Articles | Volume 23, issue 7
https://doi.org/10.5194/acp-23-4149-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-4149-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| Highlight paper
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05 Apr 2023
Research article | Highlight paper |
| 05 Apr 2023
| 05 Apr 2023
Foreign emissions exacerbate PM2.5 pollution in China through nitrate chemistry
Jun-Wei Xu
Laboratory for Climate and Ocean–Atmosphere Studies, Department of
Atmospheric and Oceanic Sciences, School of Physics, Peking University,
Beijing, China
Laboratory for Climate and Ocean–Atmosphere Studies, Department of
Atmospheric and Oceanic Sciences, School of Physics, Peking University,
Beijing, China
Atmospheric Sciences Research Center, University at Albany, Albany,
NY, USA
Jamiu Adeniran
Laboratory for Climate and Ocean–Atmosphere Studies, Department of
Atmospheric and Oceanic Sciences, School of Physics, Peking University,
Beijing, China
Hao Kong
Laboratory for Climate and Ocean–Atmosphere Studies, Department of
Atmospheric and Oceanic Sciences, School of Physics, Peking University,
Beijing, China
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Gan Luo, Fangqun Yu, and Jonathan M. Moch
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Fangqun Yu, Alexey B. Nadykto, Gan Luo, and Jason Herb
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Fangqun Yu, Gan Luo, Arshad Arjunan Nair, James J. Schwab, James P. Sherman, and Yanda Zhang
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Viral Shah, Daniel J. Jacob, Ke Li, Rachel F. Silvern, Shixian Zhai, Mengyao Liu, Jintai Lin, and Qiang Zhang
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Hao Kong, Jintai Lin, Ruixiong Zhang, Mengyao Liu, Hongjian Weng, Ruijing Ni, Lulu Chen, Jingxu Wang, Yingying Yan, and Qiang Zhang
Atmos. Chem. Phys., 19, 12835–12856, https://doi.org/10.5194/acp-19-12835-2019, https://doi.org/10.5194/acp-19-12835-2019, 2019
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Atmos. Chem. Phys., 19, 8591–8617, https://doi.org/10.5194/acp-19-8591-2019, https://doi.org/10.5194/acp-19-8591-2019, 2019
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Xiao Lu, Lin Zhang, Youfan Chen, Mi Zhou, Bo Zheng, Ke Li, Yiming Liu, Jintai Lin, Tzung-May Fu, and Qiang Zhang
Atmos. Chem. Phys., 19, 8339–8361, https://doi.org/10.5194/acp-19-8339-2019, https://doi.org/10.5194/acp-19-8339-2019, 2019
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Lei Sun, Likun Xue, Yuhang Wang, Longlei Li, Jintai Lin, Ruijing Ni, Yingying Yan, Lulu Chen, Juan Li, Qingzhu Zhang, and Wenxing Wang
Atmos. Chem. Phys., 19, 1455–1469, https://doi.org/10.5194/acp-19-1455-2019, https://doi.org/10.5194/acp-19-1455-2019, 2019
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Yingying Yan, David Cabrera-Perez, Jintai Lin, Andrea Pozzer, Lu Hu, Dylan B. Millet, William C. Porter, and Jos Lelieveld
Geosci. Model Dev., 12, 111–130, https://doi.org/10.5194/gmd-12-111-2019, https://doi.org/10.5194/gmd-12-111-2019, 2019
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Mengyao Liu, Jintai Lin, K. Folkert Boersma, Gaia Pinardi, Yang Wang, Julien Chimot, Thomas Wagner, Pinhua Xie, Henk Eskes, Michel Van Roozendael, François Hendrick, Pucai Wang, Ting Wang, Yingying Yan, Lulu Chen, and Ruijing Ni
Atmos. Meas. Tech., 12, 1–21, https://doi.org/10.5194/amt-12-1-2019, https://doi.org/10.5194/amt-12-1-2019, 2019
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Fangqun Yu, Alexey B. Nadykto, Jason Herb, Gan Luo, Kirill M. Nazarenko, and Lyudmila A. Uvarova
Atmos. Chem. Phys., 18, 17451–17474, https://doi.org/10.5194/acp-18-17451-2018, https://doi.org/10.5194/acp-18-17451-2018, 2018
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By integrating several modeling methods, we find considerable contributions of foreign anthropogenic emissions to surface ozone over China (2–11 ppb). For anthropogenic ozone over China, the foreign contribution is 40–50 % below 2 km and 85 % in the upper troposphere. For total foreign anthropogenic ozone over China, the portion of transboundary ozone produced within foreign emission source regions is less than 50 %, with the rest produced by precursors transported out of those source regions.
Jingbo Mao, Fangqun Yu, Yan Zhang, Jingyu An, Lin Wang, Jun Zheng, Lei Yao, Gan Luo, Weichun Ma, Qi Yu, Cheng Huang, Li Li, and Limin Chen
Atmos. Chem. Phys., 18, 7933–7950, https://doi.org/10.5194/acp-18-7933-2018, https://doi.org/10.5194/acp-18-7933-2018, 2018
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A few pptv of gaseous amines have been observed to affect particle nucleation and growth, and it is necessary to understand the sources and concentrations of atmospheric amines. This study presents the source-dependent amines to ammonia emission ratios and simulates methylamines concentrations in a polluted region in China with WRF-Chem. The performance of simulations based on source-dependent ratios is much better than those based on fixed ratios that have been assumed in all previous studies.
Yingying Yan, Andrea Pozzer, Narendra Ojha, Jintai Lin, and Jos Lelieveld
Atmos. Chem. Phys., 18, 5589–5605, https://doi.org/10.5194/acp-18-5589-2018, https://doi.org/10.5194/acp-18-5589-2018, 2018
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Surface-based measurements from the EMEP network and EMAC model simulations are used to estimate the European surface ozone changes over 1995–2014. It shows a significantly decreasing trend in the 95th percentile ozone concentrations, while increasing in the 5th percentile ozone. Sensitivity simulations and statistical analysis show that a decrease in European anthropogenic emissions had contrasting effects on surface ozone trends between the 95th and 5th percentile levels.
Yingying Yan, Jintai Lin, and Cenlin He
Atmos. Chem. Phys., 18, 1185–1202, https://doi.org/10.5194/acp-18-1185-2018, https://doi.org/10.5194/acp-18-1185-2018, 2018
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Examining observed and simulated ozone at about 1000 sites during 1990–2014, we find a clear diurnal cycle both in the magnitude of ozone trends and in the relative importance of climate variability versus anthropogenic emissions to ozone changes, which has policy implications to mitigate ozone at night and other non-peak hours.
Maria Sand, Bjørn H. Samset, Yves Balkanski, Susanne Bauer, Nicolas Bellouin, Terje K. Berntsen, Huisheng Bian, Mian Chin, Thomas Diehl, Richard Easter, Steven J. Ghan, Trond Iversen, Alf Kirkevåg, Jean-François Lamarque, Guangxing Lin, Xiaohong Liu, Gan Luo, Gunnar Myhre, Twan van Noije, Joyce E. Penner, Michael Schulz, Øyvind Seland, Ragnhild B. Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Fangqun Yu, Kai Zhang, and Hua Zhang
Atmos. Chem. Phys., 17, 12197–12218, https://doi.org/10.5194/acp-17-12197-2017, https://doi.org/10.5194/acp-17-12197-2017, 2017
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The role of aerosols in the changing polar climate is not well understood and the aerosols are poorly constrained in the models. In this study we have compared output from 16 different aerosol models with available observations at both poles. We show that the model median is representative of the observations, but the model spread is large. The Arctic direct aerosol radiative effect over the industrial area is positive during spring due to black carbon and negative during summer due to sulfate.
Hongyan Zhao, Xin Li, Qiang Zhang, Xujia Jiang, Jintai Lin, Glen P. Peters, Meng Li, Guannan Geng, Bo Zheng, Hong Huo, Lin Zhang, Haikun Wang, Steven J. Davis, and Kebin He
Atmos. Chem. Phys., 17, 10367–10381, https://doi.org/10.5194/acp-17-10367-2017, https://doi.org/10.5194/acp-17-10367-2017, 2017
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Effective and efficient control of air pollution relies upon an understanding of the pollution sources. We conduct an interdisciplinary study and find that 33 % of China’s PM2.5-related premature mortality in 2010 were caused by production emission in other regions; 56 % of the mortality was related to consumption in other regions. Multilateral and multi-stage cooperation under a regional sustainable development framework is in urgent need to mitigate air pollution and related health impacts.
Katherine R. Travis, Daniel J. Jacob, Christoph A. Keller, Shi Kuang, Jintai Lin, Michael J. Newchurch, and Anne M. Thompson
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-596, https://doi.org/10.5194/acp-2017-596, 2017
Preprint retracted
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Models severely overestimate surface ozone in the Southeast US during summertime which has implications for the design of air quality regulations. We use a model (GEOS-Chem) to interpret ozone observations from a suite of observations taken during August–September 2013. The model is unbiased relative to observations below 1 km but is biased high at the surface. We attribute this bias to model representation error, an underestimate in low-cloud, and insufficient treatment of vertical mixing.
Fangqun Yu, Gan Luo, Alexey B. Nadykto, and Jason Herb
Atmos. Chem. Phys., 17, 4997–5005, https://doi.org/10.5194/acp-17-4997-2017, https://doi.org/10.5194/acp-17-4997-2017, 2017
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H2SO4–organics clustering thermodynamics from quantum studies has been employed to develop a scheme to include temperature dependence in an H2SO4–organics nucleation parameterization. We show that temperature has a strong impact on nucleation rates, particle number concentrations, and aerosol first indirect radiative forcing in summer. To our knowledge, the study represents the first attempt to study the temperature effect on organics-mediated nucleation in the global atmosphere.
Guannan Geng, Qiang Zhang, Randall V. Martin, Jintai Lin, Hong Huo, Bo Zheng, Siwen Wang, and Kebin He
Atmos. Chem. Phys., 17, 4131–4145, https://doi.org/10.5194/acp-17-4131-2017, https://doi.org/10.5194/acp-17-4131-2017, 2017
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We investigated the impact of spatial proxies on the representation of gridded emissions by comparing six gridded NOx emission datasets over China developed from the same magnitude of emissions and different spatial proxies. GEOS-Chem-modeled NO2 columns from the six gridded emissions are compared with satellite-based columns from OMI. Results show that differences between modeled and satellite-based NO2 columns are sensitive to the spatial proxies used in the gridded emission inventories.
Alba Lorente, K. Folkert Boersma, Huan Yu, Steffen Dörner, Andreas Hilboll, Andreas Richter, Mengyao Liu, Lok N. Lamsal, Michael Barkley, Isabelle De Smedt, Michel Van Roozendael, Yang Wang, Thomas Wagner, Steffen Beirle, Jin-Tai Lin, Nickolay Krotkov, Piet Stammes, Ping Wang, Henk J. Eskes, and Maarten Krol
Atmos. Meas. Tech., 10, 759–782, https://doi.org/10.5194/amt-10-759-2017, https://doi.org/10.5194/amt-10-759-2017, 2017
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Choices and assumptions made to represent the state of the atmosphere introduce an uncertainty of 42 % in the air mass factor calculation in trace gas satellite retrievals in polluted regions. The AMF strongly depends on the choice of a priori trace gas profile, surface albedo data set and the correction method to account for clouds and aerosols. We call for well-designed validation exercises focusing on situations when AMF structural uncertainty has the highest impact on satellite retrievals.
Yuanzheng Cui, Jintai Lin, Chunqiao Song, Mengyao Liu, Yingying Yan, Yuan Xu, and Bo Huang
Atmos. Chem. Phys., 16, 6207–6221, https://doi.org/10.5194/acp-16-6207-2016, https://doi.org/10.5194/acp-16-6207-2016, 2016
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We find rapid NO2 growth over Western China over 2005–2013 at a rate which exceeds the rates over the well-known polluted regions in the east. A nested GEOS-Chem simulation and Chinese official emission data confirm that anthropogenic emissions are the main driver of NO2 variations. Additional socioeconomic analysis suggests that this rapid NO2 growth is likely related to the fast industrialization and urbanization along with the "Go West" movement as well as relatively weak emission controls.
Yingying Yan, Jintai Lin, Jinxuan Chen, and Lu Hu
Atmos. Chem. Phys., 16, 2381–2400, https://doi.org/10.5194/acp-16-2381-2016, https://doi.org/10.5194/acp-16-2381-2016, 2016
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We use a newly built two-way coupling system of the GEOS-Chem CTM to simulate the global tropospheric O3 in 2009. It significantly improves the simulation upon the global model by comparisons with a suite of ground, aircraft, and satellite measurements, also reduces the global OH by 5 % with enhancements by 5 % in the lifetimes of MCF and methane. Therefore, improving model representations of small-scale processes is a critical step forward to understanding the global tropospheric chemistry.
