Articles | Volume 18, issue 14
https://doi.org/10.5194/acp-18-10557-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-10557-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
24 Jul 2018
Research article |
| 24 Jul 2018
| 24 Jul 2018
Multi-year monitoring of atmospheric total gaseous mercury at a remote high-altitude site (Nam Co, 4730 m a.s.l.) in the inland Tibetan Plateau region
Xiufeng Yin
State Key Laboratory of Cryospheric Science, Northwest Institute of
Eco-Environment and Resources, Chinese Academy of Science, Lanzhou, 730000, China
Key Laboratory of Tibetan Environment Changes and Land Surface
Processes, Institute of Tibetan Plateau Research, Chinese Academy of Sciences, Beijing, 100101, China
University of Chinese Academy of Sciences, Beijing, 100039, China
Department of Earth and Atmospheric Sciences, Saint Louis University, St. Louis, MO 63108, USA
Shichang Kang
CORRESPONDING AUTHOR
State Key Laboratory of Cryospheric Science, Northwest Institute of
Eco-Environment and Resources, Chinese Academy of Science, Lanzhou, 730000, China
CAS Center for Excellence in Tibetan Plateau Earth Sciences, Beijing, 100101, China
Benjamin de Foy
Department of Earth and Atmospheric Sciences, Saint Louis University, St. Louis, MO 63108, USA
Yaoming Ma
Key Laboratory of Tibetan Environment Changes and Land Surface
Processes, Institute of Tibetan Plateau Research, Chinese Academy of Sciences, Beijing, 100101, China
CAS Center for Excellence in Tibetan Plateau Earth Sciences, Beijing, 100101, China
Yindong Tong
School of Environmental Science and Engineering, Tianjin University, Tianjin, 300072, China
Wei Zhang
School of Environment and Natural Resources, Renmin University of China, Beijing, 100872, China
Xuejun Wang
College of Urban and Environmental Sciences, Peking University, Beijing, 100871, China
Guoshuai Zhang
Key Laboratory of Tibetan Environment Changes and Land Surface
Processes, Institute of Tibetan Plateau Research, Chinese Academy of Sciences, Beijing, 100101, China
Qianggong Zhang
CORRESPONDING AUTHOR
Key Laboratory of Tibetan Environment Changes and Land Surface
Processes, Institute of Tibetan Plateau Research, Chinese Academy of Sciences, Beijing, 100101, China
CAS Center for Excellence in Tibetan Plateau Earth Sciences, Beijing, 100101, China
Related authors
Yuling Hu, Haipeng Yu, Shichang Kang, Junhua Yang, Mukesh Rai, Xiufeng Yin, Xintong Chen, and Pengfei Chen
Atmos. Chem. Phys., 24, 85–107, https://doi.org/10.5194/acp-24-85-2024, https://doi.org/10.5194/acp-24-85-2024, 2024
Short summary
Short summary
The Tibetan Plateau (TP) saw a record-breaking aerosol pollution event from April 20 to May 10, 2016. We studied the impact of aerosol–meteorology feedback on the transboundary transport flux of black carbon (BC) during this severe pollution event. It was found that the aerosol–meteorology feedback decreases the transboundary transport flux of BC from the central and western Himalayas towards the TP. This study is of great significance for the protection of the ecological environment of the TP.
Xiufeng Yin, Dipesh Rupakheti, Guoshuai Zhang, Jiali Luo, Shichang Kang, Benjamin de Foy, Junhua Yang, Zhenming Ji, Zhiyuan Cong, Maheswar Rupakheti, Ping Li, Yuling Hu, and Qianggong Zhang
Atmos. Chem. Phys., 23, 10137–10143, https://doi.org/10.5194/acp-23-10137-2023, https://doi.org/10.5194/acp-23-10137-2023, 2023
Short summary
Short summary
The monthly mean surface ozone concentrations peaked earlier in the south in April and May and later in the north in June and July over the Tibetan Plateau. The migration of monthly surface ozone peaks was coupled with the synchronous movement of tropopause folds and the westerly jet that created conditions conducive to stratospheric ozone intrusion. Stratospheric ozone intrusion significantly contributed to surface ozone across the Tibetan Plateau.
Xiufeng Yin, Shichang Kang, Benjamin de Foy, Zhiyuan Cong, Jiali Luo, Lang Zhang, Yaoming Ma, Guoshuai Zhang, Dipesh Rupakheti, and Qianggong Zhang
Atmos. Chem. Phys., 17, 11293–11311, https://doi.org/10.5194/acp-17-11293-2017, https://doi.org/10.5194/acp-17-11293-2017, 2017
Short summary
Short summary
We presented 5-year surface ozone measurements at Nam Co in the inland Tibetan Plateau and made a synthesis comparison of diurnal and seasonal patterns on regional and hemispheric scales. Surface ozone at Nam Co is mainly dominated by natural processes and is less influenced by stratospheric intrusions and human activities than on the rim of the Tibetan Plateau. Ozone at Nam Co is representative of background that is valuable for studying ozone-related effects on large scales.
Cunbo Han, Yaoming Ma, Weiqiang Ma, Fanglin Sun, Yunshuai Zhang, Wei Hu, Hanying Xu, Chunhui Duan, and Zhenhua Xi
EGUsphere, https://doi.org/10.5194/egusphere-2024-1963, https://doi.org/10.5194/egusphere-2024-1963, 2024
Short summary
Short summary
Wind speed spectra analysis is very important for understanding boundary layer turbulence characteristics, atmospheric numerical model development, and wind energy assessment. However, wind speed spectra studies in mountainous areas are extremely scarce. In this study, using a 15-year time series of wind speed observed by a PBL tower and eddy-covariance tower at a site on the north slope of Mt. Everest, we investigated the characteristics of wind speed and wind speed spectrum.
Yaoming Ma, Zhipeng Xie, Yingying Chen, Shaomin Liu, Tao Che, Ziwei Xu, Lunyu Shang, Xiaobo He, Xianhong Meng, Weiqiang Ma, Baiqing Xu, Huabiao Zhao, Junbo Wang, Guangjian Wu, and Xin Li
Earth Syst. Sci. Data, 16, 3017–3043, https://doi.org/10.5194/essd-16-3017-2024, https://doi.org/10.5194/essd-16-3017-2024, 2024
Short summary
Short summary
Current models and satellites struggle to accurately represent the land–atmosphere (L–A) interactions over the Tibetan Plateau. We present the most extensive compilation of in situ observations to date, comprising 17 years of data on L–A interactions across 12 sites. This quality-assured benchmark dataset provides independent validation to improve models and remote sensing for the region, and it enables new investigations of fine-scale L–A processes and their mechanistic drivers.
M. Omar Nawaz, Jeremiah Johnson, Greg Yarwood, Benjamin de Foy, Laura Judd, and Daniel L. Goldberg
Atmos. Chem. Phys., 24, 6719–6741, https://doi.org/10.5194/acp-24-6719-2024, https://doi.org/10.5194/acp-24-6719-2024, 2024
Short summary
Short summary
NO2 is a gas with implications for air pollution. A campaign conducted in Houston provided an opportunity to compare NO2 from different instruments and a model. Aircraft and satellite observations agreed well with measurements on the ground; however, the latter estimated lower values. We find that model-simulated NO2 was lower than observations, especially downtown, suggesting that NO2 sources associated with the urban core of Houston, such as vehicle emissions, may be underestimated.
Chaman Gul, Shichang Kang, Yuanjian Yang, Xinlei Ge, and Dong Guo
EGUsphere, https://doi.org/10.5194/egusphere-2024-1144, https://doi.org/10.5194/egusphere-2024-1144, 2024
Preprint archived
Short summary
Short summary
Long-term variations in upper atmospheric temperature and water vapor in the selected domains of time and space are presented. The temperature during the past two decades showed a cooling trend and water vapor showed an increasing trend and had an inverse relation with temperature in selected domains of space and time. Seasonal temperature variations are distinct, with a summer minimum and a winter maximum. Our results can be an early warning indication for future climate change.
Jianzhong Xu, Xinghua Zhang, Wenhui Zhao, Lixiang Zhai, Miao Zhong, Jinsen Shi, Junying Sun, Yanmei Liu, Conghui Xie, Yulong Tan, Kemei Li, Xinlei Ge, Qi Zhang, and Shichang Kang
Earth Syst. Sci. Data, 16, 1875–1900, https://doi.org/10.5194/essd-16-1875-2024, https://doi.org/10.5194/essd-16-1875-2024, 2024
Short summary
Short summary
A comprehensive aerosol observation project was carried out in the Tibetan Plateau (TP) and its surroundings in recent years to investigate the properties and sources of atmospheric aerosols as well as their regional differences by performing multiple intensive field observations. The release of this dataset can provide basic and systematic data for related research in the atmospheric, cryospheric, and environmental sciences in this unique region.
Ling Yuan, Xuelong Chen, Yaoming Ma, Cunbo Han, Binbin Wang, and Weiqiang Ma
Earth Syst. Sci. Data, 16, 775–801, https://doi.org/10.5194/essd-16-775-2024, https://doi.org/10.5194/essd-16-775-2024, 2024
Short summary
Short summary
Accurately monitoring and understanding the spatial–temporal variability of evapotranspiration (ET) components over the Tibetan Plateau (TP) remains difficult. Here, 37 years (1982–2018) of monthly ET component data for the TP was produced, and the data are consistent with measurements. The annual average ET for the TP was about 0.93 (± 0.037) × 103 Gt yr−1. The rate of increase of the ET was around 0.96 mm yr−1. The increase in the ET can be explained by warming and wetting of the climate.
Yuling Hu, Haipeng Yu, Shichang Kang, Junhua Yang, Mukesh Rai, Xiufeng Yin, Xintong Chen, and Pengfei Chen
Atmos. Chem. Phys., 24, 85–107, https://doi.org/10.5194/acp-24-85-2024, https://doi.org/10.5194/acp-24-85-2024, 2024
Short summary
Short summary
The Tibetan Plateau (TP) saw a record-breaking aerosol pollution event from April 20 to May 10, 2016. We studied the impact of aerosol–meteorology feedback on the transboundary transport flux of black carbon (BC) during this severe pollution event. It was found that the aerosol–meteorology feedback decreases the transboundary transport flux of BC from the central and western Himalayas towards the TP. This study is of great significance for the protection of the ecological environment of the TP.
Xiufeng Yin, Dipesh Rupakheti, Guoshuai Zhang, Jiali Luo, Shichang Kang, Benjamin de Foy, Junhua Yang, Zhenming Ji, Zhiyuan Cong, Maheswar Rupakheti, Ping Li, Yuling Hu, and Qianggong Zhang
Atmos. Chem. Phys., 23, 10137–10143, https://doi.org/10.5194/acp-23-10137-2023, https://doi.org/10.5194/acp-23-10137-2023, 2023
Short summary
Short summary
The monthly mean surface ozone concentrations peaked earlier in the south in April and May and later in the north in June and July over the Tibetan Plateau. The migration of monthly surface ozone peaks was coupled with the synchronous movement of tropopause folds and the westerly jet that created conditions conducive to stratospheric ozone intrusion. Stratospheric ozone intrusion significantly contributed to surface ozone across the Tibetan Plateau.
Peizhen Li, Lei Zhong, Yaoming Ma, Yunfei Fu, Meilin Cheng, Xian Wang, Yuting Qi, and Zixin Wang
Atmos. Chem. Phys., 23, 9265–9285, https://doi.org/10.5194/acp-23-9265-2023, https://doi.org/10.5194/acp-23-9265-2023, 2023
Short summary
Short summary
In this paper, all-sky downwelling shortwave radiation (DSR) over the entire Tibetan Plateau (TP) at a spatial resolution of 1 km was estimated using an improved parameterization scheme. The influence of topography and different radiative attenuations were comprehensively taken into account. The derived DSR showed good agreement with in situ measurements. The accuracy was better than six other DSR products. The derived DSR also provided more reasonable and detailed spatial patterns.
Huiming Lin, Yindong Tong, Long Chen, Chenghao Yu, Zhaohan Chu, Qianru Zhang, Xiufeng Yin, Qianggong Zhang, Shichang Kang, Junfeng Liu, James Schauer, Benjamin de Foy, and Xuejun Wang
Atmos. Chem. Phys., 23, 3937–3953, https://doi.org/10.5194/acp-23-3937-2023, https://doi.org/10.5194/acp-23-3937-2023, 2023
Short summary
Short summary
Lhasa is the largest city in the Tibetan Plateau, and its atmospheric mercury concentrations represent the highest level of pollution in this region. Unexpectedly high concentrations of atmospheric mercury species were found. Combined with the trajectory analysis, the high atmospheric mercury concentrations may have originated from external long-range transport. Local sources, especially special mercury-related sources, are important factors influencing the variability of atmospheric mercury.
Shaoyong Wang, Xiaobo He, Shichang Kang, Hui Fu, and Xiaofeng Hong
The Cryosphere, 16, 5023–5040, https://doi.org/10.5194/tc-16-5023-2022, https://doi.org/10.5194/tc-16-5023-2022, 2022
Short summary
Short summary
This study used the sine-wave exponential model and long-term water stable isotopic data to estimate water mean residence time (MRT) and its influencing factors in a high-altitude permafrost catchment (5300 m a.s.l.) in the central Tibetan Plateau (TP). MRT for stream and supra-permafrost water was estimated at 100 and 255 d, respectively. Climate and vegetation factors affected the MRT of stream and supra-permafrost water mainly by changing the thickness of the permafrost active layer.
Pei Zhang, Donghai Zheng, Rogier van der Velde, Jun Wen, Yaoming Ma, Yijian Zeng, Xin Wang, Zuoliang Wang, Jiali Chen, and Zhongbo Su
Earth Syst. Sci. Data, 14, 5513–5542, https://doi.org/10.5194/essd-14-5513-2022, https://doi.org/10.5194/essd-14-5513-2022, 2022
Short summary
Short summary
Soil moisture and soil temperature (SMST) are important state variables for quantifying the heat–water exchange between land and atmosphere. Yet, long-term, regional-scale in situ SMST measurements at multiple depths are scarce on the Tibetan Plateau (TP). The presented dataset would be valuable for the evaluation and improvement of long-term satellite- and model-based SMST products on the TP, enhancing the understanding of TP hydrometeorological processes and their response to climate change.
Jizu Chen, Wentao Du, Shichang Kang, Xiang Qin, Weijun Sun, Yang Li, Yushuo Liu, Lihui Luo, and Youyan Jiang
The Cryosphere Discuss., https://doi.org/10.5194/tc-2022-179, https://doi.org/10.5194/tc-2022-179, 2022
Preprint withdrawn
Short summary
Short summary
This study developed a dynamic deposition model of light absorbing particles (LAPs), which coupled with a surface energy and mass balance model. Based on the coupled model, we assessed atmospheric deposited BC effect on glacier melting, and quantified global warming and increment of emitted black carbon respective contributions to current accelerated glacier melting.
Daniel L. Goldberg, Monica Harkey, Benjamin de Foy, Laura Judd, Jeremiah Johnson, Greg Yarwood, and Tracey Holloway
Atmos. Chem. Phys., 22, 10875–10900, https://doi.org/10.5194/acp-22-10875-2022, https://doi.org/10.5194/acp-22-10875-2022, 2022
Short summary
Short summary
TROPOMI measurements offer a valuable means to validate emissions inventories and ozone formation regimes, with important limitations. Lightning NOx is important to account for in Texas and can contribute up to 24 % of the column NO2 in rural areas and 8 % in urban areas. Modeled NO2 in urban areas agrees with TROPOMI NO2 to within 20 % in most circumstances, with a small underestimate in Dallas (−13 %) and Houston (−20 %). Near Texas power plants, the satellite appears to underrepresent NO2.
Chaman Gul, Shichang Kang, Siva Praveen Puppala, Xiaokang Wu, Cenlin He, Yangyang Xu, Inka Koch, Sher Muhammad, Rajesh Kumar, and Getachew Dubache
Atmos. Chem. Phys., 22, 8725–8737, https://doi.org/10.5194/acp-22-8725-2022, https://doi.org/10.5194/acp-22-8725-2022, 2022
Short summary
Short summary
This work aims to understand concentrations, spatial variability, and potential source regions of light-absorbing impurities (black carbon aerosols, dust particles, and organic carbon) in the surface snow of central and western Himalayan glaciers and their impact on snow albedo and radiative forcing.
Xinghua Zhang, Wenhui Zhao, Lixiang Zhai, Miao Zhong, Jinsen Shi, Junying Sun, Yanmei Liu, Conghui Xie, Yulong Tan, Kemei Li, Xinlei Ge, Qi Zhang, Shichang Kang, and Jianzhong Xu
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2022-211, https://doi.org/10.5194/essd-2022-211, 2022
Manuscript not accepted for further review
Short summary
Short summary
A comprehensive aerosol observation project was carried out in the Tibetan Plateau (TP) in recent years to investigate the properties and sources of atmospheric aerosols as well as their regional differences by performing multiple short-term intensive field observations. The real-time online high-time-resolution (hourly) data of aerosol properties in the different TP region are integrated in a new dataset and can provide supporting for related studies in in the TP.
Yongqin Liu, Pengcheng Fang, Bixi Guo, Mukan Ji, Pengfei Liu, Guannan Mao, Baiqing Xu, Shichang Kang, and Junzhi Liu
Earth Syst. Sci. Data, 14, 2303–2314, https://doi.org/10.5194/essd-14-2303-2022, https://doi.org/10.5194/essd-14-2303-2022, 2022
Short summary
Short summary
Glaciers are an important pool of microorganisms, organic carbon, and nitrogen. This study constructed the first dataset of microbial abundance and total nitrogen in Tibetan Plateau (TP) glaciers and the first dataset of dissolved organic carbon in ice cores on the TP. These new data could provide valuable information for research on the glacier carbon and nitrogen cycle and help in assessing the potential impacts of glacier retreat due to global warming on downstream ecosystems.
Maoshan Li, Wei Fu, Na Chang, Ming Gong, Pei Xu, Yaoming Ma, Zeyong Hu, Yaoxian Yang, and Fanglin Sun
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-257, https://doi.org/10.5194/acp-2022-257, 2022
Revised manuscript not accepted
Short summary
Short summary
Compared with the plain area, the land-atmosphere interaction on the Tibetan Plateau (TP) is intense and complex, which affects the structure of the boundary layer. The observed height of the convective boundary layer on the TP under the influence of the southern branch of the westerly wind was higher than that during the Asian monsoon season. The height of the boundary layer was positively correlated with the sensible heat flux and negatively correlated with latent heat flux.
