Articles | Volume 15, issue 6
https://doi.org/10.5194/acp-15-3497-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-3497-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
31 Mar 2015
Research article |
| 31 Mar 2015
Aerosol processing and CCN formation of an intense Saharan dust plume during the EUCAARI 2008 campaign
N. Bègue
Laboratoire de l'Atmosphère et des Cyclones, UMR 8105 CNRS, University of Réunion Island, Reunion Island, France
Laboratoire de l'Atmosphère et des Cyclones, UMR 8105 CNRS, University of Réunion Island, Reunion Island, France
J. Pelon
Laboratoire Atmosphère Milieux Observations Spatiales, University of Paris VI, Paris, France
B. Aouizerats
Faculty of Earth and Life Sciences, VU University Amsterdam, Amsterdam, the Netherlands
A. Berger
Laboratoire d'Aérologie, University of Paul Sabatier, CNRS, Toulouse, France
A. Schwarzenboeck
Laboratoire de Météorologie Physique, CNRS, UMR 6016 University Blaise-Pascal, Clermont-Ferrand, France
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Dominique Gantois, Guillaume Payen, Michaël Sicard, Valentin Duflot, Nelson Bègue, Nicolas Marquestaut, Thierry Portafaix, Sophie Godin-Beekmann, Patrick Hernandez, and Eric Golubic
Earth Syst. Sci. Data, 16, 4137–4159, https://doi.org/10.5194/essd-16-4137-2024, https://doi.org/10.5194/essd-16-4137-2024, 2024
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We describe three instruments that have been measuring interactions between aerosols (particles of various origin) and light over Réunion Island since 2012. Aerosols directly or indirectly influence the temperature in the atmosphere and can interact with clouds. Details are given on how we derived aerosol properties from our measurements and how we assessed the quality of our data before sharing them with the scientific community. A good correlation was found between the three instruments.
Gabriela Dornelles Bittencourt, Hassan Bencherif, Damaris Kirsch Pinheiro, Nelson Begue, Lucas Vaz Peres, José Valentin Bageston, Douglas Lima de Bem, Francisco Raimundo da Silva, and Tristan Millet
Atmos. Meas. Tech., 17, 5201–5220, https://doi.org/10.5194/amt-17-5201-2024, https://doi.org/10.5194/amt-17-5201-2024, 2024
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The study examines the behavior of ozone at equatorial and subtropical latitudes in South America, in a multi-instrumental analysis. The methodology applied used ozonesondes (SHADOZ/NASA) and satellite data (TIMED/SABER), as well as analysis with ground-based and satellite instruments, allowing a more in-depth study at both latitudes. The main motivation is to understand how latitudinal differences in the observation of ozone content can interfere with the behavior of this trace gas.
Tristan Millet, Hassan Bencherif, Thierry Portafaix, Nelson Bègue, Alexandre Baron, Valentin Duflot, Cathy Clerbaux, Pierre-François Coheur, Andrea Pazmino, Michaël Sicard, Jean-Marc Metzger, Guillaume Payen, Nicolas Marquestaut, and Sophie Godin-Beekmann
EGUsphere, https://doi.org/10.5194/egusphere-2024-2350, https://doi.org/10.5194/egusphere-2024-2350, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
On 15 January 2022, the Hunga volcano erupted, releasing aerosols, sulfur dioxide, and water vapor into the stratosphere, impacting ozone levels over the Indian Ocean. MLS and IASI data show that the volcanic plume decreased ozone levels within the stratospheric ozone layer, shaping a structure similar to an ozone mini-hole. A stable stratosphere, free of dynamical barriers, enabled the volcanic plume's transport over the Indian Ocean.
Nelson Bègue, Alexandre Baron, Gisèle Krysztofiak, Gwenaël Berthet, Corinna Kloss, Fabrice Jégou, Sergey Khaykin, Marion Ranaivombola, Tristan Millet, Thierry Portafaix, Valentin Duflot, Philippe Keckhut, Hélène Vérèmes, Guillaume Payen, Mahesh Kumar Sha, Pierre-François Coheur, Cathy Clerbaux, Michaël Sicard, Tetsu Sakai, Richard Querel, Ben Liley, Dan Smale, Isamu Morino, Osamu Uchino, Tomohiro Nagai, Penny Smale, John Robinson, and Hassan Bencherif
Atmos. Chem. Phys., 24, 8031–8048, https://doi.org/10.5194/acp-24-8031-2024, https://doi.org/10.5194/acp-24-8031-2024, 2024
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During the 2020 austral summer, the pristine atmosphere of the southwest Indian Ocean basin experienced significant perturbations. Numerical models indicated that the lower-stratospheric aerosol content was influenced by the intense and persistent stratospheric aerosol layer generated during the 2019–2020 extreme Australian bushfire events. Ground-based observations at Réunion confirmed the simultaneous presence of African and Australian aerosol layers.
Michael Sicard, Alexandre Baron, Marion Ranaivombola, Dominique Gantois, Tristan Millet, Pasquale Sellitto, Nelson Bègue, Hassan Bencherif, Guillaume Payen, Nicolas Marquestaut, and Valentin Duflot
EGUsphere, https://doi.org/10.22541/essoar.170231679.99186200/v1, https://doi.org/10.22541/essoar.170231679.99186200/v1, 2024
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This study quantifies the radiative impact over Reunion Island (21° S, 55° E) of the aerosols and water vapor injected in the stratosphere by the Hunga Tonga-Hunga Ha'apai volcano in the South Pacific. The overall aerosol and water vapor impact on the Earth’s radiation budget for the whole period is negative (cooling, -0.54 ± 0.29 W m-2) and dominated by the aerosols. At the Earth’s surface, aerosols are the main driver and produce a negative (cooling, -1.19 ± 0.40 W m-2) radiative impact.
Marion Ranaivombola, Nelson Bègue, Farahnaz Fazel-Rastgar, Venkataraman Sivakumar, Gisèle Krysztofiak, Gwenaël Berthet, Fabrice Jegou, Stuart Piketh, and Hassan Bencherif
EGUsphere, https://doi.org/10.5194/egusphere-2024-921, https://doi.org/10.5194/egusphere-2024-921, 2024
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From September to October 2022, the Biomass Burning Aerosol Campaign (BiBAC) in Kruger National Park revealed a significant aerosol loading linked to biomass burning activity, with a southeastward transport over Southern Africa and the southwestern of Indian Ocean (SWIO) basin. The "river of smoke" phenomenon drove the plume during September toward the SWIO. One discusses the long-range transport of biomass burning from South America to Southern Africa is likely driven by climate forcings.
Tristan Millet, Hassan Bencherif, Thierry Portafaix, Nelson Bègue, Alexandre Baron, Valentin Duflot, Michaël Sicard, Jean-Marc Metzger, Guillaume Payen, Nicolas Marquestaut, and Sophie Godin-Beekmann
EGUsphere, https://doi.org/10.5194/egusphere-2023-2645, https://doi.org/10.5194/egusphere-2023-2645, 2023
Preprint withdrawn
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The eruption of the Hunga Tonga volcano in January 2022 released substantial amounts of aerosols, sulfur dioxide, and water vapor into the stratosphere. Satellite and ground instruments followed the displacement of the volcanic aerosol plume and its impact on ozone levels over the Indian Ocean. Ozone data reveal the presence of a persistent ozone mini-hole structure from 17 January to 22 January, with most ozone depletion occurring within the ozone layer at the location of the aerosol plume.
Gabriela Dornelles Bittencourt, Damaris Kirsch Pinheiro, Hassan Bencherif, Lucas Vaz Peres, Nelson Begue, José Valentin Bageston, Douglas Lima de Bem, Vagner Anabor, and Luiz Angelo Steffenel
EGUsphere, https://doi.org/10.5194/egusphere-2023-1471, https://doi.org/10.5194/egusphere-2023-1471, 2023
Preprint archived
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The study examines ozone depletions at mid-latitudes in Brazil during austral spring Antarctic Ozone Hole influence events. The methodology applied used data from the total column ozone, vertical profile of the atmosphere, and reanalysis data to analyze the atmospheric dynamics. The main motivation of this work is to show how this important trace gas dynamically behaves in the atmosphere in the active period of the Antarctic Ozone Hole in regions of medium latitudes.
Nelson Bègue, Lerato Shikwambana, Hassan Bencherif, Juan Pallotta, Venkataraman Sivakumar, Elian Wolfram, Nkanyiso Mbatha, Facundo Orte, David Jean Du Preez, Marion Ranaivombola, Stuart Piketh, and Paola Formenti
Ann. Geophys., 38, 395–420, https://doi.org/10.5194/angeo-38-395-2020, https://doi.org/10.5194/angeo-38-395-2020, 2020
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This study investigates the influence of the 2015 Calbuco eruption (41.2°S, 72.4°W; Chile) on the total columnar aerosol optical properties in the Southern Hemisphere. The well-known technique of sun photometry was applied to the investigation of the transport and the spatio-temporal evolution of the optical properties of the volcanic plume. The CIMEL sun photometer measurements performed over six South American and three African sites were statistically analyzed.
Corinna Kloss, Gwenaël Berthet, Pasquale Sellitto, Felix Ploeger, Silvia Bucci, Sergey Khaykin, Fabrice Jégou, Ghassan Taha, Larry W. Thomason, Brice Barret, Eric Le Flochmoen, Marc von Hobe, Adriana Bossolasco, Nelson Bègue, and Bernard Legras
Atmos. Chem. Phys., 19, 13547–13567, https://doi.org/10.5194/acp-19-13547-2019, https://doi.org/10.5194/acp-19-13547-2019, 2019
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With satellite measurements and transport models, we show that a plume resulting from strong Canadian fires in July/August 2017 was not only distributed throughout the northern/higher latitudes, but also reached the faraway tropics, aided by the circulation of Asian monsoon anticyclone. The regional climate impact in the wider Asian monsoon area in September exceeds the impact of the Asian tropopause aerosol layer by a factor of ~ 3 and compares to that of an advected moderate volcanic eruption.
Pablo Facundo Orte, Elian Wolfram, Jacobo Salvador, Akira Mizuno, Nelson Bègue, Hassan Bencherif, Juan Lucas Bali, Raúl D'Elia, Andrea Pazmiño, Sophie Godin-Beekmann, Hirofumi Ohyama, and Jonathan Quiroga
Ann. Geophys., 37, 613–629, https://doi.org/10.5194/angeo-37-613-2019, https://doi.org/10.5194/angeo-37-613-2019, 2019
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We analysed an event of short-term ozone variability due to the passage of the polar vortex over Río Gallegos (southern Argentina) with the aim of highlighting the capability of a millimetre-wave radiometer to observe ozone in the stratosphere and the low mesosphere with a high temporal resolution. It is particularly important in this subpolar region due to the high variation that this gas can suffer as a consequence of the passage of the polar vortex and the ozone hole during spring.
David J. du Preez, Jelena V. Ajtić, Hassan Bencherif, Nelson Bègue, Jean-Maurice Cadet, and Caradee Y. Wright
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Reduced atmospheric ozone results in increased solar ultraviolet radiation (UVR) at the surface which may potentially negative impact public health. We aimed to assess whether or not the break-up of the Antarctic ozone hole had an impact on ozone and UVR at Cape Point (South Africa). We found a moderate inverse relationship between ozone and UVR at midday on clear-sky days. The Antarctic ozone hole had a limited effect on ozone levels while tropical air masses more frequently affected the site.
Abdoulwahab Mohamed Toihir, Thierry Portafaix, Venkataraman Sivakumar, Hassan Bencherif, Andréa Pazmiño, and Nelson Bègue
Ann. Geophys., 36, 381–404, https://doi.org/10.5194/angeo-36-381-2018, https://doi.org/10.5194/angeo-36-381-2018, 2018
Nelson Bègue, Damien Vignelles, Gwenaël Berthet, Thierry Portafaix, Guillaume Payen, Fabrice Jégou, Hassan Benchérif, Julien Jumelet, Jean-Paul Vernier, Thibaut Lurton, Jean-Baptiste Renard, Lieven Clarisse, Vincent Duverger, Françoise Posny, Jean-Marc Metzger, and Sophie Godin-Beekmann
Atmos. Chem. Phys., 17, 15019–15036, https://doi.org/10.5194/acp-17-15019-2017, https://doi.org/10.5194/acp-17-15019-2017, 2017
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The space–time evolutions of the Calbuco plume are investigated by combining satellite, in situ aerosol counting and lidar observations, and a numerical model. All the data at Reunion Island reveal a twofold increase in the amount of aerosol with respect to the values observed before the eruption. The dynamic context has favored the spread of the plume exclusively in the Southern Hemisphere. This study highlights the role played by dynamical barriers in the transport of atmospheric species.
Nelson Bègue, Nkanyiso Mbatha, Hassan Bencherif, René Tato Loua, Venkataraman Sivakumar, and Thierry Leblanc
Ann. Geophys., 35, 1177–1194, https://doi.org/10.5194/angeo-35-1177-2017, https://doi.org/10.5194/angeo-35-1177-2017, 2017
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In this investigation a statistical analysis of the characteristics of mesospheric inversion layers (MILs) over tropical regions is presented. This study involves the analysis of 16 years of lidar observations recorded at Reunion (20.8° S, 55.5° E) and 21 years of lidar observations recorded at Mauna Loa (19.5° N, 155.6° W) together with SABER observations at these two locations. Results presented in this study confirm that SAO contributes to the formation of MILs over the tropical region.
Gwenaël Berthet, Fabrice Jégou, Valéry Catoire, Gisèle Krysztofiak, Jean-Baptiste Renard, Adam E. Bourassa, Doug A. Degenstein, Colette Brogniez, Marcel Dorf, Sebastian Kreycy, Klaus Pfeilsticker, Bodo Werner, Franck Lefèvre, Tjarda J. Roberts, Thibaut Lurton, Damien Vignelles, Nelson Bègue, Quentin Bourgeois, Daniel Daugeron, Michel Chartier, Claude Robert, Bertrand Gaubicher, and Christophe Guimbaud
Atmos. Chem. Phys., 17, 2229–2253, https://doi.org/10.5194/acp-17-2229-2017, https://doi.org/10.5194/acp-17-2229-2017, 2017
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Since the last major volcanic event, i.e. the Pinatubo eruption in 1991, only
moderateeruptions have regularly injected sulfur into the stratosphere, typically enhancing the aerosol loading for several months. We investigate here for the first time the chemical perturbation associated with the Sarychev eruption in June 2009, using balloon-borne instruments and model calculations. Some chemical compounds are significantly affected by the aerosols, but the impact on stratospheric ozone is weak.
Lucas Vaz Peres, Hassan Bencherif, Nkanyiso Mbatha, André Passaglia Schuch, Abdoulwahab Mohamed Toihir, Nelson Bègue, Thierry Portafaix, Vagner Anabor, Damaris Kirsch Pinheiro, Neusa Maria Paes Leme, José Valentin Bageston, and Nelson Jorge Schuch
Ann. Geophys., 35, 25–37, https://doi.org/10.5194/angeo-35-25-2017, https://doi.org/10.5194/angeo-35-25-2017, 2017
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In this paper, we analyze the total ozone column over the Southern Space Observatory, Brazil, between 1992 and 2014 by Brewer spectrometer and TOMS and OMI satellite instruments, finding good agreement between the two. In addition, the seasonal TOC variation is dominated by an annual cycle, and the Quasi-Biennial Oscillation modulation was the main mode of interannual variability and in opposite phase to the total ozone column anomaly time series.
Dominique Gantois, Guillaume Payen, Michaël Sicard, Valentin Duflot, Nelson Bègue, Nicolas Marquestaut, Thierry Portafaix, Sophie Godin-Beekmann, Patrick Hernandez, and Eric Golubic
Earth Syst. Sci. Data, 16, 4137–4159, https://doi.org/10.5194/essd-16-4137-2024, https://doi.org/10.5194/essd-16-4137-2024, 2024
Short summary
Short summary
We describe three instruments that have been measuring interactions between aerosols (particles of various origin) and light over Réunion Island since 2012. Aerosols directly or indirectly influence the temperature in the atmosphere and can interact with clouds. Details are given on how we derived aerosol properties from our measurements and how we assessed the quality of our data before sharing them with the scientific community. A good correlation was found between the three instruments.
Gabriela Dornelles Bittencourt, Hassan Bencherif, Damaris Kirsch Pinheiro, Nelson Begue, Lucas Vaz Peres, José Valentin Bageston, Douglas Lima de Bem, Francisco Raimundo da Silva, and Tristan Millet
Atmos. Meas. Tech., 17, 5201–5220, https://doi.org/10.5194/amt-17-5201-2024, https://doi.org/10.5194/amt-17-5201-2024, 2024
Short summary
Short summary
The study examines the behavior of ozone at equatorial and subtropical latitudes in South America, in a multi-instrumental analysis. The methodology applied used ozonesondes (SHADOZ/NASA) and satellite data (TIMED/SABER), as well as analysis with ground-based and satellite instruments, allowing a more in-depth study at both latitudes. The main motivation is to understand how latitudinal differences in the observation of ozone content can interfere with the behavior of this trace gas.