F. Yu, G. Luo, S. C. Pryor, P. R. Pillai, S. H. Lee, J. Ortega, J. J. Schwab, A. G. Hallar, W. R. Leaitch, V. P. Aneja, J. N. Smith, J. T. Walker, O. Hogrefe, and K. L. Demerjian
Atmos. Chem. Phys., 15, 13993–14003, https://doi.org/10.5194/acp-15-13993-2015, https://doi.org/10.5194/acp-15-13993-2015, 2015
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The role of low-volatility organics in new particle formation (NPF) in the atmosphere is assessed. An empirical formulation in which formation rate is a function of the concentrations of sulfuric acid and low-volatility organics significantly overpredicts NPF in the summer.
Two different schemes predict quite different nucleation rates (including their spatial patterns), concentrations of cloud condensation nuclei, and aerosol first indirect radiative forcing in North America.
J.-T. Lin, M.-Y. Liu, J.-Y. Xin, K. F. Boersma, R. Spurr, R. Martin, and Q. Zhang
Atmos. Chem. Phys., 15, 11217–11241, https://doi.org/10.5194/acp-15-11217-2015, https://doi.org/10.5194/acp-15-11217-2015, 2015
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We conduct an improved OMI-based retrieval of tropospheric NO2 VCDs (POMINO) over China by explicitly accounting for aerosol optical effects and surface reflectance anisotropy. Compared to the traditional implicit aerosol treatment, an explicit treatment greatly lowers NO2 VCDs and subsequently estimated NOx emissions over eastern China, but with large spatiotemporal dependence. An explicit treatment also better captures high-pollution days. Effects of surface reflectance treatments are smaller.
Z. Jiang, J. R. Worden, D. B. A. Jones, J.-T. Lin, W. W. Verstraeten, and D. K. Henze
Atmos. Chem. Phys., 15, 99–112, https://doi.org/10.5194/acp-15-99-2015, https://doi.org/10.5194/acp-15-99-2015, 2015
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We use satellite measurements of O3, CO and NO2 from TES, MOPITT and OMI to quantify O3 precursor emissions for 2006 and their impact on free tropospheric O3 over northeastern Asia. Using the adjoint of GEOS-Chem, we found that Chinese emissions have the largest influence on the free tropospheric O3. The contributions from lightning NOx in summer and India and southeastern Asia emissions in winter are sizable, comparable with Chinese emissions.
Y.-Y. Yan, J.-T. Lin, Y. Kuang, D. Yang, and L. Zhang
Atmos. Chem. Phys., 14, 12649–12663, https://doi.org/10.5194/acp-14-12649-2014, https://doi.org/10.5194/acp-14-12649-2014, 2014
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Limited by coarse resolutions, global chemical transport models cannot well capture small-scale nonlinear processes. To alleviate the problem, we develop a two-way coupled system to integrate the global GEOS-Chem model and its three high-resolution nested models covering Asia, Europe and North America. Confirmed by comparisons with observations, the coupled system improves upon the global model with a 10% increase in global tropospheric CO, a 4% decrease in OH and a 4% increase in MCF lifetime.
F. Yu and G. Luo
Atmos. Chem. Phys., 14, 12455–12464, https://doi.org/10.5194/acp-14-12455-2014, https://doi.org/10.5194/acp-14-12455-2014, 2014
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Global lifetimes and concentrations of gaseous methylamines (MMA, DMA, and TMA) have been simulated.
Oxidation and aerosol uptakes are dominant sinks for these methylamines. The oxidation alone leads to their lifetimes of 5-10h in most parts of low and middle latitude regions. The uptake by secondary species can shorten their lifetime to as low as 1-2h over central Europe, eastern Asia, and the eastern US.
The modeled concentrations are substantially lower than observed values available.
G. W. Mann, K. S. Carslaw, C. L. Reddington, K. J. Pringle, M. Schulz, A. Asmi, D. V. Spracklen, D. A. Ridley, M. T. Woodhouse, L. A. Lee, K. Zhang, S. J. Ghan, R. C. Easter, X. Liu, P. Stier, Y. H. Lee, P. J. Adams, H. Tost, J. Lelieveld, S. E. Bauer, K. Tsigaridis, T. P. C. van Noije, A. Strunk, E. Vignati, N. Bellouin, M. Dalvi, C. E. Johnson, T. Bergman, H. Kokkola, K. von Salzen, F. Yu, G. Luo, A. Petzold, J. Heintzenberg, A. Clarke, J. A. Ogren, J. Gras, U. Baltensperger, U. Kaminski, S. G. Jennings, C. D. O'Dowd, R. M. Harrison, D. C. S. Beddows, M. Kulmala, Y. Viisanen, V. Ulevicius, N. Mihalopoulos, V. Zdimal, M. Fiebig, H.-C. Hansson, E. Swietlicki, and J. S. Henzing
Atmos. Chem. Phys., 14, 4679–4713, https://doi.org/10.5194/acp-14-4679-2014, https://doi.org/10.5194/acp-14-4679-2014, 2014
J.-T. Lin, R. V. Martin, K. F. Boersma, M. Sneep, P. Stammes, R. Spurr, P. Wang, M. Van Roozendael, K. Clémer, and H. Irie
Atmos. Chem. Phys., 14, 1441–1461, https://doi.org/10.5194/acp-14-1441-2014, https://doi.org/10.5194/acp-14-1441-2014, 2014
J.-T. Lin, Z. Liu, Q. Zhang, H. Liu, J. Mao, and G. Zhuang
Atmos. Chem. Phys., 12, 12255–12275, https://doi.org/10.5194/acp-12-12255-2012, https://doi.org/10.5194/acp-12-12255-2012, 2012
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Modelling of atmospheric variability in gas and aerosols during the ACROSS campaign 2022 of the greater Paris area: evaluation of the meteorology, dynamics and chemistry
Spatial–temporal patterns in anthropogenic and biomass burning emission contributions to air pollution and mortality burden changes in India from 1995 to 2014
A comprehensive global modeling assessment of nitrate heterogeneous formation on desert dust
AERO-MAP: a data compilation and modeling approach to understand spatial variability in fine- and coarse-mode aerosol composition
Long-term trends in aerosol properties derived from AERONET measurements
Impacts of sea ice leads on sea salt aerosols and atmospheric chemistry in the Arctic
Dimethyl sulfide chemistry over the industrial era: comparison of key oxidation mechanisms and long-term observations
Driving factors of aerosol acidity: a new hierarchical quantitative analysis framework and its application in Changzhou, China
Understanding the long-term trend of organic aerosol and the influences from anthropogenic emission and regional climate change in China
Population exposure to outdoor NO2, black carbon, and ultrafine and fine particles over Paris with multi-scale modelling down to the street scale
Predicted impacts of heterogeneous chemical pathways on particulate sulfur over Fairbanks (Alaska), the Northern Hemisphere, and the Contiguous United States
Critical load exceedances for North America and Europe using an ensemble of models and an investigation of causes of environmental impact estimate variability: an AQMEII4 study
Impacts of meteorology and emission reductions on haze pollution during the lockdown in the North China Plain
Impact of mineral dust on the global nitrate aerosol direct and indirect radiative effect
The surface tension and cloud condensation nuclei (CCN) activation of sea spray aerosol particles
Exploring the processes controlling secondary inorganic aerosol: evaluating the global GEOS-Chem simulation using a suite of aircraft campaigns
Influence of land cover change on atmospheric organic gases, aerosols, and radiative effects
Quantifying the impacts of marine aerosols over the southeast Atlantic Ocean using a chemical transport model: implications for aerosol–cloud interactions
Quantifying the impact of global nitrate aerosol on tropospheric composition fields and its production from lightning NOx
Source-explicit estimation of brown carbon in the polluted atmosphere over North China Plain: implications for distribution, absorption and direct radiative effect
Rapid oxidation of phenolic compounds by O3 and HO●: effects of the air–water interface and mineral dust in tropospheric chemical processes
Uncertainties in the effects of organic aerosol coatings on polycyclic aromatic hydrocarbon concentrations and their estimated health effects
Modeling the contribution of leads to sea spray aerosol in the high Arctic
Trends and Drivers of Soluble Iron Deposition from East Asian Dust to the Northwest Pacific: A Springtime Analysis (2001–2017)
Implications of Reduced-Complexity Aerosol Thermodynamics on Organic Aerosol Mass Concentration and Composition over North America
Importance of aerosol composition and aerosol vertical profiles in global spatial variation in the relationship between PM2.5 and aerosol optical depth
The co-benefits of a low-carbon future for PM2.5 and O3 air pollution in Europe
Assessing the effectiveness of SO2, NOx, and NH3 emission reductions in mitigating winter PM2.5 in Taiwan using CMAQ
Modelling of atmospheric concentrations of fungal spores: a 2-year simulation over France using CHIMERE
Cluster-dynamics-based parameterization for sulfuric acid–dimethylamine nucleation: comparison and selection through box and three-dimensional modeling
Observed and CMIP6-model-simulated organic aerosol response to drought in the contiguous United States during summertime
Cooling radiative forcing effect enhancement of atmospheric amines and mineral particles caused by heterogeneous uptake and oxidation
Source-resolved atmospheric metal emissions, concentrations, and deposition fluxes into the East Asian seas
Analysis of secondary inorganic aerosols over the greater Athens area using the EPISODE–CityChem source dispersion and photochemistry model
Global estimates of ambient reactive nitrogen components during 2000–2100 based on the multi-stage model
The role of naphthalene and its derivatives in the formation of secondary organic aerosol in the Yangtze River Delta region, China
Unveiling the optimal regression model for source apportionment of the oxidative potential of PM10
Investigating the contribution of grown new particles to cloud condensation nuclei with largely varying preexisting particles – Part 2: Modeling chemical drivers and 3-D new particle formation occurrence
Technical note: Influence of different averaging metrics and temporal resolutions on the aerosol pH calculated by thermodynamic modeling
Dual roles of the inorganic aqueous phase on secondary organic aerosol growth from benzene and phenol
Global source apportionment of aerosols into major emission regions and sectors over 1850–2017
Modeling atmospheric brown carbon in the GISS ModelE Earth system model
Observation-constrained kinetic modeling of isoprene SOA formation in the atmosphere
Significant impact of urban tree biogenic emissions on air quality estimated by a bottom-up inventory and chemistry transport modeling
Secondary organic aerosols derived from intermediate-volatility n-alkanes adopt low-viscous phase state
Modeling the drivers of fine PM pollution over Central Europe: impacts and contributions of emissions from different sources
Reaction of SO3 with H2SO4 and its implications for aerosol particle formation in the gas phase and at the air–water interface
Weakened aerosol–radiation interaction exacerbating ozone pollution in eastern China since China's clean air actions
Uncertainties from biomass burning aerosols in air quality models obscure public health impacts in Southeast Asia
Oxidative potential apportionment of atmospheric PM1: a new approach combining high-sensitive online analysers for chemical composition and offline OP measurement technique
Ludovico Di Antonio, Matthias Beekmann, Guillaume Siour, Vincent Michoud, Christopher Cantrell, Astrid Bauville, Antonin Bergé, Mathieu Cazaunau, Servanne Chevaillier, Manuela Cirtog, Joel F. de Brito, Paola Formenti, Cecile Gaimoz, Olivier Garret, Aline Gratien, Valérie Gros, Martial Haeffelin, Lelia N. Hawkins, Simone Kotthaus, Gael Noyalet, Diana L. Pereira, Jean-Eudes Petit, Eva Drew Pronovost, Véronique Riffault, Chenjie Yu, Gilles Foret, Jean-François Doussin, and Claudia Di Biagio
Atmos. Chem. Phys., 25, 4803–4831, https://doi.org/10.5194/acp-25-4803-2025, https://doi.org/10.5194/acp-25-4803-2025, 2025
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The summer of 2022 has been considered a proxy for future climate scenarios due to its hot and dry conditions. In this paper, we use the measurements from the Atmospheric Chemistry of the Suburban Forest (ACROSS) campaign, conducted in the Paris area in June–July 2022, along with observations from existing networks, to evaluate a 3D chemistry transport model (WRF–CHIMERE) simulation. Results are shown to be satisfactory, allowing us to explain the gas and aerosol variability at the campaign sites.
