Articles | Volume 24, issue 22
https://doi.org/10.5194/acp-24-12985-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-24-12985-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Technical note
| 
25 Nov 2024
Technical note |
| 25 Nov 2024
| 25 Nov 2024
Technical note: High-resolution analyses of concentrations and sizes of refractory black carbon particles deposited in northwestern Greenland over the past 350 years – Part 1: Continuous flow analysis of the SIGMA-D ice core using the wide-range Single-Particle Soot Photometer and a high-efficiency nebulizer
National Institute of Polar Research, Tachikawa, Tokyo, 190-8518, Japan
SOKENDAI, Shonan Village, Hayama, Kanagawa, 240-0193, Japan
Remi Dallmayr
National Institute of Polar Research, Tachikawa, Tokyo, 190-8518, Japan
now at: Alfred Wegener Institute for Polar and Marine Research, Bremerhaven, Germany
Yoshimi Ogawa-Tsukagawa
National Institute of Polar Research, Tachikawa, Tokyo, 190-8518, Japan
Nobuhiro Moteki
Department of Chemistry, Graduate School of Science, Tokyo Metropolitan University, Hachioji, Tokyo, 192-0397, Japan
Tatsuhiro Mori
Department of Applied Chemistry, Faculty of Science and Technology, Keio University, Yokohama, Kanagawa, 223-8522, Japan
Sho Ohata
Institute for Space–Earth Environmental Research, Nagoya University, Nagoya, 464-8601, Japan
Yutaka Kondo
National Institute of Polar Research, Tachikawa, Tokyo, 190-8518, Japan
Makoto Koike
Department of Earth and Planetary Science, Graduate School of Science, University of Tokyo, Bunkyo-ku, 113-0033, Japan
Motohiro Hirabayashi
National Institute of Polar Research, Tachikawa, Tokyo, 190-8518, Japan
Jun Ogata
National Institute of Polar Research, Tachikawa, Tokyo, 190-8518, Japan
Kyotaro Kitamura
National Institute of Polar Research, Tachikawa, Tokyo, 190-8518, Japan
Kenji Kawamura
National Institute of Polar Research, Tachikawa, Tokyo, 190-8518, Japan
SOKENDAI, Shonan Village, Hayama, Kanagawa, 240-0193, Japan
Koji Fujita
Graduate School of Environmental Studies, Nagoya University, Nagoya, 464-8601, Japan
Sumito Matoba
Institute of Low Temperature Science, Hokkaido University, Sapporo, 060-0819, Japan
Naoko Nagatsuka
National Institute of Polar Research, Tachikawa, Tokyo, 190-8518, Japan
now at: Japan Agency for Marine-Earth Science and Technology, Yokosuka, Kanagawa, 237-0061, Japan
Akane Tsushima
National Institute of Polar Research, Tachikawa, Tokyo, 190-8518, Japan
now at: Graduate School of Integrated Science and Technology, Nagasaki University, Nagasaki, 852-8521, Japan
Kaori Fukuda
National Institute of Polar Research, Tachikawa, Tokyo, 190-8518, Japan
Teruo Aoki
National Institute of Polar Research, Tachikawa, Tokyo, 190-8518, Japan
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Preprint archived
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The Cryosphere, 17, 4207–4221, https://doi.org/10.5194/tc-17-4207-2023, https://doi.org/10.5194/tc-17-4207-2023, 2023
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Stable water isotopes from firn cores provide valuable information on past climates, yet their utility is hampered by stratigraphic noise, i.e. the irregular deposition and wind-driven redistribution of snow. We found stratigraphic noise on the Antarctic Plateau to be related to the local accumulation rate, snow surface roughness and slope inclination, which can guide future decisions on sampling locations and thus increase the resolution of climate reconstructions from low-accumulation areas.
Yukihiko Onuma, Koji Fujita, Nozomu Takeuchi, Masashi Niwano, and Teruo Aoki
The Cryosphere, 17, 3309–3328, https://doi.org/10.5194/tc-17-3309-2023, https://doi.org/10.5194/tc-17-3309-2023, 2023
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We established a novel model that simulates the temporal changes in cryoconite hole (CH) depth using heat budgets calculated independently at the ice surface and CH bottom based on hole shape geometry. The simulations suggest that CH depth is governed by the balance between the intensity of the diffuse component of downward shortwave radiation and the wind speed. The meteorological conditions may be important factors contributing to the recent ice surface darkening via the redistribution of CHs.
