Articles | Volume 22, issue 4
https://doi.org/10.5194/acp-22-2365-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-2365-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Microphysical processes producing high ice water contents (HIWCs) in tropical convective clouds during the HAIC-HIWC field campaign: dominant role of secondary ice production
Yongjie Huang
CORRESPONDING AUTHOR
Center for Analysis and Prediction of Storms, University of Oklahoma, Norman, OK, USA
Cooperative Institute for Severe and High-Impact Weather Research and Operations, University of Oklahoma, Norman, OK, USA
Cooperative Institute for Severe and High-Impact Weather Research and Operations, University of Oklahoma, Norman, OK, USA
School of Meteorology, University of Oklahoma, Norman, OK, USA
Ming Xue
Center for Analysis and Prediction of Storms, University of Oklahoma, Norman, OK, USA
School of Meteorology, University of Oklahoma, Norman, OK, USA
Hugh Morrison
Mesoscale and Microscale Meteorology Laboratory, National Center for Atmospheric Research, Boulder, CO, USA
Jason Milbrandt
Environment and Climate Change Canada, Dorval, Quebec, Canada
Alexei V. Korolev
Environment and Climate Change Canada, Toronto, ON, Canada
Yachao Hu
Cooperative Institute for Severe and High-Impact Weather Research and Operations, University of Oklahoma, Norman, OK, USA
Department of Atmospheric and Oceanic Sciences, School of Physics, Peking University, Beijing, China
Zhipeng Qu
Environment and Climate Change Canada, Toronto, ON, Canada
Mengistu Wolde
National Research Council Canada, Ottawa, Canada
Cuong Nguyen
National Research Council Canada, Ottawa, Canada
Alfons Schwarzenboeck
Université Clermont Auvergne, CNRS, UMR 6016, Laboratoire de Météor Physique, Clermont-Ferrand, France
Ivan Heckman
Environment and Climate Change Canada, Toronto, ON, Canada
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Sergey Y. Matrosov, Alexei Korolev, Mengistu Wolde, and Cuong Nguyen
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Paul A. Barrett, Steven J. Abel, Hugh Coe, Ian Crawford, Amie Dobracki, James Haywood, Steve Howell, Anthony Jones, Justin Langridge, Greg M. McFarquhar, Graeme J. Nott, Hannah Price, Jens Redemann, Yohei Shinozuka, Kate Szpek, Jonathan W. Taylor, Robert Wood, Huihui Wu, Paquita Zuidema, Stéphane Bauguitte, Ryan Bennett, Keith Bower, Hong Chen, Sabrina Cochrane, Michael Cotterell, Nicholas Davies, David Delene, Connor Flynn, Andrew Freedman, Steffen Freitag, Siddhant Gupta, David Noone, Timothy B. Onasch, James Podolske, Michael R. Poellot, Sebastian Schmidt, Stephen Springston, Arthur J. Sedlacek III, Jamie Trembath, Alan Vance, Maria A. Zawadowicz, and Jianhao Zhang
Atmos. Meas. Tech., 15, 6329–6371, https://doi.org/10.5194/amt-15-6329-2022, https://doi.org/10.5194/amt-15-6329-2022, 2022
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To better understand weather and climate, it is vital to go into the field and collect observations. Often measurements take place in isolation, but here we compared data from two aircraft and one ground-based site. This was done in order to understand how well measurements made on one platform compared to those made on another. Whilst this is easy to do in a controlled laboratory setting, it is more challenging in the real world, and so these comparisons are as valuable as they are rare.
Alexei Korolev, Paul J. DeMott, Ivan Heckman, Mengistu Wolde, Earle Williams, David J. Smalley, and Michael F. Donovan
Atmos. Chem. Phys., 22, 13103–13113, https://doi.org/10.5194/acp-22-13103-2022, https://doi.org/10.5194/acp-22-13103-2022, 2022
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The present study provides the first explicit in situ observation of secondary ice production at temperatures as low as −27 °C, which is well outside the range of the Hallett–Mossop process (−3 to −8 °C). This observation expands our knowledge of the temperature range of initiation of secondary ice in clouds. The obtained results are intended to stimulate laboratory and theoretical studies to develop physically based parameterizations for weather prediction and climate models.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, Michael R. Poellot, David J. Delene, Ian Chang, Lan Gao, Feng Xu, and Jens Redemann
Atmos. Chem. Phys., 22, 12923–12943, https://doi.org/10.5194/acp-22-12923-2022, https://doi.org/10.5194/acp-22-12923-2022, 2022
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Katherine L. Hayden, Shao-Meng Li, John Liggio, Michael J. Wheeler, Jeremy J. B. Wentzell, Amy Leithead, Peter Brickell, Richard L. Mittermeier, Zachary Oldham, Cristian M. Mihele, Ralf M. Staebler, Samar G. Moussa, Andrea Darlington, Mengistu Wolde, Daniel Thompson, Jack Chen, Debora Griffin, Ellen Eckert, Jenna C. Ditto, Megan He, and Drew R. Gentner
Atmos. Chem. Phys., 22, 12493–12523, https://doi.org/10.5194/acp-22-12493-2022, https://doi.org/10.5194/acp-22-12493-2022, 2022
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Zhipeng Qu, Alexei Korolev, Jason A. Milbrandt, Ivan Heckman, Yongjie Huang, Greg M. McFarquhar, Hugh Morrison, Mengistu Wolde, and Cuong Nguyen
Atmos. Chem. Phys., 22, 12287–12310, https://doi.org/10.5194/acp-22-12287-2022, https://doi.org/10.5194/acp-22-12287-2022, 2022
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Dongwei Fu, Larry Di Girolamo, Robert M. Rauber, Greg M. McFarquhar, Stephen W. Nesbitt, Jesse Loveridge, Yulan Hong, Bastiaan van Diedenhoven, Brian Cairns, Mikhail D. Alexandrov, Paul Lawson, Sarah Woods, Simone Tanelli, Sebastian Schmidt, Chris Hostetler, and Amy Jo Scarino
Atmos. Chem. Phys., 22, 8259–8285, https://doi.org/10.5194/acp-22-8259-2022, https://doi.org/10.5194/acp-22-8259-2022, 2022
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Po-Lun Ma, Bryce E. Harrop, Vincent E. Larson, Richard B. Neale, Andrew Gettelman, Hugh Morrison, Hailong Wang, Kai Zhang, Stephen A. Klein, Mark D. Zelinka, Yuying Zhang, Yun Qian, Jin-Ho Yoon, Christopher R. Jones, Meng Huang, Sheng-Lun Tai, Balwinder Singh, Peter A. Bogenschutz, Xue Zheng, Wuyin Lin, Johannes Quaas, Hélène Chepfer, Michael A. Brunke, Xubin Zeng, Johannes Mülmenstädt, Samson Hagos, Zhibo Zhang, Hua Song, Xiaohong Liu, Michael S. Pritchard, Hui Wan, Jingyu Wang, Qi Tang, Peter M. Caldwell, Jiwen Fan, Larry K. Berg, Jerome D. Fast, Mark A. Taylor, Jean-Christophe Golaz, Shaocheng Xie, Philip J. Rasch, and L. Ruby Leung
Geosci. Model Dev., 15, 2881–2916, https://doi.org/10.5194/gmd-15-2881-2022, https://doi.org/10.5194/gmd-15-2881-2022, 2022
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An alternative set of parameters for E3SM Atmospheric Model version 1 has been developed based on a tuning strategy that focuses on clouds. When clouds in every regime are improved, other aspects of the model are also improved, even though they are not the direct targets for calibration. The recalibrated model shows a lower sensitivity to anthropogenic aerosols and surface warming, suggesting potential improvements to the simulated climate in the past and future.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, Michael R. Poellot, David J. Delene, Rose M. Miller, and Jennifer D. Small Griswold
Atmos. Chem. Phys., 22, 2769–2793, https://doi.org/10.5194/acp-22-2769-2022, https://doi.org/10.5194/acp-22-2769-2022, 2022
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This study evaluates the impact of biomass burning aerosols on precipitation in marine stratocumulus clouds using observations from the NASA ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) field campaign over the Southeast Atlantic. Instances of contact and separation between aerosol and cloud layers show polluted clouds have a lower precipitation rate and a lower precipitation susceptibility. This information will help improve cloud representation in Earth system models.
Cuong M. Nguyen, Mengistu Wolde, Alessandro Battaglia, Leonid Nichman, Natalia Bliankinshtein, Samuel Haimov, Kenny Bala, and Dirk Schuettemeyer
Atmos. Meas. Tech., 15, 775–795, https://doi.org/10.5194/amt-15-775-2022, https://doi.org/10.5194/amt-15-775-2022, 2022
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An analysis of airborne triple-frequency radar and almost perfectly co-located coincident in situ data from an Arctic storm confirms the main findings of modeling work with radar dual-frequency ratios (DFRs) at different zones of the DFR plane associated with different ice habits. High-resolution CPI images provide accurate identification of rimed particles within the DFR plane. The relationships between the triple-frequency signals and cloud microphysical properties are also presented.
Matthew W. Christensen, Andrew Gettelman, Jan Cermak, Guy Dagan, Michael Diamond, Alyson Douglas, Graham Feingold, Franziska Glassmeier, Tom Goren, Daniel P. Grosvenor, Edward Gryspeerdt, Ralph Kahn, Zhanqing Li, Po-Lun Ma, Florent Malavelle, Isabel L. McCoy, Daniel T. McCoy, Greg McFarquhar, Johannes Mülmenstädt, Sandip Pal, Anna Possner, Adam Povey, Johannes Quaas, Daniel Rosenfeld, Anja Schmidt, Roland Schrödner, Armin Sorooshian, Philip Stier, Velle Toll, Duncan Watson-Parris, Robert Wood, Mingxi Yang, and Tianle Yuan
Atmos. Chem. Phys., 22, 641–674, https://doi.org/10.5194/acp-22-641-2022, https://doi.org/10.5194/acp-22-641-2022, 2022
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Trace gases and aerosols (tiny airborne particles) are released from a variety of point sources around the globe. Examples include volcanoes, industrial chimneys, forest fires, and ship stacks. These sources provide opportunistic experiments with which to quantify the role of aerosols in modifying cloud properties. We review the current state of understanding on the influence of aerosol on climate built from the wide range of natural and anthropogenic laboratories investigated in recent decades.
Kamil Mroz, Alessandro Battaglia, Cuong Nguyen, Andrew Heymsfield, Alain Protat, and Mengistu Wolde
Atmos. Meas. Tech., 14, 7243–7254, https://doi.org/10.5194/amt-14-7243-2021, https://doi.org/10.5194/amt-14-7243-2021, 2021
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A method for estimating microphysical properties of ice clouds based on radar measurements is presented. The algorithm exploits the information provided by differences in the radar response at different frequency bands in relation to changes in the snow morphology. The inversion scheme is based on a statistical relation between the radar simulations and the properties of snow calculated from in-cloud sampling.
Rose M. Miller, Greg M. McFarquhar, Robert M. Rauber, Joseph R. O'Brien, Siddhant Gupta, Michal Segal-Rozenhaimer, Amie N. Dobracki, Arthur J. Sedlacek, Sharon P. Burton, Steven G. Howell, Steffen Freitag, and Caroline Dang
Atmos. Chem. Phys., 21, 14815–14831, https://doi.org/10.5194/acp-21-14815-2021, https://doi.org/10.5194/acp-21-14815-2021, 2021
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A large stratocumulus cloud deck resides off the west coast of central Africa. Biomass burning in Africa produces a large plume of aerosol that is carried by the wind over this stratocumulus cloud deck. This paper shows that particles with sizes from 0.01 to 1 mm reside within this plume. Past studies have shown that biomass burning produces such particles, but this is the first study to show that they can be transported westward, over long distances, to the Atlantic stratocumulus cloud deck.
Wojciech W. Grabowski and Hugh Morrison
Atmos. Chem. Phys., 21, 13997–14018, https://doi.org/10.5194/acp-21-13997-2021, https://doi.org/10.5194/acp-21-13997-2021, 2021
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The paper provides a discussion of key elements of moist convective dynamics: cloud buoyancy, latent heating, precipitation, and entrainment. The motivation comes from recent discussions concerning differences in convective dynamics in polluted and pristine environments.
Haoran Li, Alexei Korolev, and Dmitri Moisseev
Atmos. Chem. Phys., 21, 13593–13608, https://doi.org/10.5194/acp-21-13593-2021, https://doi.org/10.5194/acp-21-13593-2021, 2021
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Kelvin–Helmholtz (K–H) clouds embedded in a stratiform precipitation event were uncovered via radar Doppler spectral analysis. Given the unprecedented detail of the observations, we show that multiple populations of secondary ice columns were generated in the pockets where larger cloud droplets are formed and not at some constant level within the cloud. Our results highlight that the K–H instability is favorable for liquid droplet growth and secondary ice formation.
Ruhi S. Humphries, Melita D. Keywood, Sean Gribben, Ian M. McRobert, Jason P. Ward, Paul Selleck, Sally Taylor, James Harnwell, Connor Flynn, Gourihar R. Kulkarni, Gerald G. Mace, Alain Protat, Simon P. Alexander, and Greg McFarquhar
Atmos. Chem. Phys., 21, 12757–12782, https://doi.org/10.5194/acp-21-12757-2021, https://doi.org/10.5194/acp-21-12757-2021, 2021
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The Southern Ocean region is one of the most pristine in the world and serves as an important proxy for the pre-industrial atmosphere. Improving our understanding of the natural processes in this region is likely to result in the largest reductions in the uncertainty of climate and earth system models. In this paper we present a statistical summary of the latitudinal gradient of aerosol and cloud condensation nuclei concentrations obtained from five voyages spanning the Southern Ocean.
Jing Feng, Yi Huang, and Zhipeng Qu
Atmos. Meas. Tech., 14, 5717–5734, https://doi.org/10.5194/amt-14-5717-2021, https://doi.org/10.5194/amt-14-5717-2021, 2021
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It is challenging to measure the atmospheric conditions above convective storms. In this study, a method of retrieving thermodynamic variables above convective storms using a combination of satellite-based observations from a hyperspectral infrared sounder and active sensors is developed. We find that this method captures the spatial distributions of thermodynamic anomalies above convective clouds well. This method is potentially applicable to observations from current and future satellites.
Paul A. Makar, Ayodeji Akingunola, Jack Chen, Balbir Pabla, Wanmin Gong, Craig Stroud, Christopher Sioris, Kerry Anderson, Philip Cheung, Junhua Zhang, and Jason Milbrandt
Atmos. Chem. Phys., 21, 10557–10587, https://doi.org/10.5194/acp-21-10557-2021, https://doi.org/10.5194/acp-21-10557-2021, 2021
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We have examined the effects of airborne particles on absorption and scattering of incoming sunlight by the particles themselves via cloud formation. We used an advanced, combined high-resolution weather forecast and chemical transport computer model, for western North America, and simulations with and without the connections between particles and weather enabled. Feedbacks improved weather and air pollution forecasts and changed cloud behaviour and forest-fire pollutant amount and height.
Konstantin Baibakov, Samuel LeBlanc, Keyvan Ranjbar, Norman T. O'Neill, Mengistu Wolde, Jens Redemann, Kristina Pistone, Shao-Meng Li, John Liggio, Katherine Hayden, Tak W. Chan, Michael J. Wheeler, Leonid Nichman, Connor Flynn, and Roy Johnson
Atmos. Chem. Phys., 21, 10671–10687, https://doi.org/10.5194/acp-21-10671-2021, https://doi.org/10.5194/acp-21-10671-2021, 2021
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We find that the airborne measurements of the vertical extinction due to aerosols (aerosol optical depth, AOD) obtained in the Athabasca Oil Sands Region (AOSR) can significantly exceed ground-based values. This can have an effect on estimating the AOSR radiative impact and is relevant to satellite validation based on ground-based measurements. We also show that the AOD can marginally increase as the plumes are being transported away from the source and the new particles are being formed.
