Articles | Volume 22, issue 9
https://doi.org/10.5194/acp-22-6347-2022
https://doi.org/10.5194/acp-22-6347-2022
Research article
 | 
17 May 2022
Research article |  | 17 May 2022

Using atmospheric trace gas vertical profiles to evaluate model fluxes: a case study of Arctic-CAP observations and GEOS simulations for the ABoVE domain

Colm Sweeney, Abhishek Chatterjee, Sonja Wolter, Kathryn McKain, Robert Bogue, Stephen Conley, Tim Newberger, Lei Hu, Lesley Ott, Benjamin Poulter, Luke Schiferl, Brad Weir, Zhen Zhang, and Charles E. Miller

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Cited articles

Allen, M., Erickson, D., Kendall, W., Fu, J., Ott, L., and Pawson, S.: The influence of internal model variability in GEOS-5 on interhemispheric CO2 exchange, J. Geophys. Res.-Atmos., 117, D10107, https://doi.org/10.1029/2011jd017059, 2012. 
Baier, B. C., Sweeney, C., Choi, Y., Davis, K. J., DiGangi, J. P., Feng, S., Fried, A., Halliday, H., Higgs, J., Lauvaux, T., Miller, B. R., Montzka, S. A., Newberger, T., Nowak, J. B., Patra, P., Richter, D., Walega, J., and Weibring, P.: Multispecies Assessment of Factors Influencing Regional CO2 and CH4 Enhancements During the Winter 2017 ACT-America Campaign, J. Geophys. Res.-Atmos., 125, e2019JD031339, https://doi.org/10.1029/2019jd031339, 2020. 
Baldocchi, D. D., Krebs, T., and Leclerc, M. Y.: “Wet/dry Daisyworld”: a conceptual tool for quantifying the spatial scaling of heterogeneous landscapes and its impact on the subgrid variability of energy fluxes, Tellus B, 57, 175–188, https://doi.org/10.1111/j.1600-0889.2005.00149.x, 2005. 
Bosilovich, M. G., Chern, J.-D., Mocko, D., Robertson, F. R., and da Silva, A. M.: Evaluating Observation Influence on Regional Water Budgets in Reanalyses, J. Climate, 28, 3631–3649, https://doi.org/10.1175/jcli-d-14-00623.1, 2015. 
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Short summary
The Arctic Carbon Atmospheric Profiles (Arctic-CAP) project demonstrates the utility of aircraft profiles for independent evaluation of model-derived emissions and uptake of atmospheric CO2, CH4, and CO from land and ocean. Comparison with the Goddard Earth Observing System (GEOS) modeling system suggests that fluxes of CO2 are very consistent with observations, while those of CH4 have some regional and seasonal biases, and that CO comparison is complicated by transport errors.
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