Naoko Nagatsuka, Kumiko Goto-Azuma, Koji Fujita, Yuki Komuro, Motohiro Hirabayashi, Jun Ogata, Kaori Fukuda, Yoshimi Ogawa-Tsukagawa, Kyotaro Kitamura, Ayaka Yonekura, Fumio Nakazawa, Yukihiko Onuma, Naoyuki Kurita, Sune Olander Rasmussen, Giulia Sinnl, Trevor James Popp, and Dorthe Dahl-Jensen
EGUsphere, https://doi.org/10.5194/egusphere-2023-1666, https://doi.org/10.5194/egusphere-2023-1666, 2023
Preprint archived
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We present a new high-temporal-resolution record of mineral composition in a northeastern Greenland ice-core (EGRIP) over the past 100 years. The ice core dust composition and its variation differed significantly from a northwestern Greenland ice core, which is likely due to differences in the geological sources of the dust. Our results suggest that the EGRIP ice core dust was constantly supplied from Northern Eurasia, North America, and Asia with minor contribution from Greenland coast.
Takashi Obase, Ayako Abe-Ouchi, Fuyuki Saito, Shun Tsutaki, Shuji Fujita, Kenji Kawamura, and Hideaki Motoyama
The Cryosphere, 17, 2543–2562, https://doi.org/10.5194/tc-17-2543-2023, https://doi.org/10.5194/tc-17-2543-2023, 2023
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We use a one-dimensional ice-flow model to examine the most suitable core location near Dome Fuji (DF), Antarctica. This model computes the temporal evolution of age and temperature from past to present. We investigate the influence of different parameters of climate and ice sheet on the ice's basal age and compare the results with ground radar surveys. We find that the local ice thickness primarily controls the age because it is critical to the basal melting, which can eliminate the old ice.
Franz Martin Schnaiter, Claudia Linke, Eija Asmi, Henri Servomaa, Antti-Pekka Hyvärinen, Sho Ohata, Yutaka Kondo, and Emma Järvinen
Atmos. Meas. Tech., 16, 2753–2769, https://doi.org/10.5194/amt-16-2753-2023, https://doi.org/10.5194/amt-16-2753-2023, 2023
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Light-absorbing particles from combustion processes are important contributors to climate warming. Their highly variable spectral light absorption properties need to be monitored in the field. Commonly used methods show measurement artefacts that are difficult to correct. We introduce a new instrument that is based on the photoacoustic effect. Long-term operation in the Finnish Arctic demonstrates the applicability of the new instrument for unattended light absorption monitoring.
Christo Buizert, Sarah Shackleton, Jeffrey P. Severinghaus, William H. G. Roberts, Alan Seltzer, Bernhard Bereiter, Kenji Kawamura, Daniel Baggenstos, Anaïs J. Orsi, Ikumi Oyabu, Benjamin Birner, Jacob D. Morgan, Edward J. Brook, David M. Etheridge, David Thornton, Nancy Bertler, Rebecca L. Pyne, Robert Mulvaney, Ellen Mosley-Thompson, Peter D. Neff, and Vasilii V. Petrenko
Clim. Past, 19, 579–606, https://doi.org/10.5194/cp-19-579-2023, https://doi.org/10.5194/cp-19-579-2023, 2023
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It is unclear how different components of the global atmospheric circulation, such as the El Niño effect, respond to large-scale climate change. We present a new ice core gas proxy, called krypton-86 excess, that reflects past storminess in Antarctica. We present data from 11 ice cores that suggest the new proxy works. We present a reconstruction of changes in West Antarctic storminess over the last 24 000 years and suggest these are caused by north–south movement of the tropical rain belt.