Katherine Hayden, Shao-Meng Li, Paul Makar, John Liggio, Samar G. Moussa, Ayodeji Akingunola, Robert McLaren, Ralf M. Staebler, Andrea Darlington, Jason O'Brien, Junhua Zhang, Mengistu Wolde, and Leiming Zhang
Atmos. Chem. Phys., 21, 8377–8392, https://doi.org/10.5194/acp-21-8377-2021, https://doi.org/10.5194/acp-21-8377-2021, 2021
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We developed a method using aircraft measurements to determine lifetimes with respect to dry deposition for oxidized sulfur and nitrogen compounds over the boreal forest in Alberta, Canada. Atmospheric lifetimes were significantly shorter than derived from chemical transport models with differences related to modelled dry deposition velocities. The shorter lifetimes suggest models need to reassess dry deposition treatment and predictions of sulfur and nitrogen in the atmosphere and ecosystems.
Yongjie Huang, Wei Wu, Greg M. McFarquhar, Xuguang Wang, Hugh Morrison, Alexander Ryzhkov, Yachao Hu, Mengistu Wolde, Cuong Nguyen, Alfons Schwarzenboeck, Jason Milbrandt, Alexei V. Korolev, and Ivan Heckman
Atmos. Chem. Phys., 21, 6919–6944, https://doi.org/10.5194/acp-21-6919-2021, https://doi.org/10.5194/acp-21-6919-2021, 2021
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Numerous small ice crystals in the tropical convective storms are difficult to detect and could be potentially hazardous for commercial aircraft. This study evaluated the numerical models against the airborne observations and investigated the potential cloud processes that could lead to the production of these large numbers of small ice crystals. It is found that key microphysical processes are still lacking or misrepresented in current numerical models to realistically simulate the phenomenon.
Andrew M. Dzambo, Tristan L'Ecuyer, Kenneth Sinclair, Bastiaan van Diedenhoven, Siddhant Gupta, Greg McFarquhar, Joseph R. O'Brien, Brian Cairns, Andrzej P. Wasilewski, and Mikhail Alexandrov
Atmos. Chem. Phys., 21, 5513–5532, https://doi.org/10.5194/acp-21-5513-2021, https://doi.org/10.5194/acp-21-5513-2021, 2021
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This work highlights a new algorithm using data collected from the 2016–2018 NASA ORACLES field campaign. This algorithm synthesizes cloud and rain measurements to attain estimates of cloud and precipitation properties over the southeast Atlantic Ocean. Estimates produced by this algorithm compare well against in situ estimates. Increased rain fractions and rain rates are found in regions of atmospheric instability. This dataset can be used to explore aerosol–cloud–precipitation interactions.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, David J. Delene, Michael R. Poellot, Amie Dobracki, James R. Podolske, Jens Redemann, Samuel E. LeBlanc, Michal Segal-Rozenhaimer, and Kristina Pistone
Atmos. Chem. Phys., 21, 4615–4635, https://doi.org/10.5194/acp-21-4615-2021, https://doi.org/10.5194/acp-21-4615-2021, 2021
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Observations from the 2016 NASA ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) field campaign examine how biomass burning aerosols from southern Africa affect marine stratocumulus cloud decks over the Southeast Atlantic. Instances of contact and separation between aerosols and clouds are examined to quantify the impact of aerosol mixing into cloud top on cloud drop numbers and sizes. This information is needed for improving Earth system models and satellite retrievals.
Jens Redemann, Robert Wood, Paquita Zuidema, Sarah J. Doherty, Bernadette Luna, Samuel E. LeBlanc, Michael S. Diamond, Yohei Shinozuka, Ian Y. Chang, Rei Ueyama, Leonhard Pfister, Ju-Mee Ryoo, Amie N. Dobracki, Arlindo M. da Silva, Karla M. Longo, Meloë S. Kacenelenbogen, Connor J. Flynn, Kristina Pistone, Nichola M. Knox, Stuart J. Piketh, James M. Haywood, Paola Formenti, Marc Mallet, Philip Stier, Andrew S. Ackerman, Susanne E. Bauer, Ann M. Fridlind, Gregory R. Carmichael, Pablo E. Saide, Gonzalo A. Ferrada, Steven G. Howell, Steffen Freitag, Brian Cairns, Brent N. Holben, Kirk D. Knobelspiesse, Simone Tanelli, Tristan S. L'Ecuyer, Andrew M. Dzambo, Ousmane O. Sy, Greg M. McFarquhar, Michael R. Poellot, Siddhant Gupta, Joseph R. O'Brien, Athanasios Nenes, Mary Kacarab, Jenny P. S. Wong, Jennifer D. Small-Griswold, Kenneth L. Thornhill, David Noone, James R. Podolske, K. Sebastian Schmidt, Peter Pilewskie, Hong Chen, Sabrina P. Cochrane, Arthur J. Sedlacek, Timothy J. Lang, Eric Stith, Michal Segal-Rozenhaimer, Richard A. Ferrare, Sharon P. Burton, Chris A. Hostetler, David J. Diner, Felix C. Seidel, Steven E. Platnick, Jeffrey S. Myers, Kerry G. Meyer, Douglas A. Spangenberg, Hal Maring, and Lan Gao
Atmos. Chem. Phys., 21, 1507–1563, https://doi.org/10.5194/acp-21-1507-2021, https://doi.org/10.5194/acp-21-1507-2021, 2021
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Southern Africa produces significant biomass burning emissions whose impacts on regional and global climate are poorly understood. ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) is a 5-year NASA investigation designed to study the key processes that determine these climate impacts. The main purpose of this paper is to familiarize the broader scientific community with the ORACLES project, the dataset it produced, and the most important initial findings.
Georgia Sotiropoulou, Étienne Vignon, Gillian Young, Hugh Morrison, Sebastian J. O'Shea, Thomas Lachlan-Cope, Alexis Berne, and Athanasios Nenes
Atmos. Chem. Phys., 21, 755–771, https://doi.org/10.5194/acp-21-755-2021, https://doi.org/10.5194/acp-21-755-2021, 2021
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Summer clouds have a significant impact on the radiation budget of the Antarctic surface and thus on ice-shelf melting. However, these are poorly represented in climate models due to errors in their microphysical structure, including the number of ice crystals that they contain. We show that breakup from ice particle collisions can substantially magnify the ice crystal number concentration with significant implications for surface radiation. This process is currently missing in climate models.
Alexei Korolev and Thomas Leisner
Atmos. Chem. Phys., 20, 11767–11797, https://doi.org/10.5194/acp-20-11767-2020, https://doi.org/10.5194/acp-20-11767-2020, 2020
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Secondary ice production (SIP) plays a key role in the formation of ice particles in tropospheric clouds. This work presents a critical review of the laboratory studies related to secondary ice production. It aims to identify gaps in our knowledge of SIP as well as to stimulate further laboratory studies focused on obtaining a quantitative description of efficiencies for each SIP mechanism.
Cyrielle Denjean, Thierry Bourrianne, Frederic Burnet, Marc Mallet, Nicolas Maury, Aurélie Colomb, Pamela Dominutti, Joel Brito, Régis Dupuy, Karine Sellegri, Alfons Schwarzenboeck, Cyrille Flamant, and Peter Knippertz
Atmos. Chem. Phys., 20, 4735–4756, https://doi.org/10.5194/acp-20-4735-2020, https://doi.org/10.5194/acp-20-4735-2020, 2020
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This paper presents aircraft measurements of aerosol optical properties over southern West Africa. We show that aerosol optical properties in the boundary layer were dominated by a persistent biomass burning loading from the Southern Hemisphere. Biomass burning aerosols were more light absorbing that those previously measured in other areas (Amazonia, North America). Our study suggests that lens-coated black carbon particles were the dominant absorber for these biomass burning aerosols.
Zhipeng Qu, Yi Huang, Paul A. Vaillancourt, Jason N. S. Cole, Jason A. Milbrandt, Man-Kong Yau, Kaley Walker, and Jean de Grandpré
Atmos. Chem. Phys., 20, 2143–2159, https://doi.org/10.5194/acp-20-2143-2020, https://doi.org/10.5194/acp-20-2143-2020, 2020
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This study aims to better understand the mechanism of transport of water vapour through the mid-latitude tropopause. The results affirm the strong influence of overshooting convection on lower-stratospheric water vapour and highlight the importance of both dynamics and cloud microphysics in simulating water vapour distribution in the region of the upper troposphere–lower stratosphere.
Alexei Korolev, Ivan Heckman, Mengistu Wolde, Andrew S. Ackerman, Ann M. Fridlind, Luis A. Ladino, R. Paul Lawson, Jason Milbrandt, and Earle Williams
Atmos. Chem. Phys., 20, 1391–1429, https://doi.org/10.5194/acp-20-1391-2020, https://doi.org/10.5194/acp-20-1391-2020, 2020
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This study attempts identification of mechanisms of secondary ice production (SIP) based on the observation of small faceted ice crystals. It was found that in both mesoscale convective systems and frontal clouds, SIP was observed right above the melting layer and extended to the higher altitudes with colder temperatures. A principal conclusion of this work is that the freezing drop shattering mechanism is plausibly accounting for the measured ice concentrations in the observed condition.
Edward Gryspeerdt, Johannes Mülmenstädt, Andrew Gettelman, Florent F. Malavelle, Hugh Morrison, David Neubauer, Daniel G. Partridge, Philip Stier, Toshihiko Takemura, Hailong Wang, Minghuai Wang, and Kai Zhang
Atmos. Chem. Phys., 20, 613–623, https://doi.org/10.5194/acp-20-613-2020, https://doi.org/10.5194/acp-20-613-2020, 2020
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Aerosol radiative forcing is a key uncertainty in our understanding of the human forcing of the climate, with much of this uncertainty coming from aerosol impacts on clouds. Observation-based estimates of the radiative forcing are typically smaller than those from global models, but it is not clear if they are more reliable. This work shows how the forcing components in global climate models can be identified, highlighting similarities between the two methods and areas for future investigation.
Sophie L. Haslett, Jonathan W. Taylor, Mathew Evans, Eleanor Morris, Bernhard Vogel, Alima Dajuma, Joel Brito, Anneke M. Batenburg, Stephan Borrmann, Johannes Schneider, Christiane Schulz, Cyrielle Denjean, Thierry Bourrianne, Peter Knippertz, Régis Dupuy, Alfons Schwarzenböck, Daniel Sauer, Cyrille Flamant, James Dorsey, Ian Crawford, and Hugh Coe
Atmos. Chem. Phys., 19, 15217–15234, https://doi.org/10.5194/acp-19-15217-2019, https://doi.org/10.5194/acp-19-15217-2019, 2019
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Three aircraft datasets from the DACCIWA campaign in summer 2016 are used here to show there is a background mass of pollution present in the lower atmosphere in southern West Africa. We suggest that this likely comes from biomass burning in central and southern Africa, which has been carried into the region over the Atlantic Ocean. This would have a negative health impact on populations living near the coast and may alter the impact of growing city emissions on cloud formation and the monsoon.
Cuong M. Nguyen, Mengistu Wolde, and Alexei Korolev
Atmos. Meas. Tech., 12, 5897–5911, https://doi.org/10.5194/amt-12-5897-2019, https://doi.org/10.5194/amt-12-5897-2019, 2019
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This paper presents a methodology for high ice water content (HIWC) (up to 3.5 g m−3) retrieval from a dual-polarization side-looking X-band airborne radar. Zdr and Kdp are used to mitigate the effects of ice crystal shape and orientation on the variation in IWC – specific differential phase (Kdp) joint distribution. Empirical analysis shows that the proposed method improves the estimation bias by 35 % and increases the correlation by 4 % on average, compared to the method using Kdp alone.
Jonathan W. Taylor, Sophie L. Haslett, Keith Bower, Michael Flynn, Ian Crawford, James Dorsey, Tom Choularton, Paul J. Connolly, Valerian Hahn, Christiane Voigt, Daniel Sauer, Régis Dupuy, Joel Brito, Alfons Schwarzenboeck, Thierry Bourriane, Cyrielle Denjean, Phil Rosenberg, Cyrille Flamant, James D. Lee, Adam R. Vaughan, Peter G. Hill, Barbara Brooks, Valéry Catoire, Peter Knippertz, and Hugh Coe
Atmos. Chem. Phys., 19, 8503–8522, https://doi.org/10.5194/acp-19-8503-2019, https://doi.org/10.5194/acp-19-8503-2019, 2019
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Low-level clouds cover a wide area of southern West Africa (SWA) and play an important role in the region's climate, reflecting sunlight away from the surface. We performed aircraft measurements of aerosols and clouds over SWA during the 2016 summer monsoon and found pollution, and polluted clouds, across the whole region. Smoke from biomass burning in Central Africa is transported to West Africa, causing a polluted background which limits the effect of local pollution on cloud properties.
Thibault Vaillant de Guélis, Alfons Schwarzenböck, Valery Shcherbakov, Christophe Gourbeyre, Bastien Laurent, Régis Dupuy, Pierre Coutris, and Christophe Duroure
Atmos. Meas. Tech., 12, 2513–2529, https://doi.org/10.5194/amt-12-2513-2019, https://doi.org/10.5194/amt-12-2513-2019, 2019
Joseph A. Finlon, Greg M. McFarquhar, Stephen W. Nesbitt, Robert M. Rauber, Hugh Morrison, Wei Wu, and Pengfei Zhang
Atmos. Chem. Phys., 19, 3621–3643, https://doi.org/10.5194/acp-19-3621-2019, https://doi.org/10.5194/acp-19-3621-2019, 2019
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A new approach describing the relationship between ice crystal mass (m) and dimension (D) is derived, characterizing it as a set of
equally realizableparameters based on the natural variability in cloud conditions observed by aircraft over the Great Plains. Results from this approach address shortcomings of microphysical parameterization schemes and remote sensing retrievals that employ a single m–D relation for a given ice species or environment.
Sophie L. Haslett, Jonathan W. Taylor, Konrad Deetz, Bernhard Vogel, Karmen Babić, Norbert Kalthoff, Andreas Wieser, Cheikh Dione, Fabienne Lohou, Joel Brito, Régis Dupuy, Alfons Schwarzenboeck, Paul Zieger, and Hugh Coe
Atmos. Chem. Phys., 19, 1505–1520, https://doi.org/10.5194/acp-19-1505-2019, https://doi.org/10.5194/acp-19-1505-2019, 2019
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As the population in West Africa grows and air pollution increases, it is becoming ever more important to understand the effects of this pollution on the climate and on health. Aerosol particles can grow by absorbing water from the air around them. This paper shows that during the monsoon season, aerosol particles in the region are likely to grow significantly because of the high moisture in the air. This means that climate effects from increasing pollution will be enhanced.
Mengistu Wolde, Alessandro Battaglia, Cuong Nguyen, Andrew L. Pazmany, and Anthony Illingworth
Atmos. Meas. Tech., 12, 253–269, https://doi.org/10.5194/amt-12-253-2019, https://doi.org/10.5194/amt-12-253-2019, 2019
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This paper presents an implementation of polarization diversity pulse-pair processing (PDPP) on the National Research Council of Canada airborne W-band radar (NAW) system. A description of the NAW PDPP pulsing schemes and an analysis of comprehensive airborne data collected in diverse weather conditions in Canada is presented. The analysis shows a successful airborne measurement of Doppler velocity exceeding 100 m s−1 using PDPP approach, the first such measurement from a moving platform.
Junshik Um, Greg M. McFarquhar, Jeffrey L. Stith, Chang Hoon Jung, Seoung Soo Lee, Ji Yi Lee, Younghwan Shin, Yun Gon Lee, Yiseok Isaac Yang, Seong Soo Yum, Byung-Gon Kim, Joo Wan Cha, and A-Reum Ko
Atmos. Chem. Phys., 18, 16915–16930, https://doi.org/10.5194/acp-18-16915-2018, https://doi.org/10.5194/acp-18-16915-2018, 2018
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During the 2012 Deep Convective Clouds and Chemistry experiment upper anvils of two storms were sampled. The occurrence of well-defined pristine crystals was low in the anvils, while single frozen droplets and frozen droplet aggregates (FDAs) were the dominant habits. A new algorithm was developed to automatically identify the number, size, and relative position of element frozen droplets within FDAs. The morphological characteristics of FDAs were compared with those of black carbon aggregates.
