Articles | Volume 22, issue 9
https://doi.org/10.5194/acp-22-6231-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-22-6231-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
New particle formation in coastal New Zealand with a focus on open-ocean air masses
Laboratoire de Météorologie Physique, LaMP-UMR 6016, CNRS, Université Clermont Auvergne, 63178, Aubière, France
Clémence Rose
Laboratoire de Météorologie Physique, LaMP-UMR 6016, CNRS, Université Clermont Auvergne, 63178, Aubière, France
Jonathan V. Trueblood
Laboratoire de Météorologie Physique, LaMP-UMR 6016, CNRS, Université Clermont Auvergne, 63178, Aubière, France
Sally Gray
National Institute of Water & Atmospheric Research Ltd (NIWA), Private Bag 14-901, Wellington/Te Whanganui-a-Tara, New Zealand
Mike Harvey
National Institute of Water & Atmospheric Research Ltd (NIWA), Private Bag 14-901, Wellington/Te Whanganui-a-Tara, New Zealand
Karine Sellegri
CORRESPONDING AUTHOR
Laboratoire de Météorologie Physique, LaMP-UMR 6016, CNRS, Université Clermont Auvergne, 63178, Aubière, France
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During the Sea2cloud campaign in the Southern Pacific Ocean, we measured air-sea emissions from phytopankton of two key atmospheric compounds: DMS and MeSH. These compounds are well-known to play a great role in atmospheric chemistry and climate. We see in this paper that these compounds are most emited by the nanophytoplankton population. We provide here parameters for climate models to predict future trends of the emissions of these compounds and their roles and impacts on the global warming.
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This preprint is open for discussion and under review for Biogeosciences (BG).
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Zoé Brasseur, Dimitri Castarède, Erik S. Thomson, Michael P. Adams, Saskia Drossaart van Dusseldorp, Paavo Heikkilä, Kimmo Korhonen, Janne Lampilahti, Mikhail Paramonov, Julia Schneider, Franziska Vogel, Yusheng Wu, Jonathan P. D. Abbatt, Nina S. Atanasova, Dennis H. Bamford, Barbara Bertozzi, Matthew Boyer, David Brus, Martin I. Daily, Romy Fösig, Ellen Gute, Alexander D. Harrison, Paula Hietala, Kristina Höhler, Zamin A. Kanji, Jorma Keskinen, Larissa Lacher, Markus Lampimäki, Janne Levula, Antti Manninen, Jens Nadolny, Maija Peltola, Grace C. E. Porter, Pyry Poutanen, Ulrike Proske, Tobias Schorr, Nsikanabasi Silas Umo, János Stenszky, Annele Virtanen, Dmitri Moisseev, Markku Kulmala, Benjamin J. Murray, Tuukka Petäjä, Ottmar Möhler, and Jonathan Duplissy
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The present measurement report introduces the ice nucleation campaign organized in Hyytiälä, Finland, in 2018 (HyICE-2018). We provide an overview of the campaign settings, and we describe the measurement infrastructure and operating procedures used. In addition, we use results from ice nucleation instrument inter-comparison to show that the suite of these instruments deployed during the campaign reports consistent results.
Clémence Rose, Martine Collaud Coen, Elisabeth Andrews, Yong Lin, Isaline Bossert, Cathrine Lund Myhre, Thomas Tuch, Alfred Wiedensohler, Markus Fiebig, Pasi Aalto, Andrés Alastuey, Elisabeth Alonso-Blanco, Marcos Andrade, Begoña Artíñano, Todor Arsov, Urs Baltensperger, Susanne Bastian, Olaf Bath, Johan Paul Beukes, Benjamin T. Brem, Nicolas Bukowiecki, Juan Andrés Casquero-Vera, Sébastien Conil, Konstantinos Eleftheriadis, Olivier Favez, Harald Flentje, Maria I. Gini, Francisco Javier Gómez-Moreno, Martin Gysel-Beer, Anna Gannet Hallar, Ivo Kalapov, Nikos Kalivitis, Anne Kasper-Giebl, Melita Keywood, Jeong Eun Kim, Sang-Woo Kim, Adam Kristensson, Markku Kulmala, Heikki Lihavainen, Neng-Huei Lin, Hassan Lyamani, Angela Marinoni, Sebastiao Martins Dos Santos, Olga L. Mayol-Bracero, Frank Meinhardt, Maik Merkel, Jean-Marc Metzger, Nikolaos Mihalopoulos, Jakub Ondracek, Marco Pandolfi, Noemi Pérez, Tuukka Petäjä, Jean-Eudes Petit, David Picard, Jean-Marc Pichon, Veronique Pont, Jean-Philippe Putaud, Fabienne Reisen, Karine Sellegri, Sangeeta Sharma, Gerhard Schauer, Patrick Sheridan, James Patrick Sherman, Andreas Schwerin, Ralf Sohmer, Mar Sorribas, Junying Sun, Pierre Tulet, Ville Vakkari, Pieter Gideon van Zyl, Fernando Velarde, Paolo Villani, Stergios Vratolis, Zdenek Wagner, Sheng-Hsiang Wang, Kay Weinhold, Rolf Weller, Margarita Yela, Vladimir Zdimal, and Paolo Laj
