Articles | Volume 24, issue 1
https://doi.org/10.5194/acp-24-235-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-24-235-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
10 Jan 2024
Research article |
| 10 Jan 2024
| 10 Jan 2024
Assessing the assimilation of Himawari-8 observations on aerosol forecasts and radiative effects during pollution transport from South Asia to the Tibetan Plateau
Min Zhao
State Key Laboratory of Tibetan Plateau Earth System, Environment and Resources (TPESER), Institute of Tibetan Plateau Research, Chinese Academy of Sciences, Beijing, China
State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, China
Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters/ Key Laboratory of Meteorological Disaster of Ministry of Education, Nanjing University of Information Science and Technology, Nanjing, China
Daisuke Goto
National Institute for Environmental Studies, Tsukuba, Japan
International Center for Climate and Environment Science, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, China
Guangyu Shi
State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, China
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Chihiro Kodama, Tomoki Ohno, Tatsuya Seiki, Hisashi Yashiro, Akira T. Noda, Masuo Nakano, Yohei Yamada, Woosub Roh, Masaki Satoh, Tomoko Nitta, Daisuke Goto, Hiroaki Miura, Tomoe Nasuno, Tomoki Miyakawa, Ying-Wen Chen, and Masato Sugi
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Atmos. Chem. Phys., 20, 15307–15322, https://doi.org/10.5194/acp-20-15307-2020, https://doi.org/10.5194/acp-20-15307-2020, 2020
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Atmos. Chem. Phys., 20, 3589–3607, https://doi.org/10.5194/acp-20-3589-2020, https://doi.org/10.5194/acp-20-3589-2020, 2020
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APHH-Beijing is a collaborative international research programme to study the sources, processes and health effects of air pollution in Beijing. This introduction to the special issue provides an overview of (i) the APHH-Beijing programme, (ii) the measurement and modelling activities performed as part of it and (iii) the air quality and meteorological conditions during joint intensive field campaigns as a core activity within APHH-Beijing.
Huizheng Che, Bing Qi, Hujia Zhao, Xiangao Xia, Thomas F. Eck, Philippe Goloub, Oleg Dubovik, Victor Estelles, Emilio Cuevas-Agulló, Luc Blarel, Yunfei Wu, Jun Zhu, Rongguang Du, Yaqiang Wang, Hong Wang, Ke Gui, Jie Yu, Yu Zheng, Tianze Sun, Quanliang Chen, Guangyu Shi, and Xiaoye Zhang
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Sun photometer measurements from seven sites in the Yangtze River Delta (YRD) from 2011 to 2015 were used to characterize the climatology of aerosol microphysical and optical properties, calculate direct aerosol radiative forcing (DARF) and classify aerosols based on size and absorption. This study contributes to our understanding of aerosols and regional climate/air quality, and the results will be useful for validating satellite retrievals and for improving climate models and remote sensing.
Nick Schutgens, Svetlana Tsyro, Edward Gryspeerdt, Daisuke Goto, Natalie Weigum, Michael Schulz, and Philip Stier
Atmos. Chem. Phys., 17, 9761–9780, https://doi.org/10.5194/acp-17-9761-2017, https://doi.org/10.5194/acp-17-9761-2017, 2017
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We estimate representativeness errors in observations due to mismatching spatio-temporal sampling, on timescales of hours to a year and length scales of 50 to 200 km, for a variety of observing systems (in situ or remote sensing ground sites, satellites with imagers or lidar, etc.) and develop strategies to reduce them. This study is relevant to the use of observations in constructing satellite L3 products, observational intercomparison and model evaluation.
Nick A. J. Schutgens, Edward Gryspeerdt, Natalie Weigum, Svetlana Tsyro, Daisuke Goto, Michael Schulz, and Philip Stier
Atmos. Chem. Phys., 16, 6335–6353, https://doi.org/10.5194/acp-16-6335-2016, https://doi.org/10.5194/acp-16-6335-2016, 2016
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We show that evaluating global aerosol model data with observations of very different spatial scales (200 vs. 10 km) can lead to large discrepancies, solely due to different spatial sampling. Strategies for reducing these sampling errors are developed and tested using a set of high-resolution model simulations.
Josiane Mélançon, Maurice Levasseur, Martine Lizotte, Michael Scarratt, Jean-Éric Tremblay, Philippe Tortell, Gui-Peng Yang, Guang-Yu Shi, Huiwang Gao, David Semeniuk, Marie Robert, Michael Arychuk, Keith Johnson, Nes Sutherland, Marty Davelaar, Nina Nemcek, Angelica Peña, and Wendy Richardson
Biogeosciences, 13, 1677–1692, https://doi.org/10.5194/bg-13-1677-2016, https://doi.org/10.5194/bg-13-1677-2016, 2016
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Ocean acidification is likely to affect iron-limited phytoplankton fertilization by desert dust. Short incubations of northeast subarctic Pacific waters enriched with dust and set at pH 8.0 and 7.8 were conducted. Acidification led to a significant reduction (by 16–38 %) of the final concentration of chl a reached after enrichment. These results show that dust deposition events in a low-pH iron-limited ocean are likely to stimulate phytoplankton growth to a lesser extent than in today's ocean.
Z. Wang, D. Liu, Y. Wang, Z. Wang, and G. Shi
Atmos. Meas. Tech., 8, 2901–2907, https://doi.org/10.5194/amt-8-2901-2015, https://doi.org/10.5194/amt-8-2901-2015, 2015
H. Che, X.-Y. Zhang, X. Xia, P. Goloub, B. Holben, H. Zhao, Y. Wang, X.-C. Zhang, H. Wang, L. Blarel, B. Damiri, R. Zhang, X. Deng, Y. Ma, T. Wang, F. Geng, B. Qi, J. Zhu, J. Yu, Q. Chen, and G. Shi
Atmos. Chem. Phys., 15, 7619–7652, https://doi.org/10.5194/acp-15-7619-2015, https://doi.org/10.5194/acp-15-7619-2015, 2015
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This work studied more than 10 years of measurements of aerosol optical depths (AODs) made for 50 sites of CARSNET compiled into a climatology of aerosol optical properties for China. It lets us see a detailed full-scale description of AOD observations over China. The results would benefit us a lot in comprehending the temporal and special distribution aerosol optical property over China. Also the data would be valuable to communities of aerosol satellite retrieval, modelling, etc.
H. Wang, G. Y. Shi, X. Y. Zhang, S. L. Gong, S. C. Tan, B. Chen, H. Z. Che, and T. Li
Atmos. Chem. Phys., 15, 3277–3287, https://doi.org/10.5194/acp-15-3277-2015, https://doi.org/10.5194/acp-15-3277-2015, 2015
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Solar radiation reaching the ground decreases about 15% in Chinese 3JNS region and by 20 to 25% in the region with the highest AOD. Aerosol cools the PBL atmosphere but warms the atmosphere above it, leading to a more stable atmosphere that causes a decrease in turbulence diffusion of about 52% and in PBL height of about 33%; this results in a positive feedback on the PM2.5 concentration within the PBL and the surface as well as the haze formation.
D. Goto, T. Dai, M. Satoh, H. Tomita, J. Uchida, S. Misawa, T. Inoue, H. Tsuruta, K. Ueda, C. F. S. Ng, A. Takami, N. Sugimoto, A. Shimizu, T. Ohara, and T. Nakajima
Geosci. Model Dev., 8, 235–259, https://doi.org/10.5194/gmd-8-235-2015, https://doi.org/10.5194/gmd-8-235-2015, 2015
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An aerosol-coupled global non-hydrostatic model with a stretched-grid system has been developed to simulate aerosols on a region scale of 10 km grids. The regional simulation does require either a nesting technique or lateral boundary conditions, as opposed to general regional models. It generally reproduces monthly mean distributions of the observed sulfate and SO2 over East Asia as well as the diurnal and synoptic variations of the observed ones around the main target region, Tokyo/Japan.
