Articles | Volume 16, issue 7
https://doi.org/10.5194/acp-16-4379-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-4379-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Developing and bounding ice particle mass- and area-dimension expressions for use in atmospheric models and remote sensing
Desert Research Institute, Reno, Nevada, USA
Graduate Program in Atmospheric Sciences, University of Nevada, Reno, Nevada, USA
David L. Mitchell
Desert Research Institute, Reno, Nevada, USA
Related authors
David L. Mitchell, Anne Garnier, Jacques Pelon, and Ehsan Erfani
Atmos. Chem. Phys., 18, 17325–17354, https://doi.org/10.5194/acp-18-17325-2018, https://doi.org/10.5194/acp-18-17325-2018, 2018
Short summary
Short summary
To realistically model a changing climate, global measurements of cirrus cloud ice-particle number concentration (N) and size (De) are needed, through which one may infer the general mechanism of ice formation. A satellite remote sensing method was developed to measure N and De. It was found that N was highest and De lowest at high latitudes. In the Arctic, cirrus clouds occurred much more often during winter, which may have an impact on mid-latitude winter weather.
Ehsan Erfani and David L. Mitchell
Atmos. Chem. Phys., 17, 1241–1257, https://doi.org/10.5194/acp-17-1241-2017, https://doi.org/10.5194/acp-17-1241-2017, 2017
Short summary
Short summary
Rimed particle projected area- and mass-dimension expressions are developed and validated.
A convenient means of relating the unrimed and rimed m – D and A – D expressions was developed.
Equations are provided to calculate collision efficiency for use in models.
David L. Mitchell, Anne Garnier, Melody Avery, and Ehsan Erfani
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-1062, https://doi.org/10.5194/acp-2016-1062, 2016
Revised manuscript not accepted
Short summary
Short summary
Although the main objective of our DOE/Atmospheric Systems Research project was to use aircraft measurements to determine the formation (i.e. ice nucleation) mechanism of cirrus clouds, it soon became evident that the formation mechanism will depend on latitude, season and surface topography. A new satellite remote sensing method was developed to discover this dependency, which shows that roughly half or more of the cirrus clouds at high latitudes form through homogeneous ice nucleation.
David L. Mitchell, Anne Emilie Garnier, and Sarah Woods
EGUsphere, https://doi.org/10.5194/egusphere-2024-3790, https://doi.org/10.5194/egusphere-2024-3790, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
Motivated by the need to better understand the physics of cirrus clouds, a satellite retrieval for cirrus cloud ice water content, ice particle number concentration and effective size was developed by exploiting relationships between cirrus cloud measurements made during field campaigns and cloud radiative properties measured by satellite. These retrievals tested favorably when compared against corresponding aircraft measurements and were found to depend on the visual opacity of the cloud.
David L. Mitchell and Anne Garnier
EGUsphere, https://doi.org/10.5194/egusphere-2024-3814, https://doi.org/10.5194/egusphere-2024-3814, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
Arguably the greatest knowledge gap in cirrus cloud research is the relative roles of homogeneous and heterogeneous ice nucleation in cirrus cloud formation. Since this depends on temperature, latitude, season, and topography, a satellite remote sensing method was developed to measure cirrus cloud properties. It was found that cirrus clouds strongly affected by homogeneous ice nucleation may account for over half of the overall cirrus cloud radiative effect during winter outside the tropics.
Anne Garnier, Jacques Pelon, Nicolas Pascal, Mark A. Vaughan, Philippe Dubuisson, Ping Yang, and David L. Mitchell
Atmos. Meas. Tech., 14, 3253–3276, https://doi.org/10.5194/amt-14-3253-2021, https://doi.org/10.5194/amt-14-3253-2021, 2021
Short summary
Short summary
The IIR Level 2 data products include cloud effective emissivities and cloud microphysical properties such as effective diameter (De) and ice or liquid water path estimates. This paper (Part I) describes the improvements in the V4 algorithms compared to those used in the version 3 (V3) release, while results are presented in a companion paper (Part II).
Anne Garnier, Jacques Pelon, Nicolas Pascal, Mark A. Vaughan, Philippe Dubuisson, Ping Yang, and David L. Mitchell
Atmos. Meas. Tech., 14, 3277–3299, https://doi.org/10.5194/amt-14-3277-2021, https://doi.org/10.5194/amt-14-3277-2021, 2021
Short summary
Short summary
The IIR Level 2 data products include cloud effective emissivities and cloud microphysical properties such as effective diameter (De) and ice or liquid water path estimates. This paper (Part II) shows retrievals over ocean and describes the improvements made with respect to version 3 as a result of the significant changes implemented in the version 4 algorithms, which are presented in a companion paper (Part I).
David L. Mitchell, John Mejia, Anne Garnier, Yuta Tomii, Martina Krämer, and Farnaz Hosseinpour
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-846, https://doi.org/10.5194/acp-2020-846, 2020
Publication in ACP not foreseen
Short summary
Short summary
This may be the first estimate of the radiative contribution of homogeneous ice nucleation in cirrus clouds on a global, regional and seasonal scale. This is achieved by constraining an atmospheric global climate model with measured cirrus cloud properties via satellite remote sensing. The results show that the overall radiative warming contributed by homogeneous ice nucleation at the top of the atmosphere is 2.4 W m-2 outside the ± 30° latitude zone during non-summer months (JJA).
David L. Mitchell, Anne Garnier, Jacques Pelon, and Ehsan Erfani
Atmos. Chem. Phys., 18, 17325–17354, https://doi.org/10.5194/acp-18-17325-2018, https://doi.org/10.5194/acp-18-17325-2018, 2018
Short summary
Short summary
To realistically model a changing climate, global measurements of cirrus cloud ice-particle number concentration (N) and size (De) are needed, through which one may infer the general mechanism of ice formation. A satellite remote sensing method was developed to measure N and De. It was found that N was highest and De lowest at high latitudes. In the Arctic, cirrus clouds occurred much more often during winter, which may have an impact on mid-latitude winter weather.
Ehsan Erfani and David L. Mitchell
Atmos. Chem. Phys., 17, 1241–1257, https://doi.org/10.5194/acp-17-1241-2017, https://doi.org/10.5194/acp-17-1241-2017, 2017
Short summary
Short summary
Rimed particle projected area- and mass-dimension expressions are developed and validated.
A convenient means of relating the unrimed and rimed m – D and A – D expressions was developed.
Equations are provided to calculate collision efficiency for use in models.
David L. Mitchell, Anne Garnier, Melody Avery, and Ehsan Erfani
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-1062, https://doi.org/10.5194/acp-2016-1062, 2016
Revised manuscript not accepted
Short summary
Short summary
Although the main objective of our DOE/Atmospheric Systems Research project was to use aircraft measurements to determine the formation (i.e. ice nucleation) mechanism of cirrus clouds, it soon became evident that the formation mechanism will depend on latitude, season and surface topography. A new satellite remote sensing method was developed to discover this dependency, which shows that roughly half or more of the cirrus clouds at high latitudes form through homogeneous ice nucleation.
Related subject area
Subject: Clouds and Precipitation | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Microphysical view of the development and ice production of mid-latitude stratiform clouds with embedded convection during an extratropical cyclone
Clouds and precipitation in the initial phase of marine cold-air outbreaks as observed by airborne remote sensing
Estimating the snow density using collocated Parsivel and Micro-Rain Radar measurements: a preliminary study from ICE-POP 2017/2018
Technical note: On the ice microphysics of isolated thunderstorms and non-thunderstorms in southern China – a radar polarimetric perspective
Distinctive aerosol–cloud–precipitation interactions in marine boundary layer clouds from the ACE-ENA and SOCRATES aircraft field campaigns
Theoretical Framework for Measuring Cloud Effective Supersaturation Fluctuations with an Advanced Optical System
Drivers of droplet formation in east Mediterranean orographic clouds
Observability of moisture transport divergence in Arctic atmospheric rivers by dropsondes
Elucidating the boundary layer turbulence dissipation rate using high-resolution measurements from a radar wind profiler network over the Tibetan Plateau
Environmental controls on isolated convection during the Amazonian wet season
Isotopic composition of convective rainfall in the inland tropics of Brazil
Measurement report: Cloud and environmental properties associated with aggregated shallow marine cumulus and cumulus congestus
How does riming influence the observed spatial variability of ice water in mixed-phase clouds?
