24-5337-2024, 2024
Short summary
Short summary
We calculate the dust direct radiative effect (DRE) in an Earth system model accounting for regionally varying soil mineralogy through a new observationally constrained method. Linking dust absorption at solar wavelengths to the varying amount of specific minerals (i.e., iron oxides) improves the modeled range of dust single scattering albedo compared to observations and increases the global cooling by dust. Our results may contribute to improved estimates of the dust DRE and its climate impact.
Charlotte M. Beall, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Adam Varble, Kentaroh Suzuki, and Takuro Michibata
Atmos. Chem. Phys., 24, 5287–5302, https://doi.org/10.5194/acp-24-5287-2024, https://doi.org/10.5194/acp-24-5287-2024, 2024
Short summary
Short summary
Single-layer warm liquid clouds cover nearly one-third of the Earth's surface, and uncertainties regarding the impact of aerosols on their radiative properties pose a significant challenge to climate prediction. Here, we demonstrate how satellite observations can be used to constrain Earth system model estimates of the radiative forcing from the interactions of aerosols with clouds due to warm rain processes.
Zijun Li, Angela Buchholz, and Noora Hyttinen
EGUsphere, https://doi.org/10.5194/egusphere-2024-1182, https://doi.org/10.5194/egusphere-2024-1182, 2024
Short summary
Short summary
Evaluating organosulfur (OS) hygroscopicity is important for assessing the aerosol-cloud climate interactions in the post-fossil fuel future, when SO2 emissions decrease and OS compounds become increasingly important. Here, a state-of-the-art quantum-chemistry-based method was used to predict the hygroscopic growth factors (HGFs) of a group of atmospherically relevant OS compounds and their mixtures with AS. A good agreement was observed between their model-estimated and experimental HGFs.
Xiaoli Wei, Qian Cui, Leiming Ma, Feng Zhang, Wenwen Li, and Peng Liu
Atmos. Chem. Phys., 24, 5025–5045, https://doi.org/10.5194/acp-24-5025-2024, https://doi.org/10.5194/acp-24-5025-2024, 2024
Short summary
Short summary
A new aerosol-type classification algorithm has been proposed. It includes an optical database built by Mie scattering and a complex refractive index working as a baseline to identify different aerosol types. The new algorithm shows high accuracy and efficiency. Hence, a global map of aerosol types was generated to characterize aerosol types across the five continents. It will help improve the accuracy of aerosol inversion and determine the sources of aerosol pollution.
Zhiqiang Zhang, Ying Li, Haiyan Ran, Junling An, Yu Qu, Wei Zhou, Weiqi Xu, Weiwei Hu, Hongbin Xie, Zifa Wang, Yele Sun, and Manabu Shiraiwa
Atmos. Chem. Phys., 24, 4809–4826, https://doi.org/10.5194/acp-24-4809-2024, https://doi.org/10.5194/acp-24-4809-2024, 2024
Short summary
Short summary
Secondary organic aerosols (SOAs) can exist in liquid, semi-solid, or amorphous solid states, which are rarely accounted for in current chemical transport models. We predict the phase state of SOA particles over China and find that in northwestern China SOA particles are mostly highly viscous or glassy solid. Our results indicate that the particle phase state should be considered in SOA formation in chemical transport models for more accurate prediction of SOA mass concentrations.
Alejandro Baró Pérez, Michael S. Diamond, Frida A.-M. Bender, Abhay Devasthale, Matthias Schwarz, Julien Savre, Juha Tonttila, Harri Kokkola, Hyunho Lee, David Painemal, and Annica M. L. Ekman
Atmos. Chem. Phys., 24, 4591–4610, https://doi.org/10.5194/acp-24-4591-2024, https://doi.org/10.5194/acp-24-4591-2024, 2024
Short summary
Short summary
We use a numerical model to study interactions between humid light-absorbing aerosol plumes, clouds, and radiation over the southeast Atlantic. We find that the warming produced by the aerosols reduces cloud cover, especially in highly polluted situations. Aerosol impacts on drizzle play a minor role. However, aerosol effects on cloud reflectivity and moisture-induced changes in cloud cover dominate the climatic response and lead to an overall cooling by the biomass burning plumes.
Sampa Das, Peter R. Colarco, Huisheng Bian, and Santiago Gassó
Atmos. Chem. Phys., 24, 4421–4449, https://doi.org/10.5194/acp-24-4421-2024, https://doi.org/10.5194/acp-24-4421-2024, 2024
Short summary
Short summary
The smoke aerosols emitted from vegetation burning can alter the regional energy budget via multiple pathways. We utilized detailed observations from the NASA ORACLES airborne campaign based in Namibia during September 2016 to improve the representation of smoke aerosol properties and lifetimes in our GEOS Earth system model. The improved model simulations are for the first time able to capture the observed changes in the smoke absorption during long-range plume transport.
Jia Liu, Cancan Zhu, Donghui Zhou, and Jinbao Han
EGUsphere, https://doi.org/10.5194/egusphere-2024-1000, https://doi.org/10.5194/egusphere-2024-1000, 2024
Short summary
Short summary
The hydrophilic coatings of aged black carbon (BC) particles absorb moisture during the hygroscopic growth process, but it is difficult to characterize how much water is absorbed under different relative humidities (RHs). In this study, we propose a method to obtain the water content in the coatings based on the equivalent complex refractive index retrieved from optical properties, and this method is verified from theoretical inspect. This method performs well for thickly coated BC at high RHs.
Jingmin Li, Mattia Righi, Johannes Hendricks, Christof G. Beer, Ulrike Burkhardt, and Anja Schmidt
EGUsphere, https://doi.org/10.5194/egusphere-2024-1024, https://doi.org/10.5194/egusphere-2024-1024, 2024
Short summary
Short summary
Aiming to understand underlying patterns and trends in aerosols, we characterize the spatial patterns and long-term evolution of lower tropospheric aerosols by clustering multiple aerosol properties from preindustrial times to the year 2050 under three SSP scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Falei Xu, Shuang Wang, Yan Li, and Juan Feng
EGUsphere, https://doi.org/10.5194/egusphere-2024-955, https://doi.org/10.5194/egusphere-2024-955, 2024
Short summary
Short summary
This study examines how the North Atlantic Oscillation (NAO) and El Niño-Southern Oscillation (ENSO) in the previous winter affect spring dust activities in North China. The results show that NAO and ENSO, particularly in their negative phases, greatly influence dust activities. When both NAO and ENSO are negative, their combined effect on dust activities is even greater. This research underscores the importance of these climate patterns in predicting spring dust activities in North China.
