Articles | Volume 22, issue 24
https://doi.org/10.5194/acp-22-15867-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-15867-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
19 Dec 2022
Research article |
| 19 Dec 2022
| 19 Dec 2022
An assessment of land energy balance over East Asia from multiple lines of evidence and the roles of the Tibet Plateau, aerosols, and clouds
Qiuyan Wang
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Nanjing University of Information Science and Technology, Nanjing 210044, China
State Key Laboratory of Severe Weather, Chinese Academy of
Meteorological Sciences, Beijing 100081, China
Institute for Atmospheric and Climate Science, ETH Zurich, 8092
Zurich, Switzerland
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Nanjing University of Information Science and Technology, Nanjing 210044, China
State Key Laboratory of Severe Weather, Chinese Academy of
Meteorological Sciences, Beijing 100081, China
Su Yang
National Meteorological Information Center, China Meteorological
Administration, Beijing 100081, China
Qi Chen
State Key Laboratory of Severe Weather, Chinese Academy of
Meteorological Sciences, Beijing 100081, China
Xixun Zhou
State Key Laboratory of Severe Weather, Chinese Academy of
Meteorological Sciences, Beijing 100081, China
Bing Xie
Laboratory for Climate Studies of China Meteorological
Administration, National Climate Center, Beijing 100081, China
Yuying Wang
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Nanjing University of Information Science and Technology, Nanjing 210044, China
Guangyu Shi
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Nanjing University of Information Science and Technology, Nanjing 210044, China
State Key Laboratory of Numerical Modeling for Atmospheric Sciences
and Geophysical Fluid Dynamics, Institute of Atmospheric Physics, Chinese
Academy of Sciences, Beijing 100029, China
Martin Wild
Institute for Atmospheric and Climate Science, ETH Zurich, 8092
Zurich, Switzerland
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A MAX-DOAS instrument was operated to derive tropospheric vertical profiles of NO2, SO2, HONO, HCHO, CHOCHO and aerosols in the central western North China Plain in May and June 2016. The MAX-DOAS results are verified by comparisons with a collocated Raman lidar, overpass aircraft measurements, a sun photometer and in situ measurements. The contributions of regional transports and local emissions to the pollutants are evaluated based on case studies and statistic analysis.
Hao He, Xinrong Ren, Sarah E. Benish, Zhanqing Li, Fei Wang, Yuying Wang, Timothy P. Canty, Xiaobo Dong, Feng Lv, Yongtao Hu, Tong Zhu, and Russell R. Dickerson
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2019-248, https://doi.org/10.5194/acp-2019-248, 2019
Revised manuscript not accepted
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We conducted aircraft measurements of air pollution in the North China Plain. Concentrations of air pollutants higher than the air quality standards were observed. Our modeling study indicates that the rate of ozone (one major air pollutant) production is determined by volatile organic compounds (VOCs), which is confirmed by satellite observations. Currently, VOCs are not well regulated in China, so this study suggests the future direction of control measures to improve air quality in China.
Jun Chen, Zhanqing Li, Min Lv, Yuying Wang, Wei Wang, Yingjie Zhang, Haofei Wang, Xing Yan, Yele Sun, and Maureen Cribb
Atmos. Chem. Phys., 19, 1327–1342, https://doi.org/10.5194/acp-19-1327-2019, https://doi.org/10.5194/acp-19-1327-2019, 2019
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The hygroscopic growth function of aerosol particles is derived from Raman lidar, whose dependence on aerosol chemical composition is investigated using data from an aerosol chemical speciation monitor (ACSM) and a hygroscopic tandem differential mobility analyzer (H-TDMA) deployed in China. Two distinct cases were chosen with marked differences in their hygroscopic growth, which was fitted by the Kasten model. The differences were attributed to different amounts of chemical species.
Yingjie Zhang, Wei Du, Yuying Wang, Qingqing Wang, Haofei Wang, Haitao Zheng, Fang Zhang, Hongrong Shi, Yuxuan Bian, Yongxiang Han, Pingqing Fu, Francesco Canonaco, André S. H. Prévôt, Tong Zhu, Pucai Wang, Zhanqing Li, and Yele Sun
Atmos. Chem. Phys., 18, 14637–14651, https://doi.org/10.5194/acp-18-14637-2018, https://doi.org/10.5194/acp-18-14637-2018, 2018
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We have a comprehensive characterization of aerosol chemistry and particle growth events at a downwind site of a highly polluted city in the North China Plain. Aerosol particles at the urban downwind site were highly aged and mainly from secondary formation. New particle growth events were also frequently observed on both clean and polluted days. While both sulfate and SOA played important roles in particle growth during clean periods, SOA was more important than sulfate during polluted events.
Yuying Wang, Zhanqing Li, Yingjie Zhang, Wei Du, Fang Zhang, Haobo Tan, Hanbing Xu, Tianyi Fan, Xiaoai Jin, Xinxin Fan, Zipeng Dong, Qiuyan Wang, and Yele Sun
Atmos. Chem. Phys., 18, 11739–11752, https://doi.org/10.5194/acp-18-11739-2018, https://doi.org/10.5194/acp-18-11739-2018, 2018
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Very different aerosol hygroscopicities and mixing states were found at these sites in the North China Plain. The PDF for 40–200 nm particles showed the particles were highly aged and internally mixed at Xingtai because of high pollution and strong photochemical reactions. A good proxy for the chemical comical composition (kappa = 0.31) in calculating CCN concentration was found. Importantly, our study investigated the influence of industrial emissions on the aerosol properties.
Wei Zhou, Jian Zhao, Bin Ouyang, Archit Mehra, Weiqi Xu, Yuying Wang, Thomas J. Bannan, Stephen D. Worrall, Michael Priestley, Asan Bacak, Qi Chen, Conghui Xie, Qingqing Wang, Junfeng Wang, Wei Du, Yingjie Zhang, Xinlei Ge, Penglin Ye, James D. Lee, Pingqing Fu, Zifa Wang, Douglas Worsnop, Roderic Jones, Carl J. Percival, Hugh Coe, and Yele Sun
Atmos. Chem. Phys., 18, 11581–11597, https://doi.org/10.5194/acp-18-11581-2018, https://doi.org/10.5194/acp-18-11581-2018, 2018
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We present measurements of gas-phase N2O5 and ClNO2 by ToF-CIMS during summer in urban Beijing as part of the APHH campaign. High reactivity of N2O5 indicative of active nocturnal chemistry was observed. The lifetime of N2O5 as a function of aerosol surface area and relative humidity was characterized, and N2O5 uptake coefficients were estimated. We also found that the N2O5 loss in this study is mainly attributed to its indirect loss via reactions of NO3 with VOCs and NO.
Gehui Wang, Fang Zhang, Jianfei Peng, Lian Duan, Yuemeng Ji, Wilmarie Marrero-Ortiz, Jiayuan Wang, Jianjun Li, Can Wu, Cong Cao, Yuan Wang, Jun Zheng, Jeremiah Secrest, Yixin Li, Yuying Wang, Hong Li, Na Li, and Renyi Zhang
Atmos. Chem. Phys., 18, 10123–10132, https://doi.org/10.5194/acp-18-10123-2018, https://doi.org/10.5194/acp-18-10123-2018, 2018
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Several studies using thermodynamic models estimated pH and sulfate formation rate during pollution periods in China are highly conflicting. Here we show distinct sulfate formation for organic seed particles from that of (NH4)2SO4 seeds, when the particles are exposed to SO2, NO2, and NH3 at high RH. Our results reveal that the pH value of ambient organics-dominated aerosols is sufficiently high to promote efficient SO2 oxidation by NO2 with NH3 neutralization under polluted conditions in China.