Lifecycle of updrafts and mass flux in isolated deep convection over the Amazon rainforest: insights from cell tracking
Thermodynamic and cloud evolution in a cold-air outbreak during HALO-(AC)3: quasi-Lagrangian observations compared to the ERA5 and CARRA reanalyses
Powering aircraft with 100 % sustainable aviation fuel reduces ice crystals in contrails
Supercooled liquid water clouds observed over Dome C, Antarctica: temperature sensitivity and cloud radiative forcing
Role of thermodynamic and turbulence processes on the fog life cycle during SOFOG3D experiment
Characterizing the near-global cloud vertical structures over land using high-resolution radiosonde measurements
Investigating the role of typhoon-induced gravity waves and stratospheric hydration in the formation of tropopause cirrus clouds observed during the 2017 Asian monsoon
Differences in microphysical properties of cirrus at high and mid-latitudes
Sub-cloud rain evaporation in the North Atlantic winter trade winds derived by pairing isotopic data with a bin-resolved microphysical model
Overview and statistical analysis of boundary layer clouds and precipitation over the western North Atlantic Ocean
A set of methods to evaluate the below-cloud evaporation effect on local precipitation isotopic composition: a case study for Xi'an, China
Earth-system-model evaluation of cloud and precipitation occurrence for supercooled and warm clouds over the Southern Ocean's Macquarie Island
Pollution slightly enhances atmospheric cooling by low-level clouds in tropical West Africa
Investigating an indirect aviation effect on mid-latitude cirrus clouds – linking lidar-derived optical properties to in situ measurements
Investigating the vertical extent and short-wave radiative effects of the ice phase in Arctic summertime low-level clouds
Microphysical and thermodynamic phase analyses of Arctic low-level clouds measured above the sea ice and the open ocean in spring and summer
Aircraft observations of gravity wave activity and turbulence in the tropical tropopause layer: prevalence, influence on cirrus clouds, and comparison with global storm-resolving models
Influence of air mass origin on microphysical properties of low-level clouds in a subarctic environment
Sensitivity of convectively driven tropical tropopause cirrus properties to ice habits in high-resolution simulations
Upper-tropospheric slightly ice-subsaturated regions: frequency of occurrence and statistical evidence for the appearance of contrail cirrus
Examination of aerosol indirect effects during cirrus cloud evolution
In situ microphysics observations of intense pyroconvection from a large wildfire
Conditions favorable for secondary ice production in Arctic mixed-phase clouds
Interaction between cloud–radiation, atmospheric dynamics and thermodynamics based on observational data from GoAmazon 2014/15 and a cloud-resolving model
Snowfall in Northern Finland derives mostly from ice clouds
Observation of secondary ice production in clouds at low temperatures
In situ and satellite-based estimates of cloud properties and aerosol–cloud interactions over the southeast Atlantic Ocean
Ice fog observed at cirrus temperatures at Dome C, Antarctic Plateau
Life cycle of stratocumulus clouds over 1 year at the coast of the Atacama Desert
Experimental study on the evolution of droplet size distribution during the fog life cycle
Significant continental source of ice-nucleating particles at the tip of Chile's southernmost Patagonia region
Retrieving ice-nucleating particle concentration and ice multiplication factors using active remote sensing validated by in situ observations
Temporal and vertical distributions of the occurrence of cirrus clouds over a coastal station in the Indian monsoon region
Continental thunderstorm ground enhancement observed at an exceptionally low altitude
Ice-nucleating particles from multiple aerosol sources in the urban environment of Beijing under mixed-phase cloud conditions
In situ observation of riming in mixed-phase clouds using the PHIPS probe
Measurement report: Introduction to the HyICE-2018 campaign for measurements of ice-nucleating particles and instrument inter-comparison in the Hyytiälä boreal forest
Yuanmou Du, Dantong Liu, Delong Zhao, Mengyu Huang, Ping Tian, Dian Wen, Wei Xiao, Wei Zhou, Hui He, Baiwan Pan, Dongfei Zuo, Xiange Liu, Yingying Jing, Rong Zhang, Jiujiang Sheng, Fei Wang, Yu Huang, Yunbo Chen, and Deping Ding
Atmos. Chem. Phys., 24, 13429–13444, https://doi.org/10.5194/acp-24-13429-2024, https://doi.org/10.5194/acp-24-13429-2024, 2024
Short summary
Short summary
By conducting in situ measurements, we investigated ice production processes in stratiform clouds with embedded convection over the North China Plain. The results show that the ice number concentration is strongly related to the distance to the cloud top, and the level with a larger distance to the cloud top has more graupel falling from upper levels, which promotes collision and coalescence between graupel and droplets and enhances secondary ice production.
Imke Schirmacher, Sabrina Schnitt, Marcus Klingebiel, Nina Maherndl, Benjamin Kirbus, André Ehrlich, Mario Mech, and Susanne Crewell
Atmos. Chem. Phys., 24, 12823–12842, https://doi.org/10.5194/acp-24-12823-2024, https://doi.org/10.5194/acp-24-12823-2024, 2024
Short summary
Short summary
During Arctic marine cold-air outbreaks, cold air flows from sea ice over open water. Roll circulations evolve, forming cloud streets. We investigate the initial circulation and cloud development using high-resolution airborne measurements. We compute the distance an air mass traveled over water (fetch) from back trajectories. Cloud streets form at 15 km fetch, cloud cover strongly increases at around 20 km, and precipitation forms at around 30 km.
Wei-Yu Chang, Yung-Chuan Yang, Chen-Yu Hung, Kwonil Kim, Gyuwon Lee, and Ali Tokay
Atmos. Chem. Phys., 24, 11955–11979, https://doi.org/10.5194/acp-24-11955-2024, https://doi.org/10.5194/acp-24-11955-2024, 2024
Short summary
Short summary
Snow density is derived by collocated Micro-Rain Radar (MRR) and Parsivel (ICE-POP 2017/2018). We apply the particle size distribution from Parsivel to a T-matrix backscattering simulation and compare with ZHH from MRR. Bulk density and bulk water fractions are derived from comparing simulated and calculated ZHH. Retrieved bulk density is validated by comparing snowfall rate measurements from Pluvio and the Precipitation Imaging Package. Snowfall rate consistency confirms the algorithm.
Chuanhong Zhao, Yijun Zhang, Dong Zheng, Haoran Li, Sai Du, Xueyan Peng, Xiantong Liu, Pengguo Zhao, Jiafeng Zheng, and Juan Shi
Atmos. Chem. Phys., 24, 11637–11651, https://doi.org/10.5194/acp-24-11637-2024, https://doi.org/10.5194/acp-24-11637-2024, 2024
Short summary
Short summary
Understanding lightning activity is important for meteorology and atmospheric chemistry. However, the occurrence of lightning activity in clouds is uncertain. In this study, we quantified the difference between isolated thunderstorms and non-thunderstorms. We showed that lightning activity was more likely to occur with more graupel volume and/or riming. A deeper ZDR column was associated with lightning occurrence. This information can aid in a deeper understanding of lighting physics.
Xiaojian Zheng, Xiquan Dong, Baike Xi, Timothy Logan, and Yuan Wang
Atmos. Chem. Phys., 24, 10323–10347, https://doi.org/10.5194/acp-24-10323-2024, https://doi.org/10.5194/acp-24-10323-2024, 2024
Short summary
Short summary
The marine boundary layer aerosol–cloud interactions (ACIs) are examined using in situ measurements from two aircraft campaigns over the eastern North Atlantic (ACE-ENA) and Southern Ocean (SOCRATES). The SOCRATES clouds have more and smaller cloud droplets. The ACE-ENA clouds exhibit stronger drizzle formation and growth. Results found distinctive aerosol–cloud interactions for two campaigns. The drizzle processes significantly alter sub-cloud aerosol budgets and impact the ACI assessments.
Ye Kuang, Jiangchuan Tao, Hanbin Xu, Li Liu, Pengfei Liu, Wanyun Xu, Weiqi Xu, Yele Sun, and Chunsheng Zhao
EGUsphere, https://doi.org/10.5194/egusphere-2024-2698, https://doi.org/10.5194/egusphere-2024-2698, 2024
Short summary
Short summary
This study presents a novel optical framework to measure supersaturation, a fundamental parameter in cloud physics, by observing the scattering properties of particles that have or have not grown into cloud droplets. The technique offers high-resolution measurements, capturing essential fluctuations in supersaturation necessary for understanding cloud physics.