Emilio Cuevas-Agulló, David Barriopedro, Rosa Delia García, Silvia Alonso-Pérez, Juan Jesús González-Alemán, Ernest Werner, David Suárez, Juan José Bustos, Gerardo García-Castrillo, Omaira García, África Barreto, and Sara Basart
Atmos. Chem. Phys., 24, 4083–4104, https://doi.org/10.5194/acp-24-4083-2024, https://doi.org/10.5194/acp-24-4083-2024, 2024
Short summary
Short summary
During February–March (FM) 2020–2022, unusually intense dust storms from northern Africa hit the western Euro-Mediterranean (WEM). Using dust products from satellites and atmospheric reanalysis for 2003–2022, results show that cut-off lows and European blocking are key drivers of FM dust intrusions over the WEM. A higher frequency of cut-off lows associated with subtropical ridges is observed in the late 2020–2022 period.
Yahui Che, Bofu Yu, and Katherine Bracco
Atmos. Chem. Phys., 24, 4105–4128, https://doi.org/10.5194/acp-24-4105-2024, https://doi.org/10.5194/acp-24-4105-2024, 2024
Short summary
Short summary
Dust events occur more frequently during the Austral spring and summer in dust regions, including central Australia, the southwest of Western Australia, and the northern and southern regions of eastern Australia using remote sensing and reanalysis datasets. High-concentration dust is distributed around central Australia and in the downwind northern and southern Australia. Typically, around 50 % of the dust lifted settles on Australian land, with the remaining half being deposited in the ocean.
Jonathan Elsey, Nicolas Bellouin, and Claire Ryder
Atmos. Chem. Phys., 24, 4065–4081, https://doi.org/10.5194/acp-24-4065-2024, https://doi.org/10.5194/acp-24-4065-2024, 2024
Short summary
Short summary
Aerosols influence the Earth's energy balance. The uncertainty in this radiative forcing is large depending partly on uncertainty in measurements of aerosol optical properties. We have developed a freely available new framework of millions of radiative transfer simulations spanning aerosol uncertainty and assess the impact on radiative forcing uncertainty. We find that reducing these uncertainties would reduce radiative forcing uncertainty, but non-aerosol uncertainties must also be considered.
Jing Li, Nan Wu, Biwu Chu, An Ning, and Xiuhui Zhang
Atmos. Chem. Phys., 24, 3989–4000, https://doi.org/10.5194/acp-24-3989-2024, https://doi.org/10.5194/acp-24-3989-2024, 2024
Short summary
Short summary
Iodic acid (HIO3) nucleates with iodous acid (HIO2) efficiently in marine areas; however, whether methanesulfonic acid (MSA) can synergistically participate in the HIO3–HIO2-based nucleation is unclear. We provide molecular-level evidence that MSA can efficiently promote the formation of HIO3–HIO2-based clusters using a theoretical approach. The proposed MSA-enhanced iodine nucleation mechanism may help us to deeply understand marine new particle formation events with bursts of iodine particles.
Yueming Cheng, Tie Dai, Junji Cao, Daisuke Goto, Jianbing Jin, Teruyuki Nakajima, and Guangyu Shi
EGUsphere, https://doi.org/10.5194/egusphere-2024-840, https://doi.org/10.5194/egusphere-2024-840, 2024
Short summary
Short summary
In March 2021, East Asia experienced an outbreak of severe dust storms after an absence of one and a half decades. Here, we innovative used the time-lagged ground-based aerosol size information with the fixed-lag ensemble Kalman smoother to optimize the dust emission and reproduce the dust storm. This work is valuable for the quantification of health damage, aviation risks, and profound impacts on the Earth system, but also to reveal the climatic driving force and the process of desertification.
Hao Wang, Xiaohong Liu, Chenglai Wu, and Guangxing Lin
Atmos. Chem. Phys., 24, 3309–3328, https://doi.org/10.5194/acp-24-3309-2024, https://doi.org/10.5194/acp-24-3309-2024, 2024
Short summary
Short summary
We quantified different global- and regional-scale drivers of biogenic volatile organic compound (BVOC) emission trends over the past 20 years. The results show that global greening trends significantly boost BVOC emissions and deforestation reduces BVOC emissions in South America and Southeast Asia. Elevated temperature in Europe and increased soil moisture in East and South Asia enhance BVOC emissions. The results deepen our understanding of long-term BVOC emission trends in hotspots.
Christof G. Beer, Johannes Hendricks, and Mattia Righi
Atmos. Chem. Phys., 24, 3217–3240, https://doi.org/10.5194/acp-24-3217-2024, https://doi.org/10.5194/acp-24-3217-2024, 2024
Short summary
Short summary
Ice-nucleating particles (INPs) have important influences on cirrus clouds and the climate system; however, the understanding of their global impacts is still uncertain. We perform numerical simulations with a global aerosol–climate model to analyse INP-induced cirrus changes and the resulting climate impacts. We evaluate various sources of uncertainties, e.g. the ice-nucleating ability of INPs and the role of model dynamics, and provide a new estimate for the global INP–cirrus effect.
Jiawei Li, Zhiwei Han, Pingqing Fu, Xiaohong Yao, and Mingjie Liang
Atmos. Chem. Phys., 24, 3129–3161, https://doi.org/10.5194/acp-24-3129-2024, https://doi.org/10.5194/acp-24-3129-2024, 2024
Short summary
Short summary
Organic aerosols of marine origin are important for aerosol climatic effects but are poorly understood. For the first time, an online coupled regional chemistry–climate model is applied to explore the characteristics of emission, distribution, and direct and indirect radiative effects of marine organic aerosols over the western Pacific, which reveals an important role of marine organic aerosols in perturbing cloud and radiation and promotes understanding of global aerosol climatic impact.
Yawen Liu, Yun Qian, Philip J. Rasch, Kai Zhang, Lai-yung Ruby Leung, Yuhang Wang, Minghuai Wang, Hailong Wang, Xin Huang, and Xiu-Qun Yang
Atmos. Chem. Phys., 24, 3115–3128, https://doi.org/10.5194/acp-24-3115-2024, https://doi.org/10.5194/acp-24-3115-2024, 2024
Short summary
Short summary
Fire management has long been a challenge. Here we report that spring-peak fire activity over southern Mexico and Central America (SMCA) has a distinct quasi-biennial signal by measuring multiple fire metrics. This signal is initially driven by quasi-biennial variability in precipitation and is further amplified by positive feedback of fire–precipitation interaction at short timescales. This work highlights the importance of fire–climate interactions in shaping fires on an interannual scale.
Xu Feng, Loretta J. Mickley, Michelle L. Bell, Tianjia Liu, Jenny A. Fisher, and Maria Val Martin
Atmos. Chem. Phys., 24, 2985–3007, https://doi.org/10.5194/acp-24-2985-2024, https://doi.org/10.5194/acp-24-2985-2024, 2024
Short summary
Short summary
During severe wildfire seasons, smoke can have a significant impact on air quality in Australia. Our study demonstrates that characterization of the smoke plume injection fractions greatly affects estimates of surface smoke PM2.5. Using the plume behavior predicted by the machine learning method leads to the best model agreement with observed surface PM2.5 in key cities across Australia, with smoke PM2.5 accounting for 5 %–52 % of total PM2.5 on average during fire seasons from 2009 to 2020.