Bin Luo, Yuqiang Zhang, Tao Tang, Hongliang Zhang, Jianlin Hu, Jiangshan Mu, Wenxing Wang, and Likun Xue
Atmos. Chem. Phys., 25, 4767–4783, https://doi.org/10.5194/acp-25-4767-2025, https://doi.org/10.5194/acp-25-4767-2025, 2025
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India is facing a severe air pollution crisis that poses significant health risks, particularly from PM2.5 and O3. Our study reveals rising levels of both pollutants from 1995 to 2014, leading to increased premature mortality. While anthropogenic emissions play a significant role, biomass burning also impacts air quality, in particular seasons and regions in India. This study underscores the urgent need for localized policies to protect public health amid escalating environmental challenges.
Rubén Soussé Villa, Oriol Jorba, María Gonçalves Ageitos, Dene Bowdalo, Marc Guevara, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 25, 4719–4753, https://doi.org/10.5194/acp-25-4719-2025, https://doi.org/10.5194/acp-25-4719-2025, 2025
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Desert dust forms nitrate coatings as it travels through the atmosphere. However, current models that predict this process vary greatly due to different methods and inaccuracies. We examined how nitrate forms in a global model, focusing on how gases condense on dust, the lifespan of different particles, and the impact of alkalinity. Our findings show that models work best when they consider reversible gas condensation with alkalinity. This should lead to better estimates of climate impacts.
Natalie M. Mahowald, Longlei Li, Julius Vira, Marje Prank, Douglas S. Hamilton, Hitoshi Matsui, Ron L. Miller, P. Louis Lu, Ezgi Akyuz, Daphne Meidan, Peter Hess, Heikki Lihavainen, Christine Wiedinmyer, Jenny Hand, Maria Grazia Alaimo, Célia Alves, Andres Alastuey, Paulo Artaxo, Africa Barreto, Francisco Barraza, Silvia Becagli, Giulia Calzolai, Shankararaman Chellam, Ying Chen, Patrick Chuang, David D. Cohen, Cristina Colombi, Evangelia Diapouli, Gaetano Dongarra, Konstantinos Eleftheriadis, Johann Engelbrecht, Corinne Galy-Lacaux, Cassandra Gaston, Dario Gomez, Yenny González Ramos, Roy M. Harrison, Chris Heyes, Barak Herut, Philip Hopke, Christoph Hüglin, Maria Kanakidou, Zsofia Kertesz, Zbigniew Klimont, Katriina Kyllönen, Fabrice Lambert, Xiaohong Liu, Remi Losno, Franco Lucarelli, Willy Maenhaut, Beatrice Marticorena, Randall V. Martin, Nikolaos Mihalopoulos, Yasser Morera-Gómez, Adina Paytan, Joseph Prospero, Sergio Rodríguez, Patricia Smichowski, Daniela Varrica, Brenna Walsh, Crystal L. Weagle, and Xi Zhao
Atmos. Chem. Phys., 25, 4665–4702, https://doi.org/10.5194/acp-25-4665-2025, https://doi.org/10.5194/acp-25-4665-2025, 2025
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Aerosol particles are an important part of the Earth system, but their concentrations are spatially and temporally heterogeneous, as well as being variable in size and composition. Here, we present a new compilation of PM2.5 and PM10 aerosol observations, focusing on the spatial variability across different observational stations, including composition, and demonstrate a method for comparing the data sets to model output.
Zhenyu Zhang, Jing Li, Huizheng Che, Yueming Dong, Oleg Dubovik, Thomas Eck, Pawan Gupta, Brent Holben, Jhoon Kim, Elena Lind, Trailokya Saud, Sachchida Nand Tripathi, and Tong Ying
Atmos. Chem. Phys., 25, 4617–4637, https://doi.org/10.5194/acp-25-4617-2025, https://doi.org/10.5194/acp-25-4617-2025, 2025
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We used ground-based remote sensing data from the Aerosol Robotic Network to examine long-term trends in aerosol characteristics. We found aerosol loadings generally decreased globally, and aerosols became more scattering. These changes are closely related to variations in aerosol compositions, such as decreased anthropogenic emissions over East Asia, Europe, and North America; increased anthropogenic sources over northern India; and increased dust activity over the Arabian Peninsula.
Erin J. Emme and Hannah M. Horowitz
Atmos. Chem. Phys., 25, 4531–4545, https://doi.org/10.5194/acp-25-4531-2025, https://doi.org/10.5194/acp-25-4531-2025, 2025
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There is uncertainty in the sources of Arctic cold-season (November–April) sea salt aerosols. Using a chemical transport model and satellite observations, we quantify Arctic-wide sea salt aerosol emissions from fractures in sea ice, called open sea ice leads, and their atmospheric chemistry impacts for the cold season. We show that sea ice leads contribute to Arctic sea salt aerosols and bromine, especially in under-observed regions.
Ursula A. Jongebloed, Jacob I. Chalif, Linia Tashmim, William C. Porter, Kelvin H. Bates, Qianjie Chen, Erich C. Osterberg, Bess G. Koffman, Jihong Cole-Dai, Dominic A. Winski, David G. Ferris, Karl J. Kreutz, Cameron P. Wake, and Becky Alexander
Atmos. Chem. Phys., 25, 4083–4106, https://doi.org/10.5194/acp-25-4083-2025, https://doi.org/10.5194/acp-25-4083-2025, 2025
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Marine phytoplankton emit dimethyl sulfide (DMS), which forms methanesulfonic acid (MSA) and sulfate. MSA concentrations in ice cores decreased over the industrial era, which has been attributed to pollution-driven changes in DMS chemistry. We use a model to investigate DMS chemistry compared to observations of DMS, MSA, and sulfate. We find that modeled DMS, MSA, and sulfate are influenced by pollution-sensitive oxidant concentrations, characterization of DMS chemistry, and other variables.
Xiaolin Duan, Guangjie Zheng, Chuchu Chen, Qiang Zhang, and Kebin He
Atmos. Chem. Phys., 25, 3919–3928, https://doi.org/10.5194/acp-25-3919-2025, https://doi.org/10.5194/acp-25-3919-2025, 2025
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Aerosol acidity is an important parameter in atmospheric chemistry, while its driving factors, especially chemical profiles versus meteorological conditions, are not yet fully understood. Here, we established a hierarchical quantitative analysis framework to understand the driving factors of aerosol acidity on different timescales. Its application in Changzhou, China, revealed distinct driving factors and corresponding mechanisms of aerosol acidity from annual trends to random residuals.
Wenxin Zhang, Yaman Liu, Man Yue, Xinyi Dong, Kan Huang, and Minghuai Wang
Atmos. Chem. Phys., 25, 3857–3872, https://doi.org/10.5194/acp-25-3857-2025, https://doi.org/10.5194/acp-25-3857-2025, 2025
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Understanding long-term organic aerosol (OA) trends and their driving factors is important for air quality management. Our modeling revealed that OA in China increased by 5.6 % from 1990 to 2019, primarily due to a 32.3 % increase in secondary organic aerosols (SOAs) and an 8.1 % decrease in primary organic aerosols (POAs), both largely driven by changes in anthropogenic emissions. Biogenic SOA increased due to warming but showed little response to changes in anthropogenic nitrogen oxide emissions.
Soo-Jin Park, Lya Lugon, Oscar Jacquot, Youngseob Kim, Alexia Baudic, Barbara D'Anna, Ludovico Di Antonio, Claudia Di Biagio, Fabrice Dugay, Olivier Favez, Véronique Ghersi, Aline Gratien, Julien Kammer, Jean-Eudes Petit, Olivier Sanchez, Myrto Valari, Jérémy Vigneron, and Karine Sartelet
Atmos. Chem. Phys., 25, 3363–3387, https://doi.org/10.5194/acp-25-3363-2025, https://doi.org/10.5194/acp-25-3363-2025, 2025
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To accurately represent the population exposure to outdoor concentrations of pollutants of interest to health (NO2, PM2.5, black carbon, and ultrafine particles), multi-scale modelling down to the street scale is set up and evaluated using measurements from field campaigns. An exposure scaling factor is defined, allowing regional-scale simulations to be corrected to evaluate population exposure. Urban heterogeneities strongly influence NO2, black carbon, and ultrafine particles but less strongly PM2.5.
Sara L. Farrell, Havala O. T. Pye, Robert Gilliam, George Pouliot, Deanna Huff, Golam Sarwar, William Vizuete, Nicole Briggs, Fengkui Duan, Tao Ma, Shuping Zhang, and Kathleen Fahey
Atmos. Chem. Phys., 25, 3287–3312, https://doi.org/10.5194/acp-25-3287-2025, https://doi.org/10.5194/acp-25-3287-2025, 2025
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In this work we implement heterogeneous sulfur chemistry into the Community Multiscale Air Quality (CMAQ) model. This new chemistry accounts for the formation of sulfate via aqueous oxidation of SO2 in aerosol liquid water and the formation of hydroxymethanesulfonate (HMS) – often confused by measurement techniques as sulfate. Model performance in predicting sulfur PM2.5 in Fairbanks, Alaska, and other places that experience dark and cold winters is improved.
Paul A. Makar, Philip Cheung, Christian Hogrefe, Ayodeji Akingunola, Ummugulsum Alyuz, Jesse O. Bash, Michael D. Bell, Roberto Bellasio, Roberto Bianconi, Tim Butler, Hazel Cathcart, Olivia E. Clifton, Alma Hodzic, Ioannis Kioutsioukis, Richard Kranenburg, Aurelia Lupascu, Jason A. Lynch, Kester Momoh, Juan L. Perez-Camanyo, Jonathan Pleim, Young-Hee Ryu, Roberto San Jose, Donna Schwede, Thomas Scheuschner, Mark W. Shephard, Ranjeet S. Sokhi, and Stefano Galmarini
Atmos. Chem. Phys., 25, 3049–3107, https://doi.org/10.5194/acp-25-3049-2025, https://doi.org/10.5194/acp-25-3049-2025, 2025
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The large range of sulfur and nitrogen deposition estimates from air quality models results in a large range of predicted impacts. We used models and deposition diagnostics to identify the processes controlling atmospheric sulfur and nitrogen deposition variability. Controlling factors included the uptake of gases and aerosols by hydrometeors, aerosol inorganic chemistry, particle dry deposition, ammonia bidirectional fluxes, gas deposition via plant cuticles and soil, and land use data.
Lang Liu, Xin Long, Yi Li, Zengliang Zang, Fengwen Wang, Yan Han, Zhier Bao, Yang Chen, Tian Feng, and Jinxin Yang
Atmos. Chem. Phys., 25, 1569–1585, https://doi.org/10.5194/acp-25-1569-2025, https://doi.org/10.5194/acp-25-1569-2025, 2025
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This study uses WRF-Chem to assess how meteorological conditions and emission reductions affected fine particulate matter (PM2.5) in the North China Plain (NCP). It highlights regional disparities: in the northern NCP, adverse weather negated emission reduction effects. In contrast, the southern NCP featured a PM2.5 decrease due to favorable weather and emission reductions. The research highlighted the interaction between emissions, meteorology, and PM2.5.
Alexandros Milousis, Klaus Klingmüller, Alexandra P. Tsimpidi, Jasper F. Kok, Maria Kanakidou, Athanasios Nenes, and Vlassis A. Karydis
Atmos. Chem. Phys., 25, 1333–1351, https://doi.org/10.5194/acp-25-1333-2025, https://doi.org/10.5194/acp-25-1333-2025, 2025
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This study investigates the impact of dust on the global radiative effect of nitrate aerosols. The results indicate both positive and negative regional shortwave and longwave radiative effects due to aerosol–radiation interactions and cloud adjustments. The global average net REari and REaci of nitrate aerosols are −0.11 and +0.17 W m−2, respectively, mainly affecting the shortwave spectrum. Sensitivity simulations evaluated the influence of mineral dust composition and emissions on the results.
Judith Kleinheins, Nadia Shardt, Ulrike Lohmann, and Claudia Marcolli
Atmos. Chem. Phys., 25, 881–903, https://doi.org/10.5194/acp-25-881-2025, https://doi.org/10.5194/acp-25-881-2025, 2025
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We model the cloud condensation nuclei (CCN) activation of sea spray aerosol particles with classical Köhler theory and with a new model approach that takes surface tension lowering into account. We categorize organic compounds into weak, intermediate, and strong surfactants, and we outline for which composition surface tension lowering is important. The results suggest that surface tension lowering allows sea spray aerosol particles in the Aitken mode to be a source of CCN in marine updraughts.