Emmanouil Oikonomakis, Sebnem Aksoyoglu, Martin Wild, Giancarlo Ciarelli, Urs Baltensperger, and André Stephan Henry Prévôt
Atmos. Chem. Phys., 18, 9741–9765, https://doi.org/10.5194/acp-18-9741-2018, https://doi.org/10.5194/acp-18-9741-2018, 2018
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We report a model sensitivity study on the impact of aerosol–radiation interaction (ARI) changes in Europe between 1990 and 2010 on summer surface ozone via effects on photolysis rates and biogenic emissions. The overall impact of ARI changes on ozone was relatively small when compared to the total ozone concentrations, but it was more important when compared to the order of magnitude of ozone trends, indicating a potential partial damping of the effects of ozone precursor emissions' reduction.
Jiming Li, Qiaoyi Lv, Bida Jian, Min Zhang, Chuanfeng Zhao, Qiang Fu, Kazuaki Kawamoto, and Hua Zhang
Atmos. Chem. Phys., 18, 7329–7343, https://doi.org/10.5194/acp-18-7329-2018, https://doi.org/10.5194/acp-18-7329-2018, 2018
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The accurate representation of cloud vertical overlap in atmospheric models is very important for predicting the total cloud cover and calculating the radiative budget. We propose a valid scheme for quantifying the degree of overlap over the Tibetan Plateau (TP). The new scheme parameterizes decorrelation length scale L as a function of wind shear and atmospheric stability and improves the simulation of total cloud cover over TP when the separations between cloud layers are greater than 1 km.
Jingye Ren, Fang Zhang, Yuying Wang, Don Collins, Xinxin Fan, Xiaoai Jin, Weiqi Xu, Yele Sun, Maureen Cribb, and Zhanqing Li
Atmos. Chem. Phys., 18, 6907–6921, https://doi.org/10.5194/acp-18-6907-2018, https://doi.org/10.5194/acp-18-6907-2018, 2018
Tianyi Fan, Xiaohong Liu, Po-Lun Ma, Qiang Zhang, Zhanqing Li, Yiquan Jiang, Fang Zhang, Chuanfeng Zhao, Xin Yang, Fang Wu, and Yuying Wang
Atmos. Chem. Phys., 18, 1395–1417, https://doi.org/10.5194/acp-18-1395-2018, https://doi.org/10.5194/acp-18-1395-2018, 2018
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We found that 22–28 % of the low AOD bias in eastern China simulated by the Community Atmosphere Model version 5 can be improved by using a new emission inventory. The concentrations of primary aerosols are closely related to the emission, while the seasonal variations of secondary aerosols depend more on atmospheric processes. This study highlights the importance of improving both the emission and atmospheric processes in modeling the atmospheric aerosols and their radiative effects.
Huizheng Che, Bing Qi, Hujia Zhao, Xiangao Xia, Thomas F. Eck, Philippe Goloub, Oleg Dubovik, Victor Estelles, Emilio Cuevas-Agulló, Luc Blarel, Yunfei Wu, Jun Zhu, Rongguang Du, Yaqiang Wang, Hong Wang, Ke Gui, Jie Yu, Yu Zheng, Tianze Sun, Quanliang Chen, Guangyu Shi, and Xiaoye Zhang
Atmos. Chem. Phys., 18, 405–425, https://doi.org/10.5194/acp-18-405-2018, https://doi.org/10.5194/acp-18-405-2018, 2018
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Sun photometer measurements from seven sites in the Yangtze River Delta (YRD) from 2011 to 2015 were used to characterize the climatology of aerosol microphysical and optical properties, calculate direct aerosol radiative forcing (DARF) and classify aerosols based on size and absorption. This study contributes to our understanding of aerosols and regional climate/air quality, and the results will be useful for validating satellite retrievals and for improving climate models and remote sensing.
Maria Sand, Bjørn H. Samset, Yves Balkanski, Susanne Bauer, Nicolas Bellouin, Terje K. Berntsen, Huisheng Bian, Mian Chin, Thomas Diehl, Richard Easter, Steven J. Ghan, Trond Iversen, Alf Kirkevåg, Jean-François Lamarque, Guangxing Lin, Xiaohong Liu, Gan Luo, Gunnar Myhre, Twan van Noije, Joyce E. Penner, Michael Schulz, Øyvind Seland, Ragnhild B. Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Fangqun Yu, Kai Zhang, and Hua Zhang
Atmos. Chem. Phys., 17, 12197–12218, https://doi.org/10.5194/acp-17-12197-2017, https://doi.org/10.5194/acp-17-12197-2017, 2017
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The role of aerosols in the changing polar climate is not well understood and the aerosols are poorly constrained in the models. In this study we have compared output from 16 different aerosol models with available observations at both poles. We show that the model median is representative of the observations, but the model spread is large. The Arctic direct aerosol radiative effect over the industrial area is positive during spring due to black carbon and negative during summer due to sulfate.
Stephan Nyeki, Stefan Wacker, Julian Gröbner, Wolfgang Finsterle, and Martin Wild
Atmos. Meas. Tech., 10, 3057–3071, https://doi.org/10.5194/amt-10-3057-2017, https://doi.org/10.5194/amt-10-3057-2017, 2017
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A large number of radiometers used to measure solar and terrestrial broadband radiation are traceable to World Standard Groups at PMOD/WRC in Davos, Switzerland. A small correction of each group may be required in the future, and this study examines the methods and implications of this on data sets collected at four remote baseline stations since the 1990s. The goal is to develop a better estimate of the solar and terrestrial radiation budget at the Earth's surface.
Martin Wild, Atsumu Ohmura, Christoph Schär, Guido Müller, Doris Folini, Matthias Schwarz, Maria Zyta Hakuba, and Arturo Sanchez-Lorenzo
Earth Syst. Sci. Data, 9, 601–613, https://doi.org/10.5194/essd-9-601-2017, https://doi.org/10.5194/essd-9-601-2017, 2017
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The Global Energy Balance Archive (GEBA) is a database for the central storage of worldwide measured energy fluxes at the Earth's surface, maintained at ETH Zurich (Switzerland). This paper documents the status of the GEBA version 2017 database, presents the new web interface and user access, and reviews the scientific impact that GEBA data had in various applications. GEBA has continuously been expanded and updated and to date contains around 500 000 monthly mean entries from 2500 locations.
Yawen Wang, Martin Wild, Arturo Sanchez-Lorenzo, and Veronica Manara
Ann. Geophys., 35, 839–851, https://doi.org/10.5194/angeo-35-839-2017, https://doi.org/10.5194/angeo-35-839-2017, 2017
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Through the selection of 172 urban–rural station pairs, this study noted that urbanization significantly influenced the dimming trend in sunshine duration in China from 1960 until it leveled off after 1990. During 1960–1989, rural dimming was around two-thirds the rate of urban dimming; this ratio generally shows a positive correlation with urbanization level. There may be an overestimation of dimming in China when a dataset with more urban-scale sites than rural-scale sites is applied.
Wei Du, Jian Zhao, Yuying Wang, Yingjie Zhang, Qingqing Wang, Weiqi Xu, Chen Chen, Tingting Han, Fang Zhang, Zhanqing Li, Pingqing Fu, Jie Li, Zifa Wang, and Yele Sun
Atmos. Chem. Phys., 17, 6797–6811, https://doi.org/10.5194/acp-17-6797-2017, https://doi.org/10.5194/acp-17-6797-2017, 2017
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We conducted the first simultaneous measurements of size-resolved particle number concentrations at ground level and 260 m in urban Beijing. The vertical differences strongly depend on particle sizes, with accumulation-mode particles being highly correlated at the two heights. We further demonstrated that regional emission controls have a dominant impact on accumulation-mode particles, while the influences on Aitken particles were much smaller due to the enhanced NPF events.
