Articles | Volume 24, issue 24
https://doi.org/10.5194/acp-24-13975-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-24-13975-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
17 Dec 2024
Research article |
| 17 Dec 2024
| 17 Dec 2024
Seasonal, regional, and vertical characteristics of high-carbon-monoxide plumes along with their associated ozone anomalies, as seen by IAGOS between 2002 and 2019
Thibaut Lebourgeois
CORRESPONDING AUTHOR
Laboratoire d'Aérologie, Université de Toulouse, CNRS, UPS, Toulouse, France
CNRM, Météo-France, Université de Toulouse, CNRS, Toulouse, France
Bastien Sauvage
Laboratoire d'Aérologie, Université de Toulouse, CNRS, UPS, Toulouse, France
Pawel Wolff
Observatoire Midi-Pyrénées, Université de Toulouse, CNRS, UPS, 31400 Toulouse, France
Béatrice Josse
CNRM, Météo-France, Université de Toulouse, CNRS, Toulouse, France
Virginie Marécal
CNRM, Météo-France, Université de Toulouse, CNRS, Toulouse, France
Yasmine Bennouna
Laboratoire d'Aérologie, Université de Toulouse, CNRS, UPS, Toulouse, France
Romain Blot
Laboratoire d'Aérologie, Université de Toulouse, CNRS, UPS, Toulouse, France
Damien Boulanger
Observatoire Midi-Pyrénées, Université de Toulouse, CNRS, UPS, 31400 Toulouse, France
Hannah Clark
IAGOS-AISBL, 98 Rue du Trône, Brussels, Belgium
Jean-Marc Cousin
Laboratoire d'Aérologie, Université de Toulouse, CNRS, UPS, Toulouse, France
Philippe Nedelec
Laboratoire d'Aérologie, Université de Toulouse, CNRS, UPS, Toulouse, France
Valérie Thouret
Laboratoire d'Aérologie, Université de Toulouse, CNRS, UPS, Toulouse, France
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Anne M. Thompson, Ryan M. Stauffer, Debra E. Kollonige, Jerald R. Ziemke, Bryan J. Johnson, Gary A. Morris, Patrick Cullis, María Cazorla, Jorge Andres Diaz, Ankie Piters, Igor Nedeljkovic, Truus Warsodikromo, Francisco Raimundo Silva, E. Thomas Northam, Patrick Benjamin, Thumeka Mkololo, Tshidi Machinini, Christian Félix, Gonzague Romanens, Syprose Nyadida, Jérôme Brioude, Stéphanie Evan, Jean-Marc Metzger, Ambun Dindang, Yuzaimi B. Mahat, Mohan Kumar Sammathuria, Norazura Binti Zakaria, Ninong Komala, Shin-Ya Ogino, Nguyen Thi Quyen, Francis S. Mani, Miriama Vuiyasawa, David Nardini, Matthew Martinsen, Darryl T. Kuniyuki, Katrin Müller, Pawel Wolff, and Bastien Sauvage
Atmos. Chem. Phys., 25, 18475–18507, https://doi.org/10.5194/acp-25-18475-2025, https://doi.org/10.5194/acp-25-18475-2025, 2025
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Ozone profile trends from SHADOZ sondes and IAGOS aircraft show that ozone in the tropical free troposphere (FT) is not growing fast except over equatorial SE Asia. This agrees with HEGIFTOM (Van Malderen et al., 2025), Stauffer et al. (2024) and Gaudel et al. (2024) TOAR-II papers. Other findings are as follows: (1) our trends are independent of method (QR, MLR) and (2) sample number (SN) (i.e., SHADOZ sampling is sufficient), and (3) all ground-based trends constitute the gold standard for satellite-derived trends.
Sergey Khaykin, Slimane Bekki, Sophie Godin-Beekmann, Michael D. Fromm, Philippe Goloub, Qiaoyun Hu, Béatrice Josse, Alexandra Laeng, Mehdi Meziane, David A. Peterson, Sophie Pelletier, and Valérie Thouret
Atmos. Chem. Phys., 25, 14551–14571, https://doi.org/10.5194/acp-25-14551-2025, https://doi.org/10.5194/acp-25-14551-2025, 2025
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In 2023, massive wildfires in Canada injected huge amounts of smoke into the atmosphere. Surprisingly, despite their intensity, the smoke did not rise very high but lingered at flight cruising altitudes, causing widespread pollution. This study shows how two different pathways lifted smoke into the lower stratosphere and reveals new insights into how wildfires affect air quality and climate, challenging what we thought we knew about fire and atmospheric impacts.
Pasquale Sellitto, Audrey Gaudel, and Bastien Sauvage
Atmos. Chem. Phys., 25, 13299–13309, https://doi.org/10.5194/acp-25-13299-2025, https://doi.org/10.5194/acp-25-13299-2025, 2025
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Tropospheric ozone is a potent greenhouse gas: its anthropogenic levels rise contributes to climate change. We evaluate tropospheric ozone trends and climate impacts with aircraft data and a radiative model, comparing a baseline period (1994–2004) to different recent time periods (2011–2016 to 2020-2023). Tropospheric ozone levels increasing trends progressively stopped and even decreased in the upper troposphere. Correspondingly, the decadal ozone radiative forcing is progressively decreasing.
Eric Martial Yao, Fabien Solmon, Marcellin Adon, Claire Delon, Corinne Galy-Lacaux, Graziano Giuliani, Bastien Sauvage, and Véronique Yoboue
Atmos. Chem. Phys., 25, 12101–12136, https://doi.org/10.5194/acp-25-12101-2025, https://doi.org/10.5194/acp-25-12101-2025, 2025
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As climate change and human activities intensify in Africa, understanding how air pollution, climate, and natural cycles interact is crucial. This study explores how nitrogen oxide emissions from African soils, especially in dry regions, contribute to atmospheric pollution. By using a climate-chemistry model, we show that considering these emissions improves predictions of nitrogen dioxide, nitric acid and ozone, although some discrepancies remain compared to observations.
Paul D. Hamer, Miha Markelj, Oscar Rojas-Munoz, Bertrand Bonan, Jean-Christophe Calvet, Virginie Marécal, Alex Guenther, Heidi Trimmel, Islen Vallejo, Sabine Eckhardt, Gabriela Sousa Santos, Katerina Sindelarova, David Simpson, Norbert Schmidbauer, and Leonor Tarrasón
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2025-442, https://doi.org/10.5194/essd-2025-442, 2025
Preprint under review for ESSD
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Plants release gases like isoprene that can form ozone and affect air quality. Using models and satellite data, we mapped the emissions of isoprene from plants across Europe and found that droughts can reduce leaf growth, leading to lower emissions. This shows that to understand and predict air quality, we must also understand how drought impacts vegetation. Our findings highlight the value of linking extreme weather, plant health, and pollution in models of the Earth system as a whole.
Herman G. J. Smit, Torben Galle, Romain Blot, Florian Obersteiner, Philippe Nédélec, Andreas Zahn, Jean-Marc Cousin, Ulrich Bundke, Andreas Petzold, Valerie Thouret, and Hannah Clark
Atmos. Meas. Tech., 18, 4985–5001, https://doi.org/10.5194/amt-18-4985-2025, https://doi.org/10.5194/amt-18-4985-2025, 2025
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The two ozone instruments of IAGOS (In-service Aircraft for a Global Observation System) have been compared with the Ozone PhotoMeter (OPM) of the World Calibration Center of Ozone Sondes (WCCOS) in an atmospheric simulation chamber under realistic flight conditions of pressure, temperature, and ozone concentrations. The two IAGOS-instruments showed good agreement with the OPM within 5–6 %. The observed differences are small but systematic and reproducible during the intercomparison.
Roeland Van Malderen, Zhou Zang, Kai-Lan Chang, Robin Björklund, Owen R. Cooper, Jane Liu, Eliane Maillard Barras, Corinne Vigouroux, Irina Petropavlovskikh, Thierry Leblanc, Valérie Thouret, Pawel Wolff, Peter Effertz, Audrey Gaudel, David W. Tarasick, Herman G. J. Smit, Anne M. Thompson, Ryan M. Stauffer, Debra E. Kollonige, Deniz Poyraz, Gérard Ancellet, Marie-Renée De Backer, Matthias M. Frey, James W. Hannigan, José L. Hernandez, Bryan J. Johnson, Nicholas Jones, Rigel Kivi, Emmanuel Mahieu, Isamu Morino, Glen McConville, Katrin Müller, Isao Murata, Justus Notholt, Ankie Piters, Maxime Prignon, Richard Querel, Vincenzo Rizi, Dan Smale, Wolfgang Steinbrecht, Kimberly Strong, and Ralf Sussmann
Atmos. Chem. Phys., 25, 9905–9935, https://doi.org/10.5194/acp-25-9905-2025, https://doi.org/10.5194/acp-25-9905-2025, 2025
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Tropospheric ozone is an important greenhouse gas and an air pollutant whose distribution and time variability are mainly governed by anthropogenic emissions and dynamics. In this paper, we assess regional trends of tropospheric ozone column amounts, based on two different approaches of merging or synthesizing ground-based observations and their trends within specific regions. Our findings clearly demonstrate regional trend differences but also consistently higher pre-COVID than post-COVID trends.
Xiao Lu, Yiming Liu, Jiayin Su, Xiang Weng, Tabish Ansari, Yuqiang Zhang, Guowen He, Yuqi Zhu, Haolin Wang, Ganquan Zeng, Jingyu Li, Cheng He, Shuai Li, Teerachai Amnuaylojaroen, Tim Butler, Qi Fan, Shaojia Fan, Grant L. Forster, Meng Gao, Jianlin Hu, Yugo Kanaya, Mohd Talib Latif, Keding Lu, Philippe Nédélec, Peer Nowack, Bastien Sauvage, Xiaobin Xu, Lin Zhang, Ke Li, Ja-Ho Koo, and Tatsuya Nagashima
Atmos. Chem. Phys., 25, 7991–8028, https://doi.org/10.5194/acp-25-7991-2025, https://doi.org/10.5194/acp-25-7991-2025, 2025
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This study analyzes summertime ozone trends in East and Southeast Asia derived from a comprehensive observational database spanning from 1995 to 2019, incorporating aircraft observations, ozonesonde data, and measurements from 2500 surface sites. Multiple models are applied to attribute to changes in anthropogenic emissions and climate. The results highlight that increases in anthropogenic emissions are the primary driver of ozone increases both in the free troposphere and at the surface.