H. Che, X. Xia, J. Zhu, Z. Li, O. Dubovik, B. Holben, P. Goloub, H. Chen, V. Estelles, E. Cuevas-Agulló, L. Blarel, H. Wang, H. Zhao, X. Zhang, Y. Wang, J. Sun, R. Tao, X. Zhang, and G. Shi
Atmos. Chem. Phys., 14, 2125–2138, https://doi.org/10.5194/acp-14-2125-2014, https://doi.org/10.5194/acp-14-2125-2014, 2014
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
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Measurement report: Source attribution and estimation of black carbon levels in an urban hotspot of the central Po Valley – an integrated approach combining high-resolution dispersion modelling and micro-aethalometers
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In-plume and out-of-plume analysis of aerosol–cloud interactions derived from the 2014–2015 Holuhraun volcanic eruption
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The role of interfacial tension in the size-dependent phase separation of atmospheric aerosol particles
Modeling impacts of dust mineralogy on fast climate response
Representation of iron aerosol size distributions is critical in evaluating atmospheric soluble iron input to the ocean
Uncertainties in laboratory-measured shortwave refractive indices of mineral dust aerosols and derived optical properties: a theoretical assessment
Diagnosing uncertainties in global biomass burning emission inventories and their impact on modeled air pollutants
Solar radiation estimation in West Africa: impact of dust conditions during 2021 dry season
Role of atmospheric aerosols in severe winter fog over the Indo-Gangetic Plain of India: a case study
Long-term variability in black carbon emissions constrained by gap-filled absorption aerosol optical depth and associated premature mortality in China
Intercomparison of aerosol optical depths from four reanalyses and their multi-reanalysis consensus
Global aviation contrail climate effects from 2019 to 2021
Multi-model effective radiative forcing of the 2020 sulphur cap for shipping
Rapid iodine oxoacid nucleation enhanced by dimethylamine in broad marine regions
Simulations of the impact of cloud condensation nuclei and ice-nucleating particles perturbations on the microphysics and radar reflectivity factor of stratiform mixed-phase clouds
Warming effects of reduced sulfur emissions from shipping
Aerosols in the central Arctic cryosphere: satellite and model integrated insights during Arctic spring and summer
Observationally constrained regional variations of shortwave absorption by iron oxides emphasize the cooling effect of dust
Droplet collection efficiencies inferred from satellite retrievals constrain effective radiative forcing of aerosol–cloud interactions
Global aerosol-type classification using a new hybrid algorithm and Aerosol Robotic Network data
Simulated phase state and viscosity of secondary organic aerosols over China
Comparing the simulated influence of biomass burning plumes on low-level clouds over the southeastern Atlantic under varying smoke conditions
A global dust emission dataset for estimating dust radiative forcings in climate models
Improved simulations of biomass burning aerosol optical properties and lifetimes in the NASA GEOS Model during the ORACLES-I campaign
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Sharp increase in Saharan dust intrusions over the western Euro-Mediterranean in February–March 2020–2022 and associated atmospheric circulation
Temporal and spatial variations in dust activity in Australia based on remote sensing and reanalysis datasets
Sensitivity of global direct aerosol shortwave radiative forcing to uncertainties in aerosol optical properties
Molecular-level study on the role of methanesulfonic acid in iodine oxoacid nucleation
Regional to global distributions, trends, and drivers of biogenic volatile organic compound emission from 2001 to 2020
Impacts of ice-nucleating particles on cirrus clouds and radiation derived from global model simulations with MADE3 in EMAC
Seasonal characteristics of emission, distribution, and radiative effect of marine organic aerosols over the western Pacific Ocean: an investigation with a coupled regional climate aerosol model
Fire–precipitation interactions amplify the quasi-biennial variability in fires over southern Mexico and Central America
Improved estimates of smoke exposure during Australia fire seasons: importance of quantifying plume injection heights
New particle formation induced by anthropogenic–biogenic interactions on the southeastern Tibetan Plateau
Investigation of observed dust trends over the Middle East region in NASA Goddard Earth Observing System (GEOS) model simulations
Yueming Cheng, Tie Dai, Junji Cao, Daisuke Goto, Jianbing Jin, Teruyuki Nakajima, and Guangyu Shi
Atmos. Chem. Phys., 24, 12643–12659, https://doi.org/10.5194/acp-24-12643-2024, https://doi.org/10.5194/acp-24-12643-2024, 2024
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Marc Mallet, Aurore Voldoire, Fabien Solmon, Pierre Nabat, Thomas Drugé, and Romain Roehrig
Atmos. Chem. Phys., 24, 12509–12535, https://doi.org/10.5194/acp-24-12509-2024, https://doi.org/10.5194/acp-24-12509-2024, 2024
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This study investigates the interactions between smoke aerosols and climate in tropical Africa using a coupled ocean–atmosphere–aerosol climate model. The work shows that smoke plumes have a significant impact by increasing the low-cloud fraction, decreasing the ocean and continental surface temperature and reducing the precipitation of coastal western Africa. It also highlights the role of the ocean temperature response and its feedbacks for the September–November season.
Jia Liu, Cancan Zhu, Donghui Zhou, and Jinbao Han
Atmos. Chem. Phys., 24, 12341–12354, https://doi.org/10.5194/acp-24-12341-2024, https://doi.org/10.5194/acp-24-12341-2024, 2024
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The hydrophilic coatings of aged black carbon (BC) particles absorb moisture during the hygroscopic growth process, but it is difficult to characterize how much water is absorbed under different relative humidities (RHs). In this study, we propose a method to obtain the water content in the coatings based on the equivalent complex refractive index retrieved from optical properties. This method is verified from a theoretical perspective, and it performs well for thickly coated BC at high RHs.
Zijun Li, Angela Buchholz, and Noora Hyttinen
Atmos. Chem. Phys., 24, 11717–11725, https://doi.org/10.5194/acp-24-11717-2024, https://doi.org/10.5194/acp-24-11717-2024, 2024
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Evaluating organosulfur (OS) hygroscopicity is important for assessing aerosol–cloud climate interactions in the post-fossil-fuel future, when SO2 emissions decrease and OS compounds become increasingly important. Here a state-of-the-art quantum-chemistry-based method was used to predict the hygroscopic growth factors (HGFs) of a group of atmospherically relevant OS compounds and their mixtures with (NH4)2SO4. A good agreement was observed between their model-estimated and experimental HGFs.
Jamie R. Banks, Bernd Heinold, and Kerstin Schepanski
Atmos. Chem. Phys., 24, 11451–11475, https://doi.org/10.5194/acp-24-11451-2024, https://doi.org/10.5194/acp-24-11451-2024, 2024
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The Aralkum is a new desert in Central Asia formed by the desiccation of the Aral Sea. This has created a source of atmospheric dust, with implications for the balance of solar and thermal radiation. Simulating these effects using a dust transport model, we find that Aralkum dust adds radiative cooling effects to the surface and atmosphere on average but also adds heating events. Increases in surface pressure due to Aralkum dust strengthen the Siberian High and weaken the summer Asian heat low.
Xinyue Shao, Minghuai Wang, Xinyi Dong, Yaman Liu, Wenxiang Shen, Stephen R. Arnold, Leighton A. Regayre, Meinrat O. Andreae, Mira L. Pöhlker, Duseong S. Jo, Man Yue, and Ken S. Carslaw
Atmos. Chem. Phys., 24, 11365–11389, https://doi.org/10.5194/acp-24-11365-2024, https://doi.org/10.5194/acp-24-11365-2024, 2024
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Falei Xu, Shuang Wang, Yan Li, and Juan Feng
Atmos. Chem. Phys., 24, 10689–10705, https://doi.org/10.5194/acp-24-10689-2024, https://doi.org/10.5194/acp-24-10689-2024, 2024
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This study examines how the winter North Atlantic Oscillation (NAO) and El Niño–Southern Oscillation (ENSO) affect dust activities in North China during the following spring. The results show that the NAO and ENSO, particularly in their negative phases, greatly influence dust activities. When both are negative, their combined effect on dust activities is even greater. This research highlights the importance of these climate patterns in predicting spring dust activities in North China.
Hengheng Zhang, Wei Huang, Xiaoli Shen, Ramakrishna Ramisetty, Junwei Song, Olga Kiseleva, Christopher Claus Holst, Basit Khan, Thomas Leisner, and Harald Saathoff
Atmos. Chem. Phys., 24, 10617–10637, https://doi.org/10.5194/acp-24-10617-2024, https://doi.org/10.5194/acp-24-10617-2024, 2024
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Our study unravels how stagnant winter conditions elevate aerosol levels in Stuttgart. Cloud cover at night plays a pivotal role, impacting morning air quality. Validating a key model, our findings aid accurate air quality predictions, crucial for effective pollution mitigation in urban areas.
Giorgio Veratti, Alessandro Bigi, Michele Stortini, Sergio Teggi, and Grazia Ghermandi
Atmos. Chem. Phys., 24, 10475–10512, https://doi.org/10.5194/acp-24-10475-2024, https://doi.org/10.5194/acp-24-10475-2024, 2024
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In a study of two consecutive winter seasons, we used measurements and modelling tools to identify the levels and sources of black carbon pollution in a medium-sized urban area of the Po Valley, Italy. Our findings show that biomass burning and traffic-related emissions (especially from Euro 4 diesel cars) significantly contribute to BC concentrations. This research offers crucial insights for policymakers and urban planners aiming to improve air quality in cities.
Pascal Lemaitre, Arnaud Quérel, Alexis Dépée, Alice Guerra Devigne, Marie Monier, Thibault Hiron, Chloé Soto Minguez, Daniel Hardy, and Andrea Flossmann
Atmos. Chem. Phys., 24, 9713–9732, https://doi.org/10.5194/acp-24-9713-2024, https://doi.org/10.5194/acp-24-9713-2024, 2024
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A new in-cloud scavenging scheme is proposed. It is based on a microphysical model of cloud formation and may be applied to long-distance atmospheric transport models (> 100 km) and climatic models. This model is applied to the two most extreme precipitating cloud types in terms of both relative humidity and vertical extension: cumulonimbus and stratus.
Alex Rowell, James Brean, David C. S. Beddows, Tuukka Petäjä, Máté Vörösmarty, Imre Salma, Jarkko V. Niemi, Hanna E. Manninen, Dominik van Pinxteren, Thomas Tuch, Kay Weinhold, Zongbo Shi, and Roy M. Harrison
Atmos. Chem. Phys., 24, 9515–9531, https://doi.org/10.5194/acp-24-9515-2024, https://doi.org/10.5194/acp-24-9515-2024, 2024
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Different sources of airborne particles in the atmospheres of four European cities were distinguished by recognising their particle size distributions using a statistical procedure, positive matrix factorisation. The various sources responded differently to the changes in emissions associated with COVID-19 lockdowns, and the reasons are investigated. While traffic emissions generally decreased, particles formed from reactions of atmospheric gases decreased in some cities but increased in others.
Amy H. Peace, Ying Chen, George Jordan, Daniel G. Partridge, Florent Malavelle, Eliza Duncan, and Jim M. Haywood
Atmos. Chem. Phys., 24, 9533–9553, https://doi.org/10.5194/acp-24-9533-2024, https://doi.org/10.5194/acp-24-9533-2024, 2024
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Natural aerosols from volcanic eruptions can help us understand how anthropogenic aerosols modify climate. We use observations and model simulations of the 2014–2015 Holuhraun eruption plume to examine aerosol–cloud interactions in September 2014. We find a shift to clouds with smaller, more numerous cloud droplets in the first 2 weeks of the eruption. In the third week, the background meteorology and previous conditions experienced by air masses modulate the aerosol perturbation to clouds.
Hua Lu, Min Xie, Bingliang Zhuang, Danyang Ma, Bojun Liu, Yangzhihao Zhan, Tijian Wang, Shu Li, Mengmeng Li, and Kuanguang Zhu
Atmos. Chem. Phys., 24, 8963–8982, https://doi.org/10.5194/acp-24-8963-2024, https://doi.org/10.5194/acp-24-8963-2024, 2024
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To identify cloud, aerosol, and planetary boundary layer (PBL) interactions from an air quality perspective, we summarized two pollution patterns characterized by denser liquid cloud and by obvious cloud radiation interaction (CRI). Numerical simulation experiments showed CRI could cause a 50 % reduction in aerosol radiation interaction (ARI) under a low-trough system. The results emphasized the nonnegligible role of CRI and its inhibition of ARI under wet and cloudy pollution synoptic patterns.