Yuying Wang, Fang Zhang, Zhanqing Li, Haobo Tan, Hanbing Xu, Jingye Ren, Jian Zhao, Wei Du, and Yele Sun
Atmos. Chem. Phys., 17, 5239–5251, https://doi.org/10.5194/acp-17-5239-2017, https://doi.org/10.5194/acp-17-5239-2017, 2017
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A series of strict emission control measures were implemented in Beijing and the surrounding seven provinces to ensure good air quality during the 2015 China Victory Day parade, rendering a unique opportunity to investigate anthropogenic impact of aerosol properties. Submicron aerosol hygroscopicity and volatility were measured during and after the control period. By comparison we found aerosol particles became more hydrophobic and volatile due to the emission control measures.
Katsumasa Tanaka, Atsumu Ohmura, Doris Folini, Martin Wild, and Nozomu Ohkawara
Atmos. Chem. Phys., 16, 13969–14001, https://doi.org/10.5194/acp-16-13969-2016, https://doi.org/10.5194/acp-16-13969-2016, 2016
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Surface solar radiation observed in Japan generally shows a strong decline until the end of the 1980s and then a recovery up until around 2000. A substantial number of measurement stations are located close to populated areas and are speculated to have been influenced by air pollution. However, data obtained at 14 meteorological observatories suggest that the large decadal variations in surface solar radiation occur on a large scale and not limited to urban areas.
Veronica Manara, Michele Brunetti, Angela Celozzi, Maurizio Maugeri, Arturo Sanchez-Lorenzo, and Martin Wild
Atmos. Chem. Phys., 16, 11145–11161, https://doi.org/10.5194/acp-16-11145-2016, https://doi.org/10.5194/acp-16-11145-2016, 2016
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This paper presents the temporal evolution of solar radiation over Italy for the 1959–2013 period and discusses possible reasons for differences between all-sky and clear-sky conditions in order to understand which part of the solar radiation variability depends on aerosols or clouds. The results give evidence of a relevant influence of both anthropogenic and natural aerosols on solar radiation long-term variability.
Yawen Wang, Martin Wild, Arturo Sanchez-Lorenzo, Yonghui Yang, Veronica Manara, and Dandan Ren
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-657, https://doi.org/10.5194/acp-2016-657, 2016
Revised manuscript not accepted
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The strong decadal variations in surface solar radiation, known as "global dimming and brightening", are considered to be related to anthropogenic activities. Based on a comprehensive set of sunshine duration measurements in China, the present study investigates to what extent these changes occurred, only in cities or also in remote areas. The quantification of this "urbanization effect" enables a more accurate determination of the large scale variations of surface solar radiation over China.
Josiane Mélançon, Maurice Levasseur, Martine Lizotte, Michael Scarratt, Jean-Éric Tremblay, Philippe Tortell, Gui-Peng Yang, Guang-Yu Shi, Huiwang Gao, David Semeniuk, Marie Robert, Michael Arychuk, Keith Johnson, Nes Sutherland, Marty Davelaar, Nina Nemcek, Angelica Peña, and Wendy Richardson
Biogeosciences, 13, 1677–1692, https://doi.org/10.5194/bg-13-1677-2016, https://doi.org/10.5194/bg-13-1677-2016, 2016
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Ocean acidification is likely to affect iron-limited phytoplankton fertilization by desert dust. Short incubations of northeast subarctic Pacific waters enriched with dust and set at pH 8.0 and 7.8 were conducted. Acidification led to a significant reduction (by 16–38 %) of the final concentration of chl a reached after enrichment. These results show that dust deposition events in a low-pH iron-limited ocean are likely to stimulate phytoplankton growth to a lesser extent than in today's ocean.
Adel Imamovic, Katsumasa Tanaka, Doris Folini, and Martin Wild
Atmos. Chem. Phys., 16, 2719–2725, https://doi.org/10.5194/acp-16-2719-2016, https://doi.org/10.5194/acp-16-2719-2016, 2016
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Systematic measurements of surface solar radiation revealed a worldwide decrease from the 1960s to the mid-1980s. The role of urbanization for this so called global dimming is still under debate. We developed a set of population-data based urbanization indicators and found no correlation between urbanization and global dimming for Europe and Japan, while an urbanization impact can't be precluded for Asia. It is thus called into question whether the global dimming was mainly a local phenomenon.
A. I. Stegehuis, R. Vautard, P. Ciais, A. J. Teuling, D. G. Miralles, and M. Wild
Geosci. Model Dev., 8, 2285–2298, https://doi.org/10.5194/gmd-8-2285-2015, https://doi.org/10.5194/gmd-8-2285-2015, 2015
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Many climate models have difficulties in properly reproducing climate extremes such as heat wave conditions. We use a regional climate model with different atmospheric physics schemes to simulate the heat wave events of 2003 in western Europe and 2010 in Russia. The five best-performing and diverse physics scheme combinations may be used in the future to perform heat wave analysis and to investigate the impact of climate change in summer in Europe.
S. Fuzzi, U. Baltensperger, K. Carslaw, S. Decesari, H. Denier van der Gon, M. C. Facchini, D. Fowler, I. Koren, B. Langford, U. Lohmann, E. Nemitz, S. Pandis, I. Riipinen, Y. Rudich, M. Schaap, J. G. Slowik, D. V. Spracklen, E. Vignati, M. Wild, M. Williams, and S. Gilardoni
Atmos. Chem. Phys., 15, 8217–8299, https://doi.org/10.5194/acp-15-8217-2015, https://doi.org/10.5194/acp-15-8217-2015, 2015
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Particulate matter (PM) constitutes one of the most challenging problems both for air quality and climate change policies. This paper reviews the most recent scientific results on the issue and the policy needs that have driven much of the increase in monitoring and mechanistic research over the last 2 decades. The synthesis reveals many new processes and developments in the science underpinning climate-PM interactions and the effects of PM on human health and the environment.
Z. Wang, D. Liu, Y. Wang, Z. Wang, and G. Shi
Atmos. Meas. Tech., 8, 2901–2907, https://doi.org/10.5194/amt-8-2901-2015, https://doi.org/10.5194/amt-8-2901-2015, 2015
H. Che, X.-Y. Zhang, X. Xia, P. Goloub, B. Holben, H. Zhao, Y. Wang, X.-C. Zhang, H. Wang, L. Blarel, B. Damiri, R. Zhang, X. Deng, Y. Ma, T. Wang, F. Geng, B. Qi, J. Zhu, J. Yu, Q. Chen, and G. Shi
Atmos. Chem. Phys., 15, 7619–7652, https://doi.org/10.5194/acp-15-7619-2015, https://doi.org/10.5194/acp-15-7619-2015, 2015
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This work studied more than 10 years of measurements of aerosol optical depths (AODs) made for 50 sites of CARSNET compiled into a climatology of aerosol optical properties for China. It lets us see a detailed full-scale description of AOD observations over China. The results would benefit us a lot in comprehending the temporal and special distribution aerosol optical property over China. Also the data would be valuable to communities of aerosol satellite retrieval, modelling, etc.