Pierre Tulet, Joel Van Baelen, Pierre Bosser, Jérome Brioude, Aurélie Colomb, Philippe Goloub, Andrea Pazmino, Thierry Portafaix, Michel Ramonet, Karine Sellegri, Melilotus Thyssen, Léa Gest, Nicolas Marquestaut, Dominique Mékiès, Jean-Marc Metzger, Gilles Athier, Luc Blarel, Marc Delmotte, Guillaume Desprairies, Mérédith Dournaux, Gaël Dubois, Valentin Duflot, Kevin Lamy, Lionel Gardes, Jean-François Guillemot, Valérie Gros, Joanna Kolasinski, Morgan Lopez, Olivier Magand, Erwan Noury, Manuel Nunes-Pinharanda, Guillaume Payen, Joris Pianezze, David Picard, Olivier Picard, Sandrine Prunier, François Rigaud-Louise, Michael Sicard, and Benjamin Torres
Earth Syst. Sci. Data, 16, 3821–3849, https://doi.org/10.5194/essd-16-3821-2024, https://doi.org/10.5194/essd-16-3821-2024, 2024
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The MAP-IO program aims to compensate for the lack of atmospheric and oceanographic observations in the Southern Ocean by equipping the ship Marion Dufresne with a set of 17 scientific instruments. This program collected 700 d of measurements under different latitudes, seasons, sea states, and weather conditions. These new data will support the calibration and validation of numerical models and the understanding of the atmospheric composition of this region of Earth.
Tristan Millet, Hassan Bencherif, Thierry Portafaix, Nelson Bègue, Alexandre Baron, Valentin Duflot, Cathy Clerbaux, Pierre-François Coheur, Andrea Pazmino, Michaël Sicard, Jean-Marc Metzger, Guillaume Payen, Nicolas Marquestaut, and Sophie Godin-Beekmann
EGUsphere, https://doi.org/10.5194/egusphere-2024-2350, https://doi.org/10.5194/egusphere-2024-2350, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
On 15 January 2022, the Hunga volcano erupted, releasing aerosols, sulfur dioxide, and water vapor into the stratosphere, impacting ozone levels over the Indian Ocean. MLS and IASI data show that the volcanic plume decreased ozone levels within the stratospheric ozone layer, shaping a structure similar to an ozone mini-hole. A stable stratosphere, free of dynamical barriers, enabled the volcanic plume's transport over the Indian Ocean.
Nelson Bègue, Alexandre Baron, Gisèle Krysztofiak, Gwenaël Berthet, Corinna Kloss, Fabrice Jégou, Sergey Khaykin, Marion Ranaivombola, Tristan Millet, Thierry Portafaix, Valentin Duflot, Philippe Keckhut, Hélène Vérèmes, Guillaume Payen, Mahesh Kumar Sha, Pierre-François Coheur, Cathy Clerbaux, Michaël Sicard, Tetsu Sakai, Richard Querel, Ben Liley, Dan Smale, Isamu Morino, Osamu Uchino, Tomohiro Nagai, Penny Smale, John Robinson, and Hassan Bencherif
Atmos. Chem. Phys., 24, 8031–8048, https://doi.org/10.5194/acp-24-8031-2024, https://doi.org/10.5194/acp-24-8031-2024, 2024
Short summary
Short summary
During the 2020 austral summer, the pristine atmosphere of the southwest Indian Ocean basin experienced significant perturbations. Numerical models indicated that the lower-stratospheric aerosol content was influenced by the intense and persistent stratospheric aerosol layer generated during the 2019–2020 extreme Australian bushfire events. Ground-based observations at Réunion confirmed the simultaneous presence of African and Australian aerosol layers.
Michael Sicard, Alexandre Baron, Marion Ranaivombola, Dominique Gantois, Tristan Millet, Pasquale Sellitto, Nelson Bègue, Hassan Bencherif, Guillaume Payen, Nicolas Marquestaut, and Valentin Duflot
EGUsphere, https://doi.org/10.22541/essoar.170231679.99186200/v1, https://doi.org/10.22541/essoar.170231679.99186200/v1, 2024
Short summary
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This study quantifies the radiative impact over Reunion Island (21° S, 55° E) of the aerosols and water vapor injected in the stratosphere by the Hunga Tonga-Hunga Ha'apai volcano in the South Pacific. The overall aerosol and water vapor impact on the Earth’s radiation budget for the whole period is negative (cooling, -0.54 ± 0.29 W m-2) and dominated by the aerosols. At the Earth’s surface, aerosols are the main driver and produce a negative (cooling, -1.19 ± 0.40 W m-2) radiative impact.
Thomas Lesigne, François Ravetta, Aurélien Podglajen, Vincent Mariage, and Jacques Pelon
Atmos. Chem. Phys., 24, 5935–5952, https://doi.org/10.5194/acp-24-5935-2024, https://doi.org/10.5194/acp-24-5935-2024, 2024
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Upper tropical clouds have a strong impact on Earth's climate but are challenging to observe. We report the first long-duration observations of tropical clouds from lidars flying on board stratospheric balloons. Comparisons with spaceborne observations reveal the enhanced sensitivity of balloon-borne lidar to optically thin cirrus. These clouds, which have a significant coverage and lie in the uppermost troposphere, are linked with the dehydration of air masses on their way to the stratosphere.
Lucas Pailler, Laurent Deguillaume, Hélène Lavanant, Isabelle Schmitz, Marie Hubert, Edith Nicol, Mickaël Ribeiro, Jean-Marc Pichon, Mickaël Vaïtilingom, Pamela Dominutti, Frédéric Burnet, Pierre Tulet, Maud Leriche, and Angelica Bianco
Atmos. Chem. Phys., 24, 5567–5584, https://doi.org/10.5194/acp-24-5567-2024, https://doi.org/10.5194/acp-24-5567-2024, 2024
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The composition of dissolved organic matter of cloud water has been investigated through non-targeted high-resolution mass spectrometry on only a few samples collected in the Northern Hemisphere. In this work, the chemical composition of samples collected at Réunion Island (SH) is investigated and compared to samples collected at Puy de Dôme (NH). Sampling, analysis and data treatment with the same methodology produced a unique dataset for investigating the molecular composition of clouds.
Marion Ranaivombola, Nelson Bègue, Farahnaz Fazel-Rastgar, Venkataraman Sivakumar, Gisèle Krysztofiak, Gwenaël Berthet, Fabrice Jegou, Stuart Piketh, and Hassan Bencherif
EGUsphere, https://doi.org/10.5194/egusphere-2024-921, https://doi.org/10.5194/egusphere-2024-921, 2024
Short summary
Short summary
From September to October 2022, the Biomass Burning Aerosol Campaign (BiBAC) in Kruger National Park revealed a significant aerosol loading linked to biomass burning activity, with a southeastward transport over Southern Africa and the southwestern of Indian Ocean (SWIO) basin. The "river of smoke" phenomenon drove the plume during September toward the SWIO. One discusses the long-range transport of biomass burning from South America to Southern Africa is likely driven by climate forcings.
Gerard Ancellet, Camille Viatte, Anne Boynard, François Ravetta, Jacques Pelon, Cristelle Cailteau-Fischbach, Pascal Genau, Julie Capo, Axel Roy, and Philippe Nédélec
EGUsphere, https://doi.org/10.5194/egusphere-2024-892, https://doi.org/10.5194/egusphere-2024-892, 2024
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Characterization of ozone pollution in urban areas has benefited from a measurement campaign in summer 2022 in the Paris region. The analysis is based on 21 days of lidar and aircraft observations. The main objective is a sensitivity analysis of ozone pollution to first the micrometeorological processes in the urban atmospheric boundary layer, and second, the transport of regional pollution. The paper also discuss to what extent satellite observations can track the observed ozone plumes.
Safae Oumami, Joaquim Arteta, Vincent Guidard, Pierre Tulet, and Paul David Hamer
Geosci. Model Dev., 17, 3385–3408, https://doi.org/10.5194/gmd-17-3385-2024, https://doi.org/10.5194/gmd-17-3385-2024, 2024
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In this paper, we coupled the SURFEX and MEGAN models. The aim of this coupling is to improve the estimation of biogenic fluxes by using the SURFEX canopy environment model. The coupled model results were validated and several sensitivity tests were performed. The coupled-model total annual isoprene flux is 442 Tg; this value is within the range of other isoprene estimates reported. The ultimate aim of this coupling is to predict the impact of climate change on biogenic emissions.
Maud Leriche, Pierre Tulet, Laurent Deguillaume, Frédéric Burnet, Aurélie Colomb, Agnès Borbon, Corinne Jambert, Valentin Duflot, Stéphan Houdier, Jean-Luc Jaffrezo, Mickaël Vaïtilingom, Pamela Dominutti, Manon Rocco, Camille Mouchel-Vallon, Samira El Gdachi, Maxence Brissy, Maroua Fathalli, Nicolas Maury, Bert Verreyken, Crist Amelynck, Niels Schoon, Valérie Gros, Jean-Marc Pichon, Mickael Ribeiro, Eric Pique, Emmanuel Leclerc, Thierry Bourrianne, Axel Roy, Eric Moulin, Joël Barrie, Jean-Marc Metzger, Guillaume Péris, Christian Guadagno, Chatrapatty Bhugwant, Jean-Mathieu Tibere, Arnaud Tournigand, Evelyn Freney, Karine Sellegri, Anne-Marie Delort, Pierre Amato, Muriel Joly, Jean-Luc Baray, Pascal Renard, Angelica Bianco, Anne Réchou, and Guillaume Payen
Atmos. Chem. Phys., 24, 4129–4155, https://doi.org/10.5194/acp-24-4129-2024, https://doi.org/10.5194/acp-24-4129-2024, 2024
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Aerosol particles in the atmosphere play a key role in climate change and air pollution. A large number of aerosol particles are formed from the oxidation of volatile organic compounds (VOCs and secondary organic aerosols – SOA). An important field campaign was organized on Réunion in March–April 2019 to understand the formation of SOA in a tropical atmosphere mostly influenced by VOCs emitted by forest and in the presence of clouds. This work synthesizes the results of this campaign.
Romain Salignat, Matti Rissanen, Siddharth Iyer, Jean-Luc Baray, Pierre Tulet, Jean-Marc Metzger, Jérôme Brioude, Karine Sellegri, and Clémence Rose
Atmos. Chem. Phys., 24, 3785–3812, https://doi.org/10.5194/acp-24-3785-2024, https://doi.org/10.5194/acp-24-3785-2024, 2024
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Using mass spectrometry data collected at the Maïdo Observatory (2160 m a.s.l., Réunion), we provide the first detailed analysis of molecular cluster chemical composition specifically in the marine free troposphere. The abundance of the identified species is related both to in situ meteorological parameters and air mass history, which also provide insight into their origin. Our work makes an important contribution to documenting the chemistry and physics of the marine free troposphere.
Tristan Millet, Hassan Bencherif, Thierry Portafaix, Nelson Bègue, Alexandre Baron, Valentin Duflot, Michaël Sicard, Jean-Marc Metzger, Guillaume Payen, Nicolas Marquestaut, and Sophie Godin-Beekmann
EGUsphere, https://doi.org/10.5194/egusphere-2023-2645, https://doi.org/10.5194/egusphere-2023-2645, 2023
Preprint withdrawn
Short summary
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The eruption of the Hunga Tonga volcano in January 2022 released substantial amounts of aerosols, sulfur dioxide, and water vapor into the stratosphere. Satellite and ground instruments followed the displacement of the volcanic aerosol plume and its impact on ozone levels over the Indian Ocean. Ozone data reveal the presence of a persistent ozone mini-hole structure from 17 January to 22 January, with most ozone depletion occurring within the ozone layer at the location of the aerosol plume.
Lambert Delbeke, Chien Wang, Pierre Tulet, Cyrielle Denjean, Maurin Zouzoua, Nicolas Maury, and Adrien Deroubaix
Atmos. Chem. Phys., 23, 13329–13354, https://doi.org/10.5194/acp-23-13329-2023, https://doi.org/10.5194/acp-23-13329-2023, 2023
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Low-level stratiform clouds (LLSCs) appear frequently over southern West Africa during the West African monsoon. Local and remote aerosol sources (biomass burning aerosols from central Africa) play a significant role in the LLSC life cycle. Based on measurements by the DACCIWA campaign, large-eddy simulation (LES) was conducted using different aerosol scenarios. The results show that both indirect and semi-direct effects can act individually or jointly to influence the life cycles of LLSCs.
Gabriela Dornelles Bittencourt, Damaris Kirsch Pinheiro, Hassan Bencherif, Lucas Vaz Peres, Nelson Begue, José Valentin Bageston, Douglas Lima de Bem, Vagner Anabor, and Luiz Angelo Steffenel
EGUsphere, https://doi.org/10.5194/egusphere-2023-1471, https://doi.org/10.5194/egusphere-2023-1471, 2023
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The study examines ozone depletions at mid-latitudes in Brazil during austral spring Antarctic Ozone Hole influence events. The methodology applied used data from the total column ozone, vertical profile of the atmosphere, and reanalysis data to analyze the atmospheric dynamics. The main motivation of this work is to show how this important trace gas dynamically behaves in the atmosphere in the active period of the Antarctic Ozone Hole in regions of medium latitudes.
Meryl Wimmer, Gwendal Rivière, Philippe Arbogast, Jean-Marcel Piriou, Julien Delanoë, Carole Labadie, Quitterie Cazenave, and Jacques Pelon
Weather Clim. Dynam., 3, 863–882, https://doi.org/10.5194/wcd-3-863-2022, https://doi.org/10.5194/wcd-3-863-2022, 2022
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The effect of deep convection representation on the jet stream above the cold front of an extratropical cyclone is investigated in the global numerical weather prediction model ARPEGE. Two simulations using different deep convection schemes are compared with (re)analysis datasets and NAWDEX airborne observations. A deeper jet stream is observed with the less active scheme. The diabatic origin of this difference is interpreted by backward Lagrangian trajectories and potential vorticity budgets.
Thibault Vaillant de Guélis, Gérard Ancellet, Anne Garnier, Laurent C.-Labonnote, Jacques Pelon, Mark A. Vaughan, Zhaoyan Liu, and David M. Winker
Atmos. Meas. Tech., 15, 1931–1956, https://doi.org/10.5194/amt-15-1931-2022, https://doi.org/10.5194/amt-15-1931-2022, 2022
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A new IIR-based cloud and aerosol discrimination (CAD) algorithm is developed using the IIR brightness temperature differences for cloud and aerosol features confidently identified by the CALIOP version 4 CAD algorithm. IIR classifications agree with the majority of V4 cloud identifications, reduce the ambiguity in a notable fraction of
not confidentV4 cloud classifications, and correct a few V4 misclassifications of cloud layers identified as dense dust or elevated smoke layers by CALIOP.
Yongjie Huang, Wei Wu, Greg M. McFarquhar, Ming Xue, Hugh Morrison, Jason Milbrandt, Alexei V. Korolev, Yachao Hu, Zhipeng Qu, Mengistu Wolde, Cuong Nguyen, Alfons Schwarzenboeck, and Ivan Heckman
Atmos. Chem. Phys., 22, 2365–2384, https://doi.org/10.5194/acp-22-2365-2022, https://doi.org/10.5194/acp-22-2365-2022, 2022
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Numerous small ice crystals in tropical convective storms are difficult to detect and could be potentially hazardous for commercial aircraft. Previous numerical simulations failed to reproduce this phenomenon and hypothesized that key microphysical processes are still lacking in current models to realistically simulate the phenomenon. This study uses numerical experiments to confirm the dominant role of secondary ice production in the formation of these large numbers of small ice crystals.
Pamela A. Dominutti, Pascal Renard, Mickaël Vaïtilingom, Angelica Bianco, Jean-Luc Baray, Agnès Borbon, Thierry Bourianne, Frédéric Burnet, Aurélie Colomb, Anne-Marie Delort, Valentin Duflot, Stephan Houdier, Jean-Luc Jaffrezo, Muriel Joly, Martin Leremboure, Jean-Marc Metzger, Jean-Marc Pichon, Mickaël Ribeiro, Manon Rocco, Pierre Tulet, Anthony Vella, Maud Leriche, and Laurent Deguillaume
Atmos. Chem. Phys., 22, 505–533, https://doi.org/10.5194/acp-22-505-2022, https://doi.org/10.5194/acp-22-505-2022, 2022
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We present here the results obtained during an intensive field campaign conducted in March to April 2019 in Reunion. Our study integrates a comprehensive chemical and microphysical characterization of cloud water. Our investigations reveal that air mass history and cloud microphysical properties do not fully explain the variability observed in their chemical composition. This highlights the complexity of emission sources, multiphasic exchanges, and transformations in clouds.
Clémence Rose, Martine Collaud Coen, Elisabeth Andrews, Yong Lin, Isaline Bossert, Cathrine Lund Myhre, Thomas Tuch, Alfred Wiedensohler, Markus Fiebig, Pasi Aalto, Andrés Alastuey, Elisabeth Alonso-Blanco, Marcos Andrade, Begoña Artíñano, Todor Arsov, Urs Baltensperger, Susanne Bastian, Olaf Bath, Johan Paul Beukes, Benjamin T. Brem, Nicolas Bukowiecki, Juan Andrés Casquero-Vera, Sébastien Conil, Konstantinos Eleftheriadis, Olivier Favez, Harald Flentje, Maria I. Gini, Francisco Javier Gómez-Moreno, Martin Gysel-Beer, Anna Gannet Hallar, Ivo Kalapov, Nikos Kalivitis, Anne Kasper-Giebl, Melita Keywood, Jeong Eun Kim, Sang-Woo Kim, Adam Kristensson, Markku Kulmala, Heikki Lihavainen, Neng-Huei Lin, Hassan Lyamani, Angela Marinoni, Sebastiao Martins Dos Santos, Olga L. Mayol-Bracero, Frank Meinhardt, Maik Merkel, Jean-Marc Metzger, Nikolaos Mihalopoulos, Jakub Ondracek, Marco Pandolfi, Noemi Pérez, Tuukka Petäjä, Jean-Eudes Petit, David Picard, Jean-Marc Pichon, Veronique Pont, Jean-Philippe Putaud, Fabienne Reisen, Karine Sellegri, Sangeeta Sharma, Gerhard Schauer, Patrick Sheridan, James Patrick Sherman, Andreas Schwerin, Ralf Sohmer, Mar Sorribas, Junying Sun, Pierre Tulet, Ville Vakkari, Pieter Gideon van Zyl, Fernando Velarde, Paolo Villani, Stergios Vratolis, Zdenek Wagner, Sheng-Hsiang Wang, Kay Weinhold, Rolf Weller, Margarita Yela, Vladimir Zdimal, and Paolo Laj
Atmos. Chem. Phys., 21, 17185–17223, https://doi.org/10.5194/acp-21-17185-2021, https://doi.org/10.5194/acp-21-17185-2021, 2021
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Aerosol particles are a complex component of the atmospheric system the effects of which are among the most uncertain in climate change projections. Using data collected at 62 stations, this study provides the most up-to-date picture of the spatial distribution of particle number concentration and size distribution worldwide, with the aim of contributing to better representation of aerosols and their interactions with clouds in models and, therefore, better evaluation of their impact on climate.