Nana Wei, Eloise A. Marais, Gongda Lu, Robert G. Ryan, and Bastien Sauvage
Atmos. Chem. Phys., 25, 7925–7940, https://doi.org/10.5194/acp-25-7925-2025, https://doi.org/10.5194/acp-25-7925-2025, 2025
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This study uses reactive nitrogen observations from NASA DC-8 research aircraft and the In-service Aircraft for a Global Observing System (IAGOS) campaigns to characterize reactive nitrogen seasonality and composition in the global upper troposphere and to diagnose the greatest knowledge gaps from comparison to a state-of-the-science model, GEOS-Chem, that need to be resolved for climate, nitrogen cycle, and air pollution assessments.
Roeland Van Malderen, Anne M. Thompson, Debra E. Kollonige, Ryan M. Stauffer, Herman G. J. Smit, Eliane Maillard Barras, Corinne Vigouroux, Irina Petropavlovskikh, Thierry Leblanc, Valérie Thouret, Pawel Wolff, Peter Effertz, David W. Tarasick, Deniz Poyraz, Gérard Ancellet, Marie-Renée De Backer, Stéphanie Evan, Victoria Flood, Matthias M. Frey, James W. Hannigan, José L. Hernandez, Marco Iarlori, Bryan J. Johnson, Nicholas Jones, Rigel Kivi, Emmanuel Mahieu, Glen McConville, Katrin Müller, Tomoo Nagahama, Justus Notholt, Ankie Piters, Natalia Prats, Richard Querel, Dan Smale, Wolfgang Steinbrecht, Kimberly Strong, and Ralf Sussmann
Atmos. Chem. Phys., 25, 7187–7225, https://doi.org/10.5194/acp-25-7187-2025, https://doi.org/10.5194/acp-25-7187-2025, 2025
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Tropospheric ozone is an important greenhouse gas and is an air pollutant. The time variability of tropospheric ozone is mainly driven by anthropogenic emissions. In this paper, we study the distribution and time variability of ozone from harmonized ground-based observations from five different measurement techniques. Our findings provide clear standard references for atmospheric models and evolving tropospheric ozone satellite data for the 2000–2022 period.
Yann Cohen, Didier Hauglustaine, Nicolas Bellouin, Marianne Tronstad Lund, Sigrun Matthes, Agnieszka Skowron, Robin Thor, Ulrich Bundke, Andreas Petzold, Susanne Rohs, Valérie Thouret, Andreas Zahn, and Helmut Ziereis
Atmos. Chem. Phys., 25, 5793–5836, https://doi.org/10.5194/acp-25-5793-2025, https://doi.org/10.5194/acp-25-5793-2025, 2025
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The chemical composition of the atmosphere near the tropopause is a key parameter for evaluating the climate impact of subsonic aviation pollutants. This study uses in situ data collected aboard passenger aircraft to assess the ability of four chemistry–climate models to reproduce (bi-)decadal climatologies of ozone, carbon monoxide, water vapour, and reactive nitrogen in this region. The models reproduce the very distinct ozone seasonality in the upper troposphere and in the lower stratosphere well.
Martin Cussac, Martine Michou, Pierre Nabat, Béatrice Josse, and Sophie Pelletier
EGUsphere, https://doi.org/10.5194/egusphere-2025-1933, https://doi.org/10.5194/egusphere-2025-1933, 2025
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This study evaluates three chemistry schemes of varying complexity, one mainly stratospheric and two tropospheric-stratospheric, in the latest version of the climate model ARPEGE-Climat. Stratospheric ozone and water vapour are better represented. Despite issues with carbon monoxide in one scheme and with winter nitrogen species in the other, tropospheric ozone is overall realistically simulated. These modelling evolutions strengthen future research on chemistry-climate interactions.
Brice Barret, Pierre Loicq, Eric Le Flochmoën, Yasmine Bennouna, Juliette Hadji-Lazaro, Daniel Hurtmans, and Bastien Sauvage
Atmos. Meas. Tech., 18, 129–149, https://doi.org/10.5194/amt-18-129-2025, https://doi.org/10.5194/amt-18-129-2025, 2025
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Profiles of carbon monoxide (CO) retrieved from the Infrared Atmospheric Sounding Interferometer (IASI) with the SOftware for a Fast Retrieval of IASI Data (SOFRID) and Fast Optimal Retrievals on Layers for IASI (FORLI) are validated with 8500 observations at 33 airports from the In-service Aircraft for a Global Observing System (IAGOS) for 2008–2019. IASI retrievals underestimate CO, with stronger bias in the middle to upper troposphere for SOFRID and in the lower troposphere for FORLI.
Fang Li, Xiang Song, Sandy P. Harrison, Jennifer R. Marlon, Zhongda Lin, L. Ruby Leung, Jörg Schwinger, Virginie Marécal, Shiyu Wang, Daniel S. Ward, Xiao Dong, Hanna Lee, Lars Nieradzik, Sam S. Rabin, and Roland Séférian
Geosci. Model Dev., 17, 8751–8771, https://doi.org/10.5194/gmd-17-8751-2024, https://doi.org/10.5194/gmd-17-8751-2024, 2024
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This study provides the first comprehensive assessment of historical fire simulations from 19 Earth system models in phase 6 of the Coupled Model Intercomparison Project (CMIP6). Most models reproduce global totals, spatial patterns, seasonality, and regional historical changes well but fail to simulate the recent decline in global burned area and underestimate the fire response to climate variability. CMIP6 simulations address three critical issues of phase-5 models.
Gérard Ancellet, Camille Viatte, Anne Boynard, François Ravetta, Jacques Pelon, Cristelle Cailteau-Fischbach, Pascal Genau, Julie Capo, Axel Roy, and Philippe Nédélec
Atmos. Chem. Phys., 24, 12963–12983, https://doi.org/10.5194/acp-24-12963-2024, https://doi.org/10.5194/acp-24-12963-2024, 2024
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Characterization of ozone pollution in urban areas benefited from a measurement campaign in summer 2022 in the Paris region. The analysis is based on 21 d of lidar and aircraft observations. The main objective is an analysis of the sensitivity of ozone pollution to the micrometeorological processes in the urban atmospheric boundary layer and the transport of regional pollution. The paper also discusses to what extent satellite observations can track observed ozone plumes.
Marie Lothon, François Gheusi, Fabienne Lohou, Véronique Pont, Serge Soula, Corinne Jambert, Solène Derrien, Yannick Bezombes, Emmanuel Leclerc, Gilles Athier, Antoine Vial, Alban Philibert, Bernard Campistron, Frédérique Saïd, Jeroen Sonke, Julien Amestoy, Erwan Bargain, Pierre Bosser, Damien Boulanger, Guillaume Bret, Renaud Bodichon, Laurent Cabanas, Guylaine Canut, Jean-Bernard Estrampes, Eric Gardrat, Zaida Gomez Kuri, Jérémy Gueffier, Fabienne Guesdon, Morgan Lopez, Olivier Masson, Pierre-Yves Meslin, Yves Meyerfeld, Nicolas Pascal, Eric Pique, Michel Ramonet, Felix Starck, and Romain Vidal
Atmos. Meas. Tech., 17, 6265–6300, https://doi.org/10.5194/amt-17-6265-2024, https://doi.org/10.5194/amt-17-6265-2024, 2024
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The Pyrenean Platform for Observation of the Atmosphere (P2OA) is a coupled plain–mountain instrumented platform in southwestern France for the monitoring of climate variables and the study of meteorological processes in a mountainous region. A comprehensive description of this platform is presented for the first time: its instrumentation, the associated dataset, and a meteorological characterization the site. The potential of the P2OA is illustrated through several examples of process studies.
Honglei Wang, David W. Tarasick, Jane Liu, Herman G. J. Smit, Roeland Van Malderen, Lijuan Shen, Romain Blot, and Tianliang Zhao
Atmos. Chem. Phys., 24, 11927–11942, https://doi.org/10.5194/acp-24-11927-2024, https://doi.org/10.5194/acp-24-11927-2024, 2024
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In this study, we identify 23 suitable pairs of sites from World Ozone and Ultraviolet Radiation Data Centre (WOUDC) and In-service Aircraft for a Global Observing System (IAGOS) datasets (1995 to 2021), compare the average vertical distributions of tropospheric O3 from ozonesonde and aircraft measurements, and analyze the differences based on ozonesonde type and station–airport distance.
Audrey Gaudel, Ilann Bourgeois, Meng Li, Kai-Lan Chang, Jerald Ziemke, Bastien Sauvage, Ryan M. Stauffer, Anne M. Thompson, Debra E. Kollonige, Nadia Smith, Daan Hubert, Arno Keppens, Juan Cuesta, Klaus-Peter Heue, Pepijn Veefkind, Kenneth Aikin, Jeff Peischl, Chelsea R. Thompson, Thomas B. Ryerson, Gregory J. Frost, Brian C. McDonald, and Owen R. Cooper
Atmos. Chem. Phys., 24, 9975–10000, https://doi.org/10.5194/acp-24-9975-2024, https://doi.org/10.5194/acp-24-9975-2024, 2024
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The study examines tropical tropospheric ozone changes. In situ data from 1994–2019 display increased ozone, notably over India, Southeast Asia, and Malaysia and Indonesia. Sparse in situ data limit trend detection for the 15-year period. In situ and satellite data, with limited sampling, struggle to consistently detect trends. Continuous observations are vital over the tropical Pacific Ocean, Indian Ocean, western Africa, and South Asia for accurate ozone trend estimation in these regions.