Romanos Foskinis, Ghislain Motos, Maria I. Gini, Olga Zografou, Kunfeng Gao, Stergios Vratolis, Konstantinos Granakis, Ville Vakkari, Kalliopi Violaki, Andreas Aktypis, Christos Kaltsonoudis, Zongbo Shi, Mika Komppula, Spyros N. Pandis, Konstantinos Eleftheriadis, Alexandros Papayannis, and Athanasios Nenes
Atmos. Chem. Phys., 24, 9827–9842, https://doi.org/10.5194/acp-24-9827-2024, https://doi.org/10.5194/acp-24-9827-2024, 2024
Short summary
Short summary
Analysis of modeling, in situ, and remote sensing measurements reveals the microphysical state of orographic clouds and their response to aerosol from the boundary layer and free troposphere. We show that cloud response to aerosol is robust, as predicted supersaturation and cloud droplet number levels agree with those determined from in-cloud measurements. The ability to determine if clouds are velocity- or aerosol-limited allows for novel model constraints and remote sensing products.
Henning Dorff, Heike Konow, Vera Schemann, and Felix Ament
Atmos. Chem. Phys., 24, 8771–8795, https://doi.org/10.5194/acp-24-8771-2024, https://doi.org/10.5194/acp-24-8771-2024, 2024
Short summary
Short summary
Using synthetic dropsondes, we assess how discrete spatial sampling and temporal evolution during flight affect the accuracy of real sonde-based moisture transport divergence in Arctic atmospheric rivers (ARs). Non-instantaneous sampling during temporal AR evolution deteriorates the divergence values more than spatial undersampling. Moisture advection is the dominating factor but most sensitive to the sampling method. We suggest a minimum of seven sondes to resolve the AR divergence components.
Deli Meng, Jianping Guo, Xiaoran Guo, Yinjun Wang, Ning Li, Yuping Sun, Zhen Zhang, Na Tang, Haoran Li, Fan Zhang, Bing Tong, Hui Xu, and Tianmeng Chen
Atmos. Chem. Phys., 24, 8703–8720, https://doi.org/10.5194/acp-24-8703-2024, https://doi.org/10.5194/acp-24-8703-2024, 2024
Short summary
Short summary
The turbulence in the planetary boundary layer (PBL) over the Tibetan Plateau (TP) remains unclear. Here we elucidate the vertical profile of and temporal variation in the turbulence dissipation rate in the PBL over the TP based on a radar wind profiler (RWP) network. To the best of our knowledge, this is the first time that the turbulence profile over the whole TP has been revealed. Furthermore, the possible mechanisms of clouds acting on the PBL turbulence structure are investigated.
Leandro Alex Moreira Viscardi, Giuseppe Torri, David K. Adams, and Henrique de Melo Jorge Barbosa
Atmos. Chem. Phys., 24, 8529–8548, https://doi.org/10.5194/acp-24-8529-2024, https://doi.org/10.5194/acp-24-8529-2024, 2024
Short summary
Short summary
We evaluate the environmental conditions that control how clouds grow from fair weather cumulus into severe thunderstorms during the Amazonian wet season. Days with rain clouds begin with more moisture in the air and have strong convergence in the afternoon, while precipitation intensity increases with large-scale vertical velocity, moisture, and low-level wind. These results contribute to understanding how clouds form over the rainforest.
Vinicius dos Santos, Didier Gastmans, Ana María Durán-Quesada, Ricardo Sánchez-Murillo, Kazimierz Rozanski, Oliver Kracht, and Demilson de Assis Quintão
Atmos. Chem. Phys., 24, 6663–6680, https://doi.org/10.5194/acp-24-6663-2024, https://doi.org/10.5194/acp-24-6663-2024, 2024
Short summary
Short summary
We present novel findings on convective rainfall, summer rain in the late afternoon, by coupling water stable isotopes, micro rain radar, and satellite data. We found the tallest clouds in the afternoon and much smaller clouds at night, resulting in differences in day–night ratios in water stable isotopes. We sampled rain and meteorological variables every 5–10 min, allowing us to evaluate the development of convective rainfall, contributing to knowledge of rainfall related to extreme events.
Ewan Crosbie, Luke D. Ziemba, Michael A. Shook, Taylor Shingler, Johnathan W. Hair, Armin Sorooshian, Richard A. Ferrare, Brian Cairns, Yonghoon Choi, Joshua DiGangi, Glenn S. Diskin, Chris Hostetler, Simon Kirschler, Richard H. Moore, David Painemal, Claire Robinson, Shane T. Seaman, K. Lee Thornhill, Christiane Voigt, and Edward Winstead
Atmos. Chem. Phys., 24, 6123–6152, https://doi.org/10.5194/acp-24-6123-2024, https://doi.org/10.5194/acp-24-6123-2024, 2024
Short summary
Short summary
Marine clouds are found to clump together in regions or lines, readily discernible from satellite images of the ocean. While clustering is also a feature of deep storm clouds, we focus on smaller cloud systems associated with fair weather and brief localized showers. Two aircraft sampled the region around these shallow systems: one incorporated measurements taken within, adjacent to, and below the clouds, while the other provided a survey from above using remote sensing techniques.
Nina Maherndl, Manuel Moser, Imke Schirmacher, Aaron Bansemer, Johannes Lucke, Christiane Voigt, and Maximilian Maahn
EGUsphere, https://doi.org/10.5194/egusphere-2024-1214, https://doi.org/10.5194/egusphere-2024-1214, 2024
Short summary
Short summary
It is not clear, why ice crystals in clouds occur in clusters. Here, airborne measurements of clouds in mid- and high-latitudes are used to study the spatial variability of ice. Further, we investigate the influence of riming, which occurs when liquid droplets freeze onto ice crystals. We find that riming enhances the occurrence of ice clusters. In the Arctic, riming leads to ice clustering at spatial scales of 3–5 km. This is due to updrafts, not necessary higher amounts of liquid water.
Siddhant Gupta, Dié Wang, Scott E. Giangrande, Thiago S. Biscaro, and Michael P. Jensen
Atmos. Chem. Phys., 24, 4487–4510, https://doi.org/10.5194/acp-24-4487-2024, https://doi.org/10.5194/acp-24-4487-2024, 2024
Short summary
Short summary
We examine the lifecycle of isolated deep convective clouds (DCCs) in the Amazon rainforest. Weather radar echoes from the DCCs are tracked to evaluate their lifecycle. The DCC size and intensity increase, reach a peak, and then decrease over the DCC lifetime. Vertical profiles of air motion and mass transport from different seasons are examined to understand the transport of energy and momentum within DCC cores and to address the deficiencies in simulating DCCs using weather and climate models.
Benjamin Kirbus, Imke Schirmacher, Marcus Klingebiel, Michael Schäfer, André Ehrlich, Nils Slättberg, Johannes Lucke, Manuel Moser, Hanno Müller, and Manfred Wendisch
Atmos. Chem. Phys., 24, 3883–3904, https://doi.org/10.5194/acp-24-3883-2024, https://doi.org/10.5194/acp-24-3883-2024, 2024
Short summary
Short summary
A research aircraft is used to track the changes in air temperature, moisture, and cloud properties for air that moves from cold Arctic sea ice onto warmer oceanic waters. The measurements are compared to two reanalysis models named ERA5 and CARRA. The biggest differences are found for air temperature over the sea ice and moisture over the ocean. CARRA data are more accurate than ERA5 because they better simulate the sea ice, the transition from sea ice to open ocean, and the forming clouds.
Raphael Satoru Märkl, Christiane Voigt, Daniel Sauer, Rebecca Katharina Dischl, Stefan Kaufmann, Theresa Harlaß, Valerian Hahn, Anke Roiger, Cornelius Weiß-Rehm, Ulrike Burkhardt, Ulrich Schumann, Andreas Marsing, Monika Scheibe, Andreas Dörnbrack, Charles Renard, Maxime Gauthier, Peter Swann, Paul Madden, Darren Luff, Reetu Sallinen, Tobias Schripp, and Patrick Le Clercq
Atmos. Chem. Phys., 24, 3813–3837, https://doi.org/10.5194/acp-24-3813-2024, https://doi.org/10.5194/acp-24-3813-2024, 2024
Short summary
Short summary
In situ measurements of contrails from a large passenger aircraft burning 100 % sustainable aviation fuel (SAF) show a 56 % reduction in contrail ice crystal numbers compared to conventional Jet A-1. Results from a climate model initialized with the observations suggest a significant decrease in radiative forcing from contrails. Our study confirms that future increased use of low aromatic SAF can reduce the climate impact from aviation.