Lilian Loyer, Jean-Christophe Raut, Claudia Di Biagio, Julia Maillard, Vincent Mariage, and Jacques Pelon
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2021-326, https://doi.org/10.5194/amt-2021-326, 2021
Revised manuscript not accepted
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The Arctic is facing drastic climate changes, and more observations are needed to better understand what is happening. Unfortunately observations are limited in the High Arctic. To obtain more observations, multiples buoys equipped with lidar, have been deployed in this region. This paper presents an approach to estimate the optical properties of clouds, and solar plus terrestrial energies from lidar measurements in the Arctic.
Gwendal Rivière, Meryl Wimmer, Philippe Arbogast, Jean-Marcel Piriou, Julien Delanoë, Carole Labadie, Quitterie Cazenave, and Jacques Pelon
Weather Clim. Dynam., 2, 1011–1031, https://doi.org/10.5194/wcd-2-1011-2021, https://doi.org/10.5194/wcd-2-1011-2021, 2021
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Inacurracies in representing processes occurring at spatial scales smaller than the grid scales of the weather forecast models are important sources of forecast errors. This is the case of deep convection representation in models with 10 km grid spacing. We performed simulations of a real extratropical cyclone using a model with different representations of deep convection. These forecasts lead to different behaviors in the ascending air masses of the cyclone and the jet stream aloft.
Didier Bruneau and Jacques Pelon
Atmos. Meas. Tech., 14, 4375–4402, https://doi.org/10.5194/amt-14-4375-2021, https://doi.org/10.5194/amt-14-4375-2021, 2021
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Taking advantage of Aeolus success and of our airborne lidar system expertise, we present a new spaceborne wind lidar design for operational Aeolus follow-on missions, keeping most of the initial lidar system but relying on a single Mach–Zehnder interferometer to relax operational constraints and reduce measurement bias. System parameters are optimized. Random and systematic errors are shown to be compliant with the initial mission requirements. In addition, the system allows unbiased retrieval.
Anne Garnier, Jacques Pelon, Nicolas Pascal, Mark A. Vaughan, Philippe Dubuisson, Ping Yang, and David L. Mitchell
Atmos. Meas. Tech., 14, 3253–3276, https://doi.org/10.5194/amt-14-3253-2021, https://doi.org/10.5194/amt-14-3253-2021, 2021
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The IIR Level 2 data products include cloud effective emissivities and cloud microphysical properties such as effective diameter (De) and ice or liquid water path estimates. This paper (Part I) describes the improvements in the V4 algorithms compared to those used in the version 3 (V3) release, while results are presented in a companion paper (Part II).
Anne Garnier, Jacques Pelon, Nicolas Pascal, Mark A. Vaughan, Philippe Dubuisson, Ping Yang, and David L. Mitchell
Atmos. Meas. Tech., 14, 3277–3299, https://doi.org/10.5194/amt-14-3277-2021, https://doi.org/10.5194/amt-14-3277-2021, 2021
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The IIR Level 2 data products include cloud effective emissivities and cloud microphysical properties such as effective diameter (De) and ice or liquid water path estimates. This paper (Part II) shows retrievals over ocean and describes the improvements made with respect to version 3 as a result of the significant changes implemented in the version 4 algorithms, which are presented in a companion paper (Part I).
Clémence Rose, Matti P. Rissanen, Siddharth Iyer, Jonathan Duplissy, Chao Yan, John B. Nowak, Aurélie Colomb, Régis Dupuy, Xu-Cheng He, Janne Lampilahti, Yee Jun Tham, Daniela Wimmer, Jean-Marc Metzger, Pierre Tulet, Jérôme Brioude, Céline Planche, Markku Kulmala, and Karine Sellegri
Atmos. Chem. Phys., 21, 4541–4560, https://doi.org/10.5194/acp-21-4541-2021, https://doi.org/10.5194/acp-21-4541-2021, 2021
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Sulfuric acid (H2SO4) is commonly accepted as a key precursor for atmospheric new particle formation. However, direct measurements of [H2SO4] remain challenging, motivating the development of proxies. Using data collected in two different volcanic plumes, we show, under these specific conditions, the good performance of a proxy from the literature and also highlight the benefit of the newly developed proxies for the prediction of the highest [H2SO4] values.
David L. A. Flack, Gwendal Rivière, Ionela Musat, Romain Roehrig, Sandrine Bony, Julien Delanoë, Quitterie Cazenave, and Jacques Pelon
Weather Clim. Dynam., 2, 233–253, https://doi.org/10.5194/wcd-2-233-2021, https://doi.org/10.5194/wcd-2-233-2021, 2021
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The representation of an extratropical cyclone in simulations of two climate models is studied by comparing them to observations of the international field campaign NAWDEX. We show that the current resolution used to run climate model projections (more than 100 km) is not enough to represent the life cycle accurately, but the use of 50 km resolution is good enough. Despite these encouraging results, cloud properties (partitioning liquid and solid) are found to be far from the observations.
Julia Maillard, François Ravetta, Jean-Christophe Raut, Vincent Mariage, and Jacques Pelon
Atmos. Chem. Phys., 21, 4079–4101, https://doi.org/10.5194/acp-21-4079-2021, https://doi.org/10.5194/acp-21-4079-2021, 2021
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Clouds remain a major source of uncertainty in understanding the Arctic climate, due in part to the lack of measurements over the sea ice. In this paper, we exploit a series of lidar profiles acquired from autonomous drifting buoys deployed in the Arctic Ocean and derive a statistic of low cloud frequency and macrophysical properties. We also show that clouds contribute to warm the surface in the shoulder seasons but not significantly from May to September.
Keun-Ok Lee, Brice Barret, Eric L. Flochmoën, Pierre Tulet, Silvia Bucci, Marc von Hobe, Corinna Kloss, Bernard Legras, Maud Leriche, Bastien Sauvage, Fabrizio Ravegnani, and Alexey Ulanovsky
Atmos. Chem. Phys., 21, 3255–3274, https://doi.org/10.5194/acp-21-3255-2021, https://doi.org/10.5194/acp-21-3255-2021, 2021
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This paper focuses on the emission sources and pathways of pollution from the boundary layer to the Asian monsoon anticyclone (AMA) during the StratoClim aircraft campaign period. Simulations with the Meso-NH cloud-chemistry model at a horizontal resolution of 15 km are performed over the Asian region to characterize the impact of monsoon deep convection on the composition of AMA and on the formation of the Asian tropopause aerosol layer during the StratoClim campaign.
Setigui Aboubacar Keita, Eric Girard, Jean-Christophe Raut, Maud Leriche, Jean-Pierre Blanchet, Jacques Pelon, Tatsuo Onishi, and Ana Cirisan
Geosci. Model Dev., 13, 5737–5755, https://doi.org/10.5194/gmd-13-5737-2020, https://doi.org/10.5194/gmd-13-5737-2020, 2020
Melody A. Avery, Robert A. Ryan, Brian J. Getzewich, Mark A. Vaughan, David M. Winker, Yongxiang Hu, Anne Garnier, Jacques Pelon, and Carolus A. Verhappen
Atmos. Meas. Tech., 13, 4539–4563, https://doi.org/10.5194/amt-13-4539-2020, https://doi.org/10.5194/amt-13-4539-2020, 2020
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CALIOP data users will find more cloud layers detected in V4, with edges that extend further than in V3, for an increase in total atmospheric cloud volume of 6 %–9 % for high-confidence cloud phases and 1 %–2 % for all cloudy bins, including cloud fringes and unknown cloud phases. In V4 there are many fewer cloud layers identified as horizontally oriented ice, particularly in the 3° off-nadir view. Depolarization at 532 nm is the predominant parameter determining cloud thermodynamic phase.
Paolo Laj, Alessandro Bigi, Clémence Rose, Elisabeth Andrews, Cathrine Lund Myhre, Martine Collaud Coen, Yong Lin, Alfred Wiedensohler, Michael Schulz, John A. Ogren, Markus Fiebig, Jonas Gliß, Augustin Mortier, Marco Pandolfi, Tuukka Petäja, Sang-Woo Kim, Wenche Aas, Jean-Philippe Putaud, Olga Mayol-Bracero, Melita Keywood, Lorenzo Labrador, Pasi Aalto, Erik Ahlberg, Lucas Alados Arboledas, Andrés Alastuey, Marcos Andrade, Begoña Artíñano, Stina Ausmeel, Todor Arsov, Eija Asmi, John Backman, Urs Baltensperger, Susanne Bastian, Olaf Bath, Johan Paul Beukes, Benjamin T. Brem, Nicolas Bukowiecki, Sébastien Conil, Cedric Couret, Derek Day, Wan Dayantolis, Anna Degorska, Konstantinos Eleftheriadis, Prodromos Fetfatzis, Olivier Favez, Harald Flentje, Maria I. Gini, Asta Gregorič, Martin Gysel-Beer, A. Gannet Hallar, Jenny Hand, Andras Hoffer, Christoph Hueglin, Rakesh K. Hooda, Antti Hyvärinen, Ivo Kalapov, Nikos Kalivitis, Anne Kasper-Giebl, Jeong Eun Kim, Giorgos Kouvarakis, Irena Kranjc, Radovan Krejci, Markku Kulmala, Casper Labuschagne, Hae-Jung Lee, Heikki Lihavainen, Neng-Huei Lin, Gunter Löschau, Krista Luoma, Angela Marinoni, Sebastiao Martins Dos Santos, Frank Meinhardt, Maik Merkel, Jean-Marc Metzger, Nikolaos Mihalopoulos, Nhat Anh Nguyen, Jakub Ondracek, Noemi Pérez, Maria Rita Perrone, Jean-Eudes Petit, David Picard, Jean-Marc Pichon, Veronique Pont, Natalia Prats, Anthony Prenni, Fabienne Reisen, Salvatore Romano, Karine Sellegri, Sangeeta Sharma, Gerhard Schauer, Patrick Sheridan, James Patrick Sherman, Maik Schütze, Andreas Schwerin, Ralf Sohmer, Mar Sorribas, Martin Steinbacher, Junying Sun, Gloria Titos, Barbara Toczko, Thomas Tuch, Pierre Tulet, Peter Tunved, Ville Vakkari, Fernando Velarde, Patricio Velasquez, Paolo Villani, Sterios Vratolis, Sheng-Hsiang Wang, Kay Weinhold, Rolf Weller, Margarita Yela, Jesus Yus-Diez, Vladimir Zdimal, Paul Zieger, and Nadezda Zikova
Atmos. Meas. Tech., 13, 4353–4392, https://doi.org/10.5194/amt-13-4353-2020, https://doi.org/10.5194/amt-13-4353-2020, 2020
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The paper establishes the fiducial reference of the GAW aerosol network providing the fully characterized value chain to the provision of four climate-relevant aerosol properties from ground-based sites. Data from almost 90 stations worldwide are reported for a reference year, 2017, providing a unique and very robust view of the variability of these variables worldwide. Current gaps in the GAW network are analysed and requirements for the Global Climate Monitoring System are proposed.
Cyrielle Denjean, Thierry Bourrianne, Frederic Burnet, Marc Mallet, Nicolas Maury, Aurélie Colomb, Pamela Dominutti, Joel Brito, Régis Dupuy, Karine Sellegri, Alfons Schwarzenboeck, Cyrille Flamant, and Peter Knippertz
Atmos. Chem. Phys., 20, 4735–4756, https://doi.org/10.5194/acp-20-4735-2020, https://doi.org/10.5194/acp-20-4735-2020, 2020
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This paper presents aircraft measurements of aerosol optical properties over southern West Africa. We show that aerosol optical properties in the boundary layer were dominated by a persistent biomass burning loading from the Southern Hemisphere. Biomass burning aerosols were more light absorbing that those previously measured in other areas (Amazonia, North America). Our study suggests that lens-coated black carbon particles were the dominant absorber for these biomass burning aerosols.
Antonin Zabukovec, Gerard Ancellet, Iwan E. Penner, Mikhail Arshinov, Valery Kozlov, Jacques Pelon, Jean-Daniel Paris, Grigory Kokhanenko, Yuri S. Balin, Dmitry Chernov, and Boris D. Belan
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-195, https://doi.org/10.5194/acp-2020-195, 2020
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Description of two aircraft campaigns results carried out over Siberia in 2013 and 2017 to characterize aerosol emission. A methodology is proposed to derive the aerosol types using transport model and satellite observations. The extinction to backscatter ratio for each aerosol types is reported as it is a key parameter to constrain their radiative impact. These results are compared to previous work conducted in other regions and to aerosol data products observed by spaceborne lidars.
Nelson Bègue, Lerato Shikwambana, Hassan Bencherif, Juan Pallotta, Venkataraman Sivakumar, Elian Wolfram, Nkanyiso Mbatha, Facundo Orte, David Jean Du Preez, Marion Ranaivombola, Stuart Piketh, and Paola Formenti
Ann. Geophys., 38, 395–420, https://doi.org/10.5194/angeo-38-395-2020, https://doi.org/10.5194/angeo-38-395-2020, 2020
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This study investigates the influence of the 2015 Calbuco eruption (41.2°S, 72.4°W; Chile) on the total columnar aerosol optical properties in the Southern Hemisphere. The well-known technique of sun photometry was applied to the investigation of the transport and the spatio-temporal evolution of the optical properties of the volcanic plume. The CIMEL sun photometer measurements performed over six South American and three African sites were statistically analyzed.
Sophie L. Haslett, Jonathan W. Taylor, Mathew Evans, Eleanor Morris, Bernhard Vogel, Alima Dajuma, Joel Brito, Anneke M. Batenburg, Stephan Borrmann, Johannes Schneider, Christiane Schulz, Cyrielle Denjean, Thierry Bourrianne, Peter Knippertz, Régis Dupuy, Alfons Schwarzenböck, Daniel Sauer, Cyrille Flamant, James Dorsey, Ian Crawford, and Hugh Coe
Atmos. Chem. Phys., 19, 15217–15234, https://doi.org/10.5194/acp-19-15217-2019, https://doi.org/10.5194/acp-19-15217-2019, 2019
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Three aircraft datasets from the DACCIWA campaign in summer 2016 are used here to show there is a background mass of pollution present in the lower atmosphere in southern West Africa. We suggest that this likely comes from biomass burning in central and southern Africa, which has been carried into the region over the Atlantic Ocean. This would have a negative health impact on populations living near the coast and may alter the impact of growing city emissions on cloud formation and the monsoon.
Corinna Kloss, Gwenaël Berthet, Pasquale Sellitto, Felix Ploeger, Silvia Bucci, Sergey Khaykin, Fabrice Jégou, Ghassan Taha, Larry W. Thomason, Brice Barret, Eric Le Flochmoen, Marc von Hobe, Adriana Bossolasco, Nelson Bègue, and Bernard Legras
Atmos. Chem. Phys., 19, 13547–13567, https://doi.org/10.5194/acp-19-13547-2019, https://doi.org/10.5194/acp-19-13547-2019, 2019
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With satellite measurements and transport models, we show that a plume resulting from strong Canadian fires in July/August 2017 was not only distributed throughout the northern/higher latitudes, but also reached the faraway tropics, aided by the circulation of Asian monsoon anticyclone. The regional climate impact in the wider Asian monsoon area in September exceeds the impact of the Asian tropopause aerosol layer by a factor of ~ 3 and compares to that of an advected moderate volcanic eruption.
Clémence Rose, Brice Foucart, David Picard, Aurélie Colomb, Jean-Marc Metzger, Pierre Tulet, and Karine Sellegri
Atmos. Chem. Phys., 19, 13243–13265, https://doi.org/10.5194/acp-19-13243-2019, https://doi.org/10.5194/acp-19-13243-2019, 2019
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New particle formation (NPF) is a significant climate-relevant source of aerosols in the atmosphere. We show that during the eruptive periods of the Piton de la Fournaise in 2015, NPF was favoured compared to regular days. Using the largest dataset ever reported in volcanic plume conditions, we quantify the emission rates of particles over a broad size range and provide a new statistically robust parameterization to take into account this important source of atmospheric particles in models.
Valentin Duflot, Pierre Tulet, Olivier Flores, Christelle Barthe, Aurélie Colomb, Laurent Deguillaume, Mickael Vaïtilingom, Anne Perring, Alex Huffman, Mark T. Hernandez, Karine Sellegri, Ellis Robinson, David J. O'Connor, Odessa M. Gomez, Frédéric Burnet, Thierry Bourrianne, Dominique Strasberg, Manon Rocco, Allan K. Bertram, Patrick Chazette, Julien Totems, Jacques Fournel, Pierre Stamenoff, Jean-Marc Metzger, Mathilde Chabasset, Clothilde Rousseau, Eric Bourrianne, Martine Sancelme, Anne-Marie Delort, Rachel E. Wegener, Cedric Chou, and Pablo Elizondo
Atmos. Chem. Phys., 19, 10591–10618, https://doi.org/10.5194/acp-19-10591-2019, https://doi.org/10.5194/acp-19-10591-2019, 2019
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The Forests gAses aeRosols Clouds Exploratory (FARCE) campaign was conducted in March–April 2015 on the tropical island of La Réunion. For the first time, several scientific teams from different disciplines collaborated to provide reference measurements and characterization of La Réunion vegetation, volatile organic compounds (VOCs), biogenic VOCs (BVOCs), (bio)aerosols and composition of clouds, with a strong focus on the Maïdo mount slope area.
