Articles | Volume 23, issue 17
https://doi.org/10.5194/acp-23-10057-2023
https://doi.org/10.5194/acp-23-10057-2023
Research article
 | 
08 Sep 2023
Research article |  | 08 Sep 2023

Deposition freezing, pore condensation freezing and adsorption: three processes, one description?

Mária Lbadaoui-Darvas, Ari Laaksonen, and Athanasios Nenes

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Cited articles

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Barahona, D.: Thermodynamic derivation of the activation energy for ice nucleation, Atmos. Chem. Phys., 15, 13819–13831, https://doi.org/10.5194/acp-15-13819-2015, 2015. a
Bentsen, M., Bethke, I., Debernard, J. B., Iversen, T., Kirkevåg, A., Seland, Ø., Drange, H., Roelandt, C., Seierstad, I. A., Hoose, C., and Kristjánsson, J. E.: The Norwegian Earth System Model, NorESM1-M – Part 1: Description and basic evaluation of the physical climate, Geosci. Model Dev., 6, 687–720, https://doi.org/10.5194/gmd-6-687-2013, 2013. a
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Short summary
Heterogeneous ice nucleation is the main ice formation mechanism in clouds. The mechanism of different freezing modes is to date unknown, which results in large model biases. Experiments do not allow for direct observation of ice nucleation at its native resolution. This work uses first principles molecular simulations to determine the mechanism of the least-understood ice nucleation mode and link it to adsorption through a novel modeling framework that unites ice and droplet formation.
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