Articles | Volume 24, issue 21
https://doi.org/10.5194/acp-24-12355-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-24-12355-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
08 Nov 2024
Research article |
| 08 Nov 2024
| 08 Nov 2024
Projected future changes in extreme precipitation over China under stratospheric aerosol intervention in the UKESM1 climate model
Ou Wang
State Key Laboratory of Pollution Control and Resources Reuse, School of Environment, Nanjing University, Nanjing, 210023, China
Department of Agricultural Meteorology, College of Resources and Environmental Sciences, China Agriculture University, Beijing 100193, China
Yuchen Gu
Department of Earth Science, Mathematical and Physical Sciences, University College London, London WC1E 6BT, UK
Jim M. Haywood
Department of Mathematics, Faculty of Environment, Science and the Economy, University of Exeter, Exeter EX4 4QE, UK
Met Office Hadley Centre, Exeter EX1 3PB, UK
Ying Chen
School of Geography Earth and Environment Sciences, University of Birmingham, Birmingham B15 2TT, UK
Chenwei Fang
Key Laboratory of Meteorological Disaster, Ministry of Education (KLME), Joint International Research Laboratory of Climate and Environment Change (ILCEC), Collaborative Innovation Centre on Forecast and Evaluation of Meteorological Disasters, Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, Nanjing University of Information Science & Technology, Nanjing, 210044, China
State Key Laboratory of Pollution Control and Resources Reuse, School of Environment, Nanjing University, Nanjing, 210023, China
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Atmos. Chem. Phys., 24, 13253–13268, https://doi.org/10.5194/acp-24-13253-2024, https://doi.org/10.5194/acp-24-13253-2024, 2024
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Stratospheric aerosol injection (SAI) refers to a climate intervention by which aerosols are intentionally added to the high atmosphere to increase the amount of reflected sunlight and reduce Earth's temperature. The climate outcomes of SAI depend on the latitude of injection. While injecting aerosols at the Equator has undesirable side effects, injecting away from the Equator has different effects on temperature, rainfall, ozone, and atmospheric circulation, which are analysed in this work.
Philip J. Rasch, Haruki Hirasawa, Mingxuan Wu, Sarah J. Doherty, Robert Wood, Hailong Wang, Andy Jones, James Haywood, and Hansi Singh
Geosci. Model Dev., 17, 7963–7994, https://doi.org/10.5194/gmd-17-7963-2024, https://doi.org/10.5194/gmd-17-7963-2024, 2024
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Atmos. Chem. Phys., 24, 9533–9553, https://doi.org/10.5194/acp-24-9533-2024, https://doi.org/10.5194/acp-24-9533-2024, 2024
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Daniele Visioni, Alan Robock, Jim Haywood, Matthew Henry, Simone Tilmes, Douglas G. MacMartin, Ben Kravitz, Sarah J. Doherty, John Moore, Chris Lennard, Shingo Watanabe, Helene Muri, Ulrike Niemeier, Olivier Boucher, Abu Syed, Temitope S. Egbebiyi, Roland Séférian, and Ilaria Quaglia
Geosci. Model Dev., 17, 2583–2596, https://doi.org/10.5194/gmd-17-2583-2024, https://doi.org/10.5194/gmd-17-2583-2024, 2024
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George Jordan, Florent Malavelle, Ying Chen, Amy Peace, Eliza Duncan, Daniel G. Partridge, Paul Kim, Duncan Watson-Parris, Toshihiko Takemura, David Neubauer, Gunnar Myhre, Ragnhild Skeie, Anton Laakso, and James Haywood
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Jim M. Haywood, Andy Jones, Anthony C. Jones, Paul Halloran, and Philip J. Rasch
Atmos. Chem. Phys., 23, 15305–15324, https://doi.org/10.5194/acp-23-15305-2023, https://doi.org/10.5194/acp-23-15305-2023, 2023
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The difficulties in ameliorating global warming and the associated climate change via conventional mitigation are well documented, with all climate model scenarios exceeding 1.5 °C above the preindustrial level in the near future. There is therefore a growing interest in geoengineering to reflect a greater proportion of sunlight back to space and offset some of the global warming. We use a state-of-the-art Earth-system model to investigate two of the most prominent geoengineering strategies.
Calvin Howes, Pablo E. Saide, Hugh Coe, Amie Dobracki, Steffen Freitag, Jim M. Haywood, Steven G. Howell, Siddhant Gupta, Janek Uin, Mary Kacarab, Chongai Kuang, L. Ruby Leung, Athanasios Nenes, Greg M. McFarquhar, James Podolske, Jens Redemann, Arthur J. Sedlacek, Kenneth L. Thornhill, Jenny P. S. Wong, Robert Wood, Huihui Wu, Yang Zhang, Jianhao Zhang, and Paquita Zuidema
Atmos. Chem. Phys., 23, 13911–13940, https://doi.org/10.5194/acp-23-13911-2023, https://doi.org/10.5194/acp-23-13911-2023, 2023
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To better understand smoke properties and its interactions with clouds, we compare the WRF-CAM5 model with observations from ORACLES, CLARIFY, and LASIC field campaigns in the southeastern Atlantic in August 2017. The model transports and mixes smoke well but does not fully capture some important processes. These include smoke chemical and physical aging over 4–12 days, smoke removal by rain, sulfate particle formation, aerosol activation into cloud droplets, and boundary layer turbulence.
Matthew Henry, Jim Haywood, Andy Jones, Mohit Dalvi, Alice Wells, Daniele Visioni, Ewa M. Bednarz, Douglas G. MacMartin, Walker Lee, and Mari R. Tye
Atmos. Chem. Phys., 23, 13369–13385, https://doi.org/10.5194/acp-23-13369-2023, https://doi.org/10.5194/acp-23-13369-2023, 2023
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Solar climate interventions, such as injecting sulfur in the stratosphere, may be used to offset some of the adverse impacts of global warming. We use two independently developed Earth system models to assess the uncertainties around stratospheric sulfur injections. The injection locations and amounts are optimized to maintain the same pattern of surface temperature. While both models show reduced warming, the change in rainfall patterns (even without sulfur injections) is uncertain.