Ikumi Oyabu, Kenji Kawamura, Shuji Fujita, Ryo Inoue, Hideaki Motoyama, Kotaro Fukui, Motohiro Hirabayashi, Yu Hoshina, Naoyuki Kurita, Fumio Nakazawa, Hiroshi Ohno, Konosuke Sugiura, Toshitaka Suzuki, Shun Tsutaki, Ayako Abe-Ouchi, Masashi Niwano, Frédéric Parrenin, Fuyuki Saito, and Masakazu Yoshimori
Clim. Past, 19, 293–321, https://doi.org/10.5194/cp-19-293-2023, https://doi.org/10.5194/cp-19-293-2023, 2023
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We reconstructed accumulation rate around Dome Fuji, Antarctica, over the last 5000 years from 15 shallow ice cores and seven snow pits. We found a long-term decreasing trend in the preindustrial period, which may be associated with secular surface cooling and sea ice expansion. Centennial-scale variations were also found, which may partly be related to combinations of volcanic, solar and greenhouse gas forcings. The most rapid and intense increases of accumulation rate occurred since 1850 CE.
Kouji Adachi, Yutaka Tobo, Makoto Koike, Gabriel Freitas, Paul Zieger, and Radovan Krejci
Atmos. Chem. Phys., 22, 14421–14439, https://doi.org/10.5194/acp-22-14421-2022, https://doi.org/10.5194/acp-22-14421-2022, 2022
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Ambient aerosol and cloud residual particles in the fine mode were collected at Zeppelin Observatory in Svalbard and were analyzed using transmission electron microscopy. Fractions of mineral dust and sea salt particles increased in cloud residual samples collected at ambient temperatures below 0 °C. This study highlights the variety of aerosol and cloud residual particle compositions and mixing states that influence or are influenced by aerosol–cloud interactions in Arctic low-level clouds.
Shun Tsutaki, Shuji Fujita, Kenji Kawamura, Ayako Abe-Ouchi, Kotaro Fukui, Hideaki Motoyama, Yu Hoshina, Fumio Nakazawa, Takashi Obase, Hiroshi Ohno, Ikumi Oyabu, Fuyuki Saito, Konosuke Sugiura, and Toshitaka Suzuki
The Cryosphere, 16, 2967–2983, https://doi.org/10.5194/tc-16-2967-2022, https://doi.org/10.5194/tc-16-2967-2022, 2022
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We constructed an ice thickness map across the Dome Fuji region, East Antarctica, from improved radar data and previous data that had been collected since the late 1980s. The data acquired using the improved radar systems allowed basal topography to be identified with higher accuracy. The new ice thickness data show the bedrock topography, particularly the complex terrain of subglacial valleys and highlands south of Dome Fuji, with substantially high detail.
Tomotaka Saruya, Shuji Fujita, Yoshinori Iizuka, Atsushi Miyamoto, Hiroshi Ohno, Akira Hori, Wataru Shigeyama, Motohiro Hirabayashi, and Kumiko Goto-Azuma
The Cryosphere, 16, 2985–3003, https://doi.org/10.5194/tc-16-2985-2022, https://doi.org/10.5194/tc-16-2985-2022, 2022
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Crystal orientation fabrics (COF) of the Dome Fuji ice core were investigated with an innovative method with unprecedentedly high statistical significance and dense depth coverage. The COF profile and its fluctuation were found to be highly dependent on concentrations of chloride ion and dust. The data suggest deformation of ice at the deepest zone is highly influenced by COF fluctuations that progressively develop from the near-surface firn toward the deepest zone within ice sheets.
Jacob D. Morgan, Christo Buizert, Tyler J. Fudge, Kenji Kawamura, Jeffrey P. Severinghaus, and Cathy M. Trudinger
The Cryosphere, 16, 2947–2966, https://doi.org/10.5194/tc-16-2947-2022, https://doi.org/10.5194/tc-16-2947-2022, 2022
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The composition of air bubbles in Antarctic ice cores records information about past changes in properties of the snowpack. We find that, near the South Pole, thinner snowpack in the past is often due to steeper surface topography, in which faster winds erode the snow and deposit it in flatter areas. The slope and wind seem to also cause a seasonal bias in the composition of air bubbles in the ice core. These findings will improve interpretation of other ice cores from places with steep slopes.