Z. L. Wang, H. Zhang, and X. Y. Zhang
Atmos. Chem. Phys., 15, 3671–3685, https://doi.org/10.5194/acp-15-3671-2015, https://doi.org/10.5194/acp-15-3671-2015, 2015
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This study highlights that there are no effective ways to remove the black carbon exclusively without influencing the other co-emitted components, our results therefore indicate that a reduction in BC emission can lead to an unexpected warming on the Earth’s climate system in the future.
H. Wang, G. Y. Shi, X. Y. Zhang, S. L. Gong, S. C. Tan, B. Chen, H. Z. Che, and T. Li
Atmos. Chem. Phys., 15, 3277–3287, https://doi.org/10.5194/acp-15-3277-2015, https://doi.org/10.5194/acp-15-3277-2015, 2015
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Solar radiation reaching the ground decreases about 15% in Chinese 3JNS region and by 20 to 25% in the region with the highest AOD. Aerosol cools the PBL atmosphere but warms the atmosphere above it, leading to a more stable atmosphere that causes a decrease in turbulence diffusion of about 52% and in PBL height of about 33%; this results in a positive feedback on the PM2.5 concentration within the PBL and the surface as well as the haze formation.
K. Tsigaridis, N. Daskalakis, M. Kanakidou, P. J. Adams, P. Artaxo, R. Bahadur, Y. Balkanski, S. E. Bauer, N. Bellouin, A. Benedetti, T. Bergman, T. K. Berntsen, J. P. Beukes, H. Bian, K. S. Carslaw, M. Chin, G. Curci, T. Diehl, R. C. Easter, S. J. Ghan, S. L. Gong, A. Hodzic, C. R. Hoyle, T. Iversen, S. Jathar, J. L. Jimenez, J. W. Kaiser, A. Kirkevåg, D. Koch, H. Kokkola, Y. H Lee, G. Lin, X. Liu, G. Luo, X. Ma, G. W. Mann, N. Mihalopoulos, J.-J. Morcrette, J.-F. Müller, G. Myhre, S. Myriokefalitakis, N. L. Ng, D. O'Donnell, J. E. Penner, L. Pozzoli, K. J. Pringle, L. M. Russell, M. Schulz, J. Sciare, Ø. Seland, D. T. Shindell, S. Sillman, R. B. Skeie, D. Spracklen, T. Stavrakou, S. D. Steenrod, T. Takemura, P. Tiitta, S. Tilmes, H. Tost, T. van Noije, P. G. van Zyl, K. von Salzen, F. Yu, Z. Wang, Z. Wang, R. A. Zaveri, H. Zhang, K. Zhang, Q. Zhang, and X. Zhang
Atmos. Chem. Phys., 14, 10845–10895, https://doi.org/10.5194/acp-14-10845-2014, https://doi.org/10.5194/acp-14-10845-2014, 2014
M. Calisto, D. Folini, M. Wild, and L. Bengtsson
Ann. Geophys., 32, 793–807, https://doi.org/10.5194/angeo-32-793-2014, https://doi.org/10.5194/angeo-32-793-2014, 2014
J. Huttunen, A. Arola, G. Myhre, A. V. Lindfors, T. Mielonen, S. Mikkonen, J. S. Schafer, S. N. Tripathi, M. Wild, M. Komppula, and K. E. J. Lehtinen
Atmos. Chem. Phys., 14, 6103–6110, https://doi.org/10.5194/acp-14-6103-2014, https://doi.org/10.5194/acp-14-6103-2014, 2014
T. Stavrakou, J.-F. Müller, M. Bauwens, I. De Smedt, M. Van Roozendael, A. Guenther, M. Wild, and X. Xia
Atmos. Chem. Phys., 14, 4587–4605, https://doi.org/10.5194/acp-14-4587-2014, https://doi.org/10.5194/acp-14-4587-2014, 2014
H. Zhang, X. Jing, and J. Li
Geosci. Model Dev., 7, 737–754, https://doi.org/10.5194/gmd-7-737-2014, https://doi.org/10.5194/gmd-7-737-2014, 2014
H. Che, X. Xia, J. Zhu, Z. Li, O. Dubovik, B. Holben, P. Goloub, H. Chen, V. Estelles, E. Cuevas-Agulló, L. Blarel, H. Wang, H. Zhao, X. Zhang, Y. Wang, J. Sun, R. Tao, X. Zhang, and G. Shi
Atmos. Chem. Phys., 14, 2125–2138, https://doi.org/10.5194/acp-14-2125-2014, https://doi.org/10.5194/acp-14-2125-2014, 2014
N. Schaller, J. Cermak, M. Wild, and R. Knutti
Earth Syst. Dynam., 4, 253–266, https://doi.org/10.5194/esd-4-253-2013, https://doi.org/10.5194/esd-4-253-2013, 2013
C. A. Randles, S. Kinne, G. Myhre, M. Schulz, P. Stier, J. Fischer, L. Doppler, E. Highwood, C. Ryder, B. Harris, J. Huttunen, Y. Ma, R. T. Pinker, B. Mayer, D. Neubauer, R. Hitzenberger, L. Oreopoulos, D. Lee, G. Pitari, G. Di Genova, J. Quaas, F. G. Rose, S. Kato, S. T. Rumbold, I. Vardavas, N. Hatzianastassiou, C. Matsoukas, H. Yu, F. Zhang, H. Zhang, and P. Lu
Atmos. Chem. Phys., 13, 2347–2379, https://doi.org/10.5194/acp-13-2347-2013, https://doi.org/10.5194/acp-13-2347-2013, 2013
Related subject area
Subject: Radiation | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
First reported detection of a winter continental gamma-ray glow in Europe
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Tethered balloon-borne observations of thermal-infrared irradiance and cooling rate profiles in the Arctic atmospheric boundary layer
Assessing the cloud radiative bias at Macquarie Island in the ACCESS-AM2 model
Surface energy balance fluxes in a suburban area of Beijing: energy partitioning variability
Effects of variable ice–ocean surface properties and air mass transformation on the Arctic radiative energy budget
Airborne observations of the surface cloud radiative effect during different seasons over sea ice and open ocean in the Fram Strait
Assessment of spectral UV radiation at Marambio Base, Antarctic Peninsula
Parameterization of downward long-wave radiation based on long-term baseline surface radiation measurements in China
Ozone, DNA-active UV radiation, and cloud changes for the near-global mean and at high latitudes due to enhanced greenhouse gas concentrations
In situ observation of warm atmospheric layer and the heat contribution of suspended dust over the Tarim Basin
Eight-year variations in atmospheric radiocesium in Fukushima city
Variability and trends in surface solar spectral ultraviolet irradiance in Italy: on the influence of geopotential height and lower-stratospheric ozone
Fifty-six years of surface solar radiation and sunshine duration over São Paulo, Brazil: 1961–2016
Changes in the surface broadband shortwave radiation budget during the 2017 eclipse
Reassessment of shortwave surface cloud radiative forcing in the Arctic: consideration of surface-albedo–cloud interactions
Deposition of brown carbon onto snow: changes in snow optical and radiative properties
Solar UV radiation measurements in Marambio, Antarctica, during years 2017–2019
A revisiting of the parametrization of downward longwave radiation in summer over the Tibetan Plateau based on high-temporal-resolution measurements
Trends in surface radiation and cloud radiative effect at four Swiss sites for the 1996–2015 period
Can downwelling far-infrared radiances over Antarctica be estimated from mid-infrared information?