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Atmos. Chem. Phys., 23, 8341–8368, https://doi.org/10.5194/acp-23-8341-2023, https://doi.org/10.5194/acp-23-8341-2023, 2023
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Ernesto Reyes-Villegas, Douglas Lowe, Jill S. Johnson, Kenneth S. Carslaw, Eoghan Darbyshire, Michael Flynn, James D. Allan, Hugh Coe, Ying Chen, Oliver Wild, Scott Archer-Nicholls, Alex Archibald, Siddhartha Singh, Manish Shrivastava, Rahul A. Zaveri, Vikas Singh, Gufran Beig, Ranjeet Sokhi, and Gordon McFiggans
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Ju Liang and Jim Haywood
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The recent record-breaking flood events in China during the summer of 2021 highlight the importance of mitigating the risks from future changes in high-impact weather systems under global warming. Based on a state-of-the-art Earth system model, we demonstrate a pilot study on the responses of atmospheric rivers and extreme precipitation over East Asia to anthropogenically induced climate warming and an unconventional mitigation strategy – stratospheric aerosol injection.
Daniele Visioni, Ewa M. Bednarz, Walker R. Lee, Ben Kravitz, Andy Jones, Jim M. Haywood, and Douglas G. MacMartin
Atmos. Chem. Phys., 23, 663–685, https://doi.org/10.5194/acp-23-663-2023, https://doi.org/10.5194/acp-23-663-2023, 2023
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The paper constitutes Part 1 of a study performing a first systematic inter-model comparison of the atmospheric responses to stratospheric sulfate aerosol injections (SAIs) at various latitudes as simulated by three state-of-the-art Earth system models. We identify similarities and differences in the modeled aerosol burden, investigate the differences in the aerosol approaches between the models, and ultimately show the differences produced in surface climate, temperature and precipitation.
Ewa M. Bednarz, Daniele Visioni, Ben Kravitz, Andy Jones, James M. Haywood, Jadwiga Richter, Douglas G. MacMartin, and Peter Braesicke
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Building on Part 1 of this two-part study, we demonstrate the role of biases in climatological circulation and specific aspects of model microphysics in driving the differences in simulated sulfate distributions amongst three Earth system models. We then characterize the simulated changes in stratospheric and free-tropospheric temperatures, ozone, water vapor, and large-scale circulation, elucidating the role of the above aspects in the surface responses discussed in Part 1.
Paul A. Barrett, Steven J. Abel, Hugh Coe, Ian Crawford, Amie Dobracki, James Haywood, Steve Howell, Anthony Jones, Justin Langridge, Greg M. McFarquhar, Graeme J. Nott, Hannah Price, Jens Redemann, Yohei Shinozuka, Kate Szpek, Jonathan W. Taylor, Robert Wood, Huihui Wu, Paquita Zuidema, Stéphane Bauguitte, Ryan Bennett, Keith Bower, Hong Chen, Sabrina Cochrane, Michael Cotterell, Nicholas Davies, David Delene, Connor Flynn, Andrew Freedman, Steffen Freitag, Siddhant Gupta, David Noone, Timothy B. Onasch, James Podolske, Michael R. Poellot, Sebastian Schmidt, Stephen Springston, Arthur J. Sedlacek III, Jamie Trembath, Alan Vance, Maria A. Zawadowicz, and Jianhao Zhang
Atmos. Meas. Tech., 15, 6329–6371, https://doi.org/10.5194/amt-15-6329-2022, https://doi.org/10.5194/amt-15-6329-2022, 2022
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To better understand weather and climate, it is vital to go into the field and collect observations. Often measurements take place in isolation, but here we compared data from two aircraft and one ground-based site. This was done in order to understand how well measurements made on one platform compared to those made on another. Whilst this is easy to do in a controlled laboratory setting, it is more challenging in the real world, and so these comparisons are as valuable as they are rare.
Flossie Brown, Gerd A. Folberth, Stephen Sitch, Susanne Bauer, Marijn Bauters, Pascal Boeckx, Alexander W. Cheesman, Makoto Deushi, Inês Dos Santos Vieira, Corinne Galy-Lacaux, James Haywood, James Keeble, Lina M. Mercado, Fiona M. O'Connor, Naga Oshima, Kostas Tsigaridis, and Hans Verbeeck
Atmos. Chem. Phys., 22, 12331–12352, https://doi.org/10.5194/acp-22-12331-2022, https://doi.org/10.5194/acp-22-12331-2022, 2022
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Surface ozone can decrease plant productivity and impair human health. In this study, we evaluate the change in surface ozone due to climate change over South America and Africa using Earth system models. We find that if the climate were to change according to the worst-case scenario used here, models predict that forested areas in biomass burning locations and urban populations will be at increasing risk of ozone exposure, but other areas will experience a climate benefit.
Jim M. Haywood, Andy Jones, Ben T. Johnson, and William McFarlane Smith
Atmos. Chem. Phys., 22, 6135–6150, https://doi.org/10.5194/acp-22-6135-2022, https://doi.org/10.5194/acp-22-6135-2022, 2022
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Simulations are presented investigating the influence of moderately absorbing aerosol in the stratosphere to combat the impacts of climate change. A number of detrimental impacts are noted compared to sulfate aerosol, including (i) reduced cooling efficiency, (ii) increased deficits in global precipitation, (iii) delays in the recovery of the stratospheric ozone hole, and (iv) disruption of the stratospheric circulation and the wintertime storm tracks that impact European precipitation.