Emma Järvinen, Olivier Jourdan, David Neubauer, Bin Yao, Chao Liu, Meinrat O. Andreae, Ulrike Lohmann, Manfred Wendisch, Greg M. McFarquhar, Thomas Leisner, and Martin Schnaiter
Atmos. Chem. Phys., 18, 15767–15781, https://doi.org/10.5194/acp-18-15767-2018, https://doi.org/10.5194/acp-18-15767-2018, 2018
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Using light diffraction it is possible to detect microscopic features within ice particles that have not yet been fully characterized. Here, this technique was applied in airborne measurements, where it was found that majority of atmospheric ice particles have features that significantly change the way ice particles interact with solar light. The microscopic features make ice-containing clouds more reflective than previously thought, which could have consequences for predicting our climate.
Robert Jackson, Jeffrey R. French, David C. Leon, David M. Plummer, Sonia Lasher-Trapp, Alan M. Blyth, and Alexei Korolev
Atmos. Chem. Phys., 18, 15329–15344, https://doi.org/10.5194/acp-18-15329-2018, https://doi.org/10.5194/acp-18-15329-2018, 2018
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This paper looks at microphysical observations of growing cumulus clouds in the southwest United Kingdom sampled during the COnvective Precipitation Experiment (COPE). Our results suggest that secondary ice production processes are contributing to the observed concentrations and that entrainment of particles from remnant cloud layers may have acted to aid in secondary ice production.
Cyrille Flamant, Adrien Deroubaix, Patrick Chazette, Joel Brito, Marco Gaetani, Peter Knippertz, Andreas H. Fink, Gaëlle de Coetlogon, Laurent Menut, Aurélie Colomb, Cyrielle Denjean, Rémi Meynadier, Philip Rosenberg, Regis Dupuy, Pamela Dominutti, Jonathan Duplissy, Thierry Bourrianne, Alfons Schwarzenboeck, Michel Ramonet, and Julien Totems
Atmos. Chem. Phys., 18, 12363–12389, https://doi.org/10.5194/acp-18-12363-2018, https://doi.org/10.5194/acp-18-12363-2018, 2018
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This work sheds light on the complex mechanisms by which coastal shallow circulations distribute atmospheric pollutants over the densely populated southern West African region. Pollutants of concern are anthropogenic emissions from coastal cities, as well as biomass burning aerosol and dust associated with long-range transport. The complex vertical distribution of aerosols over coastal southern West Africa is investigated using airborne observations and numerical simulations.
Aurélien Chauvigné, Olivier Jourdan, Alfons Schwarzenboeck, Christophe Gourbeyre, Jean François Gayet, Christiane Voigt, Hans Schlager, Stefan Kaufmann, Stephan Borrmann, Sergej Molleker, Andreas Minikin, Tina Jurkat, and Ulrich Schumann
Atmos. Chem. Phys., 18, 9803–9822, https://doi.org/10.5194/acp-18-9803-2018, https://doi.org/10.5194/acp-18-9803-2018, 2018
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This paper demonstrates a new form of statistical analysis of contrail to cirrus evolution. The authors show well-separated analyses of the different stages of the contrail's evolution, which allows us to study their optical, microphysical, and chemical properties. These results could be used to develop representative parameterizations of the scattering and geometrical properties of the ice crystals’ shapes and sizes, observed in the visible wavelength range.
Stephan E. Bansmer, Arne Baumert, Stephan Sattler, Inken Knop, Delphine Leroy, Alfons Schwarzenboeck, Tina Jurkat-Witschas, Christiane Voigt, Hugo Pervier, and Biagio Esposito
Atmos. Meas. Tech., 11, 3221–3249, https://doi.org/10.5194/amt-11-3221-2018, https://doi.org/10.5194/amt-11-3221-2018, 2018
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Snow, frost formation and ice cubes in our drinks are part of our daily life. But what about our technical innovations like aviation, electrical power transmission and wind-energy production, can they cope with icing? Icing Wind Tunnels are an ideal laboratory environment to answer that question. In this paper, we show how the icing wind tunnel in Braunschweig (Germany) was built and how we can use it for engineering and climate research.
Sabour Baray, Andrea Darlington, Mark Gordon, Katherine L. Hayden, Amy Leithead, Shao-Meng Li, Peter S. K. Liu, Richard L. Mittermeier, Samar G. Moussa, Jason O'Brien, Ralph Staebler, Mengistu Wolde, Doug Worthy, and Robert McLaren
Atmos. Chem. Phys., 18, 7361–7378, https://doi.org/10.5194/acp-18-7361-2018, https://doi.org/10.5194/acp-18-7361-2018, 2018
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Methane emissions from major oil sands facilities in the Athabasca Oil Sands Region (AOSR) of Alberta were measured in the summer of 2013 using two related aircraft mass-balance approaches. Tailings ponds and fugitive emissions of methane from open pit mines were found to be the major sources of methane in the region. Total methane emissions in the AOSR were measured to be ~ 20 tonnes of CH4 per hour, which is 48 % higher than the Canadian Greenhouse Gas Reporting Program Emissions Inventory.
Joel Brito, Evelyn Freney, Pamela Dominutti, Agnes Borbon, Sophie L. Haslett, Anneke M. Batenburg, Aurelie Colomb, Regis Dupuy, Cyrielle Denjean, Frederic Burnet, Thierry Bourriane, Adrien Deroubaix, Karine Sellegri, Stephan Borrmann, Hugh Coe, Cyrille Flamant, Peter Knippertz, and Alfons Schwarzenboeck
Atmos. Chem. Phys., 18, 757–772, https://doi.org/10.5194/acp-18-757-2018, https://doi.org/10.5194/acp-18-757-2018, 2018
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This work focuses on sources of submicron aerosol particles over southern West Africa (SWA). Results have shown that isoprene, a gas-phase compound of biogenic origin, is responsible for roughly 25 % of the organic aerosol (OA) loading, under most background or urban plumes alike. This fraction represents a lower estimate from the biogenic contribution in this fairly polluted region. This work sheds light upon the role of anthropogenic and biogenic emissions on the pollution burden over SWA.
Maximilian Maahn, Gijs de Boer, Jessie M. Creamean, Graham Feingold, Greg M. McFarquhar, Wei Wu, and Fan Mei
Atmos. Chem. Phys., 17, 14709–14726, https://doi.org/10.5194/acp-17-14709-2017, https://doi.org/10.5194/acp-17-14709-2017, 2017
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Liquid-containing clouds are a key component of the Arctic climate system and their radiative properties depend strongly on cloud drop sizes. Here, we investigate how cloud drop sizes are modified in the presence of local emissions from industrial facilities at the North Slope of Alaska using aircraft in situ observations. We show that near local anthropogenic sources, the concentrations of black carbon and condensation nuclei are enhanced and cloud drop sizes are reduced.
Gwennolé Guyot, Frans Olofson, Peter Tunved, Christophe Gourbeyre, Guy Fevbre, Régis Dupuy, Christophe Bernard, Gérard Ancellet, Kathy Law, Boris Quennehen, Alfons Schwarzenboeck, Kostas Eleftheriadis, and Olivier Jourdan
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-672, https://doi.org/10.5194/acp-2017-672, 2017
Revised manuscript has not been submitted
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Cloud and aerosol properties are key parameters in the accelerated arctic warming. In this context, this study will focus on in situ cloud microphysical and optical characterization of arctic Mixed Phase Cloud combined with aerosol measurements and air mass backtrajectory simulations during the ground based CLIMSLIP-NyA campaign performed in Ny-Alesund, Svalbard. The goal is to parameterize the arctic aerosol-cloud interaction and assess the influence of anthropogenic pollution.
Guillaume Mioche, Olivier Jourdan, Julien Delanoë, Christophe Gourbeyre, Guy Febvre, Régis Dupuy, Marie Monier, Frédéric Szczap, Alfons Schwarzenboeck, and Jean-François Gayet
Atmos. Chem. Phys., 17, 12845–12869, https://doi.org/10.5194/acp-17-12845-2017, https://doi.org/10.5194/acp-17-12845-2017, 2017
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This paper is a study about the mixed-phase clouds frequently occurring in the Arctic region. It is based on airborne measurements and highlights the microphysical properties of these particular clouds composed of liquid droplets at cloud top and ice crystals below precipitating down to the surface. This work may help to improve the representation of the mixed-phase clouds in numerical prediction models as well as the retrieval of their properties from remote sensing observations.
Bethan White, Edward Gryspeerdt, Philip Stier, Hugh Morrison, Gregory Thompson, and Zak Kipling
Atmos. Chem. Phys., 17, 12145–12175, https://doi.org/10.5194/acp-17-12145-2017, https://doi.org/10.5194/acp-17-12145-2017, 2017
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Aerosols influence cloud and precipitation by modifying cloud droplet number concentrations (CDNCs). We simulate three different types of convective cloud using two different cloud microphysics parameterisations. The simulated cloud and precipitation depends much more strongly on the choice of microphysics scheme than on CDNC. The uncertainty differs between types of convection. Our results highlight a large uncertainty in cloud and precipitation responses to aerosol in current models.
John Liggio, Samar G. Moussa, Jeremy Wentzell, Andrea Darlington, Peter Liu, Amy Leithead, Katherine Hayden, Jason O'Brien, Richard L. Mittermeier, Ralf Staebler, Mengistu Wolde, and Shao-Meng Li
Atmos. Chem. Phys., 17, 8411–8427, https://doi.org/10.5194/acp-17-8411-2017, https://doi.org/10.5194/acp-17-8411-2017, 2017
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The emission and formation of gaseous organic acids from the oil sands industry in Canada is explored through aircraft measurements directly over and downwind wind of industrial facilities. Results demonstrated that the formation of organic acids through atmospheric chemical reactions dominated over the direct emissions from mining activities but could not be explicitly modeled. The results highlight the need for improved understanding of photochemical mechanisms leading to these species.
Emmanuel Fontaine, Delphine Leroy, Alfons Schwarzenboeck, Julien Delanoë, Alain Protat, Fabien Dezitter, Alice Grandin, John Walter Strapp, and Lyle Edward Lilie
Atmos. Meas. Tech., 10, 2239–2252, https://doi.org/10.5194/amt-10-2239-2017, https://doi.org/10.5194/amt-10-2239-2017, 2017
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In this study we evaluate a method to estimate cloud water content (CWC) knowing cloud reflectivity. Ice hydrometeors are replace by ice oblate spheroids to simulate their reflectivity. There is no assumption on the relation between mass and their size. Then, a broad range of CWCs are compared with direct measurements of CWC. The accuracy of the method is ~ ±32 %. This study is performed in areas of convective clouds where reflectivity and CWC are especially high, what makes it unique.
Ann M. Fridlind, Xiaowen Li, Di Wu, Marcus van Lier-Walqui, Andrew S. Ackerman, Wei-Kuo Tao, Greg M. McFarquhar, Wei Wu, Xiquan Dong, Jingyu Wang, Alexander Ryzhkov, Pengfei Zhang, Michael R. Poellot, Andrea Neumann, and Jason M. Tomlinson
Atmos. Chem. Phys., 17, 5947–5972, https://doi.org/10.5194/acp-17-5947-2017, https://doi.org/10.5194/acp-17-5947-2017, 2017
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Understanding observed storm microphysics via computer simulation requires measurements of aerosol on which most hydrometeors form. We prepare aerosol input data for six storms observed over Oklahoma. We demonstrate their use in simulations of a case with widespread ice outflow well sampled by aircraft. Simulations predict too few ice crystals that are too large. We speculate that microphysics found in tropical storms occurred here, likely associated with poorly understood ice multiplication.
Valery Shcherbakov, Olivier Jourdan, Christiane Voigt, Jean-Francois Gayet, Aurélien Chauvigne, Alfons Schwarzenboeck, Andreas Minikin, Marcus Klingebiel, Ralf Weigel, Stephan Borrmann, Tina Jurkat, Stefan Kaufmann, Romy Schlage, Christophe Gourbeyre, Guy Febvre, Tatyana Lapyonok, Wiebke Frey, Sergej Molleker, and Bernadett Weinzierl
Atmos. Chem. Phys., 16, 11883–11897, https://doi.org/10.5194/acp-16-11883-2016, https://doi.org/10.5194/acp-16-11883-2016, 2016
W. Richard Leaitch, Alexei Korolev, Amir A. Aliabadi, Julia Burkart, Megan D. Willis, Jonathan P. D. Abbatt, Heiko Bozem, Peter Hoor, Franziska Köllner, Johannes Schneider, Andreas Herber, Christian Konrad, and Ralf Brauner
Atmos. Chem. Phys., 16, 11107–11124, https://doi.org/10.5194/acp-16-11107-2016, https://doi.org/10.5194/acp-16-11107-2016, 2016
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Thought to be mostly unimportant for summertime Arctic liquid-water clouds, airborne observations show that atmospheric aerosol particles 50 nm in diameter or smaller and most likely from natural sources are often involved in cloud formation in the pristine Arctic summer. The result expands the reference for aerosol forcing of climate. Further, for extremely low droplet concentrations, no evidence is found for a connection between cloud liquid water and aerosol particle concentrations.
Alexei Korolev, Alex Khain, Mark Pinsky, and Jeffrey French
Atmos. Chem. Phys., 16, 9235–9254, https://doi.org/10.5194/acp-16-9235-2016, https://doi.org/10.5194/acp-16-9235-2016, 2016
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Relationships between basic microphysical parameters are studied within the framework of homogeneous and extreme inhomogeneous mixing. Analytical expressions and numerical simulations of relationships between droplet concentration, extinction coefficient, liquid water content, and mean volume droplet size are presented. The obtained relationships between moments are used to identify type of mixing for in situ observations obtained in convective clouds.
Mark Pinsky, Alexander Khain, Alexei Korolev, and Leehi Magaritz-Ronen
Atmos. Chem. Phys., 16, 9255–9272, https://doi.org/10.5194/acp-16-9255-2016, https://doi.org/10.5194/acp-16-9255-2016, 2016
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The evolution of monodisperse and polydisperse droplet size distributions (DSDs) during
homogeneous mixing is analyzed. It is shown that the classic conceptual scheme, according to which homogeneous mixing leads to a decrease in the droplet mass under constant droplet concentration, is valid only in cases of initially very narrow DSDs. In cases of wide DSDs a decrease of both mass and concentration take place such that the characteristic droplet sizes remain nearly constant.
Mark Pinsky, Alexander Khain, and Alexei Korolev
Atmos. Chem. Phys., 16, 9273–9297, https://doi.org/10.5194/acp-16-9273-2016, https://doi.org/10.5194/acp-16-9273-2016, 2016
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An idealized diffusion--evaporation model of time-dependent mixing between cloud and non-cloud volumes is analyzed. It is shown that the evolution of microphysical variables and the final equilibrium stage are unambiguously determined by two non-dimensional parameters. Delimitation between the types of mixing on the plane of these parameters is carried out. The definitions of homogeneous and inhomogeneous mixings are reconsidered and clarified. Results are compared with the classical concept.
Ann M. Fridlind, Rachel Atlas, Bastiaan van Diedenhoven, Junshik Um, Greg M. McFarquhar, Andrew S. Ackerman, Elisabeth J. Moyer, and R. Paul Lawson
Atmos. Chem. Phys., 16, 7251–7283, https://doi.org/10.5194/acp-16-7251-2016, https://doi.org/10.5194/acp-16-7251-2016, 2016
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Images of crystals within mid-latitude cirrus clouds are used to derive consistent ice physical and optical properties for a detailed cloud microphysics model, including size-dependent mass, projected area, and fall speed. Based on habits found, properties are derived for bullet rosettes, their aggregates, and crystals with irregular shapes. Derived bullet rosette fall speeds are substantially greater than reported in past studies, owing to differences in mass, area, or diameter representation.
Shipeng Zhang, Minghuai Wang, Steven J. Ghan, Aijun Ding, Hailong Wang, Kai Zhang, David Neubauer, Ulrike Lohmann, Sylvaine Ferrachat, Toshihiko Takeamura, Andrew Gettelman, Hugh Morrison, Yunha Lee, Drew T. Shindell, Daniel G. Partridge, Philip Stier, Zak Kipling, and Congbin Fu
Atmos. Chem. Phys., 16, 2765–2783, https://doi.org/10.5194/acp-16-2765-2016, https://doi.org/10.5194/acp-16-2765-2016, 2016
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The variation of aerosol indirect effects (AIE) in several climate models is investigated across different dynamical regimes. Regimes with strong large-scale ascent are shown to be as important as stratocumulus regimes in studying AIE. AIE over regions with high monthly large-scale surface precipitation rate contributes the most to the total aerosol indirect forcing. These results point to the need to reduce the uncertainty in AIE in different dynamical regimes.