Measurements of spectral irradiance during the solar eclipse of 21 August 2017: reassessment of the effect of solar limb darkening and of changes in total ozone
UV measurements at Marambio and Ushuaia during 2000–2010
On the suitability of current atmospheric reanalyses for regional warming studies over China
A long-term time series of global and diffuse photosynthetically active radiation in the Mediterranean: interannual variability and cloud effects
Long-term series and trends in surface solar radiation in Athens, Greece
Reconstruction and analysis of erythemal UV radiation time series from Hradec Králové (Czech Republic) over the past 50 years
Trends in erythemal doses at the Polish Polar Station, Hornsund, Svalbard based on the homogenized measurements (1996–2016) and reconstructed data (1983–1995)
Effects of vernal equinox solar eclipse on temperature and wind direction in Switzerland
Sky radiance at a coastline and effects of land and ocean reflectivities
Impact of aerosols and clouds on decadal trends in all-sky solar radiation over the Netherlands (1966–2015)
Contributions of surface solar radiation and precipitation to the spatiotemporal patterns of surface and air warming in China from 1960 to 2003
Multiresolution analysis of the spatiotemporal variability in global radiation observed by a dense network of 99 pyranometers
Validation of satellite-based noontime UVI with NDACC ground-based instruments: influence of topography, environment and satellite overpass time
Is global dimming and brightening in Japan limited to urban areas?
The climatology of planetary boundary layer height in China derived from radiosonde and reanalysis data
Detection of dimming/brightening in Italy from homogenized all-sky and clear-sky surface solar radiation records and underlying causes (1959–2013)
Comparison of land–atmosphere interaction at different surface types in the mid- to lower reaches of the Yangtze River valley
Spectral optical layer properties of cirrus from collocated airborne measurements and simulations
Local short-term variability in solar irradiance
The contrasting roles of water and dust in controlling daily variations in radiative heating of the summertime Saharan heat low
Global dimming and urbanization: did stronger negative SSR trends collocate with regions of population growth?
Short- and long-term variability of spectral solar UV irradiance at Thessaloniki, Greece: effects of changes in aerosols, total ozone and clouds
On the progress of the 2015–2016 El Niño event
Role of radiatively forced temperature changes in enhanced semi-arid warming in the cold season over east Asia
Assessment of long-term WRF–CMAQ simulations for understanding direct aerosol effects on radiation "brightening" in the United States
Comparison of OMI UV observations with ground-based measurements at high northern latitudes
Characterisation of J(O1D) at Cape Grim 2000–2005
On the scaling of the solar incident flux
Analysis of actinic flux profiles measured from an ozonesonde balloon
Jakub Šlegl, Zbyněk Sokol, Petr Pešice, Ronald Langer, Igor Strhárský, Jana Popová, Martin Kákona, Iva Ambrožová, and Ondřej Ploc
Atmos. Chem. Phys., 25, 8443–8454, https://doi.org/10.5194/acp-25-8443-2025, https://doi.org/10.5194/acp-25-8443-2025, 2025
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We present the first-ever reported gamma-ray glows from a winter thunderstorm in continental Europe. Although two glows were detected at the same time, only one was ended by a discharge. Using advanced instruments such as the Ka-band vertically oriented Doppler radar and SEVAN detector, we gained new insights into the inner thunderstorm processes even in a cloud only 3 km in height.
Kristopher Scarci, Ryan C. Scott, Madison L. Ghiz, Andrew M. Vogelmann, and Dan Lubin
Atmos. Chem. Phys., 24, 6681–6697, https://doi.org/10.5194/acp-24-6681-2024, https://doi.org/10.5194/acp-24-6681-2024, 2024
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We demonstrate what can be learned about an Antarctic region's climate from basic atmospheric irradiance measurements made by broadband and filter radiometers, instruments suitable for deployment at very remote sites, assisted by meteorological reanalysis and satellite remote sensing. Analysis of shortwave and longwave irradiance reveals subtle contrasts between meteorological regimes favoring cloud ice versus liquid water, relevant to onset versus inhibition of surface melt over ice shelves.
Michael Lonardi, Elisa F. Akansu, André Ehrlich, Mauro Mazzola, Christian Pilz, Matthew D. Shupe, Holger Siebert, and Manfred Wendisch
Atmos. Chem. Phys., 24, 1961–1978, https://doi.org/10.5194/acp-24-1961-2024, https://doi.org/10.5194/acp-24-1961-2024, 2024
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Profiles of thermal-infrared irradiance were measured at two Arctic sites. The presence or lack of clouds influences the vertical structure of these observations. In particular, the cloud top region is a source of radiative energy that can promote cooling and mixing in the cloud layer. Simulations are used to further characterize how the amount of water in the cloud modifies this forcing. A case study additionally showcases the evolution of the radiation profiles in a dynamic atmosphere.
Zhangcheng Pei, Sonya L. Fiddes, W. John R. French, Simon P. Alexander, Marc D. Mallet, Peter Kuma, and Adrian McDonald
Atmos. Chem. Phys., 23, 14691–14714, https://doi.org/10.5194/acp-23-14691-2023, https://doi.org/10.5194/acp-23-14691-2023, 2023
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In this paper, we use ground-based observations to evaluate a climate model and a satellite product in simulating surface radiation and investigate how radiation biases are influenced by cloud properties over the Southern Ocean. We find that significant radiation biases exist in both the model and satellite. The cloud fraction and cloud occurrence play an important role in affecting radiation biases. We suggest further development for the model and satellite using ground-based observations.
Junxia Dou, Sue Grimmond, Shiguang Miao, Bei Huang, Huimin Lei, and Mingshui Liao
Atmos. Chem. Phys., 23, 13143–13166, https://doi.org/10.5194/acp-23-13143-2023, https://doi.org/10.5194/acp-23-13143-2023, 2023
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Multi-timescale variations in surface energy fluxes in a suburb of Beijing are analyzed using 16-month observations. Compared to previous suburban areas, this study site has larger seasonal variability in energy partitioning, and summer and winter Bowen ratios are at the lower and higher end of those at other suburban sites, respectively. Our analysis indicates that precipitation, irrigation, crop/vegetation growth activity, and land use/cover all play critical roles in energy partitioning.
Manfred Wendisch, Johannes Stapf, Sebastian Becker, André Ehrlich, Evelyn Jäkel, Marcus Klingebiel, Christof Lüpkes, Michael Schäfer, and Matthew D. Shupe
Atmos. Chem. Phys., 23, 9647–9667, https://doi.org/10.5194/acp-23-9647-2023, https://doi.org/10.5194/acp-23-9647-2023, 2023
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Atmospheric radiation measurements have been conducted during two field campaigns using research aircraft. The data are analyzed to see if the near-surface air in the Arctic is warmed or cooled if warm–humid air masses from the south enter the Arctic or cold–dry air moves from the north from the Arctic to mid-latitude areas. It is important to study these processes and to check if climate models represent them well. Otherwise it is not possible to reliably forecast the future Arctic climate.
Sebastian Becker, André Ehrlich, Michael Schäfer, and Manfred Wendisch
Atmos. Chem. Phys., 23, 7015–7031, https://doi.org/10.5194/acp-23-7015-2023, https://doi.org/10.5194/acp-23-7015-2023, 2023
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This study analyses the variability of the warming or cooling effect of clouds on the Arctic surface. Therefore, aircraft radiation measurements were performed over sea ice and open ocean during three seasonally different campaigns. It is found that clouds cool the open-ocean surface most strongly in summer. Over sea ice, clouds warm the surface in spring but have a neutral effect in summer. Due to the variable sea ice extent, clouds warm the surface during spring but cool it during late summer.