Simone Tilmes, Daniele Visioni, Andy Jones, James Haywood, Roland Séférian, Pierre Nabat, Olivier Boucher, Ewa Monica Bednarz, and Ulrike Niemeier
Atmos. Chem. Phys., 22, 4557–4579, https://doi.org/10.5194/acp-22-4557-2022, https://doi.org/10.5194/acp-22-4557-2022, 2022
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This study assesses the impacts of climate interventions, using stratospheric sulfate aerosol and solar dimming on stratospheric ozone, based on three Earth system models with interactive stratospheric chemistry. The climate interventions have been applied to a high emission (baseline) scenario in order to reach global surface temperatures of a medium emission scenario. We find significant increases and decreases in total column ozone, depending on regions and seasons.
Yu Wang, Aristeidis Voliotis, Dawei Hu, Yunqi Shao, Mao Du, Ying Chen, Judith Kleinheins, Claudia Marcolli, M. Rami Alfarra, and Gordon McFiggans
Atmos. Chem. Phys., 22, 4149–4166, https://doi.org/10.5194/acp-22-4149-2022, https://doi.org/10.5194/acp-22-4149-2022, 2022
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Aerosol water uptake plays a key role in atmospheric physicochemical processes. We designed chamber experiments on aerosol water uptake of secondary organic aerosol (SOA) from mixed biogenic and anthropogenic precursors with inorganic seed. Our results highlight this chemical composition influences the reconciliation of the sub- and super-saturated water uptake, providing laboratory evidence for understanding the chemical controls of water uptake of the multi-component aerosol.
Andy Jones, Jim M. Haywood, Adam A. Scaife, Olivier Boucher, Matthew Henry, Ben Kravitz, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Roland Séférian, Simone Tilmes, and Daniele Visioni
Atmos. Chem. Phys., 22, 2999–3016, https://doi.org/10.5194/acp-22-2999-2022, https://doi.org/10.5194/acp-22-2999-2022, 2022
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Simulations by six Earth-system models of geoengineering by introducing sulfuric acid aerosols into the tropical stratosphere are compared. A robust impact on the northern wintertime North Atlantic Oscillation is found, exacerbating precipitation reduction over parts of southern Europe. In contrast, the models show no consistency with regard to impacts on the Quasi-Biennial Oscillation, although results do indicate a risk that the oscillation could become locked into a permanent westerly phase.
Zixia Liu, Martin Osborne, Karen Anderson, Jamie D. Shutler, Andy Wilson, Justin Langridge, Steve H. L. Yim, Hugh Coe, Suresh Babu, Sreedharan K. Satheesh, Paquita Zuidema, Tao Huang, Jack C. H. Cheng, and James Haywood
Atmos. Meas. Tech., 14, 6101–6118, https://doi.org/10.5194/amt-14-6101-2021, https://doi.org/10.5194/amt-14-6101-2021, 2021
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This paper first validates the performance of an advanced aerosol observation instrument POPS against a reference instrument and examines any biases introduced by operating it on a quadcopter drone. The results show the POPS performs relatively well on the ground. The impact of the UAV rotors on the POPS is small at low wind speeds, but when operating under higher wind speeds, larger discrepancies occur. It appears that the POPS measures sub-micron aerosol particles more accurately on the UAV.
Chao Qin, Yafeng Gou, Yuhang Wang, Yuhao Mao, Hong Liao, Qin'geng Wang, and Mingjie Xie
Atmos. Chem. Phys., 21, 12141–12153, https://doi.org/10.5194/acp-21-12141-2021, https://doi.org/10.5194/acp-21-12141-2021, 2021
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In this study, we found that the aqueous solution in aerosols is an important absorbing phase for gaseous polyols in the atmosphere, indicating that the dissolution in aerosol liquid water should not be ignored when investigating gas–particle partitioning of water-soluble organics. The exponential increase in effective partitioning coefficients of polyol tracers with sulfate ion concentrations could be attributed to organic–inorganic interactions in the particle phase.
Yu Wang, Aristeidis Voliotis, Yunqi Shao, Taomou Zong, Xiangxinyue Meng, Mao Du, Dawei Hu, Ying Chen, Zhijun Wu, M. Rami Alfarra, and Gordon McFiggans
Atmos. Chem. Phys., 21, 11303–11316, https://doi.org/10.5194/acp-21-11303-2021, https://doi.org/10.5194/acp-21-11303-2021, 2021
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Aerosol phase behaviour plays a profound role in atmospheric physicochemical processes. We designed dedicated chamber experiments to study the phase state of secondary organic aerosol from biogenic and anthropogenic mixed precursors. Our results highlight the key role of the organic–inorganic ratio and relative humidity in phase state, but the sources and organic composition are less important. The result provides solid laboratory evidence for understanding aerosol phase in a complex atmosphere.
Tabish Umar Ansari, Oliver Wild, Edmund Ryan, Ying Chen, Jie Li, and Zifa Wang
Atmos. Chem. Phys., 21, 4471–4485, https://doi.org/10.5194/acp-21-4471-2021, https://doi.org/10.5194/acp-21-4471-2021, 2021
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We use novel modelling approaches to quantify the lingering effects of 1 d local and regional emission controls on subsequent days, the effects of longer continuous emission controls of individual sectors over different regions, and the effects of combined emission controls of multiple sectors and regions on air quality in Beijing under varying weather conditions to inform precise short-term emission control policies for avoiding heavy haze pollution in Beijing.
Ben Kravitz, Douglas G. MacMartin, Daniele Visioni, Olivier Boucher, Jason N. S. Cole, Jim Haywood, Andy Jones, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Alan Robock, Roland Séférian, and Simone Tilmes
Atmos. Chem. Phys., 21, 4231–4247, https://doi.org/10.5194/acp-21-4231-2021, https://doi.org/10.5194/acp-21-4231-2021, 2021
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This study investigates multi-model response to idealized geoengineering (high CO2 with solar reduction) across two different generations of climate models. We find that, with the exception of a few cases, the results are unchanged between the different generations. This gives us confidence that broad conclusions about the response to idealized geoengineering are robust.