Philippe Ricaud, Massimo Del Guasta, Angelo Lupi, Romain Roehrig, Eric Bazile, Pierre Durand, Jean-Luc Attié, Alessia Nicosia, and Paolo Grigioni
Atmos. Chem. Phys., 24, 613–630, https://doi.org/10.5194/acp-24-613-2024, https://doi.org/10.5194/acp-24-613-2024, 2024
Short summary
Short summary
Clouds affect the Earth's climate in ways that depend on the type of cloud (solid/liquid water). From observations at Concordia (Antarctica), we show that in supercooled liquid water (liquid water for temperatures below 0°C) clouds (SLWCs), temperature and SLWC radiative forcing increase with liquid water (up to 70 W m−2). We extrapolated that the maximum SLWC radiative forcing can reach 40 W m−2 over the Antarctic Peninsula, highlighting the importance of SLWCs for global climate prediction.
Cheikh Dione, Martial Haeffelin, Frédéric Burnet, Christine Lac, Guylaine Canut, Julien Delanoë, Jean-Charles Dupont, Susana Jorquera, Pauline Martinet, Jean-François Ribaud, and Felipe Toledo
Atmos. Chem. Phys., 23, 15711–15731, https://doi.org/10.5194/acp-23-15711-2023, https://doi.org/10.5194/acp-23-15711-2023, 2023
Short summary
Short summary
This paper documents the role of thermodynamics and turbulence in the fog life cycle over southwestern France. It is based on a unique dataset collected during the SOFOG3D field campaign in autumn and winter 2019–2020. The paper gives a threshold for turbulence driving the different phases of the fog life cycle and the role of advection in the night-time dissipation of fog. The results can be operationalised to nowcast fog and improve short-range forecasts in numerical weather prediction models.
Hui Xu, Jianping Guo, Bing Tong, Jinqiang Zhang, Tianmeng Chen, Xiaoran Guo, Jian Zhang, and Wenqing Chen
Atmos. Chem. Phys., 23, 15011–15038, https://doi.org/10.5194/acp-23-15011-2023, https://doi.org/10.5194/acp-23-15011-2023, 2023
Short summary
Short summary
The radiative effect of cloud remains one of the largest uncertain factors in climate change, largely due to the lack of cloud vertical structure (CVS) observations. The study presents the first near-global CVS climatology using high-vertical-resolution soundings. Single-layer cloud mainly occurs over arid regions. As the number of cloud layers increases, clouds tend to have lower bases and thinner layer thicknesses. The occurrence frequency of cloud exhibits a pronounced seasonal diurnal cycle.
Amit Kumar Pandit, Jean-Paul Vernier, Thomas Duncan Fairlie, Kristopher M. Bedka, Melody A. Avery, Harish Gadhavi, Madineni Venkat Ratnam, Sanjeev Dwivedi, Kasimahanthi Amar Jyothi, Frank G. Wienhold, Holger Vömel, Hongyu Liu, Bo Zhang, Buduru Suneel Kumar, Tra Dinh, and Achuthan Jayaraman
EGUsphere, https://doi.org/10.5194/egusphere-2023-2236, https://doi.org/10.5194/egusphere-2023-2236, 2023
Short summary
Short summary
This study investigates the formation mechanism of a tropopause cirrus cloud layer observed at extremely cold temperatures over Hyderabad in India during the 2017 Asian summer monsoon using balloon-borne sensors. Ice crystals smaller than 50 microns were found in this optically thin cirrus cloud layer. Combined analysis of back-trajectories, satellite, and model data revealed that the formation of this layer was influenced by gravity waves and stratospheric hydration induced by typhoon Hato.
Elena De La Torre Castro, Tina Jurkat-Witschas, Armin Afchine, Volker Grewe, Valerian Hahn, Simon Kirschler, Martina Krämer, Johannes Lucke, Nicole Spelten, Heini Wernli, Martin Zöger, and Christiane Voigt
Atmos. Chem. Phys., 23, 13167–13189, https://doi.org/10.5194/acp-23-13167-2023, https://doi.org/10.5194/acp-23-13167-2023, 2023
Short summary
Short summary
In this study, we show the differences in the microphysical properties between high-latitude (HL) cirrus and mid-latitude (ML) cirrus over the Arctic, North Atlantic, and central Europe during summer. The in situ measurements are combined with backward trajectories to investigate the influence of the region on cloud formation. We show that HL cirrus are characterized by a lower concentration of larger ice crystals when compared to ML cirrus.
Mampi Sarkar, Adriana Bailey, Peter Blossey, Simon P. de Szoeke, David Noone, Estefanía Quiñones Meléndez, Mason D. Leandro, and Patrick Y. Chuang
Atmos. Chem. Phys., 23, 12671–12690, https://doi.org/10.5194/acp-23-12671-2023, https://doi.org/10.5194/acp-23-12671-2023, 2023
Short summary
Short summary
We study rain evaporation characteristics below shallow cumulus clouds over the North Atlantic Ocean by pairing isotope observations with a microphysical model. The modeled fraction of rain mass that evaporates below the cloud strongly depends on the raindrop size and distribution width. Moreover, the higher the rain mass fraction evaporated, the greater the change in deuterium excess. In this way, rain evaporation could be studied independently using only isotope and microphysical observations.
Simon Kirschler, Christiane Voigt, Bruce E. Anderson, Gao Chen, Ewan C. Crosbie, Richard A. Ferrare, Valerian Hahn, Johnathan W. Hair, Stefan Kaufmann, Richard H. Moore, David Painemal, Claire E. Robinson, Kevin J. Sanchez, Amy J. Scarino, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Edward L. Winstead, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 23, 10731–10750, https://doi.org/10.5194/acp-23-10731-2023, https://doi.org/10.5194/acp-23-10731-2023, 2023
Short summary
Short summary
In this study we present an overview of liquid and mixed-phase clouds and precipitation in the marine boundary layer over the western North Atlantic Ocean. We compare microphysical properties of pure liquid clouds to mixed-phase clouds and show that the initiation of the ice phase in mixed-phase clouds promotes precipitation. The observational data presented in this study are well suited for investigating the processes that give rise to liquid and mixed-phase clouds, ice, and precipitation.
Meng Xing, Weiguo Liu, Jing Hu, and Zheng Wang
Atmos. Chem. Phys., 23, 9123–9136, https://doi.org/10.5194/acp-23-9123-2023, https://doi.org/10.5194/acp-23-9123-2023, 2023
Short summary
Short summary
The below-cloud evaporation effect (BCE) on precipitation largely impacts the final isotopic composition. However, determining the BCE effect remains poorly constrained. Our work used a ΔdΔδ diagram to differentiate the below-cloud processes. Moreover, by comparing two different computing methods, we considered that both methods are suitable for evaluation the BCE, except for snowfall events. Overall, our work compiled a set of effective methods to evaluate the BCE effect.
McKenna W. Stanford, Ann M. Fridlind, Israel Silber, Andrew S. Ackerman, Greg Cesana, Johannes Mülmenstädt, Alain Protat, Simon Alexander, and Adrian McDonald
Atmos. Chem. Phys., 23, 9037–9069, https://doi.org/10.5194/acp-23-9037-2023, https://doi.org/10.5194/acp-23-9037-2023, 2023
Short summary
Short summary
Clouds play an important role in the Earth’s climate system as they modulate the amount of radiation that either reaches the surface or is reflected back to space. This study demonstrates an approach to robustly evaluate surface-based observations against a large-scale model. We find that the large-scale model precipitates too infrequently relative to observations, contrary to literature documentation suggesting otherwise based on satellite measurements.
Valerian Hahn, Ralf Meerkötter, Christiane Voigt, Sonja Gisinger, Daniel Sauer, Valéry Catoire, Volker Dreiling, Hugh Coe, Cyrille Flamant, Stefan Kaufmann, Jonas Kleine, Peter Knippertz, Manuel Moser, Philip Rosenberg, Hans Schlager, Alfons Schwarzenboeck, and Jonathan Taylor
Atmos. Chem. Phys., 23, 8515–8530, https://doi.org/10.5194/acp-23-8515-2023, https://doi.org/10.5194/acp-23-8515-2023, 2023
Short summary
Short summary
During the DACCIWA campaign in West Africa, we found a 35 % increase in the cloud droplet concentration that formed in a polluted compared with a less polluted environment and a decrease of 17 % in effective droplet diameter. Radiative transfer simulations, based on the measured cloud properties, reveal that these low-level polluted clouds radiate only 2.6 % more energy back to space, compared with a less polluted cloud. The corresponding additional decrease in temperature is rather small.