Mukesh Rai, Shichang Kang, Junhua Yang, Maheswar Rupakheti, Dipesh Rupakheti, Lekhendra Tripathee, Yuling Hu, and Xintong Chen
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-199, https://doi.org/10.5194/acp-2022-199, 2022
Revised manuscript not accepted
Short summary
Short summary
Our study revealed distinctive seasonality with the maximum and minimum aerosol concentrations during the winter and summer seasons respectively. However, interestingly summer high (AOD > 0.8) was observed over South Asia. The highest aerosols are laden over South Asia and East China within 1–2 km, however, aerosol overshooting found up to 10 km due to the deep convection process. Whereas, integrated aerosol transport for OC during spring was found to be 5 times higher than the annual mean.
Huiming Lin, Yindong Tong, Chenghao Yu, Long Chen, Xiufeng Yin, Qianggong Zhang, Shichang Kang, Lun Luo, James Schauer, Benjamin de Foy, and Xuejun Wang
Atmos. Chem. Phys., 22, 2651–2668, https://doi.org/10.5194/acp-22-2651-2022, https://doi.org/10.5194/acp-22-2651-2022, 2022
Short summary
Short summary
The Tibetan Plateau is known as
The Third Poleand is generally considered to be a clean area owing to its high altitude. However, it may receive be impacted by air pollutants transported from the Indian subcontinent. Pollutants generally enter the Tibetan Plateau in several ways. Among them is the Yarlung Zangbu–Brahmaputra Grand Canyon. In this study, we identified the influence of the Indian summer monsoon on the origin, transport, and behavior of mercury in this area.
Shichang Kang, Yulan Zhang, Pengfei Chen, Junming Guo, Qianggong Zhang, Zhiyuan Cong, Susan Kaspari, Lekhendra Tripathee, Tanguang Gao, Hewen Niu, Xinyue Zhong, Xintong Chen, Zhaofu Hu, Xiaofei Li, Yang Li, Bigyan Neupane, Fangping Yan, Dipesh Rupakheti, Chaman Gul, Wei Zhang, Guangming Wu, Ling Yang, Zhaoqing Wang, and Chaoliu Li
Earth Syst. Sci. Data, 14, 683–707, https://doi.org/10.5194/essd-14-683-2022, https://doi.org/10.5194/essd-14-683-2022, 2022
Short summary
Short summary
The Tibetan Plateau is important to the Earth’s climate. However, systematically observed data here are scarce. To perform more integrated and in-depth investigations of the origins and distributions of atmospheric pollutants and their impacts on cryospheric change, systematic data of black carbon and organic carbon from the atmosphere, glaciers, snow cover, precipitation, and lake sediment cores over the plateau based on the Atmospheric Pollution and Cryospheric Change program are provided.
Jinlei Chen, Shichang Kang, Wentao Du, Junming Guo, Min Xu, Yulan Zhang, Xinyue Zhong, Wei Zhang, and Jizu Chen
The Cryosphere, 15, 5473–5482, https://doi.org/10.5194/tc-15-5473-2021, https://doi.org/10.5194/tc-15-5473-2021, 2021
Short summary
Short summary
Sea ice is retreating with rapid warming in the Arctic. It will continue and approach the worst predicted pathway released by the IPCC. The irreversible tipping point might show around 2060 when the oldest ice will have completely disappeared. It has a huge impact on human production. Ordinary merchant ships will be able to pass the Northeast Passage and Northwest Passage by the midcentury, and the opening time will advance to the next 10 years for icebreakers with moderate ice strengthening.
Wendong Ge, Junfeng Liu, Kan Yi, Jiayu Xu, Yizhou Zhang, Xiurong Hu, Jianmin Ma, Xuejun Wang, Yi Wan, Jianying Hu, Zhaobin Zhang, Xilong Wang, and Shu Tao
Atmos. Chem. Phys., 21, 16093–16120, https://doi.org/10.5194/acp-21-16093-2021, https://doi.org/10.5194/acp-21-16093-2021, 2021
Short summary
Short summary
Compared with the observations, the results incorporating detailed cloud aqueous-phase chemistry greatly reduced SO2 overestimation. The biases in annual simulated SO2 concentrations (or mixing ratios) decreased by 46 %, 41 %, and 22 % in Europe, the USA, and China, respectively. Fe chemistry and HOx chemistry contributed more to SO2 oxidation than N chemistry. Higher concentrations of soluble Fe and higher pH values could further enhance the oxidation capacity.
Yunshuai Zhang, Qian Huang, Yaoming Ma, Jiali Luo, Chan Wang, Zhaoguo Li, and Yan Chou
Atmos. Chem. Phys., 21, 15949–15968, https://doi.org/10.5194/acp-21-15949-2021, https://doi.org/10.5194/acp-21-15949-2021, 2021
Short summary
Short summary
The source region of the Yellow River has an important role in issues related to water resources, ecological environment, and climate changes in China. We utilized large eddy simulation to understand whether the surface heterogeneity promotes or inhibits the boundary-layer turbulence, the great contribution of the thermal circulations induced by surface heterogeneity to the water and heat exchange between land/lake and air. Moreover, the turbulence in key locations is characterized.
Lian Liu, Yaoming Ma, Massimo Menenti, Rongmingzhu Su, Nan Yao, and Weiqiang Ma
Hydrol. Earth Syst. Sci., 25, 4967–4981, https://doi.org/10.5194/hess-25-4967-2021, https://doi.org/10.5194/hess-25-4967-2021, 2021
Short summary
Short summary
Albedo is a key factor in land surface energy balance, which is difficult to successfully reproduce by models. Here, we select eight snow events on the Tibetan Plateau to evaluate the universal improvements of our improved albedo scheme. The RMSE relative reductions for temperature, albedo, sensible heat flux and snow depth reach 27%, 32%, 13% and 21%, respectively, with remarkable increases in the correlation coefficients. This presents a strong potential of our scheme for modeling snow events.
Zhipeng Xie, Yaoming Ma, Weiqiang Ma, Zeyong Hu, and Genhou Sun
The Cryosphere Discuss., https://doi.org/10.5194/tc-2021-260, https://doi.org/10.5194/tc-2021-260, 2021
Preprint withdrawn
Short summary
Short summary
Wind-driven snow transport greatly influences spatial-temporal distribution of snow in mountainous areas. Knowledge of the spatiotemporal variability of blowing snow is in its infancy because of inaccuracies in satellite-based blowing snow algorithms and the absence of quantitative assessments. Here, we present the spatiotemporal variability and magnitude of blowing snow events, and explore the potential links with ambient meteorological conditions using near surface blowing snow observations.
Yongkang Xue, Tandong Yao, Aaron A. Boone, Ismaila Diallo, Ye Liu, Xubin Zeng, William K. M. Lau, Shiori Sugimoto, Qi Tang, Xiaoduo Pan, Peter J. van Oevelen, Daniel Klocke, Myung-Seo Koo, Tomonori Sato, Zhaohui Lin, Yuhei Takaya, Constantin Ardilouze, Stefano Materia, Subodh K. Saha, Retish Senan, Tetsu Nakamura, Hailan Wang, Jing Yang, Hongliang Zhang, Mei Zhao, Xin-Zhong Liang, J. David Neelin, Frederic Vitart, Xin Li, Ping Zhao, Chunxiang Shi, Weidong Guo, Jianping Tang, Miao Yu, Yun Qian, Samuel S. P. Shen, Yang Zhang, Kun Yang, Ruby Leung, Yuan Qiu, Daniele Peano, Xin Qi, Yanling Zhan, Michael A. Brunke, Sin Chan Chou, Michael Ek, Tianyi Fan, Hong Guan, Hai Lin, Shunlin Liang, Helin Wei, Shaocheng Xie, Haoran Xu, Weiping Li, Xueli Shi, Paulo Nobre, Yan Pan, Yi Qin, Jeff Dozier, Craig R. Ferguson, Gianpaolo Balsamo, Qing Bao, Jinming Feng, Jinkyu Hong, Songyou Hong, Huilin Huang, Duoying Ji, Zhenming Ji, Shichang Kang, Yanluan Lin, Weiguang Liu, Ryan Muncaster, Patricia de Rosnay, Hiroshi G. Takahashi, Guiling Wang, Shuyu Wang, Weicai Wang, Xu Zhou, and Yuejian Zhu
Geosci. Model Dev., 14, 4465–4494, https://doi.org/10.5194/gmd-14-4465-2021, https://doi.org/10.5194/gmd-14-4465-2021, 2021
Short summary
Short summary
The subseasonal prediction of extreme hydroclimate events such as droughts/floods has remained stubbornly low for years. This paper presents a new international initiative which, for the first time, introduces spring land surface temperature anomalies over high mountains to improve precipitation prediction through remote effects of land–atmosphere interactions. More than 40 institutions worldwide are participating in this effort. The experimental protocol and preliminary results are presented.
Cunbo Han, Yaoming Ma, Binbin Wang, Lei Zhong, Weiqiang Ma, Xuelong Chen, and Zhongbo Su
Earth Syst. Sci. Data, 13, 3513–3524, https://doi.org/10.5194/essd-13-3513-2021, https://doi.org/10.5194/essd-13-3513-2021, 2021
Short summary
Short summary
Actual terrestrial evapotranspiration (ETa) is a key parameter controlling the land–atmosphere interaction processes and water cycle. However, the spatial distribution and temporal changes in ETa over the Tibetan Plateau (TP) remain very uncertain. Here we estimate the multiyear (2001–2018) monthly ETa and its spatial distribution on the TP by a combination of meteorological data and satellite products. Results have been validated at six eddy-covariance monitoring sites and show high accuracy.
Zhipeng Xie, Weiqiang Ma, Yaoming Ma, Zeyong Hu, Genhou Sun, Yizhe Han, Wei Hu, Rongmingzhu Su, and Yixi Fan
Hydrol. Earth Syst. Sci., 25, 3783–3804, https://doi.org/10.5194/hess-25-3783-2021, https://doi.org/10.5194/hess-25-3783-2021, 2021
Short summary
Short summary
Ground information on the occurrence of blowing snow has been sorely lacking because direct observations of blowing snow are sparse in time and space. In this paper, we investigated the potential capability of the decision tree model to detect blowing snow events in the European Alps. Trained with routine meteorological observations, the decision tree model can be used as an efficient tool to detect blowing snow occurrences across different regions requiring limited meteorological variables.
Youwen Sun, Hao Yin, Yuan Cheng, Qianggong Zhang, Bo Zheng, Justus Notholt, Xiao Lu, Cheng Liu, Yuan Tian, and Jianguo Liu
Atmos. Chem. Phys., 21, 9201–9222, https://doi.org/10.5194/acp-21-9201-2021, https://doi.org/10.5194/acp-21-9201-2021, 2021
Short summary
Short summary
We quantified the variability, source, and transport of urban CO over the Himalayas and Tibetan Plateau (HTP) by using measurement, model simulation, and the analysis of meteorological fields. Urban CO over the HTP is dominated by anthropogenic and biomass burning emissions from local, South Asia and East Asia, and oxidation sources. The decreasing trends in surface CO since 2015 in most cities over the HTP are attributed to the reduction in local and transported CO emissions in recent years.
Yanbin Lei, Tandong Yao, Kun Yang, Lazhu, Yaoming Ma, and Broxton W. Bird
Hydrol. Earth Syst. Sci., 25, 3163–3177, https://doi.org/10.5194/hess-25-3163-2021, https://doi.org/10.5194/hess-25-3163-2021, 2021
Short summary
Short summary
Lake evaporation from Paiku Co on the TP is low in spring and summer and high in autumn and early winter. There is a ~ 5-month lag between net radiation and evaporation due to large lake heat storage. High evaporation and low inflow cause significant lake-level decrease in autumn and early winter, while low evaporation and high inflow cause considerable lake-level increase in summer. This study implies that evaporation can affect the different amplitudes of lake-level variations on the TP.
Kun Wang, Shohei Hattori, Mang Lin, Sakiko Ishino, Becky Alexander, Kazuki Kamezaki, Naohiro Yoshida, and Shichang Kang
Atmos. Chem. Phys., 21, 8357–8376, https://doi.org/10.5194/acp-21-8357-2021, https://doi.org/10.5194/acp-21-8357-2021, 2021
Short summary
Short summary
Sulfate aerosols play an important climatic role and exert adverse effects on the ecological environment and human health. In this study, we present the triple oxygen isotopic composition of sulfate from the Mt. Everest region, southern Tibetan Plateau, and decipher the formation mechanisms of atmospheric sulfate in this pristine environment. The results indicate the important role of the S(IV) + O3 pathway in atmospheric sulfate formation promoted by conditions of high cloud water pH.
Maoshan Li, Xiaoran Liu, Lei Shu, Shucheng Yin, Lingzhi Wang, Wei Fu, Yaoming Ma, Yaoxian Yang, and Fanglin Sun
Hydrol. Earth Syst. Sci., 25, 2915–2930, https://doi.org/10.5194/hess-25-2915-2021, https://doi.org/10.5194/hess-25-2915-2021, 2021
Short summary
Short summary
In this study, using MODIS satellite data and site atmospheric turbulence observation data in the Nagqu area of the northern Tibetan Plateau, with the Massman-retrieved model and a single height observation to determine aerodynamic surface roughness, temporal and spatial variation characteristics of the surface roughness were analyzed. The result is feasible, and it can be applied to improve the model parameters of the land surface model and the accuracy of model simulation in future work.
Ziyu Huang, Lei Zhong, Yaoming Ma, and Yunfei Fu
Geosci. Model Dev., 14, 2827–2841, https://doi.org/10.5194/gmd-14-2827-2021, https://doi.org/10.5194/gmd-14-2827-2021, 2021
Short summary
Short summary
Spectral nudging is an effective dynamical downscaling method used to improve precipitation simulations of regional climate models (RCMs). However, the biases of the driving fields over the Tibetan Plateau (TP) would possibly introduce extra biases when spectral nudging is applied. The results show that the precipitation simulations were significantly improved when limiting the application of spectral nudging toward the potential temperature and water vapor mixing ratio over the TP.
Genhou Sun, Zeyong Hu, Yaoming Ma, Zhipeng Xie, Jiemin Wang, and Song Yang
Hydrol. Earth Syst. Sci., 24, 5937–5951, https://doi.org/10.5194/hess-24-5937-2020, https://doi.org/10.5194/hess-24-5937-2020, 2020
Short summary
Short summary
We investigate the influence of soil conditions on the planetary boundary layer (PBL) thermodynamics and convective cloud formations over a typical underlying surface, based on a series of simulations on a sunny day in the Tibetan Plateau, using the Weather Research and Forecasting (WRF) model. The real-case simulation and sensitivity simulations indicate that the soil moisture could have a strong impact on PBL thermodynamics, which may be favorable for the convective cloud formations.
Yaoming Ma, Zeyong Hu, Zhipeng Xie, Weiqiang Ma, Binbin Wang, Xuelong Chen, Maoshan Li, Lei Zhong, Fanglin Sun, Lianglei Gu, Cunbo Han, Lang Zhang, Xin Liu, Zhangwei Ding, Genhou Sun, Shujin Wang, Yongjie Wang, and Zhongyan Wang
Earth Syst. Sci. Data, 12, 2937–2957, https://doi.org/10.5194/essd-12-2937-2020, https://doi.org/10.5194/essd-12-2937-2020, 2020
Short summary
Short summary
In comparison with other terrestrial regions of the world, meteorological observations are scarce over the Tibetan Plateau.
This has limited our understanding of the mechanisms underlying complex interactions between the different earth spheres with heterogeneous land surface conditions.
The release of this continuous and long-term dataset with high temporal resolution is expected to facilitate broad multidisciplinary communities in understanding key processes on the
Third Pole of the world.
Felix Nieberding, Christian Wille, Gerardo Fratini, Magnus O. Asmussen, Yuyang Wang, Yaoming Ma, and Torsten Sachs
Earth Syst. Sci. Data, 12, 2705–2724, https://doi.org/10.5194/essd-12-2705-2020, https://doi.org/10.5194/essd-12-2705-2020, 2020
Short summary
Short summary
We present the first long-term eddy covariance CO2 and H2O flux measurements from the large but underrepresented alpine steppe ecosystem on the central Tibetan Plateau. We applied careful corrections and rigorous quality filtering and analyzed the turbulent flow regime to provide meaningful fluxes. This comprehensive data set allows potential users to put the gas flux dynamics into context with ecosystem properties and potential flux drivers and allows for comparisons with other data sets.
Shuang Yi, Chunqiao Song, Kosuke Heki, Shichang Kang, Qiuyu Wang, and Le Chang
The Cryosphere, 14, 2267–2281, https://doi.org/10.5194/tc-14-2267-2020, https://doi.org/10.5194/tc-14-2267-2020, 2020
Short summary
Short summary
High-Asia glaciers have been observed to be retreating the fastest in the southeastern Tibeten Plateau, where vast amounts of glacier and snow feed the streamflow of the Brahmaputra. Here, we provide the first monthly glacier and snow mass balance during 2002–2017 based on satellite gravimetry. The results confirm previous long-term decreases but reveal strong seasonal variations. This work helps resolve previous divergent model estimates and underlines the importance of meltwater.
Meixin Zhang, Chun Zhao, Zhiyuan Cong, Qiuyan Du, Mingyue Xu, Yu Chen, Ming Chen, Rui Li, Yunfei Fu, Lei Zhong, Shichang Kang, Delong Zhao, and Yan Yang
Atmos. Chem. Phys., 20, 5923–5943, https://doi.org/10.5194/acp-20-5923-2020, https://doi.org/10.5194/acp-20-5923-2020, 2020
Short summary
Short summary
Analysis of multiple numerical experiments over the Himalayas and Tibetan Plateau (TP) shows that the complex topography results in 50 % stronger overall cross-Himalayan transport during the pre-monsoon season primarily due to the strengthened efficiency of near-surface meridional transport towards the TP, enhanced wind speed in some valleys and deeper valley channels associated with larger transported BC mass volume, which leads to 30–50 % stronger BC radiative heating over the TP.
Yanbin Lei, Tandong Yao, Kun Yang, Zhu La, Yaoming Ma, and Broxton W. Bird
Hydrol. Earth Syst. Sci. Discuss., https://doi.org/10.5194/hess-2019-421, https://doi.org/10.5194/hess-2019-421, 2019
Revised manuscript not accepted
Xinghua Zhang, Jianzhong Xu, Shichang Kang, Qi Zhang, and Junying Sun
Atmos. Chem. Phys., 19, 7897–7911, https://doi.org/10.5194/acp-19-7897-2019, https://doi.org/10.5194/acp-19-7897-2019, 2019
Short summary
Short summary
Highly time resolved chemistry and sources of PM1 were measured by an Aerodyne HR-ToF-AMS at Waliguan Baseline Observatory, a high-altitude background station at the northeastern edge of Qinghai–Tibet Plateau (QTP), during summer 2017. Relatively higher mass concentration of PM1 and dominant sulfate contribution were observed in this site compared to those at other high-elevation sites in the southern or central QTP, indicating the different aerosol sources between them.