C. Denjean, F. Cassola, A. Mazzino, S. Triquet, S. Chevaillier, N. Grand, T. Bourrianne, G. Momboisse, K. Sellegri, A. Schwarzenbock, E. Freney, M. Mallet, and P. Formenti
Atmos. Chem. Phys., 16, 1081–1104, https://doi.org/10.5194/acp-16-1081-2016, https://doi.org/10.5194/acp-16-1081-2016, 2016
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This study investigates the size distribution, chemical composition, and optical properties of Saharan mineral dust transported over the western Mediterranean using in situ measurements collected from aircraft. Their variability due to altitude, time of transport, and mixing rate with pollution particles are discussed. We found moderate light absorption of the dust plumes even in the presence of pollution particles and the persistence of large dust particles after transport in the Mediterranean.
J. W. Taylor, T. W. Choularton, A. M. Blyth, Z. Liu, K. N. Bower, J. Crosier, M. W. Gallagher, P. I. Williams, J. R. Dorsey, M. J. Flynn, L. J. Bennett, Y. Huang, J. French, A. Korolev, and P. R. A. Brown
Atmos. Chem. Phys., 16, 799–826, https://doi.org/10.5194/acp-16-799-2016, https://doi.org/10.5194/acp-16-799-2016, 2016
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We present microphysical observations of cumulus clouds measured over south-west England during COPE in summer 2013. Detailed sampling focused on an isolated liquid cloud that glaciated as it matured to merge with a band of cloud downwind. The first ice particles observed were frozen drizzle, while columnar ice dominated in the mature stages. We discuss the interactions between the warm rain and secondary ice processes, and their importance for the formation of precipitation.
L. M. Zamora, R. A. Kahn, M. J. Cubison, G. S. Diskin, J. L. Jimenez, Y. Kondo, G. M. McFarquhar, A. Nenes, K. L. Thornhill, A. Wisthaler, A. Zelenyuk, and L. D. Ziemba
Atmos. Chem. Phys., 16, 715–738, https://doi.org/10.5194/acp-16-715-2016, https://doi.org/10.5194/acp-16-715-2016, 2016
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Based on extensive aircraft campaigns, we quantify how biomass burning smoke affects subarctic and Arctic liquid cloud microphysical properties. Enhanced cloud albedo may decrease short-wave radiative flux by between 2 and 4 Wm2 or more in some subarctic conditions. Smoke halved average cloud droplet diameter. In one case study, it also appeared to limit droplet formation. Numerous Arctic background Aitken particles can also interact with combustion particles, perhaps affecting their properties.
M. Mallet, F. Dulac, P. Formenti, P. Nabat, J. Sciare, G. Roberts, J. Pelon, G. Ancellet, D. Tanré, F. Parol, C. Denjean, G. Brogniez, A. di Sarra, L. Alados-Arboledas, J. Arndt, F. Auriol, L. Blarel, T. Bourrianne, P. Chazette, S. Chevaillier, M. Claeys, B. D'Anna, Y. Derimian, K. Desboeufs, T. Di Iorio, J.-F. Doussin, P. Durand, A. Féron, E. Freney, C. Gaimoz, P. Goloub, J. L. Gómez-Amo, M. J. Granados-Muñoz, N. Grand, E. Hamonou, I. Jankowiak, M. Jeannot, J.-F. Léon, M. Maillé, S. Mailler, D. Meloni, L. Menut, G. Momboisse, J. Nicolas, T. Podvin, V. Pont, G. Rea, J.-B. Renard, L. Roblou, K. Schepanski, A. Schwarzenboeck, K. Sellegri, M. Sicard, F. Solmon, S. Somot, B Torres, J. Totems, S. Triquet, N. Verdier, C. Verwaerde, F. Waquet, J. Wenger, and P. Zapf
Atmos. Chem. Phys., 16, 455–504, https://doi.org/10.5194/acp-16-455-2016, https://doi.org/10.5194/acp-16-455-2016, 2016
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The aim of this article is to present an experimental campaign over the Mediterranean focused on aerosol-radiation measurements and modeling. Results indicate an important atmospheric loading associated with a moderate absorbing ability of mineral dust. Observations suggest a complex vertical structure and size distributions characterized by large aerosols within dust plumes. The radiative effect is highly variable, with negative forcing over the Mediterranean and positive over northern Africa.
Q. J. Zhang, M. Beekmann, E. Freney, K. Sellegri, J. M. Pichon, A. Schwarzenboeck, A. Colomb, T. Bourrianne, V. Michoud, and A. Borbon
Atmos. Chem. Phys., 15, 13973–13992, https://doi.org/10.5194/acp-15-13973-2015, https://doi.org/10.5194/acp-15-13973-2015, 2015
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Secondary organic aerosol (SOA) is an important pollutant formed from megacity emissions at a regional scale. An original method based on ratios of different pollutants is used to specifically validate the aerosol scheme (the volatility basis set approach) within a CTM. The method is applied to airborne measurements performed within the Paris plume during the MEGAPOLI summer campaign. Simulations indicate that SOA of anthropogenic origin has a significant impact on regional air quality.
M. W. Shephard, C. A. McLinden, K. E. Cady-Pereira, M. Luo, S. G. Moussa, A. Leithead, J. Liggio, R. M. Staebler, A. Akingunola, P. Makar, P. Lehr, J. Zhang, D. K. Henze, D. B. Millet, J. O. Bash, L. Zhu, K. C. Wells, S. L. Capps, S. Chaliyakunnel, M. Gordon, K. Hayden, J. R. Brook, M. Wolde, and S.-M. Li
Atmos. Meas. Tech., 8, 5189–5211, https://doi.org/10.5194/amt-8-5189-2015, https://doi.org/10.5194/amt-8-5189-2015, 2015
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This study provides direct validations of Tropospheric Emission Spectrometer (TES) satellite retrieved profiles against coincident aircraft profiles of carbon monoxide, ammonia, methanol, and formic acid, all of which are of interest for air quality. The comparisons are performed over the Canadian oil sands region during an intensive field campaign in support of the Joint Canada-Alberta Implementation Plan for the Oil Sands Monitoring (JOSM). Initial model evaluations are also provided.
K. Thayer-Calder, A. Gettelman, C. Craig, S. Goldhaber, P. A. Bogenschutz, C.-C. Chen, H. Morrison, J. Höft, E. Raut, B. M. Griffin, J. K. Weber, V. E. Larson, M. C. Wyant, M. Wang, Z. Guo, and S. J. Ghan
Geosci. Model Dev., 8, 3801–3821, https://doi.org/10.5194/gmd-8-3801-2015, https://doi.org/10.5194/gmd-8-3801-2015, 2015
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This study evaluates a unified cloud parameterization and a Monte Carlo microphysics interface that is implemented in CAM v5.3. We show mean climate and tropical variability results from global simulations. The model has a degradation in precipitation skill but improvements in shortwave cloud forcing, liquid water path, long-wave cloud forcing, precipitable water, and tropical wave simulation. We also show estimation of computational expense and sensitivity to number of subcolumns.
A. M. Fridlind, A. S. Ackerman, A. Grandin, F. Dezitter, M. Weber, J. W. Strapp, A. V. Korolev, and C. R. Williams
Atmos. Chem. Phys., 15, 11713–11728, https://doi.org/10.5194/acp-15-11713-2015, https://doi.org/10.5194/acp-15-11713-2015, 2015
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Airbus measurements at elevations circa 11 km within large storm systems near Darwin and Santiago indicate ice mass distributed over area-equivalent diameters of 100-500 µm. Profiler-observed radar reflectivity and mean Doppler velocity under similar conditions are found to be consistent with measurements and with 1D simulations of steady-state stratiform rain columns initialized with observed ice size distributions. Results motivate investigation of ice formation pathways in Part II.
A. S. Ackerman, A. M. Fridlind, A. Grandin, F. Dezitter, M. Weber, J. W. Strapp, and A. V. Korolev
Atmos. Chem. Phys., 15, 11729–11751, https://doi.org/10.5194/acp-15-11729-2015, https://doi.org/10.5194/acp-15-11729-2015, 2015
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An updraft parcel model with size-resolved microphysics is used to investigate microphysical pathways leading to ice water content > 2 g m-3 with mass median area-equivalent diameter of 200-300 micron reported at ~11 km in tropical deep convection. Parcel simulations require substantial source of small crystals at temperatures > ~-10 deg C growing by vapor deposition. Warm rain in weaker updrafts surprisingly leads to greater ice mass owing to reduced competition for available water vapor.
M. Gordon, S.-M. Li, R. Staebler, A. Darlington, K. Hayden, J. O'Brien, and M. Wolde
Atmos. Meas. Tech., 8, 3745–3765, https://doi.org/10.5194/amt-8-3745-2015, https://doi.org/10.5194/amt-8-3745-2015, 2015
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Aircraft-based measurements of air pollutants from sources in the Canadian oil sands were made during a summer intensive field campaign in 2013. This paper describes the top-down emission rate retrieval algorithm (TERRA) to determine facility emissions of pollutants, using SO2 and CH4 as examples. Uncertainty of the emission rates estimated with TERRA is estimated as less than 30%, which is primarily due to the unknown SO2 and CH4 mixing ratios near the surface below the lowest flight level.
M. Pikridas, J. Sciare, F. Freutel, S. Crumeyrolle, S.-L. von der Weiden-Reinmüller, A. Borbon, A. Schwarzenboeck, M. Merkel, M. Crippa, E. Kostenidou, M. Psichoudaki, L. Hildebrandt, G. J. Engelhart, T. Petäjä, A. S. H. Prévôt, F. Drewnick, U. Baltensperger, A. Wiedensohler, M. Kulmala, M. Beekmann, and S. N. Pandis
Atmos. Chem. Phys., 15, 10219–10237, https://doi.org/10.5194/acp-15-10219-2015, https://doi.org/10.5194/acp-15-10219-2015, 2015
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Aerosol size distribution measurements from three ground sites, two mobile laboratories, and one airplane are combined to investigate the spatial and temporal variability of ultrafine particles in and around Paris during the summer and winter MEGAPOLI campaigns. The role of nucleation as a particle source and the influence of Paris emissions on their surroundings are examined.
C. Rose, K. Sellegri, E. Freney, R. Dupuy, A. Colomb, J.-M. Pichon, M. Ribeiro, T. Bourianne, F. Burnet, and A. Schwarzenboeck
Atmos. Chem. Phys., 15, 10203–10218, https://doi.org/10.5194/acp-15-10203-2015, https://doi.org/10.5194/acp-15-10203-2015, 2015
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In the present paper we report airborne measurements of new particle formation (NPF) above the Mediterranean Sea (HYMEX campaign). We show that NPF occurs over large areas above the sea, but the process is clearly promoted at high altitude, above 1000m, i.e. frequently in the free troposphere. NPF also seems to be mainly influenced by local processes occurring above the sea. After their formation, particles slowly grow at high altitude while not being greatly depleted or affected by coagulation.
P. Tuccella, G. Curci, G. A. Grell, G. Visconti, S. Crumeyrolle, A. Schwarzenboeck, and A. A. Mensah
Geosci. Model Dev., 8, 2749–2776, https://doi.org/10.5194/gmd-8-2749-2015, https://doi.org/10.5194/gmd-8-2749-2015, 2015
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A parameterization for secondary organic aerosol (SOA) production based on the volatility basis set (VBS) approach has been coupled with microphysics and radiative schemes in the WRF-Chem model. The new chemistry was evaluated on a cloud-resolving scale against ground-based and aircraft measurements collected during the IMPACT-EUCAARI campaign, and complemented with satellite data from MODIS. Sensitivity tests have been performed to study the impact of SOA on cloud prediction and development.
H. Petetin, M. Beekmann, A. Colomb, H. A. C. Denier van der Gon, J.-C. Dupont, C. Honoré, V. Michoud, Y. Morille, O. Perrussel, A. Schwarzenboeck, J. Sciare, A. Wiedensohler, and Q. J. Zhang
Atmos. Chem. Phys., 15, 9799–9818, https://doi.org/10.5194/acp-15-9799-2015, https://doi.org/10.5194/acp-15-9799-2015, 2015
M. Beekmann, A. S. H. Prévôt, F. Drewnick, J. Sciare, S. N. Pandis, H. A. C. Denier van der Gon, M. Crippa, F. Freutel, L. Poulain, V. Ghersi, E. Rodriguez, S. Beirle, P. Zotter, S.-L. von der Weiden-Reinmüller, M. Bressi, C. Fountoukis, H. Petetin, S. Szidat, J. Schneider, A. Rosso, I. El Haddad, A. Megaritis, Q. J. Zhang, V. Michoud, J. G. Slowik, S. Moukhtar, P. Kolmonen, A. Stohl, S. Eckhardt, A. Borbon, V. Gros, N. Marchand, J. L. Jaffrezo, A. Schwarzenboeck, A. Colomb, A. Wiedensohler, S. Borrmann, M. Lawrence, A. Baklanov, and U. Baltensperger
Atmos. Chem. Phys., 15, 9577–9591, https://doi.org/10.5194/acp-15-9577-2015, https://doi.org/10.5194/acp-15-9577-2015, 2015
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A detailed characterization of air quality in the Paris (France) agglomeration, a megacity, during two summer and winter intensive campaigns and from additional 1-year observations, revealed that about 70% of the fine particulate matter (PM) at urban background is transported into the megacity from upwind regions. Unexpectedly, a major part of organic PM is of modern origin (woodburning and cooking activities, secondary formation from biogenic VOC).
J. Um, G. M. McFarquhar, Y. P. Hong, S.-S. Lee, C. H. Jung, R. P. Lawson, and Q. Mo
Atmos. Chem. Phys., 15, 3933–3956, https://doi.org/10.5194/acp-15-3933-2015, https://doi.org/10.5194/acp-15-3933-2015, 2015
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Dimensions of ice crystals increased with an increase in temperature and the L-W relationships of crystals with a given L depended heavily on temperature, whereas the aspect ratio depended only weakly on temperature. The relative frequency of occurrence of plates was much larger in anvil clouds compared to that of columnar crystals (i.e., columns and bullet rosettes), whereas the relative occurrence frequency of columnar crystals was much larger in non-anvil clouds.