Silke Groß, Tina Jurkat-Witschas, Qiang Li, Martin Wirth, Benedikt Urbanek, Martina Krämer, Ralf Weigel, and Christiane Voigt
Atmos. Chem. Phys., 23, 8369–8381, https://doi.org/10.5194/acp-23-8369-2023, https://doi.org/10.5194/acp-23-8369-2023, 2023
Short summary
Short summary
Aviation-emitted aerosol can have an impact on cirrus clouds. We present optical and microphysical properties of mid-latitude cirrus clouds which were formed under the influence of aviation-emitted aerosol or which were formed under rather pristine conditions. We find that cirrus clouds affected by aviation-emitted aerosol show larger values of the particle linear depolarization ratio, larger mean effective ice particle diameters and decreased ice particle number concentrations.
Emma Järvinen, Franziska Nehlert, Guanglang Xu, Fritz Waitz, Guillaume Mioche, Regis Dupuy, Olivier Jourdan, and Martin Schnaiter
Atmos. Chem. Phys., 23, 7611–7633, https://doi.org/10.5194/acp-23-7611-2023, https://doi.org/10.5194/acp-23-7611-2023, 2023
Short summary
Short summary
The Arctic is warming faster than other regions. Arctic low-level mixed-phase clouds, where ice crystals and liquid droplets co-exist, are thought to have an important role in Arctic warming. Here we show airborne measurements of vertical distribution of liquid and ice particles and their relative abundance. Ice particles are found in relative warm clouds, which can be explained by multiplication of existing ice crystals. However, the role of ice particles in redistributing sun light is minimal.
Manuel Moser, Christiane Voigt, Tina Jurkat-Witschas, Valerian Hahn, Guillaume Mioche, Olivier Jourdan, Régis Dupuy, Christophe Gourbeyre, Alfons Schwarzenboeck, Johannes Lucke, Yvonne Boose, Mario Mech, Stephan Borrmann, André Ehrlich, Andreas Herber, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys., 23, 7257–7280, https://doi.org/10.5194/acp-23-7257-2023, https://doi.org/10.5194/acp-23-7257-2023, 2023
Short summary
Short summary
This study provides a comprehensive microphysical and thermodynamic phase analysis of low-level clouds in the northern Fram Strait, above the sea ice and the open ocean, during spring and summer. Using airborne in situ cloud data, we show that the properties of Arctic low-level clouds vary significantly with seasonal meteorological situations and surface conditions. The observations presented in this study can help one to assess the role of clouds in the Arctic climate system.
Rachel Atlas and Christopher S. Bretherton
Atmos. Chem. Phys., 23, 4009–4030, https://doi.org/10.5194/acp-23-4009-2023, https://doi.org/10.5194/acp-23-4009-2023, 2023
Short summary
Short summary
The tropical tropopause layer exists between the troposphere and the stratosphere in the tropics. Very thin cirrus clouds cool Earth's surface by scrubbing water vapor (a greenhouse gas) out of air parcels as they ascend through the tropical tropopause layer on their way to the stratosphere. We show observational evidence from aircraft that small-scale (< 100 km) gravity waves and turbulence increase the amount of ice in these clouds and may allow them to remove more water vapor from the air.
Konstantinos Matthaios Doulgeris, Ville Vakkari, Ewan J. O'Connor, Veli-Matti Kerminen, Heikki Lihavainen, and David Brus
Atmos. Chem. Phys., 23, 2483–2498, https://doi.org/10.5194/acp-23-2483-2023, https://doi.org/10.5194/acp-23-2483-2023, 2023
Short summary
Short summary
We investigated how different long-range-transported air masses can affect the microphysical properties of low-level clouds in a clean subarctic environment. A connection was revealed. Higher values of cloud droplet number concentrations were related to continental air masses, whereas the lowest values of number concentrations were related to marine air masses. These were characterized by larger cloud droplets. Clouds in all regions were sensitive to increases in cloud number concentration.
Fayçal Lamraoui, Martina Krämer, Armin Afchine, Adam B. Sokol, Sergey Khaykin, Apoorva Pandey, and Zhiming Kuang
Atmos. Chem. Phys., 23, 2393–2419, https://doi.org/10.5194/acp-23-2393-2023, https://doi.org/10.5194/acp-23-2393-2023, 2023
Short summary
Short summary
Cirrus in the tropical tropopause layer (TTL) can play a key role in vertical transport. We investigate the role of different cloud regimes and the associated ice habits in regulating the properties of the TTL. We use high-resolution numerical experiments at the scales of large-eddy simulations (LESs) and aircraft measurements. We found that LES-scale parameterizations that predict ice shape are crucial for an accurate representation of TTL cirrus and thus the associated (de)hydration process.
Yun Li, Christoph Mahnke, Susanne Rohs, Ulrich Bundke, Nicole Spelten, Georgios Dekoutsidis, Silke Groß, Christiane Voigt, Ulrich Schumann, Andreas Petzold, and Martina Krämer
Atmos. Chem. Phys., 23, 2251–2271, https://doi.org/10.5194/acp-23-2251-2023, https://doi.org/10.5194/acp-23-2251-2023, 2023
Short summary
Short summary
The radiative effect of aviation-induced cirrus is closely related to ambient conditions and its microphysical properties. Our study investigated the occurrence of contrail and natural cirrus measured above central Europe in spring 2014. It finds that contrail cirrus appears frequently in the pressure range 200 to 245 hPa and occurs more often in slightly ice-subsaturated environments than expected. Avoiding slightly ice-subsaturated regions by aviation might help mitigate contrail cirrus.
Flor Vanessa Maciel, Minghui Diao, and Ryan Patnaude
Atmos. Chem. Phys., 23, 1103–1129, https://doi.org/10.5194/acp-23-1103-2023, https://doi.org/10.5194/acp-23-1103-2023, 2023
Short summary
Short summary
Aerosol indirect effects on cirrus clouds are investigated during cirrus evolution, using global-scale in situ observations and climate model simulations. As cirrus evolves, the mechanisms to form ice crystals also change with time. Both small and large aerosols are found to affect cirrus properties. Southern Hemisphere cirrus appears to be more sensitive to additional aerosols. The climate model underestimates ice crystal mass, likely due to biases of relative humidity and vertical velocity.
David E. Kingsmill, Jeffrey R. French, and Neil P. Lareau
Atmos. Chem. Phys., 23, 1–21, https://doi.org/10.5194/acp-23-1-2023, https://doi.org/10.5194/acp-23-1-2023, 2023
Short summary
Short summary
This study uses in situ aircraft measurements to characterize the size and shape distributions of 10 µm to 6 mm diameter particles observed during six penetrations of wildfire-induced pyroconvection. Particles sampled in one penetration of a smoke plume are most likely pyrometeors composed of ash. The other penetrations are through pyrocumulus clouds where particle composition is most likely a combination of hydrometeors (ice particles) and pyrometeors (ash).
Julie Thérèse Pasquier, Jan Henneberger, Fabiola Ramelli, Annika Lauber, Robert Oscar David, Jörg Wieder, Tim Carlsen, Rosa Gierens, Marion Maturilli, and Ulrike Lohmann
Atmos. Chem. Phys., 22, 15579–15601, https://doi.org/10.5194/acp-22-15579-2022, https://doi.org/10.5194/acp-22-15579-2022, 2022
Short summary
Short summary
It is important to understand how ice crystals and cloud droplets form in clouds, as their concentrations and sizes determine the exact radiative properties of the clouds. Normally, ice crystals form from aerosols, but we found evidence for the formation of additional ice crystals from the original ones over a large temperature range within Arctic clouds. In particular, additional ice crystals were formed during collisions of several ice crystals or during the freezing of large cloud droplets.
Layrson J. M. Gonçalves, Simone M. S. C. Coelho, Paulo Y. Kubota, and Dayana C. Souza
Atmos. Chem. Phys., 22, 15509–15526, https://doi.org/10.5194/acp-22-15509-2022, https://doi.org/10.5194/acp-22-15509-2022, 2022
Short summary
Short summary
This research aims to study the environmental conditions that are favorable and not favorable to cloud formation, in this case specifically for the Amazon region. The results found in this research will be used to improve the representation of clouds in numerical models that are used in weather and climate prediction. In general, it is expected that with better knowledge regarding the cloud–radiation interaction, it is possible to make a better forecast of weather and climate.
Claudia Mignani, Lukas Zimmermann, Rigel Kivi, Alexis Berne, and Franz Conen
Atmos. Chem. Phys., 22, 13551–13568, https://doi.org/10.5194/acp-22-13551-2022, https://doi.org/10.5194/acp-22-13551-2022, 2022
Short summary
Short summary
We determined over the course of 8 winter months the phase of clouds associated with snowfall in Northern Finland using radiosondes and observations of ice particle habits at ground level. We found that precipitating clouds were extending from near ground to at least 2.7 km altitude and approximately three-quarters of them were likely glaciated. Possible moisture sources and ice formation processes are discussed.