Olivia G. Norman, Colette L. Heald, Solomon Bililign, Pedro Campuzano-Jost, Hugh Coe, Marc N. Fiddler, Jaime R. Green, Jose L. Jimenez, Katharina Kaiser, Jin Liao, Ann M. Middlebrook, Benjamin A. Nault, John B. Nowak, Johannes Schneider, and André Welti
Atmos. Chem. Phys., 25, 771–795, https://doi.org/10.5194/acp-25-771-2025, https://doi.org/10.5194/acp-25-771-2025, 2025
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This study finds that one component of secondary inorganic aerosols, nitrate, is greatly overestimated by a global atmospheric chemistry model compared to observations from 11 flight campaigns. None of the loss and production pathways explored can explain the nitrate bias alone. The model’s inability to capture the variability in the observations remains and requires future investigation to avoid biases in policy-related studies (i.e., air quality, health, climate impacts of these aerosols).
Ryan Vella, Matthew Forrest, Andrea Pozzer, Alexandra P. Tsimpidi, Thomas Hickler, Jos Lelieveld, and Holger Tost
Atmos. Chem. Phys., 25, 243–262, https://doi.org/10.5194/acp-25-243-2025, https://doi.org/10.5194/acp-25-243-2025, 2025
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This study examines how land cover changes influence biogenic volatile organic compound (BVOC) emissions and atmospheric states. Using a coupled chemistry–climate–vegetation model, we compare present-day land cover (deforested for crops and grazing) with natural vegetation and an extreme reforestation scenario. We find that vegetation changes significantly impact global BVOC emissions and organic aerosols but have a relatively small effect on total aerosols, clouds, and radiative effects.
Mashiat Hossain, Rebecca M. Garland, and Hannah M. Horowitz
Atmos. Chem. Phys., 24, 14123–14143, https://doi.org/10.5194/acp-24-14123-2024, https://doi.org/10.5194/acp-24-14123-2024, 2024
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Our research examines aerosol dynamics over the southeast Atlantic, a region with significant uncertainties in aerosol radiative forcings. Using the GEOS-Chem model, we find that at cloud altitudes, organic aerosols dominate during the biomass burning season, while sulfate aerosols, driven by marine emissions, prevail during peak primary production. These findings highlight the need for accurate representation of marine aerosols in models to improve climate predictions and reduce uncertainties.
Ashok K. Luhar, Anthony C. Jones, and Jonathan M. Wilkinson
Atmos. Chem. Phys., 24, 14005–14028, https://doi.org/10.5194/acp-24-14005-2024, https://doi.org/10.5194/acp-24-14005-2024, 2024
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Nitrate aerosol is often omitted in global chemistry–climate models, partly due to the chemical complexity of its formation process. Using a global model, we show that including nitrate aerosol significantly impacts tropospheric composition fields, such as ozone, and radiation. Additionally, lightning-generated oxides of nitrogen influence both nitrate aerosol mass concentrations and aerosol size distribution, which has important implications for radiative fluxes and indirect aerosol effects.
Jiamao Zhou, Jiarui Wu, Xiaoli Su, Ruonan Wang, Xia Li, Qian Jiang, Ting Zhang, Wenting Dai, Junji Cao, Xuexi Tie, and Guohui Li
EGUsphere, https://doi.org/10.5194/egusphere-2024-3468, https://doi.org/10.5194/egusphere-2024-3468, 2024
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Brown carbon (BrC) is a type of airborne particle produced from various combustion sources which is light absorption. Historically, climate models have categorizing organic particles as either non-absorbing or purely reflective. Our study shows that BrC can reduce the usual cooling effect of organic particles. While BrC is often linked to biomass burning, however, BrC from fossil fuels contributes significantly to atmospheric heating.
Yanru Huo, Mingxue Li, Xueyu Wang, Jianfei Sun, Yuxin Zhou, Yuhui Ma, and Maoxia He
Atmos. Chem. Phys., 24, 12409–12423, https://doi.org/10.5194/acp-24-12409-2024, https://doi.org/10.5194/acp-24-12409-2024, 2024
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This work found that the air–water (A–W) interface and TiO2 clusters promote the oxidation of phenolic compounds (PhCs) to varying degrees compared with the gas phase and bulk water. Some byproducts are more harmful than their parent compounds. This work provides important evidence for the rapid oxidation observed in O3/HO• + PhC experiments at the A–W interface and in mineral dust.
Sijia Lou, Manish Shrivastava, Alexandre Albinet, Sophie Tomaz, Deepchandra Srivastava, Olivier Favez, Huizhong Shen, and Aijun Ding
EGUsphere, https://doi.org/10.5194/egusphere-2024-3269, https://doi.org/10.5194/egusphere-2024-3269, 2024
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PAHs, emitted from incomplete combustion, pose serious health risks due to their carcinogenic properties. This research demonstrates that viscous organic aerosol coatings significantly hinder PAH oxidation, with spatial distributions sensitive to the degradation modelling approach. Our findings underscore the importance of accurately modelling these processes for risk assessments, highlighting the need to consider both fresh and oxidized PAHs in evaluating human exposure and health risks.
Rémy Lapere, Louis Marelle, Pierre Rampal, Laurent Brodeau, Christian Melsheimer, Gunnar Spreen, and Jennie L. Thomas
Atmos. Chem. Phys., 24, 12107–12132, https://doi.org/10.5194/acp-24-12107-2024, https://doi.org/10.5194/acp-24-12107-2024, 2024
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Elongated open-water areas in sea ice, called leads, can release marine aerosols into the atmosphere. In the Arctic, this source of atmospheric particles could play an important role for climate. However, the amount, seasonality and spatial distribution of such emissions are all mostly unknown. Here, we propose a first parameterization for sea spray aerosols emitted through leads in sea ice and quantify their impact on aerosol populations in the high Arctic.
Hanzheng Zhu, Yaman Liu, Man Yue, Shihui Feng, Pingqing Fu, Kan Huang, Xinyi Dong, and Minghuai Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-2293, https://doi.org/10.5194/egusphere-2024-2293, 2024
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Dust soluble iron deposition from East Asia plays an important role in the marine ecology of the Northwest Pacific. Using the developed model, our findings highlight a dual trend: a decrease in the overall deposition of soluble iron from dust, but an increase in the solubility of the iron itself due to the enhanced atmospheric processing. It underscores the critical roles of both dust emission and atmospheric processing in soluble iron deposition and marine ecology.
Camilo Serrano Damha, Kyle Gorkowski, and Andreas Zuend
EGUsphere, https://doi.org/10.5194/egusphere-2024-2712, https://doi.org/10.5194/egusphere-2024-2712, 2024
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Organic aerosol water content impacts the gas–particle partitioning of semivolatile organics. We used an aerosol thermodynamic model in the GEOS-Chem chemical transport model to efficiently account for organic aerosol water uptake and nonideal mixing. This led to a substantial enhancement in mean organic aerosol mass concentration with respect to GEOS-Chem's most advanced scheme. The water-sensitive scheme could be a valuable tool for reconciling model estimations and field measurements.
Haihui Zhu, Randall V. Martin, Aaron van Donkelaar, Melanie S. Hammer, Chi Li, Jun Meng, Christopher R. Oxford, Xuan Liu, Yanshun Li, Dandan Zhang, Inderjeet Singh, and Alexei Lyapustin
Atmos. Chem. Phys., 24, 11565–11584, https://doi.org/10.5194/acp-24-11565-2024, https://doi.org/10.5194/acp-24-11565-2024, 2024
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Ambient fine particulate matter (PM2.5) contributes to 4 million deaths globally each year. Satellite remote sensing of aerosol optical depth (AOD), coupled with a simulated PM2.5–AOD relationship (η), can provide global PM2.5 estimations. This study aims to understand the spatial patterns and driving factors of η to guide future measurement and modeling efforts. We quantified η globally and regionally and found that its spatial variation is strongly influenced by aerosol composition.
Connor J. Clayton, Daniel R. Marsh, Steven T. Turnock, Ailish M. Graham, Kirsty J. Pringle, Carly L. Reddington, Rajesh Kumar, and James B. McQuaid
Atmos. Chem. Phys., 24, 10717–10740, https://doi.org/10.5194/acp-24-10717-2024, https://doi.org/10.5194/acp-24-10717-2024, 2024
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We demonstrate that strong climate mitigation could improve air quality in Europe; however, less ambitious mitigation does not result in these co-benefits. We use a high-resolution atmospheric chemistry model. This allows us to demonstrate how this varies across European countries and analyse the underlying chemistry. This may help policy-facing researchers understand which sectors and regions need to be prioritised to achieve strong air quality co-benefits of climate mitigation.
Ping-Chieh Huang, Hui-Ming Hung, Hsin-Chih Lai, and Charles C.-K. Chou
Atmos. Chem. Phys., 24, 10759–10772, https://doi.org/10.5194/acp-24-10759-2024, https://doi.org/10.5194/acp-24-10759-2024, 2024
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Models were used to study ways to reduce particulate matter (PM) pollution in Taiwan during winter. After considering various factors, such as physical processes and chemical reactions, we found that reducing NOx or NH3 emissions is more effective at mitigating PM2.5 than reducing SO2 emissions. When considering both efficiency and cost, reducing NH3 emissions seems to be a more suitable policy for the studied environment in Taiwan.
Matthieu Vida, Gilles Foret, Guillaume Siour, Florian Couvidat, Olivier Favez, Gaelle Uzu, Arineh Cholakian, Sébastien Conil, Matthias Beekmann, and Jean-Luc Jaffrezo
Atmos. Chem. Phys., 24, 10601–10615, https://doi.org/10.5194/acp-24-10601-2024, https://doi.org/10.5194/acp-24-10601-2024, 2024
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We simulate 2 years of atmospheric fungal spores over France and use observations of polyols and primary biogenic factors from positive matrix factorisation. The representation of emissions taking into account a proxy for vegetation surface and specific humidity enables us to reproduce very accurately the seasonal cycle of fungal spores. Furthermore, we estimate that fungal spores can account for 20 % of PM10 and 40 % of the organic fraction of PM10 over vegetated areas in summer.
Jiewen Shen, Bin Zhao, Shuxiao Wang, An Ning, Yuyang Li, Runlong Cai, Da Gao, Biwu Chu, Yang Gao, Manish Shrivastava, Jingkun Jiang, Xiuhui Zhang, and Hong He
Atmos. Chem. Phys., 24, 10261–10278, https://doi.org/10.5194/acp-24-10261-2024, https://doi.org/10.5194/acp-24-10261-2024, 2024
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We extensively compare various cluster-dynamics-based parameterizations for sulfuric acid–dimethylamine nucleation and identify a newly developed parameterization derived from Atmospheric Cluster Dynamic Code (ACDC) simulations as being the most reliable one. This study offers a valuable reference for developing parameterizations of other nucleation systems and is meaningful for the accurate quantification of the environmental and climate impacts of new particle formation.
Wei Li and Yuxuan Wang
Atmos. Chem. Phys., 24, 9339–9353, https://doi.org/10.5194/acp-24-9339-2024, https://doi.org/10.5194/acp-24-9339-2024, 2024
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Droughts immensely increased organic aerosol (OA) in the contiguous United States in summer (1998–2019), notably in the Pacific Northwest (PNW) and Southeast (SEUS). The OA rise in the SEUS is driven by the enhanced formation of epoxydiol-derived secondary organic aerosol due to the increase in biogenic volatile organic compounds and sulfate, while in the PNW, it is caused by wildfires. A total of 10 climate models captured the OA increase in the PNW yet greatly underestimated it in the SEUS.
Weina Zhang, Jianhua Mai, Zhichao Fan, Yongpeng Ji, Yuemeng Ji, Guiying Li, Yanpeng Gao, and Taicheng An
Atmos. Chem. Phys., 24, 9019–9030, https://doi.org/10.5194/acp-24-9019-2024, https://doi.org/10.5194/acp-24-9019-2024, 2024
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This study reveals heterogeneous oxidation causes further radiative forcing effect (RFE) enhancement of amine–mineral mixed particles. Note that RFE increment is higher under clean conditions than that under polluted conditions, which is contributed to high-oxygen-content products. The enhanced RFE of amine–mineral particles caused by heterogenous oxidation is expected to alleviate warming effects.
Shenglan Jiang, Yan Zhang, Guangyuan Yu, Zimin Han, Junri Zhao, Tianle Zhang, and Mei Zheng
Atmos. Chem. Phys., 24, 8363–8381, https://doi.org/10.5194/acp-24-8363-2024, https://doi.org/10.5194/acp-24-8363-2024, 2024
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This study aims to provide gridded data on sea-wide concentrations, deposition fluxes, and soluble deposition fluxes with detailed source categories of metals using the modified CMAQ model. We developed a monthly emission inventory of six metals – Fe, Al, V, Ni, Zn, and Cu – from terrestrial anthropogenic, ship, and dust sources in East Asia in 2017. Our results reveal the contribution of each source to the emissions, concentrations, and deposition fluxes of metals in the East Asian seas.
