Articles | Volume 22, issue 10
https://doi.org/10.5194/acp-22-6899-2022
https://doi.org/10.5194/acp-22-6899-2022
Research article
 | 
30 May 2022
Research article |  | 30 May 2022

Towards reconstructing the Arctic atmospheric methane history over the 20th century: measurement and modelling results for the North Greenland Ice Core Project firn

Taku Umezawa, Satoshi Sugawara, Kenji Kawamura, Ikumi Oyabu, Stephen J. Andrews, Takuya Saito, Shuji Aoki, and Takakiyo Nakazawa

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Cited articles

Aoki, S., Nakazawa, T., Murayama, S., and Kawaguchi, S.: Measurements of atmospheric methane at the Japanese Antarctic Station, Syowa, Tellus B, 44, 273–281, https://doi.org/10.1034/j.1600-0889.1992.t01-3-00005.x, 1992. 
Blunier, T., Chappellaz, J. A., Schwander, J., Barnola, J.-M., Desperts, T., Stauffer, B., and Raynaud D.: Atmospheric methane, record from a Greenland Ice Core over the last 1000 year, Geophys. Res. Lett., 20, 2219–2222, https://doi.org/10.1029/93GL02414, 1993. 
Chandra, N., Patra, P. K., Bisht, J. S. H., Ito, A., Umezawa, T., Saigusa, N., Morimoto, S., Aoki, S., Janssens-Maenhout, G., Fujita, R., Takigawa, M., Watanabe, S., Saitoh, N., and Canadell, J. G.: Emissions from the oil and gas sectors, coal mining and ruminant farming drive methane growth over the past three decades, J. Meteorol. Soci. Jpn., 99, 309–337, https://doi.org/10.2151/jmsj.2021-015, 2021. 
Dlugokencky, E. J., Houweling, S., Bruhwiler, L., Masarie, K. A., Lang, P. M., Miller, J. B., and Tans P. P.: Atmospheric methane levels off: Temporary pause or a new steady-state?, Geophys. Res. Lett., 30, 1992, https://doi.org/10.1029/2003GL018126, 2003. 
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Greenhouse gas methane in the Arctic atmosphere has not been accurately reported for 1900–1980 from either direct observations or ice core reconstructions. By using trace gas data from firn (compacted snow layers above ice sheet), air samples at two Greenland sites, and a firn air transport model, this study suggests a likely range of the Arctic methane reconstruction for the 20th century. Atmospheric scenarios from two previous studies are also evaluated for consistency with the firn data sets.
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