Alexei Korolev, Paul J. DeMott, Ivan Heckman, Mengistu Wolde, Earle Williams, David J. Smalley, and Michael F. Donovan
Atmos. Chem. Phys., 22, 13103–13113, https://doi.org/10.5194/acp-22-13103-2022, https://doi.org/10.5194/acp-22-13103-2022, 2022
Short summary
Short summary
The present study provides the first explicit in situ observation of secondary ice production at temperatures as low as −27 °C, which is well outside the range of the Hallett–Mossop process (−3 to −8 °C). This observation expands our knowledge of the temperature range of initiation of secondary ice in clouds. The obtained results are intended to stimulate laboratory and theoretical studies to develop physically based parameterizations for weather prediction and climate models.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, Michael R. Poellot, David J. Delene, Ian Chang, Lan Gao, Feng Xu, and Jens Redemann
Atmos. Chem. Phys., 22, 12923–12943, https://doi.org/10.5194/acp-22-12923-2022, https://doi.org/10.5194/acp-22-12923-2022, 2022
Short summary
Short summary
The ability of NASA’s Terra and Aqua satellites to retrieve cloud properties and estimate the changes in cloud properties due to aerosol–cloud interactions (ACI) was examined. There was good agreement between satellite retrievals and in situ measurements over the southeast Atlantic Ocean. This suggests that, combined with information on aerosol properties, satellite retrievals of cloud properties can be used to study ACI over larger domains and longer timescales in the absence of in situ data.
Étienne Vignon, Lea Raillard, Christophe Genthon, Massimo Del Guasta, Andrew J. Heymsfield, Jean-Baptiste Madeleine, and Alexis Berne
Atmos. Chem. Phys., 22, 12857–12872, https://doi.org/10.5194/acp-22-12857-2022, https://doi.org/10.5194/acp-22-12857-2022, 2022
Short summary
Short summary
The near-surface atmosphere over the Antarctic Plateau is cold and pristine and resembles to a certain extent the high troposphere where cirrus clouds form. In this study, we use innovative humidity measurements at Concordia Station to study the formation of ice fogs at temperatures <−40°C. We provide observational evidence that ice fogs can form through the homogeneous freezing of solution aerosols, a common nucleation pathway for cirrus clouds.
Jan H. Schween, Camilo del Rio, Juan-Luis García, Pablo Osses, Sarah Westbrook, and Ulrich Löhnert
Atmos. Chem. Phys., 22, 12241–12267, https://doi.org/10.5194/acp-22-12241-2022, https://doi.org/10.5194/acp-22-12241-2022, 2022
Short summary
Short summary
Marine stratocumulus clouds of the eastern Pacific play an essential role in the Earth's climate. These clouds form the major source of water to parts of the extreme dry Atacama Desert at the northern coast of Chile. For the first time these clouds are observed over a whole year with three remote sensing instruments. It is shown how these clouds are influenced by the land–sea wind system and the distribution of ocean temperatures.
Marie Mazoyer, Frédéric Burnet, and Cyrielle Denjean
Atmos. Chem. Phys., 22, 11305–11321, https://doi.org/10.5194/acp-22-11305-2022, https://doi.org/10.5194/acp-22-11305-2022, 2022
Short summary
Short summary
The evolution of the droplet size distribution during the fog life cycle remains poorly understood and progress is required to reduce the uncertainty of fog forecasts. To gain insights into the physical processes driving the microphysics, intensive field campaigns were conducted during three winters at the SIRTA site in the south of Paris. This study analyzed the variations in fog microphysical properties and their potential interactions at the different evolutionary stages of the fog events.
Xianda Gong, Martin Radenz, Heike Wex, Patric Seifert, Farnoush Ataei, Silvia Henning, Holger Baars, Boris Barja, Albert Ansmann, and Frank Stratmann
Atmos. Chem. Phys., 22, 10505–10525, https://doi.org/10.5194/acp-22-10505-2022, https://doi.org/10.5194/acp-22-10505-2022, 2022
Short summary
Short summary
The sources of ice-nucleating particles (INPs) are poorly understood in the Southern Hemisphere (SH). We studied INPs in the boundary layer in the southern Patagonia region. No seasonal cycle of INP concentrations was observed. The majority of INPs are biogenic particles, likely from local continental sources. The INP concentrations are higher when strong precipitation occurs. While previous studies focused on marine INP sources in SH, we point out the importance of continental sources of INPs.
Jörg Wieder, Nikola Ihn, Claudia Mignani, Moritz Haarig, Johannes Bühl, Patric Seifert, Ronny Engelmann, Fabiola Ramelli, Zamin A. Kanji, Ulrike Lohmann, and Jan Henneberger
Atmos. Chem. Phys., 22, 9767–9797, https://doi.org/10.5194/acp-22-9767-2022, https://doi.org/10.5194/acp-22-9767-2022, 2022
Short summary
Short summary
Ice formation and its evolution in mixed-phase clouds are still uncertain. We evaluate the lidar retrieval of ice-nucleating particle concentration in dust-dominated and continental air masses over the Swiss Alps with in situ observations. A calibration factor to improve the retrieval from continental air masses is proposed. Ice multiplication factors are obtained with a new method utilizing remote sensing. Our results indicate that secondary ice production occurs at temperatures down to −30 °C.
Saleem Ali, Sanjay Kumar Mehta, Aravindhavel Ananthavel, and Tondapu Venkata Ramesh Reddy
Atmos. Chem. Phys., 22, 8321–8342, https://doi.org/10.5194/acp-22-8321-2022, https://doi.org/10.5194/acp-22-8321-2022, 2022
Short summary
Short summary
Multiple cirrus clouds frequently occur over regions of deep convection in the tropics. Tropical convection has a strong diurnal pattern, with peaks in the afternoon to early evening, over the continents. Continuous micropulse lidar observations over a coastal station in the Indian monsoon region enable us, for the first time, to demonstrate a robust diurnal pattern of single and multiple cirrus occurrences, with peaks during the late afternoon and early morning hours, respectively.
Ivana Kolmašová, Ondřej Santolík, Jakub Šlegl, Jana Popová, Zbyněk Sokol, Petr Zacharov, Ondřej Ploc, Gerhard Diendorfer, Ronald Langer, Radek Lán, and Igor Strhárský
Atmos. Chem. Phys., 22, 7959–7973, https://doi.org/10.5194/acp-22-7959-2022, https://doi.org/10.5194/acp-22-7959-2022, 2022
Short summary
Short summary
Gamma ray radiation related to thunderstorms was previously observed at the high-altitude mountain observatories or on the western coast of Japan, usually being terminated by lightning discharges. We show unusual observations of gamma rays at an altitude below 1000 m, coinciding with peculiar rapid variations in the vertical electric field, which are linked to inverted intracloud lightning discharges. This indicates that a strong, lower positive-charge region was present inside the thundercloud.
Cuiqi Zhang, Zhijun Wu, Jingchuan Chen, Jie Chen, Lizi Tang, Wenfei Zhu, Xiangyu Pei, Shiyi Chen, Ping Tian, Song Guo, Limin Zeng, Min Hu, and Zamin A. Kanji
Atmos. Chem. Phys., 22, 7539–7556, https://doi.org/10.5194/acp-22-7539-2022, https://doi.org/10.5194/acp-22-7539-2022, 2022
Short summary
Short summary
The immersion ice nucleation effectiveness of aerosols from multiple sources in the urban environment remains elusive. In this study, we demonstrate that the immersion ice-nucleating particle (INP) concentration increased dramatically during a dust event in an urban atmosphere. Pollutant aerosols, including inorganic salts formed through secondary transformation (SIA) and black carbon (BC), might not act as effective INPs under mixed-phase cloud conditions.
Fritz Waitz, Martin Schnaiter, Thomas Leisner, and Emma Järvinen
Atmos. Chem. Phys., 22, 7087–7103, https://doi.org/10.5194/acp-22-7087-2022, https://doi.org/10.5194/acp-22-7087-2022, 2022
Short summary
Short summary
Riming, i.e., the accretion of small droplets on the surface of ice particles via collision, is one of the major uncertainties in model prediction of mixed-phase clouds. We discuss the occurrence (up to 50% of particles) and aging of rimed ice particles and show correlations of the occurrence and the degree of riming with ambient meteorological parameters using data gathered by the Particle Habit Imaging and Polar Scattering (PHIPS) probe during three airborne in situ field campaigns.