Stelios Myriokefalitakis, Matthias Karl, Kim A. Weiss, Dimitris Karagiannis, Eleni Athanasopoulou, Anastasia Kakouri, Aikaterini Bougiatioti, Eleni Liakakou, Iasonas Stavroulas, Georgios Papangelis, Georgios Grivas, Despina Paraskevopoulou, Orestis Speyer, Nikolaos Mihalopoulos, and Evangelos Gerasopoulos
Atmos. Chem. Phys., 24, 7815–7835, https://doi.org/10.5194/acp-24-7815-2024, https://doi.org/10.5194/acp-24-7815-2024, 2024
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A state-of-the-art thermodynamic model has been coupled with the city-scale chemistry transport model EPISODE–CityChem to investigate the equilibrium between the inorganic gas and aerosol phases over the greater Athens area, Greece. The simulations indicate that the formation of nitrates in an urban environment is significantly affected by local nitrogen oxide emissions, as well as ambient temperature, relative humidity, photochemical activity, and the presence of non-volatile cations.
Rui Li, Yining Gao, Lijia Zhang, Yubing Shen, Tianzhao Xu, Wenwen Sun, and Gehui Wang
Atmos. Chem. Phys., 24, 7623–7636, https://doi.org/10.5194/acp-24-7623-2024, https://doi.org/10.5194/acp-24-7623-2024, 2024
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A three-stage model was developed to obtain the global maps of reactive nitrogen components during 2000–2100. The results implied that cross-validation R2 values of four species showed satisfactory performance (R2 > 0.55). Most reactive nitrogen components, except NH3, in China showed increases during 2000–2013. In the future scenarios, SSP3-7.0 (traditional-energy scenario) and SSP1-2.6 (carbon neutrality scenario) showed the highest and lowest reactive nitrogen component concentrations.
Fei Ye, Jingyi Li, Yaqin Gao, Hongli Wang, Jingyu An, Cheng Huang, Song Guo, Keding Lu, Kangjia Gong, Haowen Zhang, Momei Qin, and Jianlin Hu
Atmos. Chem. Phys., 24, 7467–7479, https://doi.org/10.5194/acp-24-7467-2024, https://doi.org/10.5194/acp-24-7467-2024, 2024
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Naphthalene (Nap) and methylnaphthalene (MN) are key precursors of secondary organic aerosol (SOA), yet their sources and sinks are often inadequately represented in air quality models. In this study, we incorporated detailed emissions, gas-phase chemistry, and SOA parameterization of Nap and MN into CMAQ to address this issue. The findings revealed remarkably high SOA formation potentials for these compounds despite their low emissions in the Yangtze River Delta region during summer.
Vy Dinh Ngoc Thuy, Jean-Luc Jaffrezo, Ian Hough, Pamela A. Dominutti, Guillaume Salque Moreton, Grégory Gille, Florie Francony, Arabelle Patron-Anquez, Olivier Favez, and Gaëlle Uzu
Atmos. Chem. Phys., 24, 7261–7282, https://doi.org/10.5194/acp-24-7261-2024, https://doi.org/10.5194/acp-24-7261-2024, 2024
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The capacity of particulate matter (PM) to generate reactive oxygen species in vivo is represented by oxidative potential (OP). This study focuses on finding the appropriate model to evaluate the oxidative character of PM sources in six sites using the PM sources and OP. Eight regression techniques are introduced to assess the OP of PM. The study highlights the importance of selecting a model according to the input data characteristics and establishes some recommendations for the procedure.
Ming Chu, Xing Wei, Shangfei Hai, Yang Gao, Huiwang Gao, Yujiao Zhu, Biwu Chu, Nan Ma, Juan Hong, Yele Sun, and Xiaohong Yao
Atmos. Chem. Phys., 24, 6769–6786, https://doi.org/10.5194/acp-24-6769-2024, https://doi.org/10.5194/acp-24-6769-2024, 2024
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We used a 20-bin WRF-Chem model to simulate NPF events in the NCP during a three-week observational period in the summer of 2019. The model was able to reproduce the observations during June 29–July 6, which was characterized by a high frequency of NPF occurrence.
Haoqi Wang, Xiao Tian, Wanting Zhao, Jiacheng Li, Haoyu Yu, Yinchang Feng, and Shaojie Song
Atmos. Chem. Phys., 24, 6583–6592, https://doi.org/10.5194/acp-24-6583-2024, https://doi.org/10.5194/acp-24-6583-2024, 2024
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pH is a key property of ambient aerosols, which affect many atmospheric processes. As aerosol pH is a non-conservative parameter, diverse averaging metrics and temporal resolutions may influence the pH values calculated by thermodynamic models. This technical note seeks to quantitatively evaluate the average pH using varied metrics and resolutions. The ultimate goal is to establish standardized reporting practices in future research endeavors.
Jiwon Choi, Myoseon Jang, and Spencer Blau
Atmos. Chem. Phys., 24, 6567–6582, https://doi.org/10.5194/acp-24-6567-2024, https://doi.org/10.5194/acp-24-6567-2024, 2024
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Persistent phenoxy radical (PPR), formed by phenol gas oxidation and its aqueous reaction, catalytically destroys O3 and retards secondary organic aerosol (SOA) growth. Explicit gas mechanisms including the formation of PPR and low-volatility products from the oxidation of phenol or benzene are applied to the UNIPAR model to predict SOA mass via multiphase reactions of precursors. Aqueous reactions of reactive organics increase SOA mass but retard SOA growth via heterogeneously formed PPR.
Yang Yang, Shaoxuan Mou, Hailong Wang, Pinya Wang, Baojie Li, and Hong Liao
Atmos. Chem. Phys., 24, 6509–6523, https://doi.org/10.5194/acp-24-6509-2024, https://doi.org/10.5194/acp-24-6509-2024, 2024
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The variations in anthropogenic aerosol concentrations and source contributions and their subsequent radiative impact in major emission regions during historical periods are quantified based on an aerosol-tagging system in E3SMv1. Due to the industrial development and implementation of economic policies, sources of anthropogenic aerosols show different variations, which has important implications for pollution prevention and control measures and decision-making for global collaboration.
Maegan A. DeLessio, Kostas Tsigaridis, Susanne E. Bauer, Jacek Chowdhary, and Gregory L. Schuster
Atmos. Chem. Phys., 24, 6275–6304, https://doi.org/10.5194/acp-24-6275-2024, https://doi.org/10.5194/acp-24-6275-2024, 2024
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This study presents the first explicit representation of brown carbon aerosols in the GISS ModelE Earth system model (ESM). Model sensitivity to a range of brown carbon parameters and model performance compared to AERONET and MODIS retrievals of total aerosol properties were assessed. A summary of best practices for incorporating brown carbon into ModelE is also included.
Chuanyang Shen, Xiaoyan Yang, Joel Thornton, John Shilling, Chenyang Bi, Gabriel Isaacman-VanWertz, and Haofei Zhang
Atmos. Chem. Phys., 24, 6153–6175, https://doi.org/10.5194/acp-24-6153-2024, https://doi.org/10.5194/acp-24-6153-2024, 2024
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In this work, a condensed multiphase isoprene oxidation mechanism was developed to simulate isoprene SOA formation from chamber and field studies. Our results show that the measured isoprene SOA mass concentrations can be reasonably reproduced. The simulation results indicate that multifunctional low-volatility products contribute significantly to total isoprene SOA. Our findings emphasize that the pathways to produce these low-volatility species should be considered in models.
Alice Maison, Lya Lugon, Soo-Jin Park, Alexia Baudic, Christopher Cantrell, Florian Couvidat, Barbara D'Anna, Claudia Di Biagio, Aline Gratien, Valérie Gros, Carmen Kalalian, Julien Kammer, Vincent Michoud, Jean-Eudes Petit, Marwa Shahin, Leila Simon, Myrto Valari, Jérémy Vigneron, Andrée Tuzet, and Karine Sartelet
Atmos. Chem. Phys., 24, 6011–6046, https://doi.org/10.5194/acp-24-6011-2024, https://doi.org/10.5194/acp-24-6011-2024, 2024
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This study presents the development of a bottom-up inventory of urban tree biogenic emissions. Emissions are computed for each tree based on their location and characteristics and are integrated in the regional air quality model WRF-CHIMERE. The impact of these biogenic emissions on air quality is quantified for June–July 2022. Over Paris city, urban trees increase the concentrations of particulate organic matter by 4.6 %, of PM2.5 by 0.6 %, and of ozone by 1.0 % on average over 2 months.
Tommaso Galeazzo, Bernard Aumont, Marie Camredon, Richard Valorso, Yong B. Lim, Paul J. Ziemann, and Manabu Shiraiwa
Atmos. Chem. Phys., 24, 5549–5565, https://doi.org/10.5194/acp-24-5549-2024, https://doi.org/10.5194/acp-24-5549-2024, 2024
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Secondary organic aerosol (SOA) derived from n-alkanes is a major component of anthropogenic particulate matter. We provide an analysis of n-alkane SOA by chemistry modeling, machine learning, and laboratory experiments, showing that n-alkane SOA adopts low-viscous semi-solid or liquid states. Our results indicate few kinetic limitations of mass accommodation in SOA formation, supporting the application of equilibrium partitioning for simulating n-alkane SOA in large-scale atmospheric models.
Lukáš Bartík, Peter Huszár, Jan Karlický, Ondřej Vlček, and Kryštof Eben
Atmos. Chem. Phys., 24, 4347–4387, https://doi.org/10.5194/acp-24-4347-2024, https://doi.org/10.5194/acp-24-4347-2024, 2024
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The presented study deals with the attribution of fine particulate matter (PM2.5) concentrations to anthropogenic emissions over Central Europe using regional-scale models. It calculates the present-day contributions of different emissions sectors to concentrations of PM2.5 and its secondary components. Moreover, the study investigates the effect of chemical nonlinearities by using multiple source attribution methods and secondary organic aerosol calculation methods.
Rui Wang, Yang Cheng, Shasha Chen, Rongrong Li, Yue Hu, Xiaokai Guo, Tianlei Zhang, Fengmin Song, and Hao Li
Atmos. Chem. Phys., 24, 4029–4046, https://doi.org/10.5194/acp-24-4029-2024, https://doi.org/10.5194/acp-24-4029-2024, 2024
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We used quantum chemical calculations, Born–Oppenheimer molecular dynamics simulations, and the ACDC kinetic model to characterize SO3–H2SO4 interaction in the gas phase and at the air–water interface and to study the effect of H2S2O7 on H2SO4–NH3-based clusters. The work expands our understanding of new pathways for the loss of SO3 in acidic polluted areas and helps reveal some missing sources of NPF in metropolitan industrial regions and understand the atmospheric organic–sulfur cycle better.
Hao Yang, Lei Chen, Hong Liao, Jia Zhu, Wenjie Wang, and Xin Li
Atmos. Chem. Phys., 24, 4001–4015, https://doi.org/10.5194/acp-24-4001-2024, https://doi.org/10.5194/acp-24-4001-2024, 2024
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The present study quantifies the response of aerosol–radiation interaction (ARI) to anthropogenic emission reduction from 2013 to 2017, with the main focus on the contribution to changed O3 concentrations over eastern China both in summer and winter using the WRF-Chem model. The weakened ARI due to decreased anthropogenic emission aggravates the summer (winter) O3 pollution by +0.81 ppb (+0.63 ppb), averaged over eastern China.
Margaret R. Marvin, Paul I. Palmer, Fei Yao, Mohd Talib Latif, and Md Firoz Khan
Atmos. Chem. Phys., 24, 3699–3715, https://doi.org/10.5194/acp-24-3699-2024, https://doi.org/10.5194/acp-24-3699-2024, 2024
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We use an atmospheric chemistry model to investigate aerosols emitted from fire activity across Southeast Asia. We find that the limited nature of measurements in this region leads to large uncertainties that significantly hinder the model representation of these aerosols and their impacts on air quality. As a result, the number of monthly attributable deaths is underestimated by as many as 4500, particularly in March at the peak of the mainland burning season.
Julie Camman, Benjamin Chazeau, Nicolas Marchand, Amandine Durand, Grégory Gille, Ludovic Lanzi, Jean-Luc Jaffrezo, Henri Wortham, and Gaëlle Uzu
Atmos. Chem. Phys., 24, 3257–3278, https://doi.org/10.5194/acp-24-3257-2024, https://doi.org/10.5194/acp-24-3257-2024, 2024
Short summary
Short summary
Fine particle (PM1) pollution is a major health issue in the city of Marseille, which is subject to numerous pollution sources. Sampling carried out during the summer enabled a fine characterization of the PM1 sources and their oxidative potential, a promising new metric as a proxy for health impact. PM1 came mainly from combustion sources, secondary ammonium sulfate, and organic nitrate, while the oxidative potential of PM1 came from these sources and from resuspended dust in the atmosphere.