Hitoshi Matsui, Tatsuhiro Mori, Sho Ohata, Nobuhiro Moteki, Naga Oshima, Kumiko Goto-Azuma, Makoto Koike, and Yutaka Kondo
Atmos. Chem. Phys., 22, 8989–9009, https://doi.org/10.5194/acp-22-8989-2022, https://doi.org/10.5194/acp-22-8989-2022, 2022
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Using a global aerosol model, we find that the source contributions to radiative effects of black carbon (BC) in the Arctic are quite different from those to mass concentrations and deposition flux of BC in the Arctic. This is because microphysical properties (e.g., mixing state), altitudes, and seasonal variations of BC in the atmosphere differ among emissions sources. These differences need to be considered for accurate simulations of Arctic BC and its source contributions and climate impacts.
Yota Sato, Koji Fujita, Hiroshi Inoue, Akiko Sakai, and Karma
The Cryosphere, 16, 2643–2654, https://doi.org/10.5194/tc-16-2643-2022, https://doi.org/10.5194/tc-16-2643-2022, 2022
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We investigate fluctuations in Bhutanese lake-terminating glaciers focusing on the dynamics change before and after proglacial lake formation at Thorthormi Glacier (TG) based on photogrammetry, satellite, and GPS surveys. The thinning rate of TG became double compared to before proglacial lake formation, and the flow velocity has also sped up considerably. Those changes would be due to the reduction in longitudinal ice compression by the detachment of the glacier terminus from the end moraine.
Giyoon Lee, Jinho Ahn, Hyeontae Ju, Florian Ritterbusch, Ikumi Oyabu, Christo Buizert, Songyi Kim, Jangil Moon, Sambit Ghosh, Kenji Kawamura, Zheng-Tian Lu, Sangbum Hong, Chang Hee Han, Soon Do Hur, Wei Jiang, and Guo-Min Yang
The Cryosphere, 16, 2301–2324, https://doi.org/10.5194/tc-16-2301-2022, https://doi.org/10.5194/tc-16-2301-2022, 2022
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Blue-ice areas (BIAs) have several advantages for reconstructing past climate. However, the complicated ice flow in the area hinders constraining the age. We applied state-of-the-art techniques and found that the ages cover the last deglaciation period. Our study demonstrates that the BIA in northern Victoria Land may help reconstruct the past climate during the termination of the last glacial period.
Taku Umezawa, Satoshi Sugawara, Kenji Kawamura, Ikumi Oyabu, Stephen J. Andrews, Takuya Saito, Shuji Aoki, and Takakiyo Nakazawa
Atmos. Chem. Phys., 22, 6899–6917, https://doi.org/10.5194/acp-22-6899-2022, https://doi.org/10.5194/acp-22-6899-2022, 2022
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Greenhouse gas methane in the Arctic atmosphere has not been accurately reported for 1900–1980 from either direct observations or ice core reconstructions. By using trace gas data from firn (compacted snow layers above ice sheet), air samples at two Greenland sites, and a firn air transport model, this study suggests a likely range of the Arctic methane reconstruction for the 20th century. Atmospheric scenarios from two previous studies are also evaluated for consistency with the firn data sets.
Yange Deng, Hiroaki Fujinari, Hikari Yai, Kojiro Shimada, Yuzo Miyazaki, Eri Tachibana, Dhananjay K. Deshmukh, Kimitaka Kawamura, Tomoki Nakayama, Shiori Tatsuta, Mingfu Cai, Hanbing Xu, Fei Li, Haobo Tan, Sho Ohata, Yutaka Kondo, Akinori Takami, Shiro Hatakeyama, and Michihiro Mochida
Atmos. Chem. Phys., 22, 5515–5533, https://doi.org/10.5194/acp-22-5515-2022, https://doi.org/10.5194/acp-22-5515-2022, 2022
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Offline analyses of the hygroscopicity and composition of atmospheric aerosols are complementary to online analyses in view of the applicability to broader sizes, specific compound groups, and investigations at remote sites. This offline study characterized the composition of water-soluble matter in aerosols and their humidity-dependent hygroscopicity on Okinawa, a receptor site of East Asian outflow. Further, comparison with online analyses showed the appropriateness of the offline method.