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Alexandre Kukui, Michel Chartier, Jinhe Wang, Hui Chen, Sébastien Dusanter, Stéphane Sauvage, Vincent Michoud, Nadine Locoge, Valérie Gros, Thierry Bourrianne, Karine Sellegri, and Jean-Marc Pichon
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Clémence Rose, Matti P. Rissanen, Siddharth Iyer, Jonathan Duplissy, Chao Yan, John B. Nowak, Aurélie Colomb, Régis Dupuy, Xu-Cheng He, Janne Lampilahti, Yee Jun Tham, Daniela Wimmer, Jean-Marc Metzger, Pierre Tulet, Jérôme Brioude, Céline Planche, Markku Kulmala, and Karine Sellegri
Atmos. Chem. Phys., 21, 4541–4560, https://doi.org/10.5194/acp-21-4541-2021, https://doi.org/10.5194/acp-21-4541-2021, 2021
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Sulfuric acid (H2SO4) is commonly accepted as a key precursor for atmospheric new particle formation. However, direct measurements of [H2SO4] remain challenging, motivating the development of proxies. Using data collected in two different volcanic plumes, we show, under these specific conditions, the good performance of a proxy from the literature and also highlight the benefit of the newly developed proxies for the prediction of the highest [H2SO4] values.
Alkuin Maximilian Koenig, Olivier Magand, Paolo Laj, Marcos Andrade, Isabel Moreno, Fernando Velarde, Grover Salvatierra, René Gutierrez, Luis Blacutt, Diego Aliaga, Thomas Reichler, Karine Sellegri, Olivier Laurent, Michel Ramonet, and Aurélien Dommergue
Atmos. Chem. Phys., 21, 3447–3472, https://doi.org/10.5194/acp-21-3447-2021, https://doi.org/10.5194/acp-21-3447-2021, 2021
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The environmental cycling of atmospheric mercury, a harmful global contaminant, is still not sufficiently constrained, partly due to missing data in remote regions. Here, we address this issue by presenting 20 months of atmospheric mercury measurements, sampled in the Bolivian Andes. We observe a significant seasonal pattern, whose key features we explore. Moreover, we deduce ratios to constrain South American biomass burning mercury emissions and the mercury uptake by the Amazon rainforest.
Nikolaos Evangeliou, Stephen M. Platt, Sabine Eckhardt, Cathrine Lund Myhre, Paolo Laj, Lucas Alados-Arboledas, John Backman, Benjamin T. Brem, Markus Fiebig, Harald Flentje, Angela Marinoni, Marco Pandolfi, Jesus Yus-Dìez, Natalia Prats, Jean P. Putaud, Karine Sellegri, Mar Sorribas, Konstantinos Eleftheriadis, Stergios Vratolis, Alfred Wiedensohler, and Andreas Stohl
Atmos. Chem. Phys., 21, 2675–2692, https://doi.org/10.5194/acp-21-2675-2021, https://doi.org/10.5194/acp-21-2675-2021, 2021
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Following the transmission of SARS-CoV-2 to Europe, social distancing rules were introduced to prevent further spread. We investigate the impacts of the European lockdowns on black carbon (BC) emissions by means of in situ observations and inverse modelling. BC emissions declined by 23 kt in Europe during the lockdowns as compared with previous years and by 11 % as compared to the period prior to lockdowns. Residential combustion prevailed in Eastern Europe, as confirmed by remote sensing data.
André Welti, E. Keith Bigg, Paul J. DeMott, Xianda Gong, Markus Hartmann, Mike Harvey, Silvia Henning, Paul Herenz, Thomas C. J. Hill, Blake Hornblow, Caroline Leck, Mareike Löffler, Christina S. McCluskey, Anne Marie Rauker, Julia Schmale, Christian Tatzelt, Manuela van Pinxteren, and Frank Stratmann
Atmos. Chem. Phys., 20, 15191–15206, https://doi.org/10.5194/acp-20-15191-2020, https://doi.org/10.5194/acp-20-15191-2020, 2020
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Ship-based measurements of maritime ice nuclei concentrations encompassing all oceans are compiled. From this overview it is found that maritime ice nuclei concentrations are typically 10–100 times lower than over continents, while concentrations are surprisingly similar in different oceanic regions. The analysis of the influence of ship emissions shows no effect on the data, making ship-based measurements an efficient strategy for the large-scale exploration of ice nuclei concentrations.