Zoé Brasseur, Dimitri Castarède, Erik S. Thomson, Michael P. Adams, Saskia Drossaart van Dusseldorp, Paavo Heikkilä, Kimmo Korhonen, Janne Lampilahti, Mikhail Paramonov, Julia Schneider, Franziska Vogel, Yusheng Wu, Jonathan P. D. Abbatt, Nina S. Atanasova, Dennis H. Bamford, Barbara Bertozzi, Matthew Boyer, David Brus, Martin I. Daily, Romy Fösig, Ellen Gute, Alexander D. Harrison, Paula Hietala, Kristina Höhler, Zamin A. Kanji, Jorma Keskinen, Larissa Lacher, Markus Lampimäki, Janne Levula, Antti Manninen, Jens Nadolny, Maija Peltola, Grace C. E. Porter, Pyry Poutanen, Ulrike Proske, Tobias Schorr, Nsikanabasi Silas Umo, János Stenszky, Annele Virtanen, Dmitri Moisseev, Markku Kulmala, Benjamin J. Murray, Tuukka Petäjä, Ottmar Möhler, and Jonathan Duplissy
Atmos. Chem. Phys., 22, 5117–5145, https://doi.org/10.5194/acp-22-5117-2022, https://doi.org/10.5194/acp-22-5117-2022, 2022
Short summary
Short summary
The present measurement report introduces the ice nucleation campaign organized in Hyytiälä, Finland, in 2018 (HyICE-2018). We provide an overview of the campaign settings, and we describe the measurement infrastructure and operating procedures used. In addition, we use results from ice nucleation instrument inter-comparison to show that the suite of these instruments deployed during the campaign reports consistent results.
Cited articles
Avramov, A., Ackerman, A. S., Fridlind, A. M., van Diedenhoven, B., Botta, G., Aydin, K., Verlinde, J., Korolev, A. V., Strapp, J. W., McFarquhar, G. M., Jackson, R., Brooks, S. D., Glen, A., and Wolde, M.: Toward ice formation closure in Arctic mixed-phase boundary layer clouds during ISDAC, J. Geophys. Res.-Atmos., 116, D00T08, https://doi.org/10.1029/2011JD015910, 2011.
Bailey, M. P. and Hallett, J.: Growth Rates and Habits of Ice Crystals between −20° and −70 °C, J. Atmos. Sci., 61, 514–544, 2004.
Bailey, M. P. and Hallett, J.: A Comprehensive Habit Diagram for Atmospheric Ice Crystals: Confirmation from the Laboratory, AIRS II, and Other Field Studies, J. Atmos. Sci., 66, 2888–2899, https://doi.org/10.1175/2009JAS2883.1, 2009.
Baker, B. and Lawson, R. P.: Improvement in determination of ice water content from two-dimensional particle imagery. Part I: Image-to-mass relationships, J. Appl. Meteorol. Clim., 45, 1282–1290, https://doi.org/10.1175/jam2398.1, 2006a.
Baker, B. A. and Lawson, R. P.: In Situ Observations of the Microphysical Properties of Wave, Cirrus, and Anvil Clouds. Part I: Wave Clouds, J. Atmos. Sci., 63, 3160–3185, 2006b.
Baran, A. J.: From the single-scattering properties of ice crystals to climate prediction: A way forward, Atmos. Res., 112, 45–69, https://doi.org/10.1016/j.atmosres.2012.04.010, 2012.
Brown, P. R. A. and Francis, P. N.: Improved measurements of the ice water content in cirrus using a total-water probe, J. Atmos. Ocean. Tech., 12, 410–414, https://doi.org/10.1175/1520-0426(1995)012<0410:imotiw>2.0.co;2, 1995.
Cotton, R. J., Field, P. R., Ulanowski, Z., Kaye, P. H., Hirst, E., Greenaway, R. S., Crawford, I., Crosier, J., and Dorsey, J.: The effective density of small ice particles obtained from in situ aircraft observations of mid-latitude cirrus, Q. J. Roy. Meteor. Soc., 139, 1923–1934, https://doi.org/10.1002/qj.2058, 2013.
Delanoe, J. and Hogan, R. J.: Combined CloudSat-CALIPSO-MODIS retrievals of the properties of ice clouds, J. Geophys. Res.-Atmos., 115, D00h29, https://doi.org/10.1029/2009jd012346, 2010.
Eidhammer, T., Morrison, H., Mitchell, D. L., Gettelman, A., and Erfani, E.: Improvements in the Community Atmosphere Model (CAM5) microphysics using a consistent representation of ice particle properties, J. Climate, accepted, 2016.
Fontaine, E., Schwarzenboeck, A., Delanoë, J., Wobrock, W., Leroy, D., Dupuy, R., Gourbeyre, C., and Protat, A.: Constraining mass–diameter relations from hydrometeor images and cloud radar reflectivities in tropical continental and oceanic convective anvils, Atmos. Chem. Phys., 14, 11367–11392, https://doi.org/10.5194/acp-14-11367-2014, 2014.
Foot, J. S.: Some observations of the optical properties of clouds. Part II: Cirrus, Q. J. Roy. Meteor. Soc., 114, 145–164, 1988.
Fu, Q.: An accurate parameterization of the solar radiative properties of cirrus clouds for climate models, J. Climate, 9, 2058–2082, https://doi.org/10.1175/1520-0442(1996)009<2058:aapots>2.0.co;2, 1996.
Fu, Q., Yang, P., and Sun, W. B.: An accurate parameterization of the infrared radiative properties of cirrus clouds for climate models, J. Climate, 11, 2223–2237, https://doi.org/10.1175/1520-0442(1998)011<2223:aapoti>2.0.co;2, 1998.
Gettelman, A., Liu, X., Ghan, S. J., Morrison, H., Park, S., Conley, A. J., Klein, S. A., Boyle, J., Mitchell, D. L., and Li, J. L. F.: Global simulations of ice nucleation and ice supersaturation with an improved cloud scheme in the Community Atmosphere Model, J. Geophys. Res.-Atmos., 115, D18216, https://doi.org/10.1029/2009jd013797, 2010.
Heymsfield, A. J. and Westbrook, C. D.: Advances in the Estimation of Ice Particle Fall Speeds Using Laboratory and Field Measurements, J. Atmos. Sci., 67, 2469–2482, https://doi.org/10.1175/2010jas3379.1, 2010.
Heymsfield, A. J., Lewis, S., Bansemer, A., Iaquinta, J., Miloshevich, L. M., Kajikawa, M., Twohy, C., and Poellot, M. R.: A general approach for deriving the properties of cirrus and stratiform ice cloud particles, J. Atmos. Sci., 59, 3–29, https://doi.org/10.1175/1520-0469(2002)059<0003:agafdt>2.0.co;2, 2002.
Heymsfield, A. J., Bansemer, A., Schmitt, C., Twohy, C., and Poellot, M. R.: Effective ice particle densities derived from aircraft data, J. Atmos. Sci., 61, 982–1003, https://doi.org/10.1175/1520-0469(2004)061<0982:eipddf>2.0.co;2, 2004.
Heymsfield, A. J., Bansemer, A., and Twohy, C. H.: Refinements to ice particle mass dimensional and terminal velocity relationships for ice clouds. Part I: Temperature dependence, J. Atmos. Sci., 64, 1047–1067, https://doi.org/10.1175/jas3890.1, 2007.
Heymsfield, A. J., Schmitt, C., Bansemer, A., and Twohy, C. H.: Improved Representation of Ice Particle Masses Based on Observations in Natural Clouds, J. Atmos. Sci., 67, 3303–3318, https://doi.org/10.1175/2010jas3507.1, 2010.
Jackson, R. C., McFarquhar, G. M., Korolev, A. V., Earle, M. E., Liu, P. S., Lawson, R. P., Brooks, S., Wolde, M., Laskin, A., and Freer, M.: The dependence of ice microphysics on aerosol concentration in arctic mixed-phase stratus clouds during ISDAC and M-PACE, J. Geophys. Res.-Atmos., 117, D15207, https://doi.org/10.1029/2012JD017668, 2012.
Jensen, E. J., Lawson, R. P., Bergman, J. W., Pfister, L., Bui, T. P., and Schmitt, C. G.: Physical processes controlling ice concentrations in synoptically forced, midlatitude cirrus, J. Geophys. Res.-Atmos., 118, 5348–5360, https://doi.org/10.1002/jgrd.50421, 2013.
Korolev, A.: Reconstruction of the sizes of spherical particles from their shadow images. Part I: Theoretical considerations, J. Atmos. Ocean. Tech., 24, 376–389, https://doi.org/10.1175/jtech1980.1, 2007.