Tobias Erhardt, Matthias Bigler, Urs Federer, Gideon Gfeller, Daiana Leuenberger, Olivia Stowasser, Regine Röthlisberger, Simon Schüpbach, Urs Ruth, Birthe Twarloh, Anna Wegner, Kumiko Goto-Azuma, Takayuki Kuramoto, Helle A. Kjær, Paul T. Vallelonga, Marie-Louise Siggaard-Andersen, Margareta E. Hansson, Ailsa K. Benton, Louise G. Fleet, Rob Mulvaney, Elizabeth R. Thomas, Nerilie Abram, Thomas F. Stocker, and Hubertus Fischer
Earth Syst. Sci. Data, 14, 1215–1231, https://doi.org/10.5194/essd-14-1215-2022, https://doi.org/10.5194/essd-14-1215-2022, 2022
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The datasets presented alongside this manuscript contain high-resolution concentration measurements of chemical impurities in deep ice cores, NGRIP and NEEM, from the Greenland ice sheet. The impurities originate from the deposition of aerosols to the surface of the ice sheet and are influenced by source, transport and deposition processes. Together, these records contain detailed, multi-parameter records of past climate variability over the last glacial period.
Rupert Holzinger, Oliver Eppers, Kouji Adachi, Heiko Bozem, Markus Hartmann, Andreas Herber, Makoto Koike, Dylan B. Millet, Nobuhiro Moteki, Sho Ohata, Frank Stratmann, and Atsushi Yoshida
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-95, https://doi.org/10.5194/acp-2022-95, 2022
Revised manuscript not accepted
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In spring 2018 the research aircraft Polar 5 conducted flights in the Arctic atmosphere. The flight operation was from Station Nord in Greenland, 1700 km north of the Arctic Circle (81°43'N, 17°47'W). Using a mass spectrometer we measured more than 100 organic compounds in the air. We found a clear signature of natural organic compounds that are transported from forests to the high Arctic. These compounds have the potential to change the cloud cover and energy budget of the Arctic region.
Ikumi Oyabu, Kenji Kawamura, Tsutomu Uchida, Shuji Fujita, Kyotaro Kitamura, Motohiro Hirabayashi, Shuji Aoki, Shinji Morimoto, Takakiyo Nakazawa, Jeffrey P. Severinghaus, and Jacob D. Morgan
The Cryosphere, 15, 5529–5555, https://doi.org/10.5194/tc-15-5529-2021, https://doi.org/10.5194/tc-15-5529-2021, 2021
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We present O2/N2 and Ar/N2 records from the Dome Fuji ice core through the bubbly ice, bubble–clathrate transition, and clathrate ice zones without gas-loss fractionation. The insolation signal is preserved through the clathrate formation. The relationship between Ar/Ν2 and Ο2/Ν2 suggests that the fractionation for the bubble–clathrate transition is mass independent, while the bubble close-off process involves a combination of mass-independent and mass-dependent fractionation for O2 and Ar.
Sho Ohata, Makoto Koike, Atsushi Yoshida, Nobuhiro Moteki, Kouji Adachi, Naga Oshima, Hitoshi Matsui, Oliver Eppers, Heiko Bozem, Marco Zanatta, and Andreas B. Herber
Atmos. Chem. Phys., 21, 15861–15881, https://doi.org/10.5194/acp-21-15861-2021, https://doi.org/10.5194/acp-21-15861-2021, 2021
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Vertical profiles of black carbon (BC) in the Arctic were measured during the PAMARCMiP aircraft-based experiment in spring 2018 and compared with those observed during previous aircraft campaigns in 2008, 2010, and 2015. Their differences were explained primarily by the year-to-year variation of biomass burning activities in northern midlatitudes over Eurasia. Our observations provide a bases to evaluate numerical model simulations that assess the BC radiative effects in the Arctic spring.
Sho Ohata, Tatsuhiro Mori, Yutaka Kondo, Sangeeta Sharma, Antti Hyvärinen, Elisabeth Andrews, Peter Tunved, Eija Asmi, John Backman, Henri Servomaa, Daniel Veber, Konstantinos Eleftheriadis, Stergios Vratolis, Radovan Krejci, Paul Zieger, Makoto Koike, Yugo Kanaya, Atsushi Yoshida, Nobuhiro Moteki, Yongjing Zhao, Yutaka Tobo, Junji Matsushita, and Naga Oshima
Atmos. Meas. Tech., 14, 6723–6748, https://doi.org/10.5194/amt-14-6723-2021, https://doi.org/10.5194/amt-14-6723-2021, 2021
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Reliable values of mass absorption cross sections (MACs) of black carbon (BC) are required to determine mass concentrations of BC at Arctic sites using different types of filter-based absorption photometers. We successfully estimated MAC values for these instruments through comparison with independent measurements of BC by a continuous soot monitoring system called COSMOS. These MAC values are consistent with each other and applicable to study spatial and temporal variation in BC in the Arctic.