Emilie Fons, Ann Kristin Naumann, David Neubauer, Theresa Lang, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 8653–8675, https://doi.org/10.5194/acp-24-8653-2024, https://doi.org/10.5194/acp-24-8653-2024, 2024
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Aerosols can modify the liquid water path (LWP) of stratocumulus and, thus, their radiative effect. We compare storm-resolving model and satellite data that disagree on the sign of LWP adjustments and diagnose this discrepancy with causal inference. We find that strong precipitation, the absence of wet scavenging, and cloud deepening under a weak inversion contribute to positive LWP adjustments to aerosols in the model, despite weak negative effects from cloud-top entrainment enhancement.
Muhammed Irfan, Thomas Kühn, Taina Yli-Juuti, Anton Laakso, Eemeli Holopainen, Douglas R. Worsnop, Annele Virtanen, and Harri Kokkola
Atmos. Chem. Phys., 24, 8489–8506, https://doi.org/10.5194/acp-24-8489-2024, https://doi.org/10.5194/acp-24-8489-2024, 2024
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The study examines how the volatility of semi-volatile organic compounds affects secondary organic aerosol (SOA) formation and climate. Our simulations show that uncertainties in these volatilities influence aerosol mass and climate impacts. Accurate representation of these compounds in climate models is crucial for predicting global climate patterns.
Alkiviadis Kalisoras, Aristeidis K. Georgoulias, Dimitris Akritidis, Robert J. Allen, Vaishali Naik, Chaincy Kuo, Sophie Szopa, Pierre Nabat, Dirk Olivié, Twan van Noije, Philippe Le Sager, David Neubauer, Naga Oshima, Jane Mulcahy, Larry W. Horowitz, and Prodromos Zanis
Atmos. Chem. Phys., 24, 7837–7872, https://doi.org/10.5194/acp-24-7837-2024, https://doi.org/10.5194/acp-24-7837-2024, 2024
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Effective radiative forcing (ERF) is a metric for estimating how human activities and natural agents change the energy flow into and out of the Earth’s climate system. We investigate the anthropogenic aerosol ERF, and we estimate the contribution of individual processes to the total ERF using simulations from Earth system models within the Coupled Model Intercomparison Project Phase 6 (CMIP6). Our findings highlight that aerosol–cloud interactions drive ERF variability during the last 150 years.
Ryan Schmedding and Andreas Zuend
EGUsphere, https://doi.org/10.5194/egusphere-2024-1690, https://doi.org/10.5194/egusphere-2024-1690, 2024
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Four different approaches for computing the interfacial tension between liquid phases in aerosol particles were tested for particles with diameters from 10 nm to more than 5 μm. Antonov's rule led to the strongest reductions in the onset relative humidity of liquid–liquid phase separation and reproduced measured interfacial tensions for highly immiscible systems. A modified form of the Butler equation was able to best reproduce measured interfacial tensions in more miscible systems.
Qianqian Song, Paul Ginoux, María Gonçalves Ageitos, Ron L. Miller, Vincenzo Obiso, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 7421–7446, https://doi.org/10.5194/acp-24-7421-2024, https://doi.org/10.5194/acp-24-7421-2024, 2024
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We implement and simulate the distribution of eight dust minerals in the GFDL AM4.0 model. We found that resolving the eight minerals reduces dust absorption compared to the homogeneous dust used in the standard GFDL AM4.0 model that assumes a globally uniform hematite content of 2.7 % by volume. Resolving dust mineralogy results in significant impacts on radiation, land surface temperature, surface winds, and precipitation over North Africa in summer.
Mingxu Liu, Hitoshi Matsui, Douglas Hamilton, Sagar Rathod, Kara Lamb, and Natalie Mahowald
EGUsphere, https://doi.org/10.5194/egusphere-2024-1454, https://doi.org/10.5194/egusphere-2024-1454, 2024
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Atmospheric aerosol deposition provides iron to promote marine primary production, yet its amount remains highly uncertain. This study demonstrates that iron-containing particle size at emission is a critical factor in regulating their input to open oceans by performing global aerosol simulations. Further observational constraints on this are needed to reduce modelling uncertainties.
Senyi Kong, Zheng Wang, and Lei Bi
Atmos. Chem. Phys., 24, 6911–6935, https://doi.org/10.5194/acp-24-6911-2024, https://doi.org/10.5194/acp-24-6911-2024, 2024
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The retrieval of refractive indices of dust aerosols from laboratory optical measurements is commonly done assuming spherical particles. This paper aims to investigate the uncertainties in the shortwave refractive indices and corresponding optical properties by considering non-spherical and inhomogeneous models for dust samples. The study emphasizes the significance of using non-spherical models for simulating dust aerosols.
Wenxuan Hua, Sijia Lou, Xin Huang, Lian Xue, Ke Ding, Zilin Wang, and Aijun Ding
Atmos. Chem. Phys., 24, 6787–6807, https://doi.org/10.5194/acp-24-6787-2024, https://doi.org/10.5194/acp-24-6787-2024, 2024
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In this study, we diagnose uncertainties in carbon monoxide and organic carbon emissions from four inventories for seven major wildfire-prone regions. Uncertainties in vegetation classification methods, fire detection products, and cloud obscuration effects lead to bias in these biomass burning (BB) emission inventories. By comparing simulations with measurements, we provide certain inventory recommendations. Our study has implications for reducing uncertainties in emissions in further studies.
Léo Clauzel, Sandrine Anquetin, Christophe Lavaysse, Gilles Bergametti, Christel Bouet, Guillaume Siour, Rémy Lapere, Béatrice Marticorena, and Jennie Thomas
EGUsphere, https://doi.org/10.5194/egusphere-2024-1604, https://doi.org/10.5194/egusphere-2024-1604, 2024
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Solar energy production in West Africa is set to rise, needing accurate solar radiation estimates, which is affected by desert dust. This work analyses a March 2021 dust event using a modelling strategy incorporating desert dust. Results show that considering desert dust cut errors in solar radiation estimates by 75 % and reduces surface solar radiation by 18 %. This highlights the importance of incorporating dust aerosols into solar forecasting for better accuracy.
Chandrakala Bharali, Mary Barth, Rajesh Kumar, Sachin D. Ghude, Vinayak Sinha, and Baerbel Sinha
Atmos. Chem. Phys., 24, 6635–6662, https://doi.org/10.5194/acp-24-6635-2024, https://doi.org/10.5194/acp-24-6635-2024, 2024
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This study examines the role of atmospheric aerosols in winter fog over the Indo-Gangetic Plains of India using WRF-Chem. The increase in RH with aerosol–radiation feedback (ARF) is found to be important for fog formation as it promotes the growth of aerosols in the polluted environment. Aqueous-phase chemistry in the fog increases PM2.5 concentration, further affecting ARF. ARF and aqueous-phase chemistry affect the fog intensity and the timing of fog formation by ~1–2 h.
Wenxin Zhao, Yu Zhao, Yu Zheng, Dong Chen, Jinyuan Xin, Kaitao Li, Huizheng Che, Zhengqiang Li, Mingrui Ma, and Yun Hang
Atmos. Chem. Phys., 24, 6593–6612, https://doi.org/10.5194/acp-24-6593-2024, https://doi.org/10.5194/acp-24-6593-2024, 2024
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We evaluate the long-term (2000–2020) variabilities of aerosol absorption optical depth, black carbon emissions, and associated health risks in China with an integrated framework that combines multiple observations and modeling techniques. We demonstrate the remarkable emission abatement resulting from the implementation of national pollution controls and show how human activities affected the emissions with a spatiotemporal heterogeneity, thus supporting differentiated policy-making by region.
Peng Xian, Jeffrey S. Reid, Melanie Ades, Angela Benedetti, Peter R. Colarco, Arlindo da Silva, Tom F. Eck, Johannes Flemming, Edward J. Hyer, Zak Kipling, Samuel Rémy, Tsuyoshi Thomas Sekiyama, Taichu Tanaka, Keiya Yumimoto, and Jianglong Zhang
Atmos. Chem. Phys., 24, 6385–6411, https://doi.org/10.5194/acp-24-6385-2024, https://doi.org/10.5194/acp-24-6385-2024, 2024
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The study compares and evaluates monthly AOD of four reanalyses (RA) and their consensus (i.e., ensemble mean). The basic verification characteristics of these RA versus both AERONET and MODIS retrievals are presented. The study discusses the strength of each RA and identifies regions where divergence and challenges are prominent. The RA consensus usually performs very well on a global scale in terms of how well it matches the observational data, making it a good choice for various applications.
Roger Teoh, Zebediah Engberg, Ulrich Schumann, Christiane Voigt, Marc Shapiro, Susanne Rohs, and Marc E. J. Stettler
Atmos. Chem. Phys., 24, 6071–6093, https://doi.org/10.5194/acp-24-6071-2024, https://doi.org/10.5194/acp-24-6071-2024, 2024
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The radiative forcing (RF) due to aviation contrails is comparable to that caused by CO2. We estimate that global contrail net RF in 2019 was 62.1 mW m−2. This is ~1/2 the previous best estimate for 2018. Contrail RF varies regionally due to differences in conditions required for persistent contrails. COVID-19 reduced contrail RF by 54% in 2020 relative to 2019. Globally, 2 % of all flights account for 80 % of the annual contrail energy forcing, suggesting a opportunity to mitigate contrail RF.
Ragnhild Bieltvedt Skeie, Rachael Byrom, Øivind Hodnebrog, Caroline Jouan, and Gunnar Myhre
EGUsphere, https://doi.org/10.5194/egusphere-2024-1394, https://doi.org/10.5194/egusphere-2024-1394, 2024
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In 2020 new regulations by the International Maritime Organization of sulphur emissions came into force that reduced emissions of SO2 from the shipping sector by approximately 80 %. In this study, we use multiple models to calculate by how much the Earth energy balance changed due to the emission reduction, the so called effective radiative forcing. The calculated effective radiative forcing is weak, comparable to the effect of the increase in CO2 over the last two to three years.