L. Marelle, J.-C. Raut, J. L. Thomas, K. S. Law, B. Quennehen, G. Ancellet, J. Pelon, A. Schwarzenboeck, and J. D. Fast
Atmos. Chem. Phys., 15, 3831–3850, https://doi.org/10.5194/acp-15-3831-2015, https://doi.org/10.5194/acp-15-3831-2015, 2015
N. Bègue, P. Tulet, J. Pelon, B. Aouizerats, A. Berger, and A. Schwarzenboeck
Atmos. Chem. Phys., 15, 3497–3516, https://doi.org/10.5194/acp-15-3497-2015, https://doi.org/10.5194/acp-15-3497-2015, 2015
A. Korolev and P. R. Field
Atmos. Meas. Tech., 8, 761–777, https://doi.org/10.5194/amt-8-761-2015, https://doi.org/10.5194/amt-8-761-2015, 2015
E. Fontaine, A. Schwarzenboeck, J. Delanoë, W. Wobrock, D. Leroy, R. Dupuy, C. Gourbeyre, and A. Protat
Atmos. Chem. Phys., 14, 11367–11392, https://doi.org/10.5194/acp-14-11367-2014, https://doi.org/10.5194/acp-14-11367-2014, 2014
T. Eidhammer, H. Morrison, A. Bansemer, A. Gettelman, and A. J. Heymsfield
Atmos. Chem. Phys., 14, 10103–10118, https://doi.org/10.5194/acp-14-10103-2014, https://doi.org/10.5194/acp-14-10103-2014, 2014
D. Barahona, A. Molod, J. Bacmeister, A. Nenes, A. Gettelman, H. Morrison, V. Phillips, and A. Eichmann
Geosci. Model Dev., 7, 1733–1766, https://doi.org/10.5194/gmd-7-1733-2014, https://doi.org/10.5194/gmd-7-1733-2014, 2014
G. Ancellet, J. Pelon, Y. Blanchard, B. Quennehen, A. Bazureau, K. S. Law, and A. Schwarzenboeck
Atmos. Chem. Phys., 14, 8235–8254, https://doi.org/10.5194/acp-14-8235-2014, https://doi.org/10.5194/acp-14-8235-2014, 2014
A. Gettelman, H. Morrison, C. R. Terai, and R. Wood
Atmos. Chem. Phys., 13, 9855–9867, https://doi.org/10.5194/acp-13-9855-2013, https://doi.org/10.5194/acp-13-9855-2013, 2013
Related subject area
Subject: Clouds and Precipitation | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Effect of secondary ice production processes on the simulation of ice pellets using the Predicted Particle Properties microphysics scheme
Simulated particle evolution within a winter storm: contributions of riming to radar moments and precipitation fallout
A thermal-driven graupel generation process to explain dry-season convective vigor over the Amazon
Modeling homogeneous ice nucleation from drop-freezing experiments: impact of droplet volume dispersion and cooling rates
Cloud water adjustments to aerosol perturbations are buffered by solar heating in non-precipitating marine stratocumuli
Glaciation of mixed-phase clouds: insights from bulk model and bin-microphysics large-eddy simulation informed by laboratory experiment
Microphysical processes involving the vapour phase dominate in simulated low-level Arctic clouds
Understanding aerosol–cloud interactions using a single-column model for a cold-air outbreak case during the ACTIVATE campaign
On the sensitivity of aerosol–cloud interactions to changes in sea surface temperature in radiative–convective equilibrium
Exploring aerosol–cloud interactions in liquid-phase clouds over eastern China and its adjacent ocean using the WRF-Chem–SBM model
Finite domains cause bias in measured and modeled distributions of cloud sizes
A systematic evaluation of high-cloud controlling factors
Tracking precipitation features and associated large-scale environments over southeastern Texas
Revisiting the evolution of downhill thunderstorms over Beijing: a new perspective from a radar wind profiler mesonet
How well can persistent contrails be predicted? An update
Potential impacts of marine fuel regulations on Arctic clouds and radiative feedbacks
Present-day correlations are insufficient to predict cloud albedo change by anthropogenic aerosols in E3SM v2
Simulations of primary and secondary ice production during an Arctic mixed-phase cloud case from the Ny-Ålesund Aerosol Cloud Experiment (NASCENT) campaign
Microphysical characteristics of precipitation within convective overshooting over East China observed by GPM DPR and ERA5
Effects of radiative cooling on advection fog over the northwest Pacific Ocean: observations and large-eddy simulations
Evaluating the Wegener–Bergeron–Findeisen process in ICON in large-eddy mode with in situ observations from the CLOUDLAB project
Aerosol-induced closure of marine cloud cells: enhanced effects in the presence of precipitation
Impact of ice multiplication on the cloud electrification of a cold-season thunderstorm: a numerical case study
Developing a climatological simplification of aerosols to enter the cloud microphysics of a global climate model
High ice water content in tropical mesoscale convective systems (a conceptual model)
Interactions between trade wind clouds and local forcings over the Great Barrier Reef: a case study using convection-permitting simulations
Variability in the properties of the distribution of the relative humidity with respect to ice: implications for contrail formation
Diurnal variation of amplified canopy urban heat island in Beijing megacity during heat wave periods: Roles of mountain-valley circulation and urban morphology
Simulating the seeder–feeder impacts on cloud ice and precipitation over the Alps
Cloud response to co-condensation of water and organic vapors over the boreal forest
Distribution and morphology of non-persistent contrail and persistent contrail formation areas in ERA5
Diurnal evolution of non-precipitating marine stratocumuli in an LES ensemble
Above-cloud concentrations of cloud condensation nuclei help to sustain some Arctic low-level clouds
WRF-SBM Numerical Simulation of Aerosol Effects on Stratiform Warm Clouds in Jiangxi, China
The presence of clouds lowers climate sensitivity in the MPI-ESM1.2 climate model
Evolution of Cloud Droplet Temperature and Lifetime in Spatiotemporally Varying Subsaturated Environments with Implications for Ice Nucleation at Cloud Edges
Contrail formation on ambient aerosol particles for aircraft with hydrogen combustion: a box model trajectory study
Effects of intermittent aerosol forcing on the stratocumulus-to-cumulus transition
Cloud properties and their projected changes in CMIP models with low to high climate sensitivity
Water isotopic characterisation of the cloud–circulation coupling in the North Atlantic trades – Part 2: The imprint of the atmospheric circulation at different scales
Impact of urban land use on mean and heavy rainfall during the Indian summer monsoon
Towards a more reliable forecast of ice supersaturation: concept of a one-moment ice-cloud scheme that avoids saturation adjustment
Opinion: Tropical cirrus – from micro-scale processes to climate-scale impacts
Water isotopic characterisation of the cloud–circulation coupling in the North Atlantic trades – Part 1: A process-oriented evaluation of COSMOiso simulations with EUREC4A observations
Assimilation of 3D polarimetric microphysical retrievals in a convective-scale NWP system
Sensitivity of cloud-phase distribution to cloud microphysics and thermodynamics in simulated deep convective clouds and SEVIRI retrievals
Assessing the destructiveness of tropical cyclones induced by anthropogenic aerosols in an atmosphere–ocean coupled framework
Opinion: A critical evaluation of the evidence for aerosol invigoration of deep convection
Historical (1960–2014) lightning and LNOx trends and their controlling factors in a chemistry–climate model
The chance of freezing – a conceptional study to parameterize temperature-dependent freezing by including randomness of ice-nucleating particle concentrations
Mathieu Lachapelle, Mélissa Cholette, and Julie M. Thériault
Atmos. Chem. Phys., 24, 11285–11304, https://doi.org/10.5194/acp-24-11285-2024, https://doi.org/10.5194/acp-24-11285-2024, 2024
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Hazardous precipitation types such as ice pellets and freezing rain are difficult to predict because they are associated with complex microphysical processes. Using Predicted Particle Properties (P3), this work shows that secondary ice production processes increase the amount of ice pellets simulated while decreasing the amount of freezing rain. Moreover, the properties of the simulated precipitation compare well with those that were measured.
Andrew DeLaFrance, Lynn A. McMurdie, Angela K. Rowe, and Andrew J. Heymsfield
Atmos. Chem. Phys., 24, 11191–11206, https://doi.org/10.5194/acp-24-11191-2024, https://doi.org/10.5194/acp-24-11191-2024, 2024
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Using a numerical model, the process whereby falling ice crystals accumulate supercooled liquid water droplets is investigated to elucidate its effects on radar-based measurements and surface precipitation. We demonstrate that this process accounted for 55% of the precipitation during a wintertime storm and is uniquely discernable from other ice crystal growth processes in Doppler velocity measurements. These results have implications for measurements from airborne and spaceborne platforms.
Toshi Matsui, Daniel Hernandez-Deckers, Scott E. Giangrande, Thiago S. Biscaro, Ann Fridlind, and Scott Braun
Atmos. Chem. Phys., 24, 10793–10814, https://doi.org/10.5194/acp-24-10793-2024, https://doi.org/10.5194/acp-24-10793-2024, 2024
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Using computer simulations and real measurements, we discovered that storms over the Amazon were narrower but more intense during the dry periods, producing heavier rain and more ice particles in the clouds. Our research showed that cumulus bubbles played a key role in creating these intense storms. This study can improve the representation of the effect of continental and ocean environments on tropical regions' rainfall patterns in simulations.
Ravi Kumar Reddy Addula, Ingrid de Almeida Ribeiro, Valeria Molinero, and Baron Peters
Atmos. Chem. Phys., 24, 10833–10848, https://doi.org/10.5194/acp-24-10833-2024, https://doi.org/10.5194/acp-24-10833-2024, 2024
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Ice nucleation from supercooled droplets is important in many weather and climate modeling efforts. For experiments where droplets are steadily supercooled from the freezing point, our work combines nucleation theory and survival probability analysis to predict the nucleation spectrum, i.e., droplet freezing probabilities vs. temperature. We use the new framework to extract approximately consistent rate parameters from experiments with different cooling rates and droplet sizes.
Jianhao Zhang, Yao-Sheng Chen, Takanobu Yamaguchi, and Graham Feingold
Atmos. Chem. Phys., 24, 10425–10440, https://doi.org/10.5194/acp-24-10425-2024, https://doi.org/10.5194/acp-24-10425-2024, 2024
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Quantifying cloud response to aerosol perturbations presents a major challenge in understanding the human impact on climate. Using a large number of process-resolving simulations of marine stratocumulus, we show that solar heating drives a negative feedback mechanism that buffers the persistent negative trend in cloud water adjustment after sunrise. This finding has implications for the dependence of the cloud cooling effect on the timing of deliberate aerosol perturbations.
Aaron Wang, Steve Krueger, Sisi Chen, Mikhail Ovchinnikov, Will Cantrell, and Raymond A. Shaw
Atmos. Chem. Phys., 24, 10245–10260, https://doi.org/10.5194/acp-24-10245-2024, https://doi.org/10.5194/acp-24-10245-2024, 2024
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We employ two methods to examine a laboratory experiment on clouds with both ice and liquid phases. The first assumes well-mixed properties; the second resolves the spatial distribution of turbulence and cloud particles. Results show that while the trends in mean properties generally align, when turbulence is resolved, liquid droplets are not fully depleted by ice due to incomplete mixing. This underscores the threshold of ice mass fraction in distinguishing mixed-phase clouds from ice clouds.
Theresa Kiszler, Davide Ori, and Vera Schemann
Atmos. Chem. Phys., 24, 10039–10053, https://doi.org/10.5194/acp-24-10039-2024, https://doi.org/10.5194/acp-24-10039-2024, 2024
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Microphysical processes impact the phase-partitioning of clouds. In this study we evaluate these processes while focusing on low-level Arctic clouds. To achieve this we used an extensive simulation set in combination with a new diagnostic tool. This study presents our findings on the relevance of these processes and their behaviour under different thermodynamic regimes.
Shuaiqi Tang, Hailong Wang, Xiang-Yu Li, Jingyi Chen, Armin Sorooshian, Xubin Zeng, Ewan Crosbie, Kenneth L. Thornhill, Luke D. Ziemba, and Christiane Voigt
Atmos. Chem. Phys., 24, 10073–10092, https://doi.org/10.5194/acp-24-10073-2024, https://doi.org/10.5194/acp-24-10073-2024, 2024
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We examined marine boundary layer clouds and their interactions with aerosols in the E3SM single-column model (SCM) for a case study. The SCM shows good agreement when simulating the clouds with high-resolution models. It reproduces the relationship between cloud droplet and aerosol particle number concentrations as produced in global models. However, the relationship between cloud liquid water and droplet number concentration is different, warranting further investigation.
Suf Lorian and Guy Dagan
Atmos. Chem. Phys., 24, 9323–9338, https://doi.org/10.5194/acp-24-9323-2024, https://doi.org/10.5194/acp-24-9323-2024, 2024
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We examine the combined effect of aerosols and sea surface temperature (SST) on clouds under equilibrium conditions in cloud-resolving radiative–convective equilibrium simulations. We demonstrate that the aerosol–cloud interaction's effect on top-of-atmosphere energy gain strongly depends on the underlying SST, while the shortwave part of the spectrum is significantly more sensitive to SST. Furthermore, increasing aerosols influences upper-troposphere stability and thus anvil cloud fraction.
Jianqi Zhao, Xiaoyan Ma, Johannes Quaas, and Hailing Jia
Atmos. Chem. Phys., 24, 9101–9118, https://doi.org/10.5194/acp-24-9101-2024, https://doi.org/10.5194/acp-24-9101-2024, 2024
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We explore aerosol–cloud interactions in liquid-phase clouds over eastern China and its adjacent ocean in winter based on the WRF-Chem–SBM model, which couples a spectral-bin microphysics scheme and an online aerosol module. Our study highlights the differences in aerosol–cloud interactions between land and ocean and between precipitation clouds and non-precipitation clouds, and it differentiates and quantifies their underlying mechanisms.
Thomas D. DeWitt and Timothy J. Garrett
Atmos. Chem. Phys., 24, 8457–8472, https://doi.org/10.5194/acp-24-8457-2024, https://doi.org/10.5194/acp-24-8457-2024, 2024
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There is considerable disagreement on mathematical parameters that describe the number of clouds of different sizes as well as the size of the largest clouds. Both are key defining characteristics of Earth's atmosphere. A previous study provided an incorrect explanation for the disagreement. Instead, the disagreement may be explained by prior studies not properly accounting for the size of their measurement domain. We offer recommendations for how the domain size can be accounted for.
Sarah Wilson Kemsley, Paulo Ceppi, Hendrik Andersen, Jan Cermak, Philip Stier, and Peer Nowack
Atmos. Chem. Phys., 24, 8295–8316, https://doi.org/10.5194/acp-24-8295-2024, https://doi.org/10.5194/acp-24-8295-2024, 2024
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Aiming to inform parameter selection for future observational constraint analyses, we incorporate five candidate meteorological drivers specifically targeting high clouds into a cloud controlling factor framework within a range of spatial domain sizes. We find a discrepancy between optimal domain size for predicting locally and globally aggregated cloud radiative anomalies and identify upper-tropospheric static stability as an important high-cloud controlling factor.
Ye Liu, Yun Qian, Larry K. Berg, Zhe Feng, Jianfeng Li, Jingyi Chen, and Zhao Yang
Atmos. Chem. Phys., 24, 8165–8181, https://doi.org/10.5194/acp-24-8165-2024, https://doi.org/10.5194/acp-24-8165-2024, 2024
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Deep convection under various large-scale meteorological patterns (LSMPs) shows distinct precipitation features. In southeastern Texas, mesoscale convective systems (MCSs) contribute significantly to precipitation year-round, while isolated deep convection (IDC) is prominent in summer and fall. Self-organizing maps (SOMs) reveal convection can occur without large-scale lifting or moisture convergence. MCSs and IDC events have distinct life cycles influenced by specific LSMPs.
Xiaoran Guo, Jianping Guo, Tianmeng Chen, Ning Li, Fan Zhang, and Yuping Sun
Atmos. Chem. Phys., 24, 8067–8083, https://doi.org/10.5194/acp-24-8067-2024, https://doi.org/10.5194/acp-24-8067-2024, 2024
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The prediction of downhill thunderstorms (DSs) remains elusive. We propose an objective method to identify DSs, based on which enhanced and dissipated DSs are discriminated. A radar wind profiler (RWP) mesonet is used to derive divergence and vertical velocity. The mid-troposphere divergence and prevailing westerlies enhance the intensity of DSs, whereas low-level divergence is observed when the DS dissipates. The findings highlight the key role that an RWP mesonet plays in the evolution of DSs.
Sina Hofer, Klaus Gierens, and Susanne Rohs
Atmos. Chem. Phys., 24, 7911–7925, https://doi.org/10.5194/acp-24-7911-2024, https://doi.org/10.5194/acp-24-7911-2024, 2024
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We try to improve the forecast of ice supersaturation (ISS) and potential persistent contrails using data on dynamical quantities in addition to temperature and relative humidity in a modern kind of regression model. Although the results are improved, they are not good enough for flight routing. The origin of the problem is the strong overlap of probability densities conditioned on cases with and without ice-supersaturated regions (ISSRs) in the important range of 70–100 %.
Luís Filipe Escusa dos Santos, Hannah C. Frostenberg, Alejandro Baró Pérez, Annica M. L. Ekman, Luisa Ickes, and Erik S. Thomson
EGUsphere, https://doi.org/10.5194/egusphere-2024-1891, https://doi.org/10.5194/egusphere-2024-1891, 2024
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The Arctic is experiencing enhanced surface warming. The observed decline in Arctic sea-ice extent is projected to lead to an increase in Arctic shipping activity which may lead to further climatic feedbacks. We investigate, using an atmospheric model and results from marine engine experiments which focused on fuel sulfur content reduction and exhaust wet scrubbing, how ship exhaust particles influence the properties of Arctic clouds. Implications for radiative surface processes are discussed.