Eija Asmi, John Backman, Henri Servomaa, Aki Virkkula, Maria I. Gini, Konstantinos Eleftheriadis, Thomas Müller, Sho Ohata, Yutaka Kondo, and Antti Hyvärinen
Atmos. Meas. Tech., 14, 5397–5413, https://doi.org/10.5194/amt-14-5397-2021, https://doi.org/10.5194/amt-14-5397-2021, 2021
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Absorbing aerosols are warming the planet and accurate measurements of their concentrations in pristine environments are needed. We applied eight different absorbing-aerosol measurement methods in a field campaign at the Arctic Pallas station. The filter-based techniques were found to be the most sensitive to detect the minuscule amounts of black carbon present, showing a 40 % agreement between them. Our results help to reduce uncertainties in absorbing aerosol measurements.
Naoko Nagatsuka, Kumiko Goto-Azuma, Akane Tsushima, Koji Fujita, Sumito Matoba, Yukihiko Onuma, Remi Dallmayr, Moe Kadota, Motohiro Hirabayashi, Jun Ogata, Yoshimi Ogawa-Tsukagawa, Kyotaro Kitamura, Masahiro Minowa, Yuki Komuro, Hideaki Motoyama, and Teruo Aoki
Clim. Past, 17, 1341–1362, https://doi.org/10.5194/cp-17-1341-2021, https://doi.org/10.5194/cp-17-1341-2021, 2021
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Here we present a first high-temporal-resolution record of mineral composition in a Greenland ice core (SIGMA-D) over the past 100 years using SEM–EDS analysis. Our results show that the ice core dust composition varied on multi-decadal scales, which was likely affected by local temperature changes. We suggest that the ice core dust was constantly supplied from distant sources (mainly northern Canada) as well as local ice-free areas in warm periods (1915 to 1949 and 2005 to 2013).
Linn Karlsson, Radovan Krejci, Makoto Koike, Kerstin Ebell, and Paul Zieger
Atmos. Chem. Phys., 21, 8933–8959, https://doi.org/10.5194/acp-21-8933-2021, https://doi.org/10.5194/acp-21-8933-2021, 2021
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Aerosol–cloud interactions in the Arctic are poorly understood largely due to a lack of observational data. We present the first direct, long-term measurements of cloud residuals, i.e. the particles that remain when cloud droplets and ice crystals are dried. These detailed observations of cloud residuals cover more than 2 years, which is unique for the Arctic and globally. This work studies the size distributions of cloud residuals, their seasonality, and dependence on meteorology.
Kouji Adachi, Naga Oshima, Sho Ohata, Atsushi Yoshida, Nobuhiro Moteki, and Makoto Koike
Atmos. Chem. Phys., 21, 3607–3626, https://doi.org/10.5194/acp-21-3607-2021, https://doi.org/10.5194/acp-21-3607-2021, 2021
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Aerosol particles influence the Arctic climate by interacting with solar radiation, forming clouds, and melting surface snow and ice. Individual-particle analyses using transmission electron microscopy (TEM) and model simulations provide evidence of biomass burning and anthropogenic contributions to the Arctic aerosols by showing a wide range of compositions and mixing states depending on sampling altitude. Our results reveal the aerosol aging processes and climate influences in the Arctic.
Ikumi Oyabu, Kenji Kawamura, Kyotaro Kitamura, Remi Dallmayr, Akihiro Kitamura, Chikako Sawada, Jeffrey P. Severinghaus, Ross Beaudette, Anaïs Orsi, Satoshi Sugawara, Shigeyuki Ishidoya, Dorthe Dahl-Jensen, Kumiko Goto-Azuma, Shuji Aoki, and Takakiyo Nakazawa
Atmos. Meas. Tech., 13, 6703–6731, https://doi.org/10.5194/amt-13-6703-2020, https://doi.org/10.5194/amt-13-6703-2020, 2020
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Air in polar ice cores provides information on past atmosphere and climate. We present a new method for simultaneously measuring eight gases (CH4, N2O and CO2 concentrations; isotopic ratios of N2 and O2; elemental ratios between N2, O2 and Ar; and total air content) from single ice-core samples with high precision.