Klára Čížková, Kamil Láska, Ladislav Metelka, and Martin Staněk
Atmos. Chem. Phys., 23, 4617–4636, https://doi.org/10.5194/acp-23-4617-2023, https://doi.org/10.5194/acp-23-4617-2023, 2023
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The study deals with ultraviolet (UV) radiation in southern polar conditions, where ozone depletion occurs each spring. A 10-year-long time series of UV spectra from Marambio Base, Antarctic Peninsula, has been studied, with a focus on the changes of UV radiation at different wavelengths and the effects of atmospheric and terrestrial variables like ozone, solar elevation, or cloudiness. At the very short wavelengths, the effect of ozone and its deficiency was clearly observed.
Junli Yang, Jianglin Hu, Qiying Chen, and Weijun Quan
Atmos. Chem. Phys., 23, 4419–4430, https://doi.org/10.5194/acp-23-4419-2023, https://doi.org/10.5194/acp-23-4419-2023, 2023
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Downward long-wave radiation (DLR) affects energy exchange between the land surface and the atmosphere, while it is seldom observed at conventional radiation stations. Therefore, parameterization of DLR based on the near-surface meteorological variables provides a chance to estimate the DLR over most meteorological stations. This work established three parameterizations suited to estimating the DLR over China by using the measurements from the CBSRN with an accuracy of ~6.1 %.
Kostas Eleftheratos, John Kapsomenakis, Ilias Fountoulakis, Christos S. Zerefos, Patrick Jöckel, Martin Dameris, Alkiviadis F. Bais, Germar Bernhard, Dimitra Kouklaki, Kleareti Tourpali, Scott Stierle, J. Ben Liley, Colette Brogniez, Frédérique Auriol, Henri Diémoz, Stana Simic, Irina Petropavlovskikh, Kaisa Lakkala, and Kostas Douvis
Atmos. Chem. Phys., 22, 12827–12855, https://doi.org/10.5194/acp-22-12827-2022, https://doi.org/10.5194/acp-22-12827-2022, 2022
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We present the future evolution of DNA-active ultraviolet (UV) radiation in view of increasing greenhouse gases (GHGs) and decreasing ozone depleting substances (ODSs). It is shown that DNA-active UV radiation might increase after 2050 between 50° N–50° S due to GHG-induced reductions in clouds and ozone, something that is likely not to happen at high latitudes, where DNA-active UV radiation will continue its downward trend mainly due to stratospheric ozone recovery from the reduction in ODSs.
Chenglong Zhou, Yuzhi Liu, Qingzhe Zhu, Qing He, Tianliang Zhao, Fan Yang, Wen Huo, Xinghua Yang, and Ali Mamtimin
Atmos. Chem. Phys., 22, 5195–5207, https://doi.org/10.5194/acp-22-5195-2022, https://doi.org/10.5194/acp-22-5195-2022, 2022
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Based on the radiosonde observations, an anomalously warm layer is measured at altitudes between 500 and 300 hPa over the Tarim Basin (TB) with an average intensity of 2.53 and 1.39 K in the spring and summer, respectively. The heat contributions of dust to this anomalously warm atmospheric layer in spring and summer were 13.77 and 10.25 %, respectively. Topographically, the TB is adjacent to the Tibetan Plateau; we propose the concept of the Tibetan heat source’s northward extension.
Akira Watanabe, Mizuo Kajino, Kazuhiko Ninomiya, Yoshitaka Nagahashi, and Atsushi Shinohara
Atmos. Chem. Phys., 22, 675–692, https://doi.org/10.5194/acp-22-675-2022, https://doi.org/10.5194/acp-22-675-2022, 2022
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This study summarizes continuous measurements of surface air concentrations and deposition of radiocesium in Fukushima city over 8 years after the Fukushima nuclear accident. The concentration in the city was high in winter and low in summer (inverse of the forest area). The decreasing trends were much faster in the earlier stage, probably because dissolved cesium discharged faster from the local environment. Biotite might play a key role in circulation of particulate cesium in Fukushima city.
Ilias Fountoulakis, Henri Diémoz, Anna Maria Siani, Alcide di Sarra, Daniela Meloni, and Damiano M. Sferlazzo
Atmos. Chem. Phys., 21, 18689–18705, https://doi.org/10.5194/acp-21-18689-2021, https://doi.org/10.5194/acp-21-18689-2021, 2021
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The variability and trends of solar spectral UV irradiance have been studied for the periods 1996–2020 (for Rome) and 2006–2020 (for Lampedusa, Rome, and Aosta) with respect to the variability and trends of total ozone and geopotential height. Analyses revealed increasing UV in particular months at all sites, possibly due to decreasing lower-stratospheric ozone (at Rome in 1996–2020) and decreasing attenuation by aerosols and/or clouds (at all stations in 2006–2020).
Marcia Akemi Yamasoe, Nilton Manuel Évora Rosário, Samantha Novaes Santos Martins Almeida, and Martin Wild
Atmos. Chem. Phys., 21, 6593–6603, https://doi.org/10.5194/acp-21-6593-2021, https://doi.org/10.5194/acp-21-6593-2021, 2021
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Spatio-temporal disparity to assess global dimming and brightening phenomena has been a critical topic. For instance, few studies addressed surface solar irradiation (SSR) long-term trend in South America. In this study, SSR, sunshine duration (SD) and the diurnal temperature range (DTR) are analysed for São Paulo, Brazil. We found a dimming phase, identified by SSR, SD and DTR, extending till 1983. Then, while SSR is still declining, consistent with cloud increasing, SD and DTR are increasing.
Guoyong Wen, Alexander Marshak, Si-Chee Tsay, Jay Herman, Ukkyo Jeong, Nader Abuhassan, Robert Swap, and Dong Wu
Atmos. Chem. Phys., 20, 10477–10491, https://doi.org/10.5194/acp-20-10477-2020, https://doi.org/10.5194/acp-20-10477-2020, 2020
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We combine the ground-based observations and radiative transfer model to quantify the impact of the 2017 solar eclipse on surface shortwave irradiation reduction. We find that the eclipse caused local reductions of time-averaged surface flux of about 379 W m-2 (50 %) and 329 W m-2 (46 %) during the ~ 3 h course of the eclipse at the Casper and Columbia sites, respectively. We estimate that the Moon’s shadow caused a reduction of approximately 7 %–8 % in global average surface broadband SW radiation.
Johannes Stapf, André Ehrlich, Evelyn Jäkel, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys., 20, 9895–9914, https://doi.org/10.5194/acp-20-9895-2020, https://doi.org/10.5194/acp-20-9895-2020, 2020
Nicholas D. Beres, Deep Sengupta, Vera Samburova, Andrey Y. Khlystov, and Hans Moosmüller
Atmos. Chem. Phys., 20, 6095–6114, https://doi.org/10.5194/acp-20-6095-2020, https://doi.org/10.5194/acp-20-6095-2020, 2020
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Brown carbon (BrC) aerosol can be produced by the smoldering combustion of peat, a wildland fuel common at high latitude, often adjacent to the cryosphere. However, little is known about how BrC deposition onto snow changes snow optical and radiative properties. Here, we artificially deposited BrC onto natural snow surfaces, monitored changes of the spectral surface albedo, characterized optical properties of deposited aerosol, and compared to modeled values of albedo and radiative forcing.