Henk Eskes, Athanasios Tsikerdekis, Melanie Ades, Mihai Alexe, Anna Carlin Benedictow, Yasmine Bennouna, Lewis Blake, Idir Bouarar, Simon Chabrillat, Richard Engelen, Quentin Errera, Johannes Flemming, Sebastien Garrigues, Jan Griesfeller, Vincent Huijnen, Luka Ilić, Antje Inness, John Kapsomenakis, Zak Kipling, Bavo Langerock, Augustin Mortier, Mark Parrington, Isabelle Pison, Mikko Pitkänen, Samuel Remy, Andreas Richter, Anja Schoenhardt, Michael Schulz, Valerie Thouret, Thorsten Warneke, Christos Zerefos, and Vincent-Henri Peuch
Atmos. Chem. Phys., 24, 9475–9514, https://doi.org/10.5194/acp-24-9475-2024, https://doi.org/10.5194/acp-24-9475-2024, 2024
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The Copernicus Atmosphere Monitoring Service (CAMS) provides global analyses and forecasts of aerosols and trace gases in the atmosphere. On 27 June 2023 a major upgrade, Cy48R1, became operational. Comparisons with in situ, surface remote sensing, aircraft, and balloon and satellite observations show that the new CAMS system is a significant improvement. The results quantify the skill of CAMS to forecast impactful events, such as wildfires, dust storms and air pollution peaks.
Kuo-Ying Wang, Philippe Nedelec, Valerie Thouret, Hannah Clark, Andreas Wahner, and Andreas Petzold
EGUsphere, https://doi.org/10.5194/egusphere-2024-2414, https://doi.org/10.5194/egusphere-2024-2414, 2024
Preprint archived
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We use routine in-service commercial passenger airplanes Airbus A340 and A330 to collect air pollutants in the upper troposphere. The beauty in using commercial airplanes is that these commercial airplanes, like taxi on the ground, keep flying all the time. We find that short-lived air pollutants are very sensitive to ground-level emissions. Effective regulation in ground-level emissions can help to reduce air pollution in the upper troposphere.
Andreas Petzold, Ulrich Bundke, Anca Hienola, Paolo Laj, Cathrine Lund Myhre, Alex Vermeulen, Angeliki Adamaki, Werner Kutsch, Valerie Thouret, Damien Boulanger, Markus Fiebig, Markus Stocker, Zhiming Zhao, and Ari Asmi
Atmos. Chem. Phys., 24, 5369–5388, https://doi.org/10.5194/acp-24-5369-2024, https://doi.org/10.5194/acp-24-5369-2024, 2024
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Easy and fast access to long-term and high-quality observational data is recognised as fundamental to environmental research and the development of climate forecasting and assessment services. We discuss the potential new directions in atmospheric sciences offered by the atmosphere-centric European research infrastructures ACTRIS, IAGOS, and ICOS, building on their capabilities for standardised provision of data through open access combined with tools and methods of data-intensive science.
Yann Cohen, Didier Hauglustaine, Bastien Sauvage, Susanne Rohs, Patrick Konjari, Ulrich Bundke, Andreas Petzold, Valérie Thouret, Andreas Zahn, and Helmut Ziereis
Atmos. Chem. Phys., 23, 14973–15009, https://doi.org/10.5194/acp-23-14973-2023, https://doi.org/10.5194/acp-23-14973-2023, 2023
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The upper troposphere–lower stratosphere (UTLS) is a key region regarding the lower atmospheric composition. This study consists of a comprehensive evaluation of an up-to-date chemistry–climate model in this layer, using regular in situ measurements based on passenger aircraft. For this purpose, a specific software (Interpol-IAGOS) has been updated and made publicly available. The model reproduces the carbon monoxide peaks due to biomass burning over the continental tropics particularly well.
Maria Tsivlidou, Bastien Sauvage, Yasmine Bennouna, Romain Blot, Damien Boulanger, Hannah Clark, Eric Le Flochmoën, Philippe Nédélec, Valérie Thouret, Pawel Wolff, and Brice Barret
Atmos. Chem. Phys., 23, 14039–14063, https://doi.org/10.5194/acp-23-14039-2023, https://doi.org/10.5194/acp-23-14039-2023, 2023
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The tropics are a region where the ozone increase has been most apparent since 1980 and where observations are sparse. Using aircraft, satellite, and model data, we document the characteristics of tropospheric ozone and CO over the whole tropics for the last 2 decades. We explore the origin of the observed CO anomalies and investigate transport processes driving the tropical CO and O3 distribution. Our study highlights the importance of anthropogenic emissions, mostly over the northern tropics.
Herizo Narivelo, Paul David Hamer, Virginie Marécal, Luke Surl, Tjarda Roberts, Sophie Pelletier, Béatrice Josse, Jonathan Guth, Mickaël Bacles, Simon Warnach, Thomas Wagner, Stefano Corradini, Giuseppe Salerno, and Lorenzo Guerrieri
Atmos. Chem. Phys., 23, 10533–10561, https://doi.org/10.5194/acp-23-10533-2023, https://doi.org/10.5194/acp-23-10533-2023, 2023
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Volcanic emissions emit large quantities of gases and primary aerosols that can play an important role in atmospheric chemistry. We present a study of the fate of volcanic bromine emissions from the eruption of Mount Etna around Christmas 2018. Using a numerical model and satellite observations, we analyse the impact of the volcanic plume and how it modifies the composition of the air over the whole Mediterranean basin, in particular on tropospheric ozone through the bromine-explosion cycle.
Marina Friedel, Gabriel Chiodo, Timofei Sukhodolov, James Keeble, Thomas Peter, Svenja Seeber, Andrea Stenke, Hideharu Akiyoshi, Eugene Rozanov, David Plummer, Patrick Jöckel, Guang Zeng, Olaf Morgenstern, and Béatrice Josse
Atmos. Chem. Phys., 23, 10235–10254, https://doi.org/10.5194/acp-23-10235-2023, https://doi.org/10.5194/acp-23-10235-2023, 2023
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Previously, it has been suggested that springtime Arctic ozone depletion might worsen in the coming decades due to climate change, which might counteract the effect of reduced ozone-depleting substances. Here, we show with different chemistry–climate models that springtime Arctic ozone depletion will likely decrease in the future. Further, we explain why models show a large spread in the projected development of Arctic ozone depletion and use the model spread to constrain future projections.
Marie Dumont, Simon Gascoin, Marion Réveillet, Didier Voisin, François Tuzet, Laurent Arnaud, Mylène Bonnefoy, Montse Bacardit Peñarroya, Carlo Carmagnola, Alexandre Deguine, Aurélie Diacre, Lukas Dürr, Olivier Evrard, Firmin Fontaine, Amaury Frankl, Mathieu Fructus, Laure Gandois, Isabelle Gouttevin, Abdelfateh Gherab, Pascal Hagenmuller, Sophia Hansson, Hervé Herbin, Béatrice Josse, Bruno Jourdain, Irene Lefevre, Gaël Le Roux, Quentin Libois, Lucie Liger, Samuel Morin, Denis Petitprez, Alvaro Robledano, Martin Schneebeli, Pascal Salze, Delphine Six, Emmanuel Thibert, Jürg Trachsel, Matthieu Vernay, Léo Viallon-Galinier, and Céline Voiron
Earth Syst. Sci. Data, 15, 3075–3094, https://doi.org/10.5194/essd-15-3075-2023, https://doi.org/10.5194/essd-15-3075-2023, 2023
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Saharan dust outbreaks have profound effects on ecosystems, climate, health, and the cryosphere, but the spatial deposition pattern of Saharan dust is poorly known. Following the extreme dust deposition event of February 2021 across Europe, a citizen science campaign was launched to sample dust on snow over the Pyrenees and the European Alps. This campaign triggered wide interest and over 100 samples. The samples revealed the high variability of the dust properties within a single event.
Virginie Marécal, Ronan Voisin-Plessis, Tjarda Jane Roberts, Alessandro Aiuppa, Herizo Narivelo, Paul David Hamer, Béatrice Josse, Jonathan Guth, Luke Surl, and Lisa Grellier
Geosci. Model Dev., 16, 2873–2898, https://doi.org/10.5194/gmd-16-2873-2023, https://doi.org/10.5194/gmd-16-2873-2023, 2023
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We implemented a halogen volcanic chemistry scheme in a one-dimensional modelling framework preparing for further use in a three-dimensional global chemistry-transport model. The results of the simulations for an eruption of Mt Etna in 2008, including various sensitivity tests, show a good consistency with previous modelling studies.
Clément Narbaud, Jean-Daniel Paris, Sophie Wittig, Antoine Berchet, Marielle Saunois, Philippe Nédélec, Boris D. Belan, Mikhail Y. Arshinov, Sergei B. Belan, Denis Davydov, Alexander Fofonov, and Artem Kozlov
Atmos. Chem. Phys., 23, 2293–2314, https://doi.org/10.5194/acp-23-2293-2023, https://doi.org/10.5194/acp-23-2293-2023, 2023
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We measured CH4 and CO2 from aircraft over the Russian Arctic. Analyzing our data with the Lagrangian model FLEXPART, we find a sharp east–west gradient in atmospheric composition. Western Siberia is influenced by strong wetland CH4 emissions, deep CO2 gradient from biospheric uptake, and long-range transport from Europe and North America. Eastern flights document less variability. Over the Arctic Ocean, we find a small influence from marine CH4 emissions compatible with reasonable inventories.