Zongbo Shi, Tuan Vu, Simone Kotthaus, Roy M. Harrison, Sue Grimmond, Siyao Yue, Tong Zhu, James Lee, Yiqun Han, Matthias Demuzere, Rachel E. Dunmore, Lujie Ren, Di Liu, Yuanlin Wang, Oliver Wild, James Allan, W. Joe Acton, Janet Barlow, Benjamin Barratt, David Beddows, William J. Bloss, Giulia Calzolai, David Carruthers, David C. Carslaw, Queenie Chan, Lia Chatzidiakou, Yang Chen, Leigh Crilley, Hugh Coe, Tie Dai, Ruth Doherty, Fengkui Duan, Pingqing Fu, Baozhu Ge, Maofa Ge, Daobo Guan, Jacqueline F. Hamilton, Kebin He, Mathew Heal, Dwayne Heard, C. Nicholas Hewitt, Michael Hollaway, Min Hu, Dongsheng Ji, Xujiang Jiang, Rod Jones, Markus Kalberer, Frank J. Kelly, Louisa Kramer, Ben Langford, Chun Lin, Alastair C. Lewis, Jie Li, Weijun Li, Huan Liu, Junfeng Liu, Miranda Loh, Keding Lu, Franco Lucarelli, Graham Mann, Gordon McFiggans, Mark R. Miller, Graham Mills, Paul Monk, Eiko Nemitz, Fionna O'Connor, Bin Ouyang, Paul I. Palmer, Carl Percival, Olalekan Popoola, Claire Reeves, Andrew R. Rickard, Longyi Shao, Guangyu Shi, Dominick Spracklen, David Stevenson, Yele Sun, Zhiwei Sun, Shu Tao, Shengrui Tong, Qingqing Wang, Wenhua Wang, Xinming Wang, Xuejun Wang, Zifang Wang, Lianfang Wei, Lisa Whalley, Xuefang Wu, Zhijun Wu, Pinhua Xie, Fumo Yang, Qiang Zhang, Yanli Zhang, Yuanhang Zhang, and Mei Zheng
Atmos. Chem. Phys., 19, 7519–7546, https://doi.org/10.5194/acp-19-7519-2019, https://doi.org/10.5194/acp-19-7519-2019, 2019
Short summary
Short summary
APHH-Beijing is a collaborative international research programme to study the sources, processes and health effects of air pollution in Beijing. This introduction to the special issue provides an overview of (i) the APHH-Beijing programme, (ii) the measurement and modelling activities performed as part of it and (iii) the air quality and meteorological conditions during joint intensive field campaigns as a core activity within APHH-Beijing.
X. Chen, Z. Su, and Y. Ma
Int. Arch. Photogramm. Remote Sens. Spatial Inf. Sci., XLII-2-W13, 1729–1733, https://doi.org/10.5194/isprs-archives-XLII-2-W13-1729-2019, https://doi.org/10.5194/isprs-archives-XLII-2-W13-1729-2019, 2019
Lei Zhong, Yaoming Ma, Zeyong Hu, Yunfei Fu, Yuanyuan Hu, Xian Wang, Meilin Cheng, and Nan Ge
Atmos. Chem. Phys., 19, 5529–5541, https://doi.org/10.5194/acp-19-5529-2019, https://doi.org/10.5194/acp-19-5529-2019, 2019
Short summary
Short summary
Fine-temporal-resolution turbulent heat fluxes at the plateau scale have significant importance for studying diurnal variation characteristics of atmospheric boundary and weather systems in the Tibetan Plateau (TP) and its surroundings. Time series of land surface heat fluxes with high temporal resolution over the entire TP were derived. The derived surface heat fluxes proved to be in good agreement with in situ measurements and were superior to GLDAS flux products.
Xin Wan, Shichang Kang, Maheswar Rupakheti, Qianggong Zhang, Lekhendra Tripathee, Junming Guo, Pengfei Chen, Dipesh Rupakheti, Arnico K. Panday, Mark G. Lawrence, Kimitaka Kawamura, and Zhiyuan Cong
Atmos. Chem. Phys., 19, 2725–2747, https://doi.org/10.5194/acp-19-2725-2019, https://doi.org/10.5194/acp-19-2725-2019, 2019
Short summary
Short summary
The sources of primary and secondary aerosols in the Hindu Kush–Himalayan–Tibetan Plateau region are not well known. Organic molecular tracers are useful for aerosol source apportionment. The characterization of molecular tracers were first systemically investigated and the contribution from primary and secondary sources to carbonaceous aerosols was estimated in the Kathmandu Valley. Our results demonstrate that biomass burning contributed a significant fraction to OC in the Kathmandu Valley.
Daniel L. Goldberg, Pablo E. Saide, Lok N. Lamsal, Benjamin de Foy, Zifeng Lu, Jung-Hun Woo, Younha Kim, Jinseok Kim, Meng Gao, Gregory Carmichael, and David G. Streets
Atmos. Chem. Phys., 19, 1801–1818, https://doi.org/10.5194/acp-19-1801-2019, https://doi.org/10.5194/acp-19-1801-2019, 2019
Short summary
Short summary
Using satellite data, we are able to estimate the emissions of NOx (NOx=NO+NO2), a toxic group of air pollutants, in the Seoul metropolitan area. We first develop an enhanced satellite product that better observes NO2 in urban regions. Using this new product, we derive NOx emissions to be twice as large as the emissions reported by the South Korean government. The implication is that the measures taken to reduce NOx emissions in South Korea have not been as effective as regulators have thought.
Huiming Lin, Yindong Tong, Xiufeng Yin, Qianggong Zhang, Hui Zhang, Haoran Zhang, Long Chen, Shichang Kang, Wei Zhang, James Schauer, Benjamin de Foy, Xiaoge Bu, and Xuejun Wang
Atmos. Chem. Phys., 19, 1373–1391, https://doi.org/10.5194/acp-19-1373-2019, https://doi.org/10.5194/acp-19-1373-2019, 2019
Short summary
Short summary
Located in the world's
third Poleand a remote region connecting the Indian and Eurasian plates, Qomolangma National Nature Preserve is an ideal region to study the long-range transport of atmospheric pollutants. Covering both the pre-Indian summer monsoon and Indian summer monsoon periods, our measurement and modeling results have addressed the need for more specific identification of Hg sources in this area and the importance of international cooperation regarding global mercury controls.
Yanqing An, Jianzhong Xu, Lin Feng, Xinghua Zhang, Yanmei Liu, Shichang Kang, Bin Jiang, and Yuhong Liao
Atmos. Chem. Phys., 19, 1115–1128, https://doi.org/10.5194/acp-19-1115-2019, https://doi.org/10.5194/acp-19-1115-2019, 2019
Short summary
Short summary
Detailed molecular chemical composition of water-soluble organic matter in the Himalayas was characterized by positive electrospray ionization Fourier transform ion cyclotron resonance mass spectrometry for the first time. Many products formed from biogenic volatile organic compounds and biomass-burning-emitted compounds were found in the organic compounds, suggesting the important contribution of these two sources in the Himalayas.
Zhiwen Dong, Shichang Kang, Dahe Qin, Yaping Shao, Sven Ulbrich, and Xiang Qin
The Cryosphere, 12, 3877–3890, https://doi.org/10.5194/tc-12-3877-2018, https://doi.org/10.5194/tc-12-3877-2018, 2018
Short summary
Short summary
This study aimed to provide a first and unique record of physicochemical properties and mixing states of LAPs at the glacier and atmosphere interface over the northeastern Tibetan Plateau to determine the individual LAPs' structure aging and mixing state changes through the atmospheric deposition process from atmosphere to glacier–snowpack surface, thereby helping to characterize the LAPs' radiative forcing and climate effects in the cryosphere region.
Zhiyuan Cong, Shaopeng Gao, Wancang Zhao, Xin Wang, Guangming Wu, Yulan Zhang, Shichang Kang, Yongqin Liu, and Junfeng Ji
The Cryosphere, 12, 3177–3186, https://doi.org/10.5194/tc-12-3177-2018, https://doi.org/10.5194/tc-12-3177-2018, 2018
Short summary
Short summary
Cryoconites from glaciers on the Tibetan Plateau and surrounding area were studied for iron oxides. We found that goethite is the predominant iron oxide form. Using the abundance, speciation and optical properties of iron oxides, the total light absorption was quantitatively attributed to goethite, hematite, black carbon and organic matter. Such findings are essential to understand the relative significance of anthropogenic and natural impacts.
Xintong Chen, Shichang Kang, Zhiyuan Cong, Junhua Yang, and Yaoming Ma
Atmos. Chem. Phys., 18, 12859–12875, https://doi.org/10.5194/acp-18-12859-2018, https://doi.org/10.5194/acp-18-12859-2018, 2018
Short summary
Short summary
To understand the impact of transboundary atmospheric black carbon on the Mt. Everest region and depict the transport pathways in different spatiotemporal scales, we first investigated the concentration level, temporal variation, and sources of black carbon based on high-resolution (2-year) measurements at Qomolangma (Mt. Everest) Station (4276 m a.s.l.). Next, the WRF-Chem simulations were used to reveal the transport mechanisms of black carbon from southern Asia to the Mt. Everest region.
Cenlin He, Mark G. Flanner, Fei Chen, Michael Barlage, Kuo-Nan Liou, Shichang Kang, Jing Ming, and Yun Qian
Atmos. Chem. Phys., 18, 11507–11527, https://doi.org/10.5194/acp-18-11507-2018, https://doi.org/10.5194/acp-18-11507-2018, 2018
Short summary
Short summary
Snow albedo plays a key role in the Earth and climate system. It can be affected by impurities and snow properties. This study implements new parameterizations into a widely used snow model to account for effects of snow shape and black carbon–snow mixing state on snow albedo reduction in the Tibetan Plateau. This study points toward an imperative need for extensive measurements and improved model characterization of snow grain shape and aerosol–snow mixing state in Tibet and elsewhere.
Hewen Niu, Shichang Kang, Hailong Wang, Rudong Zhang, Xixi Lu, Yun Qian, Rukumesh Paudyal, Shijin Wang, Xiaofei Shi, and Xingguo Yan
Atmos. Chem. Phys., 18, 6441–6460, https://doi.org/10.5194/acp-18-6441-2018, https://doi.org/10.5194/acp-18-6441-2018, 2018
Short summary
Short summary
Deposition of light-absorbing carbonaceous aerosol on the surface of glaciers can greatly alter the energy fluxes of glaciers. Two years of continuous observations of carbonaceous aerosols in a glacierized region are analyzed. We mainly studied the light absorption properties of carbonaceous aerosol and have employed a global aerosol–climate model to estimate source attributions of atmospheric black carbon.
D. Rupakheti, S. Kang, Z. Cong, M. Rupakheti, L. Tripathee, A. K. Panday, and B. Holben
Int. Arch. Photogramm. Remote Sens. Spatial Inf. Sci., XLII-3, 1493–1497, https://doi.org/10.5194/isprs-archives-XLII-3-1493-2018, https://doi.org/10.5194/isprs-archives-XLII-3-1493-2018, 2018
Chaman Gul, Siva Praveen Puppala, Shichang Kang, Bhupesh Adhikary, Yulan Zhang, Shaukat Ali, Yang Li, and Xiaofei Li
Atmos. Chem. Phys., 18, 4981–5000, https://doi.org/10.5194/acp-18-4981-2018, https://doi.org/10.5194/acp-18-4981-2018, 2018
Short summary
Short summary
Snow and ice samples were collected from six glaciers and multiple mountain valleys from northern Pakistan. Samples were analyzed for black carbon and water-insoluble organic carbon. Relatively high concentrations of black carbon, organic carbon, and dust were reported. Snow albedo and radiative forcing were estimated for the snow samples. Possible source regions of pollutants were identified through various techniques.
Xinghua Zhang, Jianzhong Xu, Shichang Kang, Yanmei Liu, and Qi Zhang
Atmos. Chem. Phys., 18, 4617–4638, https://doi.org/10.5194/acp-18-4617-2018, https://doi.org/10.5194/acp-18-4617-2018, 2018
Short summary
Short summary
Highly time and chemically resolved submicron aerosol properties were characterized online for the first time in a high-altitude site (Qomolangma station, 4276 m a.s.l.) in the northern Himalayas by using the Aerodyne HR-ToF-AMS. Biomass burning plumes were frequently observed and the dynamic processes (emissions, transport, and chemical processing) were characterized. The source and chemical composition of organic aerosol were further elucidated using positive matrix factorization analysis.
Haipeng Wang, Jianhui Chen, Shengda Zhang, David D. Zhang, Zongli Wang, Qinghai Xu, Shengqian Chen, Shijin Wang, Shichang Kang, and Fahu Chen
Clim. Past, 14, 383–396, https://doi.org/10.5194/cp-14-383-2018, https://doi.org/10.5194/cp-14-383-2018, 2018
Short summary
Short summary
The chironomid-inferred temperature record from Gonghai Lake exhibits a stepwise decreasing trend since 4 ka. A cold event in the Era of Disunity, the Sui-Tang Warm Period, the Medieval Warm Period and the Little Ice Age can all be recognized in our record, as well as in many other temperature reconstructions in China. Local wars in Shanxi Province, documented in the historical literature during the past 2700 years, are statistically significantly correlated with changes in temperature.
Yulan Zhang, Shichang Kang, Michael Sprenger, Zhiyuan Cong, Tanguang Gao, Chaoliu Li, Shu Tao, Xiaofei Li, Xinyue Zhong, Min Xu, Wenjun Meng, Bigyan Neupane, Xiang Qin, and Mika Sillanpää
The Cryosphere, 12, 413–431, https://doi.org/10.5194/tc-12-413-2018, https://doi.org/10.5194/tc-12-413-2018, 2018
Short summary
Short summary
Light-absorbing impurities deposited on snow can reduce surface albedo and contribute to the near-worldwide melting of snowpack and ice. This study focused on the black carbon and mineral dust in snow cover on the Tibetan Plateau. We discussed their concentrations, distributions, possible sources, and albedo reduction and radiative forcing. Findings indicated that the impacts of black carbon and mineral dust need to be properly accounted for in future regional climate projections.
Xinyue Zhong, Tingjun Zhang, Shichang Kang, Kang Wang, Lei Zheng, Yuantao Hu, and Huijuan Wang
The Cryosphere, 12, 227–245, https://doi.org/10.5194/tc-12-227-2018, https://doi.org/10.5194/tc-12-227-2018, 2018
Jianzhong Xu, Qi Zhang, Jinsen Shi, Xinlei Ge, Conghui Xie, Junfeng Wang, Shichang Kang, Ruixiong Zhang, and Yuhang Wang
Atmos. Chem. Phys., 18, 427–443, https://doi.org/10.5194/acp-18-427-2018, https://doi.org/10.5194/acp-18-427-2018, 2018
Short summary
Short summary
This manuscript presents results from a comprehensive field study using an HR-AMS coupled with a suite of other instruments in central Tibetan Plateau. The study discusses the chemical composition, sources, and processes of submicron aerosol during the transition from pre-monsoon to monsoon. Organic aerosol was overall highly oxidized during the entire study with higher O / C ratios during the pre-monsoon period. Sensitivity of air pollution transport with synoptic process was also evaluated.
Lin Feng, Yanqing An, Jianzhong Xu, Shichang Kang, Xiaofei Li, Yongqiang Zhou, Yunlin Zhang, Bin Jiang, and Yuhong Liao
Biogeosciences Discuss., https://doi.org/10.5194/bg-2017-507, https://doi.org/10.5194/bg-2017-507, 2017
Revised manuscript not accepted
Chaoliu Li, Fangping Yan, Shichang Kang, Pengfei Chen, Xiaowen Han, Zhaofu Hu, Guoshuai Zhang, Ye Hong, Shaopeng Gao, Bin Qu, Zhejing Zhu, Jiwei Li, Bing Chen, and Mika Sillanpää
Atmos. Chem. Phys., 17, 11899–11912, https://doi.org/10.5194/acp-17-11899-2017, https://doi.org/10.5194/acp-17-11899-2017, 2017
Short summary
Short summary
In this study, we found, due to contribution of carbonates, previously reported BC concentration in atmosphere of the Himalayas and Tibetan Plateau (HTP) were overestimated by around 39–52 %. Meanwhile, we found BC deposition of lake cores overestimated the atmospheric deposition of BC in the HTP; BC depositions of glacier region reflected actual values of 17.9 ± 5.3 mg m−2 a−1. The above results are critical for studying atmospheric distribution and chemical transport of BC in and around the HTP.
Xiufeng Yin, Shichang Kang, Benjamin de Foy, Zhiyuan Cong, Jiali Luo, Lang Zhang, Yaoming Ma, Guoshuai Zhang, Dipesh Rupakheti, and Qianggong Zhang
Atmos. Chem. Phys., 17, 11293–11311, https://doi.org/10.5194/acp-17-11293-2017, https://doi.org/10.5194/acp-17-11293-2017, 2017
Short summary
Short summary
We presented 5-year surface ozone measurements at Nam Co in the inland Tibetan Plateau and made a synthesis comparison of diurnal and seasonal patterns on regional and hemispheric scales. Surface ozone at Nam Co is mainly dominated by natural processes and is less influenced by stratospheric intrusions and human activities than on the rim of the Tibetan Plateau. Ozone at Nam Co is representative of background that is valuable for studying ozone-related effects on large scales.
Dipesh Rupakheti, Bhupesh Adhikary, Puppala Siva Praveen, Maheswar Rupakheti, Shichang Kang, Khadak Singh Mahata, Manish Naja, Qianggong Zhang, Arnico Kumar Panday, and Mark G. Lawrence
Atmos. Chem. Phys., 17, 11041–11063, https://doi.org/10.5194/acp-17-11041-2017, https://doi.org/10.5194/acp-17-11041-2017, 2017
Short summary
Short summary
For the first time, atmospheric composition was monitored during pre-monsoon season of 2013 at Lumbini (UNESCO world heritage site as birthplace of the Buddha). PM and O3 frequently exceeded WHO guidelines. Pollution concentration, diurnal characteristics and influence of open burning on air quality in Lumbini were investigated. Potential source regions were also identified. Results show that air pollution at this site is of a great concern, requiring prompt attention for mitigation.