Shiyi Lai, Ximeng Qi, Xin Huang, Sijia Lou, Xuguang Chi, Liangduo Chen, Chong Liu, Yuliang Liu, Chao Yan, Mengmeng Li, Tengyu Liu, Wei Nie, Veli-Matti Kerminen, Tuukka Petäjä, Markku Kulmala, and Aijun Ding
Atmos. Chem. Phys., 24, 2535–2553, https://doi.org/10.5194/acp-24-2535-2024, https://doi.org/10.5194/acp-24-2535-2024, 2024
Short summary
Short summary
By combining in situ measurements and chemical transport modeling, this study investigates new particle formation (NPF) on the southeastern Tibetan Plateau. We found that the NPF was driven by the presence of biogenic gases and the transport of anthropogenic precursors. The NPF was vertically heterogeneous and shaped by the vertical mixing. This study highlights the importance of anthropogenic–biogenic interactions and meteorological dynamics in NPF in this climate-sensitive region.
Adriana Rocha-Lima, Peter R. Colarco, Anton S. Darmenov, Edward P. Nowottnick, Arlindo M. da Silva, and Luke D. Oman
Atmos. Chem. Phys., 24, 2443–2464, https://doi.org/10.5194/acp-24-2443-2024, https://doi.org/10.5194/acp-24-2443-2024, 2024
Short summary
Short summary
Observations show an increasing aerosol optical depth trend in the Middle East between 2003–2012. We evaluate the NASA Goddard Earth Observing System (GEOS) model's ability to capture these trends and examine the meteorological and surface parameters driving dust emissions. Our results highlight the importance of data assimilation for long-term trends of atmospheric aerosols and support the hypothesis that vegetation cover loss may have contributed to increasing dust emissions in the period.
Marc Mallet, Aurore Voldoire, Fabien Solmon, Pierre Nabat, Thomas Drugé, and Romain Roehrig
EGUsphere, https://doi.org/10.5194/egusphere-2024-496, https://doi.org/10.5194/egusphere-2024-496, 2024
Short summary
Short summary
This study investigates the interactions between smoke aerosols and climate in tropical Africa using a coupled ocean-atmosphere-aerosol climate model. The work shows that smoke plumes have a significant impact by increasing the low cloud fraction, decreasing the ocean and continental surface temperature and by reducing the precipitation of the coastal Western Africa. It also highlights the key role of the ocean temperature response and its feedbacks for the September to November season.
Danny M. Leung, Jasper F. Kok, Longlei Li, Natalie M. Mahowald, David M. Lawrence, Simone Tilmes, Erik Kluzek, Martina Klose, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 2287–2318, https://doi.org/10.5194/acp-24-2287-2024, https://doi.org/10.5194/acp-24-2287-2024, 2024
Short summary
Short summary
This study uses a premier Earth system model to evaluate a new desert dust emission scheme proposed in our companion paper. We show that our scheme accounts for more dust emission physics, hence matching better against observations than other existing dust emission schemes do. Our scheme's dust emissions also couple tightly with meteorology, hence likely improving the modeled dust sensitivity to climate change. We believe this work is vital for improving dust representation in climate models.
Ruth A. R. Digby, Nathan P. Gillett, Adam H. Monahan, Knut von Salzen, Antonis Gkikas, Qianqian Song, and Zhibo Zhang
Atmos. Chem. Phys., 24, 2077–2097, https://doi.org/10.5194/acp-24-2077-2024, https://doi.org/10.5194/acp-24-2077-2024, 2024
Short summary
Short summary
The COVID-19 lockdowns reduced aerosol emissions. We ask whether these reductions affected regional aerosol optical depth (AOD) and compare the observed changes to predictions from Earth system models. Only India has an observed AOD reduction outside of typical variability. Models overestimate the response in some regions, but when key biases have been addressed, the agreement is improved. Our results suggest that current models can realistically predict the effects of future emission changes.
Xinyue Shao, Minghuai Wang, Xinyi Dong, Yaman Liu, Wenxiang Shen, Stephen Arnold, Leighton Regayre, Meinrat Andreae, Mira Pöhlker, Duseong Jo, Man Yue, and Ken Carslaw
EGUsphere, https://doi.org/10.5194/egusphere-2024-401, https://doi.org/10.5194/egusphere-2024-401, 2024
Short summary
Short summary
Highly oxygenated organic molecules (HOMs) play an important role in atmospheric new particle formation (NPF). By explicitly coupling the chemical mechanism of HOMs and a comprehensive nucleation scheme in a global climate model. The updated model shows better agreement with measurements of nucleation rate, growth rate, NPF event frequency. Our results reveal that HOMs-driven NPF leads to a considerable increase in particle and cloud condensation nuclei burden globally.
Huisheng Bian, Mian Chin, Peter R. Colarco, Eric C. Apel, Donald R. Blake, Karl Froyd, Rebecca S. Hornbrook, Jose Jimenez, Pedro Campuzano Jost, Michael Lawler, Mingxu Liu, Marianne Tronstad Lund, Hitoshi Matsui, Benjamin A. Nault, Joyce E. Penner, Andrew W. Rollins, Gregory Schill, Ragnhild B. Skeie, Hailong Wang, Lu Xu, Kai Zhang, and Jialei Zhu
Atmos. Chem. Phys., 24, 1717–1741, https://doi.org/10.5194/acp-24-1717-2024, https://doi.org/10.5194/acp-24-1717-2024, 2024
Short summary
Short summary
This work studies sulfur in the remote troposphere at global and seasonal scales using aircraft measurements and multi-model simulations. The goal is to understand the sulfur cycle over remote oceans, spread of model simulations, and observation–model discrepancies. Such an understanding and comparison with real observations are crucial to narrow down the uncertainties in model sulfur simulations and improve understanding of the sulfur cycle in atmospheric air quality, climate, and ecosystems.
Gargi Sengupta, Minjie Zheng, and Nønne L. Prisle
Atmos. Chem. Phys., 24, 1467–1487, https://doi.org/10.5194/acp-24-1467-2024, https://doi.org/10.5194/acp-24-1467-2024, 2024
Short summary
Short summary
The effect of organic acid aerosol on sulfur chemistry and cloud properties was investigated in an atmospheric model. Organic acid dissociation was considered using both bulk and surface-related properties. We found that organic acid dissociation leads to increased hydrogen ion concentrations and sulfate aerosol mass in aqueous aerosols, increasing cloud formation. This could be important in large-scale climate models as many organic aerosol components are both acidic and surface-active.
