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Volume 15, issue 4
Atmos. Chem. Phys., 15, 1621–1632, 2015
https://doi.org/10.5194/acp-15-1621-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.

Special issue: Interactions between climate change and the Cryosphere: SVALI,...

Atmos. Chem. Phys., 15, 1621–1632, 2015
https://doi.org/10.5194/acp-15-1621-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 16 Feb 2015

Research article | 16 Feb 2015

Deposition-mode ice nucleation reexamined at temperatures below 200 K

E. S. Thomson et al.

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Cited articles

Adamson, A. and Gast, A.: Physical Chemistry of Surfaces, Wiley, New York, NY, 784 pp., 1997.
Allouche, A. and Bahr, S.: Acetic Acid–Water Interaction in Solid Interfaces, J. Phys. Chem. B, 110, 8640–8648, https://doi.org/10.1021/jp0559736, 2006.
Andersson, P. U., Suter, M. T., Marković, N., and Pettersson, J. B. C.: Water condensation on graphite studied by elastic helium scattering and molecular dynamics simulations, J. Phys. Chem. C, 111, 15258–15266, 2007.
Chen, J.-P., Hazra, A., and Levin, Z.: Parameterizing ice nucleation rates using contact angle and activation energy derived from laboratory data, Atmos. Chem. Phys., 8, 7431–7449, https://doi.org/10.5194/acp-8-7431-2008, 2008.
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We present new observations of ice nucleation on substrate surfaces that affirm the ``puzzle'' of very high supersaturations required for nucleation from the vapor phase. To explain the observations, the kinetics and thermodynamics of nucleation theory are explored. The results explicitly connect the nucleation to the substrate material's surface binding energy and demonstrate that an improved fundamental understanding must include a strict understanding of the relevant microphysics.
We present new observations of ice nucleation on substrate surfaces that affirm the ``puzzle''...
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