Haotian Zu, Biwu Chu, Yiqun Lu, Ling Liu, and Xiuhui Zhang
Atmos. Chem. Phys., 24, 5823–5835, https://doi.org/10.5194/acp-24-5823-2024, https://doi.org/10.5194/acp-24-5823-2024, 2024
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The nucleation of iodic acid (HIO3) and iodous acid (HIO2) was proven to be critical in marine areas. However, HIO3–HIO2 nucleation cannot effectively derive the rapid nucleation in some polluted coasts. We find a significant enhancement of dimethylamine (DMA) on the HIO3–HIO2 nucleation in marine and polar regions with abundant DMA sources, which may establish reasonable connections between the HIO3–HIO2 nucleation and the rapid formation of new particles in polluted marine and polar regions.
Junghwa Lee, Patric Seifert, Tempei Hashino, Maximilian Maahn, Fabian Senf, and Oswald Knoth
Atmos. Chem. Phys., 24, 5737–5756, https://doi.org/10.5194/acp-24-5737-2024, https://doi.org/10.5194/acp-24-5737-2024, 2024
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Spectral bin model simulations of an idealized supercooled stratiform cloud were performed with the AMPS model for variable CCN and INP concentrations. We performed radar forward simulations with PAMTRA to transfer the simulations into radar observational space. The derived radar reflectivity factors were compared to observational studies of stratiform mixed-phase clouds. These studies report a similar response of the radar reflectivity factor to aerosol perturbations as we found in our study.
Masaru Yoshioka, Daniel P. Grosvenor, Ben B. B. Booth, Colin P. Morice, and Kenneth S. Carslaw
EGUsphere, https://doi.org/10.5194/egusphere-2024-1428, https://doi.org/10.5194/egusphere-2024-1428, 2024
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Sulfur emissions from shipping has been reduced by about 80 % as a result of the new regulation introduced in 2020. This has reduced aerosol in the atmosphere and its cooling effect through interactions with clouds. As a result, our coupled climate model simulations predict a global warming of 0.04 K averaged over three decades, potentially surpassing the Paris target of 1.5 K or contributing to recent temperature spikes, particularly notable in the Arctic with a mean warming of 0.15 K.
Basudev Swain, Marco Vountas, Aishwarya Singh, Nidhi L. Anchan, Adrien Deroubaix, Luca Lelli, Yanick Ziegler, Sachin S. Gunthe, Hartmut Bösch, and John P. Burrows
Atmos. Chem. Phys., 24, 5671–5693, https://doi.org/10.5194/acp-24-5671-2024, https://doi.org/10.5194/acp-24-5671-2024, 2024
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Arctic amplification (AA) accelerates the warming of the central Arctic cryosphere and affects aerosol dynamics. Limited observations hinder a comprehensive analysis. This study uses AEROSNOW aerosol optical density (AOD) data and GEOS-Chem simulations to assess AOD variability. Discrepancies highlight the need for improved observational integration into models to refine our understanding of aerosol effects on cloud microphysics, ice nucleation, and radiative forcing under evolving AA.
Vincenzo Obiso, María Gonçalves Ageitos, Carlos Pérez García-Pando, Jan P. Perlwitz, Gregory L. Schuster, Susanne E. Bauer, Claudia Di Biagio, Paola Formenti, Kostas Tsigaridis, and Ron L. Miller
Atmos. Chem. Phys., 24, 5337–5367, https://doi.org/10.5194/acp-24-5337-2024, https://doi.org/10.5194/acp-24-5337-2024, 2024
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We calculate the dust direct radiative effect (DRE) in an Earth system model accounting for regionally varying soil mineralogy through a new observationally constrained method. Linking dust absorption at solar wavelengths to the varying amount of specific minerals (i.e., iron oxides) improves the modeled range of dust single scattering albedo compared to observations and increases the global cooling by dust. Our results may contribute to improved estimates of the dust DRE and its climate impact.
Charlotte M. Beall, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Adam Varble, Kentaroh Suzuki, and Takuro Michibata
Atmos. Chem. Phys., 24, 5287–5302, https://doi.org/10.5194/acp-24-5287-2024, https://doi.org/10.5194/acp-24-5287-2024, 2024
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Single-layer warm liquid clouds cover nearly one-third of the Earth's surface, and uncertainties regarding the impact of aerosols on their radiative properties pose a significant challenge to climate prediction. Here, we demonstrate how satellite observations can be used to constrain Earth system model estimates of the radiative forcing from the interactions of aerosols with clouds due to warm rain processes.
Xiaoli Wei, Qian Cui, Leiming Ma, Feng Zhang, Wenwen Li, and Peng Liu
Atmos. Chem. Phys., 24, 5025–5045, https://doi.org/10.5194/acp-24-5025-2024, https://doi.org/10.5194/acp-24-5025-2024, 2024
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A new aerosol-type classification algorithm has been proposed. It includes an optical database built by Mie scattering and a complex refractive index working as a baseline to identify different aerosol types. The new algorithm shows high accuracy and efficiency. Hence, a global map of aerosol types was generated to characterize aerosol types across the five continents. It will help improve the accuracy of aerosol inversion and determine the sources of aerosol pollution.
Zhiqiang Zhang, Ying Li, Haiyan Ran, Junling An, Yu Qu, Wei Zhou, Weiqi Xu, Weiwei Hu, Hongbin Xie, Zifa Wang, Yele Sun, and Manabu Shiraiwa
Atmos. Chem. Phys., 24, 4809–4826, https://doi.org/10.5194/acp-24-4809-2024, https://doi.org/10.5194/acp-24-4809-2024, 2024
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Secondary organic aerosols (SOAs) can exist in liquid, semi-solid, or amorphous solid states, which are rarely accounted for in current chemical transport models. We predict the phase state of SOA particles over China and find that in northwestern China SOA particles are mostly highly viscous or glassy solid. Our results indicate that the particle phase state should be considered in SOA formation in chemical transport models for more accurate prediction of SOA mass concentrations.
Alejandro Baró Pérez, Michael S. Diamond, Frida A.-M. Bender, Abhay Devasthale, Matthias Schwarz, Julien Savre, Juha Tonttila, Harri Kokkola, Hyunho Lee, David Painemal, and Annica M. L. Ekman
Atmos. Chem. Phys., 24, 4591–4610, https://doi.org/10.5194/acp-24-4591-2024, https://doi.org/10.5194/acp-24-4591-2024, 2024
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We use a numerical model to study interactions between humid light-absorbing aerosol plumes, clouds, and radiation over the southeast Atlantic. We find that the warming produced by the aerosols reduces cloud cover, especially in highly polluted situations. Aerosol impacts on drizzle play a minor role. However, aerosol effects on cloud reflectivity and moisture-induced changes in cloud cover dominate the climatic response and lead to an overall cooling by the biomass burning plumes.
Danny M. Leung, Jasper F. Kok, Longlei Li, David M. Lawrence, Natalie M. Mahowald, Simone Tilmes, and Erik Kluzek
EGUsphere, https://doi.org/10.5194/egusphere-2024-1124, https://doi.org/10.5194/egusphere-2024-1124, 2024
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This study derives a desert dust emission dataset for 1841–2000, by employing a combination of observed dust records from sedimentary cores as well as reanalyzed global dust cycle constraints. We evaluate the ability of global models to replicate the observed historical dust variability by using the emission dataset to force a historical simulation in an Earth system model. We show that prescribing our emissions forces the model to match better against observations than other mechanistic models.
Sampa Das, Peter R. Colarco, Huisheng Bian, and Santiago Gassó
Atmos. Chem. Phys., 24, 4421–4449, https://doi.org/10.5194/acp-24-4421-2024, https://doi.org/10.5194/acp-24-4421-2024, 2024
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The smoke aerosols emitted from vegetation burning can alter the regional energy budget via multiple pathways. We utilized detailed observations from the NASA ORACLES airborne campaign based in Namibia during September 2016 to improve the representation of smoke aerosol properties and lifetimes in our GEOS Earth system model. The improved model simulations are for the first time able to capture the observed changes in the smoke absorption during long-range plume transport.
Jingmin Li, Mattia Righi, Johannes Hendricks, Christof G. Beer, Ulrike Burkhardt, and Anja Schmidt
EGUsphere, https://doi.org/10.5194/egusphere-2024-1024, https://doi.org/10.5194/egusphere-2024-1024, 2024
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Aiming to understand underlying patterns and trends in aerosols, we characterize the spatial patterns and long-term evolution of lower tropospheric aerosols by clustering multiple aerosol properties from preindustrial times to the year 2050 under three SSP scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Emilio Cuevas-Agulló, David Barriopedro, Rosa Delia García, Silvia Alonso-Pérez, Juan Jesús González-Alemán, Ernest Werner, David Suárez, Juan José Bustos, Gerardo García-Castrillo, Omaira García, África Barreto, and Sara Basart
Atmos. Chem. Phys., 24, 4083–4104, https://doi.org/10.5194/acp-24-4083-2024, https://doi.org/10.5194/acp-24-4083-2024, 2024
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During February–March (FM) 2020–2022, unusually intense dust storms from northern Africa hit the western Euro-Mediterranean (WEM). Using dust products from satellites and atmospheric reanalysis for 2003–2022, results show that cut-off lows and European blocking are key drivers of FM dust intrusions over the WEM. A higher frequency of cut-off lows associated with subtropical ridges is observed in the late 2020–2022 period.
Yahui Che, Bofu Yu, and Katherine Bracco
Atmos. Chem. Phys., 24, 4105–4128, https://doi.org/10.5194/acp-24-4105-2024, https://doi.org/10.5194/acp-24-4105-2024, 2024
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Dust events occur more frequently during the Austral spring and summer in dust regions, including central Australia, the southwest of Western Australia, and the northern and southern regions of eastern Australia using remote sensing and reanalysis datasets. High-concentration dust is distributed around central Australia and in the downwind northern and southern Australia. Typically, around 50 % of the dust lifted settles on Australian land, with the remaining half being deposited in the ocean.
Jonathan Elsey, Nicolas Bellouin, and Claire Ryder
Atmos. Chem. Phys., 24, 4065–4081, https://doi.org/10.5194/acp-24-4065-2024, https://doi.org/10.5194/acp-24-4065-2024, 2024
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Aerosols influence the Earth's energy balance. The uncertainty in this radiative forcing is large depending partly on uncertainty in measurements of aerosol optical properties. We have developed a freely available new framework of millions of radiative transfer simulations spanning aerosol uncertainty and assess the impact on radiative forcing uncertainty. We find that reducing these uncertainties would reduce radiative forcing uncertainty, but non-aerosol uncertainties must also be considered.