Leena Kangas, Jaakko Kukkonen, Mari Kauhaniemi, Kari Riikonen, Mikhail Sofiev, Anu Kousa, Jarkko V. Niemi, and Ari Karppinen
Atmos. Chem. Phys., 24, 1489–1507, https://doi.org/10.5194/acp-24-1489-2024, https://doi.org/10.5194/acp-24-1489-2024, 2024
Short summary
Short summary
Residential wood combustion is a major source of fine particulate matter. This study has evaluated the contribution of residential wood combustion to fine particle concentrations and its year-to-year and seasonal variation in te Helsinki metropolitan area. The average concentrations attributed to wood combustion in winter were up to 10- or 15-fold compared to summer. Wood combustion caused 12 % to 14 % of annual fine particle concentrations. In winter, the contribution ranged from 16 % to 21 %.
Arto Heitto, Cheng Wu, Diego Aliaga, Luis Blacutt, Xuemeng Chen, Yvette Gramlich, Liine Heikkinen, Wei Huang, Radovan Krejci, Paolo Laj, Isabel Moreno, Karine Sellegri, Fernando Velarde, Kay Weinhold, Alfred Wiedensohler, Qiaozhi Zha, Federico Bianchi, Marcos Andrade, Kari E. J. Lehtinen, Claudia Mohr, and Taina Yli-Juuti
Atmos. Chem. Phys., 24, 1315–1328, https://doi.org/10.5194/acp-24-1315-2024, https://doi.org/10.5194/acp-24-1315-2024, 2024
Short summary
Short summary
Particle growth at the Chacaltaya station in Bolivia was simulated based on measured vapor concentrations and ambient conditions. Major contributors to the simulated growth were low-volatility organic compounds (LVOCs). Also, sulfuric acid had major role when volcanic activity was occurring in the area. This study provides insight on nanoparticle growth at this high-altitude Southern Hemispheric site and hence contributes to building knowledge of early growth of atmospheric particles.
Steven Soon-Kai Kong, Saginela Ravindra Babu, Sheng-Hsiang Wang, Stephen M. Griffith, Jackson Hian-Wui Chang, Ming-Tung Chuang, Guey-Rong Sheu, and Neng-Huei Lin
Atmos. Chem. Phys., 24, 1041–1058, https://doi.org/10.5194/acp-24-1041-2024, https://doi.org/10.5194/acp-24-1041-2024, 2024
Short summary
Short summary
In this study, we combined ground observations from 7-SEAS Dongsha Experiment, MERRA-2 reanalysis, and MODIS satellite images for evaluation and improvement of the CMAQ dust model for cases of East Asian Dust reaching the Taiwan region, including Dongsha in the western Pacific. We proposed a better CMAQ dust treatment over East Asia and for the first time revealed the impact of typhoons on dust transport.
Hengheng Zhang, Wei Huang, Xiaoli Shen, Ramakrishna Ramisetty, Junwei Song, Olga Kiseleva, Christopher Claus Holst, Basit Khan, Thomas Leisner, and Harald Saathoff
EGUsphere, https://doi.org/10.5194/egusphere-2024-90, https://doi.org/10.5194/egusphere-2024-90, 2024
Short summary
Short summary
Our study unravels how stagnant winter conditions elevate aerosol levels in Stuttgart. Cloud cover at night plays a pivotal role, impacting morning air quality. Validating a key model, our findings aid accurate air quality predictions, crucial for effective pollution mitigation in urban areas.
Cited articles
Abudu, S., Cui, C. L., King, J. P., Moreno, J., and Bawazir, A. S.: Modeling
of daily pan evaporation using partial least squares regression, Sci. China
Technol. Sc., 54, 163–174, https://doi.org/10.1007/s11431-010-4205-z, 2011.
Arora, V. K., Scinocca, J. F., Boer, G. J., Christian, J. R., Denman, K. L.,
Flato, G. M., Kharin, V. V., Lee, W. G., and Merryfield, W. J.: Carbon
emission limits required to satisfy future representative concentration
pathways of greenhouse gases, Geophys. Res. Lett., 38, L05805,
https://doi.org/10.1029/2010gl046270, 2011.
Ashpole, I. and Washington, R.: A new high-resolution central and western
Saharan summertime dust source map from automated satellite dust plume
tracking, J. Geophys. Res.-Atmos., 118, 6981–6995, https://doi.org/10.1002/jgrd.50554, 2013.
Baddock, M. C., Ginoux, P., Bullard, J. E., and Gill, T. E.: Do
MODIS-defined dust sources have a geomorphological signature?, Geophys. Res.
Lett., 43, 2606–2613, https://doi.org/10.1002/2015gl067327, 2016.
Bangert, M., Nenes, A., Vogel, B., Vogel, H., Barahona, D., Karydis, V. A., Kumar, P.,
Kottmeier, C., and Blahak, U.: Saharan dust event impacts on cloud formation and radiation
over Western Europe, Atmos. Chem. Phys., 12, 4045–4063, https://doi.org/10.5194/acp-12-4045-2012, 2012.
Bellouin, N., Rae, J., Jones, A., Johnson, C., Haywood, J., and Boucher, O.:
Aerosol forcing in the Climate Model Intercomparison Project (CMIP5)
simulations by HadGEM2-ES and the role of ammonium nitrate, J. Geophys.
Res.-Atmos., 116, D20206, https://doi.org/10.1029/2011jd016074, 2011.
Bentsen, M., Bethke, I., Debernard, J. B., Iversen, T., Kirkevåg, A., Seland, Ø., Drange, H.,
Roelandt, C., Seierstad, I. A., Hoose, C., and Kristjánsson, J. E.: The Norwegian
Earth System Model, NorESM1-M – Part 1: Description and basic evaluation of the
physical climate, Geosci. Model Dev., 6, 687–720, https://doi.org/10.5194/gmd-6-687-2013, 2013.
Boville, B. A. and Gent, P. R.: The NCAR Climate System Model, version one,
J. Climate, 11, 1115–1130,
https://doi.org/10.1175/1520-0442(1998)011<1115:TNCSMV>2.0.CO;2, 1998.
Chen, M. Y., Xie, P. P., Janowiak, J. E., and Arkin, P. A.: Global land
precipitation: A 50-yr monthly analysis based on gauge observations, J.
Hydrometeorol., 3, 249–266,
https://doi.org/10.1175/1525-7541(2002)003<0249:GLPAYM>2.0.CO;2, 2002.
Claverie, M., Matthews, J. L., Vermote, E. F., and Justice, C. O.: A 30+
Year AVHRR LAI and FAPAR Climate Data Record: Algorithm Description and
Validation, Remote Sens.-Basel, 8, 263, https://doi.org/10.3390/rs8030263, 2016.