Ilona Ylivinkka, Santeri Kaupinmäki, Meri Virman, Maija Peltola, Ditte Taipale, Tuukka Petäjä, Veli-Matti Kerminen, Markku Kulmala, and Ekaterina Ezhova
Atmos. Meas. Tech., 13, 5595–5619, https://doi.org/10.5194/amt-13-5595-2020, https://doi.org/10.5194/amt-13-5595-2020, 2020
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Short summary
In this study, we developed a new algorithm for cloud classification using solar radiation and cloud base height measurements. Our objective was to develop a simple and inexpensive but effective algorithm for the needs of studies related to ecosystem and atmosphere interactions. In the present study, we used the algorithm for obtaining cloud statistics at a measurement station in southern Finland, and we discuss the advantages and shortcomings of the algorithm.
Martin Heinritzi, Lubna Dada, Mario Simon, Dominik Stolzenburg, Andrea C. Wagner, Lukas Fischer, Lauri R. Ahonen, Stavros Amanatidis, Rima Baalbaki, Andrea Baccarini, Paulus S. Bauer, Bernhard Baumgartner, Federico Bianchi, Sophia Brilke, Dexian Chen, Randall Chiu, Antonio Dias, Josef Dommen, Jonathan Duplissy, Henning Finkenzeller, Carla Frege, Claudia Fuchs, Olga Garmash, Hamish Gordon, Manuel Granzin, Imad El Haddad, Xucheng He, Johanna Helm, Victoria Hofbauer, Christopher R. Hoyle, Juha Kangasluoma, Timo Keber, Changhyuk Kim, Andreas Kürten, Houssni Lamkaddam, Tiia M. Laurila, Janne Lampilahti, Chuan Ping Lee, Katrianne Lehtipalo, Markus Leiminger, Huajun Mai, Vladimir Makhmutov, Hanna Elina Manninen, Ruby Marten, Serge Mathot, Roy Lee Mauldin, Bernhard Mentler, Ugo Molteni, Tatjana Müller, Wei Nie, Tuomo Nieminen, Antti Onnela, Eva Partoll, Monica Passananti, Tuukka Petäjä, Joschka Pfeifer, Veronika Pospisilova, Lauriane L. J. Quéléver, Matti P. Rissanen, Clémence Rose, Siegfried Schobesberger, Wiebke Scholz, Kay Scholze, Mikko Sipilä, Gerhard Steiner, Yuri Stozhkov, Christian Tauber, Yee Jun Tham, Miguel Vazquez-Pufleau, Annele Virtanen, Alexander L. Vogel, Rainer Volkamer, Robert Wagner, Mingyi Wang, Lena Weitz, Daniela Wimmer, Mao Xiao, Chao Yan, Penglin Ye, Qiaozhi Zha, Xueqin Zhou, Antonio Amorim, Urs Baltensperger, Armin Hansel, Markku Kulmala, António Tomé, Paul M. Winkler, Douglas R. Worsnop, Neil M. Donahue, Jasper Kirkby, and Joachim Curtius
Atmos. Chem. Phys., 20, 11809–11821, https://doi.org/10.5194/acp-20-11809-2020, https://doi.org/10.5194/acp-20-11809-2020, 2020
Short summary
Short summary
With experiments performed at CLOUD, we show how isoprene interferes in monoterpene oxidation via RO2 termination at atmospherically relevant concentrations. This interference shifts the distribution of highly oxygenated organic molecules (HOMs) away from C20 class dimers towards C15 class dimers, which subsequently reduces both biogenic nucleation and early growth rates. Our results may help to understand the absence of new-particle formation in isoprene-rich environments.
Cited articles
Boulon, J., Sellegri, K., Venzac, H., Picard, D., Weingartner, E., Wehrle, G., Collaud Coen, M., Bütikofer, R., Flückiger, E., Baltensperger, U., and Laj, P.: New particle formation and ultrafine charged aerosol climatology at a high altitude site in the Alps (Jungfraujoch, 3580 m a.s.l., Switzerland), Atmos. Chem. Phys., 10, 9333–9349,
https://doi.org/10.5194/acp-10-9333-2010, 2010. a
Brailsford, G. W., Stephens, B. B., Gomez, A. J., Riedel, K., Mikaloff Fletcher, S. E., Nichol, S. E., and Manning, M. R.: Long-term
continuous atmospheric CO2 measurements at Baring Head, New Zealand, Atmos. Meas. Tech., 5, 3109–3117, https://doi.org/10.5194/amt-5-3109-2012, 2012. a
Brean, J., Dall’Osto, M., Simó, R., Shi, Z., Beddows, D. C., and Harrison, R. M.: Open ocean and coastal new particle formation from sulfuric acid and amines around the Antarctic Peninsula, Nat. Geosci., 14, 383–388, 2021. a
Burkart, J., Hodshire, A. L., Mungall, E. L., Pierce, J. R., Collins, D. B.,