Jing Li, Nan Wu, Biwu Chu, An Ning, and Xiuhui Zhang
Atmos. Chem. Phys., 24, 3989–4000, https://doi.org/10.5194/acp-24-3989-2024, https://doi.org/10.5194/acp-24-3989-2024, 2024
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Iodic acid (HIO3) nucleates with iodous acid (HIO2) efficiently in marine areas; however, whether methanesulfonic acid (MSA) can synergistically participate in the HIO3–HIO2-based nucleation is unclear. We provide molecular-level evidence that MSA can efficiently promote the formation of HIO3–HIO2-based clusters using a theoretical approach. The proposed MSA-enhanced iodine nucleation mechanism may help us to deeply understand marine new particle formation events with bursts of iodine particles.
Hao Wang, Xiaohong Liu, Chenglai Wu, and Guangxing Lin
Atmos. Chem. Phys., 24, 3309–3328, https://doi.org/10.5194/acp-24-3309-2024, https://doi.org/10.5194/acp-24-3309-2024, 2024
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We quantified different global- and regional-scale drivers of biogenic volatile organic compound (BVOC) emission trends over the past 20 years. The results show that global greening trends significantly boost BVOC emissions and deforestation reduces BVOC emissions in South America and Southeast Asia. Elevated temperature in Europe and increased soil moisture in East and South Asia enhance BVOC emissions. The results deepen our understanding of long-term BVOC emission trends in hotspots.
Christof G. Beer, Johannes Hendricks, and Mattia Righi
Atmos. Chem. Phys., 24, 3217–3240, https://doi.org/10.5194/acp-24-3217-2024, https://doi.org/10.5194/acp-24-3217-2024, 2024
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Ice-nucleating particles (INPs) have important influences on cirrus clouds and the climate system; however, the understanding of their global impacts is still uncertain. We perform numerical simulations with a global aerosol–climate model to analyse INP-induced cirrus changes and the resulting climate impacts. We evaluate various sources of uncertainties, e.g. the ice-nucleating ability of INPs and the role of model dynamics, and provide a new estimate for the global INP–cirrus effect.
Jiawei Li, Zhiwei Han, Pingqing Fu, Xiaohong Yao, and Mingjie Liang
Atmos. Chem. Phys., 24, 3129–3161, https://doi.org/10.5194/acp-24-3129-2024, https://doi.org/10.5194/acp-24-3129-2024, 2024
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Organic aerosols of marine origin are important for aerosol climatic effects but are poorly understood. For the first time, an online coupled regional chemistry–climate model is applied to explore the characteristics of emission, distribution, and direct and indirect radiative effects of marine organic aerosols over the western Pacific, which reveals an important role of marine organic aerosols in perturbing cloud and radiation and promotes understanding of global aerosol climatic impact.
Yawen Liu, Yun Qian, Philip J. Rasch, Kai Zhang, Lai-yung Ruby Leung, Yuhang Wang, Minghuai Wang, Hailong Wang, Xin Huang, and Xiu-Qun Yang
Atmos. Chem. Phys., 24, 3115–3128, https://doi.org/10.5194/acp-24-3115-2024, https://doi.org/10.5194/acp-24-3115-2024, 2024
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Fire management has long been a challenge. Here we report that spring-peak fire activity over southern Mexico and Central America (SMCA) has a distinct quasi-biennial signal by measuring multiple fire metrics. This signal is initially driven by quasi-biennial variability in precipitation and is further amplified by positive feedback of fire–precipitation interaction at short timescales. This work highlights the importance of fire–climate interactions in shaping fires on an interannual scale.
Xu Feng, Loretta J. Mickley, Michelle L. Bell, Tianjia Liu, Jenny A. Fisher, and Maria Val Martin
Atmos. Chem. Phys., 24, 2985–3007, https://doi.org/10.5194/acp-24-2985-2024, https://doi.org/10.5194/acp-24-2985-2024, 2024
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During severe wildfire seasons, smoke can have a significant impact on air quality in Australia. Our study demonstrates that characterization of the smoke plume injection fractions greatly affects estimates of surface smoke PM2.5. Using the plume behavior predicted by the machine learning method leads to the best model agreement with observed surface PM2.5 in key cities across Australia, with smoke PM2.5 accounting for 5 %–52 % of total PM2.5 on average during fire seasons from 2009 to 2020.
Shiyi Lai, Ximeng Qi, Xin Huang, Sijia Lou, Xuguang Chi, Liangduo Chen, Chong Liu, Yuliang Liu, Chao Yan, Mengmeng Li, Tengyu Liu, Wei Nie, Veli-Matti Kerminen, Tuukka Petäjä, Markku Kulmala, and Aijun Ding
Atmos. Chem. Phys., 24, 2535–2553, https://doi.org/10.5194/acp-24-2535-2024, https://doi.org/10.5194/acp-24-2535-2024, 2024
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By combining in situ measurements and chemical transport modeling, this study investigates new particle formation (NPF) on the southeastern Tibetan Plateau. We found that the NPF was driven by the presence of biogenic gases and the transport of anthropogenic precursors. The NPF was vertically heterogeneous and shaped by the vertical mixing. This study highlights the importance of anthropogenic–biogenic interactions and meteorological dynamics in NPF in this climate-sensitive region.
Adriana Rocha-Lima, Peter R. Colarco, Anton S. Darmenov, Edward P. Nowottnick, Arlindo M. da Silva, and Luke D. Oman
Atmos. Chem. Phys., 24, 2443–2464, https://doi.org/10.5194/acp-24-2443-2024, https://doi.org/10.5194/acp-24-2443-2024, 2024
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Observations show an increasing aerosol optical depth trend in the Middle East between 2003–2012. We evaluate the NASA Goddard Earth Observing System (GEOS) model's ability to capture these trends and examine the meteorological and surface parameters driving dust emissions. Our results highlight the importance of data assimilation for long-term trends of atmospheric aerosols and support the hypothesis that vegetation cover loss may have contributed to increasing dust emissions in the period.
Cited articles
Adhikary, B., Kulkarni, S., Dallura, A., Tang, Y., Chai, T., Leung, L. R., Qian, Y., Chung, C. E., Ramanathan, V., and Carmichael, G. R.: A regional scale chemical transport modeling of Asian aerosols with data assimilation of AOD observations using optimal interpolation technique, Atmos. Environ., 42, 8600–8615, https://doi.org/10.1016/j.atmosenv.2008.08.031, 2008.
Benedetti, A., Morcrette, J. J., Boucher, O., Dethof, A., Engelen, R. J., Fisher, M., Flentje, H., Huneeus, N., Jones, L., Kaiser, J. W., Kinne, S., Mangold, A., Razinger, M., Simmons, A. J., and Suttie, M.: Aerosol analysis and forecast in the European Centre for Medium-Range Weather Forecasts Integrated Forecast System: 2. Data assimilation, J. Geophys. Res.-Atmos., 114, D13205, https://doi.org/10.1029/2008jd011115, 2009.
Bond, T. C., Doherty, S. J., Fahey, D. W., Forster, P. M., Berntsen, T., DeAngelo, B. J., Flanner, M. G., Ghan, S., Kaercher, B., Koch, D., Kinne, S., Kondo, Y., Quinn, P. K., Sarofim, M. C., Schultz, M. G., Schulz, M., Venkataraman, C., Zhang, H., Zhang, S., Bellouin, N., Guttikunda, S. K., Hopke, P. K., Jacobson, M. Z., Kaiser, J. W., Klimont, Z., Lohmann, U., Schwarz, J. P., Shindell, D., Storelvmo, T., Warren, S. G., and Zender, C. S.: Bounding the role of black carbon in the climate system: A scientific assessment, J. Geophys. Res.-Atmos., 118, 5380–5552, https://doi.org/10.1002/jgrd.50171, 2013.
Cao, J., Tie, X., Xu, B., Zhao, Z., Zhu, C., Li, G., and Liu, S.: Measuring and modeling black carbon (BC) contamination in the SE Tibetan Plateau, J. Atmos. Chem., 67, 45–60, https://doi.org/10.1007/s10874-011-9202-5, 2010.
Chen, D., Liu, Z., Schwartz, C. S., Lin, H. C., Cetola, J. D., Gu, Y., and Xue, L.: The impact of aerosol optical depth assimilation on aerosol forecasts and radiative effects during a wild fire event over the United States, Geosci. Model Dev., 7, 2709–2715, https://doi.org/10.5194/gmd-7-2709-2014, 2014.
Chen, D., Liu, Z., Davis, C., and Gu, Y.: Dust radiative effects on atmospheric thermodynamics and tropical cyclogenesis over the Atlantic Ocean using WRF-Chem coupled with an AOD data assimilation system, Atmos. Chem. Phys., 17, 7917–7939, https://doi.org/10.5194/acp-17-7917-2017, 2017.
Chen, F. and Dudhia, J.: Coupling an advanced land surface-hydrology model with the Penn State-NCAR MM5 modeling system. Part I: Model implementation and sensitivity, Mon. Weather Rev., 129, 569–585, https://doi.org/10.1175/1520-0493(2001)129<0569:Caalsh>2.0.Co;2, 2001.
Cheng, Y., Dai, T., Goto, D., Schutgens, N. A. J., Shi, G., and Nakajima, T.: Investigating the assimilation of CALIPSO global aerosol vertical observations using a four-dimensional ensemble Kalman filter, Atmos. Chem. Phys., 19, 13445–13467, https://doi.org/10.5194/acp-19-13445-2019, 2019.
Cheng, Y., Dai, T., Goto, D., Murakami, H., Yoshida, M., Shi, G., and Nakajima, T.: Enhanced Simulation of an Asian Dust Storm by Assimilating GCOM-C Observations, Remote Sens., 13, 3020, https://doi.org/10.3390/rs13153020, 2021.
Christopher, S. A., Wang, J., Ji, Q., and Tsay, S. C.: Estimation of diurnal shortwave dust aerosol radiative forcing during PRIDE, J. Geophys. Res.-Atmos., 108, 8596, https://doi.org/10.1029/2002jd002787, 2003.