Antje Inness, Ilse Aben, Melanie Ades, Tobias Borsdorff, Johannes Flemming, Luke Jones, Jochen Landgraf, Bavo Langerock, Philippe Nedelec, Mark Parrington, and Roberto Ribas
Atmos. Chem. Phys., 22, 14355–14376, https://doi.org/10.5194/acp-22-14355-2022, https://doi.org/10.5194/acp-22-14355-2022, 2022
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The Copernicus Atmosphere Monitoring Service (CAMS) provides daily global air quality forecasts to users worldwide. One of the species of interest is carbon monoxide (CO), an important trace gas in the atmosphere with anthropogenic and natural sources, produced by incomplete combustion, for example, by wildfires. This paper looks at how well CAMS can model CO in the atmosphere and shows that the fields can be improved when blending CO data from the TROPOMI instrument with the CAMS model.
Haolin Wang, Xiao Lu, Daniel J. Jacob, Owen R. Cooper, Kai-Lan Chang, Ke Li, Meng Gao, Yiming Liu, Bosi Sheng, Kai Wu, Tongwen Wu, Jie Zhang, Bastien Sauvage, Philippe Nédélec, Romain Blot, and Shaojia Fan
Atmos. Chem. Phys., 22, 13753–13782, https://doi.org/10.5194/acp-22-13753-2022, https://doi.org/10.5194/acp-22-13753-2022, 2022
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We report significant global tropospheric ozone increases in 1995–2017 based on extensive aircraft and ozonesonde observations. Using GEOS-Chem (Goddard Earth Observing System chemistry model) multi-decadal global simulations, we find that changes in global anthropogenic emissions, in particular the rapid increases in aircraft emissions, contribute significantly to the increases in tropospheric ozone and resulting radiative impact.
Boris D. Belan, Gerard Ancellet, Irina S. Andreeva, Pavel N. Antokhin, Viktoria G. Arshinova, Mikhail Y. Arshinov, Yurii S. Balin, Vladimir E. Barsuk, Sergei B. Belan, Dmitry G. Chernov, Denis K. Davydov, Alexander V. Fofonov, Georgii A. Ivlev, Sergei N. Kotel'nikov, Alexander S. Kozlov, Artem V. Kozlov, Katharine Law, Andrey V. Mikhal'chishin, Igor A. Moseikin, Sergei V. Nasonov, Philippe Nédélec, Olesya V. Okhlopkova, Sergei E. Ol'kin, Mikhail V. Panchenko, Jean-Daniel Paris, Iogannes E. Penner, Igor V. Ptashnik, Tatyana M. Rasskazchikova, Irina K. Reznikova, Oleg A. Romanovskii, Alexander S. Safatov, Denis E. Savkin, Denis V. Simonenkov, Tatyana K. Sklyadneva, Gennadii N. Tolmachev, Semyon V. Yakovlev, and Polina N. Zenkova
Atmos. Meas. Tech., 15, 3941–3967, https://doi.org/10.5194/amt-15-3941-2022, https://doi.org/10.5194/amt-15-3941-2022, 2022
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The change of the global climate is most pronounced in the Arctic, where the air temperature increases faster than the global average. This is associated with an increase in the concentration of greenhouse gases in the atmosphere. It is important to study how the air composition in the Arctic changes in the changing climate. Thus this integrated experiment was carried out to measure the composition of the troposphere in the Russian sector of the Arctic from on board the aircraft laboratory.
Jason E. Williams, Vincent Huijnen, Idir Bouarar, Mehdi Meziane, Timo Schreurs, Sophie Pelletier, Virginie Marécal, Beatrice Josse, and Johannes Flemming
Geosci. Model Dev., 15, 4657–4687, https://doi.org/10.5194/gmd-15-4657-2022, https://doi.org/10.5194/gmd-15-4657-2022, 2022
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The global CAMS air quality model is used for providing tropospheric ozone information to end users. This paper updates the chemical mechanism employed (CBA) and compares it against two other mechanisms (MOCAGE, MOZART) and a multi-decadal dataset based on a previous version of CBA. We perform extensive validation for the US using multiple surface and aircraft datasets, providing an assessment of biases and the extent of correlation across different seasons during 2014.
Dimitris Akritidis, Andrea Pozzer, Johannes Flemming, Antje Inness, Philippe Nédélec, and Prodromos Zanis
Atmos. Chem. Phys., 22, 6275–6289, https://doi.org/10.5194/acp-22-6275-2022, https://doi.org/10.5194/acp-22-6275-2022, 2022
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We perform a process-oriented evaluation of Copernicus Atmosphere Monitoring Service (CAMS) reanalysis (CAMSRA) O3 over Europe using WOUDC (World Ozone and Ultraviolet Radiation Data Centre) ozonesondes and IAGOS (In-service Aircraft for a Global Observing System) aircraft measurements. Chemical data assimilation assists CAMSRA to reproduce the observed O3 increases in the troposphere during the examined folding events, but it mostly results in O3 overestimation in the upper troposphere.
Graciela B. Raga, Darrel Baumgardner, Blanca Rios, Yanet Díaz-Esteban, Alejandro Jaramillo, Martin Gallagher, Bastien Sauvage, Pawel Wolff, and Gary Lloyd
Atmos. Chem. Phys., 22, 2269–2292, https://doi.org/10.5194/acp-22-2269-2022, https://doi.org/10.5194/acp-22-2269-2022, 2022
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The In-Service Aircraft for a Global Observing System (IAGOS) is a small fleet of commercial aircraft that carry a suite of meteorological, gas, aerosol, and cloud sensors and have been measuring worldwide for almost 9 years, since late 2011. Extreme ice events (EIEs) have been identified from the IAGOS cloud measurements and linked to surface emissions for biomass and fossil fuel consumption. The results reported here are highly relevant for climate change and flight operations forecasting.
Abhinna K. Behera, Emmanuel D. Rivière, Sergey M. Khaykin, Virginie Marécal, Mélanie Ghysels, Jérémie Burgalat, and Gerhard Held
Atmos. Chem. Phys., 22, 881–901, https://doi.org/10.5194/acp-22-881-2022, https://doi.org/10.5194/acp-22-881-2022, 2022
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Deep convection overshooting the stratosphere's contribution to the global stratospheric water budget is still being quantified. We ran three different cloud-resolving simulations of an observed case of overshoots in Bauru during the TRO-Pico balloon campaign in the context of upscaling the impact of overshoots at a large scale. These simulations, which have been validated with balloon-borne and S-band radar measurements, shed light on the local-scale variability and composition of overshoots.
Paola Formenti, Claudia Di Biagio, Yue Huang, Jasper Kok, Marc Daniel Mallet, Damien Boulanger, and Mathieu Cazaunau
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2021-403, https://doi.org/10.5194/amt-2021-403, 2021
Publication in AMT not foreseen
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This paper provides with standardized correction factors for the measurements of the most common instruments used in the atmosphere to measure the concentration per size of aerosol particles. These correction factors are provided to users with supplementary information for their use.
Matthieu Plu, Guillaume Bigeard, Bojan Sič, Emanuele Emili, Luca Bugliaro, Laaziz El Amraoui, Jonathan Guth, Beatrice Josse, Lucia Mona, and Dennis Piontek
Nat. Hazards Earth Syst. Sci., 21, 3731–3747, https://doi.org/10.5194/nhess-21-3731-2021, https://doi.org/10.5194/nhess-21-3731-2021, 2021
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Volcanic eruptions that spread out ash over large areas, like Eyjafjallajökull in 2010, may have huge economic consequences due to flight cancellations. In this article, we demonstrate the benefits of source term improvement and of data assimilation for quantifying volcanic ash concentrations. The work, which was supported by the EUNADICS-AV project, is the first one, to our knowledge, that demonstrates the benefit of the assimilation of ground-based lidar data over Europe during an eruption.
Paul D. Hamer, Virginie Marécal, Ryan Hossaini, Michel Pirre, Gisèle Krysztofiak, Franziska Ziska, Andreas Engel, Stephan Sala, Timo Keber, Harald Bönisch, Elliot Atlas, Kirstin Krüger, Martyn Chipperfield, Valery Catoire, Azizan A. Samah, Marcel Dorf, Phang Siew Moi, Hans Schlager, and Klaus Pfeilsticker
Atmos. Chem. Phys., 21, 16955–16984, https://doi.org/10.5194/acp-21-16955-2021, https://doi.org/10.5194/acp-21-16955-2021, 2021
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Bromoform is a stratospheric ozone-depleting gas released by seaweed and plankton transported to the stratosphere via convection in the tropics. We study the chemical interactions of bromoform and its derivatives within convective clouds using a cloud-scale model and observations. Our findings are that soluble bromine gases are efficiently washed out and removed within the convective clouds and that most bromine is transported vertically to the upper troposphere in the form of bromoform.
Hannah Clark, Yasmine Bennouna, Maria Tsivlidou, Pawel Wolff, Bastien Sauvage, Brice Barret, Eric Le Flochmoën, Romain Blot, Damien Boulanger, Jean-Marc Cousin, Philippe Nédélec, Andreas Petzold, and Valérie Thouret
Atmos. Chem. Phys., 21, 16237–16256, https://doi.org/10.5194/acp-21-16237-2021, https://doi.org/10.5194/acp-21-16237-2021, 2021
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We examined 27 years of IAGOS (In-service Aircraft for a Global Observing System) profiles at Frankfurt to see if there were unusual features during the spring of 2020 related to COVID-19 lockdowns in Europe. Increased ozone near the surface was partly linked to the reduction in emissions. Carbon monoxide decreased near the surface, but the impact of the lockdowns was offset by polluted air masses from elsewhere. There were small reductions in ozone and carbon monoxide in the free troposphere.