Cited articles
An, Z., Huang, R. J., Zhang, R., Tie, X., Li, G., Cao, J., Zhou, W., Shi,
Z., Han, Y., Gu, Z., and Ji, Y.: Severe haze in northern China: A synergy of
anthropogenic emissions and atmospheric processes, P. Natl. Acad. Sci. USA, 116, 8657–8666, https://doi.org/10.1073/pnas.1900125116, 2019.
Bai, Z., Winiwarter, W., Klimont, Z., Velthof, G., Misselbrook, T., Zhao,
Z., Jin, X., Oenema, O., Hu, C., and Ma, L.: Further Improvement of Air
Quality in China Needs Clear Ammonia Mitigation Target, Environ. Sci.
Technol., 53, 10542–10544, https://doi.org/10.1021/acs.est.9b04725, 2019.
Bond, T. C., Doherty, S. J., Fahey, D. W., Forster, P. M., Berntsen, T.,
DeAngelo, B. J., Flanner, M. G., Ghan, S., Kärcher, B., Koch, D., Kinne,
S., Kondo, Y., Quinn, P. K., Sarofim, M. C., Schultz, M. G., Schulz, M.,
Venkataraman, C., Zhang, H., Zhang, S., Bellouin, N., Guttikunda, S. K.,
Hopke, P. K., Jacobson, M. Z., Kaiser, J. W., Klimont, Z., Lohmann, U.,
Schwarz, J. P., Shindell, D., Storelvmo, T., Warren, S. G., and Zender, C.
S.: Bounding the role of black carbon in the climate system: A scientific
assessment, J. Geophys. Res.-Atmos., 118, 5380–5552,
https://doi.org/10.1002/jgrd.50171, 2013.
Brauer, M., Freedman, G., Frostad, J., van Donkelaar, A., Martin, R. V,
Dentener, F., Dingenen, R. van, Estep, K., Amini, H., Apte, J. S.,
Balakrishnan, K., Barregard, L., Broday, D., Feigin, V., Ghosh, S., Hopke,
P. K., Knibbs, L. D., Kokubo, Y., Liu, Y., Ma, S., Morawska, L., Sangrador,
J. L. T., Shaddick, G., Anderson, H. R., Vos, T., Forouzanfar, M. H.,
Burnett, R. T., and Cohen, A.: Ambient Air Pollution Exposure Estimation for
the Global Burden of Disease 2013, Environ. Sci. Technol., 50, 79–88,
https://doi.org/10.1021/acs.est.5b03709, 2016.
Breider, T. J., Mickley, L. J., Jacob, D. J., Ge, C., Wang, J., Payer
Sulprizio, M., Croft, B., Ridley, D. A., McConnell, J. R., Sharma, S.,
Husain, L., Dutkiewicz, V. A., Eleftheriadis, K., Skov, H., and Hopke, P. K.:
Multidecadal trends in aerosol radiative forcing over the Arctic:
Contribution of changes in anthropogenic aerosol to Arctic warming since
1980, J. Geophys. Res.-Atmos., 122, 3573–3594, https://doi.org/10.1002/2016JD025321,
2017.
Chen, Y., Xie, S., Luo, B., and Zhai, C.: Characteristics and origins of
carbonaceous aerosol in the Sichuan Basin, China, Atmos. Environ., 94,
215–223, https://doi.org/10.1016/j.atmosenv.2014.05.037, 2014.
Cheng, J., Tong, D., Liu, Y., Yu, S., Yan, L., Zheng, B., Geng, G., He, K., and Zhang, Q.: Comparison of Current and Future PM2.5 Air Quality in China
Under CMIP6 and DPEC Emission Scenarios, Geophys. Res. Lett., 48, 1–11,
https://doi.org/10.1029/2021GL093197, 2021a.
Cheng, J., Tong, D., Zhang, Q., Liu, Y., Lei, Y., Yan, G., Yan, L., Yu, S.,
Cui, R. Y., Clarke, L., Geng, G., Zheng, B., Zhang, X., Davis, S. J., and He,
K.: Pathways of China's PM2.5 air quality 2015–2060 in the context of
carbon neutrality, Natl. Sci. Rev., 0, nwab078,
https://doi.org/10.1093/nsr/nwab078, 2021b.
Choi, J., Park, R. J., Lee, H.-M., Lee, S., Jo, D. S., Jeong, J. I., Henze,
D. K., Woo, J.-H., Ban, S.-J., Lee, M.-D., Lim, C.-S., Park, M.-K., Shin, H.
J., Cho, S., Peterson, D., and Song, C.-K.: Impacts of local vs.
trans-boundary emissions from different sectors on PM2.5 exposure in South
Korea during the KORUS-AQ campaign, Atmos. Environ., 203, 196–205,
https://doi.org/10.1016/j.atmosenv.2019.02.008, 2019.
Cohen, A. J., Brauer, M., Burnett, R., Anderson, H. R., Frostad, J., Estep,
K., Balakrishnan, K., Brunekreef, B., Dandona, L., Dandona, R., Feigin, V.,
Freedman, G., Hubbell, B., Jobling, A., Kan, H., Knibbs, L., Liu, Y.,
Martin, R., Morawska, L., Pope, C. A., Shin, H., Straif, K., Shaddick, G.,
Thomas, M., van Dingenen, R., van Donkelaar, A., Vos, T., Murray, C. J. L., and Forouzanfar, M. H.: Estimates and 25-year trends of the global burden of
disease attributable to ambient air pollution: an analysis of data from the
Global Burden of Diseases Study 2015, Lancet, 389, 1907–1918,
https://doi.org/10.1016/S0140-6736(17)30505-6, 2017.
Ding, A., Huang, X., Nie, W., Chi, X., Xu, Z., Zheng, L., Xu, Z., Xie, Y.,
Qi, X., Shen, Y., Sun, P., Wang, J., Wang, L., Sun, J., Yang, X. Q., Qin,
W., Zhang, X., Cheng, W., Liu, W., Pan, L., and Fu, C.: Significant reduction
of PM2.5 in eastern China due to regional-scale emission control: Evidence
from SORPES in 2011–2018, Atmos. Chem. Phys., 19, 11791–11801,
https://doi.org/10.5194/acp-19-11791-2019, 2019.
Duncan Fairlie, T., Jacob, D. J., and Park, R. J.: The impact of transpacific
transport of mineral dust in the United States, Atmos. Environ., 41,
1251–1266, https://doi.org/10.1016/j.atmosenv.2006.09.048, 2007.
Fisher, J. A., Jacob, D. J., Wang, Q., Bahreini, R., Carouge, C. C.,
Cubison, M. J., Dibb, J. E., Diehl, T., Jimenez, J. L., Leibensperger, E.
M., Lu, Z., Meinders, M. B. J., Pye, H. O. T., Quinn, P. K., Sharma, S.,
Streets, D. G., van Donkelaar, A., and Yantosca, R. M.: Sources,
distribution, and acidity of sulfate-ammonium aerosol in the Arctic in
winter-spring, Atmos. Environ., 45, 7301–7318,
https://doi.org/10.1016/j.atmosenv.2011.08.030, 2011.
Fountoukis, C. and Nenes, A.: ISORROPIA II: a computationally efficient thermodynamic equilibrium model for K+–Ca2+–Mg2+–NH
Gao, M., Han, Z., Liu, Z., Li, M., Xin, J., Tao, Z., Li, J., Kang, J.-E.,
Huang, K., Dong, X., Zhuang, B., Li, S., Ge, B., Wu, Q., Cheng, Y., Wang,
Y., Lee, H.-J., Kim, C.-H., Fu, J. S., Wang, T., Chin, M., Woo, J.-H.,
Zhang, Q., Wang, Z., and Carmichael, G. R.: Air quality and climate change,
Topic 3 of the Model Inter-Comparison Study for Asia Phase III (MICS-Asia
III) – Part 1: Overview and model evaluation, Atmos. Chem. Phys., 18,
4859–4884, https://doi.org/10.5194/acp-18-4859-2018, 2018.
Geng, G., Zheng, Y., Zhang, Q., Xue, T., Zhao, H., Tong, D., Zheng, B., Li,
M., Liu, F., Hong, C., He, K., and Davis, S. J.: Drivers of PM2.5 air
pollution deaths in China 2002–2017, Nat. Geosci., 14, 645–650,
https://doi.org/10.1038/s41561-021-00792-3, 2021.
Gu, B., Zhang, L., Van Dingenen, R., Vieno, M., Van Grinsven, H. J. M.,
Zhang, X., Zhang, S., Chen, Y., Wang, S., Ren, C., Rao, S., Holland, M.,
Winiwarter, W., Chen, D., Xu, J., and Sutton, M. A.: Abating ammonia is more
cost-effective than nitrogen oxides for mitigating PM2.5 air pollution,
Science, 374, 758–762, https://doi.org/10.1126/science.abf8623, 2021.
Heald, C. L., J. L. Collett Jr., Lee, T., Benedict, K. B., Schwandner, F.
M., Li, Y., Clarisse, L., Hurtmans, D. R., Van Damme, M., Clerbaux, C.,
Coheur, P.-F., Philip, S., Martin, R. V., and Pye, H. O. T.: Atmospheric
ammonia and particulate inorganic nitrogen over the United States, Atmos.
Chem. Phys., 12, 10295–10312, https://doi.org/10.5194/acp-12-10295-2012, 2012.
Huang, X., Ding, A., Gao, J., Zheng, B., Zhou, D., Qi, X., Tang, R., Wang,
J., Ren, C., Nie, W., Chi, X., Xu, Z., Chen, L., Li, Y., Che, F., Pang, N.,
Wang, H., Tong, D., Qin, W., Cheng, W., Liu, W., Fu, Q., Liu, B., Chai, F.,
Davis, S. J., Zhang, Q., and He, K.: Enhanced secondary pollution offset
reduction of primary emissions during COVID-19 lockdown in China, Natl. Sci.
Rev., 8, nwaa137, https://doi.org/10.1093/nsr/nwaa137, 2021.
IEA: World Energy Outlook, International Energy Agency, IEA/OECD, France, https://www.iea.org/reports/world-energy-outlook-2021 (last access: 4 Apr 2023), 2021.
Jaeglé, L., Quinn, P. K., Bates, T. S., Alexander, B., and Lin, J.-T.:
Global distribution of sea salt aerosols: new constraints from in situ and
remote sensing observations, Atmos. Chem. Phys., 11, 3137–3157,
https://doi.org/10.5194/acp-11-3137-2011, 2011.
Jaeglé, L., Shah, V., Thornton, J. A., Lopez-Hilfiker, F. D., Lee, B.
H., McDuffie, E. E., Fibiger, D., Brown, S. S., Veres, P., Sparks, T. L.,
Ebben, C. J., Wooldridge, P. J., Kenagy, H. S., Cohen, R. C., Weinheimer, A.
J., Campos, T. L., Montzka, D. D., Digangi, J. P., Wolfe, G. M., Hanisco,
T., Schroder, J. C., Campuzano-Jost, P., Day, D. A., Jimenez, J. L.,
Sullivan, A. P., Guo, H., and Weber, R. J.: Nitrogen Oxides Emissions,
Chemistry, Deposition, and Export Over the Northeast United States During
the WINTER Aircraft Campaign, J. Geophys. Res.-Atmos., 123,
12368–12393, https://doi.org/10.1029/2018JD029133, 2018.
Jiang, H., Liao, H., Pye, H. O. T., Wu, S., Mickley, L. J., Seinfeld, J. H., and Zhang, X. Y.: Projected effect of 2000–2050 changes in climate and
emissions on aerosol levels in China and associated transboundary transport,
Atmos. Chem. Phys., 13, 7937–7960, https://doi.org/10.5194/acp-13-7937-2013, 2013.
Jin, X. and Holloway, T.: Spatial and temporal variability of ozone
sensitivity over China observed from the Ozone Monitoring Instrument, J.
Geophys. Res.-Atmos., 120, 7229–7246,
https://doi.org/10.1002/2015JD023250, 2015.
Koplitz, S. N., Jacob, D. J., Sulprizio, M. P., Myllyvirta, L., and Reid, C.:
Burden of Disease from Rising Coal-Fired Power Plant Emissions in Southeast
Asia, Environ. Sci. Technol., 51, 1467–1476,
https://doi.org/10.1021/acs.est.6b03731, 2017.
Kurokawa, J. and Ohara, T.: Long-term historical trends in air pollutant
emissions in Asia: Regional Emission inventory in ASia (REAS) version 3,
Atmos. Chem. Phys., 20, 12761–12793, https://doi.org/10.5194/acp-20-12761-2020,
2020.