Pablo Facundo Orte, Elian Wolfram, Jacobo Salvador, Akira Mizuno, Nelson Bègue, Hassan Bencherif, Juan Lucas Bali, Raúl D'Elia, Andrea Pazmiño, Sophie Godin-Beekmann, Hirofumi Ohyama, and Jonathan Quiroga
Ann. Geophys., 37, 613–629, https://doi.org/10.5194/angeo-37-613-2019, https://doi.org/10.5194/angeo-37-613-2019, 2019
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We analysed an event of short-term ozone variability due to the passage of the polar vortex over Río Gallegos (southern Argentina) with the aim of highlighting the capability of a millimetre-wave radiometer to observe ozone in the stratosphere and the low mesosphere with a high temporal resolution. It is particularly important in this subpolar region due to the high variation that this gas can suffer as a consequence of the passage of the polar vortex and the ozone hole during spring.
Jonathan W. Taylor, Sophie L. Haslett, Keith Bower, Michael Flynn, Ian Crawford, James Dorsey, Tom Choularton, Paul J. Connolly, Valerian Hahn, Christiane Voigt, Daniel Sauer, Régis Dupuy, Joel Brito, Alfons Schwarzenboeck, Thierry Bourriane, Cyrielle Denjean, Phil Rosenberg, Cyrille Flamant, James D. Lee, Adam R. Vaughan, Peter G. Hill, Barbara Brooks, Valéry Catoire, Peter Knippertz, and Hugh Coe
Atmos. Chem. Phys., 19, 8503–8522, https://doi.org/10.5194/acp-19-8503-2019, https://doi.org/10.5194/acp-19-8503-2019, 2019
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Low-level clouds cover a wide area of southern West Africa (SWA) and play an important role in the region's climate, reflecting sunlight away from the surface. We performed aircraft measurements of aerosols and clouds over SWA during the 2016 summer monsoon and found pollution, and polluted clouds, across the whole region. Smoke from biomass burning in Central Africa is transported to West Africa, causing a polluted background which limits the effect of local pollution on cloud properties.
Quitterie Cazenave, Marie Ceccaldi, Julien Delanoë, Jacques Pelon, Silke Groß, and Andrew Heymsfield
Atmos. Meas. Tech., 12, 2819–2835, https://doi.org/10.5194/amt-12-2819-2019, https://doi.org/10.5194/amt-12-2819-2019, 2019
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The impact of ice clouds on the water cycle and radiative budget is still uncertain due to the complexity of cloud processes that makes it difficult to acquire adequate observations of ice cloud properties and parameterize them into climate and weather prediction models. In this paper we present the latest refinements brought to the DARDAR-CLOUD product, which contains ice cloud microphysical properties retrieved from the cloud radar and lidar measurements from the A-Train space mission.
Thibault Vaillant de Guélis, Alfons Schwarzenböck, Valery Shcherbakov, Christophe Gourbeyre, Bastien Laurent, Régis Dupuy, Pierre Coutris, and Christophe Duroure
Atmos. Meas. Tech., 12, 2513–2529, https://doi.org/10.5194/amt-12-2513-2019, https://doi.org/10.5194/amt-12-2513-2019, 2019
David J. du Preez, Jelena V. Ajtić, Hassan Bencherif, Nelson Bègue, Jean-Maurice Cadet, and Caradee Y. Wright
Ann. Geophys., 37, 129–141, https://doi.org/10.5194/angeo-37-129-2019, https://doi.org/10.5194/angeo-37-129-2019, 2019
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Reduced atmospheric ozone results in increased solar ultraviolet radiation (UVR) at the surface which may potentially negative impact public health. We aimed to assess whether or not the break-up of the Antarctic ozone hole had an impact on ozone and UVR at Cape Point (South Africa). We found a moderate inverse relationship between ozone and UVR at midday on clear-sky days. The Antarctic ozone hole had a limited effect on ozone levels while tropical air masses more frequently affected the site.
Sophie L. Haslett, Jonathan W. Taylor, Konrad Deetz, Bernhard Vogel, Karmen Babić, Norbert Kalthoff, Andreas Wieser, Cheikh Dione, Fabienne Lohou, Joel Brito, Régis Dupuy, Alfons Schwarzenboeck, Paul Zieger, and Hugh Coe
Atmos. Chem. Phys., 19, 1505–1520, https://doi.org/10.5194/acp-19-1505-2019, https://doi.org/10.5194/acp-19-1505-2019, 2019
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As the population in West Africa grows and air pollution increases, it is becoming ever more important to understand the effects of this pollution on the climate and on health. Aerosol particles can grow by absorbing water from the air around them. This paper shows that during the monsoon season, aerosol particles in the region are likely to grow significantly because of the high moisture in the air. This means that climate effects from increasing pollution will be enhanced.
Zhaoyan Liu, Jayanta Kar, Shan Zeng, Jason Tackett, Mark Vaughan, Melody Avery, Jacques Pelon, Brian Getzewich, Kam-Pui Lee, Brian Magill, Ali Omar, Patricia Lucker, Charles Trepte, and David Winker
Atmos. Meas. Tech., 12, 703–734, https://doi.org/10.5194/amt-12-703-2019, https://doi.org/10.5194/amt-12-703-2019, 2019
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We describe the enhancements made to the cloud–aerosol discrimination (CAD) algorithms used to produce the CALIPSO version 4 (V4) data products. Revisions to the CAD probability distribution functions have greatly improved the recognition of aerosol layers lofted into the upper troposphere, and CAD is now applied to all layers detected in the stratosphere and all layers detected at single-shot resolution. Detailed comparisons show significant improvements relative to previous versions.
Gerard Ancellet, Iogannes E. Penner, Jacques Pelon, Vincent Mariage, Antonin Zabukovec, Jean Christophe Raut, Grigorii Kokhanenko, and Yuri S. Balin
Atmos. Meas. Tech., 12, 147–168, https://doi.org/10.5194/amt-12-147-2019, https://doi.org/10.5194/amt-12-147-2019, 2019
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Aerosol type seasonal variability and sources in Siberia are obtained from an automatic 808 nm micropulse lidar. A total of 540 aerosol backscatter vertical profiles have been retrieved using careful lidar calibration. Aerosol optical depth is retrieved using sun-photometer complementary observations and an aerosol source apportionment based on aerosol transport model simulations. Comparisons with satellite observations are discussed for three case studies.
Mark Vaughan, Anne Garnier, Damien Josset, Melody Avery, Kam-Pui Lee, Zhaoyan Liu, William Hunt, Jacques Pelon, Yongxiang Hu, Sharon Burton, Johnathan Hair, Jason L. Tackett, Brian Getzewich, Jayanta Kar, and Sharon Rodier
Atmos. Meas. Tech., 12, 51–82, https://doi.org/10.5194/amt-12-51-2019, https://doi.org/10.5194/amt-12-51-2019, 2019
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The version 4 (V4) release of the CALIPSO data products includes substantial improvements to the calibration of the CALIOP 1064 nm channel. In this paper we review the fundamentals of 1064 nm lidar calibration, explain the motivations for the changes made to the algorithm, and describe the mechanics of the V4 calibration technique. Internal consistency checks and comparisons to collocated high spectral resolution lidar measurements show the V4 1064 nm calibration coefficients to within ~ 3 %.
David L. Mitchell, Anne Garnier, Jacques Pelon, and Ehsan Erfani
Atmos. Chem. Phys., 18, 17325–17354, https://doi.org/10.5194/acp-18-17325-2018, https://doi.org/10.5194/acp-18-17325-2018, 2018
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To realistically model a changing climate, global measurements of cirrus cloud ice-particle number concentration (N) and size (De) are needed, through which one may infer the general mechanism of ice formation. A satellite remote sensing method was developed to measure N and De. It was found that N was highest and De lowest at high latitudes. In the Arctic, cirrus clouds occurred much more often during winter, which may have an impact on mid-latitude winter weather.
Cyrille Flamant, Adrien Deroubaix, Patrick Chazette, Joel Brito, Marco Gaetani, Peter Knippertz, Andreas H. Fink, Gaëlle de Coetlogon, Laurent Menut, Aurélie Colomb, Cyrielle Denjean, Rémi Meynadier, Philip Rosenberg, Regis Dupuy, Pamela Dominutti, Jonathan Duplissy, Thierry Bourrianne, Alfons Schwarzenboeck, Michel Ramonet, and Julien Totems
Atmos. Chem. Phys., 18, 12363–12389, https://doi.org/10.5194/acp-18-12363-2018, https://doi.org/10.5194/acp-18-12363-2018, 2018
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This work sheds light on the complex mechanisms by which coastal shallow circulations distribute atmospheric pollutants over the densely populated southern West African region. Pollutants of concern are anthropogenic emissions from coastal cities, as well as biomass burning aerosol and dust associated with long-range transport. The complex vertical distribution of aerosols over coastal southern West Africa is investigated using airborne observations and numerical simulations.
Aurélien Chauvigné, Olivier Jourdan, Alfons Schwarzenboeck, Christophe Gourbeyre, Jean François Gayet, Christiane Voigt, Hans Schlager, Stefan Kaufmann, Stephan Borrmann, Sergej Molleker, Andreas Minikin, Tina Jurkat, and Ulrich Schumann
Atmos. Chem. Phys., 18, 9803–9822, https://doi.org/10.5194/acp-18-9803-2018, https://doi.org/10.5194/acp-18-9803-2018, 2018
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This paper demonstrates a new form of statistical analysis of contrail to cirrus evolution. The authors show well-separated analyses of the different stages of the contrail's evolution, which allows us to study their optical, microphysical, and chemical properties. These results could be used to develop representative parameterizations of the scattering and geometrical properties of the ice crystals’ shapes and sizes, observed in the visible wavelength range.
Brice Foucart, Karine Sellegri, Pierre Tulet, Clémence Rose, Jean-Marc Metzger, and David Picard
Atmos. Chem. Phys., 18, 9243–9261, https://doi.org/10.5194/acp-18-9243-2018, https://doi.org/10.5194/acp-18-9243-2018, 2018
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The main objective of this study is to reinforce the observations of new particle formation (NPF) events in the Southern Hemisphere and more particularly for a site that is both marine and at altitude, the Maïdo observatory (2150 m), on Réunion. We recorded a high annual NPF frequency of 65 % and we note that monthly averages show a bimodal variation. We estimate the intensity and the characteristics of the events and describe their seasonality by comparing them to other parameters.
Stephan E. Bansmer, Arne Baumert, Stephan Sattler, Inken Knop, Delphine Leroy, Alfons Schwarzenboeck, Tina Jurkat-Witschas, Christiane Voigt, Hugo Pervier, and Biagio Esposito
Atmos. Meas. Tech., 11, 3221–3249, https://doi.org/10.5194/amt-11-3221-2018, https://doi.org/10.5194/amt-11-3221-2018, 2018
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Snow, frost formation and ice cubes in our drinks are part of our daily life. But what about our technical innovations like aviation, electrical power transmission and wind-energy production, can they cope with icing? Icing Wind Tunnels are an ideal laboratory environment to answer that question. In this paper, we show how the icing wind tunnel in Braunschweig (Germany) was built and how we can use it for engineering and climate research.
Christine Lac, Jean-Pierre Chaboureau, Valéry Masson, Jean-Pierre Pinty, Pierre Tulet, Juan Escobar, Maud Leriche, Christelle Barthe, Benjamin Aouizerats, Clotilde Augros, Pierre Aumond, Franck Auguste, Peter Bechtold, Sarah Berthet, Soline Bielli, Frédéric Bosseur, Olivier Caumont, Jean-Martial Cohard, Jeanne Colin, Fleur Couvreux, Joan Cuxart, Gaëlle Delautier, Thibaut Dauhut, Véronique Ducrocq, Jean-Baptiste Filippi, Didier Gazen, Olivier Geoffroy, François Gheusi, Rachel Honnert, Jean-Philippe Lafore, Cindy Lebeaupin Brossier, Quentin Libois, Thibaut Lunet, Céline Mari, Tomislav Maric, Patrick Mascart, Maxime Mogé, Gilles Molinié, Olivier Nuissier, Florian Pantillon, Philippe Peyrillé, Julien Pergaud, Emilie Perraud, Joris Pianezze, Jean-Luc Redelsperger, Didier Ricard, Evelyne Richard, Sébastien Riette, Quentin Rodier, Robert Schoetter, Léo Seyfried, Joël Stein, Karsten Suhre, Marie Taufour, Odile Thouron, Sandra Turner, Antoine Verrelle, Benoît Vié, Florian Visentin, Vincent Vionnet, and Philippe Wautelet
Geosci. Model Dev., 11, 1929–1969, https://doi.org/10.5194/gmd-11-1929-2018, https://doi.org/10.5194/gmd-11-1929-2018, 2018
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This paper presents the Meso-NH model version 5.4, which is an atmospheric non-hydrostatic research model that is applied on synoptic to turbulent scales. The model includes advanced numerical techniques and state-of-the-art physics parameterization schemes. It has been expanded to provide capabilities for a range of Earth system prediction applications such as chemistry and aerosols, electricity and lightning, hydrology, wildland fires, volcanic eruptions, and cyclones with ocean coupling.
Anne Garnier, Thierry Trémas, Jacques Pelon, Kam-Pui Lee, Delphine Nobileau, Lydwine Gross-Colzy, Nicolas Pascal, Pascale Ferrage, and Noëlle A. Scott
Atmos. Meas. Tech., 11, 2485–2500, https://doi.org/10.5194/amt-11-2485-2018, https://doi.org/10.5194/amt-11-2485-2018, 2018
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Residual calibration biases affecting CALIPSO IIR Version 1 calibrated radiances in the Northern Hemisphere are analyzed and reduced through in-depth analysis of the IIR internal calibration procedure in conjunction with observations such as statistical comparisons with similar MODIS/Aqua channels.
Abdoulwahab Mohamed Toihir, Thierry Portafaix, Venkataraman Sivakumar, Hassan Bencherif, Andréa Pazmiño, and Nelson Bègue
Ann. Geophys., 36, 381–404, https://doi.org/10.5194/angeo-36-381-2018, https://doi.org/10.5194/angeo-36-381-2018, 2018
Jayanta Kar, Mark A. Vaughan, Kam-Pui Lee, Jason L. Tackett, Melody A. Avery, Anne Garnier, Brian J. Getzewich, William H. Hunt, Damien Josset, Zhaoyan Liu, Patricia L. Lucker, Brian Magill, Ali H. Omar, Jacques Pelon, Raymond R. Rogers, Travis D. Toth, Charles R. Trepte, Jean-Paul Vernier, David M. Winker, and Stuart A. Young
Atmos. Meas. Tech., 11, 1459–1479, https://doi.org/10.5194/amt-11-1459-2018, https://doi.org/10.5194/amt-11-1459-2018, 2018
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We present the motivation for and the implementation of the version 4.1 nighttime 532 nm parallel-channel calibration of the CALIOP lidar. The accuracy of calibration is significantly improved by raising the molecular normalization altitude from 30–34 km to 36–39 km to substantially reduce stratospheric aerosol contamination. The new calibration procedure eliminates biases in earlier versions and leads to an improved representation of stratospheric aerosols.
Joel Brito, Evelyn Freney, Pamela Dominutti, Agnes Borbon, Sophie L. Haslett, Anneke M. Batenburg, Aurelie Colomb, Regis Dupuy, Cyrielle Denjean, Frederic Burnet, Thierry Bourriane, Adrien Deroubaix, Karine Sellegri, Stephan Borrmann, Hugh Coe, Cyrille Flamant, Peter Knippertz, and Alfons Schwarzenboeck
Atmos. Chem. Phys., 18, 757–772, https://doi.org/10.5194/acp-18-757-2018, https://doi.org/10.5194/acp-18-757-2018, 2018
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This work focuses on sources of submicron aerosol particles over southern West Africa (SWA). Results have shown that isoprene, a gas-phase compound of biogenic origin, is responsible for roughly 25 % of the organic aerosol (OA) loading, under most background or urban plumes alike. This fraction represents a lower estimate from the biogenic contribution in this fairly polluted region. This work sheds light upon the role of anthropogenic and biogenic emissions on the pollution burden over SWA.
Nelson Bègue, Damien Vignelles, Gwenaël Berthet, Thierry Portafaix, Guillaume Payen, Fabrice Jégou, Hassan Benchérif, Julien Jumelet, Jean-Paul Vernier, Thibaut Lurton, Jean-Baptiste Renard, Lieven Clarisse, Vincent Duverger, Françoise Posny, Jean-Marc Metzger, and Sophie Godin-Beekmann
Atmos. Chem. Phys., 17, 15019–15036, https://doi.org/10.5194/acp-17-15019-2017, https://doi.org/10.5194/acp-17-15019-2017, 2017
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The space–time evolutions of the Calbuco plume are investigated by combining satellite, in situ aerosol counting and lidar observations, and a numerical model. All the data at Reunion Island reveal a twofold increase in the amount of aerosol with respect to the values observed before the eruption. The dynamic context has favored the spread of the plume exclusively in the Southern Hemisphere. This study highlights the role played by dynamical barriers in the transport of atmospheric species.
Nelson Bègue, Nkanyiso Mbatha, Hassan Bencherif, René Tato Loua, Venkataraman Sivakumar, and Thierry Leblanc
Ann. Geophys., 35, 1177–1194, https://doi.org/10.5194/angeo-35-1177-2017, https://doi.org/10.5194/angeo-35-1177-2017, 2017
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In this investigation a statistical analysis of the characteristics of mesospheric inversion layers (MILs) over tropical regions is presented. This study involves the analysis of 16 years of lidar observations recorded at Reunion (20.8° S, 55.5° E) and 21 years of lidar observations recorded at Mauna Loa (19.5° N, 155.6° W) together with SABER observations at these two locations. Results presented in this study confirm that SAO contributes to the formation of MILs over the tropical region.