Ladino, L. A., Lee, A. K., Irish, V., Wentzell, J. J., Liggio, J., Papakyriakou, T., Murphy, J., and Abbatt, J.: Organic condensation and particle growth to CCN sizes in the summertime marine Arctic is driven by materials more semivolatile than at continental sites, Geophys. Res. Lett., 44, 10725–10734, 2017. a
Burkholder, J. B., Curtius, J., Ravishankara, A. R., and Lovejoy, E. R.: Laboratory studies of the homogeneous nucleation of iodine oxides, Atmos. Chem. Phys., 4, 19–34, https://doi.org/10.5194/acp-4-19-2004, 2004. a
Cainey, J. and Harvey, M.: Dimethylsulfide, a limited contributor to new
particle formation in the clean marine boundary layer, Geophys. Res. Lett., 29, 32-1–32-4, 2002. a
Carpenter, L. J., Malin, G., Liss, P., and Küpper, F.: Novel biogenic
iodine-containing trihalomethanes and other short-lived halocarbons in the
coastal east Atlantic, Global Biogeochem. Cy., 14, 1191–1204, 2000. a
Chambers, S., Williams, A., Crawford, J., Griffiths, A., Krummel, P., Steele,
L., and Schoot, V.: A radon-only technique for characterising baseline
constituent concentrations at Cape Grim, Paper presented at Atmospheric
Composition and Chemistry Observations and Modelling Conference incorporating
the Cape Grim Annual Science Meeting, 12–13 November 2014, Aspendale, Victoria, https://apo.ansto.gov.au/dspace/handle/10238/8283 (last access: 6 May 2022), 2014. a
Charlson, R. J., Lovelock, J. E., Andreae, M. O., and Warren, S. G.: Oceanic
phytoplankton, atmospheric sulphur, cloud albedo and climate, Nature, 326,
655–661, https://doi.org/10.1038/326655a0, 1987. a
CliFlo: NIWA's National Climate Database on the Web, https://cliflo.niwa.co.nz/, last access: 11 May 2022. a
Clarke, A., Varner, J., Eisele, F., Mauldin, R., Tanner, D., and Litchy, M.:
Particle production in the remote marine atmosphere: Cloud outflow and
subsidence during ACE 1, J. Geophys. Res.-Atmos., 103, 16397–16409, 1998. a
Croft, B., Martin, R. V., Moore, R. H., Ziemba, L. D., Crosbie, E. C., Liu, H., Russell, L. M., Saliba, G., Wisthaler, A., Müller, M., Schiller, A.,
Galí, M., Chang, R. Y.-W., McDuffie, E. E., Bilsback, K. R., and Pierce,
J. R.: Factors controlling marine aerosol size distributions and their climate effects over the northwest Atlantic Ocean region, Atmos. Chem. Phys., 21, 1889–1916, https://doi.org/10.5194/acp-21-1889-2021, 2021. a
Cui, T., Green, H. S., Selleck, P. W., Zhang, Z., O'Brien, R. E., Gold, A.,
Keywood, M., Kroll, J. H., and Surratt, J. D.: Chemical characterization of
isoprene-and monoterpene-derived secondary organic aerosol tracers in remote
marine aerosols over a quarter century, ACS Earth Space Chem., 3, 935–946, 2019. a
Dada, L., Chellapermal, R., Buenrostro Mazon, S., Paasonen, P., Lampilahti, J., Manninen, H. E., Junninen, H., Petäjä, T., Kerminen, V.-M., and Kulmala, M.: Refined classification and characterization of atmospheric new-particle formation events using air ions, Atmos. Chem. Phys., 18, 17883–17893, https://doi.org/10.5194/acp-18-17883-2018, 2018. a, b, c, d, e, f, g, h, i, j
Dall'Osto, M., Monahan, C., Greaney, R., Beddows, D. C. S., Harrison, R. M., Ceburnis, D., and O'Dowd, C. D.: A statistical analysis of North East Atlantic (submicron) aerosol size distributions, Atmos. Chem. Phys., 11, 12567–12578, https://doi.org/10.5194/acp-11-12567-2011, 2011. a, b, c
Dal Maso, M., Kulmala, M., Riipinen, I., Wagner, R., Hussein, T., Aalto, P. P., and Lehtinen, K. E.: Formation and growth of fresh atmospheric aerosols:
eight years of aerosol size distribution data from SMEAR II, Hyytiala,
Finland, Boreal Environ. Res., 10, 323–336, 2005. a, b, c, d, e, f, g, h, i, j, k, l
Forestieri, S., Moore, K., Martinez Borrero, R., Wang, A., Stokes, M., and
Cappa, C.: Temperature and composition dependence of sea spray aerosol
production, Geophys. Res. Lett., 45, 7218–7225, 2018. a
Fossum, K. N., Ovadnevaite, J., Ceburnis, D., Dall'Osto, M., Marullo, S.,