Xin Wan, Shichang Kang, Quanlian Li, Dipesh Rupakheti, Qianggong Zhang, Junming Guo, Pengfei Chen, Lekhendra Tripathee, Maheswar Rupakheti, Arnico K. Panday, Wu Wang, Kimitaka Kawamura, Shaopeng Gao, Guangming Wu, and Zhiyuan Cong
Atmos. Chem. Phys., 17, 8867–8885, https://doi.org/10.5194/acp-17-8867-2017, https://doi.org/10.5194/acp-17-8867-2017, 2017
Short summary
Short summary
Biomass burning (BB) tracers in the aerosols in Lumbini, northern IGP, were studied for the first time. The levoglucosan was the predominant tracer and BB significantly contributed to the air quality in Lumbini. Mixed crop residues and hardwood were main burning materials. BB emissions constituted large fraction of OC, especially during the post-monsoon season. The sources of BB aerosols in Lumbini varies seasonally due to the influence of local emissions and long-range transport.
Bin Liu, Zhiyuan Cong, Yuesi Wang, Jinyuan Xin, Xin Wan, Yuepeng Pan, Zirui Liu, Yonghong Wang, Guoshuai Zhang, Zhongyan Wang, Yongjie Wang, and Shichang Kang
Atmos. Chem. Phys., 17, 449–463, https://doi.org/10.5194/acp-17-449-2017, https://doi.org/10.5194/acp-17-449-2017, 2017
Short summary
Short summary
The first observation net of background atmospheric aerosols of the Himalayas and Tibetan Plateau were conducted in 2011–2013, and the aerosol mass loadings were especially illustrated in this paper. Consequently, these terrestrial aerosol masses were strongly ecosystem-dependent, with various seasonality and diurnal cycles at these sites. These findings implicate that regional characteristics and fine-particle emissions need to be treated sensitively when assessing their climatic effects.
Jianzhong Xu, Jinsen Shi, Qi Zhang, Xinlei Ge, Francesco Canonaco, André S. H. Prévôt, Matthias Vonwiller, Sönke Szidat, Jinming Ge, Jianmin Ma, Yanqing An, Shichang Kang, and Dahe Qin
Atmos. Chem. Phys., 16, 14937–14957, https://doi.org/10.5194/acp-16-14937-2016, https://doi.org/10.5194/acp-16-14937-2016, 2016
Short summary
Short summary
This study deployed an AMS field study in Lanzhou, a city in northwestern China, evaluating the chemical composition, sources, and processes of urban aerosols during wintertime. In comparison with the results during summer in Lanzhou, the air pollution during winter was more severe and the sources were more complex. In addition, this paper estimates the contributions of fossil and non-fossil sources of organic carbon to primary and secondary organic carbon using the carbon isotopic method.
Fangping Yan, Shichang Kang, Chaoliu Li, Yulan Zhang, Xiang Qin, Yang Li, Xiaopeng Zhang, Zhaofu Hu, Pengfei Chen, Xiaofei Li, Bin Qu, and Mika Sillanpää
The Cryosphere, 10, 2611–2621, https://doi.org/10.5194/tc-10-2611-2016, https://doi.org/10.5194/tc-10-2611-2016, 2016
Short summary
Short summary
DOC release of Laohugou Glacier No. 12 was 192 kg km−2 yr−1, of which 43.2 % could be decomposed and return to atmosphere as CO2 within 28 days, producing positive feedback in the warming process and influencing downstream ecosystems. Radiative forcing of snow pit DOC was calculated to be 0.43 W m−2, accounting for about 10 % of the radiative forcing caused by BC. Therefore, DOC is also a light-absorbing agent in glacierized regions, influencing the albedo of glacier surface and glacier melting.
Jian Peng, Alexander Loew, Xuelong Chen, Yaoming Ma, and Zhongbo Su
Hydrol. Earth Syst. Sci., 20, 3167–3182, https://doi.org/10.5194/hess-20-3167-2016, https://doi.org/10.5194/hess-20-3167-2016, 2016
Short summary
Short summary
The Tibetan Plateau plays a major role in regional and global climate. The knowledge of latent heat flux can help to better describe the complex interactions between land and atmosphere. The purpose of this paper is to provide a detailed cross-comparison of existing latent heat flux products over the TP. The results highlight the recently developed latent heat product – High Resolution Land Surface Parameters from Space (HOLAPS).
Shengyun Chen, Wenjie Liu, Qian Zhao, Lin Zhao, Qingbai Wu, Xingjie Lu, Shichang Kang, Xiang Qin, Shilong Chen, Jiawen Ren, and Dahe Qin
The Cryosphere Discuss., https://doi.org/10.5194/tc-2016-80, https://doi.org/10.5194/tc-2016-80, 2016
Revised manuscript not accepted
Short summary
Short summary
Experimental warming was manipulated using open top chambers in alpine grassland ecosystem in the permafrost regions of the Qinghai-Tibet Plateau. The results revealed variations of earlier thawing, later freezing and longer freezing-thawing periods in shallow soil. Further, the estimated permafrost table declined under the warming scenarios. The work will be helpful to evaluate the stability of Qinghai-Tibet Railway/Highway and estimate the release of carbon under the future climate warming.
Yang Li, Jizu Chen, Shichang Kang, Chaoliu Li, Bin Qu, Lekhendra Tripathee, Fangping Yan, Yulan Zhang, Junmin Guo, Chaman Gul, and Xiang Qin
The Cryosphere Discuss., https://doi.org/10.5194/tc-2016-32, https://doi.org/10.5194/tc-2016-32, 2016
Preprint withdrawn
Short summary
Short summary
To our knowledge, this study constitutes the first quantitative dataset of the impacts of light absorbing particles (LAPs) on glacier ablation estimated directly from the northeastern edge of the Tibetan Plateau (TP).The average concentrations of black carbon (BC) and mineral dust (MD) in surface snow and ice at Laohugou Glacier No. 12 (LHG) were much higher than those detected in snow pits and ice cores in TP and Tien Shan mountains.
Peng Fei Chen, Chao Liu Li, Shi Chang Kang, Maheswar Rupakheti, Arnico K. Panday, Fang Ping Yan, Quan Lian Li, Qiang Gong Zhang, Jun Ming Guo, Dipesh Rupakheti, and Wei Luo
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-71, https://doi.org/10.5194/acp-2016-71, 2016
Revised manuscript not accepted
Short summary
Short summary
PAHs were measured at six sites along two south-north transects across the central Himalayas. The annual average PAHs and their dry deposition fluxes decreased noticeably from the south to north sides, however, a similar compostion pattern was found at three remote sites, suggesting the northern slope of the Himalayas may be affected by anthropogenic emissions form Indo-Gangetic Plain. PAHs showed a clear seasonal variation at Nepal and they were mainly form biomass and fossil combustion .
C. Xu, Y. M. Ma, C. You, and Z. K. Zhu
Atmos. Chem. Phys., 15, 12065–12078, https://doi.org/10.5194/acp-15-12065-2015, https://doi.org/10.5194/acp-15-12065-2015, 2015
Short summary
Short summary
Different monthly variation patterns of aerosol optical depth are observed over the southern and northern Tibetan Plateau (TP). A dividing line of higher dust occurrence in the northern TP and lower dust occurrence in the southern TP can be observed clearly at an altitude of 6-8km. The different seasonal variation patterns between the northern and southern TP are due to many factors, including the emission sources, high-altitude terrain and atmospheric circulation.
T. Gerken, W. Babel, M. Herzog, K. Fuchs, F. Sun, Y. Ma, T. Foken, and H.-F. Graf
Hydrol. Earth Syst. Sci., 19, 4023–4040, https://doi.org/10.5194/hess-19-4023-2015, https://doi.org/10.5194/hess-19-4023-2015, 2015
Short summary
Short summary
Surface moisture is an important control for the development of clouds and precipitation on the Tibetan Plateau. While dry surface conditions do not provided enough water for the development of precipitation and convection, wet surface conditions lead to increased cloud cover and a decrease in solar irradiation, which also reduces convection development. It was found that intermediate soil moistures are associated with the strongest convection.
Z. Lu, D. G. Streets, B. de Foy, L. N. Lamsal, B. N. Duncan, and J. Xing
Atmos. Chem. Phys., 15, 10367–10383, https://doi.org/10.5194/acp-15-10367-2015, https://doi.org/10.5194/acp-15-10367-2015, 2015
Short summary
Short summary
Using an exponentially modified Gaussian method and taking into account the effect of wind on NO2 distributions, we estimate 3-year moving-average emissions of summertime NOx from 35 US urban areas directly from NO2 retrievals of the OMI during 2005−2014. Total OMI-derived NOx emissions over US urban areas decreased by 49%, consistent with reductions of 43, 49, and 44% in the bottom-up NOx emissions, the weak-wind OMI NO2 burdens, and the averaged NO2 concentrations, respectively.
W. Yu, L. Tian, Y. Ma, B. Xu, and D. Qu
Atmos. Chem. Phys., 15, 10251–10262, https://doi.org/10.5194/acp-15-10251-2015, https://doi.org/10.5194/acp-15-10251-2015, 2015
S. Song, N. E. Selin, A. L. Soerensen, H. Angot, R. Artz, S. Brooks, E.-G. Brunke, G. Conley, A. Dommergue, R. Ebinghaus, T. M. Holsen, D. A. Jaffe, S. Kang, P. Kelley, W. T. Luke, O. Magand, K. Marumoto, K. A. Pfaffhuber, X. Ren, G.-R. Sheu, F. Slemr, T. Warneke, A. Weigelt, P. Weiss-Penzias, D. C. Wip, and Q. Zhang
Atmos. Chem. Phys., 15, 7103–7125, https://doi.org/10.5194/acp-15-7103-2015, https://doi.org/10.5194/acp-15-7103-2015, 2015
Short summary
Short summary
A better knowledge of mercury (Hg) emission fluxes into the global atmosphere is important for assessing its human health impacts and evaluating the effectiveness of corresponding policy actions. We for the first time apply a top-down approach at a global scale to quantitatively estimate present-day mercury emission sources as well as key parameters in a chemical transport model, in order to better constrain the global biogeochemical cycle of mercury.
F. Salerno, N. Guyennon, S. Thakuri, G. Viviano, E. Romano, E. Vuillermoz, P. Cristofanelli, P. Stocchi, G. Agrillo, Y. Ma, and G. Tartari
The Cryosphere, 9, 1229–1247, https://doi.org/10.5194/tc-9-1229-2015, https://doi.org/10.5194/tc-9-1229-2015, 2015
Short summary
Short summary
Climate-trends data in Himalaya are completely absent at high elevation. We explore the south slopes of Mt Everest though time series reconstructed from 7 stations (2660-5600m) during 1994-2013. The main increase in temp is concentrated outside of the monsoon, minimum temp increased far more than maximum, while we note a precipitation weakening. We contribute to change the perspective on which climatic drivers (temperature vs. precipitation) led mainly the glacier responses in the last 20 yr.
S. Kang, F. Wang, U. Morgenstern, Y. Zhang, B. Grigholm, S. Kaspari, M. Schwikowski, J. Ren, T. Yao, D. Qin, and P. A. Mayewski
The Cryosphere, 9, 1213–1222, https://doi.org/10.5194/tc-9-1213-2015, https://doi.org/10.5194/tc-9-1213-2015, 2015
Short summary
B. de Foy, Y. Y. Cui, J. J. Schauer, M. Janssen, J. R. Turner, and C. Wiedinmyer
Atmos. Chem. Phys., 15, 2405–2427, https://doi.org/10.5194/acp-15-2405-2015, https://doi.org/10.5194/acp-15-2405-2015, 2015
Short summary
Short summary
Elemental carbon and organic carbon are components of fine particulate matter that are harmful to health. We use computer simulations of wind patterns and pollution dispersion to analyze a year-long time series of hourly measurements made at the St. Louis-Midwest supersite. The inverse method produced improved estimates of emissions of these pollutants by different types of sources such as on-road and off-road emissions and open burning.
X. Chen, Z. Su, Y. Ma, S. Liu, Q. Yu, and Z. Xu
Atmos. Chem. Phys., 14, 13097–13117, https://doi.org/10.5194/acp-14-13097-2014, https://doi.org/10.5194/acp-14-13097-2014, 2014
W. Babel, T. Biermann, H. Coners, E. Falge, E. Seeber, J. Ingrisch, P.-M. Schleuß, T. Gerken, J. Leonbacher, T. Leipold, S. Willinghöfer, K. Schützenmeister, O. Shibistova, L. Becker, S. Hafner, S. Spielvogel, X. Li, X. Xu, Y. Sun, L. Zhang, Y. Yang, Y. Ma, K. Wesche, H.-F. Graf, C. Leuschner, G. Guggenberger, Y. Kuzyakov, G. Miehe, and T. Foken
Biogeosciences, 11, 6633–6656, https://doi.org/10.5194/bg-11-6633-2014, https://doi.org/10.5194/bg-11-6633-2014, 2014
Y. Y. Cui, A. Hodzic, J. N. Smith, J. Ortega, J. Brioude, H. Matsui, E. J. T. Levin, A. Turnipseed, P. Winkler, and B. de Foy
Atmos. Chem. Phys., 14, 11011–11029, https://doi.org/10.5194/acp-14-11011-2014, https://doi.org/10.5194/acp-14-11011-2014, 2014
L. Chen, H. H. Wang, J. F. Liu, Y. D. Tong, L. B. Ou, W. Zhang, D. Hu, C. Chen, and X. J. Wang
Atmos. Chem. Phys., 14, 10163–10176, https://doi.org/10.5194/acp-14-10163-2014, https://doi.org/10.5194/acp-14-10163-2014, 2014
R. van der Velde, M. S. Salama, T. Pellarin, M. Ofwono, Y. Ma, and Z. Su
Hydrol. Earth Syst. Sci., 18, 1323–1337, https://doi.org/10.5194/hess-18-1323-2014, https://doi.org/10.5194/hess-18-1323-2014, 2014
C. Xu, Y. M. Ma, A. Panday, Z. Y. Cong, K. Yang, Z. K. Zhu, J. M. Wang, P. M. Amatya, and L. Zhao
Atmos. Chem. Phys., 14, 3133–3149, https://doi.org/10.5194/acp-14-3133-2014, https://doi.org/10.5194/acp-14-3133-2014, 2014
Y. Ma, Z. Zhu, L. Zhong, B. Wang, C. Han, Z. Wang, Y. Wang, L. Lu, P. M. Amatya, W. Ma, and Z. Hu
Atmos. Chem. Phys., 14, 1507–1515, https://doi.org/10.5194/acp-14-1507-2014, https://doi.org/10.5194/acp-14-1507-2014, 2014
Related subject area
Subject: Gases | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Measurement report: Urban ammonia and amines in Houston, Texas
Biomass-burning sources control ambient particulate matter, but traffic and industrial sources control volatile organic compound (VOC) emissions and secondary-pollutant formation during extreme pollution events in Delhi
Multi-year observations of variable incomplete combustion in the New York megacity
Observations of the vertical distributions of summertime atmospheric pollutants in Nam Co: OH production and source analysis
Measurement report: Elevated atmospheric ammonia may promote particle pH and HONO formation – insights from the COVID-19 pandemic
Measurement report: Vertical and temporal variability in the near-surface ozone production rate and sensitivity in an urban area in the Pearl River Delta region, China
Elevated oxidized mercury in the free troposphere: analytical advances and application at a remote continental mountaintop site
Using observed urban NOx sinks to constrain VOC reactivity and the ozone and radical budget in the Seoul Metropolitan Area
Real-world emission characteristics of VOCs from typical cargo ships and their potential contributions to secondary organic aerosol and O3 under low-sulfur fuel policies
NO3 reactivity during a summer period in a temperate forest below and above the canopy
The role of oceanic ventilation and terrestrial outflow in atmospheric non-methane hydrocarbons over the Chinese marginal seas
Concentration and source changes of nitrous acid (HONO) during the COVID-19 lockdown in Beijing
Characteristics and sources of nonmethane volatile organic compounds (NMVOCs) and O3–NOx–NMVOC relationships in Zhengzhou, China
Characterization of biogenic volatile organic compounds and their oxidation products at a stressed pine forest close to a biogas power plant
Deciphering anthropogenic and biogenic contributions to selected non-methane volatile organic compound emissions in an urban area
Emission characteristics of reactive organic gases (ROGs) from industrial volatile chemical products (VCPs) in the Pearl River Delta (PRD), China
Measurement report: Enhanced photochemical formation of formic and isocyanic acids in urban regions aloft – insights from tower-based online gradient measurements
Sources of organic gases and aerosol particles and their roles in nighttime particle growth at a rural forested site in southwest Germany
Surface snow bromide and nitrate at Eureka, Canada, in early spring and implications for polar boundary layer chemistry
Opinion: Strengthening research in the Global South – atmospheric science opportunities in South America and Africa
Analysis of ozone vertical profile day-to-day variability in the lower troposphere during the Paris-2022 ACROSS campaign
Consistency evaluation of tropospheric ozone from ozonesonde and IAGOS aircraft observations: vertical distribution, ozonesonde types and station-airport distance
Investigating Carbonyl Compounds above the Amazon Rainforest using PTR-ToF-MS with NO+ Chemical Ionization
Shipping and algae emissions have a major impact on ambient air mixing ratios of non-methane hydrocarbons (NMHCs) and methanethiol on Utö Island in the Baltic Sea
Measurement report: Long-term measurements of ozone concentrations in semi-natural African ecosystems
Contribution of cooking emissions to the urban volatile organic compounds in Las Vegas, NV
Reanalysis of NOAA H2 observations: implications for the H2 budget
A large role of missing volatile organic compound reactivity from anthropogenic emissions in ozone pollution regulation
Measurement report: Insights into the chemical composition and origin of molecular clusters and potential precursor molecules present in the free troposphere over the southern Indian Ocean: observations from the Maïdo Observatory (2150 m a.s.l., Réunion)
Ozone deposition measurements over wheat fields in the North China Plain: variability and related factors of deposition flux and velocity
Production of oxygenated volatile organic compounds from the ozonolysis of coastal seawater
Comment on “Transport of substantial stratospheric ozone to the surface by a dying typhoon and shallow convection” by Chen et al. (2022)
Observations of cyanogen bromide (BrCN) in the global troposphere and their relation to polar surface O3 destruction
CO2 and CO temporal variability over Mexico City from ground-based total column and surface measurements
Individual coal mine methane emissions constrained by eddy covariance measurements: low bias and missing sources
Discovery of reactive chlorine, sulphur and nitrogen containing ambient volatile organic compounds in the megacity of Delhi during both clean and extremely polluted seasons
Measurement report: In-flight and ground-based measurements of nitrogen oxide emissions from latest generation jet engines and 100% sustainable aviation fuel
Measurement report: Observations of ground-level ozone concentration gradients perpendicular to the Lake Ontario shoreline
Measurement report: The Palau Atmospheric Observatory and its ozonesonde record – continuous monitoring of tropospheric composition and dynamics in the tropical western Pacific
Quantifying SO2 oxidation pathways to atmospheric sulfate using stable sulfur and oxygen isotopes: laboratory simulation and field observation
Influences of downward transport and photochemistry on surface ozone over East Antarctica during austral summer: in situ observations and model simulations
Iodine oxoacids and their roles in sub-3 nm particle growth in polluted urban environments
Intensive photochemical oxidation in the marine atmosphere: evidence from direct radical measurements
Diurnal variations in oxygen and nitrogen isotopes of atmospheric nitrogen dioxide and nitrate: implications for tracing NOx oxidation pathways and emission sources
Measurement report: Method for evaluating CO2 emissions from a cement plant using atmospheric δ(O2 ∕ N2) and CO2 measurements and its implication for future detection of CO2 capture signals
Aircraft-based mass balance estimate of methane emissions from offshore gas facilities in the southern North Sea
Measurement report: Sources, sinks and lifetime of NOX in a sub-urban temperate forest at night
Parameterizations of US wildfire and prescribed fire emission ratios and emission factors based on FIREX-AQ aircraft measurements
Measurement report: Atmospheric nitrate radical chemistry in the South China Sea influenced by the urban outflow of the Pearl River Delta
The interhemispheric gradient of SF6 in the upper troposphere
Lee Tiszenkel, James H. Flynn, and Shan-Hu Lee
Atmos. Chem. Phys., 24, 11351–11363, https://doi.org/10.5194/acp-24-11351-2024, https://doi.org/10.5194/acp-24-11351-2024, 2024
Short summary
Short summary
Ammonia and amines are important ingredients for aerosol formation in urban environments, but the measurements of these compounds are extremely challenging. Our observations show that urban ammonia and amines in Houston are emitted from urban sources, and diurnal variations in their concentrations are likely governed by gas-to-particle conversion and emissions.