Gwennolé Guyot, Frans Olofson, Peter Tunved, Christophe Gourbeyre, Guy Fevbre, Régis Dupuy, Christophe Bernard, Gérard Ancellet, Kathy Law, Boris Quennehen, Alfons Schwarzenboeck, Kostas Eleftheriadis, and Olivier Jourdan
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-672, https://doi.org/10.5194/acp-2017-672, 2017
Revised manuscript has not been submitted
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Cloud and aerosol properties are key parameters in the accelerated arctic warming. In this context, this study will focus on in situ cloud microphysical and optical characterization of arctic Mixed Phase Cloud combined with aerosol measurements and air mass backtrajectory simulations during the ground based CLIMSLIP-NyA campaign performed in Ny-Alesund, Svalbard. The goal is to parameterize the arctic aerosol-cloud interaction and assess the influence of anthropogenic pollution.
Guillaume Mioche, Olivier Jourdan, Julien Delanoë, Christophe Gourbeyre, Guy Febvre, Régis Dupuy, Marie Monier, Frédéric Szczap, Alfons Schwarzenboeck, and Jean-François Gayet
Atmos. Chem. Phys., 17, 12845–12869, https://doi.org/10.5194/acp-17-12845-2017, https://doi.org/10.5194/acp-17-12845-2017, 2017
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This paper is a study about the mixed-phase clouds frequently occurring in the Arctic region. It is based on airborne measurements and highlights the microphysical properties of these particular clouds composed of liquid droplets at cloud top and ice crystals below precipitating down to the surface. This work may help to improve the representation of the mixed-phase clouds in numerical prediction models as well as the retrieval of their properties from remote sensing observations.
Lucia T. Deaconu, Fabien Waquet, Damien Josset, Nicolas Ferlay, Fanny Peers, François Thieuleux, Fabrice Ducos, Nicolas Pascal, Didier Tanré, Jacques Pelon, and Philippe Goloub
Atmos. Meas. Tech., 10, 3499–3523, https://doi.org/10.5194/amt-10-3499-2017, https://doi.org/10.5194/amt-10-3499-2017, 2017
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This study presents a comparison between active (CALIOP) and passive (POLDER) remote sensing methods, developed for retrieving aerosol above-cloud optical and microphysical properties. Main results show a good agreement when the aerosol microphysics is dominated by fine-mode particles or coarse-mode dust or when the aerosol layer is well separated from the cloud below. The paper is also focused on understanding the differences between the retrievals and the limitations of each method.
Leslie David, Olivier Bock, Christian Thom, Pierre Bosser, and Jacques Pelon
Atmos. Meas. Tech., 10, 2745–2758, https://doi.org/10.5194/amt-10-2745-2017, https://doi.org/10.5194/amt-10-2745-2017, 2017
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The Raman lidar ability to retrieve atmospheric water vapor with high accuracy makes it a premium instrument in different research fields such as climatology, meteorology, or calibration of GNSS altimetry data. In order to achieve long-term stability of the measurements, the system has to be carefully calibrated. In this work we strove to investigate and mitigate the error and instability sources through numerical simulations as well as experimental tests.
Emmanuel Fontaine, Delphine Leroy, Alfons Schwarzenboeck, Julien Delanoë, Alain Protat, Fabien Dezitter, Alice Grandin, John Walter Strapp, and Lyle Edward Lilie
Atmos. Meas. Tech., 10, 2239–2252, https://doi.org/10.5194/amt-10-2239-2017, https://doi.org/10.5194/amt-10-2239-2017, 2017
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In this study we evaluate a method to estimate cloud water content (CWC) knowing cloud reflectivity. Ice hydrometeors are replace by ice oblate spheroids to simulate their reflectivity. There is no assumption on the relation between mass and their size. Then, a broad range of CWCs are compared with direct measurements of CWC. The accuracy of the method is ~ ±32 %. This study is performed in areas of convective clouds where reflectivity and CWC are especially high, what makes it unique.
Pierre Tulet, Andréa Di Muro, Aurélie Colomb, Cyrielle Denjean, Valentin Duflot, Santiago Arellano, Brice Foucart, Jérome Brioude, Karine Sellegri, Aline Peltier, Alessandro Aiuppa, Christelle Barthe, Chatrapatty Bhugwant, Soline Bielli, Patrice Boissier, Guillaume Boudoire, Thierry Bourrianne, Christophe Brunet, Fréderic Burnet, Jean-Pierre Cammas, Franck Gabarrot, Bo Galle, Gaetano Giudice, Christian Guadagno, Fréderic Jeamblu, Philippe Kowalski, Jimmy Leclair de Bellevue, Nicolas Marquestaut, Dominique Mékies, Jean-Marc Metzger, Joris Pianezze, Thierry Portafaix, Jean Sciare, Arnaud Tournigand, and Nicolas Villeneuve
Atmos. Chem. Phys., 17, 5355–5378, https://doi.org/10.5194/acp-17-5355-2017, https://doi.org/10.5194/acp-17-5355-2017, 2017
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The STRAP campaign was conducted in 2015 to investigate the volcanic plumes of Piton de La Fournaise (La Réunion, France). For the first time, measurements were conducted at the local (near the vent) and regional scales around the island. The STRAP 2015 campaign gave a unique set of multi-disciplinary data that can now be used by modellers to improve the numerical parameterisations of the physical and chemical evolution of the volcanic plumes.
Anne Garnier, Noëlle A. Scott, Jacques Pelon, Raymond Armante, Laurent Crépeau, Bruno Six, and Nicolas Pascal
Atmos. Meas. Tech., 10, 1403–1424, https://doi.org/10.5194/amt-10-1403-2017, https://doi.org/10.5194/amt-10-1403-2017, 2017
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An assessment of IIR radiances after 9.5 years of nearly continuous operation since June 2006 is presented. First, IIR is compared with similar MODIS or SEVIRI channels in various conditions. Second, clear sky measurements in each channel are compared with simulations. The first approach detects biases and/or trends, and the second approach contributes to identifying which channel deviates from the other. The analyses are based on simulations using the 4A/OP radiative transfer model.
Gwenaël Berthet, Fabrice Jégou, Valéry Catoire, Gisèle Krysztofiak, Jean-Baptiste Renard, Adam E. Bourassa, Doug A. Degenstein, Colette Brogniez, Marcel Dorf, Sebastian Kreycy, Klaus Pfeilsticker, Bodo Werner, Franck Lefèvre, Tjarda J. Roberts, Thibaut Lurton, Damien Vignelles, Nelson Bègue, Quentin Bourgeois, Daniel Daugeron, Michel Chartier, Claude Robert, Bertrand Gaubicher, and Christophe Guimbaud
Atmos. Chem. Phys., 17, 2229–2253, https://doi.org/10.5194/acp-17-2229-2017, https://doi.org/10.5194/acp-17-2229-2017, 2017
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Since the last major volcanic event, i.e. the Pinatubo eruption in 1991, only
moderateeruptions have regularly injected sulfur into the stratosphere, typically enhancing the aerosol loading for several months. We investigate here for the first time the chemical perturbation associated with the Sarychev eruption in June 2009, using balloon-borne instruments and model calculations. Some chemical compounds are significantly affected by the aerosols, but the impact on stratospheric ozone is weak.
Lucas Vaz Peres, Hassan Bencherif, Nkanyiso Mbatha, André Passaglia Schuch, Abdoulwahab Mohamed Toihir, Nelson Bègue, Thierry Portafaix, Vagner Anabor, Damaris Kirsch Pinheiro, Neusa Maria Paes Leme, José Valentin Bageston, and Nelson Jorge Schuch
Ann. Geophys., 35, 25–37, https://doi.org/10.5194/angeo-35-25-2017, https://doi.org/10.5194/angeo-35-25-2017, 2017
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In this paper, we analyze the total ozone column over the Southern Space Observatory, Brazil, between 1992 and 2014 by Brewer spectrometer and TOMS and OMI satellite instruments, finding good agreement between the two. In addition, the seasonal TOC variation is dominated by an annual cycle, and the Quasi-Biennial Oscillation modulation was the main mode of interannual variability and in opposite phase to the total ozone column anomaly time series.
Valery Shcherbakov, Olivier Jourdan, Christiane Voigt, Jean-Francois Gayet, Aurélien Chauvigne, Alfons Schwarzenboeck, Andreas Minikin, Marcus Klingebiel, Ralf Weigel, Stephan Borrmann, Tina Jurkat, Stefan Kaufmann, Romy Schlage, Christophe Gourbeyre, Guy Febvre, Tatyana Lapyonok, Wiebke Frey, Sergej Molleker, and Bernadett Weinzierl
Atmos. Chem. Phys., 16, 11883–11897, https://doi.org/10.5194/acp-16-11883-2016, https://doi.org/10.5194/acp-16-11883-2016, 2016
Jean-Pierre Chaboureau, Cyrille Flamant, Thibaut Dauhut, Cécile Kocha, Jean-Philippe Lafore, Chistophe Lavaysse, Fabien Marnas, Mohamed Mokhtari, Jacques Pelon, Irene Reinares Martínez, Kerstin Schepanski, and Pierre Tulet
Atmos. Chem. Phys., 16, 6977–6995, https://doi.org/10.5194/acp-16-6977-2016, https://doi.org/10.5194/acp-16-6977-2016, 2016
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The Fennec field campaign conducted in June 2011 led to the first observational data set ever obtained that documents the Saharan atmospheric boundary layer under the influence of the heat low. In addition to the aircraft operation, four dust forecasts were run at low and high resolutions with convection-parameterizing and convection-permitting models, respectively. The unique airborne and ground-based data sets allowed the first ever intercomparison of dust forecasts over the western Sahara.
Gerard Ancellet, Jacques Pelon, Julien Totems, Patrick Chazette, Ariane Bazureau, Michaël Sicard, Tatiana Di Iorio, Francois Dulac, and Marc Mallet
Atmos. Chem. Phys., 16, 4725–4742, https://doi.org/10.5194/acp-16-4725-2016, https://doi.org/10.5194/acp-16-4725-2016, 2016
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A multi-lidar analysis conducted in the Mediterranean basin compares the impact of the long-range transport of North American biomass burning aerosols with the role of frequently observed Saharan dust outbreaks. This paper provides a detailed analysis of the potential North American aerosol sources, their transport to Europe and the mixing of different aerosol sources, using simulations of a particle dispersion model and lidar measurements of the aerosol optical properties.
Patrick Chazette, Julien Totems, Gérard Ancellet, Jacques Pelon, and Michaël Sicard
Atmos. Chem. Phys., 16, 2863–2875, https://doi.org/10.5194/acp-16-2863-2016, https://doi.org/10.5194/acp-16-2863-2016, 2016
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We performed synergetic active and passive remote-sensing observations at Minorca (Spain), over more than 3 weeks in spring 2013. We characterized the aerosol optical properties and type using a combination of Rayleigh–Mie–Raman lidar and sun-photometer data. Results show a high variability due to changing atmospheric transport regimes and aerosol sources. Such variability significantly influences the radiative balance through the entire atmosphere and then the climate of the Mediterranean area.
C. Denjean, F. Cassola, A. Mazzino, S. Triquet, S. Chevaillier, N. Grand, T. Bourrianne, G. Momboisse, K. Sellegri, A. Schwarzenbock, E. Freney, M. Mallet, and P. Formenti
Atmos. Chem. Phys., 16, 1081–1104, https://doi.org/10.5194/acp-16-1081-2016, https://doi.org/10.5194/acp-16-1081-2016, 2016
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This study investigates the size distribution, chemical composition, and optical properties of Saharan mineral dust transported over the western Mediterranean using in situ measurements collected from aircraft. Their variability due to altitude, time of transport, and mixing rate with pollution particles are discussed. We found moderate light absorption of the dust plumes even in the presence of pollution particles and the persistence of large dust particles after transport in the Mediterranean.
M. Mallet, F. Dulac, P. Formenti, P. Nabat, J. Sciare, G. Roberts, J. Pelon, G. Ancellet, D. Tanré, F. Parol, C. Denjean, G. Brogniez, A. di Sarra, L. Alados-Arboledas, J. Arndt, F. Auriol, L. Blarel, T. Bourrianne, P. Chazette, S. Chevaillier, M. Claeys, B. D'Anna, Y. Derimian, K. Desboeufs, T. Di Iorio, J.-F. Doussin, P. Durand, A. Féron, E. Freney, C. Gaimoz, P. Goloub, J. L. Gómez-Amo, M. J. Granados-Muñoz, N. Grand, E. Hamonou, I. Jankowiak, M. Jeannot, J.-F. Léon, M. Maillé, S. Mailler, D. Meloni, L. Menut, G. Momboisse, J. Nicolas, T. Podvin, V. Pont, G. Rea, J.-B. Renard, L. Roblou, K. Schepanski, A. Schwarzenboeck, K. Sellegri, M. Sicard, F. Solmon, S. Somot, B Torres, J. Totems, S. Triquet, N. Verdier, C. Verwaerde, F. Waquet, J. Wenger, and P. Zapf
Atmos. Chem. Phys., 16, 455–504, https://doi.org/10.5194/acp-16-455-2016, https://doi.org/10.5194/acp-16-455-2016, 2016
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The aim of this article is to present an experimental campaign over the Mediterranean focused on aerosol-radiation measurements and modeling. Results indicate an important atmospheric loading associated with a moderate absorbing ability of mineral dust. Observations suggest a complex vertical structure and size distributions characterized by large aerosols within dust plumes. The radiative effect is highly variable, with negative forcing over the Mediterranean and positive over northern Africa.
Q. J. Zhang, M. Beekmann, E. Freney, K. Sellegri, J. M. Pichon, A. Schwarzenboeck, A. Colomb, T. Bourrianne, V. Michoud, and A. Borbon
Atmos. Chem. Phys., 15, 13973–13992, https://doi.org/10.5194/acp-15-13973-2015, https://doi.org/10.5194/acp-15-13973-2015, 2015
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Secondary organic aerosol (SOA) is an important pollutant formed from megacity emissions at a regional scale. An original method based on ratios of different pollutants is used to specifically validate the aerosol scheme (the volatility basis set approach) within a CTM. The method is applied to airborne measurements performed within the Paris plume during the MEGAPOLI summer campaign. Simulations indicate that SOA of anthropogenic origin has a significant impact on regional air quality.
M. Pikridas, J. Sciare, F. Freutel, S. Crumeyrolle, S.-L. von der Weiden-Reinmüller, A. Borbon, A. Schwarzenboeck, M. Merkel, M. Crippa, E. Kostenidou, M. Psichoudaki, L. Hildebrandt, G. J. Engelhart, T. Petäjä, A. S. H. Prévôt, F. Drewnick, U. Baltensperger, A. Wiedensohler, M. Kulmala, M. Beekmann, and S. N. Pandis
Atmos. Chem. Phys., 15, 10219–10237, https://doi.org/10.5194/acp-15-10219-2015, https://doi.org/10.5194/acp-15-10219-2015, 2015
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Aerosol size distribution measurements from three ground sites, two mobile laboratories, and one airplane are combined to investigate the spatial and temporal variability of ultrafine particles in and around Paris during the summer and winter MEGAPOLI campaigns. The role of nucleation as a particle source and the influence of Paris emissions on their surroundings are examined.
C. Rose, K. Sellegri, E. Freney, R. Dupuy, A. Colomb, J.-M. Pichon, M. Ribeiro, T. Bourianne, F. Burnet, and A. Schwarzenboeck
Atmos. Chem. Phys., 15, 10203–10218, https://doi.org/10.5194/acp-15-10203-2015, https://doi.org/10.5194/acp-15-10203-2015, 2015
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In the present paper we report airborne measurements of new particle formation (NPF) above the Mediterranean Sea (HYMEX campaign). We show that NPF occurs over large areas above the sea, but the process is clearly promoted at high altitude, above 1000m, i.e. frequently in the free troposphere. NPF also seems to be mainly influenced by local processes occurring above the sea. After their formation, particles slowly grow at high altitude while not being greatly depleted or affected by coagulation.
P. Tuccella, G. Curci, G. A. Grell, G. Visconti, S. Crumeyrolle, A. Schwarzenboeck, and A. A. Mensah
Geosci. Model Dev., 8, 2749–2776, https://doi.org/10.5194/gmd-8-2749-2015, https://doi.org/10.5194/gmd-8-2749-2015, 2015
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A parameterization for secondary organic aerosol (SOA) production based on the volatility basis set (VBS) approach has been coupled with microphysics and radiative schemes in the WRF-Chem model. The new chemistry was evaluated on a cloud-resolving scale against ground-based and aircraft measurements collected during the IMPACT-EUCAARI campaign, and complemented with satellite data from MODIS. Sensitivity tests have been performed to study the impact of SOA on cloud prediction and development.