Bellacicco, M., Simó, R., Liu, D., Flynn, M., Zuend, A., and O'Dowd, C.: Summertime Primary and Secondary Contributions to Southern Ocean Cloud Condensation Nuclei, Scient. Rep., 8, 13844, https://doi.org/10.1038/s41598-018-32047-4, 2018. a, b
Gómez Martín, J. C., Saiz-Lopez, A., Cuevas, C. A., Fernandez, R. P.,
Gilfedder, B., Weller, R., Baker, A. R., Droste, E., and Lai, S.: Spatial and
temporal variability of iodine in aerosol, J. Geophys. Res.-Atmos., 126, e2020JD034410, https://doi.org/10.1029/2020JD034410, 2021. a
Gordon, H., Kirkby, J., Baltensperger, U., Bianchi, F., Breitenlechner, M.,
Curtius, J., Dias, A., Dommen, J., Donahue, N. M., Dunne, E. M., Duplissy, J., Ehrhart, S., Flagan, R. C., Frege, C., Fuchs, C., Hansel, A., Hoyle, C. R., Kulmala, M., Kürten, A., Lehtipalo, K., Makhmutov, V., Molteni, U., Rissanen, M. P., Stozkhov, Y., Tröstl, J., Tsagkogeorgas, G., Wagner, R., Williamson, C., Wimmer, D., Winkler, P. M., Yan, C., and Carslaw, K. S.: Causes and importance of new particle formation in the present-day and preindustrial atmospheres, J. Geophys. Res.-Atmos., 122, 8739–8760, 2017. a
Gras, J. L. and Keywood, M.: Cloud condensation nuclei over the Southern Ocean: wind dependence and seasonal cycles, Atmos. Chem. Phys., 17, 4419–4432, https://doi.org/10.5194/acp-17-4419-2017, 2017. a
Gras, J. L., Jimi, S. I., Siems, S. T., and Krummel, P. B.: Postfrontal
nanoparticles at Cape Grim: observations, Environ. Chem., 6, 508–514, 2009. a
Greater Wellington Regional Council: Live Data Viewer, http://graphs.gw.govt.nz/, last accessed: 31 May 2021. a
Greene, C.: landmask, MATLAB Central File Exchange, https://www.mathworks.com/matlabcentral/fileexchange/48661-landmask, last access: 11 May 2022. a
Hamed, A., Korhonen, H., Sihto, S.-L., Joutsensaari, J., Järvinen, H.,
Petäjä, T., Arnold, F., Nieminen, T., Kulmala, M., Smith, J. N., Lehtinen, K. E. J., and Laaksonen, A.: The role of relative humidity in continental new particle formation, J. Geophys. Res.-Atmos., 116, D03202, https://doi.org/10.1029/2010JD014186, 2011. a
Heintzenberg, J., Wehner, B., and Birmili, W.: `How to find bananas in the
atmospheric aerosol': new approach for analyzing atmospheric nucleation and
growth events, Tellus B, 59, 273–282, 2007. a
Humphries, R. S., Keywood, M. D., Gribben, S., McRobert, I. M., Ward, J. P.,
Selleck, P., Taylor, S., Harnwell, J., Flynn, C., Kulkarni, G. R., Mace, G. G., Protat, A., Alexander, S. P., and McFarquhar, G.: Southern Ocean latitudinal gradients of cloud condensation nuclei, Atmos. Chem. Phys., 21, 12757–12782, https://doi.org/10.5194/acp-21-12757-2021, 2021. a
Hussein, T., Martikainen, J., Junninen, H., Sogacheva, L., Wagner, R.,
Dal Maso, M., Riipinen, I., Aalto, P. P., and Kulmala, M.: Observation of
regional new particle formation in the urban atmosphere, Tellus B, 60, 509–521, 2008. a
Jokinen, T., Sipilä, M., Kontkanen, J., Vakkari, V., Tisler, P., Duplissy, E.-M., Junninen, H., Kangasluoma, J., Manninen, H., Petäjä, T., Kulmala, M., Worsnop, D. R., Kirkby, J., Virkkula, A., and Kerminen, V.-M.: Ion-induced sulfuric acid–ammonia nucleation drives particle formation in coastal Antarctica, Sci. Adv., 4, eaat9744, https://doi.org/10.1126/sciadv.aat9744, 2018. a
Jokinen, T., Lehtipalo, K., Thakur, R. C., Ylivinkka, I., Neitola, K., Sarnela, N., Laitinen, T., Kulmala, M., Petäjä, T., and Sipilä, M.: Measurement report: Long-term measurements of aerosol precursor concentrations in the Finnish subarctic boreal forest, Atmos. Chem. Phys., 22, 2237–2254, https://doi.org/10.5194/acp-22-2237-2022, 2022. a
Kerminen, V.-M., Paramonov, M., Anttila, T., Riipinen, I., Fountoukis, C., Korhonen, H., Asmi, E., Laakso, L., Lihavainen, H., Swietlicki, E., Svenningsson, B., Asmi, A., Pandis, S. N., Kulmala, M., and Petäjä, T.: Cloud condensation nuclei production associated with atmospheric nucleation: a synthesis based on existing literature and new results, Atmos. Chem. Phys., 12, 12037–12059, https://doi.org/10.5194/acp-12-12037-2012, 2012. a