Margit Aun, Kaisa Lakkala, Ricardo Sanchez, Eija Asmi, Fernando Nollas, Outi Meinander, Larisa Sogacheva, Veerle De Bock, Antti Arola, Gerrit de Leeuw, Veijo Aaltonen, David Bolsée, Klara Cizkova, Alexander Mangold, Ladislav Metelka, Erko Jakobson, Tove Svendby, Didier Gillotay, and Bert Van Opstal
Atmos. Chem. Phys., 20, 6037–6054, https://doi.org/10.5194/acp-20-6037-2020, https://doi.org/10.5194/acp-20-6037-2020, 2020
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In 2017, new measurements of UV radiation started in Marambio, Antarctica, by the Finnish Meteorological Institute in collaboration with the Argentinian Servicio Meteorológico Nacional. The paper presents the results of UV irradiance measurements from March 2017 to March 2019, and it
compares them with those from 2000–2008 and also with UV measurements at other Antarctic stations. In 2017/2018, below average UV radiation levels were recorded due to favourable ozone and cloud conditions.
Mengqi Liu, Xiangdong Zheng, Jinqiang Zhang, and Xiangao Xia
Atmos. Chem. Phys., 20, 4415–4426, https://doi.org/10.5194/acp-20-4415-2020, https://doi.org/10.5194/acp-20-4415-2020, 2020
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This study uses 1 min radiation and lidar measurements at three stations over the Tibetan Plateau (TP) to parametrize downward longwave radiation (DLR) during summer months. Clear-sky DLR can be estimated from the best parametrization with a RMSE of 3.8 W m-2 and R2 > 0.98. Additionally cloud base height under overcast conditions is shown to play an important role in cloudy DLR parametrization, which is considered in the locally calibrated parametrization over the TP for the first time.
Stephan Nyeki, Stefan Wacker, Christine Aebi, Julian Gröbner, Giovanni Martucci, and Laurent Vuilleumier
Atmos. Chem. Phys., 19, 13227–13241, https://doi.org/10.5194/acp-19-13227-2019, https://doi.org/10.5194/acp-19-13227-2019, 2019
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The trends of meteorological parameters and surface downward shortwave radiation (DSR) and downward longwave radiation (DLR) were analysed at four stations (between 370 and 3580 m a. s. l.) in Switzerland for the 1996–2015 period. Trends in DSR and DLR were positive during cloudy as well as clear conditions. The trend due to the influence of clouds decreased in magnitude, which implies a reduction in cloud cover and/or a change towards a different cloud type over the four Swiss sites.
Christophe Bellisario, Helen E. Brindley, Simon F. B. Tett, Rolando Rizzi, Gianluca Di Natale, Luca Palchetti, and Giovanni Bianchini
Atmos. Chem. Phys., 19, 7927–7937, https://doi.org/10.5194/acp-19-7927-2019, https://doi.org/10.5194/acp-19-7927-2019, 2019
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We explore the possibility of inferring far-infrared downwelling radiances from mid-infrared observations to better constrain radiation schemes in climate models. Our results imply that while it is feasible to use this type of approach, the quality of the extension will be strongly dependent on the noise characteristics of the observations and on the accurate characterisation of the atmospheric state.
Germar Bernhard and Boyan Petkov
Atmos. Chem. Phys., 19, 4703–4719, https://doi.org/10.5194/acp-19-4703-2019, https://doi.org/10.5194/acp-19-4703-2019, 2019
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Solar radiation at ultraviolet, visible, and infrared wavelengths was measured during the total solar eclipse of 21 August 2017. Data were used to study the wavelength-dependent changes of solar radiation at Earth’s surface and to validate parameterizations of solar limb darkening (LD), which describes the change in the Sun’s brightness between its center and its edge. The study highlights the importance of the LD effect when calculating total ozone and aerosol optical depth during an eclipse.
Kaisa Lakkala, Alberto Redondas, Outi Meinander, Laura Thölix, Britta Hamari, Antonio Fernando Almansa, Virgilio Carreno, Rosa Delia García, Carlos Torres, Guillermo Deferrari, Hector Ochoa, Germar Bernhard, Ricardo Sanchez, and Gerrit de Leeuw
Atmos. Chem. Phys., 18, 16019–16031, https://doi.org/10.5194/acp-18-16019-2018, https://doi.org/10.5194/acp-18-16019-2018, 2018
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Solar UV irradiances were measured at Ushuaia (54° S) and Marambio (64° S) during 2000–2013. The measurements were part of the Antarctic NILU-UV network, which was maintained as a cooperation between Spain, Argentina and Finland. The time series of the network were analysed for the first time in this study. At both stations maximum UV indices and daily doses were measured when spring-time ozone loss episodes occurred. The maximum UV index was 13 and 12 in Ushuaia and Marambio, respectively.
Chunlüe Zhou, Yanyi He, and Kaicun Wang
Atmos. Chem. Phys., 18, 8113–8136, https://doi.org/10.5194/acp-18-8113-2018, https://doi.org/10.5194/acp-18-8113-2018, 2018
Pamela Trisolino, Alcide di Sarra, Fabrizio Anello, Carlo Bommarito, Tatiana Di Iorio, Daniela Meloni, Francesco Monteleone, Giandomenico Pace, Salvatore Piacentino, and Damiano Sferlazzo
Atmos. Chem. Phys., 18, 7985–8000, https://doi.org/10.5194/acp-18-7985-2018, https://doi.org/10.5194/acp-18-7985-2018, 2018
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The long-term (2002–2016) variability of global and diffuse PAR over the central Mediterranean is investigated based on measurements from Lampedusa. PAR modulates biological processes and this study provides useful insight into its variability. Seasonal and interannual variability of global and diffuse PAR is characterized and the effects of clouds are quantified. The analysis suggests that 77 % of the global PAR interannual variability may be ascribed to clouds.
Stelios Kazadzis, Dimitra Founda, Basil E. Psiloglou, Harry Kambezidis, Nickolaos Mihalopoulos, Arturo Sanchez-Lorenzo, Charikleia Meleti, Panagiotis I. Raptis, Fragiskos Pierros, and Pierre Nabat
Atmos. Chem. Phys., 18, 2395–2411, https://doi.org/10.5194/acp-18-2395-2018, https://doi.org/10.5194/acp-18-2395-2018, 2018
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The National Observatory of Athens has been collecting solar radiation, sunshine duration, and cloud and visibility data/observations since the beginning of the 20th century. In this work we present surface solar radiation data since 1953 and reconstructed data since 1900. We have attempted to show and discuss the long-term changes in solar surface radiation over Athens, Greece, using these unique datasets.
Klára Čížková, Kamil Láska, Ladislav Metelka, and Martin Staněk
Atmos. Chem. Phys., 18, 1805–1818, https://doi.org/10.5194/acp-18-1805-2018, https://doi.org/10.5194/acp-18-1805-2018, 2018
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In order to broaden the knowledge of long-term UV radiation variability, we have reconstructed and analyzed a 50-year-long UV radiation time series from Hradec Králové, Czech Republic. The UV radiation intensities increased greatly following the decline of ozone amounts in the 1980s and 1990s. High UV radiation doses were observed in days with low ozone amounts, clear or partly cloudy skies, or snow cover.
Janusz W. Krzyścin and Piotr S. Sobolewski
Atmos. Chem. Phys., 18, 1–11, https://doi.org/10.5194/acp-18-1-2018, https://doi.org/10.5194/acp-18-1-2018, 2018
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Maintaining homogeneity of long-term UV time series taken from various instruments and thus trend estimation are challenging tasks, especially for remote Arctic sites.
Highlights: method of the UV data homogenization is proposed to be used at any remote site. Past UV data built from satellite total O3 and ground-based sunshine duration. Yearly UV doses trendless in the southern Svalbard for 34-year period since 1983. Long-term cloud effects on UV more important than the ozone effects there.
