Articles | Volume 18, issue 18
https://doi.org/10.5194/acp-18-13531-2018
https://doi.org/10.5194/acp-18-13531-2018
Research article
 | 
25 Sep 2018
Research article |  | 25 Sep 2018

Improving air quality model predictions of organic species using measurement-derived organic gaseous and particle emissions in a petrochemical-dominated region

Craig A. Stroud, Paul A. Makar, Junhua Zhang, Michael D. Moran, Ayodeji Akingunola, Shao-Meng Li, Amy Leithead, Katherine Hayden, and May Siu

Related authors

Impact of the Atmospheric Boundary Layer Height on the Concentration of Chemical Species in Numerical Model Simulations
Shuzhan Ren and Craig A. Stroud
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2023-37,https://doi.org/10.5194/acp-2023-37, 2023
Revised manuscript not accepted
Short summary
Development of aerosol optical properties for improving the MESSy photolysis module in the GEM-MACH v2.4 air quality model and application for calculating photolysis rates in a biomass burning plume
Mahtab Majdzadeh, Craig A. Stroud, Christopher Sioris, Paul A. Makar, Ayodeji Akingunola, Chris McLinden, Xiaoyi Zhao, Michael D. Moran, Ihab Abboud, and Jack Chen
Geosci. Model Dev., 15, 219–249, https://doi.org/10.5194/gmd-15-219-2022,https://doi.org/10.5194/gmd-15-219-2022, 2022
Short summary
Vehicle-induced turbulence and atmospheric pollution
Paul A. Makar, Craig Stroud, Ayodeji Akingunola, Junhua Zhang, Shuzhan Ren, Philip Cheung, and Qiong Zheng
Atmos. Chem. Phys., 21, 12291–12316, https://doi.org/10.5194/acp-21-12291-2021,https://doi.org/10.5194/acp-21-12291-2021, 2021
Short summary
Forest-fire aerosol–weather feedbacks over western North America using a high-resolution, online coupled air-quality model
Paul A. Makar, Ayodeji Akingunola, Jack Chen, Balbir Pabla, Wanmin Gong, Craig Stroud, Christopher Sioris, Kerry Anderson, Philip Cheung, Junhua Zhang, and Jason Milbrandt
Atmos. Chem. Phys., 21, 10557–10587, https://doi.org/10.5194/acp-21-10557-2021,https://doi.org/10.5194/acp-21-10557-2021, 2021
Short summary
Elucidating real-world vehicle emission factors from mobile measurements over a large metropolitan region: a focus on isocyanic acid, hydrogen cyanide, and black carbon
Sumi N. Wren, John Liggio, Yuemei Han, Katherine Hayden, Gang Lu, Cris M. Mihele, Richard L. Mittermeier, Craig Stroud, Jeremy J. B. Wentzell, and Jeffrey R. Brook
Atmos. Chem. Phys., 18, 16979–17001, https://doi.org/10.5194/acp-18-16979-2018,https://doi.org/10.5194/acp-18-16979-2018, 2018
Short summary