Gaëlle Dufour, Didier Hauglustaine, Yunjiang Zhang, Maxim Eremenko, Yann Cohen, Audrey Gaudel, Guillaume Siour, Mathieu Lachatre, Axel Bense, Bertrand Bessagnet, Juan Cuesta, Jerry Ziemke, Valérie Thouret, and Bo Zheng
Atmos. Chem. Phys., 21, 16001–16025, https://doi.org/10.5194/acp-21-16001-2021, https://doi.org/10.5194/acp-21-16001-2021, 2021
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The IASI observations and the LMDZ-OR-INCA model simulations show negative ozone trends in the Central East China region in the lower free (3–6 km column) and the upper free (6–9 km column) troposphere. Sensitivity studies from the model show that the Chinese anthropogenic emissions contribute to more than 50 % in the trend. The reduction in NOx emissions that has occurred since 2013 in China seems to lead to a decrease in ozone in the free troposphere, contrary to the increase at the surface.
Victor Lannuque, Bastien Sauvage, Brice Barret, Hannah Clark, Gilles Athier, Damien Boulanger, Jean-Pierre Cammas, Jean-Marc Cousin, Alain Fontaine, Eric Le Flochmoën, Philippe Nédélec, Hervé Petetin, Isabelle Pfaffenzeller, Susanne Rohs, Herman G. J. Smit, Pawel Wolff, and Valérie Thouret
Atmos. Chem. Phys., 21, 14535–14555, https://doi.org/10.5194/acp-21-14535-2021, https://doi.org/10.5194/acp-21-14535-2021, 2021
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The African intertropical troposphere is one of the world areas where the increase in ozone mixing ratio has been most pronounced since 1980 and where high carbon monoxide mixing ratios are found in altitude. In this article, IAGOS aircraft measurements, IASI satellite instrument observations, and SOFT-IO model products are used to explore the seasonal distribution variations and the origin of ozone and carbon monoxide over the African upper troposphere.
Roeland Van Malderen, Dirk De Muer, Hugo De Backer, Deniz Poyraz, Willem W. Verstraeten, Veerle De Bock, Andy W. Delcloo, Alexander Mangold, Quentin Laffineur, Marc Allaart, Frans Fierens, and Valérie Thouret
Atmos. Chem. Phys., 21, 12385–12411, https://doi.org/10.5194/acp-21-12385-2021, https://doi.org/10.5194/acp-21-12385-2021, 2021
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The main aim of initiating measurements of the vertical distribution of the ozone concentration by means of ozonesondes attached to weather balloons at Uccle in 1969 was to improve weather forecasts. Since then, this measurement technique has barely changed, but the dense, long-term, and homogeneous Uccle dataset currently remains crucial for studying the temporal evolution of ozone from the surface to the stratosphere and is also the backbone of the validation of satellite ozone retrievals.
Claire Lamotte, Jonathan Guth, Virginie Marécal, Martin Cussac, Paul David Hamer, Nicolas Theys, and Philipp Schneider
Atmos. Chem. Phys., 21, 11379–11404, https://doi.org/10.5194/acp-21-11379-2021, https://doi.org/10.5194/acp-21-11379-2021, 2021
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Improvements are made in a global chemical transfer model by considering a new volcanic SO2 emissions inventory, with more volcanoes referenced and more information on the altitude of injection. Better constraining volcanic emissions with this inventory improves the global, but mostly local, tropospheric sulfur composition. The tropospheric sulfur budget shows a nonlinearity to the volcanic contribution, especially to the sulfate aerosol burden and sulfur wet deposition.
Romain Blot, Philippe Nedelec, Damien Boulanger, Pawel Wolff, Bastien Sauvage, Jean-Marc Cousin, Gilles Athier, Andreas Zahn, Florian Obersteiner, Dieter Scharffe, Hervé Petetin, Yasmine Bennouna, Hannah Clark, and Valérie Thouret
Atmos. Meas. Tech., 14, 3935–3951, https://doi.org/10.5194/amt-14-3935-2021, https://doi.org/10.5194/amt-14-3935-2021, 2021
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A lack of information about temporal changes in measurement uncertainties is an area of concern for long-term trend studies of the key compounds which have a direct or indirect impact on climate change. The IAGOS program has measured O3 and CO within the troposphere and lower stratosphere for more than 25 years. In this study, we demonstrated that the IAGOS database can be treated as one continuous program and is therefore appropriate for studies of long-term trends.
Yann Cohen, Virginie Marécal, Béatrice Josse, and Valérie Thouret
Geosci. Model Dev., 14, 2659–2689, https://doi.org/10.5194/gmd-14-2659-2021, https://doi.org/10.5194/gmd-14-2659-2021, 2021
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Assessing long-term chemistry–climate simulations with in situ and frequent observations near the tropopause is possible with the IAGOS commercial aircraft data set. This study presents a method that distributes the IAGOS data (ozone and CO) on a monthly model grid, limiting the impact of resolution for the evaluation of the modelled chemical fields. We applied it to the CCMI REF-C1SD simulation from the MOCAGE CTM and notably highlighted well-reproduced O3 behaviour in the lower stratosphere.
Keun-Ok Lee, Brice Barret, Eric L. Flochmoën, Pierre Tulet, Silvia Bucci, Marc von Hobe, Corinna Kloss, Bernard Legras, Maud Leriche, Bastien Sauvage, Fabrizio Ravegnani, and Alexey Ulanovsky
Atmos. Chem. Phys., 21, 3255–3274, https://doi.org/10.5194/acp-21-3255-2021, https://doi.org/10.5194/acp-21-3255-2021, 2021
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This paper focuses on the emission sources and pathways of pollution from the boundary layer to the Asian monsoon anticyclone (AMA) during the StratoClim aircraft campaign period. Simulations with the Meso-NH cloud-chemistry model at a horizontal resolution of 15 km are performed over the Asian region to characterize the impact of monsoon deep convection on the composition of AMA and on the formation of the Asian tropopause aerosol layer during the StratoClim campaign.
Cited articles
Andreae, M. O., Artaxo, P., Fischer, H., Freitas, S., Grégoire, J.-M., Hansel, A., Hoor, P., Kormann, R., Krejci, R., Lange, L., Lelieveld, J., Lindinger, W., Longo, K., Peters, W., de Reus, M., Scheeren, B., Silva Dias, M., Ström, J., van Velthoven, P., and Williams, J.: Transport of biomass burning smoke to the upper troposphere by deep convection in the equatorial region, Geophys. Res. Lett., 28, 951–954, 2001. a
Ashmore, M.: Assessing the future global impacts of ozone on vegetation, Plant Cell Environ., 28, 949–964, 2005. a
Barret, B., Ricaud, P., Mari, C., Attié, J.-L., Bousserez, N., Josse, B., Le Flochmoën, E., Livesey, N. J., Massart, S., Peuch, V.-H., Piacentini, A., Sauvage, B., Thouret, V., and Cammas, J.-P.: Transport pathways of CO in the African upper troposphere during the monsoon season: a study based upon the assimilation of spaceborne observations, Atmos. Chem. Phys., 8, 3231–3246, https://doi.org/10.5194/acp-8-3231-2008, 2008. a
Barret, B., Sauvage, B., Bennouna, Y., and Le Flochmoen, E.: Upper-tropospheric CO and O3 budget during the Asian summer monsoon, Atmos. Chem. Phys., 16, 9129–9147, https://doi.org/10.5194/acp-16-9129-2016, 2016. a, b
Bergman, J. W., Fierli, F., Jensen, E. J., Honomichl, S., and Pan, L. L.: Boundary layer sources for the Asian anticyclone: Regional contributions to a vertical conduit, J. Geophys. Res.-Atmos., 118, 2560–2575, 2013. a
Blot, R., Nedelec, P., Boulanger, D., Wolff, P., Sauvage, B., Cousin, J.-M., Athier, G., Zahn, A., Obersteiner, F., Scharffe, D., Petetin, H., Bennouna, Y., Clark, H., and Thouret, V.: Internal consistency of the IAGOS ozone and carbon monoxide measurements for the last 25 years, Atmos. Meas. Tech., 14, 3935–3951, https://doi.org/10.5194/amt-14-3935-2021, 2021. a
Boulanger, D., Blot, R., Bundke, U., Gerbig, C., Hermann, M., Nédélec, P., Rohs, S., and Ziereis, H.: IAGOS final quality controlled Observational Data L2 – Time series, Aeris [data set], https://doi.org/10.25326/06, 2018. a
Boulanger, D., Thouret, V., and Petzold, A.: IAGOS Data Portal, AERIS [data set], https://doi.org/10.25326/20, 2019. a
Brenninkmeijer, C., Crutzen, P., Fischer, H., Güsten, H., Hans, W., Heinrich, G., Heintzenberg, J., Hermann, M., Immelmann, T., Kersting, D., Maiss, M., Nolle, M., Pitscheider, A., Pohlkamp, H., Scharffe, D., Specht, K., and Wiedensohler, A.: CARIBIC – Civil aircraft for global measurement of trace gases and aerosols in the tropopause region, J. Atmos. Ocean. Tech., 16, 1373–1383, 1999. a