Korolev, A. and Isaac, G.: Roundness and aspect ratio of particles in ice clouds, J. Atmos. Sci., 60, 1795–1808, https://doi.org/10.1175/1520-0469(2003)060<1795:raarop>2.0.co;2, 2003.
Korolev, A., Strapp, J. W., and Isaac, G. A.: Evaluation of the accuracy of PMS Optical Array Probes, J. Atmos. Ocean. Tech., 15, 708–720, https://doi.org/10.1175/1520-0426(1998)015<0708:eotaop>2.0.co;2, 1998.
Lamb, D. and Verlinde, J.: Physics and Chemistry of Clouds, Cambridge University Press, New York, NY, USA, 2011.
Lawson, R. P.: Effects of ice particles shattering on the 2D-S probe, Atmos. Meas. Tech., 4, 1361–1381, https://doi.org/10.5194/amt-4-1361-2011, 2011.
Lawson, R. P.: Improvement in Determination of Ice Water Content from Two-Dimensional Particle Imagery. Part III: Ice Particles with High a- to c-axis Ratio, J. Appl. Meteorol. Clim., submitted, 2016.
Lawson, R. P., Baker, B. A., Schmitt, C. G., and Jensen, T. L.: An overview of microphysical properties of Arctic clouds observed in May and July 1998 during FIRE ACE, J. Geophys. Res.-Atmos., 106, 14989–15014, https://doi.org/10.1029/2000jd900789, 2001.
Lawson, R. P., O'Connor, D., Zmarzly, P., Weaver, K., Baker, B., Mo, Q., and Jonsson, H.: The 2D-S (Stereo) probe: Design and preliminary tests of a new airborne, high-speed, high-resolution particle Imaging probe, J. Atmos. Ocean. Tech., 23, 1462–1477, https://doi.org/10.1175/jtech1927.1, 2006a.
Lawson, R. P., Baker, B. A., Pilson, B., and Mo, Q.: In situ observations of the microphysical properties of wave, cirrus and anvil clouds. Part II: Cirrus clouds, J. Atmos. Sci., 63, 3186–3203, 2006b.
Lawson, R. P., Jensen, E., Mitchell, D. L., Baker, B., Mo, Q., and Pilson, B.: Microphysical and radiative properties of tropical clouds investigated in TC4 and NAMMA, J. Geophys. Res.-Atmos., 115, D00j08, https://doi.org/10.1029/2009jd013017, 2010.
Locatelli, J. d. and Hobbs, P. V.: Fall speeds and masses of solid precipitation particles, J. Geophys. Res., 79, 2185–2197, https://doi.org/10.1029/JC079i015p02185, 1974.
Mace, J., Jensen, E., McFarquhar, G., Comstock, J., Ackerman, T., Mitchell, D., Liu, X., and Garrett, T.: SPARTICUS: Small Particles in Cirrus, Science and Operations Plan, Tech. Rep., DOE/SC-ARM-10-003, The Atmospheric Radiation Measurement Program, US Department of Energy, available at: https://www.arm.gov/publications/programdocs/doe-sc-arm-10-003.pdf (last access: 20 October 2015), 2009.
McFarquhar, G. M., Timlin, M. S., Rauber, R. M., Jewett, B. F., and Grim, J. A.: Vertical variability of cloud hydrometeors in the stratiform region of mesoscale convective systems and bow echoes, Mon. Weather Rev., 135, 3405–3428, https://doi.org/10.1175/mwr3444.1, 2007.
McFarquhar, G. M., Um, J., and Jackson, R.: Small Cloud Particle Shapes in Mixed-Phase Clouds, J. Appl. Meteor. Clim., 52, 1277–1293, https://doi.org/10.1175/JAMC-D-12-0114.1, 2013.
Mishra, S., Mitchell, D. L., Turner, D. D., and Lawson, R. P.: Parameterization of ice fall speeds in midlatitude cirrus: Results from SPartICus, J. Geophys. Res.-Atmos., 119, 3857–3876, https://doi.org/10.1002/2013jd020602, 2014.
Mitchell, D. L.: Evolution of snow-size spectra in cyclonic storms .1. snow growth by vapor-deposition and aggregation, J. Atmos. Sci., 45, 3431–3452, https://doi.org/10.1175/1520-0469(1988)045<3431:eosssi>2.0.co;2, 1988.
Mitchell, D. L.: Evolution of snow-size spectra in cyclonic storms. 2. deviations from the exponential form, J. Atmos. Sci., 48, 1885–1899, https://doi.org/10.1175/1520-0469(1991)048<1885:eosssi>2.0.co;2, 1991.
Mitchell, D. L.: Use of mass- and area-dimensional power laws for determining precipitation particle terminal velocities, J. Atmos. Sci., 53, 1710–1723, https://doi.org/10.1175/1520-0469(1996)053<1710:uomaad>2.0.co;2, 1996.
Mitchell, D. L.: Parameterization of the Mie extinction and absorption coefficients for water clouds, J. Atmos. Sci., 57, 1311–1326, https://doi.org/10.1175/1520-0469(2000)057<1311:potmea>2.0.co;2, 2000.
Mitchell, D. L.: Effective diameter in radiation transfer: General definition, applications, and limitations, J. Atmos. Sci., 59, 2330–2346, https://doi.org/10.1175/1520-0469(2002)059<2330:edirtg>2.0.co;2, 2002.
Mitchell, D. L., Zhang, R., and Pitter, R. L.: Mass-dimensional relationships for ice particles and the influence of riming on snowfall rates, J. Appl. Meteorol., 29, 153–163, https://doi.org/10.1175/1520-0450(1990)029<0153:mdrfip>2.0.co;2, 1990.
Mitchell, D. L., Baran, A. J., Arnott, W. P., and Schmitt, C.: Testing and comparing the modified anomalous diffraction approximation, J. Atmos. Sci., 63, 2948–2962, https://doi.org/10.1175/jas3775.1, 2006.
Mitchell, D. L., Rasch, P., Ivanova, D., McFarquhar, G., and Nousiainen, T.: Impact of small ice crystal assumptions on ice sedimentation rates in cirrus clouds and GCM simulations, Geophys. Res. Lett., 35, L09806, https://doi.org/10.1029/2008gl033552, 2008.
Mitchell, D. L., Mishra, S., and Lawson, R. P.: Representing the ice fall speed in climate models: Results from Tropical Composition, Cloud and Climate Coupling (TC4) and the Indirect and Semi-Direct Aerosol Campaign (ISDAC), J. Geophys. Res.-Atmos., 116, D00t03, https://doi.org/10.1029/2010jd015433, 2011.
Morrison, H. and Gettelman, A.: A new two-moment bulk stratiform cloud microphysics scheme in the community atmosphere model, version 3 (CAM3). Part I: Description and numerical tests, J. Climate, 21, 3642–3659, https://doi.org/10.1175/2008jcli2105.1, 2008.
Pruppacher, H. R. and Klett, J. D.: Microphysics of clouds and precipitation: 2nd Edn., Kluwer Academic Publishers, Dordrecht, the Netherlands, 1996.
Sanderson, B. M., Piani, C., Ingram, W. J., Stone, D. A., and Allen, M. R.: Towards constraining climate sensitivity by linear analysis of feedback patterns in thousands of perturbed-physics GCM simulations, Clim. Dynam., 30, 175–190, https://doi.org/10.1007/s00382-007-0280-7, 2008.
Um, J. and McFarquhar, G. M.: Dependence of the single-scattering properties of small ice crystals on idealized shape models, Atmos. Chem. Phys., 11, 3159–3171, https://doi.org/10.5194/acp-11-3159-2011, 2011.
Yang, P., Wei, H. L., Huang, H. L., Baum, B. A., Hu, Y. X., Kattawar, G. W., Mishchenko, M. I., and Fu, Q.: Scattering and absorption property database for nonspherical ice particles in the near- through far-infrared spectral region, Appl. Optics, 44, 5512–5523, https://doi.org/10.1364/ao.44.005512, 2005.
Zhao, Y., Mace, G. G., and Comstock, J. M.: The Occurrence of Particle Size Distribution Bimodality in Midlatitude Cirrus as Inferred from Ground-Based Remote Sensing Data, J. Atmos. Sci., 68, 1162–1177, https://doi.org/10.1175/2010jas3354.1, 2011.
Short summary
Ice particle projected area- and mass-dimension expressions are developed and validated, and uncertainties for power laws derived from these expressions are determined.
Ice particle projected area- and mass-dimension expressions are developed and validated, and...
Altmetrics
Final-revised paper
Preprint