Sho Ohata, Tatsuhiro Mori, Yutaka Kondo, Sangeeta Sharma, Antti Hyvärinen, Elisabeth Andrews, Peter Tunved, Eija Asmi, John Backman, Henri Servomaa, Daniel Veber, Makoto Koike, Yugo Kanaya, Atsushi Yoshida, Nobuhiro Moteki, Yongjing Zhao, Junji Matsushita, and Naga Oshima
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-1190, https://doi.org/10.5194/acp-2020-1190, 2020
Preprint withdrawn
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Reliable values of mass absorption cross sections (MAC) of black carbon (BC) are required to determine mass concentrations of BC at Arctic sites using different types of filter-based absorption photometers. We successfully estimated MAC values for these instruments through comparison with independent measurements of BC by continuous soot monitoring system called COSMOS. These MAC values are consistent with each other and applicable to study spatial and temporal variation of BC in the Arctic.
Xavier Fettweis, Stefan Hofer, Uta Krebs-Kanzow, Charles Amory, Teruo Aoki, Constantijn J. Berends, Andreas Born, Jason E. Box, Alison Delhasse, Koji Fujita, Paul Gierz, Heiko Goelzer, Edward Hanna, Akihiro Hashimoto, Philippe Huybrechts, Marie-Luise Kapsch, Michalea D. King, Christoph Kittel, Charlotte Lang, Peter L. Langen, Jan T. M. Lenaerts, Glen E. Liston, Gerrit Lohmann, Sebastian H. Mernild, Uwe Mikolajewicz, Kameswarrao Modali, Ruth H. Mottram, Masashi Niwano, Brice Noël, Jonathan C. Ryan, Amy Smith, Jan Streffing, Marco Tedesco, Willem Jan van de Berg, Michiel van den Broeke, Roderik S. W. van de Wal, Leo van Kampenhout, David Wilton, Bert Wouters, Florian Ziemen, and Tobias Zolles
The Cryosphere, 14, 3935–3958, https://doi.org/10.5194/tc-14-3935-2020, https://doi.org/10.5194/tc-14-3935-2020, 2020
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We evaluated simulated Greenland Ice Sheet surface mass balance from 5 kinds of models. While the most complex (but expensive to compute) models remain the best, the faster/simpler models also compare reliably with observations and have biases of the same order as the regional models. Discrepancies in the trend over 2000–2012, however, suggest that large uncertainties remain in the modelled future SMB changes as they are highly impacted by the meltwater runoff biases over the current climate.
Cited articles
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Arienzo, M. M., McConnell, J. R., Murphy, L. N., Chellman, N., Das S., Kipfstuhl, S., and Mulvaney, R.: Holocene black carbon in Antarctica paralleled Southern Hemisphere climate, J. Geophys. Res.-Atmos., 122, 6713–6728, https://doi.org/10.1002/2017JD026599, 2017.
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Bigler, M., Svensson, A., Kettner, E., Vallelonga, P., Nielsen, M. E., and Steffensen, J. P.: Optimization of high-resolution continuous flow analysis for transient climate signals in ice cores, Environ. Sci. Technol., 45, 4483–4489, https://doi.org/10.1021/es200118j, 2011.
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Bisiaux, M. M., Edwards, R., McConnell, J. R., Curran, M. A. J., Van Ommen, T. D., Smith, A. M., Neumann, T. A., Pasteris, D. R., Penner, J. E., and Taylor, K.: Changes in black carbon deposition to Antarctica from two high-resolution ice core records, 1850–2000 AD, Atmos. Chem. Phys., 12, 4107–4115, https://doi.org/10.5194/acp-12-4107-2012, 2012b.