Le, T., Wang, Y., Liu, L., Yang, J., Yung, Y. L., Li, G., and Seinfeld, J.
H.: Unexpected air pollution with marked emission reductions during the
COVID-19 outbreak in China, Science, 369, 702–706,
https://doi.org/10.1126/science.abb7431, 2020.
Leibensperger, E. M., Mickley, L. J., Jacob, D. J., and Barrett, S. R. H.:
Intercontinental influence of NOx and CO emissions on particulate matter air
quality, Atmos. Environ., 45, 3318–3324,
https://doi.org/10.1016/j.atmosenv.2011.02.023, 2011.
Li, H., Cheng, J., Zhang, Q., Zheng, B., Zhang, Y., Zheng, G., and He, K.:
Rapid transition in winter aerosol composition in Beijing from 2014 to 2017:
response to clean air actions, Atmos. Chem. Phys., 19, 11485–11499,
https://doi.org/10.5194/acp-19-11485-2019, 2019.
Li, P., Yan, R., Yu, S., Wang, S., Liu, W., and Bao, H.: Reinstate regional
transport of PM2.5 as a major cause of severe haze in Beijing, P. Natl.
Acad. Sci. USA, 112, E2739–E2740, https://doi.org/10.1073/pnas.1502596112, 2015.
Li, Q., Zhang, L., Wang, T., Wang, Z., Fu, X., and Zhang, Q.: “New”
Reactive Nitrogen Chemistry Reshapes the Relationship of Ozone to Its
Precursors, Environ. Sci. Technol., 52, 2810–2818,
https://doi.org/10.1021/acs.est.7b05771, 2018.
Liao, T., Wang, S., Ai, J., Gui, K., Duan, B., Zhao, Q., Zhang, X., Jiang,
W., and Sun, Y.: Heavy pollution episodes, transport pathways and potential
sources of PM2.5 during the winter of 2013 in Chengdu (China), Sci. Total
Environ., 584/585, 1056–1065,
https://doi.org/10.1016/j.scitotenv.2017.01.160, 2017.
Lin, J.-T. and McElroy, M. B.: Impacts of boundary layer mixing on pollutant
vertical profiles in the lower troposphere: Implications to satellite remote
sensing, Atmos. Environ., 44, 1726–1739,
https://doi.org/10.1016/j.atmosenv.2010.02.009, 2010.
Liu, H., Jacob, D. J., Bey, I., and Yantosca, R. M.: Constraints from 210 Pb
and 7 Be on wet deposition and transport in a global three-dimensional
chemical tracer model driven by assimilated meteorological fields, J.
Geophys. Res.-Atmos., 106, 12109–12128, https://doi.org/10.1029/2000JD900839,
2001.
Liu, M., Huang, X., Song, Y., Xu, T., Wang, S., Wu, Z., Hu, M., Zhang, L.,
Zhang, Q., Pan, Y., Liu, X., and Zhu, T.: Rapid SO2 emission reductions
significantly increase tropospheric ammonia concentrations over the North
China Plain, Atmos. Chem. Phys., 18, 17933–17943,
https://doi.org/10.5194/acp-18-17933-2018, 2018.
Liu, M., Huang, X., Song, Y., Tang, J., Cao, J., Zhang, X., Zhang, Q., Wang,
S., Xu, T., Kang, L., Cai, X., Zhang, H., Yang, F., Wang, H., Yu, J. Z.,
Lau, A. K. H., He, L., Huang, X., Duan, L., Ding, A., Xue, L., Gao, J., Liu,
B., and Zhu, T.: Ammonia emission control in China would mitigate haze
pollution and nitrogen deposition, but worsen acid rain, P. Natl. Acad.
Sci. USA, 116, 7760–7765, https://doi.org/10.1073/pnas.1814880116, 2019.
Luo, G., Yu, F., and Moch, J. M.: Further improvement of wet process
treatments in GEOS-Chem v12.6.0: Impact on global distributions of aerosols
and aerosol precursors, Geosci. Model Dev., 13, 2879–2903,
https://doi.org/10.5194/gmd-13-2879-2020, 2020.
McDuffie, E. E., Smith, S. J., O'Rourke, P., Tibrewal, K., Venkataraman, C.,
Marais, E. A., Zheng, B., Crippa, M., Brauer, M., and Martin, R. V.: A global
anthropogenic emission inventory of atmospheric pollutants from sector- And
fuel-specific sources (1970–2017): An application of the Community Emissions
Data System (CEDS), Earth Syst. Sci. Data, 12, 3413–3442,
https://doi.org/10.5194/essd-12-3413-2020, 2020.
Meng, W., Zhong, Q., Chen, Y., Shen, H., Yun, X., Smith, K. R., Li, B., Liu,
J., Wang, X., Ma, J., Cheng, H., Zeng, E. Y., Guan, D., Russell, A. G., and Tao, S.: Energy and air pollution benefits of household fuel policies in
northern China, P. Natl. Acad. Sci. USA, 116, 16773–16780,
https://doi.org/10.1073/pnas.1904182116, 2019.
Miao, R., Chen, Q., Zheng, Y., Cheng, X., Sun, Y., Palmer, P. I.,
Shrivastava, M., Guo, J., Zhang, Q., Liu, Y., Tan, Z., Ma, X., Chen, S.,
Zeng, L., Lu, K., and Zhang, Y.: Model bias in simulating major chemical
components of PM2.5 in China, Atmos. Chem. Phys., 20, 12265–12284,
https://doi.org/10.5194/acp-20-12265-2020, 2020.
Murray, L. T., Jacob, D. J., Logan, J. A., Hudman, R. C., and Koshak, W. J.:
Optimized regional and interannual variability of lightning in a global
chemical transport model constrained by LIS/OTD satellite data, J. Geophys.
Res.-Atmos., 117, D20307, https://doi.org/10.1029/2012JD017934, 2012.
Park, M. E., Song, C. H., Park, R. S., Lee, J., Kim, J., Lee, S., Woo,
J.-H., Carmichael, G. R., Eck, T. F., Holben, B. N., Lee, S.-S., Song, C. K., and Hong, Y. D.: New approach to monitor transboundary particulate pollution
over Northeast Asia, Atmos. Chem. Phys., 14, 659–674,
https://doi.org/10.5194/acp-14-659-2014, 2014.
Park, R. J., Jacob, D. J., Field, B. D., Yantosca, R. M., and Chin, M.:
Natural and transboundary pollution influences on sulfate-nitrate-ammonium
aerosols in the United States: Implications for policy, J. Geophys. Res.,
109, D15204, https://doi.org/10.1029/2003JD004473, 2004.
Peng, W., Wagner, F., Ramana, M. V., Zhai, H., Small, M. J., Dalin, C.,
Zhang, X., and Mauzerall, D. L.: Managing China's coal power plants to
address multiple environmental objectives, Nat. Sustain., 1, 693–701,
https://doi.org/10.1038/s41893-018-0174-1, 2018.
Pennington, E. A., Seltzer, K. M., Murphy, B. N., Qin, M., Seinfeld, J. H., and Pye, H. O. T.: Modeling secondary organic aerosol formation from
volatile chemical products, Atmos. Chem. Phys., 21, 18247–18261,
https://doi.org/10.5194/acp-21-18247-2021, 2021.
Philip, S., Martin, R. V., Pierce, J. R., Jimenez, J. L., Zhang, Q.,
Canagaratna, M. R., Spracklen, D. V., Nowlan, C. R., Lamsal, L. N., Cooper,
M. J., and Krotkov, N. A.: Spatially and seasonally resolved estimate of the
ratio of organic mass to organic carbon, Atmos. Environ., 87, 34–40,
https://doi.org/10.1016/j.atmosenv.2013.11.065, 2014.
Philip, S., Martin, R. V, Snider, G., Weagle, C. L., van Donkelaar, A.,
Brauer, M., Henze, D. K., Klimont, Z., Venkataraman, C., Guttikunda, S. K., and Zhang, Q.: Anthropogenic fugitive, combustion and industrial dust is a
significant, underrepresented fine particulate matter source in global
atmospheric models, Environ. Res. Lett., 12, 044018,
https://doi.org/10.1088/1748-9326/aa65a4, 2017.
Pye, H. O. T., Liao, H., Wu, S., Mickley, L. J., Jacob, D. J., Henze, D. K., and Seinfeld, J. H.: Effect of changes in climate and emissions on future
sulfate-nitrate-ammonium aerosol levels in the United States, J. Geophys.
Res.-Atmos., 114, D01205, https://doi.org/10.1029/2008JD010701, 2009.
Randerson, J. T., Van Der Werf, G. R., Giglio, L., Collatz, G. J., and Kasibhatla, P. S.: Global Fire Emissions Database, Version 4, (GFEDv4), ORNL Distributed Active Archive Center [data set],
https://doi.org/10.3334/ornldaac/1293, 2015.
Ren, C., Huang, X., Wang, Z., Sun, P., Chi, X., Ma, Y., Zhou, D., Huang, J.,
Xie, Y., Gao, J., and Ding, A.: Nonlinear response of nitrate to NOx
reduction in China during the COVID-19 pandemic, Atmos. Environ., 264,
118715, https://doi.org/10.1016/j.atmosenv.2021.118715, 2021.
Shrivastava, M., Cappa, C. D., Fan, J., Goldstein, A. H., Guenther, A. B.,
Jimenez, J. L., Kuang, C., Laskin, A., Martin, S. T., Ng, N. L., Petaja, T.,
Pierce, J. R., Rasch, P. J., Roldin, P., Seinfeld, J. H., Shilling, J.,
Smith, J. N., Thornton, J. A., Volkamer, R., Wang, J., Worsnop, D. R.,
Zaveri, R. A., Zelenyuk, A., and Zhang, Q.: Recent advances in understanding
secondary organic aerosol: Implications for global climate forcing, Rev.
Geophys., 55, 509–559, https://doi.org/10.1002/2016RG000540, 2017.
Snider, G., Weagle, C. L., Murdymootoo, K. K., Ring, A., Ritchie, Y., Stone,
E., Walsh, A., Akoshile, C., Anh, N. X., Balasubramanian, R., Brook, J.,
Qonitan, F. D., Dong, J., Griffith, D., He, K., Holben, B. N., Kahn, R.,
Lagrosas, N., Lestari, P., Ma, Z., Misra, A., Norford, L. K., Quel, E. J.,
Salam, A., Schichtel, B., Segev, L., Tripathi, S., Wang, C., Yu, C., Zhang,
Q., Zhang, Y., Brauer, M., Cohen, A., Gibson, M. D., Liu, Y., Martins, J.
V., Rudich, Y., and Martin, R. V.: Variation in global chemical composition
of PM2.5: emerging results from SPARTAN, Atmos. Chem. Phys., 16,
9629–9653, https://doi.org/10.5194/acp-16-9629-2016, 2016.
Stettler, M. E. J., Eastham, S., and Barrett, S. R. H.: Air quality and
public health impacts of UK airports, Part I: Emissions, Atmos. Environ.,
45, 5415–5424, https://doi.org/10.1016/j.atmosenv.2011.07.012, 2011.
Tang, R., Zhao, J., Liu, Y., Huang, X., Zhang, Y., Zhou, D., Ding, A.,
Nielsen, C. P., and Wang, H.: Air quality and health co-benefits of China's
carbon dioxide emissions peaking before 2030, Nat. Commun., 13, 1008,
https://doi.org/10.1038/s41467-022-28672-3, 2022.
Tao, J., Zhang, L., Cao, J., and Zhang, R.: A review of current knowledge
concerning PM2.5 chemical composition, aerosol optical properties and their
relationships across China, Atmos. Chem. Phys., 17, 9485–9518,
https://doi.org/10.5194/acp-17-9485-2017, 2017.
Tong, D., Zhang, Q., Liu, F., Geng, G., Zheng, Y., Xue, T., Hong, C., Wu,
R., Qin, Y., Zhao, H., Yan, L., and He, K.: Current Emissions and Future
Mitigation Pathways of Coal-Fired Power Plants in China from 2010 to 2030,
Environ. Sci. Technol., 52, 12905–12914, https://doi.org/10.1021/acs.est.8b02919,
2018.