Fanny Peers, Peter Francis, Steven J. Abel, Paul A. Barrett, Keith N. Bower, Michael I. Cotterell, Ian Crawford, Nicholas W. Davies, Cathryn Fox, Stuart Fox, Justin M. Langridge, Kerry G. Meyer, Steven E. Platnick, Kate Szpek, and Jim M. Haywood
Atmos. Chem. Phys., 21, 3235–3254, https://doi.org/10.5194/acp-21-3235-2021, https://doi.org/10.5194/acp-21-3235-2021, 2021
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Satellite observations at high temporal resolution are a valuable asset to monitor the transport of biomass burning plumes and the cloud diurnal cycle in the South Atlantic, but they need to be validated. Cloud and above-cloud aerosol properties retrieved from SEVIRI are compared against MODIS and measurements from the CLARIFY-2017 campaign. While some systematic differences are observed between SEVIRI and MODIS, the overall agreement in the cloud and aerosol properties is very satisfactory.
Jim M. Haywood, Steven J. Abel, Paul A. Barrett, Nicolas Bellouin, Alan Blyth, Keith N. Bower, Melissa Brooks, Ken Carslaw, Haochi Che, Hugh Coe, Michael I. Cotterell, Ian Crawford, Zhiqiang Cui, Nicholas Davies, Beth Dingley, Paul Field, Paola Formenti, Hamish Gordon, Martin de Graaf, Ross Herbert, Ben Johnson, Anthony C. Jones, Justin M. Langridge, Florent Malavelle, Daniel G. Partridge, Fanny Peers, Jens Redemann, Philip Stier, Kate Szpek, Jonathan W. Taylor, Duncan Watson-Parris, Robert Wood, Huihui Wu, and Paquita Zuidema
Atmos. Chem. Phys., 21, 1049–1084, https://doi.org/10.5194/acp-21-1049-2021, https://doi.org/10.5194/acp-21-1049-2021, 2021
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Every year, the seasonal cycle of biomass burning from agricultural practices in Africa creates a huge plume of smoke that travels many thousands of kilometres over the Atlantic Ocean. This study provides an overview of a measurement campaign called the cloud–aerosol–radiation interaction and forcing for year 2017 (CLARIFY-2017) and documents the rationale, deployment strategy, observations, and key results from the campaign which utilized the heavily equipped FAAM atmospheric research aircraft.
Mingjie Xie, Zhenzhen Zhao, Amara L. Holder, Michael D. Hays, Xi Chen, Guofeng Shen, James J. Jetter, Wyatt M. Champion, and Qin'geng Wang
Atmos. Chem. Phys., 20, 14077–14090, https://doi.org/10.5194/acp-20-14077-2020, https://doi.org/10.5194/acp-20-14077-2020, 2020
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This study investigated the composition, structures, and light absorption of N-containing aromatic compounds (NACs) in PM2.5 emitted from burning red oak and charcoal in a variety of cookstoves. The results suggest that the identified NACs might have substantial fractions remaining in the gas phase. In comparison to other sources, cookstove emissions from red oak or charcoal fuels did not exhibit unique NAC structural features but had distinct NAC composition.
Han Han, Yue Wu, Jane Liu, Tianliang Zhao, Bingliang Zhuang, Honglei Wang, Yichen Li, Huimin Chen, Ye Zhu, Hongnian Liu, Qin'geng Wang, Shu Li, Tijian Wang, Min Xie, and Mengmeng Li
Atmos. Chem. Phys., 20, 13591–13610, https://doi.org/10.5194/acp-20-13591-2020, https://doi.org/10.5194/acp-20-13591-2020, 2020
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Combining simulations from a global chemical transport model and a trajectory model, we find that black carbon aerosols from South Asia and East Asia contribute 77 % of the surface black carbon in the Tibetan Plateau. The Asian monsoon largely modulates inter-annual transport of black carbon from non-local regions to the Tibetan Plateau surface in most seasons, while inter-annual fire activities in South Asia influence black carbon concentration over the Tibetan Plateau surface mainly in spring.
Jonathan W. Taylor, Huihui Wu, Kate Szpek, Keith Bower, Ian Crawford, Michael J. Flynn, Paul I. Williams, James Dorsey, Justin M. Langridge, Michael I. Cotterell, Cathryn Fox, Nicholas W. Davies, Jim M. Haywood, and Hugh Coe
Atmos. Chem. Phys., 20, 11201–11221, https://doi.org/10.5194/acp-20-11201-2020, https://doi.org/10.5194/acp-20-11201-2020, 2020
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Every year, huge plumes of smoke hundreds of miles wide travel over the south Atlantic Ocean from fires in central and southern Africa. These plumes absorb the sun’s energy and warm the climate. We used airborne optical instrumentation to determine how absorbing the smoke was as well as the relative importance of black and brown carbon. We also tested different ways of simulating these properties that could be used in a climate model.
Gunnar Myhre, Bjørn H. Samset, Christian W. Mohr, Kari Alterskjær, Yves Balkanski, Nicolas Bellouin, Mian Chin, James Haywood, Øivind Hodnebrog, Stefan Kinne, Guangxing Lin, Marianne T. Lund, Joyce E. Penner, Michael Schulz, Nick Schutgens, Ragnhild B. Skeie, Philip Stier, Toshihiko Takemura, and Kai Zhang
Atmos. Chem. Phys., 20, 8855–8865, https://doi.org/10.5194/acp-20-8855-2020, https://doi.org/10.5194/acp-20-8855-2020, 2020
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The radiative forcing of the direct aerosol effects can be decomposed into clear-sky and cloudy-sky portions. In this study we use observational methods and two sets of multi-model global aerosol simulations over the industrial era to show that the contribution from cloudy-sky regions is likely weak.