Related subject area

Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Population exposure to outdoor NO2, black carbon, and ultrafine and fine particles over Paris with multi-scale modelling down to the street scale
Soo-Jin Park, Lya Lugon, Oscar Jacquot, Youngseob Kim, Alexia Baudic, Barbara D'Anna, Ludovico Di Antonio, Claudia Di Biagio, Fabrice Dugay, Olivier Favez, Véronique Ghersi, Aline Gratien, Julien Kammer, Jean-Eudes Petit, Olivier Sanchez, Myrto Valari, Jérémy Vigneron, and Karine Sartelet
Atmos. Chem. Phys., 25, 3363–3387, https://doi.org/10.5194/acp-25-3363-2025,https://doi.org/10.5194/acp-25-3363-2025, 2025
Short summary
Predicted impacts of heterogeneous chemical pathways on particulate sulfur over Fairbanks (Alaska), the Northern Hemisphere, and the Contiguous United States
Sara L. Farrell, Havala O. T. Pye, Robert Gilliam, George Pouliot, Deanna Huff, Golam Sarwar, William Vizuete, Nicole Briggs, Fengkui Duan, Tao Ma, Shuping Zhang, and Kathleen Fahey
Atmos. Chem. Phys., 25, 3287–3312, https://doi.org/10.5194/acp-25-3287-2025,https://doi.org/10.5194/acp-25-3287-2025, 2025
Short summary
Critical load exceedances for North America and Europe using an ensemble of models and an investigation of causes of environmental impact estimate variability: an AQMEII4 study
Paul A. Makar, Philip Cheung, Christian Hogrefe, Ayodeji Akingunola, Ummugulsum Alyuz, Jesse O. Bash, Michael D. Bell, Roberto Bellasio, Roberto Bianconi, Tim Butler, Hazel Cathcart, Olivia E. Clifton, Alma Hodzic, Ioannis Kioutsioukis, Richard Kranenburg, Aurelia Lupascu, Jason A. Lynch, Kester Momoh, Juan L. Perez-Camanyo, Jonathan Pleim, Young-Hee Ryu, Roberto San Jose, Donna Schwede, Thomas Scheuschner, Mark W. Shephard, Ranjeet S. Sokhi, and Stefano Galmarini
Atmos. Chem. Phys., 25, 3049–3107, https://doi.org/10.5194/acp-25-3049-2025,https://doi.org/10.5194/acp-25-3049-2025, 2025
Short summary
Impacts of meteorology and emission reductions on haze pollution during the lockdown in the North China Plain
Lang Liu, Xin Long, Yi Li, Zengliang Zang, Fengwen Wang, Yan Han, Zhier Bao, Yang Chen, Tian Feng, and Jinxin Yang
Atmos. Chem. Phys., 25, 1569–1585, https://doi.org/10.5194/acp-25-1569-2025,https://doi.org/10.5194/acp-25-1569-2025, 2025
Short summary
Impact of mineral dust on the global nitrate aerosol direct and indirect radiative effect
Alexandros Milousis, Klaus Klingmüller, Alexandra P. Tsimpidi, Jasper F. Kok, Maria Kanakidou, Athanasios Nenes, and Vlassis A. Karydis
Atmos. Chem. Phys., 25, 1333–1351, https://doi.org/10.5194/acp-25-1333-2025,https://doi.org/10.5194/acp-25-1333-2025, 2025
Short summary

Cited articles

Barsanti, K. C., Carlton, A. G., and Chung, S. H.: Analyzing experimental data and model parameters: implications for predictions of SOA using chemical transport models, Atmos. Chem. Phys., 13, 12073–12088, https://doi.org/10.5194/acp-13-12073-2013, 2013.
Cappa, C. D. and Jimenez, J. L.: Quantitative estimates of the volatility of ambient organic aerosol, Atmos. Chem. Phys., 10, 5409–5424, https://doi.org/10.5194/acp-10-5409-2010, 2010.
Cappa, C. D. and Wilson, K. R.: Evolution of organic aerosol mass spectra upon heating: implications for OA phase and partitioning behavior, Atmos. Chem. Phys., 11, 1895–1911, https://doi.org/10.5194/acp-11-1895-2011, 2011.
Chai, T., Kim, H.-C., Lee, P., Tong, D., Pan, L., Tang, Y., Huang, J., McQueen, J., Tsidulko, M., and Stajner, I.: Evaluation of the United States National Air Quality Forecast Capability experimental real-time predictions in 2010 using Air Quality System ozone and NO2 measurements, Geosci. Model Dev., 6, 1831–1850, https://doi.org/10.5194/gmd-6-1831-2013, 2013.
Cho, S., McEachern, P., Morris, R., Shah, T., Johnson, J., and Nopmongcol, U.: Emission sources sensitivity study for ground-level ozone and PM2.5 due to oil sands development using air quality modeling system: Part I – model evaluation for current year base case simulation, Atmos. Environ., 55, 533–541, 2012.
Download
Short summary
It is shown that using measurement-derived volatile organic compound (VOC) and organic aerosol (OA) emissions in the GEM-MACH air quality model provides better overall predictions compared to using bottom-up emission inventories. This work was done to better constrain the fugitive organic emissions from the Athabasca oil sands region, which are a challenge to estimate with bottom-up emission approaches. We use observations from the 2013 Joint Oil Sands Monitoring study.
Share
Altmetrics
Final-revised paper
Preprint