Articles | Volume 17, issue 22
https://doi.org/10.5194/acp-17-13721-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-13721-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Aerosol emissions factors from traditional biomass cookstoves in India: insights from field measurements
Center for Aerosol Science and Engineering, Department of Energy,
Environmental and Chemical Engineering, Washington University in St. Louis,
St. Louis, MO 63130, USA
Sameer Patel
Center for Aerosol Science and Engineering, Department of Energy,
Environmental and Chemical Engineering, Washington University in St. Louis,
St. Louis, MO 63130, USA
Shamsh Pervez
School of Studies in Chemistry, Pandit Ravishankar Shukla
University, Raipur, Chhattisgarh 492010, India
Suresh Tiwari
Indian Institute of
Tropical Meteorology, Pune, Maharashtra 411008, India
Gautam Yadama
Brown School
of Social Work, Washington University in St. Louis, St. Louis, MO 63130, USA
now at: School of Social Work, Boston College,
Boston, MA 02467, USA
Judith C. Chow
Division of Atmospheric Sciences, Desert Research Institute, Reno,
NV 89512, USA
John G. Watson
Division of Atmospheric Sciences, Desert Research Institute, Reno,
NV 89512, USA
Pratim Biswas
Center for Aerosol Science and Engineering, Department of Energy,
Environmental and Chemical Engineering, Washington University in St. Louis,
St. Louis, MO 63130, USA
Rajan K. Chakrabarty
CORRESPONDING AUTHOR
Center for Aerosol Science and Engineering, Department of Energy,
Environmental and Chemical Engineering, Washington University in St. Louis,
St. Louis, MO 63130, USA
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Our study delves into the elemental composition of aerosols at three sites across the Indo-Gangetic Plain (IGP), revealing distinct patterns during pollution episodes. We found significant increases in chlorine (Cl)-rich and solid fuel combustion (SFC) sources, indicating dynamic emission sources, agricultural burning impacts, and meteorological influences. Surges in Cl-rich particles during cold periods highlight their role in particle growth under high-relative-humidity conditions.
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Brown carbon (BrC) aerosols show an order-of-magnitude variation in their light absorption strength. Our understanding of BrC from real-world biomass burning remains limited, complicating the determination of its radiative impact. Our study reports absorption properties of BrC emitted from four major biomass burning sources using field measurements in India. It develops an absorption parameterization for BrC and examines the spatial variability in BrC's absorption strength across India.
Xiaoliang Wang, Hatef Firouzkouhi, Judith C. Chow, John G. Watson, Steven Sai Hang Ho, Warren Carter, and Alexandra S. M. De Vos
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Xiaoliang Wang, Hatef Firouzkouhi, Judith C. Chow, John G. Watson, Warren Carter, and Alexandra S. M. De Vos
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Payton Beeler and Rajan K. Chakrabarty
Atmos. Chem. Phys., 22, 14825–14836, https://doi.org/10.5194/acp-22-14825-2022, https://doi.org/10.5194/acp-22-14825-2022, 2022
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Jie Luo, Zhengqiang Li, Chenchong Zhang, Qixing Zhang, Yongming Zhang, Ying Zhang, Gabriele Curci, and Rajan K. Chakrabarty
Atmos. Chem. Phys., 22, 7647–7666, https://doi.org/10.5194/acp-22-7647-2022, https://doi.org/10.5194/acp-22-7647-2022, 2022
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The fractal black carbon was applied to re-evaluate the regional impacts of morphologies on aerosol–radiation interactions (ARIs), and the effects were compared between the US and China. The regional-mean clear-sky ARI is significantly affected by the BC morphology, and relative differences of 17.1 % and 38.7 % between the fractal model with a Df of 1.8 and the spherical model were observed in eastern China and the northwest US, respectively.
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Looking at characteristics and δ13C compositions of dicarboxylic acids and related compounds in BB aerosols, we used a combined combustion and aging system to generate fresh and aged aerosols from burning straw. The results showed the emission factors (EFaged) of total diacids of aging experiments were around an order of magnitude higher than EFfresh. This meant that dicarboxylic acids are involved with secondary photochemical processes in the atmosphere rather than primary emissions from BB.
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We present a comparison of the changes to light absorption behavior and chemical composition of wildfire smoke particles from day- and nighttime oxidation processes and discuss the results within the context of previous laboratory findings.
Cited articles
Andreae, M. O. and Gelencsér, A.: Black carbon or brown carbon? The nature of light-absorbing carbonaceous aerosols, Atmos. Chem. Phys., 6, 3131–3148, https://doi.org/10.5194/acp-6-3131-2006, 2006.