Chang, K.-L., Petropavlovskikh, I., Cooper, O. R., Schultz, M. G., and Wang, T.: Regional trend analysis of surface ozone observations from monitoring networks in eastern North America, Europe and East Asia, Elem. Sci. Anth., 5, 50, https://doi.org/10.1525/elementa.243, 2017. a, b
Chen, T.-M., Kuschner, W. G., Gokhale, J., and Shofer, S.: Outdoor air pollution: ozone health effects, Am. J. Med. Sci., 333, 244–248, 2007. a
Cohen, Y., Petetin, H., Thouret, V., Marécal, V., Josse, B., Clark, H., Sauvage, B., Fontaine, A., Athier, G., Blot, R., Boulanger, D., Cousin, J.-M., and Nédélec, P.: Climatology and long-term evolution of ozone and carbon monoxide in the upper troposphere–lower stratosphere (UTLS) at northern midlatitudes, as seen by IAGOS from 1995 to 2013, Atmos. Chem. Phys., 18, 5415–5453, https://doi.org/10.5194/acp-18-5415-2018, 2018. a, b, c, d, e, f, g
Cooper, O. R. and Parrish, D. D.: Air Pollution Export from and Import to North America: Experimental Evidence, in: Air Pollution: Intercontinental Transport of Air Pollution, edited by: Stohl, A., Springer, Berlin, Heidelberg, ISBN 978-3-540-40037-0, 41–67, https://doi.org/10.1007/b94523, 2004. a, b, c, d
Cooper, O. R., Forster, C., Parrish, D., Trainer, M., Dunlea, E., Ryerson, T., Hübler, G., Fehsenfeld, F., Nicks, D., Holloway, J., de Gouw, J., Warneke, C., Roberts, J. M., Flocke, F., and Moody, J.: A case study of transpacific warm conveyor belt transport: Influence of merging airstreams on trace gas import to North America, J. Geophys. Res.-Atmos., 109, D23S08, https://doi.org/10.1029/2003JD003624, 2004. a, b
Cussac, M., Marécal, V., Thouret, V., Josse, B., and Sauvage, B.: The impact of biomass burning on upper tropospheric carbon monoxide: a study using MOCAGE global model and IAGOS airborne data, Atmos. Chem. Phys., 20, 9393–9417, https://doi.org/10.5194/acp-20-9393-2020, 2020. a, b
Damoah, R., Spichtinger, N., Servranckx, R., Fromm, M., Eloranta, E. W., Razenkov, I. A., James, P., Shulski, M., Forster, C., and Stohl, A.: A case study of pyro-convection using transport model and remote sensing data, Atmos. Chem. Phys., 6, 173–185, https://doi.org/10.5194/acp-6-173-2006, 2006. a
Davison, A. and Barnes, J.: Effects of ozone on wild plants, New Phytol., 139, 135–151, 1998. a
Dentener, F., Kinne, S., Bond, T., Boucher, O., Cofala, J., Generoso, S., Ginoux, P., Gong, S., Hoelzemann, J. J., Ito, A., Marelli, L., Penner, J. E., Putaud, J.-P., Textor, C., Schulz, M., van der Werf, G. R., and Wilson, J.: Emissions of primary aerosol and precursor gases in the years 2000 and 1750 prescribed data-sets for AeroCom, Atmos. Chem. Phys., 6, 4321–4344, https://doi.org/10.5194/acp-6-4321-2006, 2006. a
Dickerson, R. R., Li, C., Li, Z., Marufu, L. T., Stehr, J. W., McClure, B., Krotkov, N., Chen, H., Wang, P., Xia, X., Ban, X., Gong, F., Yuan, J., and Yang, J.: Aircraft observations of dust and pollutants over northeast China: Insight into the meteorological mechanisms of transport, J. Geophys. Res.-Atmos., 112, D24S90, https://doi.org/10.1029/2007JD008999, 2007. a
Ding, A., Wang, T., Xue, L., Gao, J., Stohl, A., Lei, H., Jin, D., Ren, Y., Wang, X., Wei, X., Qi, Y., Liu, J., and Zhang, X.: Transport of north China air pollution by midlatitude cyclones: Case study of aircraft measurements in summer 2007, J. Geophys. Res.-Atmos., 114, D08304, https://doi.org/10.1029/2008JD011023, 2009. a, b
Duncan, B. N., West, J. J., Yoshida, Y., Fiore, A. M., and Ziemke, J. R.: The influence of European pollution on ozone in the Near East and northern Africa, Atmos. Chem. Phys., 8, 2267–2283, https://doi.org/10.5194/acp-8-2267-2008, 2008. a, b, c, d
Fadnavis, S., Buchunde, P., Ghude, S. D., Kulkarni, S., and Beig, G.: Evidence of seasonal enhancement of CO in the upper troposphere over India, International J. Remote Sens., 32, 7441–7452, 2011. a
Field, R. D., Van Der Werf, G. R., Fanin, T., Fetzer, E. J., Fuller, R., Jethva, H., Levy, R., Livesey, N. J., Luo, M., Torres, O., and Worden, H.: Indonesian fire activity and smoke pollution in 2015 show persistent nonlinear sensitivity to El Niño-induced drought, P. Natl. Acad. Sci. USA, 113, 9204–9209, 2016. a
Fuhrer, J., Skärby, L., and Ashmore, M. R.: Critical levels for ozone effects on vegetation in Europe, Environ. Pollut., 97, 91–106, 1997. a
Galanter, M., Levy, H., and Carmichael, G. R.: Impacts of biomass burning on tropospheric CO, NOx, and O3, J. Geophys. Res.-Atmos., 105, 6633–6653, 2000. a
Gamo, M.: Thickness of the dry convection and large-scale subsidence above deserts, Bound.-Lay. Meteorol., 79, 265–278, 1996. a
Gaudel, A., Cooper, O. R., Ancellet, G., Barret, B., Boynard, A., Burrows, J. P., Clerbaux, C., Coheur, P.-F., Cuesta, J., Cuevas, E., Doniki, S., Dufour, G., Ebojie, F., Foret, G., Garcia, O., Granados-Muñoz, M. J., Hannigan, J. W., Hase, F., Hassler, B., Huang, G., Hurtmans, D., Jaffe, D., Jones, N., Kalabokas, P., Kerridge, B., Kulawik, S., Latter, B., Leblanc, T., Le Flochmoën, E., Lin, W., Liu, J., Liu, X., Mahieu, E., McClure-Begley, A., Neu, J. L., Osman, M., Palm, M., Petetin, H., Petropavlovskikh, I., Querel, R., Rahpoe, N., Rozanov, A., Schultz, M. G., Schwab, J., Siddans, R., Smale, D., Steinbacher, M., Tanimoto, H., Tarasick, D. W., Thouret, V., Thompson, A. M., Trickl, T., Weatherhead, E., Wespes, C., Worden, H. M., Vigouroux, C., Xu, X., Zeng, G., and Ziemke, J.: Tropospheric Ozone Assessment Report: Present-day distribution and trends of tropospheric ozone relevant to climate and global atmospheric chemistry model evaluation, Elem. Sci. Anth., 6, 39, https://doi.org/10.1525/elementa.291, 2018. a
Gaudel, A., Cooper, O. R., Chang, K.-L., Bourgeois, I., Ziemke, J. R., Strode, S. A., Oman, L. D., Sellitto, P., Nédélec, P., Blot, R., Thouret, V., and Granier, C.: Aircraft observations since the 1990s reveal increases of tropospheric ozone at multiple locations across the Northern Hemisphere, Science Advances, 6, eaba8272, https://doi.org/10.1126/sciadv.aba8272, 2020. a
Giglio, L., Randerson, J. T., and Van Der Werf, G. R.: Analysis of daily, monthly, and annual burned area using the fourth-generation global fire emissions database (GFED4), J. Geophys. Res.-Biogeo., 118, 317–328, 2013. a
Huang, L., Fu, R., Jiang, J. H., Wright, J. S., and Luo, M.: Geographic and seasonal distributions of CO transport pathways and their roles in determining CO centers in the upper troposphere, Atmos. Chem. Phys., 12, 4683–4698, https://doi.org/10.5194/acp-12-4683-2012, 2012. a
Hudman, R. C., Jacob, D. J., Cooper, O. R., Evans, M. J., Heald, C. L., Park, R. J., Fehsenfeld, F., Flocke, F., Holloway, J., Hübler, G., Kita, K., Koike, M., Kondo, Y., Neuman, A., Nowak, J., Oltmans, S., Parrish, D., Roberts, J. M., and Ryerson, T.: Ozone production in transpacific Asian pollution plumes and implications for ozone air quality in California, J. Geophys. Res.-Atmos., 109, D23S10, https://doi.org/10.1029/2004JD004974, 2004. a
Huntrieser, H. and Schlager, H.: Air Pollution Export from and Import to Europe: Experimental Evidence, in: Air Pollution: Intercontinental Transport of Air Pollution, edited by: Stohl, A., Springer, Berlin, Heidelberg, ISBN 978-3-540-40037-0, 69–98, https://doi.org/10.1007/b94524, 2004. a, b, c
Jaffe, D., Anderson, T., Covert, D., Kotchenruther, R., Trost, B., Danielson, J., Simpson, W., Berntsen, T., Karlsdottir, S., Blake, D., Harris, J., Carmichael, G., and Uno, I.: Transport of Asian air pollution to North America, Geophys. Res. Lett., 26, 711–714, https://doi.org/10.1029/1999GL900100, 1999. a, b
Kaiser, J. W., Heil, A., Andreae, M. O., Benedetti, A., Chubarova, N., Jones, L., Morcrette, J.-J., Razinger, M., Schultz, M. G., Suttie, M., and van der Werf, G. R.: Biomass burning emissions estimated with a global fire assimilation system based on observed fire radiative power, Biogeosciences, 9, 527–554, https://doi.org/10.5194/bg-9-527-2012, 2012. a
Kar, J., Bremer, H., Drummond, J. R., Rochon, Y. J., Jones, D. B. A., Nichitiu, F., Zou, J., Liu, J., Gille, J. C., Edwards, D. P., Deeter, M. N., Francis, G., Ziskin, D., and Warner, J.: Evidence of vertical transport of carbon monoxide from Measurements of Pollution in the Troposphere (MOPITT), Geophys. Res. Lett., 31, L23105, https://doi.org/10.1029/2004GL021128, 2004. a, b, c