Kerminen, V.-M., Chen, X., Vakkari, V., Petäjä, T., Kulmala, M., and
Bianchi, F.: Atmospheric new particle formation and growth: review of field
observations, Environ. Res. Lett., 13, 103003, https://doi.org/10.1088/1748-9326/aadf3c, 2018. a
Kulmala, M., Maso, M. D., Mäkelä, J., Pirjola, L., Väkevä, M., Aalto, P., Miikkulainen, P., Hämeri, K., and O'dowd, C.: On the
formation, growth and composition of nucleation mode particles, Tellus B, 53, 479–490, 2001. a
Kulmala, M., Petäjä, T., Nieminen, T., Sipilä, M., Manninen, H. E., Lehtipalo, K., Dal Maso, M., Aalto, P. P., Junninen, H., Paasonen, P.,
Riipinen, I., Lehtinen, K. E. J., Laaksonen, A., and Kerminen, V.-M.: Measurement of the nucleation of atmospheric aerosol particles, Nat. Protocol., 7, 1651, https://doi.org/10.1038/nprot.2012.091, 2012. a
Land information New Zealand: Tide predictions, https://www.linz.govt.nz/sea/tides/tide-predictions, last access: 31 May 2021. a
Law, C. S., Smith, M. J., Harvey, M. J., Bell, T. G., Cravigan, L. T., Elliott, F. C., Lawson, S. J., Lizotte, M., Marriner, A., McGregor, J., Ristovski, Z., Safi, K. A., Saltzman, E. S., Vaattovaara, P., and Walker, C. F.: Overview and preliminary results of the Surface Ocean Aerosol Production (SOAP) campaign, Atmos. Chem. Phys., 17, 13645–13667, https://doi.org/10.5194/acp-17-13645-2017, 2017. a, b, c
Li, J., Davy, P., Harvey, M., Katzman, T., Mitchell, T., and Michalski, G.:
Nitrogen isotopes in nitrate aerosols collected in the remote marine boundary
layer: Implications for nitrogen isotopic fractionations among atmospheric
reactive nitrogen species, Atmos. Environ., 245, 118028, https://doi.org/10.1016/j.atmosenv.2020.118028, 2021. a
McCoy, D. T., Burrows, S. M., Wood, R., Grosvenor, D. P., Elliott, S. M., Ma,
P.-L., Rasch, P. J., and Hartmann, D. L.: Natural aerosols explain seasonal
and spatial patterns of Southern Ocean cloud albedo, Sci. Adv., 1, e1500157, https://doi.org/10.1126/sciadv.1500157, 2015. a
Mirme, S. and Mirme, A.: The mathematical principles and design of the NAIS – a spectrometer for the measurement of cluster ion and nanometer aerosol size distributions, Atmos. Meas. Tech., 6, 1061–1071, https://doi.org/10.5194/amt-6-1061-2013, 2013. a
Modini, R. L., Ristovski, Z. D., Johnson, G. R., He, C., Surawski, N., Morawska, L., Suni, T., and Kulmala, M.: New particle formation and growth at a remote, sub-tropical coastal location, Atmos. Chem. Phys., 9, 7607–7621, https://doi.org/10.5194/acp-9-7607-2009, 2009. a, b, c
Molloy, S. and Galbally, I.: Analysis and identification of a suitable baseline definition for tropospheric ozone at Cape Grim, Tasmania, Baseline
Atmospheric Program Australia, Baseline: 2009–2010, 7–16,
http://www.bom.gov.au/inside/cgbaps/baseline/Baseline_2009-2010.pdf (last access: 6 May 2022), 2014. a
Murphy, R., Pinkerton, M., Richardson, K., Bradford-Grieve, J., and Boyd, P.:
Phytoplankton distributions around New Zealand derived from SeaWiFS
remotely-sensed ocean colour data, N. Zeal. J. Mar. Freshw. Res., 35, 343–362, 2001. a
Nieminen, T., Kerminen, V.-M., Petäjä, T., Aalto, P. P., Arshinov, M., Asmi, E., Baltensperger, U., Beddows, D. C. S., Beukes, J. P., Collins, D., Ding, A., Harrison, R. M., Henzing, B., Hooda, R., Hu, M., Hõrrak, U., Kivekäs, N., Komsaare, K., Krejci, R., Kristensson, A., Laakso, L., Laaksonen, A., Leaitch, W. R., Lihavainen, H., Mihalopoulos, N., Németh, Z., Nie, W., O'Dowd, C., Salma, I., Sellegri, K., Svenningsson, B., Swietlicki, E., Tunved, P., Ulevicius, V., Vakkari, V., Vana, M., Wiedensohler, A., Wu, Z., Virtanen, A., and Kulmala, M.: Global analysis of continental boundary layer new particle formation based on long-term measurements, Atmos. Chem. Phys., 18, 14737–14756, https://doi.org/10.5194/acp-18-14737-2018, 2018. a, b, c, d, e, f, g
Noble, S. R. and Hudson, J. G.: Effects of continental clouds on surface Aitken and accumulation modes, J. Geophys. Res.-Atmos., 124, 5479–5502, 2019. a