Bond, T. C., Streets, D. G., Yarber, K. F., Nelson, S. M., Woo, J. H., and Klimont, Z.: A technology-based global inventory of black and organic carbon emissions from combustion, J. Geophys. Res.-Atmos., 109, https://doi.org/10.1029/2003JD003697, 2004.
Bond, T. C., Doherty, S. J., Fahey, D., Forster, P., Berntsen, T., DeAngelo, B., Flanner, M., Ghan, S., Kärcher, B., and Koch, D.: Bounding the role of black carbon in the climate system: A scientific assessment, J. Geophys. Res.-Atmos., 118, 5380–5552, 2013.
Census: Houselisting and Housing Census Data, New Delhi, 2011, Office of the Registrar General & Census Commissioner, India Ministry of Home Affairs, Government of India, available at: http://censusindia.gov.in/2011census/hlo/Houselisting_Housing_Tables.html (last access: 11 August 2017), 2011.
Chow, J. C., Watson, J. G., Lowenthal, D. H., Chen, L. W. A., Zielinska, B., Mazzoleni, L. R., and Magliano, K. L.: Evaluation of organic markers for chemical mass balance source apportionment at the Fresno Supersite, Atmos. Chem. Phys., 7, 1741–1754, https://doi.org/10.5194/acp-7-1741-2007, 2007a.
Chow, J. C., Watson, J. G., Chen, L.-W. A., Chang, M. O., Robinson, N. F., Trimble, D., and Kohl, S.: The IMPROVE_A temperature protocol for thermal/optical carbon analysis: maintaining consistency with a long-term database, J. Air Waste Ma., 57, 1014–1023, 2007b.
Chow, J. C., Watson, J. G., Robles, J., Wang, X. L., Chen, L.-W. A., Trimble, D. L., Kohl, S. D., Tropp, R. J., and Fung, K. K.: Quality assurance and quality control for thermal/optical analysis of aerosol samples for organic and elemental carbon, Anal. Bioanal. Chem., 401, 3141–3152, https://doi.org/10.1007/s00216-011-5103-3, 2011.
Chung, S. H. and Seinfeld, J. H.: Climate response of direct radiative forcing of anthropogenic black carbon, J. Geophys. Res.-Atmos., 110, https://doi.org/10.1029/2004JD005441, 2005.
CPCB: Air quality monitoring, emission inventory and source apportionment study for Indian cities, National Summary Report, Central Pollution Control Board, 2011.
Grieshop, A. P., Marshall, J. D., and Kandlikar, M.: Health and climate benefits of cookstove replacement options, Energ. Policy, 39, 7530–7542, 2011.
Guttikunda, S. K. and Calori, G.: A GIS based emissions inventory at 1 km × 1 km spatial resolution for air pollution analysis in Delhi, India, Atmos. Environ., 67, 101–111, 2013.
Habib, G., Venkataraman, C., Bond, T. C., and Schauer, J. J.: Chemical, microphysical and optical properties of primary particles from the combustion of biomass fuels, Environ. Sci. Technol., 42, 8829–8834, 2008.
Kambezidis, H., Kaskaoutis, D., Kharol, S. K., Moorthy, K. K., Satheesh, S., Kalapureddy, M., Badarinath, K., Sharma, A. R., and Wild, M.: Multi-decadal variation of the net downward shortwave radiation over south Asia: The solar dimming effect, Atmos. Environ., 50, 360–372, 2012.
Kar, A., Rehman, I. H., Burney, J., Puppala, S. P., Suresh, R., Singh, L., Singh, V. K., Ahmed, T., Ramanathan, N., and Ramanathan, V.: Real-time assessment of black carbon pollution in Indian households due to traditional and improved biomass cookstoves, Environ. Sci. Technol., 46, 2993–3000, 2012.
Kulkarni, P., Qi, C. L., and Fukushima, N.: Development of portable aerosol mobility spectrometer for personal and mobile aerosol measurement, Aerosol Sci. Technol., 50, 1167–1179, https://doi.org/10.1080/02786826.2016.1230662, 2016.
Leavey, A., Londeree, J., Priyadarshini, P., Puppala, J., Schechtman, K. B., Yadama, G., and Biswas, P.: Real-time particulate and CO concentrations from cookstoves in rural households in Udaipur, India, Environ. Sci. Technol., 49, 7423–7431, 2015.
MacCarty, N., Ogle, D., Still, D., Bond, T., and Roden, C.: A laboratory comparison of the global warming impact of five major types of biomass cooking stoves, Energy Sustain. Dev., 12, 56–65, 2008.