Kim, S.-W., Kim, K.-M., Jeong, Y., Seo, S., Park, Y., and Kim, J.: Changes in surface ozone in South Korea on diurnal to decadal timescales for the period of 2001–2021, Atmos. Chem. Phys., 23, 12867–12886, https://doi.org/10.5194/acp-23-12867-2023, 2023. a
Labonne, M., Bréon, F.-M., and Chevallier, F.: Injection height of biomass burning aerosols as seen from a spaceborne lidar, Geophys. Res. Lett., 34, L11806, https://doi.org/10.1029/2007GL029311, 2007. a
Lal, S., Venkataramani, S., Chandra, N., Cooper, O. R., Brioude, J., and Naja, M.: Transport effects on the vertical distribution of tropospheric ozone over western India, J. Geophys. Res.-Atmos., 119, 10012–10026, https://doi.org/10.1002/2014JD021854, 2014. a
Lannuque, V., Sauvage, B., Barret, B., Clark, H., Athier, G., Boulanger, D., Cammas, J.-P., Cousin, J.-M., Fontaine, A., Le Flochmoën, E., Nédélec, P., Petetin, H., Pfaffenzeller, I., Rohs, S., Smit, H. G. J., Wolff, P., and Thouret, V.: Origins and characterization of CO and O3 in the African upper troposphere, Atmos. Chem. Phys., 21, 14535–14555, https://doi.org/10.5194/acp-21-14535-2021, 2021. a, b, c, d, e, f, g, h, i, j, k, l
Lavaysse, C., Naumann, G., Alfieri, L., Salamon, P., and Vogt, J.: Predictability of the European heat and cold waves, Clim. Dynam., 52, 2481–2495, 2019. a
Lawrence, M. G.: Export of Air Pollution from Southern Asia and its Large-Scale Effects, in: Air Pollution: Intercontinental Transport of Air Pollution, edited by: Stohl, A., Springer, Berlin, Heidelberg, ISBN 978-3-540-40037-0, 131–172, https://doi.org/10.1007/b94526, 2004. a, b
Lawrence, M. G. and Lelieveld, J.: Atmospheric pollutant outflow from southern Asia: a review, Atmos. Chem. Phys., 10, 11017–11096, https://doi.org/10.5194/acp-10-11017-2010, 2010. a, b
Lelieveld, J., Crutzen, P. J., Ramanathan, V., Andreae, M. O., Brenninkmeijer, C. A. M., Campos, T., Cass, G. R., Dickerson, R. R., Fischer, H., de Gouw, J. A., Hansel, A., Jefferson, A., Kley, D., de Laat, A. T. J., Lal, S., Lawrence, M. G., Lobert, J. M., Mayol-Bracero, O. L., Mitra, A. P., Novakov, T., Oltmans, S. J., Prather, K. A., Reiner, T., Rodhe, H., Scheeren, H. A., Sikka, D., and Williams, J.: The Indian Ocean Experiment: Widespread Air Pollution from South and Southeast Asia, Science, 291, 1031–1036, https://doi.org/10.1126/science.1057103, 2001. a
Lelieveld, J., Gromov, S., Pozzer, A., and Taraborrelli, D.: Global tropospheric hydroxyl distribution, budget and reactivity, Atmos. Chem. Phys., 16, 12477–12493, https://doi.org/10.5194/acp-16-12477-2016, 2016. a, b
Li, Q., Jacob, D. J., Bey, I., Palmer, P. I., Duncan, B. N., Field, B. D., Martin, R. V., Fiore, A. M., Yantosca, R. M., Parrish, D. D., Simmonds, P. G., and Oltmans, S. J.: Transatlantic transport of pollution and its effects on surface ozone in Europe and North America, J. Geophys. Res.-Atmos., 107, ACH 4-1–ACH 4-21, https://doi.org/10.1029/2001JD001422, 2002. a
Liang, Q., Jaeglé, L., Jaffe, D. A., Weiss-Penzias, P., Heckman, A., and Snow, J. A.: Long-range transport of Asian pollution to the northeast Pacific: Seasonal variations and transport pathways of carbon monoxide, J. Geophys. Res.-Atmos., 109, D23S07, https://doi.org/10.1029/2003JD004402, 2004. a, b
Liang, Q., Jaeglé, L., Hudman, R. C., Turquety, S., Jacob, D. J., Avery, M. A., Browell, E. V., Sachse, G. W., Blake, D. R., Brune, W., Ren, X., Cohen, R. C., Dibb, J. E., Fried, A., Fuelberg, H., Porter, M., Heikes, B. G., Huey, G., Singh, H. B., and Wennberg, P. O.: Summertime influence of Asian pollution in the free troposphere over North America, J. Geophys. Res.-Atmos., 112, D12S11, https://doi.org/10.1029/2006JD007919, 2007. a, b
Liu, H., Liu, S., Xue, B., Lv, Z., Meng, Z., Yang, X., Xue, T., Yu, Q., and He, K.: Ground-level ozone pollution and its health impacts in China, Atmos. Environ., 173, 223–230, 2018. a
Lu, X., Hong, J., Zhang, L., Cooper, O. R., Schultz, M. G., Xu, X., Wang, T., Gao, M., Zhao, Y., and Zhang, Y.: Severe Surface Ozone Pollution in China: A Global Perspective, Environ. Sci. Technol. Lett., 5, 487–494, https://doi.org/10.1021/acs.estlett.8b00366, 2018. a, b
Marenco, A., Thouret, V., Nédélec, P., Smit, H., Helten, M., Kley, D., Karcher, F., Simon, P., Law, K., Pyle, J., Poschmann, G., Von Wrede, R., Hume, C., and Cook, T.: Measurement of ozone and water vapor by Airbus in-service aircraft: The MOZAIC airborne program, An overview, J. Geophys. Res.-Atmos., 103, 25631–25642, 1998. a
Mauzerall, D. L., Logan, J. A., Jacob, D. J., Anderson, B. E., Blake, D. R., Bradshaw, J. D., Heikes, B., Sachse, G. W., Singh, H., and Talbot, B.: Photochemistry in biomass burning plumes and implications for tropospheric ozone over the tropical South Atlantic, J. Geophys. Res.-Atmos., 103, 8401–8423, 1998. a
McDuffie, E. E., Smith, S. J., O'Rourke, P., Tibrewal, K., Venkataraman, C., Marais, E. A., Zheng, B., Crippa, M., Brauer, M., and Martin, R. V.: A global anthropogenic emission inventory of atmospheric pollutants from sector- and fuel-specific sources (1970–2017): an application of the Community Emissions Data System (CEDS), Earth Syst. Sci. Data, 12, 3413–3442, https://doi.org/10.5194/essd-12-3413-2020, 2020. a
Nedelec, P., Thouret, V., Brioude, J., Sauvage, B., Cammas, J.-P., and Stohl, A.: Extreme CO concentrations in the upper troposphere over northeast Asia in June 2003 from the in situ MOZAIC aircraft data, Geophys. Res. Lett., 32, L14807, https://doi.org/10.1029/2005GL023141, 2005. a
Nédélec, P., Blot, R., Boulanger, D., Athier, G., Cousin, J.-M., Gautron, B., Petzold, A., Volz-Thomas, A., and Thouret, V.: Instrumentation on commercial aircraft for monitoring the atmospheric composition on a global scale: the IAGOS system, technical overview of ozone and carbon monoxide measurements, Tellus B, 67, 27791, https://doi.org/10.3402/tellusb.v67.27791, 2015. a, b
Novelli, P. C., Masarie, K. A., and Lang, P. M.: Distributions and recent changes of carbon monoxide in the lower troposphere, J. Geophys. Res.-Atmos., 103, 19015–19033, https://doi.org/10.1029/98JD01366, 1998. a, b
Nowak, J. B., Parrish, D. D., Neuman, J. A., Holloway, J. S., Cooper, O. R., Ryerson, T. B., Nicks Jr., D. K., Flocke, F., Roberts, J. M., Atlas, E., de Gouw, J. A., Donnelly, S., Dunlea, E., Hübler, G., Huey, L. G., Schauffler, S., Tanner, D. J., Warneke, C., and Fehsenfeld, F. C.: Gas-phase chemical characteristics of Asian emission plumes observed during ITCT 2K2 over the eastern North Pacific Ocean, J. Geophys. Res.-Atmos., 109, D23S19, https://doi.org/10.1029/2003JD004488, 2004. a
Ntoumos, A., Hadjinicolaou, P., Zittis, G., Constantinidou, K., Tzyrkalli, A., and Lelieveld, J.: Evaluation of WRF Model Boundary Layer Schemes in Simulating Temperature and Heat Extremes over the Middle East–North Africa (MENA) Region, J. Appl. Meteorol. Clim., 62, 1315–1332, 2023. a
Owen, R., Cooper, O., Stohl, A., and Honrath, R.: An analysis of the mechanisms of North American pollutant transport to the central North Atlantic lower free troposphere, J. Geophys. Res.-Atmos., 111, D23S58, https://doi.org/10.1029/2006JD007062, 2006. a
Pan, L. L., Honomichl, S. B., Kinnison, D. E., Abalos, M., Randel, W. J., Bergman, J. W., and Bian, J.: Transport of chemical tracers from the boundary layer to stratosphere associated with the dynamics of the Asian summer monsoon, J. Geophys. Res.-Atmos., 121, 14159–14174, https://doi.org/10.1002/2016JD025616, 2016. a
Park, M., Randel, W. J., Gettelman, A., Massie, S. T., and Jiang, J. H.: Transport above the Asian summer monsoon anticyclone inferred from Aura Microwave Limb Sounder tracers, J. Geophys. Res.-Atmos., 112, D16309, https://doi.org/10.1029/2006JD008294, 2007. a
Park, M., Randel, W. J., Emmons, L. K., Bernath, P. F., Walker, K. A., and Boone, C. D.: Chemical isolation in the Asian monsoon anticyclone observed in Atmospheric Chemistry Experiment (ACE-FTS) data, Atmos. Chem. Phys., 8, 757–764, https://doi.org/10.5194/acp-8-757-2008, 2008. a
Paugam, R., Wooster, M., Atherton, J., Freitas, S. R., Schultz, M. G., and Kaiser, J. W.: Development and optimization of a wildfire plume rise model based on remote sensing data inputs – Part 2, Atmos. Chem. Phys. Discuss., 15, 9815–9895, https://doi.org/10.5194/acpd-15-9815-2015, 2015. a