H. Petetin, M. Beekmann, A. Colomb, H. A. C. Denier van der Gon, J.-C. Dupont, C. Honoré, V. Michoud, Y. Morille, O. Perrussel, A. Schwarzenboeck, J. Sciare, A. Wiedensohler, and Q. J. Zhang
Atmos. Chem. Phys., 15, 9799–9818, https://doi.org/10.5194/acp-15-9799-2015, https://doi.org/10.5194/acp-15-9799-2015, 2015
M. Beekmann, A. S. H. Prévôt, F. Drewnick, J. Sciare, S. N. Pandis, H. A. C. Denier van der Gon, M. Crippa, F. Freutel, L. Poulain, V. Ghersi, E. Rodriguez, S. Beirle, P. Zotter, S.-L. von der Weiden-Reinmüller, M. Bressi, C. Fountoukis, H. Petetin, S. Szidat, J. Schneider, A. Rosso, I. El Haddad, A. Megaritis, Q. J. Zhang, V. Michoud, J. G. Slowik, S. Moukhtar, P. Kolmonen, A. Stohl, S. Eckhardt, A. Borbon, V. Gros, N. Marchand, J. L. Jaffrezo, A. Schwarzenboeck, A. Colomb, A. Wiedensohler, S. Borrmann, M. Lawrence, A. Baklanov, and U. Baltensperger
Atmos. Chem. Phys., 15, 9577–9591, https://doi.org/10.5194/acp-15-9577-2015, https://doi.org/10.5194/acp-15-9577-2015, 2015
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A detailed characterization of air quality in the Paris (France) agglomeration, a megacity, during two summer and winter intensive campaigns and from additional 1-year observations, revealed that about 70% of the fine particulate matter (PM) at urban background is transported into the megacity from upwind regions. Unexpectedly, a major part of organic PM is of modern origin (woodburning and cooking activities, secondary formation from biogenic VOC).
M. Mokhtari, P. Tulet, C. Fischer, Y. Bouteloup, F. Bouyssel, and O. Brachemi
Atmos. Chem. Phys., 15, 9063–9082, https://doi.org/10.5194/acp-15-9063-2015, https://doi.org/10.5194/acp-15-9063-2015, 2015
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The seasonal cycle and optical properties of mineral dust aerosols in northern Africa were simulated for the period from 2006 to 2010 using the numerical atmospheric model ALADIN (Aire Limitée Adaptation dynamique Développement InterNational) coupled to the surface scheme SURFEX (SURFace EXternalisée). These simulations aim to quantify the dust emission and deposition and establish a three-dimensional dust aerosol distribution and extinction climatology over northern Africa.
A. Garnier, J. Pelon, M. A. Vaughan, D. M. Winker, C. R. Trepte, and P. Dubuisson
Atmos. Meas. Tech., 8, 2759–2774, https://doi.org/10.5194/amt-8-2759-2015, https://doi.org/10.5194/amt-8-2759-2015, 2015
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Cloud absorption optical depths retrieved at 12.05 microns are compared to extinction optical depths retrieved at 0.532 microns from perfectly co-located observations of single-layered semi-transparent cirrus over oceans made by the space-borne CALIPSO IIR infrared radiometer and CALIOP lidar. A new relationship describing the temperature-dependent effect of multiple scattering in the CALIOP retrievals is derived and discussed.
C. Barbet, L. Deguillaume, N. Chaumerliac, M. Leriche, A. Berger, E. Freney, A. Colomb, K. Sellegri, L. Patryl, and P. Armand
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-15-13395-2015, https://doi.org/10.5194/acpd-15-13395-2015, 2015
Preprint withdrawn
L. Marelle, J.-C. Raut, J. L. Thomas, K. S. Law, B. Quennehen, G. Ancellet, J. Pelon, A. Schwarzenboeck, and J. D. Fast
Atmos. Chem. Phys., 15, 3831–3850, https://doi.org/10.5194/acp-15-3831-2015, https://doi.org/10.5194/acp-15-3831-2015, 2015
T. Fauchez, P. Dubuisson, C. Cornet, F. Szczap, A. Garnier, J. Pelon, and K. Meyer
Atmos. Meas. Tech., 8, 633–647, https://doi.org/10.5194/amt-8-633-2015, https://doi.org/10.5194/amt-8-633-2015, 2015
F. Marenco, V. Amiridis, E. Marinou, A. Tsekeri, and J. Pelon
Atmos. Chem. Phys., 14, 11871–11881, https://doi.org/10.5194/acp-14-11871-2014, https://doi.org/10.5194/acp-14-11871-2014, 2014
E. Fontaine, A. Schwarzenboeck, J. Delanoë, W. Wobrock, D. Leroy, R. Dupuy, C. Gourbeyre, and A. Protat
Atmos. Chem. Phys., 14, 11367–11392, https://doi.org/10.5194/acp-14-11367-2014, https://doi.org/10.5194/acp-14-11367-2014, 2014
G. Ancellet, J. Pelon, Y. Blanchard, B. Quennehen, A. Bazureau, K. S. Law, and A. Schwarzenboeck
Atmos. Chem. Phys., 14, 8235–8254, https://doi.org/10.5194/acp-14-8235-2014, https://doi.org/10.5194/acp-14-8235-2014, 2014
C. Jouan, J. Pelon, E. Girard, G. Ancellet, J. P. Blanchet, and J. Delanoë
Atmos. Chem. Phys., 14, 1205–1224, https://doi.org/10.5194/acp-14-1205-2014, https://doi.org/10.5194/acp-14-1205-2014, 2014
P. Dubuisson, H. Herbin, F. Minvielle, M. Compiègne, F. Thieuleux, F. Parol, and J. Pelon
Atmos. Meas. Tech., 7, 359–371, https://doi.org/10.5194/amt-7-359-2014, https://doi.org/10.5194/amt-7-359-2014, 2014
J.-F. Gayet, V. Shcherbakov, L. Bugliaro, A. Protat, J. Delanoë, J. Pelon, and A. Garnier
Atmos. Chem. Phys., 14, 899–912, https://doi.org/10.5194/acp-14-899-2014, https://doi.org/10.5194/acp-14-899-2014, 2014
C. Tsamalis, A. Chédin, J. Pelon, and V. Capelle
Atmos. Chem. Phys., 13, 11235–11257, https://doi.org/10.5194/acp-13-11235-2013, https://doi.org/10.5194/acp-13-11235-2013, 2013
J.-L. Baray, Y. Courcoux, P. Keckhut, T. Portafaix, P. Tulet, J.-P. Cammas, A. Hauchecorne, S. Godin Beekmann, M. De Mazière, C. Hermans, F. Desmet, K. Sellegri, A. Colomb, M. Ramonet, J. Sciare, C. Vuillemin, C. Hoareau, D. Dionisi, V. Duflot, H. Vérèmes, J. Porteneuve, F. Gabarrot, T. Gaudo, J.-M. Metzger, G. Payen, J. Leclair de Bellevue, C. Barthe, F. Posny, P. Ricaud, A. Abchiche, and R. Delmas
Atmos. Meas. Tech., 6, 2865–2877, https://doi.org/10.5194/amt-6-2865-2013, https://doi.org/10.5194/amt-6-2865-2013, 2013
O. Bock, P. Bosser, T. Bourcy, L. David, F. Goutail, C. Hoareau, P. Keckhut, D. Legain, A. Pazmino, J. Pelon, K. Pipis, G. Poujol, A. Sarkissian, C. Thom, G. Tournois, and D. Tzanos
Atmos. Meas. Tech., 6, 2777–2802, https://doi.org/10.5194/amt-6-2777-2013, https://doi.org/10.5194/amt-6-2777-2013, 2013
O. Sourdeval, L. C. -Labonnote, G. Brogniez, O. Jourdan, J. Pelon, and A. Garnier
Atmos. Chem. Phys., 13, 8229–8244, https://doi.org/10.5194/acp-13-8229-2013, https://doi.org/10.5194/acp-13-8229-2013, 2013
V. Masson, P. Le Moigne, E. Martin, S. Faroux, A. Alias, R. Alkama, S. Belamari, A. Barbu, A. Boone, F. Bouyssel, P. Brousseau, E. Brun, J.-C. Calvet, D. Carrer, B. Decharme, C. Delire, S. Donier, K. Essaouini, A.-L. Gibelin, H. Giordani, F. Habets, M. Jidane, G. Kerdraon, E. Kourzeneva, M. Lafaysse, S. Lafont, C. Lebeaupin Brossier, A. Lemonsu, J.-F. Mahfouf, P. Marguinaud, M. Mokhtari, S. Morin, G. Pigeon, R. Salgado, Y. Seity, F. Taillefer, G. Tanguy, P. Tulet, B. Vincendon, V. Vionnet, and A. Voldoire
Geosci. Model Dev., 6, 929–960, https://doi.org/10.5194/gmd-6-929-2013, https://doi.org/10.5194/gmd-6-929-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Microphysical modelling of aerosol scavenging by different types of clouds: description and validation of the approach
Insights into the sources of ultrafine particle numbers at six European urban sites obtained by investigating COVID-19 lockdowns
In-plume and out-of-plume analysis of aerosol–cloud interactions derived from the 2014–2015 Holuhraun volcanic eruption
Impacts of atmospheric circulation patterns and cloud inhibition on aerosol radiative effect and boundary layer structure during winter air pollution in Sichuan Basin, China
Investigating the sign of stratocumulus adjustments to aerosols in the ICON global storm-resolving model
A model study investigating the sensitivity of aerosol forcing to the volatilities of semi-volatile organic compounds
Decomposing the effective radiative forcing of anthropogenic aerosols based on CMIP6 Earth system models
Modeling impacts of dust mineralogy on fast climate response
Uncertainties in laboratory-measured shortwave refractive indices of mineral dust aerosols and derived optical properties: a theoretical assessment
Diagnosing uncertainties in global biomass burning emission inventories and their impact on modeled air pollutants
Role of atmospheric aerosols in severe winter fog over the Indo-Gangetic Plain of India: a case study
Long-term variability in black carbon emissions constrained by gap-filled absorption aerosol optical depth and associated premature mortality in China
Intercomparison of aerosol optical depths from four reanalyses and their multi-reanalysis consensus
Global aviation contrail climate effects from 2019 to 2021
Rapid iodine oxoacid nucleation enhanced by dimethylamine in broad marine regions
Simulations of the impact of cloud condensation nuclei and ice-nucleating particles perturbations on the microphysics and radar reflectivity factor of stratiform mixed-phase clouds
Aerosols in the central Arctic cryosphere: satellite and model integrated insights during Arctic spring and summer
Observationally constrained regional variations of shortwave absorption by iron oxides emphasize the cooling effect of dust
Droplet collection efficiencies inferred from satellite retrievals constrain effective radiative forcing of aerosol–cloud interactions
Predicting Hygroscopic Growth of Organosulfur Aerosol Particles Using COSMOtherm
Global aerosol-type classification using a new hybrid algorithm and Aerosol Robotic Network data
Simulated phase state and viscosity of secondary organic aerosols over China
Comparing the simulated influence of biomass burning plumes on low-level clouds over the southeastern Atlantic under varying smoke conditions
Improved simulations of biomass burning aerosol optical properties and lifetimes in the NASA GEOS Model during the ORACLES-I campaign
Retrieval of refractive index and water content for the coating materials of aged black carbon aerosol based on optical properties: a theoretical analysis
Synergistic effects of previous winter NAO and ENSO on the spring dust activities in North China
Sharp increase in Saharan dust intrusions over the western Euro-Mediterranean in February–March 2020–2022 and associated atmospheric circulation
Temporal and spatial variations in dust activity in Australia based on remote sensing and reanalysis datasets
Sensitivity of global direct aerosol shortwave radiative forcing to uncertainties in aerosol optical properties
Molecular-level study on the role of methanesulfonic acid in iodine oxoacid nucleation
Improving estimation of a record breaking East Asian dust storm emission with lagged aerosol Ångström Exponent observations
Regional to global distributions, trends, and drivers of biogenic volatile organic compound emission from 2001 to 2020
Impacts of ice-nucleating particles on cirrus clouds and radiation derived from global model simulations with MADE3 in EMAC
Seasonal characteristics of emission, distribution, and radiative effect of marine organic aerosols over the western Pacific Ocean: an investigation with a coupled regional climate aerosol model
Fire–precipitation interactions amplify the quasi-biennial variability in fires over southern Mexico and Central America
Improved estimates of smoke exposure during Australia fire seasons: importance of quantifying plume injection heights
New particle formation induced by anthropogenic–biogenic interactions on the southeastern Tibetan Plateau
Investigation of observed dust trends over the Middle East region in NASA Goddard Earth Observing System (GEOS) model simulations
Impact of Biomass Burning Aerosols (BBA) on the tropical African climate in an ocean-atmosphere-aerosols coupled climate model
A new process-based and scale-aware desert dust emission scheme for global climate models – Part II: Evaluation in the Community Earth System Model version 2 (CESM2)
How well do Earth system models reproduce the observed aerosol response to rapid emission reductions? A COVID-19 case study
Global modeling of aerosol nucleation with an explicit chemical mechanism for highly oxygenated organic molecules (HOMs)
Measurement report: Source attribution and estimation of black carbon levels in an urban hotspot of the central Po Valley: An integrated approach combining high-resolution dispersion modelling and micro-aethalometers
Observationally constrained analysis of sulfur cycle in the marine atmosphere with NASA ATom measurements and AeroCom model simulations
Impact of acidity and surface-modulated acid dissociation on cloud response to organic aerosol
The contribution of residential wood combustion to the PM2.5 concentrations in the Helsinki metropolitan area
Analysis of atmospheric particle growth based on vapor concentrations measured at the high-altitude GAW station Chacaltaya in the Bolivian Andes
Expanding the simulation of East Asian super dust storms: physical transport mechanisms impacting the western Pacific
Aerosol composition, air quality, and boundary layer dynamics in the urban background of Stuttgart in winter
Improving 3-day deterministic air pollution forecasts using machine learning algorithms
Pascal Lemaitre, Arnaud Quérel, Alexis Dépée, Alice Guerra Devigne, Marie Monier, Thibault Hiron, Chloé Soto Minguez, Daniel Hardy, and Andrea Flossmann
Atmos. Chem. Phys., 24, 9713–9732, https://doi.org/10.5194/acp-24-9713-2024, https://doi.org/10.5194/acp-24-9713-2024, 2024
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A new in-cloud scavenging scheme is proposed. It is based on a microphysical model of cloud formation and may be applied to long-distance atmospheric transport models (> 100 km) and climatic models. This model is applied to the two most extreme precipitating cloud types in terms of both relative humidity and vertical extension: cumulonimbus and stratus.
Alex Rowell, James Brean, David C. S. Beddows, Tuukka Petäjä, Máté Vörösmarty, Imre Salma, Jarkko V. Niemi, Hanna E. Manninen, Dominik van Pinxteren, Thomas Tuch, Kay Weinhold, Zongbo Shi, and Roy M. Harrison
Atmos. Chem. Phys., 24, 9515–9531, https://doi.org/10.5194/acp-24-9515-2024, https://doi.org/10.5194/acp-24-9515-2024, 2024
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Different sources of airborne particles in the atmospheres of four European cities were distinguished by recognising their particle size distributions using a statistical procedure, positive matrix factorisation. The various sources responded differently to the changes in emissions associated with COVID-19 lockdowns, and the reasons are investigated. While traffic emissions generally decreased, particles formed from reactions of atmospheric gases decreased in some cities but increased in others.
Amy H. Peace, Ying Chen, George Jordan, Daniel G. Partridge, Florent Malavelle, Eliza Duncan, and Jim M. Haywood
Atmos. Chem. Phys., 24, 9533–9553, https://doi.org/10.5194/acp-24-9533-2024, https://doi.org/10.5194/acp-24-9533-2024, 2024
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Natural aerosols from volcanic eruptions can help us understand how anthropogenic aerosols modify climate. We use observations and model simulations of the 2014–2015 Holuhraun eruption plume to examine aerosol–cloud interactions in September 2014. We find a shift to clouds with smaller, more numerous cloud droplets in the first 2 weeks of the eruption. In the third week, the background meteorology and previous conditions experienced by air masses modulate the aerosol perturbation to clouds.
Hua Lu, Min Xie, Bingliang Zhuang, Danyang Ma, Bojun Liu, Yangzhihao Zhan, Tijian Wang, Shu Li, Mengmeng Li, and Kuanguang Zhu
Atmos. Chem. Phys., 24, 8963–8982, https://doi.org/10.5194/acp-24-8963-2024, https://doi.org/10.5194/acp-24-8963-2024, 2024
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To identify cloud, aerosol, and planetary boundary layer (PBL) interactions from an air quality perspective, we summarized two pollution patterns characterized by denser liquid cloud and by obvious cloud radiation interaction (CRI). Numerical simulation experiments showed CRI could cause a 50 % reduction in aerosol radiation interaction (ARI) under a low-trough system. The results emphasized the nonnegligible role of CRI and its inhibition of ARI under wet and cloudy pollution synoptic patterns.
Emilie Fons, Ann Kristin Naumann, David Neubauer, Theresa Lang, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 8653–8675, https://doi.org/10.5194/acp-24-8653-2024, https://doi.org/10.5194/acp-24-8653-2024, 2024
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Aerosols can modify the liquid water path (LWP) of stratocumulus and, thus, their radiative effect. We compare storm-resolving model and satellite data that disagree on the sign of LWP adjustments and diagnose this discrepancy with causal inference. We find that strong precipitation, the absence of wet scavenging, and cloud deepening under a weak inversion contribute to positive LWP adjustments to aerosols in the model, despite weak negative effects from cloud-top entrainment enhancement.
Muhammed Irfan, Thomas Kühn, Taina Yli-Juuti, Anton Laakso, Eemeli Holopainen, Douglas R. Worsnop, Annele Virtanen, and Harri Kokkola
Atmos. Chem. Phys., 24, 8489–8506, https://doi.org/10.5194/acp-24-8489-2024, https://doi.org/10.5194/acp-24-8489-2024, 2024
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The study examines how the volatility of semi-volatile organic compounds affects secondary organic aerosol (SOA) formation and climate. Our simulations show that uncertainties in these volatilities influence aerosol mass and climate impacts. Accurate representation of these compounds in climate models is crucial for predicting global climate patterns.
