Articles | Volume 26, issue 19
https://doi.org/10.5194/acp-26-14229-2026
© Author(s) 2026. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-26-14229-2026
© Author(s) 2026. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Light absorption properties and composition of water-soluble brown carbon in North China Plain: implication for an enhancing role of nitrogenous organic compounds
Can Wu
Key Lab of Geographic Information Science of the Ministry of Education, School of Geographic Sciences, East China Normal University, Shanghai 210062, China
Institute of Eco-Chongming, East China Normal University, 3663 North Zhongshan Road, Shanghai 200062, China
Huijun Zhang
Key Lab of Geographic Information Science of the Ministry of Education, School of Geographic Sciences, East China Normal University, Shanghai 210062, China
Kehan Sun
Key Lab of Geographic Information Science of the Ministry of Education, School of Geographic Sciences, East China Normal University, Shanghai 210062, China
Rongjie Li
Key Lab of Geographic Information Science of the Ministry of Education, School of Geographic Sciences, East China Normal University, Shanghai 210062, China
Ziting Yan
Key Lab of Geographic Information Science of the Ministry of Education, School of Geographic Sciences, East China Normal University, Shanghai 210062, China
Yubao Chen
Key Lab of Geographic Information Science of the Ministry of Education, School of Geographic Sciences, East China Normal University, Shanghai 210062, China
Zheng Li
Key Lab of Geographic Information Science of the Ministry of Education, School of Geographic Sciences, East China Normal University, Shanghai 210062, China
Binyu Xiao
Key Lab of Geographic Information Science of the Ministry of Education, School of Geographic Sciences, East China Normal University, Shanghai 210062, China
Yanqin Ren
State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China
Key Lab of Geographic Information Science of the Ministry of Education, School of Geographic Sciences, East China Normal University, Shanghai 210062, China
Institute of Eco-Chongming, East China Normal University, 3663 North Zhongshan Road, Shanghai 200062, China
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Yanqin Ren, Zhenhai Wu, Yuanyuan Ji, Fang Bi, Junling Li, Haijie Zhang, Hao Zhang, Hong Li, and Gehui Wang
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Junke Zhang, Yunfei Su, Chunying Chen, Wenkai Guo, Qinwen Tan, Miao Feng, Danlin Song, Tao Jiang, Qiang Chen, Yuan Li, Wei Li, Yizhi Wang, Xiaojuan Huang, Lin Han, Wanqing Wu, and Gehui Wang
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Yanqin Ren, Gehui Wang, Jie Wei, Jun Tao, Zhisheng Zhang, and Hong Li
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Rui Li, Yining Gao, Yubao Chen, Meng Peng, Weidong Zhao, Gehui Wang, and Jiming Hao
Atmos. Chem. Phys., 23, 4709–4726, https://doi.org/10.5194/acp-23-4709-2023, https://doi.org/10.5194/acp-23-4709-2023, 2023
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A random forest model was used to isolate the effects of emission and meteorology to trace elements in PM2.5 in Tangshan. The results suggested that control measures facilitated decreases of Ga, Co, Pb, Zn, and As, due to the strict implementation of coal-to-gas strategies and optimisation of industrial structure and layout. However, the deweathered levels of Ca, Cr, and Fe only displayed minor decreases, indicating that ferrous metal smelting and vehicle emission controls should be enhanced.
Can Wu, Cong Cao, Jianjun Li, Shaojun Lv, Jin Li, Xiaodi Liu, Si Zhang, Shijie Liu, Fan Zhang, Jingjing Meng, and Gehui Wang
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Over the past decade, the relative abundance of NH4NO3 in aerosol has been enhanced in most urban areas of China, which profoundly affects the PM2.5 pollution episodes. Our work finds that fine-particle nitrate and ammonium exhibited distinct, different physicochemical behaviors in the aerosol aging process.
Junling Li, Kun Li, Hao Zhang, Xin Zhang, Yuanyuan Ji, Wanghui Chu, Yuxue Kong, Yangxi Chu, Yanqin Ren, Yujie Zhang, Haijie Zhang, Rui Gao, Zhenhai Wu, Fang Bi, Xuan Chen, Xuezhong Wang, Weigang Wang, Hong Li, and Maofa Ge
Atmos. Chem. Phys., 22, 10489–10504, https://doi.org/10.5194/acp-22-10489-2022, https://doi.org/10.5194/acp-22-10489-2022, 2022
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Ozone formation is enhanced by higher OH concentration and higher temperature but is influenced little by SO2. SO2 can largely enhance the particle formation. Organo-sulfates and organo-nitrates are detected in the formed particles, and the presence of SO2 can promote the formation of organo-sulfates. The results provide a scientific basis for systematically evaluating the effects of SO2, OH concentration, and temperature on the oxidation of mixed organic gases in the atmosphere.
Shijie Liu, Dandan Huang, Yiqian Wang, Si Zhang, Xiaodi Liu, Can Wu, Wei Du, and Gehui Wang
Atmos. Chem. Phys., 21, 17759–17773, https://doi.org/10.5194/acp-21-17759-2021, https://doi.org/10.5194/acp-21-17759-2021, 2021
Short summary
Short summary
A series of chamber experiments was performed to probe the individual and common effects of NH3 and NOx on toluene secondary organic aerosol (SOA) formation through OH photooxidation. The synergetic effects of NH3 and NOx on the toluene SOA concentration and optical absorption were observed. The higher-volatility products formed in the presence of NOx could precipitate into the particle phase when NH3 was added. The formation pathways of N-containing OAs through NOx or NH3 are also discussed.
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Cao, T., Li, M., Zou, C., Fan, X., Song, J., Jia, W., Yu, C., Yu, Z., and Peng, P.: Chemical composition, optical properties, and oxidative potential of water- and methanol-soluble organic compounds emitted from the combustion of biomass materials and coal, Atmos. Chem. Phys., 21, 13187–13205, https://doi.org/10.5194/acp-21-13187-2021, 2021.
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Short summary
Nitrogenous organic compounds represent the pivotal chromophores governing the optical properties of atmospheric brown carbon (BrC) across the North China Plain, which are mainly formed through ammonia-driven aqueous reactions. Accordingly, the mitigation of ammonia emissions is indispensable for the further abatement of haze and BrC pollution in this region.
Nitrogenous organic compounds represent the pivotal chromophores governing the optical...
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