William T. Morgan, James D. Allan, Stéphane Bauguitte, Eoghan Darbyshire, Michael J. Flynn, James Lee, Dantong Liu, Ben Johnson, Jim Haywood, Karla M. Longo, Paulo E. Artaxo, and Hugh Coe
Atmos. Chem. Phys., 20, 5309–5326, https://doi.org/10.5194/acp-20-5309-2020, https://doi.org/10.5194/acp-20-5309-2020, 2020
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We flew a large atmospheric research aircraft across a number of different environments in the Amazon basin during the 2012 biomass burning season. Smoke from fires builds up and has a significant impact on weather, climate, health and natural ecosystems. Our goal was to quantify changes in the properties of the smoke emitted by fires as it is transported through the atmosphere. We found that the major control on the properties of the smoke was due to differences in the fires themselves.
Yu Wang, Ying Chen, Zhijun Wu, Dongjie Shang, Yuxuan Bian, Zhuofei Du, Sebastian H. Schmitt, Rong Su, Georgios I. Gkatzelis, Patrick Schlag, Thorsten Hohaus, Aristeidis Voliotis, Keding Lu, Limin Zeng, Chunsheng Zhao, M. Rami Alfarra, Gordon McFiggans, Alfred Wiedensohler, Astrid Kiendler-Scharr, Yuanhang Zhang, and Min Hu
Atmos. Chem. Phys., 20, 2161–2175, https://doi.org/10.5194/acp-20-2161-2020, https://doi.org/10.5194/acp-20-2161-2020, 2020
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Severe haze events, with high particulate nitrate (pNO3−) burden, frequently prevail in Beijing. In this study, we demonstrate a mutual-promotion effect between aerosol water uptake and pNO3− formation backed up by theoretical calculations and field observations throughout a typical pNO3−-dominated haze event in Beijing wintertime. This self-amplified mutual-promotion effect between aerosol water content and particulate nitrate can rapidly deteriorate air quality and degrade visibility.
Ying Chen, Yafang Cheng, Nan Ma, Chao Wei, Liang Ran, Ralf Wolke, Johannes Größ, Qiaoqiao Wang, Andrea Pozzer, Hugo A. C. Denier van der Gon, Gerald Spindler, Jos Lelieveld, Ina Tegen, Hang Su, and Alfred Wiedensohler
Atmos. Chem. Phys., 20, 771–786, https://doi.org/10.5194/acp-20-771-2020, https://doi.org/10.5194/acp-20-771-2020, 2020
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Particulate nitrate is one of the most important climate cooling agents. Our results show that interaction with sea-salt aerosol can shift nitrate to larger sized particles (redistribution effect), weakening its direct cooling effect. The modelling results indicate strong redistribution over coastal and offshore regions worldwide as well as continental Europe. Improving the consideration of the redistribution effect in global models fosters a better understanding of climate change.
Ying Chen, Oliver Wild, Edmund Ryan, Saroj Kumar Sahu, Douglas Lowe, Scott Archer-Nicholls, Yu Wang, Gordon McFiggans, Tabish Ansari, Vikas Singh, Ranjeet S. Sokhi, Alex Archibald, and Gufran Beig
Atmos. Chem. Phys., 20, 499–514, https://doi.org/10.5194/acp-20-499-2020, https://doi.org/10.5194/acp-20-499-2020, 2020
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PM2.5 and O3 are two major air pollutants. Some mitigation strategies focusing on reducing PM2.5 may lead to substantial increase in O3. We use statistical emulation combined with atmospheric transport model to perform thousands of sensitivity numerical studies to identify the major sources of PM2.5 and O3 and to develop strategies targeted at both pollutants. Our scientific evidence suggests that regional coordinated emission control is required to mitigate PM2.5 whilst preventing O3 increase.
James Brooks, Dantong Liu, James D. Allan, Paul I. Williams, Jim Haywood, Ellie J. Highwood, Sobhan K. Kompalli, S. Suresh Babu, Sreedharan K. Satheesh, Andrew G. Turner, and Hugh Coe
Atmos. Chem. Phys., 19, 13079–13096, https://doi.org/10.5194/acp-19-13079-2019, https://doi.org/10.5194/acp-19-13079-2019, 2019
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Our study presents an analysis of the vertical and horizontal black carbon properties across northern India using aircraft measurements. The Indo-Gangetic Plain saw the greatest black carbon mass concentrations during the pre-monsoon season. Two black carbon modes were recorded: a small black carbon mode (traffic emissions) in the north-west and a moderately coated mode (solid-fuel emissions) in the Indo-Gangetic Plain. In the vertical profile, absorption properties increase with height.
Fanny Peers, Peter Francis, Cathryn Fox, Steven J. Abel, Kate Szpek, Michael I. Cotterell, Nicholas W. Davies, Justin M. Langridge, Kerry G. Meyer, Steven E. Platnick, and Jim M. Haywood
Atmos. Chem. Phys., 19, 9595–9611, https://doi.org/10.5194/acp-19-9595-2019, https://doi.org/10.5194/acp-19-9595-2019, 2019
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The measurements from the geostationary satellite MSG/SEVIRI are used to retrieve the cloud and above-cloud aerosol properties over the South Atlantic. The technique relies on the spectral contrast and the magnitude of the signal in the visible to shortwave infrared region as well as the atmospheric correction based on forecasted water vapour profiles. The sensitivity analysis and the stability of the retrieval over time show great potential of the high-temporal-resolution observations.
Nicholas W. Davies, Cathryn Fox, Kate Szpek, Michael I. Cotterell, Jonathan W. Taylor, James D. Allan, Paul I. Williams, Jamie Trembath, Jim M. Haywood, and Justin M. Langridge
Atmos. Meas. Tech., 12, 3417–3434, https://doi.org/10.5194/amt-12-3417-2019, https://doi.org/10.5194/amt-12-3417-2019, 2019
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This research project assesses biases in traditional, filter-based, aerosol absorption measurements by comparison to state-of-the-art, non-filter-based, or in situ, measurements. We assess biases in traditional absorption measurements for three main aerosol types, including dust and fresh and aged biomass burning aerosols. The main results of this study are that the traditional and state-of-the-art absorption measurements are well correlated and that biases in the former are up to 45 %.