Collins, W. J., Bellouin, N., Doutriaux-Boucher, M., Gedney, N., Halloran,
P., Hinton, T., Hughes, J., Jones, C. D., Joshi, M., Liddicoat, S., Martin,
G., O'Connor, F., Rae, J., Senior, C., Sitch, S., Totterdell, I., Wiltshire,
A., and Woodward, S.: Development and evaluation of an Earth-System model –
HadGEM2, Geosci. Model Dev., 4, 1051–1075, https://doi.org/10.5194/gmd-4-1051-2011,
2011.
Cook, B. I., Miller, R. L., and Seager, R.: Dust and sea surface temperature
forcing of the 1930s “Dust Bowl” drought, Geophys. Res. Lett., 35, L08710, https://doi.org/10.1029/2008gl033486, 2008.
Cook, B. I., Miller, R. L., and Seager, R.: Amplification of the North
American “Dust Bowl” drought through human-induced land degradation, P. Natl.
Acad. Sci. USA, 106, 4997–5001, https://doi.org/10.1073/pnas.0810200106, 2009.
Cook, B. I., Seager, R., Miller, R. L., and Mason, J. A.: Intensification of
North American Megadroughts through Surface and Dust Aerosol Forcing, J. Climate, 26, 4414–4430, https://doi.org/10.1175/Jcli-D-12-00022.1, 2013.
Croft, B., Lohmann, U., and von Salzen, K.: Black carbon ageing in the Canadian
Centre for Climate modelling and analysis atmospheric general circulation model,
Atmos. Chem. Phys., 5, 1931–1949, https://doi.org/10.5194/acp-5-1931-2005, 2005.
Donner, L. J., Wyman, B. L., Hemler, R. S., Horowitz, L. W., Ming, Y., Zhao,
M., Golaz, J. C., Ginoux, P., Lin, S. J., Schwarzkopf, M. D., Austin, J.,
Alaka, G., Cooke, W. F., Delworth, T. L., Freidenreich, S. M., Gordon, C.
T., Griffies, S. M., Held, I. M., Hurlin, W. J., Klein, S. A., Knutson, T.
R., Langenhorst, A. R., Lee, H. C., Lin, Y. L., Magi, B. I., Malyshev, S.
L., Milly, P. C. D., Naik, V., Nath, M. J., Pincus, R., Ploshay, J. J.,
Ramaswamy, V., Seman, C. J., Shevliakova, E., Sirutis, J. J., Stern, W. F.,
Stouffer, R. J., Wilson, R. J., Winton, M., Wittenberg, A. T., and Zeng, F.
R.: The Dynamical Core, Physical Parameterizations, and Basic Simulation
Characteristics of the Atmospheric Component AM3 of the GFDL Global Coupled
Model CM3, J. Climate, 24, 3484–3519, https://doi.org/10.1175/2011jcli3955.1, 2011.
Dunion, J. P. and Velden, C. S.: The impact of the Saharan air layer on
Atlantic tropical cyclone activity, B. Am. Meteorol. Soc., 85, 353–365, https://doi.org/10.1175/Bams-85-3-353,
2004.
Evan, A. T., Dunion, J., Foley, J. A., Heidinger, A. K., and Velden, C. S.:
New evidence for a relationship between Atlantic tropical cyclone activity
and African dust outbreaks, Geophys. Res. Lett., 33, L19813, https://doi.org/10.1029/2006gl026408,
2006.
Evan, A. T. and Mukhopadhyay, S.: African Dust over the Northern Tropical
Atlantic: 1955–2008, J. Appl. Meteorol. Clim., 49, 2213–2229,
https://doi.org/10.1175/2010jamc2485.1, 2010.
Evan, A. T., Flamant, C., Fiedler, S., and Doherty, O.: An analysis of
aeolian dust in climate models, Geophys. Res. Lett., 41, 5996–6001,
https://doi.org/10.1002/2014gl060545, 2014.
Evan, A. T., Flamant, C., Gaetani, M., and Guichard, F.: The past, present
and future of African dust, Nature, 531, 493–495, https://doi.org/10.1038/nature17149, 2016.
Evans, S., Ginoux, P., Malyshev, S., and Shevliakova, E.: Climate-vegetation
interaction and amplification of Australian dust variability, Geophys. Res. Lett., 43, 11823–11830, https://doi.org/10.1002/2016gl071016, 2016.
Fecan, F., Marticorena, B., and Bergametti, G.: Parametrization of the
increase of the aeolian erosion threshold wind friction velocity due to soil
moisture for arid and semi-arid areas, Ann. Geophys.-Atm. Hydr., 17, 149–157,
https://doi.org/10.1007/s005850050744, 1999.
Fiedler, S., Schepanski, K., Heinold, B., Knippertz, P., and Tegen, I.:
Climatology of nocturnal low-level jets over North Africa and implications
for modeling mineral dust emission, J. Geophys. Res.-Atmos., 118, 6100–6121,
https://doi.org/10.1002/jgrd.50394, 2013.
Fiedler, S., Knippertz, P., Woodward, S., Martin, G. M., Bellouin, N., Ross,
A. N., Heinold, B., Schepanski, K., Birch, C. E., and Tegen, I.: A
process-based evaluation of dust-emitting winds in the CMIP5 simulation of
HadGEM2-ES, Clim. Dynam., 46, 1107–1130, https://doi.org/10.1007/s00382-015-2635-9, 2016.
Fung, I. Y., Meyn, S. K., Tegen, I., Doney, S. C., John, J. G., and Bishop,
J. K. B.: Iron supply and demand in the upper ocean, Global Biogeochem. Cy.,
14, 281–295, https://doi.org/10.1029/1999gb900059, 2000.
Fuss, S., Canadell, J. G., Peters, G. P., Tavoni, M., Andrew, R. M., Ciais,
P., Jackson, R. B., Jones, C. D., Kraxner, F., Nakicenovic, N., Le Quere,
C., Raupach, M. R., Sharifi, A., Smith, P., and Yamagata, Y.: COMMENTARY:
Betting on negative emissions, Nat. Clim. Change, 4, 850–853, https://doi.org/10.1038/nclimate2392, 2014.
Gillette, D. A. and Passi, R.: Modeling Dust Emission Caused by Wind
Erosion, J. Geophys. Res.-Atmos., 93, 14233–14242, https://doi.org/10.1029/JD093iD11p14233,
1988.
Ginoux, P., Chin, M., Tegen, I., Prospero, J. M., Holben, B., Dubovik, O.,
and Lin, S. J.: Sources and distributions of dust aerosols simulated with
the GOCART model, J. Geophys. Res.-Atmos., 106, 20255–20273, https://doi.org/10.1029/2000jd000053, 2001.
Ginoux, P., Garbuzov, D., and Hsu, N. C.: Identification of anthropogenic and
natural dust sources using Moderate Resolution Imaging Spectroradiometer
(MODIS) Deep Blue level 2 data, J. Geophys. Res.-Atmos., 115, D05204,
https://doi.org/10.1029/2009jd012398, 2010.