Naser Mahfouz, Johannes Mülmenstädt, and Susannah Burrows
Atmos. Chem. Phys., 24, 7253–7260, https://doi.org/10.5194/acp-24-7253-2024, https://doi.org/10.5194/acp-24-7253-2024, 2024
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Climate models are our primary tool to probe past, present, and future climate states unlike the more recent observation record. By constructing a hypothetical model configuration, we show that present-day correlations are insufficient to predict a persistent uncertainty in climate projection (how much sun because clouds will reflect in a changing climate). We hope our result will contribute to the scholarly conversation on better utilizing observations to constrain climate uncertainties.
Britta Schäfer, Robert Oscar David, Paraskevi Georgakaki, Julie Thérèse Pasquier, Georgia Sotiropoulou, and Trude Storelvmo
Atmos. Chem. Phys., 24, 7179–7202, https://doi.org/10.5194/acp-24-7179-2024, https://doi.org/10.5194/acp-24-7179-2024, 2024
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Mixed-phase clouds, i.e., clouds consisting of ice and supercooled water, are very common in the Arctic. However, how these clouds form is often not correctly represented in standard weather models. We show that both ice crystal concentrations in the cloud and precipitation from the cloud can be improved in the model when aerosol concentrations are prescribed from observations and when more processes for ice multiplication, i.e., the production of new ice particles from existing ice, are added.
Nan Sun, Gaopeng Lu, and Yunfei Fu
Atmos. Chem. Phys., 24, 7123–7135, https://doi.org/10.5194/acp-24-7123-2024, https://doi.org/10.5194/acp-24-7123-2024, 2024
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Microphysical characteristics of convective overshooting are essential but poorly understood, and we examine them by using the latest data. (1) Convective overshooting events mainly occur over NC (Northeast China) and northern MEC (Middle and East China). (2) Radar reflectivity of convective overshooting over NC accounts for a higher proportion below the zero level, while the opposite is the case for MEC and SC (South China). (3) Droplets of convective overshooting are large but sparse.
Liu Yang, Saisai Ding, Jing-Wu Liu, and Su-Ping Zhang
Atmos. Chem. Phys., 24, 6809–6824, https://doi.org/10.5194/acp-24-6809-2024, https://doi.org/10.5194/acp-24-6809-2024, 2024
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Advection fog occurs when warm and moist air moves over a cold sea surface. In this situation, the temperature of the foggy air usually drops below the sea surface temperature (SST), particularly at night. High-resolution simulations show that the cooling effect of longwave radiation from the top of the fog layer permeates through the fog, resulting in a cooling of the surface air below SST. This study emphasizes the significance of monitoring air temperature to enhance sea fog forecasting.
Nadja Omanovic, Sylvaine Ferrachat, Christopher Fuchs, Jan Henneberger, Anna J. Miller, Kevin Ohneiser, Fabiola Ramelli, Patric Seifert, Robert Spirig, Huiying Zhang, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 6825–6844, https://doi.org/10.5194/acp-24-6825-2024, https://doi.org/10.5194/acp-24-6825-2024, 2024
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We present simulations with a high-resolution numerical weather prediction model to study the growth of ice crystals in low clouds following glaciogenic seeding. We show that the simulated ice crystals grow slower than observed and do not consume as many cloud droplets as measured in the field. This may have implications for forecasting precipitation, as the ice phase is crucial for precipitation at middle and high latitudes.
Matthew W. Christensen, Peng Wu, Adam C. Varble, Heng Xiao, and Jerome D. Fast
Atmos. Chem. Phys., 24, 6455–6476, https://doi.org/10.5194/acp-24-6455-2024, https://doi.org/10.5194/acp-24-6455-2024, 2024
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Clouds are essential to keep Earth cooler by reflecting sunlight back to space. We show that an increase in aerosol concentration suppresses precipitation in clouds, causing them to accumulate water and expand in a polluted environment with stronger turbulence and radiative cooling. This process enhances their reflectance by 51 %. It is therefore prudent to account for cloud fraction changes in assessments of aerosol–cloud interactions to improve predictions of climate change.
Jing Yang, Shiye Huang, Tianqi Yang, Qilin Zhang, Yuting Deng, and Yubao Liu
Atmos. Chem. Phys., 24, 5989–6010, https://doi.org/10.5194/acp-24-5989-2024, https://doi.org/10.5194/acp-24-5989-2024, 2024
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This study contributes to filling the dearth of understanding the impacts of different secondary ice production (SIP) processes on the cloud electrification in cold-season thunderstorms. The results suggest that SIP, especially the rime-splintering process and the shattering of freezing drops, has significant impacts on the charge structure of the storm. In addition, the modeled radar composite reflectivity and flash rate are improved after implementing the SIP processes in the model.
Ulrike Proske, Sylvaine Ferrachat, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 5907–5933, https://doi.org/10.5194/acp-24-5907-2024, https://doi.org/10.5194/acp-24-5907-2024, 2024
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Climate models include treatment of aerosol particles because these influence clouds and radiation. Over time their representation has grown increasingly detailed. This complexity may hinder our understanding of model behaviour. Thus here we simplify the aerosol representation of our climate model by prescribing mean concentrations, which saves run time and helps to discover unexpected model behaviour. We conclude that simplifications provide a new perspective for model study and development.
Alexei Korolev, Zhipeng Qu, Jason Milbrandt, Ivan Heckman, Mélissa Cholette, Mengistu Wolde, Cuong Nguyen, Greg McFarquhar, Paul Lawson, and Ann Fridlind
EGUsphere, https://doi.org/10.5194/egusphere-2024-1465, https://doi.org/10.5194/egusphere-2024-1465, 2024
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The phenomenon of high ice water content (HIWC) occurs in mesoscale convective systems (MCS) when a large number of small ice particles with typical sizes of a few hundred micrometers are found at high altitudes. This study presents a conceptual model of the formation of HIWC in tropical MCSs developed based on in-situ observations and numerical simulation. It was found that secondary ice production in the vicinity of the melting layer plays a key role in the formation and maintenance of HIWC.
Wenhui Zhao, Yi Huang, Steven Siems, Michael Manton, and Daniel Harrison
Atmos. Chem. Phys., 24, 5713–5736, https://doi.org/10.5194/acp-24-5713-2024, https://doi.org/10.5194/acp-24-5713-2024, 2024
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We studied how shallow clouds and rain behave over the Great Barrier Reef (GBR) using a detailed weather model. We found that the shape of the land, especially mountains, and particles in the air play big roles in influencing these clouds. Surprisingly, the sea's temperature had a smaller effect. Our research helps us understand the GBR's climate and how various factors can influence it, where the importance of the local cloud in thermal coral bleaching has recently been identified.
Sidiki Sanogo, Olivier Boucher, Nicolas Bellouin, Audran Borella, Kevin Wolf, and Susanne Rohs
Atmos. Chem. Phys., 24, 5495–5511, https://doi.org/10.5194/acp-24-5495-2024, https://doi.org/10.5194/acp-24-5495-2024, 2024
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Relative humidity relative to ice (RHi) is a key variable in the formation of cirrus clouds and contrails. This study shows that the properties of the probability density function of RHi differ between the tropics and higher latitudes. In line with RHi and temperature variability, aircraft are likely to produce more contrails with bioethanol and liquid hydrogen as fuel. The impact of this fuel change decreases with decreasing pressure levels but increases from high latitudes to the tropics.
Tao Shi, Yuanjian Yang, Ping Qi, and Simone Lolli
EGUsphere, https://doi.org/10.5194/egusphere-2024-1200, https://doi.org/10.5194/egusphere-2024-1200, 2024
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In the background of global warming and the rapid urbanization, heat wave have emerged as increasingly frequent occurrences. Despite this, the specific roles played by local circulation patterns and urban morphology in the synergistic interaction between HW and CUHI remain elusive. To address this gap, this paper used automatic weather stations data and meachine learning model to delve into the spatiotemporal patterns governing the intricate interactions between HW and CUHI.
Zane Dedekind, Ulrike Proske, Sylvaine Ferrachat, Ulrike Lohmann, and David Neubauer
Atmos. Chem. Phys., 24, 5389–5404, https://doi.org/10.5194/acp-24-5389-2024, https://doi.org/10.5194/acp-24-5389-2024, 2024
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Ice particles precipitating into lower clouds from an upper cloud, the seeder–feeder process, can enhance precipitation. A numerical modeling study conducted in the Swiss Alps found that 48 % of observed clouds were overlapping, with the seeder–feeder process occurring in 10 % of these clouds. Inhibiting the seeder–feeder process reduced the surface precipitation and ice particle growth rates, which were further reduced when additional ice multiplication processes were included in the model.
Liine Heikkinen, Daniel G. Partridge, Sara Blichner, Wei Huang, Rahul Ranjan, Paul Bowen, Emanuele Tovazzi, Tuukka Petäjä, Claudia Mohr, and Ilona Riipinen
Atmos. Chem. Phys., 24, 5117–5147, https://doi.org/10.5194/acp-24-5117-2024, https://doi.org/10.5194/acp-24-5117-2024, 2024
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The organic vapor condensation with water vapor (co-condensation) in rising air below clouds is modeled in this work over the boreal forest because the forest air is rich in organic vapors. We show that the number of cloud droplets can increase by 20 % if considering co-condensation. The enhancements are even larger if the air contains many small, naturally produced aerosol particles. Such conditions are most frequently met in spring in the boreal forest.
Kevin Wolf, Nicolas Bellouin, and Olivier Boucher
Atmos. Chem. Phys., 24, 5009–5024, https://doi.org/10.5194/acp-24-5009-2024, https://doi.org/10.5194/acp-24-5009-2024, 2024
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The contrail formation potential and its tempo-spatial distribution are estimated for the North Atlantic flight corridor. Meteorological conditions of temperature and relative humidity are taken from the ERA5 re-analysis and IAGOS. Based on IAGOS flight tracks, crossing length, size, orientation, frequency of occurrence, and overlap of persistent contrail formation areas are determined. The presented conclusions might provide a guide for statistical flight track optimization to reduce contrails.
Yao-Sheng Chen, Jianhao Zhang, Fabian Hoffmann, Takanobu Yamaguchi, Franziska Glassmeier, Xiaoli Zhou, and Graham Feingold
EGUsphere, https://doi.org/10.5194/egusphere-2024-1033, https://doi.org/10.5194/egusphere-2024-1033, 2024
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Marine stratocumulus cloud is a type of shallow clouds that covers the vast areas of Earth's surface. They play an important role in Earth's energy balance by reflecting solar radiation back to space. We used numerical models to simulate a large number of marine stratocumuli with different characteristics. We found that how the clouds develop throughout the day is affected by the level of humidity in the air above the clouds and how closely the clouds connect to the ocean surface.
Lucas J. Sterzinger and Adele L. Igel
Atmos. Chem. Phys., 24, 3529–3540, https://doi.org/10.5194/acp-24-3529-2024, https://doi.org/10.5194/acp-24-3529-2024, 2024
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Using idealized large eddy simulations, we find that clouds forming in the Arctic in environments with low concentrations of aerosol particles may be sustained by mixing in new particles through the cloud top. Observations show that higher concentrations of these particles regularly exist above cloud top in concentrations that are sufficient to promote this sustenance.
Yi Li, Xiaoli Liu, and Hengjia Cai
EGUsphere, https://doi.org/10.5194/egusphere-2023-2644, https://doi.org/10.5194/egusphere-2023-2644, 2024
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Different aerosol modes' influence on cloud processes remains controversial. As a result, we modified the aerosol spectrum and concentration to simulated a warm stratiform cloud process in Jiangxi, China by WRF-SBM scheme. Research shows that: different aerosol spectra have diverse effects on cloud droplet spectra, cloud development, and correlation between dispersion (ε) and cloud physics quantities. Compared to cloud droplet concentration, ε is more sensitive to the volume radius.
Andrea Mosso, Thomas Hocking, and Thorsten Mauritsen
EGUsphere, https://doi.org/10.5194/egusphere-2024-618, https://doi.org/10.5194/egusphere-2024-618, 2024
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Clouds play a crucial role in the energy balance of the earth, as they can either warm up or cool down the area they cover depending on their height and depth. It is expected that they will alter their behaviour under climate change, which will affect the warming generated by greenhouse gases. This paper proposes a new method to estimate their overall effect by simulating a climate where clouds are transparent. Results show that, with the model used, clouds have a stabilising effect on climate.
Puja Roy, Robert M. Rauber, and Larry Di Girolamo
EGUsphere, https://doi.org/10.5194/egusphere-2024-526, https://doi.org/10.5194/egusphere-2024-526, 2024
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Cloud droplet temperature impacts cloud processes such as activation of ice-nucleating particles. This study investigates the thermal and radial evolution of supercooled cloud droplets and their surrounding environments, with an aim to better understand observed enhancement of ice nucleation at moderately supercooled cloud edges. This analysis shows that the magnitude of droplet cooling during evaporation is much greater than estimated from past studies, especially for drier environments.
Andreas Bier, Simon Unterstrasser, Josef Zink, Dennis Hillenbrand, Tina Jurkat-Witschas, and Annemarie Lottermoser
Atmos. Chem. Phys., 24, 2319–2344, https://doi.org/10.5194/acp-24-2319-2024, https://doi.org/10.5194/acp-24-2319-2024, 2024
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Using hydrogen as aviation fuel affects contrails' climate impact. We study contrail formation behind aircraft with H2 combustion. Due to the absence of soot emissions, contrail ice crystals are assumed to form only on ambient particles mixed into the plume. The ice crystal number, which strongly varies with temperature and aerosol number density, is decreased by more than 80 %–90 % compared to kerosene contrails. However H2 contrails can form at lower altitudes due to higher H2O emissions.
Prasanth Prabhakaran, Fabian Hoffmann, and Graham Feingold
Atmos. Chem. Phys., 24, 1919–1937, https://doi.org/10.5194/acp-24-1919-2024, https://doi.org/10.5194/acp-24-1919-2024, 2024
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In this study, we explore the impact of deliberate aerosol perturbation in the northeast Pacific region using large-eddy simulations. Our results show that cloud reflectivity is sensitive to the aerosol sprayer arrangement in the pristine system, whereas in the polluted system it is largely proportional to the total number of aerosol particles injected. These insights would aid in assessing the efficiency of various aerosol injection strategies for climate intervention applications.
Lisa Bock and Axel Lauer
Atmos. Chem. Phys., 24, 1587–1605, https://doi.org/10.5194/acp-24-1587-2024, https://doi.org/10.5194/acp-24-1587-2024, 2024
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Climate model simulations still show a large range of effective climate sensitivity (ECS) with high uncertainties. An important contribution to ECS is cloud climate feedback. We investigate the representation of cloud physical and radiative properties from Coupled Model Intercomparison Project models grouped by ECS. We compare the simulated cloud properties of today’s climate from three ECS groups and quantify how the projected changes in cloud properties and cloud radiative effects differ.
Leonie Villiger and Franziska Aemisegger
Atmos. Chem. Phys., 24, 957–976, https://doi.org/10.5194/acp-24-957-2024, https://doi.org/10.5194/acp-24-957-2024, 2024
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Three numerical simulations performed with an isotope-enabled weather forecast model are used to investigate the cloud–circulation coupling between shallow trade-wind cumulus clouds and atmospheric circulations on different scales. It is shown that stable water isotopes near cloud base in the tropics reflect (1) the diel cycle of the atmospheric circulation, which drives the formation and dissipation of clouds, and (2) changes in the large-scale circulation over the North Atlantic.
Renaud Falga and Chien Wang
Atmos. Chem. Phys., 24, 631–647, https://doi.org/10.5194/acp-24-631-2024, https://doi.org/10.5194/acp-24-631-2024, 2024
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The impact of urban land use on regional meteorology and rainfall during the Indian summer monsoon has been assessed in this study. Using a cloud-resolving model centered around Kolkata, we have shown that the urban heat island effect led to a rainfall enhancement via the amplification of convective activity, especially during the night. Furthermore, the results demonstrated that the kinetic effect of the city induced the initiation of a nighttime storm.
Dario Sperber and Klaus Gierens
Atmos. Chem. Phys., 23, 15609–15627, https://doi.org/10.5194/acp-23-15609-2023, https://doi.org/10.5194/acp-23-15609-2023, 2023
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A significant share of aviation's climate impact is due to persistent contrails. Avoiding their creation is a step toward sustainable air transportation. For this purpose, a reliable forecast of so-called ice-supersaturated regions is needed, which then allows one to plan aircraft routes without persistent contrails. Here, we propose a method that leads to the better prediction of ice-supersaturated regions.