James Brooks, James D. Allan, Paul I. Williams, Dantong Liu, Cathryn Fox, Jim Haywood, Justin M. Langridge, Ellie J. Highwood, Sobhan K. Kompalli, Debbie O'Sullivan, Suresh S. Babu, Sreedharan K. Satheesh, Andrew G. Turner, and Hugh Coe
Atmos. Chem. Phys., 19, 5615–5634, https://doi.org/10.5194/acp-19-5615-2019, https://doi.org/10.5194/acp-19-5615-2019, 2019
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Our study, for the first time, presents measurements of aerosol chemical composition and physical characteristics across northern India in the pre-monsoon and monsoon seasons of 2016 using the FAAM BAe-146 UK research aircraft. Across northern India, an elevated aerosol layer dominated by sulfate aerosol exists that diminishes with monsoon arrival. The Indo-Gangetic Plain (IGP) boundary layer is dominated by organics, whereas outside the IGP sulfate dominates with increased scattering aerosol.
Michael I. Cotterell, Andrew J. Orr-Ewing, Kate Szpek, Jim M. Haywood, and Justin M. Langridge
Atmos. Meas. Tech., 12, 2371–2385, https://doi.org/10.5194/amt-12-2371-2019, https://doi.org/10.5194/amt-12-2371-2019, 2019
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Photoacoustic spectroscopy provides measurements of absorption coefficient for aerosol and gas samples but requires careful calibration, and researchers often use concentrations of ozone. Recent work has shown that the bath gas composition impacts the accuracy of this calibration at visible wavelengths. We explore further the role of bath gas, demonstrating that the calibration accuracy is optimal for a bath gas composed of 20 % oxygen and 80 % nitrogen at wavelengths of 405, 514 and 658 nm.
Yanhong Zhu, Lingxiao Yang, Jianmin Chen, Kimitaka Kawamura, Mamiko Sato, Andreas Tilgner, Dominik van Pinxteren, Ying Chen, Likun Xue, Xinfeng Wang, Isobel J. Simpson, Hartmut Herrmann, Donald R. Blake, and Wenxing Wang
Atmos. Chem. Phys., 18, 10741–10758, https://doi.org/10.5194/acp-18-10741-2018, https://doi.org/10.5194/acp-18-10741-2018, 2018
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Molecular distributions of dicarboxylic acids, oxocarboxylic acids and α-dicarbonyls in the free troposphere are identified, and their concentration variations between 2014 and 2006 are presented. High nighttime concentrations were probably due to precursor emissions and aqueous-phase oxidation. Biomass burning was significant, but its tracer levoglucosan in 2014 was 5 times lower than 2006 concentrations. Finally, regional emission from anthropogenic activities was identified as a major source.
Xiaohui Zhang, Yan Lu, Qin'geng Wang, and Xin Qian
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-1113, https://doi.org/10.5194/acp-2017-1113, 2018
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Activity data at prefectural-city level combined with high-resolution land use data were adopted to improve spatial resolution and detailed crop rotations and harvest times in different regions were considered in determining temporal distribution. Also, MODIS fire products were applied to verify the spatial and temporal variations of the emissions. Results showed that high emissions were generally located in Eastern, Central and Northeastern China, and temporally peaking in June and October.
Ying Chen, Ralf Wolke, Liang Ran, Wolfram Birmili, Gerald Spindler, Wolfram Schröder, Hang Su, Yafang Cheng, Ina Tegen, and Alfred Wiedensohler
Atmos. Chem. Phys., 18, 673–689, https://doi.org/10.5194/acp-18-673-2018, https://doi.org/10.5194/acp-18-673-2018, 2018
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The heterogeneous hydrolysis of N2O5 on particle surfaces is crucial for the nitrogen cycle in the atmosphere. The reaction rate is determined by meteorological and particle properties, but its parameterization in previous 3-D modelling studies did not comprehensively consider these parameters. We propose a parameterization to take these into account and improve nitrate prediction; we report that the organic coating suppression on the N2O5 reaction is not as important as expected in the EU.
Qing Mu, Gerhard Lammel, Christian N. Gencarelli, Ian M. Hedgecock, Ying Chen, Petra Přibylová, Monique Teich, Yuxuan Zhang, Guangjie Zheng, Dominik van Pinxteren, Qiang Zhang, Hartmut Herrmann, Manabu Shiraiwa, Peter Spichtinger, Hang Su, Ulrich Pöschl, and Yafang Cheng
Atmos. Chem. Phys., 17, 12253–12267, https://doi.org/10.5194/acp-17-12253-2017, https://doi.org/10.5194/acp-17-12253-2017, 2017
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Polycyclic aromatic hydrocarbons (PAHs) are hazardous pollutants with the largest emissions in East Asia. The regional WRF-Chem-PAH model has been developed to reflect the state-of-the-art understanding of current PAHs studies with several new or updated features. It is able to reasonably well simulate the concentration levels and particulate mass fractions of PAHs near the sources and at a remote outflow region of East Asia, in high spatial and temporal resolutions.
Ying Chen, Yafang Cheng, Nan Ma, Ralf Wolke, Stephan Nordmann, Stephanie Schüttauf, Liang Ran, Birgit Wehner, Wolfram Birmili, Hugo A. C. Denier van der Gon, Qing Mu, Stefan Barthel, Gerald Spindler, Bastian Stieger, Konrad Müller, Guang-Jie Zheng, Ulrich Pöschl, Hang Su, and Alfred Wiedensohler
Atmos. Chem. Phys., 16, 12081–12097, https://doi.org/10.5194/acp-16-12081-2016, https://doi.org/10.5194/acp-16-12081-2016, 2016
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Sea salt aerosol (SSA) is important for primary and secondary aerosols on a global scale. During 10–20 September 2013, the SSA mass concentration was overestimated by a factor of 8–20 over central Europe by WRF-Chem model, stem from the uncertainty of its emission scheme. This could facilitate the coarse-mode nitrate formation (~ 140 % but inhibit the fine-mode nitrate formation (~−20 %). A special long-range transport mechanism could broaden this influence of SSA to a larger downwind region.