Tong, D., Cheng, J., Liu, Y., Yu, S., Yan, L., Hong, C., Qin, Y., Zhao, H.,
Zheng, Y., Geng, G., Li, M., Liu, F., Zhang, Y., Zheng, B., Clarke, L., and Zhang, Q.: Dynamic projection of anthropogenic emissions in China:
Methodology and 2015–2050 emission pathways under a range of socio-economic,
climate policy, and pollution control scenarios, Atmos. Chem. Phys., 20,
5729–5757, https://doi.org/10.5194/acp-20-5729-2020, 2020.
van Donkelaar, A., Hammer, M. S., Bindle, L., Brauer, M., Brook, J. R.,
Garay, M. J., Hsu, N. C., Kalashnikova, O. V, Kahn, R. A., Lee, C., Levy, R.
C., Lyapustin, A., Sayer, A. M., and Martin, R. V.: Monthly Global Estimates
of Fine Particulate Matter and Their Uncertainty, Environ. Sci. Technol.,
55, 15287–15300, https://doi.org/10.1021/acs.est.1c05309, 2021.
Venkataraman, C., Brauer, M., Tibrewal, K., Sadavarte, P., Ma, Q., Cohen,
A., Chaliyakunnel, S., Frostad, J., Klimont, Z., Martin, R. V., Millet, D.
B., Philip, S., Walker, K., and Wang, S.: Source influence on emission
pathways and ambient PM2.5 pollution over India (2015–2050), Atmos. Chem.
Phys., 18, 8017–8039, https://doi.org/10.5194/acp-18-8017-2018, 2018.
Wang, H., Tian, M., Chen, Y., Shi, G., Liu, Y., Yang, F., Zhang, L., Deng,
L., Yu, J., Peng, C., and Cao, X.: Seasonal characteristics, formation
mechanisms and source origins of PM2.5 in two megacities in Sichuan Basin,
China, Atmos. Chem. Phys., 18, 865–881, https://doi.org/10.5194/acp-18-865-2018,
2018.
Wang, J., Ni, R., Lin, J., Tan, X., Tong, D., Zhao, H., Zhang, Q., Lu, Z.,
Streets, D., Pan, D., Huang, Y., Guan, D., Feng, K., Yan, Y., Hu, Y., Liu,
M., Chen, L., and Liu, P.: Socioeconomic and atmospheric factors affecting
aerosol radiative forcing: Production-based versus consumption-based
perspective, Atmos. Environ., 200, 197–207,
https://doi.org/10.1016/j.atmosenv.2018.12.012, 2019.
Wang, Q., Jacob, D. J., Fisher, J. A., Mao, J., Leibensperger, E. M.,
Carouge, C. C., Le Sager, P., Kondo, Y., Jimenez, J. L., Cubison, M. J., and Doherty, S. J.: Sources of carbonaceous aerosols and deposited black carbon
in the Arctic in winter-spring: implications for radiative forcing, Atmos.
Chem. Phys., 11, 12453–12473, https://doi.org/10.5194/acp-11-12453-2011, 2011.
Wang, Q., Jacob, D. J., Spackman, J. R., Perring, A. E., Schwarz, J. P.,
Moteki, N., Marais, E. A., Ge, C., Wang, J., and Barrett, S. R. H.: Global
budget and radiative forcing of black carbon aerosol: Constraints from
pole-to-pole (HIPPO) observations across the Pacific, J. Geophys. Res.-Atmos., 119, 195–206, https://doi.org/10.1002/2013JD020824, 2014.
Wang, S., Li, S., Xing, J., Ding, Y., Hu, S., Liu, S., Qin, Y., Dong, Z., Dong, J., Song, G., and Dong, L.: Current and future prediction of inter-provincial transport of ambient PM2.5 in China, Atmos. Chem. Phys. Discuss. [preprint], https://doi.org/10.5194/acp-2022-368, 2022.
Wang, T., Xue, L., Brimblecombe, P., Lam, Y. F., Li, L., and Zhang, L.: Ozone
pollution in China: A review of concentrations, meteorological influences,
chemical precursors, and effects, Sci. Total Environ., 575, 1582–1596,
https://doi.org/10.1016/j.scitotenv.2016.10.081, 2017.
Wang, Y. X., McElroy, M. B., Jacob, D. J., and Yantosca, R. M.: A nested grid
formulation for chemical transport over Asia: Applications to CO, J.
Geophys. Res.-Atmos., 109, D22307, https://doi.org/10.1029/2004JD005237, 2004.
Weng, H., Lin, J., Martin, R., Millet, D. B., Jaeglé, L., Ridley, D.,
Keller, C., Li, C., Du, M., and Meng, J.: Global high-resolution emissions of
soil NOx, sea salt aerosols, and biogenic volatile organic compounds, Sci.
Data, 7, 148–163, https://doi.org/10.1038/s41597-020-0488-5, 2020.
West, J. J., Cohen, A., Dentener, F., Brunekreef, B., Zhu, T., Armstrong,
B., Bell, M. L., Brauer, M., Carmichael, G., Costa, D. L., Dockery, D. W.,
Kleeman, M., Krzyzanowski, M., Künzli, N., Liousse, C., Lung, S.-C. C.,
Martin, R. V, Pöschl, U., Pope, C. A., Roberts, J. M., Russell, A. G., and Wiedinmyer, C.: What We Breathe Impacts Our Health: Improving
Understanding of the Link between Air Pollution and Health, Environ. Sci.
Technol., 50, 4895–4904, https://doi.org/10.1021/acs.est.5b03827, 2016.
WHO: WHO Global Air Quality Guidelines: Particulate Matter (PM2.5 and PM10), Ozone, Nitrogen Dioxide, Sulfur Dioxide and Carbon Monoxide, World Health Organization (WHO), Geneva, Switzerland, 2021.
Wu, S., Mickley, L. J., Jacob, D. J., Logan, J. A., Yantosca, R. M., and Rind, D.: Why are there large differences between models in global budgets
of tropospheric ozone?, J. Geophys. Res.-Atmos., 112, D05302,
https://doi.org/10.1029/2006JD007801, 2007.
Xing, J., Lu, X., Wang, S., Wang, T., Ding, D., Yu, S., Shindell, D., Ou,
Y., Morawska, L., Li, S., Ren, L., Zhang, Y., Loughlin, D., Zheng, H., Zhao,
B., Liu, S., Smith, K. R., and Hao, J.: The quest for improved air quality
may push China to continue its CO2 reduction beyond the Paris Commitment,
P. Natl. Acad. Sci. USA, 117, 29535–29542,
https://doi.org/10.1073/pnas.2013297117, 2020.
Yan, Y., Zhou, Y., Kong, S., Lin, J., Wu, J., Zheng, H., Zhang, Z., Song,
A., Bai, Y., Ling, Z., Liu, D., and Zhao, T.: Effectiveness of emission
control in reducing PM2.5 pollution in central China during winter haze
episodes under various potential synoptic controls, Atmos. Chem. Phys.,
21, 3143–3162, https://doi.org/10.5194/acp-21-3143-2021, 2021a.
Yan, Y., Zheng, H., Kong, S., Lin, J., Yao, L., Wu, F., Cheng, Y., Niu, Z.,
Zheng, S., Zeng, X., Yan, Q., Wu, J., Zheng, M., Liu, M., Ni, R., Chen, L.,
Chen, N., Xu, K., Liu, D., Zhao, D., Zhao, T., and Qi, S.: On the local
anthropogenic source diversities and transboundary transport for urban
agglomeration ozone mitigation, Atmos. Environ., 245, 118005,
https://doi.org/10.1016/j.atmosenv.2020.118005, 2021b.
Yue, H., He, C., Huang, Q., Yin, D., and Bryan, B. A.: Stronger policy
required to substantially reduce deaths from PM2.5 pollution in China, Nat.
Commun., 11, 1462, https://doi.org/10.1038/s41467-020-15319-4, 2020.
Zang, H., Zhao, Y., Huo, J., Zhao, Q., Fu, Q., Duan, Y., Shao, J., Huang,
C., An, J., Xue, L., Li, Z., Li, C., and Xiao, H.: High atmospheric oxidation
capacity drives wintertime nitrate pollution in the eastern Yangtze River
Delta of China, Atmos. Chem. Phys., 22, 4355–4374,
https://doi.org/10.5194/acp-22-4355-2022, 2022.
Zender, C. S., Bian, H., and Newman, D.: Mineral Dust Entrainment and
Deposition (DEAD) model: Description and 1990s dust climatology, J. Geophys.
Res., 108, 4416, https://doi.org/10.1029/2002JD002775, 2003.
Zhai, S., Jacob, D. J., Brewer, J. F., Li, K., Moch, J. M., Kim, J., Lee,
S., Lim, H., Lee, H. C., Kuk, S. K., Park, R. J., Jeong, J. I., Wang, X.,
Liu, P., Luo, G., Yu, F., Meng, J., Martin, R. V, Travis, K. R., Hair, J.
W., Anderson, B. E., Dibb, J. E., Jimenez, J. L., Campuzano-Jost, P., Nault,
B. A., Woo, J.-H., Kim, Y., Zhang, Q., and Liao, H.: Relating geostationary
satellite measurements of aerosol optical depth (AOD) over East Asia to fine
particulate matter (PM2.5): insights from the KORUS-AQ aircraft campaign and GEOS-Chem model
simulations, Atmos. Chem. Phys., 21, 16775–16791,
https://doi.org/10.5194/acp-21-16775-2021, 2021.
Zhang, L., Liu, L., Zhao, Y., Gong, S., Zhang, X., Henze, D. K., Capps, S.
L., Fu, T.-M., Zhang, Q., and Wang, Y.: Source attribution of particulate
matter pollution over North China with the adjoint method, Environ. Res.
Lett., 10, 84011, https://doi.org/10.1088/1748-9326/10/8/084011, 2015.
Zhang, Q., Jiang, X., Tong, D., Davis, S. J., Zhao, H., Geng, G., Feng, T.,
Zheng, B., Lu, Z., Streets, D. G., Ni, R., Brauer, M., Van Donkelaar, A.,
Martin, R. V., Huo, H., Liu, Z., Pan, D., Kan, H., Yan, Y., Lin, J., He, K., and Guan, D.: Transboundary health impacts of transported global air
pollution and international trade, Nature, 543, 705–709,
https://doi.org/10.1038/nature21712, 2017.
Zhang, Q., Zheng, Y., Tong, D., Shao, M., Wang, S., Zhang, Y., Xu, X., Wang,
J., He, H., Liu, W., Ding, Y., Lei, Y., Li, J., Wang, Z., Zhang, X., Wang,
Y., Cheng, J., Liu, Y., Shi, Q., Yan, L., Geng, G., Hong, C., Li, M., Liu,
F., Zheng, B., Cao, J., Ding, A., Gao, J., Fu, Q., Huo, J., Liu, B., Liu,
Z., Yang, F., He, K., and Hao, J.: Drivers of improved PM2.5 air quality in
China from 2013 to 2017, P. Natl. Acad. Sci. USA, 116, 24463–24469,
https://doi.org/10.1073/pnas.1907956116, 2019.
Zhang, Y.-L. and Cao, F.: Fine particulate matter (PM2.5) in China at a city
level, Sci. Rep., 5, 14884, https://doi.org/10.1038/srep14884, 2015.
Zheng, B., Tong, D., Li, M., Liu, F., Hong, C., Geng, G., Li, H., Li, X.,
Peng, L., Qi, J., Yan, L., Zhang, Y., Zhao, H., Zheng, Y., He, K., and Zhang,
Q.: Trends in China's anthropogenic emissions since 2010 as the consequence
of clean air actions, Atmos. Chem. Phys., 18, 14095–14111,
https://doi.org/10.5194/acp-18-14095-2018, 2018.
Executive editor
This paper investigates the influence of internationally-transported pollution on China, with a specific highlight on the formation of secondary PM2.5 in the form of nitrate. While sources from within China have traditionally been of most interest for domestic air quality policy, these have diminished over recent years, so sources from outside China may become more significant. The topic of transboundary exchange of air pollution has long been studied in other parts of the world, in particular among CLRTAP signatory countries in North America and Europe, but East Asian transboundary pollution represents a different challenge, in part owing to differences in geography and emissions, but also compared to Europe in particular, the transportation scales are much larger. This work not only quantifies the impacts of long distance pollution on Chinese air quality, but also highlights the complex chemical interactions between the local and transboundary pollutants. Papers such as this will likely influence the debate regarding international controls of air pollutants.
This paper investigates the influence of internationally-transported pollution on China, with a...
Short summary
Research on the sources of Chinese PM2.5 pollution has focused on the contributions of China’s domestic emissions. However, the impact of foreign anthropogenic emissions has typically been simplified or neglected. Here we find that foreign anthropogenic emissions play an important role in Chinese PM2.5 pollution through chemical interactions between foreign-transported pollutants and China’s local emissions. Thus, foreign emission reductions are essential for improving Chinese air quality.
Research on the sources of Chinese PM2.5 pollution has focused on the contributions of China’s...
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