Collins, W. D., Rasch, P. J., Eaton, B. E., Khattatov, B. V., Lamarque, J. F., and Zender, C. S.: Simulating aerosols using a chemical transport model with assimilation of satellite aerosol retrievals: Methodology for INDOEX, J. Geophys. Res.-Atmos., 106, 7313–7336, https://doi.org/10.1029/2000jd900507, 2001.
Crippa, M., Guizzardi, D., Butler, T., Keating, T., Wu, R., Kaminski, J., Kuenen, J., Kurokawa, J., Chatani, S., Morikawa, T., Pouliot, G., Racine, J., Moran, M. D., Klimont, Z., Manseau, P. M., Mashayekhi, R., Henderson, B. H., Smith, S. J., Suchyta, H., Muntean, M., Solazzo, E., Banja, M., Schaaf, E., Pagani, F., Woo, J.-H., Kim, J., Monforti-Ferrario, F., Pisoni, E., Zhang, J., Niemi, D., Sassi, M., Ansari, T., and Foley, K.: The HTAP_v3 emission mosaic: merging regional and globalmonthly emissions (2000–2018) to support air quality modelling and policies, Earth Syst. Sci. Data, 15, 2667–2694, https://doi.org/10.5194/essd-15-2667-2023, 2023.
Dai, T., Goto, D., Schutgens, N. A. J., Dong, X., Shia, G., and Nakajima, T.: Simulated aerosol key optical properties over global scale using an aerosol transport model coupled with a new type of dynamic core, Atmos. Environ., 82, 71–82, https://doi.org/10.1016/j.atmosenv.2013.10.018, 2014.
Dai, T., Cheng, Y., Suzuki, K., Goto, D., Kikuchi, M., Schutgens, N. A. J., Yoshida, M., Zhang, P., Husi, L., Shi, G., and Nakajima, T.: Hourly Aerosol Assimilation of Himawari-8 AOT Using the Four-Dimensional Local Ensemble Transform Kalman Filter, J. Adv. Model. Earth Syst., 11, 680–711, https://doi.org/10.1029/2018ms001475, 2019.
Dai, T., Cheng, Y., Goto, D., Li, Y., Tang, X., Shi, G., and Nakajima, T.: Revealing the sulfur dioxide emission reductions in China by assimilating surface observations in WRF-Chem, Atmos. Chem. Phys., 21, 4357–4379, https://doi.org/10.5194/acp-21-4357-2021, 2021.
Di Tomaso, E., Schutgens, N. A. J., Jorba, O., and Garcia-Pando, C. P.: Assimilation of MODIS Dark Target and Deep Blue observations in the dust aerosol component of NMMB-MONARCH version 1.0, Geosci. Model Dev., 10, 1107–1129, https://doi.org/10.5194/gmd-10-1107-2017, 2017.
Emmons, L. K., Schwantes, R. H., Orlando, J. J., Tyndall, G., Kinnison, D., Lamarque, J.-F., Marsh, D., Mills, M. J., Tilmes, S., Bardeen, C., Buchholz, R. R., Conley, A., Gettelman, A., Garcia, R., Simpson, I., Blake, D. R., Meinardi, S., and Petron, G.: The Chemistry Mechanism in the Community Earth System Model Version 2 (CESM2), J. Adv. Model. Earth Syst., 12, e2019MS001882, https://doi.org/10.1029/2019ms001882, 2020.
Fast, J. D., Gustafson, W. I., Jr., Easter, R. C., Zaveri, R. A., Barnard, J. C., Chapman, E. G., Grell, G. A., and Peckham, S. E.: Evolution of ozone, particulates, and aerosol direct radiative forcing in the vicinity of Houston using a fully coupled meteorology-chemistry-aerosol model, J. Geophys. Res.-Atmos., 111, D21305, https://doi.org/10.1029/2005jd006721, 2006.
Fukuda, S., Nakajima, T., Takenaka, H., Higurashi, A., Kikuchi, N., Nakajima, T. Y., and Ishida, H.: New approaches to removing cloud shadows and evaluating the 380 nm surface reflectance for improved aerosol optical thickness retrievals from the GOSAT/TANSO-Cloud and Aerosol Imager, J. Geophys. Res.-Atmos., 118, 13520–13531, https://doi.org/10.1002/2013jd020090, 2013.
Gao, C., Xiu, A., Zhang, X., Tong, Q., Zhao, H., Zhang, S., Yang, G., and Zhang, M.: Two-way coupled meteorology and air quality models in Asia: a systematic review and meta-analysis of impacts of aerosol feedbacks on meteorology and air quality, Atmos. Chem. Phys., 22, 5265–5329, https://doi.org/10.5194/acp-22-5265-2022, 2022.
Generoso, S., Breon, F. M., Chevallier, F., Balkanski, Y., Schulz, M., and Bey, I.: Assimilation of POLDER aerosol optical thickness into the LMDz-INCA model: Implications for the Arctic aerosol burden, J. Geophys. Res.-Atmos., 112, D02311, https://doi.org/10.1029/2005jd006954, 2007.
Ginoux, P., Chin, M., Tegen, I., Prospero, J. M., Holben, B., Dubovik, O., and Lin, S. J.: Sources and distributions of dust aerosols simulated with the GOCART model, J. Geophys. Res.-Atmos., 106, 20255–20273, https://doi.org/10.1029/2000jd000053, 2001.
Grell, G. A. and Devenyi, D.: A generalized approach to parameterizing convection combining ensemble and data assimilation techniques, Geophys. Res. Lett., 29, 38-1–38-4, https://doi.org/10.1029/2002gl015311, 2002.
Grell, G. A., Peckham, S. E., Schmitz, R., McKeen, S. A., Frost, G., Skamarock, W. C., and Eder, B.: Fully coupled “online” chemistry within the WRF model, Atmos. Environ., 39, 6957–6975, https://doi.org/10.1016/j.atmosenv.2005.04.027, 2005.
Guenther, A., Karl, T., Harley, P., Wiedinmyer, C., Palmer, P. I., and Geron, C.: Estimates of global terrestrial isoprene emissions using MEGAN (Model of Emissions of Gases and Aerosols from Nature), Atmos. Chem. Phys., 6, 3181–3210, https://doi.org/10.5194/acp-6-3181-2006, 2006.
Gui, S., Liang, S., Wang, K., Li, L., and Zhang, X.: Assessment of Three Satellite-Estimated Land Surface Downwelling Shortwave Irradiance Data Sets, IEEE Geosci. Remote Sens. Lett., 7, 776–780, https://doi.org/10.1109/lgrs.2010.2048196, 2010.
Hansen, J. and Nazarenko, L.: Soot climate forcing via snow and ice albedos, P. Natla. Acad. Sci. USA, 101, 423–428, https://doi.org/10.1073/pnas.2237157100, 2004.
Higurashi, A. and Nakajima, T.: Development of a two-channel aerosol retrieval algorithm on a global scale using NOAA AVHRR, J. Atmos. Sci., 56, 924–941, https://doi.org/10.1175/1520-0469(1999)056<0924:Doatca>2.0.Co;2, 1999.
Higurashi, A. and Nakajima, T.: Detection of aerosol types over the East China Sea near Japan from four-channel satellite data, Geophys. Res. Lett., 29, 17-1–17-4, https://doi.org/10.1029/2002gl015357, 2002.
Hong, S.-Y., Noh, Y., and Dudhia, J.: A new vertical diffusion package with an explicit treatment of entrainment processes, Mon. Weather Rev., 134, 2318–2341, https://doi.org/10.1175/mwr3199.1, 2006.
Huang, J., Minnis, P., Yi, Y., Tang, Q., Wang, X., Hu, Y., Liu, Z., Ayers, K., Trepte, C., and Winker, D.: Summer dust aerosols detected from CALIPSO over the Tibetan Plateau, Geophys. Res. Lett., 34, L18805, https://doi.org/10.1029/2007gl029938, 2007.
Hunt, B. R., Kostelich, E. J., and Szunyogh, I.: Efficient data assimilation for spatiotemporal chaos: A local ensemble transform Kalman filter, Physica D, 230, 112–126, https://doi.org/10.1016/j.physd.2006.11.008, 2007.
Iacono, M. J., Delamere, J. S., Mlawer, E. J., Shephard, M. W., Clough, S. A., and Collins, W. D.: Radiative forcing by long-lived greenhouse gases: Calculations with the AER radiative transfer models, J. Geophys. Res.-Atmos., 113, D13103, https://doi.org/10.1029/2008jd009944, 2008.
Jacobson, M. Z.: Strong radiative heating due to the mixing state of black carbon in atmospheric aerosols, Nature, 409, 695–697, https://doi.org/10.1038/35055518, 2001.
JAXA: AHI, Himawari-8 data, http://www.eorc.jaxa.jp/ptree/index.html, last access: 5 January 2024.
Kato, S., Loeb, N. G., Rose, F. G., Doelling, D. R., Rutan, D. A., Caldwell, T. E., Yu, L., and Weller, R. A.: Surface Irradiances Consistent with CERES-Derived Top-of-Atmosphere Shortwave and Longwave Irradiances, J. Climate, 26, 2719–2740, https://doi.org/10.1175/jcli-d-12-00436.1, 2013.
Kikuchi, M., Murakami, H., Suzuki, K., Nagao, T. M., and Higurashi, A.: Improved Hourly Estimates of Aerosol Optical Thickness Using Spatiotemporal Variability Derived From Himawari-8 Geostationary Satellite, IEEE T. Geosci. Remote, 56, 3442–3455, https://doi.org/10.1109/tgrs.2018.2800060, 2018.
King, M. D.: Remote-sensing of cloud, aerosol and water-vapor properties from the Moderate Resolution Imaging Spectrometer (MODIS), in: 115th Course of the International School of Physics Enrico Fermi: The Use of Eos (Earth Observing System) for Studies of Atmospheric Physics, 26 June–6 July 1992, Varenna, Italy, 253–285, WOS:A1992BY55L00014, 1992.
Koren, I., Kaufman, Y. J., Remer, L. A., and Martins, J. V.: Measurement of the effect of Amazon smoke on inhibition of cloud formation, Science, 303, 1342–1345, https://doi.org/10.1126/science.1089424, 2004.
