Articles | Volume 23, issue 16
https://doi.org/10.5194/acp-23-9229-2023
https://doi.org/10.5194/acp-23-9229-2023
Measurement report
 | 
22 Aug 2023
Measurement report |  | 22 Aug 2023

Measurement report: Assessment of Asian emissions of ethane and propane with a chemistry transport model based on observations from the island of Hateruma

Adedayo R. Adedeji, Stephen J. Andrews, Matthew J. Rowlinson, Mathew J. Evans, Alastair C. Lewis, Shigeru Hashimoto, Hitoshi Mukai, Hiroshi Tanimoto, Yasunori Tohjima, and Takuya Saito

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Cited articles

Adedeji, A. R., Andrews, S. J., Evans, M. J., Lewis, A. C., and Saito, T.: GEOS-Chem model output for surface atmospheric compositions over East Asia, National Institute for Environmental Studies [data set], Japan, https://doi.org/10.17595/20230707.001, 2023. a
Akagi, S. K., Yokelson, R. J., Wiedinmyer, C., Alvarado, M. J., Reid, J. S., Karl, T., Crounse, J. D., and Wennberg, P. O.: Emission factors for open and domestic biomass burning for use in atmospheric models, Atmos. Chem. Phys., 11, 4039–4072, https://doi.org/10.5194/acp-11-4039-2011, 2011. a
Andreae, M. O. and Merlet, P.: Emission of trace gases and aerosols from biomass burning, Global Biogeochem. Cy., 15, 955–966, https://doi.org/10.1029/2000GB001382, 2001. a
Bey, I., Jacob, D. J., Yantosca, R. M., Logan, J. A., Field, B. D., Fiore, A. M., Li, Q., Liu, H. Y., Mickley, L. J., and Schultz, M. G.: Global modeling of tropospheric chemistry with assimilated meteorology: Model description and evaluation, J. Geophys. Res-.Atmos., 106, 23073–23095, https://doi.org/10.1029/2001JD000807, 2001. a
Bouwman, A. F., Lee, D. S., Asman, W. A. H., Dentener, F. J., Van Der Hoek, K. W., and Olivier, J. G. J.: A global high-resolution emission inventory for ammonia, Global Biogeochem. Cy., 11, 561–587, https://doi.org/10.1029/97GB02266, 1997. a
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We use the GEOS-Chem model to interpret observations of CO, C2H6, C3H8, NOx, NOy and O3 made from Hateruma Island in 2018. The model captures many synoptic-scale events and the seasonality of most pollutants at the site but underestimates C2H6 and C3H8 during the winter. These underestimates are unlikely to be reconciled by increases in biomass burning emissions but could be reconciled by increasing the Asian anthropogenic source of C2H6 and C3H8 by factors of around 2 and 3, respectively.
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