Nodder, S.: Short-term sediment trap fluxes from Chatham Rise, southwest
Pacific Ocean, Limnol. Oceanogr., 42, 777–783, 1997. a
O'Dowd, C., Monahan, C., and Dall'Osto, M.: On the occurrence of open ocean
particle production and growth events, Geophys. Res. Lett., 37, L19805, https://doi.org/10.1029/2010GL044679, 2010. a, b
Paasonen, P., Peltola, M., Kontkanen, J., Junninen, H., Kerminen, V.-M., and
Kulmala, M.: Comprehensive analysis of particle growth rates from nucleation
mode to cloud condensation nuclei in boreal forest, Atmos. Chem. Phys., 18, 12085–12103, https://doi.org/10.5194/acp-18-12085-2018, 2018. a, b, c, d
Quinn, P. and Bates, T.: The case against climate regulation via oceanic
phytoplankton sulphur emissions, Nature, 480, 51–56, https://doi.org/10.1038/nature10580, 2011. a
Ren, L., Nash, S., and Hartnett, M.: Observation and modeling of tide-and
wind-induced surface currents in Galway Bay, Water Sci. Eng., 8, 345–352, 2015. a
Rolph, G., Stein, A., and Stunder, B.: Real-time environmental applications and display system: READY, Environ. Model. Softw., 95, 210–228, 2017. a
Rose, C., Sellegri, K., Asmi, E., Hervo, M., Freney, E., Colomb, A., Junninen, H., Duplissy, J., Sipilä, M., Kontkanen, J., Lehtipalo, K., and Kulmala, M.: Major contribution of neutral clusters to new particle formation at the interface between the boundary layer and the free troposphere, Atmos. Chem. Phys., 15, 3413–3428, https://doi.org/10.5194/acp-15-3413-2015, 2015a. a
Rose, C., Sellegri, K., Freney, E., Dupuy, R., Colomb, A., Pichon, J.-M., Ribeiro, M., Bourianne, T., Burnet, F., and Schwarzenboeck, A.: Airborne measurements of new particle formation in the free troposphere above the Mediterranean Sea during the HYMEX campaign, Atmos. Chem. Phys., 15, 10203–10218, https://doi.org/10.5194/acp-15-10203-2015, 2015b. a
Rosenfeld, D., Zhu, Y., Wang, M., Zheng, Y., Goren, T., and Yu, S.:
Aerosol-driven droplet concentrations dominate coverage and water of oceanic
low-level clouds, Science, 363, eaav0566, https://doi.org/10.1126/science.aav0566, 2019. a, b
Sanchez, K. J., Chen, C.-L., Russell, L. M., Betha, R., Liu, J., Price, D. J., Massoli, P., Ziemba, L. D., Crosbie, E. C., Moore, R. H., Müller, M., Schiller, S. A., Wisthaler, A., Lee, A. K. Y., Quinn, P. K., Bates, T. S., Porter, J., Bell, T. G., Saltzman, E. S., Vaillancourt, R. D., and Behrenfeld, M. J.: Substantial Seasonal Contribution of Observed Biogenic Sulfate Particles to Cloud Condensation Nuclei, Scient. Rep., 8, 3235, https://doi.org/10.1038/s41598-018-21590-9, 2018. a, b
Schmale, J., Baccarini, A., Thurnherr, I., Henning, S., Efraim, A., Regayre,
L., Bolas, C., Hartmann, M., Welti, A., Lehtipalo, K., Aemisegger, F., Tatzelt, C., Landwehr, S., Modini, R. L., Tummon, F., Johnson, J. S., Harris, N., Schnaiter, M., Toffoli, A., Derkani, M., Bukowiecki, N., Stratmann, F., Dommen, J., Baltensperger, U., Wernli, H., Rosenfeld, D., Gysel-Beer, M., and Carslaw, K. S.: Overview of the Antarctic circumnavigation expedition: Study of preindustrial-like aerosols and their climate effects (ACE-SPACE), B. Am. Meteorol. Soc., 100, 2260–2283, 2019. a
Schwier, A. N., Rose, C., Asmi, E., Ebling, A. M., Landing, W. M., Marro, S.,
Pedrotti, M.-L., Sallon, A., Iuculano, F., Agusti, S., Tsiola, A., Pitta, P.,
Louis, J., Guieu, C., Gazeau, F., and Sellegri, K.: Primary marine aerosol
emissions from the Mediterranean Sea during pre-bloom and oligotrophic
conditions: correlations to seawater chlorophyll a from a mesocosm study, Atmos. Chem. Phys., 15, 7961–7976, https://doi.org/10.5194/acp-15-7961-2015, 2015. a
Sea2Cloud: Catalogue, https://sea2cloud.data-terra.org/en/catalogue/, last access: 11 May 2022. a
Sellegri, K.: Sea2Cloud – Baring-Head – CPC – Level 0, Dataterra [data set], https://doi.org/10.25326/354, 2022a. a
