Deposition freezing, pore condensation freezing and adsorption: three processes, one description?
Mária Lbadaoui-Darvas,Ari Laaksonen,and Athanasios Nenes
Mária Lbadaoui-Darvas
Laboratory of Atmospheric Processes and their Impacts, School of Architecture, Civil and Environmental Engineering, École Polytechnique Federale de Lausanne, 1015 Lausanne, Switzerland
Laboratory of Atmospheric Processes and their Impacts, School of Architecture, Civil and Environmental Engineering, École Polytechnique Federale de Lausanne, 1015 Lausanne, Switzerland
Center for the Study of Air Quality and Climate Change, Institute of Chemical Engineering Sciences, Foundation for Research and Technology Hellas, 26504 Patras, Greece
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Heterogeneous ice nucleation is the main ice formation mechanism in clouds. The mechanism of different freezing modes is to date unknown, which results in large model biases. Experiments do not allow for direct observation of ice nucleation at its native resolution. This work uses first principles molecular simulations to determine the mechanism of the least-understood ice nucleation mode and link it to adsorption through a novel modeling framework that unites ice and droplet formation.
Heterogeneous ice nucleation is the main ice formation mechanism in clouds. The mechanism of...