Blaž Gasparini, Sylvia C. Sullivan, Adam B. Sokol, Bernd Kärcher, Eric Jensen, and Dennis L. Hartmann
Atmos. Chem. Phys., 23, 15413–15444, https://doi.org/10.5194/acp-23-15413-2023, https://doi.org/10.5194/acp-23-15413-2023, 2023
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Tropical cirrus clouds are essential for climate, but our understanding of these clouds is limited due to their dependence on a wide range of small- and large-scale climate processes. In this opinion paper, we review recent advances in the study of tropical cirrus clouds, point out remaining open questions, and suggest ways to resolve them.
Leonie Villiger, Marina Dütsch, Sandrine Bony, Marie Lothon, Stephan Pfahl, Heini Wernli, Pierre-Etienne Brilouet, Patrick Chazette, Pierre Coutris, Julien Delanoë, Cyrille Flamant, Alfons Schwarzenboeck, Martin Werner, and Franziska Aemisegger
Atmos. Chem. Phys., 23, 14643–14672, https://doi.org/10.5194/acp-23-14643-2023, https://doi.org/10.5194/acp-23-14643-2023, 2023
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This study evaluates three numerical simulations performed with an isotope-enabled weather forecast model and investigates the coupling between shallow trade-wind cumulus clouds and atmospheric circulations on different scales. We show that the simulations reproduce key characteristics of shallow trade-wind clouds as observed during the field experiment EUREC4A and that the spatial distribution of stable-water-vapour isotopes is shaped by the overturning circulation associated with these clouds.
Lucas Reimann, Clemens Simmer, and Silke Trömel
Atmos. Chem. Phys., 23, 14219–14237, https://doi.org/10.5194/acp-23-14219-2023, https://doi.org/10.5194/acp-23-14219-2023, 2023
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Polarimetric radar observations were assimilated for the first time in a convective-scale numerical weather prediction system in Germany and their impact on short-term precipitation forecasts was evaluated. The assimilation was performed using microphysical retrievals of liquid and ice water content and yielded slightly improved deterministic 9 h precipitation forecasts for three intense summer precipitation cases with respect to the assimilation of radar reflectivity alone.
Cunbo Han, Corinna Hoose, Martin Stengel, Quentin Coopman, and Andrew Barrett
Atmos. Chem. Phys., 23, 14077–14095, https://doi.org/10.5194/acp-23-14077-2023, https://doi.org/10.5194/acp-23-14077-2023, 2023
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Cloud phase has been found to significantly impact cloud thermodynamics and Earth’s radiation budget, and various factors influence it. This study investigates the sensitivity of the cloud-phase distribution to the ice-nucleating particle concentration and thermodynamics. Multiple simulation experiments were performed using the ICON model at the convection-permitting resolution of 1.2 km. Simulation results were compared to two different retrieval products based on SEVIRI measurements.
Yun Lin, Yuan Wang, Jen-Shan Hsieh, Jonathan H. Jiang, Qiong Su, Lijun Zhao, Michael Lavallee, and Renyi Zhang
Atmos. Chem. Phys., 23, 13835–13852, https://doi.org/10.5194/acp-23-13835-2023, https://doi.org/10.5194/acp-23-13835-2023, 2023
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Tropical cyclones (TCs) can cause catastrophic damage to coastal regions. We used a numerical model that explicitly simulates aerosol–cloud interaction and atmosphere–ocean coupling. We show that aerosols and ocean coupling work together to make TC storms bigger but weaker. Moreover, TCs in polluted air have more rainfall and higher sea levels, leading to more severe storm surges and flooding. Our research highlights the roles of aerosols and ocean-coupling feedbacks in TC hazard assessment.
Adam C. Varble, Adele L. Igel, Hugh Morrison, Wojciech W. Grabowski, and Zachary J. Lebo
Atmos. Chem. Phys., 23, 13791–13808, https://doi.org/10.5194/acp-23-13791-2023, https://doi.org/10.5194/acp-23-13791-2023, 2023
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As atmospheric particles called aerosols increase in number, the number of droplets in clouds tends to increase, which has been theorized to increase storm intensity. We critically evaluate the evidence for this theory, showing that flaws and limitations of previous studies coupled with unaddressed cloud process complexities draw it into question. We provide recommendations for future observations and modeling to overcome current uncertainties.
Yanfeng He and Kengo Sudo
Atmos. Chem. Phys., 23, 13061–13085, https://doi.org/10.5194/acp-23-13061-2023, https://doi.org/10.5194/acp-23-13061-2023, 2023
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Lightning has big social impacts. Lightning-produced NOx (LNOx) plays a vital role in atmospheric chemistry and climate. Investigating past lightning and LNOx trends can provide essential indicators of all lightning-related phenomena. Simulations show almost flat global lightning and LNOx trends during 1960–2014. Past global warming enhances the trends positively, but increases in aerosol have the opposite effect. Moreover, global lightning decreased markedly after the Pinatubo eruption.
Hannah C. Frostenberg, André Welti, Mikael Luhr, Julien Savre, Erik S. Thomson, and Luisa Ickes
Atmos. Chem. Phys., 23, 10883–10900, https://doi.org/10.5194/acp-23-10883-2023, https://doi.org/10.5194/acp-23-10883-2023, 2023
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Observations show that ice-nucleating particle concentrations (INPCs) have a large variety and follow lognormal distributions for a given temperature. We introduce a new immersion freezing parameterization that applies this lognormal behavior. INPCs are drawn randomly from a temperature-dependent lognormal distribution. We then show that the ice content of the modeled Arctic stratocumulus cloud is highly sensitive to the probability of drawing large INPCs.
Cited articles
Ackerman, A. S., Fridlind, A. M., Grandin, A., Dezitter, F., Weber, M., Strapp, J. W., and Korolev, A. V.: High ice water content at low radar reflectivity near deep convection – Part 2: Evaluation of microphysical pathways in updraft parcel simulations, Atmos. Chem. Phys., 15, 11729–11751, https://doi.org/10.5194/acp-15-11729-2015, 2015. a
Atlas, R., Bretherton, C. S., Blossey, P. N., Gettelman, A., Bardeen, C., Lin,
P., and Ming, Y.: How Well Do Large-Eddy Simulations and Global Climate
Models Represent Observed Boundary Layer Structures and Low Clouds Over the
Summertime Southern Ocean?, J. Adv. Model. Earth Sy.,
12, e2020MS002205, https://doi.org/10.1029/2020MS002205, 2020. a
Brownscombe, J. and Thorndike, N.: Freezing and shattering of water droplets in
free fall, Nature, 220, 687–689, https://doi.org/10.1038/220687a0, 1968. a
Bryan, G. H. and Morrison, H.: Sensitivity of a simulated squall line to
horizontal resolution and parameterization of microphysics, Mon. Weather
Rev., 140, 202–225, https://doi.org/10.1175/MWR-D-11-00046.1, 2012. a
Cantrell, W. and Heymsfield, A.: Production of ice in tropospheric clouds: A
review, B. Am. Meteorol. Soc., 86, 795–808,
https://doi.org/10.1175/BAMS-86-6-795, 2005. a
Connolly, P. J., Emersic, C., and Field, P. R.: A laboratory investigation into the aggregation efficiency of small ice crystals, Atmos. Chem. Phys., 12, 2055–2076, https://doi.org/10.5194/acp-12-2055-2012, 2012. a, b
Cooper, W. A.: Ice initiation in natural clouds, Meteor. Mon., 21, 29–32,
https://doi.org/10.1175/0065-9401-21.43.29, 1986. a
Cotton, W. R., Tripoli, G. J., Rauber, R. M., and Mulvihill, E. A.: Numerical
simulation of the effects of varying ice crystal nucleation rates and
aggregation processes on orographic snowfall, J. Clim. Appl.
Meteorol., 25, 1658–1680,
https://doi.org/10.1175/1520-0450(1986)025<1658:NSOTEO>2.0.CO;2, 1986. a
D'Alessandro, J. J., Diao, M., Wu, C., Liu, X., Chen, M., Morrison, H.,
Eidhammer, T., Jensen, J. B., Bansemer, A., Zondlo, M. A., and DiGangi, J. P.: Dynamical
conditions of ice supersaturation and ice nucleation in convective systems: A
comparative analysis between in situ aircraft observations and WRF
simulations, J. Geophys. Res.-Atmos., 122, 2844–2866,
https://doi.org/10.1002/2016JD025994, 2017. a
DeMott, P. J., Hill, T. C., McCluskey, C. S., Prather, K. A., Collins, D. B.,
Sullivan, R. C., Ruppel, M. J., Mason, R. H., Irish, V. E., Lee, T., Hwang, C. Y., Rhee, T. S., Snider, J. R., McMeeking, G. R., Dhaniyala, S., Lewis, E. R., Wentzell, J. J. B., Abbatt, J., Lee, C., Sultana, C. M., Ault, A. P., Axson, J. L., Martinez, M. D., Venero, I., Santos-Figueroa, G., Stokes, M. D., Deane, G. B., Mayol-Bracero, O. L., Grassian, V. H., Bertram, T. H., Bertram, A. K., Moffett, B. F., and Franc, G. D.:
Sea spray aerosol as a unique source of ice nucleating particles, P. Natl. Acad. Sci. USA, 113, 5797–5803,
https://doi.org/10.1073/pnas.1514034112, 2016. a
Deshmukh, A., Phillips, V. T., Bansemer, A., Patade, S., and Waman, D.: New
Empirical Formulation for the Sublimational Breakup of Graupel and Dendritic
Snow, J. Atmos. Sci., 79, 317–336, https://doi.org/10.1175/JAS-D-20-0275.1,
2022. a
Diao, M., Bryan, G. H., Morrison, H., and Jensen, J. B.: Ice nucleation
parameterization and relative humidity distribution in idealized squall-line
simulations, J. Atmos. Sci., 74, 2761–2787,
https://doi.org/10.1175/JAS-D-16-0356.1, 2017. a
European Centre for Medium-Range Weather Forecasts: ERA5 Reanalysis (0.25 Degree Latitude-Longitude Grid), Research Data Archive at the National Center for Atmospheric Research, Computational and Information Systems Laboratory [data set], https://doi.org/10.5065/BH6N-5N20, 2019. a
Field, P., Heymsfield, A., and Bansemer, A.: A test of ice self-collection
kernels using aircraft data, J. Atmos. Sci., 63,
651–666, https://doi.org/10.1175/JAS3653.1, 2006. a
Field, P. R., Cotton, R., Johnson, D., Noone, K., Glantz, P., Kaye, P., Hirst,
E., Greenaway, R., Jost, C., Gabriel, R., Reiner, T., Andreae, M., Saunders, C. P. R., Archer, A., Choularton, T., Smith, M., Brooks, B., Hoell, C., Bandy, B., and Heymsfield, A.: Ice nucleation in
orographic wave clouds: Measurements made during INTACC, Q. J.
Roy. Meteor. Soc., 127, 1493–1512,
https://doi.org/10.1002/qj.49712757502, 2001. a
Field, P. R., Lawson, R. P., Brown, P. R., Lloyd, G., Westbrook, C., Moisseev,
D., Miltenberger, A., Nenes, A., Blyth, A., Choularton, T., Connolly, P. , Buehl, J., Crosier, J., Cui, Z., Dearden, C., DeMott, P., Flossmann, A., Heymsfield, A., Huang, Y., Kalesse, H., Kanji, Z. A., Korolev, A., Kirchgaessner, A., Lasher-Trapp, S., Leisner, T., McFarquhar, G., Phillips, V., Stith, J., and Sullivan, S.: Secondary
ice production: Current state of the science and recommendations for the
future, Meteor. Mon., 58, 7.1–7.20,
https://doi.org/10.1175/AMSMONOGRAPHS-D-16-0014.1, 2017. a, b, c
Franklin, C. N., Protat, A., Leroy, D., and Fontaine, E.: Controls on phase composition and ice water content in a convection-permitting model simulation of a tropical mesoscale convective system, Atmos. Chem. Phys., 16, 8767–8789, https://doi.org/10.5194/acp-16-8767-2016, 2016. a
Fridlind, A. M., Ackerman, A. S., Grandin, A., Dezitter, F., Weber, M., Strapp, J. W., Korolev, A. V., and Williams, C. R.: High ice water content at low radar reflectivity near deep convection – Part 1: Consistency of in situ and remote-sensing observations with stratiform rain column simulations, Atmos. Chem. Phys., 15, 11713–11728, https://doi.org/10.5194/acp-15-11713-2015, 2015. a
Fu, S., Deng, X., Shupe, M. D., and Xue, H.: A modelling study of the
continuous ice formation in an autumnal Arctic mixed-phase cloud case,
Atmos. Res., 228, 77–85, https://doi.org/10.1016/j.atmosres.2019.05.021,
2019. a, b
Hallett, J. and Mossop, S.: Production of secondary ice particles during the
riming process, Nature, 249, 26–28, https://doi.org/10.1038/249026a0, 1974. a, b, c
Heymsfield, A. J. and Mossop, S.: Temperature dependence of secondary ice
crystal production during soft hail growth by riming, Q. J.
Roy. Meteor. Soc., 110, 765–770,
https://doi.org/10.1002/qj.49711046512, 1984. a
Hoarau, T., Pinty, J.-P., and Barthe, C.: A representation of the collisional ice break-up process in the two-moment microphysics LIMA v1.0 scheme of Meso-NH, Geosci. Model Dev., 11, 4269–4289, https://doi.org/10.5194/gmd-11-4269-2018, 2018. a
Hobbs, P. V. and Rangno, A. L.: Ice particle concentrations in clouds, J. Atmos. Sci., 42, 2523–2549,
https://doi.org/10.1175/1520-0469(1985)042<2523:IPCIC>2.0.CO;2, 1985. a
Hu, Y., McFarquhar, G. M., Wu, W., Huang, Y., Schwarzenboeck, A., Protat, A.,
Korolev, A., Rauber, R. M., and Wang, H.: Dependence of Ice Microphysical
Properties On Environmental Parameters: Results from HAIC-HIWC Cayenne Field
Campaign, J. Atmos. Sci., 78, 2957–2981,
https://doi.org/10.1175/JAS-D-21-0015.1, 2021. a, b, c, d
Huang, Y., Wu, W., McFarquhar, G. M., Wang, X., Morrison, H., Ryzhkov, A., Hu, Y., Wolde, M., Nguyen, C., Schwarzenboeck, A., Milbrandt, J., Korolev, A. V., and Heckman, I.: Microphysical processes producing high ice water contents (HIWCs) in tropical convective clouds during the HAIC-HIWC field campaign: evaluation of simulations using bulk microphysical schemes, Atmos. Chem. Phys., 21, 6919–6944, https://doi.org/10.5194/acp-21-6919-2021, 2021. a, b, c, d, e, f, g, h, i, j, k, l, m, n, o, p, q, r, s, t
Jeevanjee, N.: Vertical velocity in the gray zone, J. Adv.
Model. Earth Sy., 9, 2304–2316, https://doi.org/10.1002/2017MS001059, 2017. a
Jiménez, P. A., Dudhia, J., González-Rouco, J. F., Navarro, J.,
Montávez, J. P., and García-Bustamante, E.: A revised scheme for the
WRF surface layer formulation, Mon. Weather Rev., 140, 898–918,
https://doi.org/10.1175/MWR-D-11-00056.1, 2012. a
Keinert, A., Spannagel, D., Leisner, T., and Kiselev, A.: Secondary ice
production upon freezing of freely falling drizzle droplets, J.
Atmos. Sci., 77, 2959–2967, https://doi.org/10.1175/JAS-D-20-0081.1, 2020. a
Kolomeychuk, R., McKay, D., and Iribarne, J.: The fragmentation and
electrification of freezing drops, J. Atmos. Sci., 32,
974–979, https://doi.org/10.1175/1520-0469(1975)032<0974:TFAEOF>2.0.CO;2, 1975. a
Koop, T., Luo, B., Tsias, A., and Peter, T.: Water activity as the determinant
for homogeneous ice nucleation in aqueous solutions, Nature, 406, 611–614,
https://doi.org/10.1038/35020537, 2000. a
Korolev, A. and Field, P. R.: Assessment of the performance of the inter-arrival time algorithm to identify ice shattering artifacts in cloud particle probe measurements, Atmos. Meas. Tech., 8, 761–777, https://doi.org/10.5194/amt-8-761-2015, 2015. a
Korolev, A. and Leisner, T.: Review of experimental studies of secondary ice production, Atmos. Chem. Phys., 20, 11767–11797, https://doi.org/10.5194/acp-20-11767-2020, 2020. a, b, c, d
Korolev, A., Emery, E., and Creelman, K.: Modification and tests of particle
probe tips to mitigate effects of ice shattering, J. Atmos.