Bond, T. C., Doherty, S. J., Fahey, D. W., Forster, P. M., Berntsen, T., DeAngelo, B. J., Flanner, M. G., Ghan, S., Kärcher, B., Koch, D., Kinne, S., Kondo, Y., Quinn, P. K., Sarofim, M. C., Schultz, M. G., Schulz, M., Venkataraman, C., Zhang, H., Zhang, S., Bellouin, N., Guttikunda, S. K., Hopke, P. K., Jacobson, M. Z., Kaiser, J. W., Klimont, Z., Lohmann, U., Schwarz, J. P., Shindell, D., Storelvmo, T., Warren, S. G., and Zender, C. S.: Bounding the role of black carbon in the climate system: A scientific assessment, J. Geophys. Res.-Atmos., 118, 5380–5552, https://doi.org/10.1002/jgrd.50171, 2013.
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Dallmayr, R., Goto-Azuma, K., Kjær, H. A., Azuma, N., Takata, M., Schüpbach, S., and Hirabayashi, M.: A high-resolution continuous flow analysis system for polar ice cores, B. Glaciol. Res., 34, 11–20, https://doi.org/10.5331/bgr.16R03, 2016.
Du, Z.-H., Xiao, C.-D., Dou, T.-F., Li, C.-J., Ding, M.-H., Sharma, S., Ma, X.-Y., Wang, S.-M., and Zhang, W.-B.: A shallow ice core from East Greenland showing a reduction in black carbon during 1990–2016, Adv. Clim. Change Res., 11, 360–369, https://doi.org/10.1016/j.accre.2020.11.009, 2020.
Erhardt, T., Jensen, C. M., Adolphi, F., Kjær, H. A., Dallmayr, R., Twarloh, B., Behrens, M., Hirabayashi, M., Fukuda, K., Ogata, J., Burgay, F., Scoto, F., Crotti, I., Spagnesi, A., Maffezzoli, N., Segato, D., Paleari, C., Mekhaldi, F., Muscheler, R., Darfeuil, S., and Fischer, H.: High-resolution aerosol data from the top 3.8 kyr of the East Greenland Ice coring Project (EGRIP) ice core, Earth Syst. Sci. Data, 15, 5079–5091, https://doi.org/10.5194/essd-15-5079-2023, 2023.
Gkinis, V., Popp, T. J., Blunier, T., Bigler, M., Schüpbach, S., Kettner, E., and Johnsen, S. J.: Water isotopic ratios from a continuously melted ice core sample, Atmos. Meas. Tech., 4, 2531–2542, https://doi.org/10.5194/amt-4-2531-2011, 2011.
Goto-Azuma, K., Dallmayr, R., Ogawa-Tsukagawa, Y., Fukuda, K., Ogata, J., Hirabayashi, M., Aoki, T., and Matoba, S.: Black carbon data from an ice core drilled at SIGMA-D, northwestern Greenland, 0.00, Arctic Data archive System (ADS) [data set], Japan, https://doi.org/10.17592/001.2019122306, 2024a.
Goto-Azuma, K., Ogawa-Tsukagawa, Y., Fukuda, K., Fujita, K., Hirabayashi, M., Dallmayr, R., Ogata, J., Moteki, N., Mori, T., Ohata, S., Kondo, Y., Koike, M., Matoba, S., and Aoki, T.: High-resolution analyses of concentrations and sizes of black carbon particles deposited on northwest Greenland over the past 350 years – Part 2: Seasonal and temporal trends in black carbon originated from fossil fuel combustion and biomass burning, EGUsphere [preprint], https://doi.org/10.5194/egusphere-2024-1498, 2024b.
Grieman, M. M., Hoffmann, H. M., Humby, J. D., Mulvaney, R., Nehrbass-Ahles, C., Rix, J., Thomas, E. R., Tuckwell, R., and Wolff, E. W.: Continuous flow analysis methods for sodium, magnesium, and calcium detection in the Skytrain ice core, J. Glaciol., 68, 90–100, https://doi.org/10.1017/jog.2021.75, 2022.
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Short summary
We developed a continuous flow analysis system to analyze an ice core from northwestern Greenland and coupled it with an improved refractory black carbon (rBC) measurement technique. This allowed accurate high-resolution analyses of size distributions and concentrations of rBC particles with diameters of 70 nm–4 μm for the past 350 years. Our results provide crucial insights into rBC's climatic effects. We also found previous ice core studies substantially underestimated rBC mass concentrations.
We developed a continuous flow analysis system to analyze an ice core from northwestern...
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