Sellegri, K.: Sea2Cloud – Baring-Head SMPS – Level 0, Dataterra [data set] https://doi.org/10.25326/356, 2022b. a
Sellegri, K.: Sea2Cloud – Baring-Head – PSM – Level 2, Dataterra [data set], https://doi.org/10.25326/355, 2022c. a
Sievering, H., Cainey, J., Harvey, M., McGregor, J., Nichol, S., and Quinn, P.: Aerosol non-sea-salt sulfate in the remote marine boundary layer under
clear-sky and normal cloudiness conditions: Ocean-derived biogenic alkalinity
enhances sea-salt sulfate production by ozone oxidation, J. Geophys. Res.-Atmos., 109, D19317, https://doi.org/10.1029/2003JD004315, 2004. a, b
Simon, M., Dada, L., Heinritzi, M., Scholz, W., Stolzenburg, D., Fischer, L., Wagner, A. C., Kürten, A., Rörup, B., He, X.-C., Almeida, J., Baalbaki, R., Baccarini, A., Bauer, P. S., Beck, L., Bergen, A., Bianchi, F., Bräkling, S., Brilke, S., Caudillo, L., Chen, D., Chu, B., Dias, A., Draper, D. C., Duplissy, J., El-Haddad, I., Finkenzeller, H., Frege, C., Gonzalez-Carracedo, L., Gordon, H., Granzin, M., Hakala, J., Hofbauer, V., Hoyle, C. R., Kim, C., Kong, W., Lamkaddam, H., Lee, C. P., Lehtipalo, K., Leiminger, M., Mai, H., Manninen, H. E., Marie, G., Marten, R., Mentler, B., Molteni, U., Nichman, L., Nie, W., Ojdanic, A., Onnela, A., Partoll, E., Petäjä, T., Pfeifer, J., Philippov, M., Quéléver, L. L. J., Ranjithkumar, A., Rissanen, M. P., Schallhart, S., Schobesberger, S., Schuchmann, S., Shen, J., Sipilä, M., Steiner, G., Stozhkov, Y., Tauber, C., Tham, Y. J., Tomé, A. R., Vazquez-Pufleau, M., Vogel, A. L., Wagner, R., Wang, M., Wang, D. S., Wang, Y., Weber, S. K., Wu, Y., Xiao, M., Yan, C., Ye, P., Ye, Q., Zauner-Wieczorek, M., Zhou, X., Baltensperger, U., Dommen, J., Flagan, R. C., Hansel, A., Kulmala, M., Volkamer, R., Winkler, P. M., Worsnop, D. R., Donahue, N. M., Kirkby, J., and Curtius, J.: Molecular understanding of new-particle formation from α-pinene between −50 and +25 ∘C, Atmos. Chem. Phys., 20, 9183–9207, https://doi.org/10.5194/acp-20-9183-2020, 2020. a
Stein, A., Draxler, R. R., Rolph, G. D., Stunder, B. J., Cohen, M., and Ngan,
F.: NOAA's HYSPLIT atmospheric transport and dispersion modeling system, B. Am. Meteorol. Soc., 96, 2059–2077, 2015. a
Sulo, J., Sarnela, N., Kontkanen, J., Ahonen, L., Paasonen, P., Laurila, T., Jokinen, T., Kangasluoma, J., Junninen, H., Sipilä, M., Petäjä, T., Kulmala, M., and Lehtipalo, K.: Long-term measurement of sub-3 nm particles and their precursor gases in the boreal forest, Atmos. Chem. Phys., 21, 695–715, https://doi.org/10.5194/acp-21-695-2021, 2021.
a
Vanhanen, J., Mikkilä, J., Lehtipalo, K., Sipilä, M., Manninen, H., Siivola, E., Petäjä, T., and Kulmala, M.: Particle size magnifier for nano-CN
detection, Aerosol Sci. Tech., 45, 533–542, 2011. a
Zheng, G., Kuang, C., Uin, J., Watson, T., and Wang, J.: Large contribution of organics to condensational growth and formation of cloud condensation nuclei (CCN) in the remote marine boundary layer, Atmos. Chem. Phys., 20, 12515–12525, https://doi.org/10.5194/acp-20-12515-2020, 2020. a
Zheng, G., Wang, Y., Wood, R., Jensen, M. P., Kuang, C., McCoy, I. L.,
Matthews, A., Mei, F., Tomlinson, J. M., Shilling, J. E., Zawadowicz,M. A., Crosbie, E., Moore, R., Ziemba, L., Andreae, M. O., and Wang, J.: New particle formation in the remote marine boundary layer, Nat. Commun., 12, 1–10, 2021. a
Short summary
Despite the importance of marine aerosol measurements for constraining climate models, these measurements are scarce. We measured the aerosol particle number size distribution in coastal New Zealand over a total period of 10 months. This paper analyses the aerosol properties at the site, with a special focus on new particle formation and marine air masses. New particle formation was observed frequently, but in marine air masses it did not follow traditional event criteria.
Despite the importance of marine aerosol measurements for constraining climate models, these...
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