Lee, K., Yu, J., Lee, S., Park, M., Hong, H., Park, S. Y., Choi, M., Kim, J., Kim, Y., Woo, J.-H., Kim, S.-W., and Song, C. H.: Development of Korean Air Quality Prediction System version 1 (KAQPS v1) with focuses on practical issues, Geosci. Model Dev., 13, 1055–1073, https://doi.org/10.5194/gmd-13-1055-2020, 2020.
Letu, H., Nakajima, T. Y., Wang, T., Shang, H., Ma, R., Yang, K., Baran, A. J., Riedi, J., Ishimoto, H., Yoshida, M., Shi, C., Khatri, P., Du, Y., Chen, L., and Shi, J.: A new benchmark for surface radiation products over the East Asia–Pacific region retrieved from the Himawari-8/AHI next-generation geostationary satellite, B. Am. Meteorol. Soc., 103, E873–E888, 2022.
Li, F., Wan, X., Wang, H., Orsolini, Y. J., Cong, Z., Gao, Y., and Kang, S.: Arctic sea-ice loss intensifies aerosol transport to the Tibetan Plateau, Nat. Clim. Change, 10, 1037–1044, https://doi.org/10.1038/s41558-020-0881-2, 2020.
Li, M., Zhang, Q., Kurokawa, J.-i., Woo, J.-H., He, K., Lu, Z., Ohara, T., Song, Y., Streets, D. G., Carmichael, G. R., Cheng, Y., Hong, C., Huo, H., Jiang, X., Kang, S., Liu, F., Su, H., and Zheng, B.: MIX: a mosaic Asian anthropogenic emission inventory under the international collaboration framework of the MICS-Asia and HTAP, Atmos. Chem. Phys., 17, 935–963, https://doi.org/10.5194/acp-17-935-2017, 2017.
Liu, Z., Liu, D., Huang, J., Vaughan, M., Uno, I., Sugimoto, N., Kittaka, C., Trepte, C., Wang, Z., Hostetler, C., and Winker, D.: Airborne dust distributions over the Tibetan Plateau and surrounding areas derived from the first year of CALIPSO lidar observations, Atmos. Chem. Phys., 8, 5045–5060, https://doi.org/10.5194/acp-8-5045-2008, 2008.
Liu, Z., Liu, Q., Lin, H.-C., Schwartz, C. S., Lee, Y.-H., and Wang, T.: Three-dimensional variational assimilation of MODIS aerosol optical depth: Implementation and application to a dust storm over East Asia, J. Geophys. Res.-Atmos., 116, D23206, https://doi.org/10.1029/2011jd016159, 2011.
Lu, Z., Streets, D. G., Zhang, Q., and Wang, S.: A novel back-trajectory analysis of the origin of black carbon transported to the Himalayas and Tibetan Plateau during 1996–2010, Geophys. Res. Lett., 39, L01809, https://doi.org/10.1029/2011gl049903, 2012.
Ma, C., Wang, T., Mizzi, A. P., Anderson, J. L., Zhuang, B., Xie, M., and Wu, R.: Multiconstituent Data Assimilation With WRF-Chem/DART: Potential for Adjusting Anthropogenic Emissions and Improving Air Quality Forecasts Over Eastern China, J. Geophys. Res.-Atmos., 124, 7393–7412, https://doi.org/10.1029/2019jd030421, 2019.
Mansell, E. R., Ziegler, C. L., and Bruning, E. C.: Simulated Electrification of a Small Thunderstorm with Two-Moment Bulk Microphysics, J. Atmos. Sci., 67, 171–194, https://doi.org/10.1175/2009jas2965.1, 2010.
Marinoni, A., Cristofanelli, P., Laj, P., Duchi, R., Calzolari, F., Decesari, S., Sellegri, K., Vuillermoz, E., Verza, G. P., Villani, P., and Bonasoni, P.: Aerosol mass and black carbon concentrations, a two year record at NCO-P (5079 m, Southern Himalayas), Atmos. Chem. Phys., 10, 8551–8562, https://doi.org/10.5194/acp-10-8551-2010, 2010.
Martins, J. V., Tanre, D., Remer, L., Kaufman, Y., Mattoo, S., and Levy, R.: MODIS Cloud screening for remote sensing of aerosols over oceans using spatial variability, Geophys. Res. Lett., 29, MOD4-1–MOD4-4, https://doi.org/10.1029/2001gl013252, 2002.
Ming, J., Wang, P., Zhao, S., and Chen, P.: Disturbance of light-absorbing aerosols on the albedo in a winter snowpack of Central Tibet, J. Environ. Sci., 25, 1601–1607, https://doi.org/10.1016/s1001-0742(12)60220-4, 2013.
Miyoshi, T., Yamane, S., and Enomoto, T.: Localizing the Error Covariance by Physical Distances within a Local Ensemble Transform Kalman Filter (LETKF), SOLA, 3, 89–92, https://doi.org/10.2151/sola.2007-023, 2007.
NASA: MYD04_L2, https://modis-atmos.gsfc.nasa.gov/products/aerosol, last access: 5 January 2024a.
NASA: level 2.0 AOT dataset, https://aeronet.gsfc.nasa.gov, last access: 5 January 2024b.
NASA: CERES, SYN1deg-1Hour, https://ceres.larc.nasa.gov/data/data-product-dois/, last access: 5 January 2024c.
Park, R. S., Song, C. H., Han, K. M., Park, M. E., Lee, S. S., Kim, S. B., and Shimizu, A.: A study on the aerosol optical properties over East Asia using a combination of CMAQ-simulated aerosol optical properties and remote-sensing data via a data assimilation technique, Atmos. Chem. Phys., 11, 12275–12296, https://doi.org/10.5194/acp-11-12275-2011, 2011.
Peng, Z., Liu, Z., Chen, D., and Ban, J.: Improving PM2.5 forecast over China by the joint adjustment of initial conditions and source emissions with an ensemble Kalman filter, Atmos. Chem. Phys., 17, 4837–4855, https://doi.org/10.5194/acp-17-4837-2017, 2017.
Qiu, J.: Environmental Science Pollutants Capture the High Ground in the Himalayas, Science, 339, 1030–1031, https://doi.org/10.1126/science.339.6123.1030, 2013.
Ramanathan, V., Crutzen, P. J., Lelieveld, J., Mitra, A. P., Althausen, D., Anderson, J., Andreae, M. O., Cantrell, W., Cass, G. R., Chung, C. E., Clarke, A. D., Coakley, J. A., Collins, W. D., Conant, W. C., Dulac, F., Heintzenberg, J., Heymsfield, A. J., Holben, B., Howell, S., Hudson, J., Jayaraman, A., Kiehl, J. T., Krishnamurti, T. N., Lubin, D., McFarquhar, G., Novakov, T., Ogren, J. A., Podgorny, I. A., Prather, K., Priestley, K., Prospero, J. M., Quinn, P. K., Rajeev, K., Rasch, P., Rupert, S., Sadourny, R., Satheesh, S. K., Shaw, G. E., Sheridan, P., and Valero, F. P. J.: Indian Ocean Experiment: An integrated analysis of the climate forcing and effects of the great Indo-Asian haze, J. Geophys. Res.-Atmos., 106, 28371–28398, https://doi.org/10.1029/2001jd900133, 2001.
Reale, O., Lau, W. K., Kim, K.-M., and Brin, E.: Atlantic Tropical Cyclogenetic Processes during SOP-3 NAMMA in the GEOS-5 Global Data Assimilation and Forecast System, J. Atmos. Sci., 66, 3563–3578, https://doi.org/10.1175/2009jas3123.1, 2009.
Reale, O., Lau, K. M., da Silva, A., and Matsui, T.: Impact of assimilated and interactive aerosol on tropical cyclogenesis, Geophys. Res. Lett., 41, 3282–3288, https://doi.org/10.1002/2014gl059918, 2014.
Rubin, J. I., Reid, J. S., Hansen, J. A., Anderson, J. L., Holben, B. N., Xian, P., Westphal, D. L., and Zhang, J.: Assimilation of AERONET and MODIS AOT observations using variational and ensemble data assimilation methods and its impact on aerosol forecasting skill, J. Geophys. Res.-Atmos., 122, 4967–4992, https://doi.org/10.1002/2016jd026067, 2017.
Salomonson, V. V., Barnes, W. L., Maymon, P. W., Montgomery, H. E., and Ostrow, H.: MODIS – Advanced Facility Instrument For Studies Of The Earth As A System, IEEE T. Geosci. Remote, 27, 145–153, https://doi.org/10.1109/36.20292, 1989.
Sarangi, C., Qian, Y., Rittger, K., Ruby Leung, L., Chand, D., Bormann, K. J., and Painter, T. H.: Dust dominates high-altitude snow darkening and melt over high-mountain Asia, Nat. Clim. Change, 10, 1045–1051, https://doi.org/10.1038/s41558-020-00909-3, 2020.
Schutgens, N. A. J., Miyoshi, T., Takemura, T., and Nakajima, T.: Sensitivity tests for an ensemble Kalman filter for aerosol assimilation, Atmos. Chem. Phys., 10, 6583–6600, https://doi.org/10.5194/acp-10-6583-2010, 2010.
Skamarock, W. C., Klemp, J. B., Dudhia, J., Gill, D. O., Barker, D. M., Wang, W., and Powers, J. G.: A description of the advanced research WRF version 2, Tech. rep., Mesoscale and Microscale Meteorology Div., National Center For Atmospheric Research, Boulder, Co, USA, https://doi.org/10.5065/D68S4MVH, 2005.
Stephens, G. L., Li, J., Wild, M., Clayson, C. A., Loeb, N., Kato, S., L'Ecuyer, T., Stackhouse Jr., P. W., Lebsock, M., and Andrews, T.: An update on Earth's energy balance in light of the latest global observations, Nat. Geosci., 5, 691–696, https://doi.org/10.1038/ngeo1580, 2012.
Tang, X., Zhu, J., Wang, Z. F., and Gbaguidi, A.: Improvement of ozone forecast over Beijing based on ensemble Kalman filter with simultaneous adjustment of initial conditions and emissions, Atmos. Chem. Phys., 11, 12901–12916, https://doi.org/10.5194/acp-11-12901-2011, 2011.