Ginoux, P., Clarisse, L., Clerbaux, C., Coheur, P.-F., Dubovik, O., Hsu, N. C.,
and Van Damme, M.: Mixing of dust and NH3 observed globally over anthropogenic dust
sources, Atmos. Chem. Phys., 12, 7351–7363, https://doi.org/10.5194/acp-12-7351-2012, 2012a.
Ginoux, P., Prospero, J. M., Gill, T. E., Hsu, N. C., and Zhao, M.:
Global-Scale Attribution of Anthropogenic and Natural Dust Sources and Their
Emission Rates Based on MODIS Deep Blue Aerosol Products, Rev. Geophys., 50, RG3005,
https://doi.org/10.1029/2012rg000388, 2012b.
Houghton, J., Ding, Y., Griggs, D. J., Noguer, M., Linden, P. J. V. D., Dai,
X., Maskell, K., and Johnson, C. A.: Climate Change 2001: The scientific
basis. Contribution of Working Group I to the Third Assessment Report of the
Intergovernmental Panel on Climate Change, Cambridge Univ. Press, Cambridge,
UK, 2001.
Hsu, N. C., Tsay, S. C., King, M. D., and Herman, J. R.: Aerosol properties
over bright-reflecting source regions, IEEE T. Geosci. Remote, 42, 557–569,
https://doi.org/10.1109/Tgrs.2004.824067, 2004.
Hsu, N. C., Tsay, S. C., King, M. D., and Herman, J. R.: Deep blue
retrievals of Asian aerosol properties during ACE-Asia, IEEE T. Geosci. Remote, 44, 3180–3195, https://doi.org/10.1109/Tgrs.2006.879540, 2006.
Hsu, N. C., Jeong, M. J., Bettenhausen, C., Sayer, A. M., Hansell, R.,
Seftor, C. S., Huang, J., and Tsay, S. C.: Enhanced Deep Blue aerosol
retrieval algorithm: The second generation, J. Geophys. Res.-Atmos., 118,
9296–9315, https://doi.org/10.1002/jgrd.50712, 2013.
Huneeus, N., Schulz, M., Balkanski, Y., Griesfeller, J., Prospero, J., Kinne, S., Bauer, S.,
Boucher, O., Chin, M., Dentener, F., Diehl, T., Easter, R., Fillmore, D., Ghan, S.,
Ginoux, P., Grini, A., Horowitz, L., Koch, D., Krol, M. C., Landing, W., Liu, X.,
Mahowald, N., Miller, R., Morcrette, J.-J., Myhre, G., Penner, J., Perlwitz, J.,
Stier, P., Takemura, T., and Zender, C. S.: Global dust model intercomparison in
AeroCom phase I, Atmos. Chem. Phys., 11, 7781–7816, https://doi.org/10.5194/acp-11-7781-2011, 2011.
Jickells, T. D., An, Z. S., Andersen, K. K., Baker, A. R., Bergametti, G.,
Brooks, N., Cao, J. J., Boyd, P. W., Duce, R. A., Hunter, K. A., Kawahata,
H., Kubilay, N., laRoche, J., Liss, P. S., Mahowald, N., Prospero, J. M.,
Ridgwell, A. J., Tegen, I., and Torres, R.: Global iron connections between
desert dust, ocean biogeochemistry, and climate, Science, 308, 67–71, https://doi.org/10.1126/science.1105959, 2005.
Jin, Q., Wei, J., Yang, Z.-L., Pu, B., and Huang, J.: Consistent response of Indian summer monsoon
to Middle East dust in observations and simulations, Atmos. Chem. Phys., 15, 9897–9915,
https://doi.org/10.5194/acp-15-9897-2015, 2015.
Jin, Q. J., Wei, J. F., and Yang, Z. L.: Positive response of Indian summer
rainfall to Middle East dust, Geophys. Res. Lett., 41, 4068–4074,
https://doi.org/10.1002/2014gl059980, 2014.
Jin, Q. J., Yang, Z. L., and Wei, J. F.: Seasonal Responses of Indian Summer
Monsoon to Dust Aerosols in the Middle East, India, and China, J. Climate,
29, 6329–6349, https://doi.org/10.1175/Jcli-D-15-0622.1, 2016.
Kim, M. K., Lau, W. K. M., Kim, K. M., Sang, J., Kim, Y. H., and Lee, W. S.:
Amplification of ENSO effects on Indian summer monsoon by absorbing
aerosols, Clim. Dynam., 46, 2657–2671, https://doi.org/10.1007/s00382-015-2722-y, 2016.
Kok, J. F., Ridley, D. A., Zhou, Q., Miller, R. L., Zhao, C., Heald, C. L.,
Ward, D. S., Albani, S., and Haustein, K.: Smaller desert dust cooling
effect estimated from analysis of dust size and abundance, Nat. Geosci., 10,
https://doi.org/10.1038/Ngeo2912, 2017.
Laurent, B., Marticorena, B., Bergametti, G., and Mei, F.: Modeling mineral
dust emissions from Chinese and Mongolian deserts, Glob. Planet Change, 52,
121–141, https://doi.org/10.1016/j.gloplacha.2006.02.012, 2006.
Levin, Z., Ganor, E., and Gladstein, V.: The effects of desert particles
coated with sulfate on rain formation in the eastern Mediterranean, J. Appl.
Meteorol., 35, 1511–1523,
https://doi.org/10.1175/1520-0450(1996)035<1511:TEODPC>2.0.CO;2,
1996.
Mahowald, N. M. and Luo, C.: A less dusty future?, Geophys. Res. Lett., 30, 1903,
https://doi.org/10.1029/2003gl017880, 2003.
Mahowald, N. M., Kloster, S., Engelstaedter, S., Moore, J. K., Mukhopadhyay, S.,
McConnell, J. R., Albani, S., Doney, S. C., Bhattacharya, A., Curran, M. A. J., Flanner,
M. G., Hoffman, F. M., Lawrence, D. M., Lindsay, K., Mayewski, P. A., Neff, J., Rothenberg,
D., Thomas, E., Thornton, P. E., and Zender, C. S.: Observed 20th century desert dust
variability: impact on climate and biogeochemistry, Atmos. Chem. Phys., 10, 10875–10893,
https://doi.org/10.5194/acp-10-10875-2010, 2010.
Marticorena, B. and Bergametti, G.: Modeling the Atmospheric Dust Cycle 1,
Design of a Soil-Derived Dust Emission Scheme, J. Geophys. Res.-Atmos., 100,
16415–16430, https://doi.org/10.1029/95jd00690, 1995.