Alkiviadis Kalisoras, Aristeidis K. Georgoulias, Dimitris Akritidis, Robert J. Allen, Vaishali Naik, Chaincy Kuo, Sophie Szopa, Pierre Nabat, Dirk Olivié, Twan van Noije, Philippe Le Sager, David Neubauer, Naga Oshima, Jane Mulcahy, Larry W. Horowitz, and Prodromos Zanis
Atmos. Chem. Phys., 24, 7837–7872, https://doi.org/10.5194/acp-24-7837-2024, https://doi.org/10.5194/acp-24-7837-2024, 2024
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Effective radiative forcing (ERF) is a metric for estimating how human activities and natural agents change the energy flow into and out of the Earth’s climate system. We investigate the anthropogenic aerosol ERF, and we estimate the contribution of individual processes to the total ERF using simulations from Earth system models within the Coupled Model Intercomparison Project Phase 6 (CMIP6). Our findings highlight that aerosol–cloud interactions drive ERF variability during the last 150 years.
Qianqian Song, Paul Ginoux, María Gonçalves Ageitos, Ron L. Miller, Vincenzo Obiso, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 7421–7446, https://doi.org/10.5194/acp-24-7421-2024, https://doi.org/10.5194/acp-24-7421-2024, 2024
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We implement and simulate the distribution of eight dust minerals in the GFDL AM4.0 model. We found that resolving the eight minerals reduces dust absorption compared to the homogeneous dust used in the standard GFDL AM4.0 model that assumes a globally uniform hematite content of 2.7 % by volume. Resolving dust mineralogy results in significant impacts on radiation, land surface temperature, surface winds, and precipitation over North Africa in summer.
Senyi Kong, Zheng Wang, and Lei Bi
Atmos. Chem. Phys., 24, 6911–6935, https://doi.org/10.5194/acp-24-6911-2024, https://doi.org/10.5194/acp-24-6911-2024, 2024
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The retrieval of refractive indices of dust aerosols from laboratory optical measurements is commonly done assuming spherical particles. This paper aims to investigate the uncertainties in the shortwave refractive indices and corresponding optical properties by considering non-spherical and inhomogeneous models for dust samples. The study emphasizes the significance of using non-spherical models for simulating dust aerosols.
Wenxuan Hua, Sijia Lou, Xin Huang, Lian Xue, Ke Ding, Zilin Wang, and Aijun Ding
Atmos. Chem. Phys., 24, 6787–6807, https://doi.org/10.5194/acp-24-6787-2024, https://doi.org/10.5194/acp-24-6787-2024, 2024
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In this study, we diagnose uncertainties in carbon monoxide and organic carbon emissions from four inventories for seven major wildfire-prone regions. Uncertainties in vegetation classification methods, fire detection products, and cloud obscuration effects lead to bias in these biomass burning (BB) emission inventories. By comparing simulations with measurements, we provide certain inventory recommendations. Our study has implications for reducing uncertainties in emissions in further studies.
Chandrakala Bharali, Mary Barth, Rajesh Kumar, Sachin D. Ghude, Vinayak Sinha, and Baerbel Sinha
Atmos. Chem. Phys., 24, 6635–6662, https://doi.org/10.5194/acp-24-6635-2024, https://doi.org/10.5194/acp-24-6635-2024, 2024
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This study examines the role of atmospheric aerosols in winter fog over the Indo-Gangetic Plains of India using WRF-Chem. The increase in RH with aerosol–radiation feedback (ARF) is found to be important for fog formation as it promotes the growth of aerosols in the polluted environment. Aqueous-phase chemistry in the fog increases PM2.5 concentration, further affecting ARF. ARF and aqueous-phase chemistry affect the fog intensity and the timing of fog formation by ~1–2 h.
Wenxin Zhao, Yu Zhao, Yu Zheng, Dong Chen, Jinyuan Xin, Kaitao Li, Huizheng Che, Zhengqiang Li, Mingrui Ma, and Yun Hang
Atmos. Chem. Phys., 24, 6593–6612, https://doi.org/10.5194/acp-24-6593-2024, https://doi.org/10.5194/acp-24-6593-2024, 2024
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We evaluate the long-term (2000–2020) variabilities of aerosol absorption optical depth, black carbon emissions, and associated health risks in China with an integrated framework that combines multiple observations and modeling techniques. We demonstrate the remarkable emission abatement resulting from the implementation of national pollution controls and show how human activities affected the emissions with a spatiotemporal heterogeneity, thus supporting differentiated policy-making by region.
Peng Xian, Jeffrey S. Reid, Melanie Ades, Angela Benedetti, Peter R. Colarco, Arlindo da Silva, Tom F. Eck, Johannes Flemming, Edward J. Hyer, Zak Kipling, Samuel Rémy, Tsuyoshi Thomas Sekiyama, Taichu Tanaka, Keiya Yumimoto, and Jianglong Zhang
Atmos. Chem. Phys., 24, 6385–6411, https://doi.org/10.5194/acp-24-6385-2024, https://doi.org/10.5194/acp-24-6385-2024, 2024
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The study compares and evaluates monthly AOD of four reanalyses (RA) and their consensus (i.e., ensemble mean). The basic verification characteristics of these RA versus both AERONET and MODIS retrievals are presented. The study discusses the strength of each RA and identifies regions where divergence and challenges are prominent. The RA consensus usually performs very well on a global scale in terms of how well it matches the observational data, making it a good choice for various applications.
Roger Teoh, Zebediah Engberg, Ulrich Schumann, Christiane Voigt, Marc Shapiro, Susanne Rohs, and Marc E. J. Stettler
Atmos. Chem. Phys., 24, 6071–6093, https://doi.org/10.5194/acp-24-6071-2024, https://doi.org/10.5194/acp-24-6071-2024, 2024
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The radiative forcing (RF) due to aviation contrails is comparable to that caused by CO2. We estimate that global contrail net RF in 2019 was 62.1 mW m−2. This is ~1/2 the previous best estimate for 2018. Contrail RF varies regionally due to differences in conditions required for persistent contrails. COVID-19 reduced contrail RF by 54% in 2020 relative to 2019. Globally, 2 % of all flights account for 80 % of the annual contrail energy forcing, suggesting a opportunity to mitigate contrail RF.
Haotian Zu, Biwu Chu, Yiqun Lu, Ling Liu, and Xiuhui Zhang
Atmos. Chem. Phys., 24, 5823–5835, https://doi.org/10.5194/acp-24-5823-2024, https://doi.org/10.5194/acp-24-5823-2024, 2024
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The nucleation of iodic acid (HIO3) and iodous acid (HIO2) was proven to be critical in marine areas. However, HIO3–HIO2 nucleation cannot effectively derive the rapid nucleation in some polluted coasts. We find a significant enhancement of dimethylamine (DMA) on the HIO3–HIO2 nucleation in marine and polar regions with abundant DMA sources, which may establish reasonable connections between the HIO3–HIO2 nucleation and the rapid formation of new particles in polluted marine and polar regions.
Junghwa Lee, Patric Seifert, Tempei Hashino, Maximilian Maahn, Fabian Senf, and Oswald Knoth
Atmos. Chem. Phys., 24, 5737–5756, https://doi.org/10.5194/acp-24-5737-2024, https://doi.org/10.5194/acp-24-5737-2024, 2024
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Spectral bin model simulations of an idealized supercooled stratiform cloud were performed with the AMPS model for variable CCN and INP concentrations. We performed radar forward simulations with PAMTRA to transfer the simulations into radar observational space. The derived radar reflectivity factors were compared to observational studies of stratiform mixed-phase clouds. These studies report a similar response of the radar reflectivity factor to aerosol perturbations as we found in our study.
Basudev Swain, Marco Vountas, Aishwarya Singh, Nidhi L. Anchan, Adrien Deroubaix, Luca Lelli, Yanick Ziegler, Sachin S. Gunthe, Hartmut Bösch, and John P. Burrows
Atmos. Chem. Phys., 24, 5671–5693, https://doi.org/10.5194/acp-24-5671-2024, https://doi.org/10.5194/acp-24-5671-2024, 2024
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Arctic amplification (AA) accelerates the warming of the central Arctic cryosphere and affects aerosol dynamics. Limited observations hinder a comprehensive analysis. This study uses AEROSNOW aerosol optical density (AOD) data and GEOS-Chem simulations to assess AOD variability. Discrepancies highlight the need for improved observational integration into models to refine our understanding of aerosol effects on cloud microphysics, ice nucleation, and radiative forcing under evolving AA.
Vincenzo Obiso, María Gonçalves Ageitos, Carlos Pérez García-Pando, Jan P. Perlwitz, Gregory L. Schuster, Susanne E. Bauer, Claudia Di Biagio, Paola Formenti, Kostas Tsigaridis, and Ron L. Miller
Atmos. Chem. Phys., 24, 5337–5367, https://doi.org/10.5194/acp-24-5337-2024, https://doi.org/10.5194/acp-24-5337-2024, 2024
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We calculate the dust direct radiative effect (DRE) in an Earth system model accounting for regionally varying soil mineralogy through a new observationally constrained method. Linking dust absorption at solar wavelengths to the varying amount of specific minerals (i.e., iron oxides) improves the modeled range of dust single scattering albedo compared to observations and increases the global cooling by dust. Our results may contribute to improved estimates of the dust DRE and its climate impact.
Charlotte M. Beall, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Adam Varble, Kentaroh Suzuki, and Takuro Michibata
Atmos. Chem. Phys., 24, 5287–5302, https://doi.org/10.5194/acp-24-5287-2024, https://doi.org/10.5194/acp-24-5287-2024, 2024
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Single-layer warm liquid clouds cover nearly one-third of the Earth's surface, and uncertainties regarding the impact of aerosols on their radiative properties pose a significant challenge to climate prediction. Here, we demonstrate how satellite observations can be used to constrain Earth system model estimates of the radiative forcing from the interactions of aerosols with clouds due to warm rain processes.
Zijun Li, Angela Buchholz, and Noora Hyttinen
EGUsphere, https://doi.org/10.5194/egusphere-2024-1182, https://doi.org/10.5194/egusphere-2024-1182, 2024
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Evaluating organosulfur (OS) hygroscopicity is important for assessing the aerosol-cloud climate interactions in the post-fossil fuel future, when SO2 emissions decrease and OS compounds become increasingly important. Here, a state-of-the-art quantum-chemistry-based method was used to predict the hygroscopic growth factors (HGFs) of a group of atmospherically relevant OS compounds and their mixtures with AS. A good agreement was observed between their model-estimated and experimental HGFs.
Xiaoli Wei, Qian Cui, Leiming Ma, Feng Zhang, Wenwen Li, and Peng Liu
Atmos. Chem. Phys., 24, 5025–5045, https://doi.org/10.5194/acp-24-5025-2024, https://doi.org/10.5194/acp-24-5025-2024, 2024
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A new aerosol-type classification algorithm has been proposed. It includes an optical database built by Mie scattering and a complex refractive index working as a baseline to identify different aerosol types. The new algorithm shows high accuracy and efficiency. Hence, a global map of aerosol types was generated to characterize aerosol types across the five continents. It will help improve the accuracy of aerosol inversion and determine the sources of aerosol pollution.
Zhiqiang Zhang, Ying Li, Haiyan Ran, Junling An, Yu Qu, Wei Zhou, Weiqi Xu, Weiwei Hu, Hongbin Xie, Zifa Wang, Yele Sun, and Manabu Shiraiwa
Atmos. Chem. Phys., 24, 4809–4826, https://doi.org/10.5194/acp-24-4809-2024, https://doi.org/10.5194/acp-24-4809-2024, 2024
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Secondary organic aerosols (SOAs) can exist in liquid, semi-solid, or amorphous solid states, which are rarely accounted for in current chemical transport models. We predict the phase state of SOA particles over China and find that in northwestern China SOA particles are mostly highly viscous or glassy solid. Our results indicate that the particle phase state should be considered in SOA formation in chemical transport models for more accurate prediction of SOA mass concentrations.
Alejandro Baró Pérez, Michael S. Diamond, Frida A.-M. Bender, Abhay Devasthale, Matthias Schwarz, Julien Savre, Juha Tonttila, Harri Kokkola, Hyunho Lee, David Painemal, and Annica M. L. Ekman
Atmos. Chem. Phys., 24, 4591–4610, https://doi.org/10.5194/acp-24-4591-2024, https://doi.org/10.5194/acp-24-4591-2024, 2024
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We use a numerical model to study interactions between humid light-absorbing aerosol plumes, clouds, and radiation over the southeast Atlantic. We find that the warming produced by the aerosols reduces cloud cover, especially in highly polluted situations. Aerosol impacts on drizzle play a minor role. However, aerosol effects on cloud reflectivity and moisture-induced changes in cloud cover dominate the climatic response and lead to an overall cooling by the biomass burning plumes.
Sampa Das, Peter R. Colarco, Huisheng Bian, and Santiago Gassó
Atmos. Chem. Phys., 24, 4421–4449, https://doi.org/10.5194/acp-24-4421-2024, https://doi.org/10.5194/acp-24-4421-2024, 2024
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The smoke aerosols emitted from vegetation burning can alter the regional energy budget via multiple pathways. We utilized detailed observations from the NASA ORACLES airborne campaign based in Namibia during September 2016 to improve the representation of smoke aerosol properties and lifetimes in our GEOS Earth system model. The improved model simulations are for the first time able to capture the observed changes in the smoke absorption during long-range plume transport.
Jia Liu, Cancan Zhu, Donghui Zhou, and Jinbao Han
EGUsphere, https://doi.org/10.5194/egusphere-2024-1000, https://doi.org/10.5194/egusphere-2024-1000, 2024
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The hydrophilic coatings of aged black carbon (BC) particles absorb moisture during the hygroscopic growth process, but it is difficult to characterize how much water is absorbed under different relative humidities (RHs). In this study, we propose a method to obtain the water content in the coatings based on the equivalent complex refractive index retrieved from optical properties, and this method is verified from theoretical inspect. This method performs well for thickly coated BC at high RHs.
Falei Xu, Shuang Wang, Yan Li, and Juan Feng
EGUsphere, https://doi.org/10.5194/egusphere-2024-955, https://doi.org/10.5194/egusphere-2024-955, 2024
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This study examines how the North Atlantic Oscillation (NAO) and El Niño-Southern Oscillation (ENSO) in the previous winter affect spring dust activities in North China. The results show that NAO and ENSO, particularly in their negative phases, greatly influence dust activities. When both NAO and ENSO are negative, their combined effect on dust activities is even greater. This research underscores the importance of these climate patterns in predicting spring dust activities in North China.
Emilio Cuevas-Agulló, David Barriopedro, Rosa Delia García, Silvia Alonso-Pérez, Juan Jesús González-Alemán, Ernest Werner, David Suárez, Juan José Bustos, Gerardo García-Castrillo, Omaira García, África Barreto, and Sara Basart
Atmos. Chem. Phys., 24, 4083–4104, https://doi.org/10.5194/acp-24-4083-2024, https://doi.org/10.5194/acp-24-4083-2024, 2024
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During February–March (FM) 2020–2022, unusually intense dust storms from northern Africa hit the western Euro-Mediterranean (WEM). Using dust products from satellites and atmospheric reanalysis for 2003–2022, results show that cut-off lows and European blocking are key drivers of FM dust intrusions over the WEM. A higher frequency of cut-off lows associated with subtropical ridges is observed in the late 2020–2022 period.
Yahui Che, Bofu Yu, and Katherine Bracco
Atmos. Chem. Phys., 24, 4105–4128, https://doi.org/10.5194/acp-24-4105-2024, https://doi.org/10.5194/acp-24-4105-2024, 2024
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Dust events occur more frequently during the Austral spring and summer in dust regions, including central Australia, the southwest of Western Australia, and the northern and southern regions of eastern Australia using remote sensing and reanalysis datasets. High-concentration dust is distributed around central Australia and in the downwind northern and southern Australia. Typically, around 50 % of the dust lifted settles on Australian land, with the remaining half being deposited in the ocean.
Jonathan Elsey, Nicolas Bellouin, and Claire Ryder
Atmos. Chem. Phys., 24, 4065–4081, https://doi.org/10.5194/acp-24-4065-2024, https://doi.org/10.5194/acp-24-4065-2024, 2024
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Aerosols influence the Earth's energy balance. The uncertainty in this radiative forcing is large depending partly on uncertainty in measurements of aerosol optical properties. We have developed a freely available new framework of millions of radiative transfer simulations spanning aerosol uncertainty and assess the impact on radiative forcing uncertainty. We find that reducing these uncertainties would reduce radiative forcing uncertainty, but non-aerosol uncertainties must also be considered.
Jing Li, Nan Wu, Biwu Chu, An Ning, and Xiuhui Zhang
Atmos. Chem. Phys., 24, 3989–4000, https://doi.org/10.5194/acp-24-3989-2024, https://doi.org/10.5194/acp-24-3989-2024, 2024
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Iodic acid (HIO3) nucleates with iodous acid (HIO2) efficiently in marine areas; however, whether methanesulfonic acid (MSA) can synergistically participate in the HIO3–HIO2-based nucleation is unclear. We provide molecular-level evidence that MSA can efficiently promote the formation of HIO3–HIO2-based clusters using a theoretical approach. The proposed MSA-enhanced iodine nucleation mechanism may help us to deeply understand marine new particle formation events with bursts of iodine particles.
Yueming Cheng, Tie Dai, Junji Cao, Daisuke Goto, Jianbing Jin, Teruyuki Nakajima, and Guangyu Shi
EGUsphere, https://doi.org/10.5194/egusphere-2024-840, https://doi.org/10.5194/egusphere-2024-840, 2024
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In March 2021, East Asia experienced an outbreak of severe dust storms after an absence of one and a half decades. Here, we innovative used the time-lagged ground-based aerosol size information with the fixed-lag ensemble Kalman smoother to optimize the dust emission and reproduce the dust storm. This work is valuable for the quantification of health damage, aviation risks, and profound impacts on the Earth system, but also to reveal the climatic driving force and the process of desertification.