Arpit Awasthi, Baerbel Sinha, Haseeb Hakkim, Sachin Mishra, Varkrishna Mummidivarapu, Gurmanjot Singh, Sachin D. Ghude, Vijay Kumar Soni, Narendra Nigam, Vinayak Sinha, and Madhavan N. Rajeevan
Atmos. Chem. Phys., 24, 10279–10304, https://doi.org/10.5194/acp-24-10279-2024, https://doi.org/10.5194/acp-24-10279-2024, 2024
Short summary
Short summary
We use 111 volatile organic compounds (VOCs), PM10, and PM2.5 in a positive matrix factorization (PMF) model to resolve 11 pollution sources validated with chemical fingerprints. Crop residue burning and heating account for ~ 50 % of the PM, while traffic and industrial emissions dominate the gas-phase VOC burden and formation potential of secondary organic aerosols (> 60 %). Non-tailpipe emissions from compressed-natural-gas-fuelled commercial vehicles dominate the transport sector's PM burden.
Luke D. Schiferl, Cong Cao, Bronte Dalton, Andrew Hallward-Driemeier, Ricardo Toledo-Crow, and Róisín Commane
Atmos. Chem. Phys., 24, 10129–10142, https://doi.org/10.5194/acp-24-10129-2024, https://doi.org/10.5194/acp-24-10129-2024, 2024
Short summary
Short summary
Carbon monoxide (CO) is an air pollutant and an important indicator of the incomplete combustion of fossil fuels in cities. Using 4 years of winter and spring observations in New York City, we found that both the magnitude and variability of CO from the metropolitan area are greater than expected. Transportation emissions cannot explain the missing and variable CO, which points to energy from buildings as a likely underappreciated source of urban air pollution and greenhouse gas emissions.
Chengzhi Xing, Cheng Liu, Chunxiang Ye, Jingkai Xue, Hongyu Wu, Xiangguang Ji, Jinping Ou, and Qihou Hu
Atmos. Chem. Phys., 24, 10093–10112, https://doi.org/10.5194/acp-24-10093-2024, https://doi.org/10.5194/acp-24-10093-2024, 2024
Short summary
Short summary
We identified the contributions of ozone (O3) and nitrous acid (HONO) to the production rates of hydroxide (OH) in vertical space on the Tibetan Plateau (TP). A new insight was offered: the contributions of HONO and O3 to the production rates of OH on the TP are even greater than in lower-altitudes areas. This study enriches the understanding of vertical distribution of atmospheric components and explains the strong atmospheric oxidation capacity (AOC) on the TP.
Xinyuan Zhang, Lingling Wang, Nan Wang, Shuangliang Ma, Shenbo Wang, Ruiqin Zhang, Dong Zhang, Mingkai Wang, and Hongyu Zhang
Atmos. Chem. Phys., 24, 9885–9898, https://doi.org/10.5194/acp-24-9885-2024, https://doi.org/10.5194/acp-24-9885-2024, 2024
Short summary
Short summary
This study highlights the importance of the redox reaction of NO2 with SO2 based on actual atmospheric observations. The particle pH in future China is expected to rise steadily. Consequently, this reaction could become a significant source of HONO in China. Therefore, it is crucial to coordinate the control of SO2, NOx, and NH3 emissions to avoid a rapid increase in the particle pH.
Jun Zhou, Chunsheng Zhang, Aiming Liu, Bin Yuan, Yan Wang, Wenjie Wang, Jie-Ping Zhou, Yixin Hao, Xiao-Bing Li, Xianjun He, Xin Song, Yubin Chen, Suxia Yang, Shuchun Yang, Yanfeng Wu, Bin Jiang, Shan Huang, Junwen Liu, Yuwen Peng, Jipeng Qi, Minhui Deng, Bowen Zhong, Yibo Huangfu, and Min Shao
Atmos. Chem. Phys., 24, 9805–9826, https://doi.org/10.5194/acp-24-9805-2024, https://doi.org/10.5194/acp-24-9805-2024, 2024
Short summary
Short summary
In-depth understanding of the near-ground vertical variability in photochemical ozone (O3) formation is crucial for mitigating O3 pollution. Utilizing a self-built vertical observation system, a direct net photochemical O3 production rate detection system, and an observation-based model, we diagnosed the vertical distributions and formation mechanism of net photochemical O3 production rates and sensitivity in the Pearl River Delta region, one of the most O3-polluted areas in China.
Eleanor J. Derry, Tyler R. Elgiar, Taylor Y. Wilmot, Nicholas W. Hoch, Noah S. Hirshorn, Peter Weiss-Penzias, Christopher F. Lee, John C. Lin, A. Gannet Hallar, Rainer Volkamer, Seth N. Lyman, and Lynne E. Gratz
Atmos. Chem. Phys., 24, 9615–9643, https://doi.org/10.5194/acp-24-9615-2024, https://doi.org/10.5194/acp-24-9615-2024, 2024
Short summary
Short summary
Mercury (Hg) is a globally distributed neurotoxic pollutant. Atmospheric deposition is the main source of Hg in ecosystems. However, measurement biases hinder understanding of the origins and abundance of the more bioavailable oxidized form. We used an improved, calibrated measurement system to study air mass composition and transport of atmospheric Hg at a remote mountaintop site in the central US. Oxidized Hg originated upwind in the low to middle free troposphere under clean, dry conditions.
Benjamin A. Nault, Katherine R. Travis, James H. Crawford, Donald R. Blake, Pedro Campuzano-Jost, Ronald C. Cohen, Joshua P. DiGangi, Glenn S. Diskin, Samuel R. Hall, L. Gregory Huey, Jose L. Jimenez, Kyung-Eun Min, Young Ro Lee, Isobel J. Simpson, Kirk Ullmann, and Armin Wisthaler
Atmos. Chem. Phys., 24, 9573–9595, https://doi.org/10.5194/acp-24-9573-2024, https://doi.org/10.5194/acp-24-9573-2024, 2024
Short summary
Short summary
Ozone (O3) is a pollutant formed from the reactions of gases emitted from various sources. In urban areas, the density of human activities can increase the O3 formation rate (P(O3)), thus impacting air quality and health. Observations collected over Seoul, South Korea, are used to constrain P(O3). A high local P(O3) was found; however, local P(O3) was partly reduced due to compounds typically ignored. These observations also provide constraints for unmeasured compounds that will impact P(O3).
Fan Zhang, Binyu Xiao, Zeyu Liu, Yan Zhang, Chongguo Tian, Rui Li, Can Wu, Yali Lei, Si Zhang, Xinyi Wan, Yubao Chen, Yong Han, Min Cui, Cheng Huang, Hongli Wang, Yingjun Chen, and Gehui Wang
Atmos. Chem. Phys., 24, 8999–9017, https://doi.org/10.5194/acp-24-8999-2024, https://doi.org/10.5194/acp-24-8999-2024, 2024
Short summary
Short summary
Mandatory use of low-sulfur fuel due to global sulfur limit regulations means large uncertainties in volatile organic compound (VOC) emissions. On-board tests of VOCs from nine cargo ships in China were carried out. Results showed that switching from heavy-fuel oil to diesel increased emission factor VOCs by 48 % on average, enhancing O3 and the secondary organic aerosol formation potential. Thus, implementing a global ultra-low-sulfur oil policy needs to be optimized in the near future.
Patrick Dewald, Tobias Seubert, Simone T. Andersen, Gunther N. T. E. Türk, Jan Schuladen, Max R. McGillen, Cyrielle Denjean, Jean-Claude Etienne, Olivier Garrouste, Marina Jamar, Sergio Harb, Manuela Cirtog, Vincent Michoud, Mathieu Cazaunau, Antonin Bergé, Christopher Cantrell, Sebastien Dusanter, Bénédicte Picquet-Varrault, Alexandre Kukui, Chaoyang Xue, Abdelwahid Mellouki, Jos Lelieveld, and John N. Crowley
Atmos. Chem. Phys., 24, 8983–8997, https://doi.org/10.5194/acp-24-8983-2024, https://doi.org/10.5194/acp-24-8983-2024, 2024
Short summary
Short summary
In the scope of a field campaign in a suburban forest near Paris in the summer of 2022, we measured the reactivity of the nitrate radical NO3 towards biogenic volatile organic compounds (BVOCs; e.g. monoterpenes) mainly below but also above the canopy. NO3 reactivity was the highest during nights with strong temperature inversions and decreased strongly with height. Reactions with BVOCs were the main removal process of NO3 throughout the diel cycle below the canopy.
Jian Wang, Lei Xue, Qianyao Ma, Feng Xu, Gaobin Xu, Shibo Yan, Jiawei Zhang, Jianlong Li, Honghai Zhang, Guiling Zhang, and Zhaohui Chen
Atmos. Chem. Phys., 24, 8721–8736, https://doi.org/10.5194/acp-24-8721-2024, https://doi.org/10.5194/acp-24-8721-2024, 2024
Short summary
Short summary
This study investigated the distribution and sources of non-methane hydrocarbons (NMHCs) in the lower atmosphere over the marginal seas of China. NMHCs, a subset of volatile organic compounds (VOCs), play a crucial role in atmospheric chemistry. Derived from systematic atmospheric sampling in coastal cities and marginal sea regions, this study offers valuable insights into the interaction between land and sea in shaping offshore atmospheric NMHCs.
Yusheng Zhang, Feixue Zheng, Zemin Feng, Chaofan Lian, Weigang Wang, Xiaolong Fan, Wei Ma, Zhuohui Lin, Chang Li, Gen Zhang, Chao Yan, Ying Zhang, Veli-Matti Kerminen, Federico Bianch, Tuukka Petäjä, Juha Kangasluoma, Markku Kulmala, and Yongchun Liu
Atmos. Chem. Phys., 24, 8569–8587, https://doi.org/10.5194/acp-24-8569-2024, https://doi.org/10.5194/acp-24-8569-2024, 2024
Short summary
Short summary
The nitrous acid (HONO) budget was validated during a COVID-19 lockdown event. The main conclusions are (1) HONO concentrations showed a significant decrease from 0.97 to 0.53 ppb during lockdown; (2) vehicle emissions accounted for 53 % of nighttime sources, with the heterogeneous conversion of NO2 on ground surfaces more important than aerosol; and (3) the dominant daytime source shifted from the homogenous reaction between NO and OH (51 %) to nitrate photolysis (53 %) during lockdown.
Dong Zhang, Xiao Li, Minghao Yuan, Yifei Xu, Qixiang Xu, Fangcheng Su, Shenbo Wang, and Ruiqin Zhang
Atmos. Chem. Phys., 24, 8549–8567, https://doi.org/10.5194/acp-24-8549-2024, https://doi.org/10.5194/acp-24-8549-2024, 2024
Short summary
Short summary
The increasing concentration of O3 precursors and unfavorable meteorological conditions are key factors in the formation of O3 pollution in Zhengzhou. Vehicular exhausts (28 %), solvent usage (27 %), and industrial production (22 %) are identified as the main sources of NMVOCs. Moreover, O3 formation in Zhengzhou is found to be in an anthropogenic volatile organic compound (AVOC)-limited regime. Thus, to reduce O3 formation, a minimum AVOCs / NOx reduction ratio ≥ 3 : 1 is recommended.
Junwei Song, Georgios I. Gkatzelis, Ralf Tillmann, Nicolas Brüggemann, Thomas Leisner, and Harald Saathoff
EGUsphere, https://doi.org/10.5194/egusphere-2024-1768, https://doi.org/10.5194/egusphere-2024-1768, 2024
Short summary
Short summary
VOCs and organic aerosol (OA) particles were measured online at an European stressed pine forest site. Higher temperatures can enhance the forest emissions of biogenic VOCs exceeding their photochemical consumption during daytime. Weakly oxidized monoterpene products dominated the VOCs during nighttime. Moreover, increasing relative humidity can promote the gas-to-particle partitioning of these weakly oxidized monoterpene products, leading to increased OA mass.
Arianna Peron, Martin Graus, Marcus Striednig, Christian Lamprecht, Georg Wohlfahrt, and Thomas Karl
Atmos. Chem. Phys., 24, 7063–7083, https://doi.org/10.5194/acp-24-7063-2024, https://doi.org/10.5194/acp-24-7063-2024, 2024
Short summary
Short summary
The anthropogenic fraction of non-methane volatile organic compound (NMVOC) emissions associated with biogenic sources (e.g., terpenes) is investigated based on eddy covariance observations. The anthropogenic fraction of terpene emissions is strongly dependent on season. When analyzing volatile chemical product (VCP) emissions in urban environments, we caution that observations from short-term campaigns might over-/underestimate their significance depending on local and seasonal circumstances.
Sihang Wang, Bin Yuan, Xianjun He, Ru Cui, Xin Song, Yubin Chen, Caihong Wu, Chaomin Wang, Yibo Huangfu, Xiao-Bing Li, Boguang Wang, and Min Shao
Atmos. Chem. Phys., 24, 7101–7121, https://doi.org/10.5194/acp-24-7101-2024, https://doi.org/10.5194/acp-24-7101-2024, 2024
Short summary
Short summary
Emissions of reactive organic gases from industrial volatile chemical product sources are measured. There are large differences among these industrial sources. We show that oxygenated species account for significant contributions to reactive organic gas emissions, especially for industrial sources utilizing water-borne chemicals.
Qing Yang, Xiao-Bing Li, Bin Yuan, Xiaoxiao Zhang, Yibo Huangfu, Lei Yang, Xianjun He, Jipeng Qi, and Min Shao
Atmos. Chem. Phys., 24, 6865–6882, https://doi.org/10.5194/acp-24-6865-2024, https://doi.org/10.5194/acp-24-6865-2024, 2024
Short summary
Short summary
Online vertical gradient measurements of formic and isocyanic acids were made based on a 320 m tower in a megacity. Vertical variations and sources of the two acids were analyzed in this study. We find that formic and isocyanic acids exhibited positive vertical gradients and were mainly contributed by photochemical formations. The formation of formic and isocyanic acids was also significantly enhanced in urban regions aloft.
Junwei Song, Harald Saathoff, Feng Jiang, Linyu Gao, Hengheng Zhang, and Thomas Leisner
Atmos. Chem. Phys., 24, 6699–6717, https://doi.org/10.5194/acp-24-6699-2024, https://doi.org/10.5194/acp-24-6699-2024, 2024
Short summary
Short summary
This study presents concurrent online measurements of organic gas and particles (VOCs and OA) at a forested site in summer. Both VOCs and OA were largely contributed by oxygenated organic compounds. Semi-volatile oxygenated OA and organic nitrate formed from monoterpenes and sesquiterpenes contributed significantly to nighttime particle growth. The results help us to understand the causes of nighttime particle growth regularly observed in summer in central European rural forested environments.
Xin Yang, Kimberly Strong, Alison S. Criscitiello, Marta Santos-Garcia, Kristof Bognar, Xiaoyi Zhao, Pierre Fogal, Kaley A. Walker, Sara M. Morris, and Peter Effertz
Atmos. Chem. Phys., 24, 5863–5886, https://doi.org/10.5194/acp-24-5863-2024, https://doi.org/10.5194/acp-24-5863-2024, 2024
Short summary
Short summary
This study uses snow samples collected from a Canadian high Arctic site, Eureka, to demonstrate that surface snow in early spring is a net sink of atmospheric bromine and nitrogen. Surface snow bromide and nitrate are significantly correlated, indicating the oxidation of reactive nitrogen is accelerated by reactive bromine. In addition, we show evidence that snow photochemical release of reactive bromine is very weak, and its emission flux is much smaller than the deposition flux of bromide.
Rebecca M. Garland, Katye E. Altieri, Laura Dawidowski, Laura Gallardo, Aderiana Mbandi, Nestor Y. Rojas, and N'datchoh E. Touré
Atmos. Chem. Phys., 24, 5757–5764, https://doi.org/10.5194/acp-24-5757-2024, https://doi.org/10.5194/acp-24-5757-2024, 2024
Short summary
Short summary
This opinion piece focuses on two geographical areas in the Global South where the authors are based that are underrepresented in atmospheric science. This opinion provides context on common challenges and constraints, with suggestions on how the community can address these. The focus is on the strengths of atmospheric science research in these regions. It is these strengths, we believe, that highlight the critical role of Global South researchers in the future of atmospheric science research.
Gerard Ancellet, Camille Viatte, Anne Boynard, François Ravetta, Jacques Pelon, Cristelle Cailteau-Fischbach, Pascal Genau, Julie Capo, Axel Roy, and Philippe Nédélec
EGUsphere, https://doi.org/10.5194/egusphere-2024-892, https://doi.org/10.5194/egusphere-2024-892, 2024
Short summary
Short summary
Characterization of ozone pollution in urban areas has benefited from a measurement campaign in summer 2022 in the Paris region. The analysis is based on 21 days of lidar and aircraft observations. The main objective is a sensitivity analysis of ozone pollution to first the micrometeorological processes in the urban atmospheric boundary layer, and second, the transport of regional pollution. The paper also discuss to what extent satellite observations can track the observed ozone plumes.
