Articles | Volume 20, issue 17
https://doi.org/10.5194/acp-20-10707-2020
https://doi.org/10.5194/acp-20-10707-2020
Research article
 | 
11 Sep 2020
Research article |  | 11 Sep 2020

Attribution of ground-level ozone to anthropogenic and natural sources of nitrogen oxides and reactive carbon in a global chemical transport model

Tim Butler, Aurelia Lupascu, and Aditya Nalam

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Cited articles

Aksoyoglu, S., Baltensperger, U., and Prévôt, A. S. H.: Contribution of ship emissions to the concentration and deposition of air pollutants in Europe, Atmos. Chem. Phys., 16, 1895–1906, https://doi.org/10.5194/acp-16-1895-2016, 2016. a
Andersson, C. and Engardt, M.: European ozone in a future climate: Importance of changes in dry deposition and isoprene emissions, J. Geophys. Res., 115, D02303, https://doi.org/10.1029/2008jd011690, 2010. a
Atkinson, R.: Atmospheric chemistry of VOCs and NOx, Atmos. Environ., 34, 2063–2101, 2000. a, b, c, d, e
Bates, K. H. and Jacob, D. J.: An Expanded Definition of the Odd Oxygen Family for Tropospheric Ozone Budgets: Implications for Ozone Lifetime and Stratospheric Influence, Geophys. Res. Lett., 47, e2019GL084486, https://doi.org/10.1029/2019gl084486, 2020. a, b
Beck, J. P., Reeves, C. E., de Leeuw, F. A., and Penkett, S. A.: The effect of aircraft emissions on tropospheric ozone in the northern hemisphere, Atmos. Environ. Part A.-Gen., 26, 17–29, https://doi.org/10.1016/0960-1686(92)90257-l, 1992. a, b
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Ground-level ozone (O3) is not directly emitted; it is formed chemically in the atmosphere. Some ground-level O3 is transported from the stratosphere, but most O3 is produced from reactive precursors that are emitted by both natural and anthropogenic sources. We present the results of a novel source apportionment method for ground-level O3. Our results are consistent with previous work and also provide new insights. In particular, we highlight the roles of methane and international shipping.
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