Trenberth, K. E., Fasullo, J. T., and Balmaseda, M. A.: Earth's Energy Imbalance, J. Climate, 27, 3129–3144, https://doi.org/10.1175/jcli-d-13-00294.1, 2014.
Tsikerdekis, A., Schutgens, N. A. J., and Hasekamp, O. P.: Assimilating aerosol optical properties related to size and absorption from POLDER/PARASOL with an ensemble data assimilation system, Atmos. Chem. Phys., 21, 2637–2674, https://doi.org/10.5194/acp-21-2637-2021, 2021.
Wang, J., Nair, U. S., and Christopher, S. A.: GOES 8 aerosol optical thickness assimilation in a mesoscale model: Online integration of aerosol radiative effects, J. Geophys. Res.-Atmos., 109, D23203, https://doi.org/10.1029/2004jd004827, 2004.
Watson-Parris, D., Schutgens, N., Cook, N., Kipling, Z., Kershaw, P., Gryspeerdt, E., Lawrence, B., and Stier, P.: Community Intercomparison Suite (CIS) v1.4.0: a tool for intercomparing models and observations, Geosci. Model Dev., 9, 3093–3110, https://doi.org/10.5194/gmd-9-3093-2016, 2016.
Wilcox, E. M.: Direct and semi-direct radiative forcing of smoke aerosols over clouds, Atmos. Chem. Phys., 12, 139–149, https://doi.org/10.5194/acp-12-139-2012, 2012.
Xia, X., Wang, P., Wang, Y., Li, Z., Xin, J., Liu, J., and Chen, H.: Aerosol optical depth over the Tibetan Plateau and its relation to aerosols over the Taklimakan Desert, Geophys. Res. Lett., 35, L16804, https://doi.org/10.1029/2008gl034981, 2008.
Xia, X., Min, J., Shen, F., Wang, Y., and Yang, C.: Aerosol Data Assimilation Using Data from Fengyun-3A and MODIS: Application to a Dust Storm over East Asia in 2011, Adv. Atmos. Sci., 36, 1–14, https://doi.org/10.1007/s00376-018-8075-9, 2019.
Xia, X., Min, J., Shen, F., Wang, Y., Xu, D., Yang, C., and Zhang, P.: Aerosol data assimilation using data from Fengyun-4A, a next-generation geostationary meteorological satellite, Atmos. Environ., 237, 117695, https://doi.org/10.1016/j.atmosenv.2020.117695, 2020.
Xu, B., Cao, J., Hansen, J., Yao, T., Joswia, D. R., Wang, N., Wu, G., Wang, M., Zhao, H., Yang, W., Liu, X., and He, J.: Black soot and the survival of Tibetan glaciers, P. Natl. Acad. Sci. USA, 106, 22114–22118, https://doi.org/10.1073/pnas.0910444106, 2009.
Xu, C., Ma, Y. M., Panday, A., Cong, Z. Y., Yang, K., Zhu, Z. K., Wang, J. M., Amatya, P. M., and Zhao, L.: Similarities and differences of aerosol optical properties between southern and northern sides of the Himalayas, Atmos. Chem. Phys., 14, 3133–3149, https://doi.org/10.5194/acp-14-3133-2014, 2014.
Yang, J., Kang, S., Ji, Z., and Chen, D.: Modeling the Origin of Anthropogenic Black Carbon and Its Climatic Effect Over the Tibetan Plateau and Surrounding Regions, J. Geophys. Res.-Atmos., 123, 671–692, https://doi.org/10.1002/2017jd027282, 2018.
Yang, K., He, J., Tang, W., Qin, J., and Cheng, C. C. K.: On downward shortwave and longwave radiations over high altitude regions: Observation and modeling in the Tibetan Plateau, Agr. Forest Meteorol., 150, 38–46, https://doi.org/10.1016/j.agrformet.2009.08.004, 2010.
Yao, T., Thompson, L., Yang, W., Yu, W., Gao, Y., Guo, X., Yang, X., Duan, K., Zhao, H., Xu, B., Pu, J., Lu, A., Xiang, Y., Kattel, D. B., and Joswiak, D.: Different glacier status with atmospheric circulations in Tibetan Plateau and surroundings, Nat. Clim. Change, 2, 663–667, https://doi.org/10.1038/nclimate1580, 2012.
Yao, T., Wu, F., Ding, L., Sun, J., Zhu, L., Piao, S., Deng, T., Ni, X., Zheng, H., and Ouyang, H.: Multispherical interactions and their effects on the Tibetan Plateau's earth system: a review of the recent researches, Nat. Sci. Rev., 2, 468–488, https://doi.org/10.1093/nsr/nwv070, 2015.
Yin, X., Dai, T., Schutgens, N. A. J., Goto, D., Nakajima, T., and Shi, G.: Effects of data assimilation on the global aerosol key optical properties simulations, Atmos. Res., 178, 175–186, https://doi.org/10.1016/j.atmosres.2016.03.016, 2016.
Yoshida, M., Kikuchi, M., Nagao, T. M., Murakami, H., Nomaki, T., and Higurashi, A.: Common Retrieval of Aerosol Properties for Imaging Satellite Sensors, J. Meteorol. Soc. Jpn., 96B, 193–209, https://doi.org/10.2151/jmsj.2018-039, 2018.
You, C., Xu, C., Xu, B., Zhao, H., and Song, L.: Levoglucosan evidence for biomass burning records over Tibetan glaciers, Environ. Pollut., 216, 173–181, https://doi.org/10.1016/j.envpol.2016.05.074, 2016.
Yu, H. B., Dickinson, R. E., Chin, M., Kaufman, Y. J., Holben, B. N., Geogdzhayev, I. V., and Mishchenko, M. I.: Annual cycle of global distributions of aerosol optical depth from integration of MODIS retrievals and GOCART model simulations, J. Geophys. Res.-Atmos., 108, 4128, https://doi.org/10.1029/2002jd002717, 2003.
Yumimoto, K. and Takemura, T.: Direct radiative effect of aerosols estimated using ensemble-based data assimilation in a global aerosol climate model, Geophy. Res. Lett., 38, L21802, https://doi.org/10.1029/2011gl049258, 2011.
Yumimoto, K., Nagao, T. M., Kikuchi, M., Sekiyama, T. T., Murakami, H., Tanaka, T. Y., Ogi, A., Irie, H., Khatri, P., Okumura, H., Arai, K., Morino, I., Uchino, O., and Maki, T.: Aerosol data assimilation using data from Himawari-8, a next-generation geostationary meteorological satellite, Geophys. Res. Lett., 43, 5886–5894, https://doi.org/10.1002/2016gl069298, 2016.
Zaveri, R. A. and Peters, L. K.: A new lumped structure photochemical mechanism for large-scale applications, J. Geophys. Res.-Atmos., 104, 30387–30415, https://doi.org/10.1029/1999jd900876, 1999.
Zaveri, R. A., Easter, R. C., Fast, J. D., and Peters, L. K.: Model for Simulating Aerosol Interactions and Chemistry (MOSAIC), J. Geophys. Res.-Atmos., 113, D13204, https://doi.org/10.1029/2007jd008782, 2008.
Zhang, J. and Reid, J. S.: MODIS aerosol product analysis for data assimilation: Assessment of over-ocean level 2 aerosol optical thickness retrievals, J. Geophys. Res.-Atmos., 111, D22207, https://doi.org/10.1029/2005jd006898, 2006.
Zhang, J., Reid, J. S., Westphal, D. L., Baker, N. L., and Hyer, E. J.: A system for operational aerosol optical depth data assimilation over global oceans, J. Geophys. Res.-Atmos., 113, D10208, https://doi.org/10.1029/2007jd009065, 2008.
Zhang, J., Campbell, J. R., Reid, J. S., Westphal, D. L., Baker, N. L., Campbell, W. F., and Hyer, E. J.: Evaluating the impact of assimilating CALIOP-derived aerosol extinction profiles on a global mass transport model, Geophys. Res. Lett., 38, L14801, https://doi.org/10.1029/2011gl047737, 2011.
Zhang, J., Xia, X., Shi, H., Zong, X., and Li, J.: Radiation and aerosol measurements over the Tibetan Plateau during the Asian summer monsoon period, Atmos. Pollut. Res., 11, 1543–1551, https://doi.org/10.1016/j.apr.2020.06.017, 2020.
Zhang, M., Zhao, C., Cong, Z., Du, Q., Xu, M., Chen, Y., Chen, M., Li, R., Fu, Y., Zhong, L., Kang, S., Zhao, D., and Yang, Y.: Impact of topography on black carbon transport to the southern Tibetan Plateau during the pre-monsoon season and its climatic implication, Atmos. Chem. Phys., 20, 5923–5943, https://doi.org/10.5194/acp-20-5923-2020, 2020.
Zhang, X., Liang, S., Wild, M., and Jiang, B.: Analysis of surface incident shortwave radiation from four satellite products, Remote Sens. Environ., 165, 186–202, https://doi.org/10.1016/j.rse.2015.05.015, 2015.
Zhao, M., Dai, T., Wang, H., Bao, Q., Liu, Y., and Shi, G.: Modelling study on the source contribution to aerosol over the Tibetan Plateau, Int. J. Climatol., 41, 3247–3265, https://doi.org/10.1002/joc.7017, 2021.
Zheng, J., Hu, M., Du, Z. F., Shang, D. J., Gong, Z. H., Qin, Y. H., Fang, J. Y., Gu, F. T., Li, M. R., Peng, J. F., Li, J., Zhang, Y. Q., Huang, X. F., He, L. Y., Wu, Y. S., and Guo, S.: Influence of biomass burning from South Asia at a high-altitude mountain receptor site in China, Atmos. Chem. Phys., 17, 6853–6864, https://doi.org/10.5194/acp-17-6853-2017, 2017.
Short summary
During a springtime pollution input from South Asia to the Tibetan Plateau, we combined atmospheric chemistry modeling and data assimilation methods to assimilate and forecast aerosols from South Asia and the Tibetan Plateau. Assimilation of observations over a whole time window leads to a more reasonable distribution of daily variations in the aerosol forecast field. We also find that aerosol assimilation can improve the surface solar energy forecast in the Tibetan Plateau region.
During a springtime pollution input from South Asia to the Tibetan Plateau, we combined...
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