Menon, S., Hansen, J., Nazarenko, L., and Luo, Y.: Climate effects of black carbon aerosols in China and India, Science, 297, 2250–2253, 2002.
MHFW, N. D.: Report of the Steering Committee on Air Pollution and Health-Related Issues., Ministry of Health and Family Welfare, Government of India, New Delhi, 2015.
Murray, C. J., Vos, T., Lozano, R., Naghavi, M., Flaxman, A. D., Michaud, C., Ezzati, M., Shibuya, K., Salomon, J. A., and Abdalla, S.: Disability-adjusted life years (DALYs) for 291 diseases and injuries in 21 regions, 1990–2010: a systematic analysis for the Global Burden of Disease Study 2010, The lancet, 380, 2197–2223, 2013.
O'Shaughnessy, P. T. and Slagley, J. M.: Photometer response determination based on aerosol physical characteristics, AIHA Journal, 63, 578–585, 2002.
Pandey, A., Sadavarte, P., Rao, A. B., and Venkataraman, C.: Trends in multi-pollutant emissions from a technology-linked inventory for India: II. Residential, agricultural and informal industry sectors, Atmos. Environ., 99, 341–352, 2014.
Pandey, A., Pervez, S., and Chakrabarty, R. K.: Filter-based measurements of UV–vis mass absorption cross sections of organic carbon aerosol from residential biomass combustion: Preliminary findings and sources of uncertainty, J. Quant. Spectrosc. Ra., 182, 296–304, 2016.
Patel, S., Li, J., Pandey, A., Pervez, S., Chakrabarty, R. K., and Biswas, P.: Spatio-temporal measurement of indoor particulate matter concentrations using a wireless network of low-cost sensors in households using solid fuels, Environ. Res., 152, 59–65, 2017.
Pope, C. A. and Dockery, D. W.: Health effects of fine particulate air pollution: lines that connect, J. Air Waste Ma., 56, 709–742, 2006.
Pope, C. A., Burnett, R. T., Krewski, D., Jerrett, M., Shi, Y., Calle, E. E., and Thun, M. J.: Cardiovascular mortality and exposure to airborne fine particulate matter and cigarette smoke, Circulation, 120, 941–948, 2009.
Ramanathan, V., Crutzen, P., Kiehl, J., and Rosenfeld, D.: Aerosols, climate, and the hydrological cycle, Science, 294, 2119–2124, 2001.
Ramanathan, V., Chung, C., Kim, D., Bettge, T., Buja, L., Kiehl, J., Washington, W., Fu, Q., Sikka, D., and Wild, M.: Atmospheric brown clouds: Impacts on South Asian climate and hydrological cycle, P. Natl. Acad. Sci. USA, 102, 5326–5333, 2005.
Ramanathan, V., Ramana, M. V., Roberts, G., Kim, D., Corrigan, C., Chung, C., and Winker, D.: Warming trends in Asia amplified by brown cloud solar absorption, Nature, 448, 575–578, 2007.
Ramanathan, V. and Carmichael, G.: Global and regional climate changes due to black carbon, Nat. Geosci., 1, 221–227, 2008.
Reid, J. S., Koppmann, R., Eck, T. F., and Eleuterio, D. P.: A review of biomass burning emissions part II: intensive physical properties of biomass burning particles, Atmos. Chem. Phys., 5, 799–825, https://doi.org/10.5194/acp-5-799-2005, 2005.
Roden, C. A., Bond, T. C., Conway, S., and Pinel, A. B. O.: Emission factors and real-time optical properties of particles emitted from traditional wood burning cookstoves, Environ. Sci. Technol., 40, 6750–6757, 2006.
Roden, C. A., Bond, T. C., Conway, S., Pinel, A. B. O., MacCarty, N., and Still, D.: Laboratory and field investigations of particulate and carbon monoxide emissions from traditional and improved cookstoves, Atmos. Environ., 43, 1170–1181, 2009.
Sadavarte, P. and Venkataraman, C.: Trends in multi-pollutant emissions from a technology-linked inventory for India: I. Industry and transport sectors, Atmos. Environ., 99, 353–364, 2014.
Sadavarte, P., Venkataraman, C., Cherian, R., Patil, N., Madhavan, B., Gupta, T., Kulkarni, S., Carmichael, G., and Adhikary, B.: Seasonal differences in aerosol abundance and radiative forcing in months of contrasting emissions and rainfall over northern South Asia, Atmos. Environ., 125, 512–523, 2016.
Sagar, A., Balakrishnan, K., Guttikunda, S., Roychowdhury, A., and Smith, K. R.: India leads the way: a health-centered strategy for air pollution, Environ. Health Perspect., 124, A116–A117, 2016.