Hao Wang, Xiaohong Liu, Chenglai Wu, and Guangxing Lin
Atmos. Chem. Phys., 24, 3309–3328, https://doi.org/10.5194/acp-24-3309-2024, https://doi.org/10.5194/acp-24-3309-2024, 2024
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We quantified different global- and regional-scale drivers of biogenic volatile organic compound (BVOC) emission trends over the past 20 years. The results show that global greening trends significantly boost BVOC emissions and deforestation reduces BVOC emissions in South America and Southeast Asia. Elevated temperature in Europe and increased soil moisture in East and South Asia enhance BVOC emissions. The results deepen our understanding of long-term BVOC emission trends in hotspots.
Christof G. Beer, Johannes Hendricks, and Mattia Righi
Atmos. Chem. Phys., 24, 3217–3240, https://doi.org/10.5194/acp-24-3217-2024, https://doi.org/10.5194/acp-24-3217-2024, 2024
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Ice-nucleating particles (INPs) have important influences on cirrus clouds and the climate system; however, the understanding of their global impacts is still uncertain. We perform numerical simulations with a global aerosol–climate model to analyse INP-induced cirrus changes and the resulting climate impacts. We evaluate various sources of uncertainties, e.g. the ice-nucleating ability of INPs and the role of model dynamics, and provide a new estimate for the global INP–cirrus effect.
Jiawei Li, Zhiwei Han, Pingqing Fu, Xiaohong Yao, and Mingjie Liang
Atmos. Chem. Phys., 24, 3129–3161, https://doi.org/10.5194/acp-24-3129-2024, https://doi.org/10.5194/acp-24-3129-2024, 2024
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Organic aerosols of marine origin are important for aerosol climatic effects but are poorly understood. For the first time, an online coupled regional chemistry–climate model is applied to explore the characteristics of emission, distribution, and direct and indirect radiative effects of marine organic aerosols over the western Pacific, which reveals an important role of marine organic aerosols in perturbing cloud and radiation and promotes understanding of global aerosol climatic impact.
Yawen Liu, Yun Qian, Philip J. Rasch, Kai Zhang, Lai-yung Ruby Leung, Yuhang Wang, Minghuai Wang, Hailong Wang, Xin Huang, and Xiu-Qun Yang
Atmos. Chem. Phys., 24, 3115–3128, https://doi.org/10.5194/acp-24-3115-2024, https://doi.org/10.5194/acp-24-3115-2024, 2024
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Fire management has long been a challenge. Here we report that spring-peak fire activity over southern Mexico and Central America (SMCA) has a distinct quasi-biennial signal by measuring multiple fire metrics. This signal is initially driven by quasi-biennial variability in precipitation and is further amplified by positive feedback of fire–precipitation interaction at short timescales. This work highlights the importance of fire–climate interactions in shaping fires on an interannual scale.
Xu Feng, Loretta J. Mickley, Michelle L. Bell, Tianjia Liu, Jenny A. Fisher, and Maria Val Martin
Atmos. Chem. Phys., 24, 2985–3007, https://doi.org/10.5194/acp-24-2985-2024, https://doi.org/10.5194/acp-24-2985-2024, 2024
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During severe wildfire seasons, smoke can have a significant impact on air quality in Australia. Our study demonstrates that characterization of the smoke plume injection fractions greatly affects estimates of surface smoke PM2.5. Using the plume behavior predicted by the machine learning method leads to the best model agreement with observed surface PM2.5 in key cities across Australia, with smoke PM2.5 accounting for 5 %–52 % of total PM2.5 on average during fire seasons from 2009 to 2020.
Shiyi Lai, Ximeng Qi, Xin Huang, Sijia Lou, Xuguang Chi, Liangduo Chen, Chong Liu, Yuliang Liu, Chao Yan, Mengmeng Li, Tengyu Liu, Wei Nie, Veli-Matti Kerminen, Tuukka Petäjä, Markku Kulmala, and Aijun Ding
Atmos. Chem. Phys., 24, 2535–2553, https://doi.org/10.5194/acp-24-2535-2024, https://doi.org/10.5194/acp-24-2535-2024, 2024
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By combining in situ measurements and chemical transport modeling, this study investigates new particle formation (NPF) on the southeastern Tibetan Plateau. We found that the NPF was driven by the presence of biogenic gases and the transport of anthropogenic precursors. The NPF was vertically heterogeneous and shaped by the vertical mixing. This study highlights the importance of anthropogenic–biogenic interactions and meteorological dynamics in NPF in this climate-sensitive region.
Adriana Rocha-Lima, Peter R. Colarco, Anton S. Darmenov, Edward P. Nowottnick, Arlindo M. da Silva, and Luke D. Oman
Atmos. Chem. Phys., 24, 2443–2464, https://doi.org/10.5194/acp-24-2443-2024, https://doi.org/10.5194/acp-24-2443-2024, 2024
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Observations show an increasing aerosol optical depth trend in the Middle East between 2003–2012. We evaluate the NASA Goddard Earth Observing System (GEOS) model's ability to capture these trends and examine the meteorological and surface parameters driving dust emissions. Our results highlight the importance of data assimilation for long-term trends of atmospheric aerosols and support the hypothesis that vegetation cover loss may have contributed to increasing dust emissions in the period.
Marc Mallet, Aurore Voldoire, Fabien Solmon, Pierre Nabat, Thomas Drugé, and Romain Roehrig
EGUsphere, https://doi.org/10.5194/egusphere-2024-496, https://doi.org/10.5194/egusphere-2024-496, 2024
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This study investigates the interactions between smoke aerosols and climate in tropical Africa using a coupled ocean-atmosphere-aerosol climate model. The work shows that smoke plumes have a significant impact by increasing the low cloud fraction, decreasing the ocean and continental surface temperature and by reducing the precipitation of the coastal Western Africa. It also highlights the key role of the ocean temperature response and its feedbacks for the September to November season.
Danny M. Leung, Jasper F. Kok, Longlei Li, Natalie M. Mahowald, David M. Lawrence, Simone Tilmes, Erik Kluzek, Martina Klose, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 2287–2318, https://doi.org/10.5194/acp-24-2287-2024, https://doi.org/10.5194/acp-24-2287-2024, 2024
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This study uses a premier Earth system model to evaluate a new desert dust emission scheme proposed in our companion paper. We show that our scheme accounts for more dust emission physics, hence matching better against observations than other existing dust emission schemes do. Our scheme's dust emissions also couple tightly with meteorology, hence likely improving the modeled dust sensitivity to climate change. We believe this work is vital for improving dust representation in climate models.
Ruth A. R. Digby, Nathan P. Gillett, Adam H. Monahan, Knut von Salzen, Antonis Gkikas, Qianqian Song, and Zhibo Zhang
Atmos. Chem. Phys., 24, 2077–2097, https://doi.org/10.5194/acp-24-2077-2024, https://doi.org/10.5194/acp-24-2077-2024, 2024
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The COVID-19 lockdowns reduced aerosol emissions. We ask whether these reductions affected regional aerosol optical depth (AOD) and compare the observed changes to predictions from Earth system models. Only India has an observed AOD reduction outside of typical variability. Models overestimate the response in some regions, but when key biases have been addressed, the agreement is improved. Our results suggest that current models can realistically predict the effects of future emission changes.
Xinyue Shao, Minghuai Wang, Xinyi Dong, Yaman Liu, Wenxiang Shen, Stephen Arnold, Leighton Regayre, Meinrat Andreae, Mira Pöhlker, Duseong Jo, Man Yue, and Ken Carslaw
EGUsphere, https://doi.org/10.5194/egusphere-2024-401, https://doi.org/10.5194/egusphere-2024-401, 2024
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Highly oxygenated organic molecules (HOMs) play an important role in atmospheric new particle formation (NPF). By explicitly coupling the chemical mechanism of HOMs and a comprehensive nucleation scheme in a global climate model. The updated model shows better agreement with measurements of nucleation rate, growth rate, NPF event frequency. Our results reveal that HOMs-driven NPF leads to a considerable increase in particle and cloud condensation nuclei burden globally.
Giorgio Veratti, Alessandro Bigi, Michele Stortini, Sergio Teggi, and Grazia Ghermandi
EGUsphere, https://doi.org/10.5194/egusphere-2023-2641, https://doi.org/10.5194/egusphere-2023-2641, 2024
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In a study of two consecutive winter seasons, we used measurements and modeling tools to identify the levels and sources of black carbon pollution in a medium-sized urban area of the Po valley, Italy. Our findings show that biomass burning and traffic-related emissions (especially from Euro 4 diesel cars), significantly contribute to BC concentrations. This research offers crucial insights for policymakers and urban planners aiming to improve air quality in cities.
Huisheng Bian, Mian Chin, Peter R. Colarco, Eric C. Apel, Donald R. Blake, Karl Froyd, Rebecca S. Hornbrook, Jose Jimenez, Pedro Campuzano Jost, Michael Lawler, Mingxu Liu, Marianne Tronstad Lund, Hitoshi Matsui, Benjamin A. Nault, Joyce E. Penner, Andrew W. Rollins, Gregory Schill, Ragnhild B. Skeie, Hailong Wang, Lu Xu, Kai Zhang, and Jialei Zhu
Atmos. Chem. Phys., 24, 1717–1741, https://doi.org/10.5194/acp-24-1717-2024, https://doi.org/10.5194/acp-24-1717-2024, 2024
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This work studies sulfur in the remote troposphere at global and seasonal scales using aircraft measurements and multi-model simulations. The goal is to understand the sulfur cycle over remote oceans, spread of model simulations, and observation–model discrepancies. Such an understanding and comparison with real observations are crucial to narrow down the uncertainties in model sulfur simulations and improve understanding of the sulfur cycle in atmospheric air quality, climate, and ecosystems.
Gargi Sengupta, Minjie Zheng, and Nønne L. Prisle
Atmos. Chem. Phys., 24, 1467–1487, https://doi.org/10.5194/acp-24-1467-2024, https://doi.org/10.5194/acp-24-1467-2024, 2024
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The effect of organic acid aerosol on sulfur chemistry and cloud properties was investigated in an atmospheric model. Organic acid dissociation was considered using both bulk and surface-related properties. We found that organic acid dissociation leads to increased hydrogen ion concentrations and sulfate aerosol mass in aqueous aerosols, increasing cloud formation. This could be important in large-scale climate models as many organic aerosol components are both acidic and surface-active.
Leena Kangas, Jaakko Kukkonen, Mari Kauhaniemi, Kari Riikonen, Mikhail Sofiev, Anu Kousa, Jarkko V. Niemi, and Ari Karppinen
Atmos. Chem. Phys., 24, 1489–1507, https://doi.org/10.5194/acp-24-1489-2024, https://doi.org/10.5194/acp-24-1489-2024, 2024
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Residential wood combustion is a major source of fine particulate matter. This study has evaluated the contribution of residential wood combustion to fine particle concentrations and its year-to-year and seasonal variation in te Helsinki metropolitan area. The average concentrations attributed to wood combustion in winter were up to 10- or 15-fold compared to summer. Wood combustion caused 12 % to 14 % of annual fine particle concentrations. In winter, the contribution ranged from 16 % to 21 %.
Arto Heitto, Cheng Wu, Diego Aliaga, Luis Blacutt, Xuemeng Chen, Yvette Gramlich, Liine Heikkinen, Wei Huang, Radovan Krejci, Paolo Laj, Isabel Moreno, Karine Sellegri, Fernando Velarde, Kay Weinhold, Alfred Wiedensohler, Qiaozhi Zha, Federico Bianchi, Marcos Andrade, Kari E. J. Lehtinen, Claudia Mohr, and Taina Yli-Juuti
Atmos. Chem. Phys., 24, 1315–1328, https://doi.org/10.5194/acp-24-1315-2024, https://doi.org/10.5194/acp-24-1315-2024, 2024
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Particle growth at the Chacaltaya station in Bolivia was simulated based on measured vapor concentrations and ambient conditions. Major contributors to the simulated growth were low-volatility organic compounds (LVOCs). Also, sulfuric acid had major role when volcanic activity was occurring in the area. This study provides insight on nanoparticle growth at this high-altitude Southern Hemispheric site and hence contributes to building knowledge of early growth of atmospheric particles.
Steven Soon-Kai Kong, Saginela Ravindra Babu, Sheng-Hsiang Wang, Stephen M. Griffith, Jackson Hian-Wui Chang, Ming-Tung Chuang, Guey-Rong Sheu, and Neng-Huei Lin
Atmos. Chem. Phys., 24, 1041–1058, https://doi.org/10.5194/acp-24-1041-2024, https://doi.org/10.5194/acp-24-1041-2024, 2024
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In this study, we combined ground observations from 7-SEAS Dongsha Experiment, MERRA-2 reanalysis, and MODIS satellite images for evaluation and improvement of the CMAQ dust model for cases of East Asian Dust reaching the Taiwan region, including Dongsha in the western Pacific. We proposed a better CMAQ dust treatment over East Asia and for the first time revealed the impact of typhoons on dust transport.
Hengheng Zhang, Wei Huang, Xiaoli Shen, Ramakrishna Ramisetty, Junwei Song, Olga Kiseleva, Christopher Claus Holst, Basit Khan, Thomas Leisner, and Harald Saathoff
EGUsphere, https://doi.org/10.5194/egusphere-2024-90, https://doi.org/10.5194/egusphere-2024-90, 2024
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Our study unravels how stagnant winter conditions elevate aerosol levels in Stuttgart. Cloud cover at night plays a pivotal role, impacting morning air quality. Validating a key model, our findings aid accurate air quality predictions, crucial for effective pollution mitigation in urban areas.
Zhiguo Zhang, Christer Johansson, Magnuz Engardt, Massimo Stafoggia, and Xiaoliang Ma
Atmos. Chem. Phys., 24, 807–851, https://doi.org/10.5194/acp-24-807-2024, https://doi.org/10.5194/acp-24-807-2024, 2024
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Up-to-date information on present and near-future air quality help people avoid exposure to high levels of air pollution. We apply different machine learning models to significantly improve traditional forecasts of PM10, NOx, and O3 in Stockholm, Sweden. It is shown that forecasts of all air pollutants are improved by the input of lagged measurements and taking calendar information into account. The final modelled errors are substantially smaller than uncertainties in the measurements.
Cited articles
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Abdul-Razzak, H. and Ghan, S.: Parameterization of the influence of organic surfactants on aerosol activation, J. Geophys. Res., 109, D03205, https://doi.org/10.1029/2003JD004043, 2004.
Almeida, G. P., Brito, J., Morales, C. A., Andrade, M. F., and Artaxo, P.: Measured and modelled cloud condensation nuclei (CCN) concentration in São Paulo, Brazil: the importance of aerosol size-resolved chemical composition on CCN concentration prediction, Atmos. Chem. Phys., 14, 7559–7572, https://doi.org/10.5194/acp-14-7559-2014, 2014.
Ansmann, A., Bosenberg, J., Chaikovsky, A., Comeron, A., Eckhardt, S., Eixmann, R., Freudenthaler, V., Ginoux, P., Komguem, L., Linne, H., Marquez, M., Matthias, V., Mattis, I., Mittev, V., Muller, D., Music, S., Nickovic, S., Pelon, J., Sauvage, L., Sobolewsky, P., Srivastava, M., Sthol, A., Toress, O., Vaughan, G., Wandinger, U., and Wiegner, M.: Long-range transport to saharan dust to northern europe: The 11–16 october 2001 outbreak observed with earlinet, J. Geophys. Res., 108, D124345, https://doi.org/10.1029/2003JD003757, 2003.
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Aouizerats, B., Thouron, O., Tulet, P., Mallet, M., Gomes, L., and Henzing, J. S.: Development of an online radiative module for the computation of aerosol optical properties in 3-D atmospheric models: validation during the EUCAARI campaign, Geosci. Model Dev., 3, 553–564, https://doi.org/10.5194/gmd-3-553-2010, 2010.
Aouizerats, B., Tulet, P., Pigeon, G., Masson, V., and Gomes, L.: High resolution modelling of aerosol dispersion regimes during the CAPITOUL field experiment: from regional to local scale interactions, Atmos. Chem. Phys., 11, 7547–7560, https://doi.org/10.5194/acp-11-7547-2011, 2011.
Aouizerats, B., Tulet, P., and Gomes, L.: 3-D direct impacts of urban aerosols on dynamics during the capitoul field experiment, Geophys. Res. Lett., 39, L23807, https://doi.org/10.1029/2012GL053781, 2012.
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Bangert, M., Nenes, A., Vogel, B., Vogel, H., Barahona, D., Karydis, V. A., Kumar, P., Kottmeier, C., and Blahak, U.: Saharan dust event impacts on cloud formation and radiation over Western Europe, Atmos. Chem. Phys., 12, 4045–4063, https://doi.org/10.5194/acp-12-4045-2012, 2012.
Baray, J.-L., Duflot, V,. Posny, F., Cammas, J.-P., Thompson, A., Gabarrot, F., Bonne, J.-L., and Zeng, G.: One year ozonesonde measurements at kerguelen island (49.2° S, 70.1° E): Influence of stratosphere-to-troposphere exchange and long-range transport of biomass burning plumes, J. Geophys. Res., 117, D06305, https://doi.org/10.1029/2011JD016717, 2012.
Barthe, C., Molinié, G., and Pinty, J.: Description and first results of an explicit electrical scheme in a 3d cloud resolving model, Atmos. Res., 76, 95–113, 2005.
Bauer, S., Balkanski, Y., Schulz, M., Hauglustaine, D., and Dententer, F.: Global modeling of heterogeneous chemistry on mineral aerosol surface: 1. the influence on tropospheric ozone chemistry and comparison to observations, J. Geophys. Res., 109, D02304, https://doi.org/10.1029/2003JD003868, 2004.
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