Ocean. Tech., 30, 690–708, https://doi.org/10.1175/JTECH-D-12-00142.1,
2013a. a
Korolev, A., Emery, E., Strapp, J., Cober, S., and Isaac, G.: Quantification of
the effects of shattering on airborne ice particle measurements, J.
Atmos. Ocean. Tech., 30, 2527–2553,
https://doi.org/10.1175/JTECH-D-13-00115.1, 2013b. a
Ladino, L. A., Korolev, A., Heckman, I., Wolde, M., Fridlind, A. M., and
Ackerman, A. S.: On the role of ice-nucleating aerosol in the formation of
ice particles in tropical mesoscale convective systems, Geophys. Res.
Lett., 44, 1574–1582, https://doi.org/10.1002/2016GL072455, 2017. a, b, c, d
Langham, E. and Mason, B. J.-N.: The heterogeneous and homogeneous nucleation
of supercooled water, P. R. Soc. Lond. A, 247, 493–504,
https://doi.org/10.1098/rspa.1958.0207, 1958. a
Lauber, A., Kiselev, A., Pander, T., Handmann, P., and Leisner, T.: Secondary
ice formation during freezing of levitated droplets, J.
Atmos. Sci., 75, 2815–2826, https://doi.org/10.1175/JAS-D-18-0052.1, 2018. a, b, c
Lebo, Z. and Morrison, H.: Effects of horizontal and vertical grid spacing on
mixing in simulated squall lines and implications for convective strength and
structure, Mon. Weather Rev., 143, 4355–4375,
https://doi.org/10.1175/MWR-D-15-0154.1, 2015. a, b
Leroy, D., Fontaine, E., Schwarzenboeck, A., and Strapp, J.: Ice crystal sizes
in high ice water content clouds. Part I: On the computation of median mass
diameter from in situ measurements, J. Atmos. Ocean.
Tech., 33, 2461–2476, https://doi.org/10.1175/JTECH-D-15-0151.1, 2016. a
Leroy, D., Fontaine, E., Schwarzenboeck, A., Strapp, J. W., Korolev, A.,
McFarquhar, G., Dupuy, R., Gourbeyre, C., Lilie, L., Protat, A., Delanoe, J., Dezitter, F., and Grandin, A.: Ice
crystal sizes in high ice water content clouds. Part II: Statistics of mass
diameter percentiles in tropical convection observed during the HAIC/HIWC
project, J. Atmos. Ocean. Tech., 34, 117–136,
https://doi.org/10.1175/JTECH-D-15-0246.1, 2017. a
Lloyd, G., Choularton, T. W., Bower, K. N., Gallagher, M. W., Connolly, P. J., Flynn, M., Farrington, R., Crosier, J., Schlenczek, O., Fugal, J., and Henneberger, J.: The origins of ice crystals measured in mixed-phase clouds at the high-alpine site Jungfraujoch, Atmos. Chem. Phys., 15, 12953–12969, https://doi.org/10.5194/acp-15-12953-2015, 2015. a
Luke, E. P., Yang, F., Kollias, P., Vogelmann, A. M., and Maahn, M.: New
insights into ice multiplication using remote-sensing observations of
slightly supercooled mixed-phase clouds in the Arctic, P.
Natl. Acad. Sci. USA, 118, e2021387118, https://doi.org/10.1073/pnas.2021387118, 2021. a
Mason, B. J. and Maybank, J.: The fragmentation and electrification of freezing
water drops, Q. J. Roy. Meteor. Soc., 86,
176–185, https://doi.org/10.1002/qj.49708636806, 1960. a, b
McFarquhar, G. M., Baumgardner, D., Bansemer, A., Abel, S. J., Crosier, J.,
French, J., Rosenberg, P., Korolev, A., Schwarzoenboeck, A., Leroy, D.,
Um, J., Wu, W., Heymsfield, A. J., Twohy, C., Detwiler, A., Field, P., Neumann, A., Cotton, R., Axisa, D., and Dong, J.: Processing of ice cloud in situ data collected by bulk water,
scattering, and imaging probes: fundamentals, uncertainties, and efforts
toward consistency, Meteor. Mon., 58, 11.1–11.33,
https://doi.org/10.1175/AMSMONOGRAPHS-D-16-0007.1, 2017. a
Milbrandt, J. and Morrison, H.: Parameterization of cloud microphysics based on
the prediction of bulk ice particle properties. Part III: Introduction of
multiple free categories, J. Atmos. Sci., 73, 975–995,
https://doi.org/10.1175/JAS-D-15-0204.1, 2016. a, b
Morrison, H.: On the numerical treatment of hydrometeor sedimentation in bulk
and hybrid bulk–bin microphysics schemes, Mon. Weather Rev., 140,
1572–1588, https://doi.org/10.1175/MWR-D-11-00140.1, 2012. a
Morrison, H. and Grabowski, W. W.: An improved representation of rimed snow and
conversion to graupel in a multicomponent bin microphysics scheme, J. Atmos. Sci., 67, 1337–1360, https://doi.org/10.1175/2010JAS3250.1, 2010. a
Morrison, H. and Milbrandt, J. A.: Parameterization of cloud microphysics based
on the prediction of bulk ice particle properties. Part I: Scheme description
and idealized tests, J. Atmos. Sci., 72, 287–311,
https://doi.org/10.1175/JAS-D-14-0065.1, 2015. a, b
Morrison, H., Curry, J., and Khvorostyanov, V.: A new double-moment
microphysics parameterization for application in cloud and climate models.
Part I: Description, J. Atmos. Sci., 62, 1665–1677,
https://doi.org/10.1175/jas3446.1, 2005. a, b
Morrison, H., van Lier-Walqui, M., Fridlind, A. M., Grabowski, W. W.,
Harrington, J. Y., Hoose, C., Korolev, A., Kumjian, M. R., Milbrandt, J. A.,
Pawlowska, H., Posselt, D. J., Prat, O. P., Reimel, K. J., Shima, S., Diedenhoven, B. V., and Xue, L.: Confronting the challenge of modeling cloud and
precipitation microphysics, J. Adv. Model. Earth Sy.,
12, e2019MS001689, https://doi.org/10.1029/2019MS001689, 2020. a
Murgatroyd, R. and Garrod, M.: Observations of precipitation elements in
cumulus clouds, Q. J. Roy. Meteor. Soc., 86,
167–175, https://doi.org/10.1002/qj.49708636805, 1960. a
Naylor, J. and Gilmore, M. S.: Convective initiation in an idealized cloud
model using an updraft nudging technique, Mon. Weather Rev., 140,
3699–3705, https://doi.org/10.1175/MWR-D-12-00163.1, 2012. a
O'Shea, S., Crosier, J., Dorsey, J., Gallagher, L., Schledewitz, W., Bower, K., Schlenczek, O., Borrmann, S., Cotton, R., Westbrook, C., and Ulanowski, Z.: Characterising optical array particle imaging probes: implications for small-ice-crystal observations, Atmos. Meas. Tech., 14, 1917–1939, https://doi.org/10.5194/amt-14-1917-2021, 2021. a
Phillips, V. T., Yano, J.-I., Formenton, M., Ilotoviz, E., Kanawade, V.,
Kudzotsa, I., Sun, J., Bansemer, A., Detwiler, A. G., Khain, A., and Tessendorf, S. A.: Ice
multiplication by breakup in ice–ice collisions. Part II: Numerical
simulations, J. Atmos. Sci., 74, 2789–2811,
https://doi.org/10.1175/JAS-D-16-0223.1, 2017a. a, b, c
Phillips, V. T., Yano, J.-I., and Khain, A.: Ice multiplication by breakup in
ice–ice collisions. Part I: Theoretical formulation, J.
Atmos. Sci., 74, 1705–1719, https://doi.org/10.1175/JAS-D-16-0224.1,
2017b. a, b, c
Protat, A., Delanoë, J., Strapp, J., Fontaine, E., Leroy, D.,
Schwarzenboeck, A., Lilie, L., Davison, C., Dezitter, F., Grandin, A.,
and Weber, M.: The measured relationship between ice water content and cloud radar
reflectivity in tropical convective clouds, J. Appl. Meteorol.
Clim., 55, 1707–1729, https://doi.org/10.1175/JAMC-D-15-0248.1, 2016. a
Pruppacher, H. and Schlamp, R.: A wind tunnel investigation on ice
multiplication by freezing of waterdrops falling at terminal velocity in air,
J. Geophys. Res., 80, 380–386, https://doi.org/10.1029/JC080i003p00380,
1975. a
Qu, Z., Barker, H. W., Korolev, A. V., Milbrandt, J. A., Heckman, I.,
Bélair, S., Leroyer, S., Vaillancourt, P. A., Wolde, M.,
Schwarzenböck, A., Leroy, D., Strapp, J. W., Cole, J. N., Nguyen, L., and Heidinger, A.: Evaluation of a high-resolution numerical
weather prediction model's simulated clouds using observations from CloudSat,
GOES-13 and in situ aircraft, Q. J. Roy. Meteor.
Soc., 144, 1681–1694, https://doi.org/10.1002/qj.3318, 2018. a
Rangno, A. L. and Hobbs, P. V.: Ice particles in stratiform clouds in the
Arctic and possible mechanisms for the production of high ice concentrations,
J. Geophys. Res.-Atmos., 106, 15065–15075,
https://doi.org/10.1029/2000JD900286, 2001. a
Saleeby, S. M. and Cotton, W. R.: A binned approach to cloud-droplet riming
implemented in a bulk microphysics model, J. Appl. Meteorol.
Clim., 47, 694–703, https://doi.org/10.1175/2007JAMC1664.1, 2008. a
Skamarock, W. C., Klemp, J. B., Dudhia, J., Gill, D. O., Liu, Z., Berner, J.,
Wang, W., Powers, J. G., Duda, M. G., Barker, D. M., and Huang, X. Y.: A description of
the advanced research WRF model version 4, National Center for Atmospheric
Research: Boulder, CO, USA, p. 145, https://doi.org/10.5065/1dfh-6p97, 2019. a
Sotiropoulou, G., Sullivan, S., Savre, J., Lloyd, G., Lachlan-Cope, T., Ekman, A. M. L., and Nenes, A.: The impact of secondary ice production on Arctic stratocumulus, Atmos. Chem. Phys., 20, 1301–1316, https://doi.org/10.5194/acp-20-1301-2020, 2020. a, b, c
Sotiropoulou, G., Vignon, É., Young, G., Morrison, H., O'Shea, S. J., Lachlan-Cope, T., Berne, A., and Nenes, A.: Secondary ice production in summer clouds over the Antarctic coast: an underappreciated process in atmospheric models, Atmos. Chem. Phys., 21, 755–771, https://doi.org/10.5194/acp-21-755-2021, 2021. a, b
Stanford, M. W., Varble, A., Zipser, E., Strapp, J. W., Leroy, D., Schwarzenboeck, A., Potts, R., and Protat, A.: A ubiquitous ice size bias in simulations of tropical deep convection, Atmos. Chem. Phys., 17, 9599–9621, https://doi.org/10.5194/acp-17-9599-2017, 2017. a
Strapp, J., Schwarzenboeck, A., Bedka, K., Bond, T., Calmels, A., Delanoë,
J., Dezitter, F., Grzych, M., Harrah, S., Korolev, A., Leroy, D., Lilie, L.,
Mason, J., Potts, R., Protat, A., Ratvasky, T., Riley, J., and Wolde, M.: An
Assessment of Cloud Total Water Content and Particle Size from Flight Test
Campaign Measurements in High Ice Water Content, Mixed Phase/Ice Crystal
Icing Conditions: Primary In-Situ Measurements, Tech. Rep., FAA Rep.
DOT/FAA/TC-18/1,
http://www.tc.faa.gov/its/worldpac/techrpt/tc18-1.pdf (last
access: 20 December 2021), 2020. a
Strapp, J. W., Schwarzenboeck, A., Bedka, K., Bond, T., Calmels, A., Delanoe,
J., Dezitter, F., Grzych, M., Harrah, S., Korolev, A., Leroy, D., Lilie, L., Mason, J., Potts, R., Protat, A., Ratvasky,
T., Riley, J., and Wolde, M.: Comparisons of
Cloud In Situ Microphysical Properties of Deep Convective Clouds to Appendix
D/P Using Data from the High-Altitude Ice Crystals-High Ice Water Content and
High Ice Water Content-RADAR I Flight Campaigns, SAE International Journal of
Aerospace, 14, 127–159, https://doi.org/10.4271/01-14-02-0007, 2021. a
Sullivan, S., Hoose, C., and Nenes, A.: Investigating the contribution of
secondary ice production to in-cloud ice crystal numbers, J.
Geophys. Res.-Atmos., 122, 9391–9412,
https://doi.org/10.1002/2017JD026546, 2017. a
Sullivan, S. C., Barthlott, C., Crosier, J., Zhukov, I., Nenes, A., and Hoose, C.: The effect of secondary ice production parameterization on the simulation of a cold frontal rainband, Atmos. Chem. Phys., 18, 16461–16480, https://doi.org/10.5194/acp-18-16461-2018, 2018a. a, b
Sullivan, S. C., Hoose, C., Kiselev, A., Leisner, T., and Nenes, A.: Initiation of secondary ice production in clouds, Atmos. Chem. Phys., 18, 1593–1610, https://doi.org/10.5194/acp-18-1593-2018, 2018b. a
Takahashi, C.: Deformations of frozen water drops and their frequencies,
J. Meteorol. Soc. Jpn. Ser. II, 53, 402–411,
https://doi.org/10.2151/jmsj1965.53.6_402, 1975.
a
Takahashi, C. and Yamashita, A.: Deformation and fragmentation of freezing
water drops in free fall, J. Meteorol. Soc. Jpn. Ser. II, 47, 431–436, https://doi.org/10.2151/jmsj1965.47.6_431, 1969. a
Takahashi, C. and Yamashita, A.: Shattering of frozen water drops in a
supercooled cloud, J. Meteorol. Soc. Jpn. Ser. II,
48, 373–376, https://doi.org/10.2151/jmsj1965.48.4_373, 1970. a
Takahashi, T., Nagao, Y., and Kushiyama, Y.: Possible high ice particle
production during graupel–graupel collisions, J. Atmos.
Sci., 52, 4523–4527,
https://doi.org/10.1175/1520-0469(1995)052<4523:PHIPPD>2.0.CO;2, 1995. a, b, c
UCAR/NCAR – Earth Observing Laboratory: HAIC-HIWC_2015: High Altitude Ice Crystals, High Ice Water Content Project, UCAR/NCAR [data set], https://data.eol.ucar.edu/master_lists/generated/haic-hiwc_2015 (last access: 26 May 2020), 2015. a
Vardiman, L.: The generation of secondary ice particles in clouds by
crystal–crystal collision, J. Atmos. Sci., 35, 2168–2180,
https://doi.org/10.1175/1520-0469(1978)035<2168:TGOSIP>2.0.CO;2, 1978. a, b
WRF Community: Weather Research and Forecasting (WRF) Model, Version 4.1.3, UCAR/NCAR [code], https://doi.org/10.5065/D6MK6B4K, 2019. a
Zhao, X. and Liu, X.: Global Importance of Secondary Ice Production,
Geophys. Res. Lett., 48, e2021GL092581, https://doi.org/10.1029/2021GL092581,
2021. a
Short summary
Numerous small ice crystals in tropical convective storms are difficult to detect and could be potentially hazardous for commercial aircraft. Previous numerical simulations failed to reproduce this phenomenon and hypothesized that key microphysical processes are still lacking in current models to realistically simulate the phenomenon. This study uses numerical experiments to confirm the dominant role of secondary ice production in the formation of these large numbers of small ice crystals.
Numerous small ice crystals in tropical convective storms are difficult to detect and could be...
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