Honglei Wang, David W. Tarasick, Jane Liu, Herman G. J. Smit, Roeland Van Malderen, Lijuan Shen, and Tianliang Zhao
EGUsphere, https://doi.org/10.5194/egusphere-2024-1015, https://doi.org/10.5194/egusphere-2024-1015, 2024
Short summary
Short summary
In this study, we identify 23 suitable pairs of sites in the WOUDC and IAGOS datasets from 1995 to 2021, compare the average vertical distribution of tropospheric O3 shown by ozonesonde and aircraft measurements, and analyze their differences by ozonesonde type and by station-airport distance.
Akima Ringsdorf, Achim Edtbauer, Bruna Holanda, Christopher Poehlker, Marta O. Sá, Alessandro Araújo, Jürgen Kesselmeier, Jos Lelieveld, and Jonathan Williams
EGUsphere, https://doi.org/10.5194/egusphere-2024-1210, https://doi.org/10.5194/egusphere-2024-1210, 2024
Short summary
Short summary
We show the average height distribution of separately observed aldehydes and ketones over a day and discuss their rainforest-specific sources and sinks and their seasonal changes above the Amazon rainforest. Ketones have much longer atmospheric lifetimes than aldehydes, and thus different implications for atmospheric chemistry. However, they are commonly observed together, which we overcome by measuring with a NO+ chemical ionization mass spectrometer for the first time in the Amazon rainforest.
Heidi Hellén, Rostislav Kouznetsov, Kaisa Kraft, Jukka Seppälä, Mika Vestenius, Jukka-Pekka Jalkanen, Lauri Laakso, and Hannele Hakola
Atmos. Chem. Phys., 24, 4717–4731, https://doi.org/10.5194/acp-24-4717-2024, https://doi.org/10.5194/acp-24-4717-2024, 2024
Short summary
Short summary
Mixing ratios of C2-C5 NMHCs and methanethiol were measured on an island in the Baltic Sea using an in situ gas chromatograph. Shipping emissions were found to be an important source of ethene, ethyne, propene, and benzene. High summertime mixing ratios of methanethiol and dependence of mixing ratios on seawater temperature and height indicated the biogenic origin to possibly be phytoplankton or macroalgae. These emissions may have a strong impact on SO2 production and new particle formation.
Hagninou Elagnon Venance Donnou, Aristide Barthélémy Akpo, Money Ossohou, Claire Delon, Véronique Yoboué, Dungall Laouali, Marie Ouafo-Leumbe, Pieter Gideon Van Zyl, Ousmane Ndiaye, Eric Gardrat, Maria Dias-Alves, and Corinne Galy-Lacaux
EGUsphere, https://doi.org/10.5194/egusphere-2024-284, https://doi.org/10.5194/egusphere-2024-284, 2024
Short summary
Short summary
Ozone is a secondary air pollutant that is detrimental to human and plant health. A better understanding of its chemical evolution is a challenge for Africa, where it is still under-sampled. Out of 14 sites examined (1995–2020), high levels of O3 are reported in southern Africa. The dominant chemical processes leading to O3 formation are identified. A decrease in O3 is observed at Katibougou (Mali) and Banizoumbou (Niger), and an increase at Zoétélé (Cameroon) and Skukuza (South Africa).
Matthew M. Coggon, Chelsea E. Stockwell, Lu Xu, Jeff Peischl, Jessica B. Gilman, Aaron Lamplugh, Henry J. Bowman, Kenneth Aikin, Colin Harkins, Qindan Zhu, Rebecca H. Schwantes, Jian He, Meng Li, Karl Seltzer, Brian McDonald, and Carsten Warneke
Atmos. Chem. Phys., 24, 4289–4304, https://doi.org/10.5194/acp-24-4289-2024, https://doi.org/10.5194/acp-24-4289-2024, 2024
Short summary
Short summary
Residential and commercial cooking emits pollutants that degrade air quality. Here, ambient observations show that cooking is an important contributor to anthropogenic volatile organic compounds (VOCs) emitted in Las Vegas, NV. These emissions are not fully presented in air quality models, and more work may be needed to quantify emissions from important sources, such as commercial restaurants.
Fabien Paulot, Gabrielle Pétron, Andrew M. Crotwell, and Matteo B. Bertagni
Atmos. Chem. Phys., 24, 4217–4229, https://doi.org/10.5194/acp-24-4217-2024, https://doi.org/10.5194/acp-24-4217-2024, 2024
Short summary
Short summary
New data from the National Oceanic and Atmospheric Administration show that hydrogen (H2) concentrations increased from 2010 to 2019, which is consistent with the simulated increase in H2 photochemical production (mainly from methane). But this cannot be reconciled with the expected decrease (increase) in H2 anthropogenic emissions (soil deposition) in the same period. This shows gaps in our knowledge of the H2 biogeochemical cycle that must be resolved to quantify the impact of higher H2 usage.
Wenjie Wang, Bin Yuan, Hang Su, Yafang Cheng, Jipeng Qi, Sihang Wang, Wei Song, Xinming Wang, Chaoyang Xue, Chaoqun Ma, Fengxia Bao, Hongli Wang, Shengrong Lou, and Min Shao
Atmos. Chem. Phys., 24, 4017–4027, https://doi.org/10.5194/acp-24-4017-2024, https://doi.org/10.5194/acp-24-4017-2024, 2024
Short summary
Short summary
This study investigates the important role of unmeasured volatile organic compounds (VOCs) in ozone formation. Based on results in a megacity of China, we show that unmeasured VOCs can contribute significantly to ozone fomation and also influence the determination of ozone control strategy. Our results show that these unmeasured VOCs are mainly from human sources.
Romain Salignat, Matti Rissanen, Siddharth Iyer, Jean-Luc Baray, Pierre Tulet, Jean-Marc Metzger, Jérôme Brioude, Karine Sellegri, and Clémence Rose
Atmos. Chem. Phys., 24, 3785–3812, https://doi.org/10.5194/acp-24-3785-2024, https://doi.org/10.5194/acp-24-3785-2024, 2024
Short summary
Short summary
Using mass spectrometry data collected at the Maïdo Observatory (2160 m a.s.l., Réunion), we provide the first detailed analysis of molecular cluster chemical composition specifically in the marine free troposphere. The abundance of the identified species is related both to in situ meteorological parameters and air mass history, which also provide insight into their origin. Our work makes an important contribution to documenting the chemistry and physics of the marine free troposphere.
Xiaoyi Zhang, Wanyun Xu, Weili Lin, Gen Zhang, Jinjian Geng, Li Zhou, Huarong Zhao, Sanxue Ren, Guangsheng Zhou, Jianmin Chen, and Xiaobin Xu
EGUsphere, https://doi.org/10.5194/egusphere-2024-643, https://doi.org/10.5194/egusphere-2024-643, 2024
Short summary
Short summary
Ozone (O3) deposition is a key process removing surface O3, affecting air quality, ecosystem and climate change. This study conducted an O3 deposition measurement over wheat canopy using a newly relaxed eddy accumulation flux system. Large variabilities of O3 deposition were detected mainly determined by crop growth and modulated by various environmental factors. More O3 deposition observations over different surfaces are needed for exploring deposition mechanism, model optimization.
Delaney B. Kilgour, Gordon A. Novak, Megan S. Claflin, Brian M. Lerner, and Timothy H. Bertram
Atmos. Chem. Phys., 24, 3729–3742, https://doi.org/10.5194/acp-24-3729-2024, https://doi.org/10.5194/acp-24-3729-2024, 2024
Short summary
Short summary
Laboratory experiments with seawater mimics suggest ozone deposition to the surface ocean can be a source of reactive carbon to the marine atmosphere. We conduct both field and laboratory measurements to assess abiotic VOC composition and yields from ozonolysis of real surface seawater. We show that C5–C11 aldehydes contribute to the observed VOC emission flux. We estimate that VOCs generated by the ozonolysis of surface seawater are competitive with biological VOC production and emission.
Xiangdong Zheng, Wen Yang, Yuting Sun, Chunmei Geng, Yingying Liu, and Xiaobin Xu
Atmos. Chem. Phys., 24, 3759–3768, https://doi.org/10.5194/acp-24-3759-2024, https://doi.org/10.5194/acp-24-3759-2024, 2024
Short summary
Short summary
Chen et al. (2022) attributed the nocturnal ozone enhancement (NOE) during the night of 31 July 2021 in the North China Plain (NCP) to "the direct stratospheric intrusion to reach the surface". We analyzed in situ data from the NCP. Our results do not suggest that there was a significant impact from the stratosphere on surface ozone during the NOE. We argue that the NOE was not caused by stratospheric intrusion but originated from fresh photochemical production in the lower troposphere.
James M. Roberts, Siyuan Wang, Patrick R. Veres, J. Andrew Neuman, Michael A. Robinson, Ilann Bourgeois, Jeff Peischl, Thomas B. Ryerson, Chelsea R. Thompson, Hannah M. Allen, John D. Crounse, Paul O. Wennberg, Samuel R. Hall, Kirk Ullmann, Simone Meinardi, Isobel J. Simpson, and Donald Blake
Atmos. Chem. Phys., 24, 3421–3443, https://doi.org/10.5194/acp-24-3421-2024, https://doi.org/10.5194/acp-24-3421-2024, 2024
Short summary
Short summary
We measured cyanogen bromide (BrCN) in the troposphere for the first time. BrCN is a product of the same active bromine chemistry that destroys ozone and removes mercury in polar surface environments and is a previously unrecognized sink for active Br compounds. BrCN has an apparent lifetime against heterogeneous loss in the range 1–10 d, so it serves as a cumulative marker of Br-radical chemistry. Accounting for BrCN chemistry is an important part of understanding polar Br cycling.
Noémie Taquet, Wolfgang Stremme, María Eugenia Gonzalez del Castillo, Victor Almanza, Alejandro Bezanilla, Olivier Laurent, Carlos Alberti, Frank Hase, Michel Ramonet, Thomas Lauvaux, Ke Che, and Michel Grutter
EGUsphere, https://doi.org/10.5194/egusphere-2024-512, https://doi.org/10.5194/egusphere-2024-512, 2024
Short summary
Short summary
We studied the variability of CO and CO2 and their ratio over Mexico City from long-term time-resolved FTIR solar absorption and surface measurements. Using the average intraday CO growth rate from total columns and TROPOMI measurements, we additionally estimate the interannual variability of CO and CO2 anthropogenic emissions of the City and relate it to the main influencing events of the last decade, such as the COVID-19 lock-down.
Kai Qin, Wei Hu, Qin He, Fan Lu, and Jason Blake Cohen
Atmos. Chem. Phys., 24, 3009–3028, https://doi.org/10.5194/acp-24-3009-2024, https://doi.org/10.5194/acp-24-3009-2024, 2024
Short summary
Short summary
We compute CH4 emissions and uncertainty on a mine-by-mine basis, including underground, overground, and abandoned mines. Mine-by-mine gas and flux data and 30 min observations from a flux tower located next to a mine shaft are integrated. The observed variability and bias correction are propagated over the emissions dataset, demonstrating that daily observations may not cover the range of variability. Comparisons show both an emissions magnitude and spatial mismatch with current inventories.
Sachin Mishra, Vinayak Sinha, Haseeb Hakkim, Arpit Awasthi, Sachin D. Ghude, Vijay Kumar Soni, Narendra Nigam, Baerbel Sinha, and Madhavan N. Rajeevan
EGUsphere, https://doi.org/10.5194/egusphere-2024-500, https://doi.org/10.5194/egusphere-2024-500, 2024
Short summary
Short summary
We quantified 111 gases using extended volatility mass spectrometry to understand how changes in seasonality and emissions lead from clean air in monsoon to extremely polluted air in the post-monsoon season in Delhi. Averaged total mass concentrations (260 µgm-3) were >4 times in polluted periods, driven by biomass burning emissions and reduced atmospheric ventilation. Reactive gaseous nitrogen, chlorine and sulphur compounds hitherto un-reported from such a polluted environment were discovered.
Theresa Harlass, Rebecca Dischl, Stefan Kaufmann, Raphael Märkl, Daniel Sauer, Monika Scheibe, Paul Stock, Tiziana Bräuer, Andreas Dörnbrack, Anke Roiger, Hans Schlager, Ulrich Schumann, Tobias Schripp, Tobias Grein, Linda Bondorf, Charles Renard, Maxime Gauthier, Mark Johnson, Darren Luff, Paul Madden, Peter Swann, Denise Ahrens, Reetu Sallinen, and Christiane Voigt
EGUsphere, https://doi.org/10.5194/egusphere-2024-454, https://doi.org/10.5194/egusphere-2024-454, 2024
Short summary
Short summary
Emissions from aircraft have a direct impact on our climate. Here, we present airborne and ground based measurement data of nitrogen oxides which were collected in the exhaust of an Airbus aircraft. We study the impact of burning fossil and sustainable aviation fuel on nitrogen oxide emissions at different engine settings related to combustor temperature, pressure and fuel flow. Further, we compare observations with engine emission models.
Yao Yan Huang and D. James Donaldson
Atmos. Chem. Phys., 24, 2387–2398, https://doi.org/10.5194/acp-24-2387-2024, https://doi.org/10.5194/acp-24-2387-2024, 2024
Short summary
Short summary
Ground-level ozone interacts at the lake–land boundary; this is important to our understanding and modelling of atmospheric chemistry and air pollution in the lower atmosphere. We show that a steep ozone gradient occurs year-round moving inland up to 1 km from the lake and that this gradient is influenced by seasonal factors on the local land environment, where more rural areas are more greatly affected seasonally.
Katrin Müller, Jordis S. Tradowsky, Peter von der Gathen, Christoph Ritter, Sharon Patris, Justus Notholt, and Markus Rex
Atmos. Chem. Phys., 24, 2169–2193, https://doi.org/10.5194/acp-24-2169-2024, https://doi.org/10.5194/acp-24-2169-2024, 2024
Short summary
Short summary
The Palau Atmospheric Observatory is introduced as an ideal site to detect changes in atmospheric composition and dynamics above the remote tropical western Pacific. We focus on the ozone sounding program from 2016–2021, including El Niño 2016. The year-round high convective activity is reflected in dominant low tropospheric ozone and high relative humidity. Their seasonal distributions are unique compared to other tropical sites and are modulated by the Intertropical Convergence Zone.
Ziyan Guo, Keding Lu, Pengxiang Qiu, Mingyi Xu, and Zhaobing Guo
Atmos. Chem. Phys., 24, 2195–2205, https://doi.org/10.5194/acp-24-2195-2024, https://doi.org/10.5194/acp-24-2195-2024, 2024
Short summary
Short summary
The formation of secondary sulfate needs to be further explored. In this work, we simultaneously measured sulfur and oxygen isotopic compositions to gain an increased understanding of specific sulfate formation processes. The results indicated that secondary sulfate was mainly ascribed to SO2 homogeneous oxidation by OH radicals and heterogeneous oxidation by H2O2 and Fe3+ / O2. This study is favourable for deeply investigating the sulfur cycle in the atmosphere.
Imran A. Girach, Narendra Ojha, Prabha R. Nair, Kandula V. Subrahmanyam, Neelakantan Koushik, Mohammed M. Nazeer, Nadimpally Kiran Kumar, Surendran Nair Suresh Babu, Jos Lelieveld, and Andrea Pozzer
Atmos. Chem. Phys., 24, 1979–1995, https://doi.org/10.5194/acp-24-1979-2024, https://doi.org/10.5194/acp-24-1979-2024, 2024
Short summary
Short summary
We investigate surface ozone variability in East Antarctica based on measurements and EMAC global model simulations during austral summer. Nearly half of the surface ozone is found to be of stratospheric origin. The east coast of Antarctica acts as a stronger sink of ozone than surrounding regions. Photochemical loss of ozone is counterbalanced by downward transport of ozone. The study highlights the intertwined role of chemistry and dynamics in governing ozone variations over East Antarctica.
Ying Zhang, Duzitian Li, Xu-Cheng He, Wei Nie, Chenjuan Deng, Runlong Cai, Yuliang Liu, Yishuo Guo, Chong Liu, Yiran Li, Liangduo Chen, Yuanyuan Li, Chenjie Hua, Tingyu Liu, Zongcheng Wang, Jiali Xie, Lei Wang, Tuukka Petäjä, Federico Bianchi, Ximeng Qi, Xuguang Chi, Pauli Paasonen, Yongchun Liu, Chao Yan, Jingkun Jiang, Aijun Ding, and Markku Kulmala
Atmos. Chem. Phys., 24, 1873–1893, https://doi.org/10.5194/acp-24-1873-2024, https://doi.org/10.5194/acp-24-1873-2024, 2024
Short summary
Short summary
This study conducts a long-term observation of gaseous iodine oxoacids in two Chinese megacities, revealing their ubiquitous presence with peak concentrations (up to 0.1 pptv) in summer. Our analysis suggests a mix of terrestrial and marine sources for iodine. Additionally, iodic acid is identified as a notable contributor to sub-3 nm particle growth and particle survival probability.
Guoxian Zhang, Renzhi Hu, Pinhua Xie, Changjin Hu, Xiaoyan Liu, Liujun Zhong, Haotian Cai, Bo Zhu, Shiyong Xia, Xiaofeng Huang, Xin Li, and Wenqing Liu
Atmos. Chem. Phys., 24, 1825–1839, https://doi.org/10.5194/acp-24-1825-2024, https://doi.org/10.5194/acp-24-1825-2024, 2024
Short summary
Short summary
Comprehensive observation of HOx radicals was conducted at a coastal site in the Pearl River Delta. Radical chemistry was influenced by different air masses in a time-dependent way. Land mass promotes a more active photochemical process, with daily averages of 7.1 × 106 and 5.2 × 108 cm−3 for OH and HO2 respectively. The rapid oxidation process was accompanied by a higher diurnal HONO concentration, which influences the ozone-sensitive system and eventually magnifies the background ozone.
Sarah Albertin, Joël Savarino, Slimane Bekki, Albane Barbero, Roberto Grilli, Quentin Fournier, Irène Ventrillard, Nicolas Caillon, and Kathy Law
Atmos. Chem. Phys., 24, 1361–1388, https://doi.org/10.5194/acp-24-1361-2024, https://doi.org/10.5194/acp-24-1361-2024, 2024
Short summary
Short summary
This study reports the first simultaneous records of oxygen (Δ17O) and nitrogen (δ15N) isotopes in nitrogen dioxide (NO2) and nitrate (NO3−). These data are combined with atmospheric observations to explore sub-daily N reactive chemistry and quantify N fractionation effects in an Alpine winter city. The results highlight the necessity of using Δ17O and δ15N in both NO2 and NO3− to avoid biased estimations of NOx sources and fates from NO3− isotopic records in urban winter environments.