Petetin, H., Thouret, V., Fontaine, A., Sauvage, B., Athier, G., Blot, R., Boulanger, D., Cousin, J.-M., and Nédélec, P.: Characterising tropospheric O3 and CO around Frankfurt over the period 1994–2012 based on MOZAIC–IAGOS aircraft measurements, Atmos. Chem. Phys., 16, 15147–15163, https://doi.org/10.5194/acp-16-15147-2016, 2016. a
Petetin, H., Jeoffrion, M., Sauvage, B., Athier, G., Blot, R., Boulanger, D., Clark, H., Cousin, J.-M., Gheusi, F., Nedelec, P., Steinbacher, M., and Thouret, V.: Representativeness of the IAGOS airborne measurements in the lower troposphere, Elem. Sci. Anth., 6, 23, https://doi.org/10.1525/elementa.280, 2018a. a, b, c
Petetin, H., Sauvage, B., Parrington, M., Clark, H., Fontaine, A., Athier, G., Blot, R., Boulanger, D., Cousin, J.-M., Nédélec, P., and Thouret, V.: The role of biomass burning as derived from the tropospheric CO vertical profiles measured by IAGOS aircraft in 2002–2017, Atmos. Chem. Phys., 18, 17277–17306, https://doi.org/10.5194/acp-18-17277-2018, 2018b. a, b, c, d, e
Petzold, A., Thouret, V., Gerbig, C., Zahn, A., Brenninkmeijer, C. A., Gallagher, M., Hermann, M., Pontaud, M., Ziereis, H., Boulanger, D., Marshall, J., Nédélec, P., Smit, H. G. J., Friess, U., Flaud, J.-M., Wahner, A., Cammas, J.-P., Volz-Thomas, A., and IAGOS Team: Global-scale atmosphere monitoring by in-service aircraft–current achievements and future prospects of the European Research Infrastructure IAGOS, Tellus B, 67, 28452, https://doi.org/10.3402/tellusb.v67.28452, 2015. a
Pochanart, P., Wild, O., and Akimoto, H.: Air pollution import to and export from East Asia, Air pollution: Intercontinental transport of air pollution, edited by: Stohl, A., Springer Berlin Heidelberg, Berlin, Heidelberg, 99–130, https://doi.org/10.1007/b94525, 2004. a, b
Qu, Z., Henze, D. K., Worden, H. M., Jiang, Z., Gaubert, B., Theys, N., and Wang, W.: Sector-based top-down estimates of NOx, SO2, and CO emissions in East Asia, Geophys. Res. Lett., 49, e2021GL096009, https://doi.org/10.1029/2021GL096009, 2022. a
Rémy, S., Veira, A., Paugam, R., Sofiev, M., Kaiser, J. W., Marenco, F., Burton, S. P., Benedetti, A., Engelen, R. J., Ferrare, R., and Hair, J. W.: Two global data sets of daily fire emission injection heights since 2003, Atmos. Chem. Phys., 17, 2921–2942, https://doi.org/10.5194/acp-17-2921-2017, 2017. a, b
Ricaud, P., Sič, B., El Amraoui, L., Attié, J.-L., Zbinden, R., Huszar, P., Szopa, S., Parmentier, J., Jaidan, N., Michou, M., Abida, R., Carminati, F., Hauglustaine, D., August, T., Warner, J., Imasu, R., Saitoh, N., and Peuch, V.-H.: Impact of the Asian monsoon anticyclone on the variability of mid-to-upper tropospheric methane above the Mediterranean Basin, Atmos. Chem. Phys., 14, 11427–11446, https://doi.org/10.5194/acp-14-11427-2014, 2014. a
Riese, M., Ploeger, F., Rap, A., Vogel, B., Konopka, P., Dameris, M., and Forster, P.: Impact of uncertainties in atmospheric mixing on simulated UTLS composition and related radiative effects, J. Geophys. Res.-Atmos., 117, D16305, https://doi.org/10.1029/2012JD017751, 2012. a
Sauvage, B., Thouret, V., Cammas, J.-P., Gheusi, F., Athier, G., and Nédélec, P.: Tropospheric ozone over Equatorial Africa: regional aspects from the MOZAIC data, Atmos. Chem. Phys., 5, 311–335, https://doi.org/10.5194/acp-5-311-2005, 2005. a
Sauvage, B., Fontaine, A., Eckhardt, S., Auby, A., Boulanger, D., Petetin, H., Paugam, R., Athier, G., Cousin, J.-M., Darras, S., Nédélec, P., Stohl, A., Turquety, S., Cammas, J.-P., and Thouret, V.: Source attribution using FLEXPART and carbon monoxide emission inventories: SOFT-IO version 1.0, Atmos. Chem. Phys., 17, 15271–15292, https://doi.org/10.5194/acp-17-15271-2017, 2017a. a, b
Sauvage, B., Wolff, P., Blot, R., Nédélec, P., and Boulanger, D.: IAGOS Carbon Monoxide contribution and interpolated modeled data from ECMWF – L4, Aeris [data set], https://doi.org/10.25326/3, 2017b. a, b
Shastri, H., Ghosh, S., and Karmakar, S.: Improving Global Forecast System of extreme precipitation events with regional statistical model: Application of quantile-based probabilistic forecasts, J. Geophys. Res.-Atmos., 122, 1617–1634, 2017. a
Smoydzin, L. and Hoor, P.: Contribution of Asian emissions to upper tropospheric CO over the remote Pacific, Atmos. Chem. Phys., 22, 7193–7206, https://doi.org/10.5194/acp-22-7193-2022, 2022. a, b
Stohl, A.: A 1-year Lagrangian “climatology” of airstreams in the northern hemisphere troposphere and lowermost stratosphere, J. Geophys. Res.-Atmos., 106, 7263–7279, https://doi.org/10.1029/2000JD900570, 2001. a
Stohl, A., Forster, C., Frank, A., Seibert, P., and Wotawa, G.: Technical note: The Lagrangian particle dispersion model FLEXPART version 6.2, Atmos. Chem. Phys., 5, 2461–2474, https://doi.org/10.5194/acp-5-2461-2005, 2005. a
Szopa, S., Naik, V., Adhikary, B., Artaxo, P., Berntsen, T., Collins, W. D., Fuzzi, S., Gallardo, L., Kiendler-Scharr, A., Klimont, Z., Liao, H., Unger, N., and Zanis, P.: Short-Lived Climate Forcers, in: Climate Change 2021: The Physical Science Basis. Contribution of Working Group I to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Masson-Delmotte, V., Zhai, P., Pirani, A., Connors, S. L., Péan, C., Berger, S., Caud, N., Chen, Y., Goldfarb, L., Gomis, M. I., Huang, M., Leitzell, K., Lonnoy, E., Matthews, J. B. R., Maycock, T. K., Waterfield, T., Yelekçi, O., Yu, R., and Zhou, B., Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, 817–922, https://doi.org/10.1017/9781009157896.008, 2021. a
Thouret, V., Marenco, A., Logan, J. A., Nédélec, P., and Grouhel, C.: Comparisons of ozone measurements from the MOZAIC airborne program and the ozone sounding network at eight locations, J. Geophys. Res.-Atmos., 103, 25695–25720, 1998. a
Thouret, V., Cammas, J.-P., Sauvage, B., Athier, G., Zbinden, R., Nédélec, P., Simon, P., and Karcher, F.: Tropopause referenced ozone climatology and inter-annual variability (1994–2003) from the MOZAIC programme, Atmos. Chem. Phys., 6, 1033–1051, https://doi.org/10.5194/acp-6-1033-2006, 2006. a, b
Thouret, V., Clark, H., Petzold, A., Nédélec, P., and Zahn, A.: IAGOS: Monitoring Atmospheric Composition for Air Quality and Climate by Passenger Aircraft, Handbook of Air Quality and Climate Change, Springer Naturem Singapore, 18, 17277–17306, https://doi.org/10.1007/978-981-15-2527-8_57-1, 2022. a
Tsivlidou, M., Sauvage, B., Bennouna, Y., Blot, R., Boulanger, D., Clark, H., Le Flochmoën, E., Nédélec, P., Thouret, V., Wolff, P., and Barret, B.: Tropical tropospheric ozone and carbon monoxide distributions: characteristics, origins, and control factors, as seen by IAGOS and IASI, Atmos. Chem. Phys., 23, 14039–14063, https://doi.org/10.5194/acp-23-14039-2023, 2023. a, b, c, d, e, f
Val Martin, M., Logan, J. A., Kahn, R. A., Leung, F.-Y., Nelson, D. L., and Diner, D. J.: Smoke injection heights from fires in North America: analysis of 5 years of satellite observations, Atmos. Chem. Phys., 10, 1491–1510, https://doi.org/10.5194/acp-10-1491-2010, 2010. a
Xia, Y., Huang, Y., and Hu, Y.: On the climate impacts of upper tropospheric and lower stratospheric ozone, J. Geophys. Res.-Atmos., 123, 730–739, 2018. a
Yang, J., Liu, J., Han, S., Yao, Q., and Cai, Z.: Study of the meteorological influence on ozone in urban areas and their use in assessing ozone trends in all seasons from 2009 to 2015 in Tianjin, China, Meteorol. Atmos. Phys., 131, 1661–1675, https://doi.org/10.1007/s00703-019-00664-x, 2019. a
Zhang, Y., Cooper, O. R., Gaudel, A., Thompson, A. M., Nédélec, P., Ogino, S.-Y., and West, J. J.: Tropospheric ozone change from 1980 to 2010 dominated by equatorward redistribution of emissions, Nat. Geosci., 9, 875–879, 2016. a
Short summary
Our study examines intense-carbon-monoxide (CO) pollution events measured by commercial aircraft from the In-service Aircraft for a Global Observing System (IAGOS) research infrastructure. We combine these measurements with the SOFT-IO model to trace the origin of the observed CO. A comprehensive analysis of the geographical origin, source type, seasonal variation, and ozone levels of these pollution events is provided.
Our study examines intense-carbon-monoxide (CO) pollution events measured by commercial aircraft...
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