Marx, S. K., McGowan, H. A., and Kamber, B. S.: Long-range dust transport
from eastern Australia: A proxy for Holocene aridity and ENSO-type climate
variability, Earth Planet. Sc. Lett., 282, 167–177, https://doi.org/10.1016/j.epsl.2009.03.013,
2009.
McConnell, J. R., Aristarain, A. J., Banta, J. R., Edwards, P. R., and
Simoes, J. C.: 20th-Century doubling in dust archived in an Antarctic
Peninsula ice core parallels climate change and desertification in South
America, P. Natl. Acad. Sci. USA, 104, 5743–5748, https://doi.org/10.1073/pnas.0607657104, 2007.
Miller, R. L. and Tegen, I.: Climate response to soil dust aerosols, J.
Climate, 11, 3247–3267,
https://doi.org/10.1175/1520-0442(1998)011<3247:CRTSDA>2.0.CO;2, 1998.
Miller, R. L., Tegen, I., and Perlwitz, J.: Surface radiative forcing by soil
dust aerosols and the hydrologic cycle, J. Geophys. Res.-Atmos., 109, D04203,
https://doi.org/10.1029/2003jd004085, 2004.
Misra, A., Kanawade, V. P., and Tripathi, S. N.: Quantitative assessment of AOD from
17 CMIP5 models based on satellite-derived AOD over India, Ann. Geophys., 34, 657–671,
https://doi.org/10.5194/angeo-34-657-2016, 2016.
Moulin, C. and Chiapello, I.: Impact of human-induced desertification on
the intensification of Sahel dust emission and export over the last decades,
Geophys. Res. Lett., 33, L18808, https://doi.org/10.1029/2006gl025923, 2006.
Myhre, G., Shindell, D., Bréon, F.-M., Collins, W., Fuglestvedt, J.,
Huang, J., Koch, D., Lamarque, J.-F., Lee, D., Mendoza, B., Nakajima, T.,
Robock, A., Stephens, G., Takemura, T., and Zhang, H.: Anthropogenic and
Natural Radiative Forcing, in: Climate Change 2013: The Physical Science
Basis, Contribution of Working Group I to the Fifth Assessment Report of the
Intergovernmental Panel on Climate Change, edited by: Stocker, T. F., Qin,
D., Plattner, G.-K., Tignor, M., Allen, S. K., Boschung, J., Nauels, A.,
Xia, Y., Bex, V., and Midgley, P. M., Cambridge University Press, Cambridge,
United Kingdom and New York, NY, USA, 2013.
Nakajima, T., Higurashi, A., Kawamoto, K., and Penner, J. E.: A possible
correlation between satellite-derived cloud and aerosol microphysical
parameters, Geophys. Res. Lett., 28, 1171–1174, https://doi.org/10.1029/2000gl012186, 2001.
Neff, J. C., Reynolds, R. L., Belnap, J., and Lamothe, P.: Multi-decadal
impacts of grazing on soil physical and biogeochemical properties in
southeast Utah, Ecol. Appl., 15, 87–95, https://doi.org/10.1890/04-0268, 2005.
Neff, J. C., Ballantyne, A. P., Farmer, G. L., Mahowald, N. M., Conroy, J.
L., Landry, C. C., Overpeck, J. T., Painter, T. H., Lawrence, C. R., and
Reynolds, R. L.: Increasing eolian dust deposition in the western United
States linked to human activity, Nat. Geosci., 1, 189–195, https://doi.org/10.1038/ngeo133,
2008.
O'Brien, R. M.: A caution regarding rules of thumb for variance inflation
factors, Qual. Quant., 41, 673–690, https://doi.org/10.1007/s11135-006-9018-6, 2007.
O'Neill, N. T., Eck, T. F., Smirnov, A., Holben, B. N., and Thulasiraman, S.:
Spectral discrimination of coarse and fine mode optical depth, J. Geophys.
Res.-Atmos., 108, 4559, https://doi.org/10.1029/2002jd002975, 2003.
Prospero, J. M. and Nees, R. T.: Impact of the North African Drought and
El-Nino on Mineral Dust in the Barbados Trade Winds, Nature, 320, 735–738,
https://doi.org/10.1038/320735a0, 1986.
Prospero, J. M. and Lamb, P. J.: African droughts and dust transport to the
Caribbean: Climate change implications, Science, 302, 1024–1027, https://doi.org/10.1126/science.1089915, 2003.
Pu, B., Fu, R., Dickinson, R. E., and Fernando, D. N.: Why do summer
droughts in the Southern Great Plains occur in some La Nina years but not
others?, J. Geophys. Res.-Atmos., 121, 1120–1137, https://doi.org/10.1002/2015jd023508, 2016.
Pu, B. and Ginoux, P.: The impact of the Pacific Decadal Oscillation on springtime
dust activity in Syria, Atmos. Chem. Phys., 16, 13431–13448, https://doi.org/10.5194/acp-16-13431-2016, 2016.
Pu, B. and Ginoux, P.: Projection of American dustiness in the late 21st
century due to climate change, Sci. Rep., 7, 5553,
https://doi.org/10.1038/s41598-017-05431-9, 2017.
Reader, M. C., Fung, I., and McFarlane, N.: The mineral dust aerosol cycle
during the last glacial maximum, J. Geophys. Res.-Atmos.,
104, 22319–22320, https://doi.org/10.1029/1999jd900434, 1999.
Riahi, K., Rao, S., Krey, V., Cho, C. H., Chirkov, V., Fischer, G.,
Kindermann, G., Nakicenovic, N., and Rafaj, P.: RCP 8.5-A scenario of
comparatively high greenhouse gas emissions, Clim. Change, 109, 33–57,
https://doi.org/10.1007/s10584-011-0149-y, 2011.
Rosenfield, J. E., Considine, D. B., Meade, P. E., Bacmeister, J. T.,
Jackman, C. H., and Schoeberl, M. R.: Stratospheric effects of Mount
Pinatubo aerosol studied with a coupled two-dimensional model, J. Geophys. Res.-Atmos., 102, 3649–3670, https://doi.org/10.1029/96jd03820, 1997.
Sanap, S. D., Ayantika, D. C., Pandithurai, G., and Niranjan, K.: Assessment
of the aerosol distribution over Indian subcontinent in CMIP5 models,
Atmos. Environ., 87, 123–137, https://doi.org/10.1016/j.atmosenv.2014.01.017, 2014.
Seland, O., Iversen, T., Kirkevag, A., and Storelvmo, T.: Aerosol-climate
interactions in the CAM-Oslo atmospheric GCM and investigation of associated
basic shortcomings, Tellus A, 60, 459–491, https://doi.org/10.1111/j.1600-0870.2008.00318.x,
2008.