Shigeyuki Ishidoya, Kazuhiro Tsuboi, Hiroaki Kondo, Kentaro Ishijima, Nobuyuki Aoki, Hidekazu Matsueda, and Kazuyuki Saito
Atmos. Chem. Phys., 24, 1059–1077, https://doi.org/10.5194/acp-24-1059-2024, https://doi.org/10.5194/acp-24-1059-2024, 2024
Short summary
Short summary
A method evaluating techniques for carbon neutrality, such as carbon capture and storage (CCS), is important. This study presents a method to evaluate CO2 emissions from a cement plant based on atmospheric O2 and CO2 measurements. The method will also be useful for evaluating CO2 capture from flue gas at CCS plants, since the plants remove CO2 from the atmosphere without causing any O2 changes, just as cement plants do, differing only in the direction of CO2 exchange with the atmosphere.
Magdalena Pühl, Anke Roiger, Alina Fiehn, Alan M. Gorchov Negron, Eric A. Kort, Stefan Schwietzke, Ignacio Pisso, Amy Foulds, James Lee, James L. France, Anna E. Jones, Dave Lowry, Rebecca E. Fisher, Langwen Huang, Jacob Shaw, Prudence Bateson, Stephen Andrews, Stuart Young, Pamela Dominutti, Tom Lachlan-Cope, Alexandra Weiss, and Grant Allen
Atmos. Chem. Phys., 24, 1005–1024, https://doi.org/10.5194/acp-24-1005-2024, https://doi.org/10.5194/acp-24-1005-2024, 2024
Short summary
Short summary
In April–May 2019 we carried out an airborne field campaign in the southern North Sea with the aim of studying methane emissions of offshore gas installations. We determined methane emissions from elevated methane measured downstream of the sampled installations. We compare our measured methane emissions with estimated methane emissions from national and global annual inventories. As a result, we find inconsistencies of inventories and large discrepancies between measurements and inventories.
Simone T. Andersen, Max R. McGillen, Chaoyang Xue, Tobias Seubert, Patrick Dewald, Gunther N. T. E. Türk, Jan Schuladen, Cyrielle Denjean, Jean-Claude Etienne, Olivier Garrouste, Marina Jamar, Sergio Harb, Manuela Cirtog, Vincent Michoud, Mathieu Cazaunau, Antonin Bergé, Christopher Cantrell, Sebastien Dusanter, Bénédicte Picquet-Varrault, Alexandre Kukui, Abdelwahid Mellouki, Lucy J. Carpenter, Jos Lelieveld, and John N. Crowley
EGUsphere, https://doi.org/10.5194/egusphere-2023-2848, https://doi.org/10.5194/egusphere-2023-2848, 2024
Short summary
Short summary
Through measurements of various trace gases in a sub-urban forest near Paris in the summer of 2022 we were able to gain insight into the sources and sinks of NOx (NO+NO2) with a special focus on their nighttime chemical/physical loss processes. NO was observed as a result of nighttime soil emissions when ozone levels were strongly depleted by deposition. NO oxidation products were not observed at night indicating that soil and/or foliar surfaces are an efficient sink of reactive nitrogen.
Georgios I. Gkatzelis, Matthew M. Coggon, Chelsea E. Stockwell, Rebecca S. Hornbrook, Hannah Allen, Eric C. Apel, Megan M. Bela, Donald R. Blake, Ilann Bourgeois, Steven S. Brown, Pedro Campuzano-Jost, Jason M. St. Clair, James H. Crawford, John D. Crounse, Douglas A. Day, Joshua P. DiGangi, Glenn S. Diskin, Alan Fried, Jessica B. Gilman, Hongyu Guo, Johnathan W. Hair, Hannah S. Halliday, Thomas F. Hanisco, Reem Hannun, Alan Hills, L. Gregory Huey, Jose L. Jimenez, Joseph M. Katich, Aaron Lamplugh, Young Ro Lee, Jin Liao, Jakob Lindaas, Stuart A. McKeen, Tomas Mikoviny, Benjamin A. Nault, J. Andrew Neuman, John B. Nowak, Demetrios Pagonis, Jeff Peischl, Anne E. Perring, Felix Piel, Pamela S. Rickly, Michael A. Robinson, Andrew W. Rollins, Thomas B. Ryerson, Melinda K. Schueneman, Rebecca H. Schwantes, Joshua P. Schwarz, Kanako Sekimoto, Vanessa Selimovic, Taylor Shingler, David J. Tanner, Laura Tomsche, Krystal T. Vasquez, Patrick R. Veres, Rebecca Washenfelder, Petter Weibring, Paul O. Wennberg, Armin Wisthaler, Glenn M. Wolfe, Caroline C. Womack, Lu Xu, Katherine Ball, Robert J. Yokelson, and Carsten Warneke
Atmos. Chem. Phys., 24, 929–956, https://doi.org/10.5194/acp-24-929-2024, https://doi.org/10.5194/acp-24-929-2024, 2024
Short summary
Short summary
This study reports emissions of gases and particles from wildfires. These emissions are related to chemical proxies that can be measured by satellite and incorporated into models to improve predictions of wildfire impacts on air quality and climate.
Jie Wang, Haichao Wang, Yee Jun Tham, Lili Ming, Zelong Zheng, Guizhen Fang, Cuizhi Sun, Zhenhao Ling, Jun Zhao, and Shaojia Fan
Atmos. Chem. Phys., 24, 977–992, https://doi.org/10.5194/acp-24-977-2024, https://doi.org/10.5194/acp-24-977-2024, 2024
Short summary
Short summary
Many works report NO3 chemistry in inland regions while less target marine regions. We measured N2O5 and related species on a typical island and found intensive nighttime chemistry and rapid NO3 loss. NO contributed significantly to NO3 loss despite its sub-ppbv level, suggesting nocturnal NO3 reactions would be largely enhanced once free from NO emissions in the open ocean. This highlights the strong influences of urban outflow on downward marine areas in terms of nighttime chemistry.
Tanja J. Schuck, Johannes Degen, Eric Hintsa, Peter Hoor, Markus Jesswein, Timo Keber, Daniel Kunkel, Fred Moore, Florian Obersteiner, Matt Rigby, Thomas Wagenhäuser, Luke M. Western, Andreas Zahn, and Andreas Engel
Atmos. Chem. Phys., 24, 689–705, https://doi.org/10.5194/acp-24-689-2024, https://doi.org/10.5194/acp-24-689-2024, 2024
Short summary
Short summary
We study the interhemispheric gradient of sulfur hexafluoride (SF6), a strong long-lived greenhouse gas. Its emissions are stronger in the Northern Hemisphere; therefore, mixing ratios in the Southern Hemisphere lag behind. Comparing the observations to a box model, the model predicts air in the Southern Hemisphere to be older. For a better agreement, the emissions used as model input need to be increased (and their spatial pattern changed), and we need to modify north–south transport.
Cited articles
AMAP/UNEP: Technical Background Report for the Global Mercury Assessment
2013, Arctic Monitoring and Assessment Programme, 2013.
Ashbaugh, L. L., Malm, W. C., and Sadeh, W. Z.: A residence time probability
analysis of sulfur concentrations at Grand Canyon National Park, Atmos.
Environ., 19, 1263–1270, 1985.
Bottenheim, J., Gallant, A. G., and Brice, K. A.: Measurements of NOy
species and O3 at 82 N latitude, Geophys. Res. Lett., 13,
113–116, 1986.
Brioude, J., Arnold, D., Stohl, A., Cassiani, M., Morton, D., Seibert, P.,
Angevine, W., Evan, S., Dingwell, A., Fast, J. D., Easter, R. C., Pisso, I.,
Burkhart, J., and Wotawa, G.: The Lagrangian particle dispersion model
FLEXPART-WRF version 3.1, Geosci. Model Dev., 6, 1889–1904,
https://doi.org/10.5194/gmd-6-1889-2013, 2013.
Burger Chakraborty, L., Qureshi, A., Vadenbo, C., and Hellweg, S.:
Anthropogenic mercury flows in India and impacts of emission controls,
Environ. Sci. Technol., 47, 8105–8113, 2013.
Chen, L., Liu, M., Xu, Z., Fan, R., Tao, J., Chen, D., Zhang, D., Xie, D.,
and Sun, J.: Variation trends and influencing factors of total gaseous
mercury in the Pearl River Delta – A highly industrialised region in South
China influenced by seasonal monsoons, Atmos. Environ., 77, 757–766,
2013.
Ci, Z., Peng, F., Xue, X., and Zhang, X.: Air-surface exchange of gaseous
mercury over permafrost soil: an investigation at a high-altitude
(4700 m a.s.l.) and remote site in the central Qinghai-Tibet Plateau, Atmos.
Chem. Phys., 16, 14741–14754, https://doi.org/10.5194/acp-16-14741-2016,
2016.
Ci, Z., Zhang, X., Wang, Z., and Niu, Z.: Atmospheric gaseous elemental
mercury (GEM) over a coastal/rural site downwind of East China: temporal
variation and long-range transport, Atmos. Environ., 45, 2480–2487,
2011.
Cong, Z., Kang, S., Liu, X., and Wang, G.: Elemental composition of aerosol
in the Nam Co region, Tibetan Plateau, during summer monsoon season,
Atmos. Environ., 41, 1180–1187, 2007.
Cong, Z., Kawamura, K., Kang, S., and Fu, P.: Penetration of biomass-burning
emissions from South Asia through the Himalayas: new insights from
atmospheric organic acids, Sci. Rep., 5, 9580, 2015.
Davies, D., Kumar, S., and Descloitres, J.: Global Fire Monitoring Use of
MODIS Near-real-time Satellite Data, GIM INT., 18, 41–43, 2004.
Dou, H., Wang, S., Wang, L., Zhang, L., and Hao, J.: Characteristics of
total gaseous mercury concentrations at a rural site of Yangtze Delta,
China, Huan jing ke xue= Huanjing kexue, 34, 1–7, 2013.
de Foy, B., Wiedinmyer, C., and Schauer, J. J.: Estimation of mercury
emissions from forest fires, lakes, regional and local sources using
measurements in Milwaukee and an inverse method, Atmos. Chem. Phys., 12,
8993–9011, https://doi.org/10.5194/acp-12-8993-2012, 2012.
de Foy, B., Lu, Z., and Streets, D. G.: Impacts of control strategies, the
great recession and weekday variations on NO2 columns above North
American cities, Atmos. Environ., 138, 74–86, 2016a.
de Foy, B., Tong, Y., Yin, X., Zhang, W., Kang, S., Zhang, Q., Zhang, G.,
Wang, X., and Schauer, J. J.: First field-based atmospheric observation of
the reduction of reactive mercury driven by sunlight, Atmos.
Environ., 134, 27–39, 2016b.
de Foy, B., Lu, Z., and Streets, D. G.: Satellite NO2 retrievals
suggest China has exceeded its NOx reduction goals from the twelfth
Five-Year Plan, Sci. Rep., 6, 35912, 2016c.
de Foy, B.: City-level variations in NOx emissions derived
from hourly monitoring data in Chicago, Atmos. Environ., 176, 128–139, 2017.
Denzler, B., Bogdal, C., Henne, S., Obrist, D., Steinbacher, M., and
Hungerbühler, K.: Inversion Approach to Validate Mercury Emissions Based on
Background Air Monitoring at the High Altitude Research Station Jungfraujoch
(3580 m), Environ. Scie. Technol., 51, 2846–2853, 2017.
Draxler, R. R. and Rolph, G.: HYSPLIT (HYbrid Single-Particle Lagrangian
Integrated Trajectory) model access via NOAA ARL READY website, available at:
http://www.arl.noaa.gov/ready/hysplit4.html (last access: October
2017), NOAA Air Resources Laboratory, Silver Spring, Md, 2003.
Ebinghaus, R., Kock, H., Coggins, A., Spain, T., Jennings, S., and,
Temme, C.: Long-term measurements of atmospheric mercury at Mace Head, Irish
west coast, between 1995 and 2001, Atmos. Environ., 36, 5267–5276,
2002.
Feng, X., Shang, L., Wang, S., Tang, S., and Zheng, W.: Temporal variation of
total gaseous mercury in the air of Guiyang, China, J. Geophys. Res., 109,
D03303, https://doi.org/10.1029/2003JD004159, 2004.
Fu, X., Feng, X., Zhu, W., Wang, S., and Lu, J.: Total gaseous mercury
concentrations in ambient air in the eastern slope of Mt. Gongga,
South-Eastern fringe of the Tibetan plateau, China, Atmos. Environ.,
42, 970–979, 2008.
Fu, X., Feng, X., Wang, S., Rothenberg, S., Shang, L., Li, Z., and Qiu, G.:
Temporal and spatial distributions of total gaseous mercury concentrations
in ambient air in a mountainous area in southwestern China: Implications for
industrial and domestic mercury emissions in remote areas in China, Sci.
Total Environ., 407, 2306–2314, 2009.
Fu, X. W., Feng, X., Dong, Z. Q., Yin, R. S., Wang, J. X., Yang, Z. R., and
Zhang, H.: Atmospheric gaseous elemental mercury (GEM) concentrations and
mercury depositions at a high-altitude mountain peak in south China, Atmos.
Chem. Phys., 10, 2425–2437, https://doi.org/10.5194/acp-10-2425-2010, 2010.
Fu, X., Feng, X., Qiu, G., Shang, L., and Zhang, H.: Speciated atmospheric
mercury and its potential source in Guiyang, China, Atmos. Environ.,
45, 4205–4212, 2011.
Fu, X. W., Feng, X., Liang, P., Deliger, Zhang, H., Ji, J., and Liu, P.:
Temporal trend and sources of speciated atmospheric mercury at Waliguan GAW
station, Northwestern China, Atmos. Chem. Phys., 12, 1951–1964,
https://doi.org/10.5194/acp-12-1951-2012, 2012a.
Fu, X. W., Feng, X., Shang, L. H., Wang, S. F., and Zhang, H.: Two years of
measurements of atmospheric total gaseous mercury (TGM) at a remote site in
Mt. Changbai area, Northeastern China, Atmos. Chem. Phys., 12, 4215–4226,
https://doi.org/10.5194/acp-12-4215-2012, 2012b.
Fu, X. W., Zhang, H., Yu, B., Wang, X., Lin, C.-J., and Feng, X. B.:
Observations of atmospheric mercury in China: a critical review, Atmos. Chem.
Phys., 15, 9455–9476, https://doi.org/10.5194/acp-15-9455-2015, 2015.
Fu, X., Marusczak, N., Heimbürger, L.-E., Sauvage, B., Gheusi, F., Prestbo,
E. M., and Sonke, J. E.: Atmospheric mercury speciation dynamics at the
high-altitude Pic du Midi Observatory, southern France, Atmos. Chem. Phys.,
16, 5623–5639, https://doi.org/10.5194/acp-16-5623-2016, 2016a.
Fu, X., Zhu, W., Zhang, H., Sommar, J., Yu, B., Yang, X., Wang, X., Lin,
C.-J., and Feng, X.: Depletion of atmospheric gaseous elemental mercury by
plant uptake at Mt. Changbai, Northeast China, Atmos. Chem. Phys., 16,
12861–12873, https://doi.org/10.5194/acp-16-12861-2016, 2016b.
Gautam, R., Hsu, N. C., Tsay, S. C., Lau, K. M., Holben, B., Bell, S.,
Smirnov, A., Li, C., Hansell, R., Ji, Q., Payra, S., Aryal, D., Kayastha, R.,
and Kim, K. M.: Accumulation of aerosols over the Indo-Gangetic plains and
southern slopes of the Himalayas: distribution, properties and radiative
effects during the 2009 pre-monsoon season, Atmos. Chem. Phys., 11,
12841–12863, https://doi.org/10.5194/acp-11-12841-2011, 2011.
Giglio, L., Descloitres, J., Justice, C. O., and Kaufman, Y. J.: An enhanced
contextual fire detection algorithm for MODIS, Remote Sens. Environ., 87,
273–282, 2003.
Goodsite, M. E., Plane, J., and Skov, H.: A theoretical study of the
oxidation of Hg0 to HgBr2 in the troposphere, Environ.
Sci. Technol., 38, 1772–1776, 2004.
Gou, P., Ye, Q., and Wei, Q.: Lake ice change at the Nam Co Lake on the
Tibetan Plateau during 2000–2013 and influencing factors, Progress in
Geography, 34, 1241–1249, 2015 (in Chinese with English abstract).
Gratz, L., Esposito, G., Dalla Torre, S., Cofone, F., Pirrone, N., and
Sprovieri, F.: First Measurements of Ambient Total Gaseous Mercury (TGM) at
the EvK2CNR Pyramid Observatory in Nepal, E3S Web of Conferences, 2013.
Holmes, C. D., Jacob, D. J., Corbitt, E. S., Mao, J., Yang, X., Talbot, R.,
and Slemr, F.: Global atmospheric model for mercury including oxidation by
bromine atoms, Atmos. Chem. Phys., 10, 12037–12057,
https://doi.org/10.5194/acp-10-12037-2010, 2010.
Horowitz, H. M., Jacob, D. J., Zhang, Y., Dibble, T. S., Slemr, F., Amos, H.
M., Schmidt, J. A., Corbitt, E. S., Marais, E. A., and Sunderland, E. M.: A
new mechanism for atmospheric mercury redox chemistry: implications for the
global mercury budget, Atmos. Chem. Phys., 17, 6353–6371,
https://doi.org/10.5194/acp-17-6353-2017, 2017.
Howard, D. and Edwards, G. C.: Mercury fluxes over an Australian alpine
grassland and observation of nocturnal atmospheric mercury depletion events,
Atmos. Chem. Phys., 18, 129–142, https://doi.org/10.5194/acp-18-129-2018, 2018.
Huang, J., Kang, S., Zhang, Q., Yan, H., Guo, J., Jenkins, M. G., Zhang, G.,
and Wang, K.: Wet deposition of mercury at a remote site in the Tibetan
Plateau: concentrations, speciation, and fluxes, Atmos. Environ.,
62, 540–550, 2012.
Huang, J., Kang, S., Wang, S., Wang, L., Zhang, Q., Guo, J., Wang, K.,
Zhang, G., and Tripathee, L.: Wet deposition of mercury at Lhasa, the
capital city of Tibet, Sci. Total Environ., 447, 123–132, 2013.
Huang, J., Kang, S., Guo, J., Zhang, Q., Cong, Z., Sillanpää, M.,
Zhang, G., Sun, S., and Tripathee, L.: Atmospheric particulate mercury in
Lhasa city, Tibetan Plateau, Atmos. Environ., 142, 433–441, 2016.
Kang, S., Yang, Y., and Zhu, L.: Modern Environmental Process and Changes in
the Basin of Nam Co in Tibetan Plateau, China Meteorological Press, Beijing,
2011 (in Chinese with English abstract).
Kang, S., Huang, J., Wang, F., Zhang, Q., Zhang, Y., Li, C., Wang, L., Chen,
P., Sharma, C. M., and Li, Q.: Atmospheric mercury depositional chronology
reconstructed from lake sediments and ice core in the Himalayas and Tibetan
Plateau, Environm. Sci. Technol., 50, 2859–2869, 2016.