Anthony C. Jones, James M. Haywood, and Andy Jones
Atmos. Chem. Phys., 16, 2843–2862, https://doi.org/10.5194/acp-16-2843-2016, https://doi.org/10.5194/acp-16-2843-2016, 2016
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In this paper we assess the potential climatic impacts of geoengineering with sulfate, black carbon and titania injection strategies. We find that black carbon injection results in severe stratospheric warming and precipitation impacts, and therefore black carbon is unsuitable for geoengineering purposes. As the injection rates and climatic impacts for titania are close to those for sulfate, there appears little benefit of using titania when compared to injection of sulfur dioxide.
Ying Chen, Ya-Fang Cheng, Stephan Nordmann, Wolfram Birmili, Hugo A. C. Denier van der Gon, Nan Ma, Ralf Wolke, Birgit Wehner, Jia Sun, Gerald Spindler, Qing Mu, Ulrich Pöschl, Hang Su, and Alfred Wiedensohler
Atmos. Chem. Phys., 16, 1823–1835, https://doi.org/10.5194/acp-16-1823-2016, https://doi.org/10.5194/acp-16-1823-2016, 2016
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We evaluated the EC point sources in Germany with high-resolution simulation by WRF-Chem, and find out that point sources contribute too much EC in the coarse mode aerosol mass. The area emissions in Eastern Europe and Russia also allocate too much EC emission in coarse mode in the EUCAARI EC emission inventory. Because of the shorter life time of coarse mode EC, about 20–40 % less EC can be transported to Melpitz from Eastern Europe. Size segregation information is important for EC inventories.
F. Pacifico, G. A. Folberth, S. Sitch, J. M. Haywood, L. V. Rizzo, F. F. Malavelle, and P. Artaxo
Atmos. Chem. Phys., 15, 2791–2804, https://doi.org/10.5194/acp-15-2791-2015, https://doi.org/10.5194/acp-15-2791-2015, 2015
Related subject area
Subject: Clouds and Precipitation | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Stratosphere | Science Focus: Physics (physical properties and processes)
Impact of mountain-wave-induced temperature fluctuations on the occurrence of polar stratospheric ice clouds: a statistical analysis based on MIPAS observations and ERA5 data
Impact of host climate model on contrail cirrus effective radiative forcing estimates
Investigating long-term changes in polar stratospheric clouds above Antarctica during past decades: a temperature-based approach using spaceborne lidar detections
A simple model to assess the impact of gravity waves on ice-crystal populations in the tropical tropopause layer
Simulation of convective moistening of the extratropical lower stratosphere using a numerical weather prediction model
Convective hydration in the tropical tropopause layer during the StratoClim aircraft campaign: pathway of an observed hydration patch
Lagrangian simulation of ice particles and resulting dehydration in the polar winter stratosphere
Effects of convective ice evaporation on interannual variability of tropical tropopause layer water vapor
Technical note: A noniterative approach to modelling moist thermodynamics
Denitrification by large NAT particles: the impact of reduced settling velocities and hints on particle characteristics
Arctic stratospheric dehydration – Part 2: Microphysical modeling
Heterogeneous formation of polar stratospheric clouds – Part 2: Nucleation of ice on synoptic scales
Heterogeneous formation of polar stratospheric clouds – Part 1: Nucleation of nitric acid trihydrate (NAT)
Cirrus and water vapor transport in the tropical tropopause layer – Part 1: A specific case modeling study
Ling Zou, Reinhold Spang, Sabine Griessbach, Lars Hoffmann, Farahnaz Khosrawi, Rolf Müller, and Ines Tritscher
Atmos. Chem. Phys., 24, 11759–11774, https://doi.org/10.5194/acp-24-11759-2024, https://doi.org/10.5194/acp-24-11759-2024, 2024
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This study provided estimates of the occurrence of ice polar stratospheric clouds (PSCs) observed by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) and their connection with temperatures above the frost point (Tice) using a Lagrangian model derived from ERA5. We found that ice PSCs above Tice with temperature fluctuations along the backward trajectory are 33 % in the Arctic and 9 % in the Antarctic. This quantitative assessment enhances our understanding of ice PSCs.
Weiyu Zhang, Kwinten Van Weverberg, Cyril J. Morcrette, Wuhu Feng, Kalli Furtado, Paul R. Field, Chih-Chieh Chen, Andrew Gettelman, Piers M. Forster, Daniel R. Marsh, and Alexandru Rap
EGUsphere, https://doi.org/10.5194/egusphere-2024-1573, https://doi.org/10.5194/egusphere-2024-1573, 2024
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Contrail cirrus is the largest, but also most uncertain contribution of aviation to global warming. We evaluate for the first time the impact of the host climate model on contrail cirrus properties. Substantial differences exist between contrail cirrus formation, persistence, and radiative effects in the host climate models. Reliable contrail cirrus simulations require advanced representation of cloud optical properties and microphysics, which should be better constrained by observations.
Mathilde Leroux and Vincent Noel
Atmos. Chem. Phys., 24, 6433–6454, https://doi.org/10.5194/acp-24-6433-2024, https://doi.org/10.5194/acp-24-6433-2024, 2024
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This study investigates the long-term changes in the polar stratospheric cloud (PSC) season from 1980 to 2021 above Antarctica. We analyzed CALIOP observations from 2006 to 2020 to build a statistical temperature-based model. We applied our model to gridded reanalysis temperatures, leading to an integrated view of PSC occurrence that is free from sampling issues, allowing us to document the past evolution of the PSC season.