Shao, Y. P., Wyrwoll, K. H., Chappell, A., Huang, J. P., Lin, Z. H.,
McTainsh, G. H., Mikami, M., Tanaka, T. Y., Wang, X. L., and Yoon, S.: Dust
cycle: An emerging core theme in Earth system science, Aeolian Res., 2,
181–204, https://doi.org/10.1016/j.aeolia.2011.02.001, 2011.
Sharma, D. and Miller, R. L.: Revisiting the observed correlation between
weekly averaged Indian monsoon precipitation and Arabian Sea aerosol optical
depth, Geophys. Res. Lett., 44, 10006–10016, https://doi.org/10.1002/2017gl074373, 2017.
Shindell, D. T., Lamarque, J.-F., Schulz, M., Flanner, M., Jiao, C.,
Chin, M., Young, P. J., Lee, Y. H., Rotstayn, L., Mahowald, N., Milly, G., Faluvegi,
G., Balkanski, Y., Collins, W. J., Conley, A. J., Dalsoren, S., Easter, R., Ghan, S.,
Horowitz, L., Liu, X., Myhre, G., Nagashima, T., Naik, V., Rumbold, S. T., Skeie, R.,
Sudo, K., Szopa, S., Takemura, T., Voulgarakis, A., Yoon, J.-H., and Lo, F.: Radiative
forcing in the ACCMIP historical and future climate simulations, Atmos. Chem. Phys.,
13, 2939–2974, https://doi.org/10.5194/acp-13-2939-2013, 2013.
Solmon, F., Nair, V. S., and Mallet, M.: Increasing Arabian dust activity and the Indian summer
monsoon, Atmos. Chem. Phys., 15, 8051–8064, https://doi.org/10.5194/acp-15-8051-2015, 2015.
Strong, J. D., Vecchi, G. A., and Ginoux, P.: The Climatological Effect of
Saharan Dust on Global Tropical Cyclones in a Fully Coupled GCM, J. Geophys. Res.-Atmos.,
123, 5538–5559, https://doi.org/10.1029/2017JD027808, 2018.
Strong, J. D. O., Vecchi, G. A., and Ginoux, P.: The Response of the
Tropical Atlantic and West African Climate to Saharan Dust in a Fully
Coupled GCM, J. Climate, 28, 7071–7092, https://doi.org/10.1175/Jcli-D-14-00797.1, 2015.
Sun, D. L., Lau, K. M., and Kafatos, M.: Contrasting the 2007 and 2005
hurricane seasons: Evidence of possible impacts of Saharan dry air and dust
on tropical cyclone activity in the Atlantic basin, Geophys. Res. Lett., 35, L15405,
https://doi.org/10.1029/2008gl034529, 2008.
Takemura, T., Okamoto, H., Maruyama, Y., Numaguti, A., Higurashi, A., and
Nakajima, T.: Global three-dimensional simulation of aerosol optical
thickness distribution of various origins, J. Geophys. Res.-Atmos., 105,
17853–17873, https://doi.org/10.1029/2000jd900265, 2000.
Taylor, K. E., Stouffer, R. J., and Meehl, G. A.: An Overview of CMIP5 and the experiment
design, Bull. Am. Meteor. Soc., 93, 485–498, https://doi.org/10.1175/BAMS-D-11-00094.1, 2012.
Tegen, I., Harrison, S. P., Kohfeld, K., Prentice, I. C., Coe, M., and
Heimann, M.: Impact of vegetation and preferential source areas on global
dust aerosol: Results from a model study, J. Geophys. Res.-Atmos., 107,
https://doi.org/10.1029/2001jd000963, 2002.
Tegen, I., Werner, M., Harrison, S. P., and Kohfeld, K. E.: Relative
importance of climate and land use in determining present and future global
soil dust emission, Geophys. Res. Lett., 31, L05105, https://doi.org/10.1029/2003gl019216,
2004.
Todd, M. C., Washington, R., Raghavan, S., Lizcano, G., and Knippertz, P.:
Regional model simulations of the Bodele low-level jet of northern Chad
during the Bodele Dust Experiment (BoDEx 2005), J. Climate, 21, 995–1012,
https://doi.org/10.1175/2007jcli1766.1, 2008.
Vinoj, V., Rasch, P. J., Wang, H. L., Yoon, J. H., Ma, P. L., Landu, K., and
Singh, B.: Short-term modulation of Indian summer monsoon rainfall by West
Asian dust, Nat. Geosci., 7, 308–313, https://doi.org/10.1038/ngeo2107, 2014.
Watanabe, S., Hajima, T., Sudo, K., Nagashima, T., Takemura, T., Okajima, H.,
Nozawa, T., Kawase, H., Abe, M., Yokohata, T., Ise, T., Sato, H., Kato, E., Takata,
K., Emori, S., and Kawamiya, M.: MIROC-ESM 2010: model description and basic results
of CMIP5-20c3m experiments, Geosci. Model Dev., 4, 845–872, https://doi.org/10.5194/gmd-4-845-2011, 2011.
Winker, D. M., Hunt, W., and Hostetler, C.: Status and performance of the
CALIOP lidar, Bba Lib., 5575, 8–15, https://doi.org/10.1117/12.571955, 2004.
Winker, D. M., Hunt, W. H., and McGill, M. J.: Initial performance
assessment of CALIOP, Geophys. Res. Lett., 34, https://doi.org/10.1029/2007gl030135, 2007.
Wong, S. and Dessler, A. E.: Suppression of deep convection over the
tropical North Atlantic by the Saharan Air Layer, Geophys. Res. Lett., 32,
https://doi.org/10.1029/2004gl022295, 2005.
Wurzler, S., Reisin, T. G., and Levin, Z.: Modification of mineral dust
particles by cloud processing and subsequent effects on drop size
distributions, J. Geophys. Res.-Atmos., 105, 4501–4512,
https://doi.org/10.1029/1999jd900980, 2000.
Zender, C. S. and Kwon, E. Y.: Regional contrasts in dust emission
responses to climate, J. Geophys. Res.-Atmos., 110, D13201, https://doi.org/10.1029/2004jd005501,
2005.
Zhao, T. L., Gong, S. L., Zhang, X. Y., Blanchet, J. P., McKendry, I. G., and
Zhou, Z. J.: A simulated climatology of Asian dust aerosol and its
trans-Pacific transport, Part I: Mean climate and validation, J. Climate, 19,
88–103, https://doi.org/10.1175/Jcli3605.1, 2006.
Short summary
Biases in dust modeling may result in biases in simulating energy budget and regional climate. Output of seven Coupled Model Intercomparison Project Phase 5 (CMIP5) models is examined. Seasonal cycle and spatial pattern of dust optical depth (DOD) in very dusty regions are largely captured by multi-model mean. But observed connections between DOD and local controlling factors such as bareness are not well represented. Future projections by CMIP5 models and a regression model are also analyzed.
Biases in dust modeling may result in biases in simulating energy budget and regional climate....
Altmetrics
Final-revised paper
Preprint