Karunasagar, D., Krishna, M. B., Anjaneyulu, Y. A., and Arunachalam, J.:
Studies of mercury pollution in a lake due to a thermometer factory situated
in a tourist resort: Kodaikkanal, India, Environ. Pollut., 143,
153–158, 2006.
Kim, S. Y.: Continental outflow of polluted air from the US to the North
Atlantic and mercury chemical cycling in various atmospheric environments,
University of New Hampshire (Natural Resources and Earth Systems Science
Program), 2010.
Kock, H., Bieber, E., Ebinghaus, R., Spain, T., and Thees, B.: Comparison of
long-term trends and seasonal variations of atmospheric mercury
concentrations at the two European coastal monitoring stations Mace Head,
Ireland, and Zingst, Germany, Atmos. Environ., 39, 7549–7556, 2005.
Lan, X., Talbot, R., Castro, M., Perry, K., and Luke, W.: Seasonal and
diurnal variations of atmospheric mercury across the US determined from AMNet
monitoring data, Atmos. Chem. Phys., 12, 10569–10582,
https://doi.org/10.5194/acp-12-10569-2012, 2012.
Landis, M. S., Stevens, R. K., Schaedlich, F., and Prestbo, E. M.:
Development and characterization of an annular denuder methodology for the
measurement of divalent inorganic reactive gaseous mercury in ambient air,
Environ. Sci. Technol., 36, 3000–3009, 2002.
Larsen, L., Thomas, C., Eppinga, M., and Coulthard, T.: Exploratory
modeling: Extracting causality from complexity, Eos, Trans. Am.
Geophys. Union, 95, 285–286, 2014.
Lee, D. S., Dollard, G. J., and Pepler, S.: Gas-phase mercury in the
atmosphere of the United Kingdom, Atmos. Environ., 32, 855–864, 1998.
Li, C., Kang, S., Zhang, Q., and Kaspari, S.: Major ionic composition of
precipitation in the Nam Co region, Central Tibetan Plateau, Atmos.
Res., 85, 351–360, 2007.
Li, C., Bosch, C., Kang, S., Andersson, A., Chen, P., Zhang, Q., Cong, Z.,
Chen, B., Qin, D., and Gustafsson, Ö.: Sources of black carbon to the
Himalayan-Tibetan Plateau glaciers, Nat. Commun., 7, 12574, 2016.
Li, Z., Xia, C., Wang, X., Xiang, Y., and Xie, Z.: Total gaseous mercury in
Pearl River Delta region, China during 2008 winter period, Atmos.
Environ., 45, 834–838, 2011.
Lin, C.-J. and Pehkonen, S. O.: The chemistry of atmospheric mercury: a
review, Atmos. Environ., 33, 2067–2079, 1999.
Lindberg, S. A. and Stratton, W.: Atmospheric mercury speciation:
concentrations and behavior of reactive gaseous mercury in ambient air,
Environ. Sci. Technol., 32, 49–57, 1998.
Liu, M., Chen, L., Xie, D., Sun, J., He, Q., Cai, L., Gao, Z., and Zhang,
Y.: Monsoon-driven transport of atmospheric mercury to the South China Sea
from the Chinese mainland and Southeast Asia – Observation of gaseous
elemental mercury at a background station in South China, Environ.
Sci. Pollut. Res., 23, 21631–21640, 2016.
Liu, N., Qiu, G., Landis, M. S., Feng, X., Fu, X., and Shang, L.:
Atmospheric mercury species measured in Guiyang, Guizhou province, southwest
China, Atmos. Res., 100, 93–102, 2011.
Liu, Y. W., Xu-Ri, Wang, Y. S., Pan, Y. P., and Piao, S. L.: Wet deposition
of atmospheric inorganic nitrogen at five remote sites in the Tibetan
Plateau, Atmos. Chem. Phys., 15, 11683–11700,
https://doi.org/10.5194/acp-15-11683-2015, 2015.
Ma, Y., Kang, S., Zhu, L., Xu, B., Tian, L., and Yao, T.: ROOF OF THE WORLD:
Tibetan observation and research platform: atmosphere-land interaction over
a heterogeneous landscape, B. Am. Meteorol. Soc.,
89, 1487–1492, 2008.
Mallik, C. and Lal, S.: Seasonal characteristics of SO2, NO2, and CO
emissions in and around the Indo-Gangetic Plain, Environ. Monit.
Assess., 186, 1295–1310, 2014.
Mukherjee, A. B., Bhattacharya, P., Sarkar, A., and Zevenhoven, R.: Mercury
emissions from industrial sources in India and its effects in the
environment, in: Mercury Fate and Transport in the Global Atmosphere,
Springer, 81–112, 2009.
Müller, D., Wip, D., Warneke, T., Holmes, C. D., Dastoor, A., and
Notholt, J.: Sources of atmospheric mercury in the tropics: continuous
observations at a coastal site in Suriname, Atmos. Chem. Phys.,
12, 7391–7397, https://doi.org/10.5194/acp-12-7391-2012, 2012.
Obrist, D., Tas, E., Peleg, M., Matveev, V., Faïn, X., Asaf, D., and
Luria, M.: Bromine-induced oxidation of mercury in the mid-latitude
atmosphere, Nat.e Geosci., 4, 22–26, 2011.
Pacyna, E. G., Pacyna, J., Sundseth, K., Munthe, J., Kindbom, K., Wilson,
S., Steenhuisen, F., and Maxson, P.: Global emission of mercury to the
atmosphere from anthropogenic sources in 2005 and projections to 2020,
Atmos. Environ., 44, 2487–2499, 2010.
Parvathi, K., Jayaprakash, K., and Sivakumar, N.: Mercury contamination due
to thermometer glass solid waste dumping-a preliminary report, Asian J. Exp.
Chem., 5, 46–48, 2010.
Peterson, C., Gustin, M., and Lyman, S.: Atmospheric mercury concentrations
and speciation measured from 2004 to 2007 in Reno, Nevada, USA, Atmos.
Environ., 43, 4646–4654, 2009.
Pirrone, N., Cinnirella, S., Feng, X., Finkelman, R. B., Friedli, H. R.,
Leaner, J., Mason, R., Mukherjee, A. B., Stracher, G. B., Streets, D. G., and
Telmer, K.: Global mercury emissions to the atmosphere from anthropogenic and
natural sources, Atmos. Chem. Phys., 10, 5951–5964,
https://doi.org/10.5194/acp-10-5951-2010, 2010.
Polissar, A., Hopke, P., Paatero, P., Kaufmann, Y., Hall, D., Bodhaine, B.,
Dutton, E., and Harris, J.: The aerosol at Barrow, Alaska: long-term trends
and source locations, Atmos. Environ., 33, 2441–2458, 1999.
Rao, S., Zurbenko, I., Neagu, R., Porter, P., Ku, J., and Henry, R.: Space
and time scales in ambient ozone data, B. Am. Meteorol. Soc., 78, 2153–2166,
1997.
Schroeder, W. H. and Munthe, J.: Atmospheric mercury – an overview, Atmos.
Environ., 32, 809–822, 1998.
Selin, H.: Global environmental law and treaty-making on hazardous
substances: the Minamata Convention and mercury abatement, Global
Environ. Polit., 14, 1–19, 2014.
Sheng, J., Wang, X., Gong, P., Joswiak, D. R., Tian, L., Yao, T., and Jones,
K. C.: Monsoon-driven transport of organochlorine pesticides and
polychlorinated biphenyls to the Tibetan Plateau: three year atmospheric
monitoring study, Environ. Sci. Technol., 47, 3199–3208,
2013.
Shia, R. L., Seigneur, C., Pai, P., Ko, M., and Sze, N. D.: Global
simulation of atmospheric mercury concentrations and deposition fluxes,
J. Geophys. Res.-Atmos., 104, 23747–23760, 1999.
Sigler, J. M., Mao, H., and Talbot, R.: Gaseous elemental and reactive
mercury in Southern New Hampshire, Atmos. Chem. Phys., 9, 1929–1942,
https://doi.org/10.5194/acp-9-1929-2009, 2009.
Slemr, F., Brunke, E.-G., Ebinghaus, R., and Kuss, J.: Worldwide trend of
atmospheric mercury since 1995, Atmos. Chem. Phys., 11, 4779–4787,
https://doi.org/10.5194/acp-11-4779-2011, 2011.
Slemr, F., Brunke, E. G., Labuschagne, C., and Ebinghaus, R.: Total gaseous
mercury concentrations at the Cape Point GAW station and their seasonality,
Geophys. Res. Lett., 35, L11807, https://doi.org/10.1029/2008GL033741, 2008.
Sprovieri, F., Pirrone, N., Bencardino, M., D'Amore, F., Carbone, F.,
Cinnirella, S., Mannarino, V., Landis, M., Ebinghaus, R., Weigelt, A.,
Brunke, E.-G., Labuschagne, C., Martin, L., Munthe, J., Wängberg, I.,
Artaxo, P., Morais, F., Barbosa, H. D. M. J., Brito, J., Cairns, W.,
Barbante, C., Diéguez, M. D. C., Garcia, P. E., Dommergue, A., Angot, H.,
Magand, O., Skov, H., Horvat, M., Kotnik, J., Read, K. A., Neves, L. M.,
Gawlik, B. M., Sena, F., Mashyanov, N., Obolkin, V., Wip, D., Feng, X. B.,
Zhang, H., Fu, X., Ramachandran, R., Cossa, D., Knoery, J., Marusczak, N.,
Nerentorp, M., and Norstrom, C.: Atmospheric mercury concentrations observed
at ground-based monitoring sites globally distributed in the framework of the
GMOS network, Atmos. Chem. Phys., 16, 11915–11935,
https://doi.org/10.5194/acp-16-11915-2016, 2016.
Stamenkovic, J., Lyman, S., and Gustin, M. S.: Seasonal and diel variation of
atmospheric mercury concentrations in the Reno (Nevada, USA) airshed, Atmos.
Environ., 41, 6662–6672, 2007.
Streets, D. G., Hao, J., Wu, Y., Jiang, J., Chan, M., Tian, H., and Feng, X.:
Anthropogenic mercury emissions in China, Atmos. Environ., 39, 7789–7806,
2005.
Subramanian, V.: Water quality in south Asia, Asian journal of water,
Environ. Pollut., 1, 41–54, 2004.
Sun, X., Wang, K., Kang, S., Guo, J., Zhang, G., Huang, J., Cong, Z., Sun,
S., and Zhang, Q.: The role of melting alpine glaciers in mercury export and
transport: An intensive sampling campaign in the Qugaqie Basin, inland
Tibetan Plateau, Environ. Pollut., 220, 936–945, 2017.
Sun, X., Zhang, Q., Kang, S., Guo, J., Li, X., Yu, Z., Zhang, G., Qu, D.,
Huang, J., and Cong, Z.: Mercury speciation and distribution in a
glacierized mountain environment and their relevance to environmental risks
in the inland Tibetan Plateau, Sci. Total Environ., 631,
270–278, 2018.
Tong, Y., Yin, X., Lin, H., Wang, H., Deng, C., Chen, L., Li, J., Zhang, W.,
Schauer, J. J., and Kang, S.: Recent Decline of Atmospheric Mercury Recorded
by Androsace tapete on the Tibetan Plateau, Environ. Sci.
Technol., 50, 13224–13231, 2016.
Wan, Q., Feng, X., Lu, J., Zheng, W., Song, X., Han, S., and Xu, H.:
Atmospheric mercury in Changbai Mountain area, northeastern China I. The
seasonal distribution pattern of total gaseous mercury and its potential
sources, Environ. Res., 109, 201–206, 2009.
Wan, X., Kang, S., Wang, Y., Xin, J., Liu, B., Guo, Y., Wen, T., Zhang, G.,
and Cong, Z.: Size distribution of carbonaceous aerosols at a high-altitude
site on the central Tibetan Plateau (Nam Co Station, 4730 m asl),
Atmos. Res., 153, 155–164, 2015.
Wang, B. and Fan, Z.: Choice of South Asian summer monsoon indices,
B. Am. Meteorol. Soc., 80, 629–638, 1999.
Wang, B., Wu, R., and Lau, K.: Interannual variability of the Asian summer
monsoon: Contrasts between the Indian and the western North Pacific–East
Asian monsoons, J. Climate, 14, 4073–4090, 2001.
Wang, Y., Zhang, X., and Draxler, R. R.: TrajStat: GIS-based software that
uses various trajectory statistical analysis methods to identify potential
sources from long-term air pollution measurement data, Environ.
Modell. Softw., 24, 938–939, 2009.
Wang, Y.: MeteoInfo: GIS software for meteorological data visualization and
analysis, Meteorol. Appl., 21, 360–368, 2014.
Wang, Y., Zhang, Y., Schauer, J. J., de Foy, B., Guo, B., and Zhang, Y.:
Relative impact of emissions controls and meteorology on air pollution
mitigation associated with the Asia-Pacific Economic Cooperation (APEC)
conference in Beijing, China, Sci. Total Environ., 571,
1467–1476, 2016.
Wang, Y., de Foy, B., Schauer, J. J., Olson, M. R., Zhang, Y., Li, Z., and
Zhang, Y.: Impacts of regional transport on black carbon in Huairou,
Beijing, China, Environ. Pollut., 221, 75–84, 2017.
Weiss-Penzias, P., Jaffe, D. A., McClintick, A., Prestbo, E. M., and Landis,
M. S.: Gaseous elemental mercury in the marine boundary layer: Evidence for
rapid removal in anthropogenic pollution, Environ. Sci.
Technol., 37, 3755–3763, 2003.
Wu, Q., Wang, S., Li, G., Liang, S., Lin, C.-J., Wang, Y., Cai, S., Liu, K.,
and Hao, J.: Temporal Trend and Spatial Distribution of Speciated
Atmospheric Mercury Emissions in China During 1978–2014, Environ.
Sci. Technol., 50, 13428–13435, 2016.
Wu, Q., Gao, W., Wang, S., and Hao, J.: Updated atmospheric speciated mercury
emissions from iron and steel production in China during 2000–2015, Atmos.
Chem. Phys., 17, 10423–10433, https://doi.org/10.5194/acp-17-10423-2017,
2017.
Xia, X., Zong, X., Cong, Z., Chen, H., Kang, S., and Wang, P.: Baseline
continental aerosol over the central Tibetan plateau and a case study of
aerosol transport from South Asia, Atmos. Environ., 45, 7370–7378,
2011.
Xiao, H., Shen, L., Su, Y., Barresi, E., DeJong, M., Hung, H., Lei, Y.-D.,
Wania, F., Reiner, E. J., and Sverko, E.: Atmospheric concentrations of
halogenated flame retardants at two remote locations: The Canadian High
Arctic and the Tibetan Plateau, Environ. Pollut., 161, 154–161, 2012.
Xiu, G., Cai, J., Zhang, W., Zhang, D., Büeler, A., Lee, S., Shen, Y.,
Xu, L., Huang, X., and Zhang, P.: Speciated mercury in size-fractionated
particles in Shanghai ambient air, Atmos. Environ., 43, 3145–3154,
2009.
Xu, L., Chen, J., Yang, L., Niu, Z., Tong, L., Yin, L., and Chen, Y.:
Characteristics and sources of atmospheric mercury speciation in a coastal
city, Xiamen, China, Chemosphere, 119, 530–539, 2015.
Yang, H., Battarbee, R. W., Turner, S. D., Rose, N. L., Derwent, R. G., Wu,
G., and Yang, R.: Historical reconstruction of mercury pollution across the
Tibetan Plateau using lake sediments, Environ. Sci. Technol.,
44, 2918–2924, 2010.
Yatavelli, R. L., Fahrni, J. K., Kim, M., Crist, K. C., Vickers, C. D.,
Winter, S. E., and Connell, D. P.: Mercury, PM 2.5 and gaseous co-pollutants
in the Ohio River Valley region: Preliminary results from the Athens
supersite, Atmos. Environ., 40, 6650–6665, 2006.
Yin, X., Kang, S., de Foy, B., Cong, Z., Luo, J., Zhang, L., Ma, Y., Zhang,
G., Rupakheti, D., and Zhang, Q.: Surface ozone at Nam Co in the inland
Tibetan Plateau: variation, synthesis comparison and regional
representativeness, Atmos. Chem. Phys., 17, 11293–11311,
https://doi.org/10.5194/acp-17-11293-2017, 2017.
You, Q., Kang, S., Li, C., Li, M., and Liu, J.: Variation features of
meteorological elements at Namco Station, Tibetan Plateau, Meteorol.
Monthly, 33, 54–60, 2007.
Yu, B., Wang, X., Lin, C. J., Fu, X., Zhang, H., Shang, L., and Feng, X.:
Characteristics and potential sources of atmospheric mercury at a
subtropical near – coastal site in East China, J. Geophys.
Res.-Atmos., 120, 8563–8574, 2015.
Zhang, L., Wang, S. X., Wang, L., and Hao, J. M.: Atmospheric mercury
concentration and chemical speciation at a rural site in Beijing, China:
implications of mercury emission sources, Atmos. Chem. Phys., 13,
10505–10516, https://doi.org/10.5194/acp-13-10505-2013, 2013.
Zhang, H., Fu, X. W., Lin, C.-J., Wang, X., and Feng, X. B.: Observation and
analysis of speciated atmospheric mercury in Shangri-La, Tibetan Plateau,
China, Atmos. Chem. Phys., 15, 653–665,
https://doi.org/10.5194/acp-15-653-2015, 2015.
Zhang, X., Ming, J., Li, Z., Wang, F., and Zhang, G.: The online measured
black carbon aerosol and source orientations in the Nam Co region, Tibet,
Environ. Sci. Pollut. Res., 24, 25021–25033, 2017.
Zhang, Y., Jacob, D. J., Horowitz, H. M., Chen, L., Amos, H. M., Krabbenhoft,
D. P., Slemr, F., Louis, V. L. S., and Sunderland, E. M.: Observed decrease
in atmospheric mercury explained by global decline in anthropogenic
emissions, P. Natl. Acad. Sci. USA, 113, 526–531, 2016.
Short summary
Total gaseous mercury concentrations were measured at Nam Co Station on the inland Tibetan Plateau for ~ 3 years. The mean concentration of TGM during the entire monitoring period was 1.33 ± 0.24 ngm-3, ranking it the lowest in China and indicating the pristine atmospheric environment of the inland Tibetan Plateau. Variation of TGM at Nam Co was affected by regional surface reemission, vertical mixing and long-range transported atmospheric mercury, which was associated with the Indian monsoon.
Total gaseous mercury concentrations were measured at Nam Co Station on the inland Tibetan...
Altmetrics
Final-revised paper
Preprint