Milena Corcos, Albert Hertzog, Riwal Plougonven, and Aurélien Podglajen
Atmos. Chem. Phys., 23, 6923–6939, https://doi.org/10.5194/acp-23-6923-2023, https://doi.org/10.5194/acp-23-6923-2023, 2023
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The role of gravity waves on tropical cirrus clouds and air-parcel dehydration was studied using the combination of Lagrangian observations of temperature fluctuations from superpressure balloons and a 1.5D model. The inclusion of the gravity waves to a reference simulation of a slow ascent around the cold-point tropopause drastically increases ice-crystal density, cloud fraction, and air-parcel dehydration, and it produces a crystal size distribution that agrees better with observations.
Zhipeng Qu, Yi Huang, Paul A. Vaillancourt, Jason N. S. Cole, Jason A. Milbrandt, Man-Kong Yau, Kaley Walker, and Jean de Grandpré
Atmos. Chem. Phys., 20, 2143–2159, https://doi.org/10.5194/acp-20-2143-2020, https://doi.org/10.5194/acp-20-2143-2020, 2020
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This study aims to better understand the mechanism of transport of water vapour through the mid-latitude tropopause. The results affirm the strong influence of overshooting convection on lower-stratospheric water vapour and highlight the importance of both dynamics and cloud microphysics in simulating water vapour distribution in the region of the upper troposphere–lower stratosphere.
Keun-Ok Lee, Thibaut Dauhut, Jean-Pierre Chaboureau, Sergey Khaykin, Martina Krämer, and Christian Rolf
Atmos. Chem. Phys., 19, 11803–11820, https://doi.org/10.5194/acp-19-11803-2019, https://doi.org/10.5194/acp-19-11803-2019, 2019
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This study focuses on the hydration patch that was measured during the StratoClim field campaign and the corresponding convective overshoots over the Sichuan Basin. Through analysis using airborne and spaceborne measurements and the numerical simulation using a non-hydrostatic model, we show the key hydration process and pathway of the hydration patch in tropical tropopause layer.
Ines Tritscher, Jens-Uwe Grooß, Reinhold Spang, Michael C. Pitts, Lamont R. Poole, Rolf Müller, and Martin Riese
Atmos. Chem. Phys., 19, 543–563, https://doi.org/10.5194/acp-19-543-2019, https://doi.org/10.5194/acp-19-543-2019, 2019
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We present Lagrangian simulations of polar stratospheric clouds (PSCs) for the Arctic winter 2009/2010 and the Antarctic winter 2011 using the Chemical Lagrangian Model of the Stratosphere (CLaMS). The paper comprises a detailed model description with ice PSCs and related dehydration being the focus of this study. Comparisons between our simulations and observations from different satellites on season-long and vortex-wide scales as well as for single PSC events show an overall good agreement.
Hao Ye, Andrew E. Dessler, and Wandi Yu
Atmos. Chem. Phys., 18, 4425–4437, https://doi.org/10.5194/acp-18-4425-2018, https://doi.org/10.5194/acp-18-4425-2018, 2018
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The deep convection in tropics can inject cloud ice into tropical tropopause layer (TTL), which moistens and increases water vapor there. We primarily study the spatial distribution of impacts from several physical processes on TTL water vapor from observations and trajectory model simulations. The analysis shows the potential moistening impact from evaporation of cloud ice on TTL water vapor. A chemistry–climate model is used to confirm the impact from evaporation of convective ice.
Nadya Moisseeva and Roland Stull
Atmos. Chem. Phys., 17, 15037–15043, https://doi.org/10.5194/acp-17-15037-2017, https://doi.org/10.5194/acp-17-15037-2017, 2017
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This technical note presents simple noniterative approximations for two common thermodynamic relationships used for moist convection. The method offers roughly 2 orders of magnitude improvement in accuracy over the only existing noniterative solution. The proposed approach alleviates the need for costly numerical integration of saturated thermodynamic equations within numerical weather prediction models and in theoretical studies.
W. Woiwode, J.-U. Grooß, H. Oelhaf, S. Molleker, S. Borrmann, A. Ebersoldt, W. Frey, T. Gulde, S. Khaykin, G. Maucher, C. Piesch, and J. Orphal
Atmos. Chem. Phys., 14, 11525–11544, https://doi.org/10.5194/acp-14-11525-2014, https://doi.org/10.5194/acp-14-11525-2014, 2014
I. Engel, B. P. Luo, S. M. Khaykin, F. G. Wienhold, H. Vömel, R. Kivi, C. R. Hoyle, J.-U. Grooß, M. C. Pitts, and T. Peter
Atmos. Chem. Phys., 14, 3231–3246, https://doi.org/10.5194/acp-14-3231-2014, https://doi.org/10.5194/acp-14-3231-2014, 2014
I. Engel, B. P. Luo, M. C. Pitts, L. R. Poole, C. R. Hoyle, J.-U. Grooß, A. Dörnbrack, and T. Peter
Atmos. Chem. Phys., 13, 10769–10785, https://doi.org/10.5194/acp-13-10769-2013, https://doi.org/10.5194/acp-13-10769-2013, 2013
C. R. Hoyle, I. Engel, B. P. Luo, M. C. Pitts, L. R. Poole, J.-U. Grooß, and T. Peter
Atmos. Chem. Phys., 13, 9577–9595, https://doi.org/10.5194/acp-13-9577-2013, https://doi.org/10.5194/acp-13-9577-2013, 2013
T. Dinh, D. R. Durran, and T. Ackerman
Atmos. Chem. Phys., 12, 9799–9815, https://doi.org/10.5194/acp-12-9799-2012, https://doi.org/10.5194/acp-12-9799-2012, 2012
Cited articles
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Short summary
As extreme precipitation events increase in China, this study explores the potential of stratospheric aerosol injection (SAI) to mitigate these effects by the end of the 21st century using the UKESM1 model. Results show that SAI reduces extreme precipitation in eastern China. However, caution is advised due to potential side effects in high-latitude regions, and further optimization is required for future SAI deployment.
As extreme precipitation events increase in China, this study explores the potential of...
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