Sahu, M., Peipert, J., Singhal, V., Yadama, G. N., and Biswas, P.: Evaluation of mass and surface area concentration of particle emissions and development of emissions indices for cookstoves in rural India, Environ. Sci. Technol., 45, 2428–2434, 2011.
Saleh, R., Hennigan, C. J., McMeeking, G. R., Chuang, W. K., Robinson, E. S., Coe, H., Donahue, N. M., and Robinson, A. L.: Absorptivity of brown carbon in fresh and photo-chemically aged biomass-burning emissions, Atmos. Chem. Phys., 13, 7683–7693, https://doi.org/10.5194/acp-13-7683-2013, 2013.
Saud, T., Gautam, R., Mandal, T., Gadi, R., Singh, D., Sharma, S., Dahiya, M., and Saxena, M.: Emission estimates of organic and elemental carbon from household biomass fuel used over the Indo-Gangetic Plain (IGP), India, Atmos. Environ., 61, 212–220, 2012.
Schulz, M., Textor, C., Kinne, S., Balkanski, Y., Bauer, S., Berntsen, T., Berglen, T., Boucher, O., Dentener, F., Guibert, S., Isaksen, I. S. A., Iversen, T., Koch, D., Kirkevåg, A., Liu, X., Montanaro, V., Myhre, G., Penner, J. E., Pitari, G., Reddy, S., Seland, Ø., Stier, P., and Takemura, T.: Radiative forcing by aerosols as derived from the AeroCom present-day and pre-industrial simulations, Atmos. Chem. Phys., 6, 5225–5246, https://doi.org/10.5194/acp-6-5225-2006, 2006.
Shindell, D., Kuylenstierna, J. C., Vignati, E., van Dingenen, R., Amann, M., Klimont, Z., Anenberg, S. C., Muller, N., Janssens-Maenhout, G., and Raes, F.: Simultaneously mitigating near-term climate change and improving human health and food security, Science, 335, 183–189, 2012.
Smith, K.: You don't get what you expect; you get what you inspect, Energy Sustain. Dev., 11, 3–4, 2007.
Smith, K. R., Uma, R., Kishore, V., Lata, K., Joshi, V., Zhang, J., Rasmussen, R., Khalil, M., and Thorneloe, S.: Greenhouse gases from small-scale combustion devices in developing countries, Phase IIa: Household Stoves in India, US Environmental Protection Agency, Research Triangle Park, NC, 98, 2000a.
Smith, K. R., Uma, R., Kishore, V. V. N., Lata, K., Joshi, V., Zhang, J., Rasmussen, R. A., and Khalil, M. A. K.: Greenhouse gases from small-scale combustion devices in developing countries: Phase IIA, Household stoves in India, US EPA, Washington DC, 89, 2000b.
Solomon, P. A., Crumpler, D., Flanagan, J. B., Jayanty, R., Rickman, E. E., and McDade, C. E.: US National PM2.5 chemical speciation monitoring networks—CSN and IMPROVE: description of networks, J. Air Waste Ma., 64, 1410–1438, 2014.
Venkataraman, C., Sagar, A., Habib, G., Lam, N., and Smith, K.: The Indian national initiative for advanced biomass cookstoves: the benefits of clean combustion, Energy Sustain. Dev., 14, 63–72, 2010.
Wang, X. L., Watson, J. G., Chow, J. C., Gronstal, S., and Kohl, S. D.: An efficient multipollutant system for measuring real-world emissions from stationary and mobile sources, Aerosol Air Qual. Res., 12, 145–160, 2012.
Zhang, H., Ye, X., Cheng, T., Chen, J., Yang, X., Wang, L., and Zhang, R.: A laboratory study of agricultural crop residue combustion in China: emission factors and emission inventory, Atmos. Environ., 42, 8432–8441, 2008.
Zhu, K., Zhang, J. F., and Lioy, P. J.: Evaluation and comparison of continuous fine particulate matter monitors for measurement of ambient aerosols, J. Air Waste Manage. Assoc., 57, 1499–1506, 2007.
Short summary
This study presents real-world aerosol mass emission factors for traditional biomass cookstoves in India to help constrain regional inventory emissions. Aerosol emissions were sampled from an in-use traditional mud stove burning common biomass fuel types in an Indian household. Measured particulate emission factors and their organic carbon content were higher than those from previous laboratory studies. Field emissions showed a distinct profile of temperature-resolved carbon mass fractions.
This study presents real-world aerosol mass emission factors for traditional biomass cookstoves...
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