Werner Eugster, Carmen Emmel, Sebastian Wolf, Nina Buchmann, Joseph P. McFadden, and Charles David Whiteman
Atmos. Chem. Phys., 17, 14887–14904, https://doi.org/10.5194/acp-17-14887-2017, https://doi.org/10.5194/acp-17-14887-2017, 2017
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The effects of penumbral shading of the solar eclipse of 20 March 2015 on near-surface meteorology across Switzerland (occultation 65.8–70.1 %) was investigated. Temperature effects at 184 weather stations are compared with temperature drops reported in the literature since 1834. A special focus is, however, put on wind direction effects observed at six flux sites (with 20 Hz data) and 165 meteorological stations (with 10 min resolution data). Results show the importance of local topography.
Axel Kreuter, Mario Blumthaler, Martin Tiefengraber, Richard Kift, and Ann R. Webb
Atmos. Chem. Phys., 17, 14353–14364, https://doi.org/10.5194/acp-17-14353-2017, https://doi.org/10.5194/acp-17-14353-2017, 2017
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We have done measurements of the sky's brightness at the Italian coast and show the influence of the underlying surface: looking towards the land, the sky can be up to 50 % brighter than opposite viewing directions towards the ocean as a result of higher land reflectivity. At low solar elevations, the specular reflection from the ocean, or sun glint, increases the zenith brightness. Understanding these effects requires a 3-D model and is important when retrieving, e.g., aerosol properties.
Reinout Boers, Theo Brandsma, and A. Pier Siebesma
Atmos. Chem. Phys., 17, 8081–8100, https://doi.org/10.5194/acp-17-8081-2017, https://doi.org/10.5194/acp-17-8081-2017, 2017
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In the Netherlands 9 W m−2 more solar radiation falls on the surface today than 50 years ago. Often this increase, which has also been detected in surrounding western Europe, has been attributed to decreasing air pollution due to improved regulatory practices. However, over the Netherlands clouds play an important but ambiguous role. Cloud cover has increased but have become optically thinner as well. Here, the impact of clouds on radiation is in fact more important than that of air pollution.
Jizeng Du, Kaicun Wang, Jiankai Wang, and Qian Ma
Atmos. Chem. Phys., 17, 4931–4944, https://doi.org/10.5194/acp-17-4931-2017, https://doi.org/10.5194/acp-17-4931-2017, 2017
Bomidi Lakshmi Madhavan, Hartwig Deneke, Jonas Witthuhn, and Andreas Macke
Atmos. Chem. Phys., 17, 3317–3338, https://doi.org/10.5194/acp-17-3317-2017, https://doi.org/10.5194/acp-17-3317-2017, 2017
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A method has been introduced to assess the representativeness of the time series of a point measurement compared to results for a larger area centered around the measurement location. This method allows one to determine the optimal accuracy that can be achieved for the validation of satellite products for a given pixel footprint, or the evaluation of an atmospheric model with a given grid-cell resolution.
Colette Brogniez, Frédérique Auriol, Christine Deroo, Antti Arola, Jukka Kujanpää, Béatrice Sauvage, Niilo Kalakoski, Mikko Riku Aleksi Pitkänen, Maxime Catalfamo, Jean-Marc Metzger, Guy Tournois, and Pierre Da Conceicao
Atmos. Chem. Phys., 16, 15049–15074, https://doi.org/10.5194/acp-16-15049-2016, https://doi.org/10.5194/acp-16-15049-2016, 2016
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The atmospheric ozone layer is changing, thus the UV radiation at the surface is changing. Due to both beneficial and adverse effects of UV on the biosphere, monitoring of UV is essential. Satellite sensors provide estimates of UV at the surface with a global coverage. Validation of satellite-sensor UV is therefore needed and this can be done by comparison with ground-based measurements. The present validation in three sites (midlatitude, tropical) shows that OMI and GOME-2 provide reliable UV.
Katsumasa Tanaka, Atsumu Ohmura, Doris Folini, Martin Wild, and Nozomu Ohkawara
Atmos. Chem. Phys., 16, 13969–14001, https://doi.org/10.5194/acp-16-13969-2016, https://doi.org/10.5194/acp-16-13969-2016, 2016
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Surface solar radiation observed in Japan generally shows a strong decline until the end of the 1980s and then a recovery up until around 2000. A substantial number of measurement stations are located close to populated areas and are speculated to have been influenced by air pollution. However, data obtained at 14 meteorological observatories suggest that the large decadal variations in surface solar radiation occur on a large scale and not limited to urban areas.
Jianping Guo, Yucong Miao, Yong Zhang, Huan Liu, Zhanqing Li, Wanchun Zhang, Jing He, Mengyun Lou, Yan Yan, Lingen Bian, and Panmao Zhai
Atmos. Chem. Phys., 16, 13309–13319, https://doi.org/10.5194/acp-16-13309-2016, https://doi.org/10.5194/acp-16-13309-2016, 2016
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The large-scale PBL climatology from sounding observations is still lacking in China. This work investigated the BLH characterization at diurnal, monthly and seasonal timescales throughout China, showing large geographic and meteorological dependences. BLH is, on average, negatively (positively) associated with the surface pressure and lower tropospheric stability (wind speed and temperature). Cloud tends to suppress the development of the PBL, which has implications for air quality forecasts.
Veronica Manara, Michele Brunetti, Angela Celozzi, Maurizio Maugeri, Arturo Sanchez-Lorenzo, and Martin Wild
Atmos. Chem. Phys., 16, 11145–11161, https://doi.org/10.5194/acp-16-11145-2016, https://doi.org/10.5194/acp-16-11145-2016, 2016
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This paper presents the temporal evolution of solar radiation over Italy for the 1959–2013 period and discusses possible reasons for differences between all-sky and clear-sky conditions in order to understand which part of the solar radiation variability depends on aerosols or clouds. The results give evidence of a relevant influence of both anthropogenic and natural aerosols on solar radiation long-term variability.
Weidong Guo, Xueqian Wang, Jianning Sun, Aijun Ding, and Jun Zou
Atmos. Chem. Phys., 16, 9875–9890, https://doi.org/10.5194/acp-16-9875-2016, https://doi.org/10.5194/acp-16-9875-2016, 2016
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Basic characteristics of land–atmosphere interactions at four neighboring sites with different underlying surfaces in southern China, a typical monsoon region, are analyzed systematically. Despite the same climate background, the differences in land surface characteristics like albedo and aerodynamic roughness length due to land use/cover change exert distinct influences on the surface radiative budget and energy allocation and result in differences of near-surface micrometeorological elements.
Fanny Finger, Frank Werner, Marcus Klingebiel, André Ehrlich, Evelyn Jäkel, Matthias Voigt, Stephan Borrmann, Peter Spichtinger, and Manfred Wendisch
Atmos. Chem. Phys., 16, 7681–7693, https://doi.org/10.5194/acp-16-7681-2016, https://doi.org/10.5194/acp-16-7681-2016, 2016
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Solar spectra of optical layer properties of cirrus have been derived from the first truly collocated airborne radiation measurements using an aircraft and a towed sensor platform. The measured layer properties differ slightly due to horizontal cirrus inhomogeneities and the influence of low-level water clouds. Applying a 1-D radiative transfer model sensitivity studies were performed. It was found that if a low-level cloud is not considered, the solar cooling of the cirrus is strongly overestimated.
Gerald M. Lohmann, Adam H. Monahan, and Detlev Heinemann
Atmos. Chem. Phys., 16, 6365–6379, https://doi.org/10.5194/acp-16-6365-2016, https://doi.org/10.5194/acp-16-6365-2016, 2016
Short summary
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Increasing numbers of photovoltaic (PV) power systems call for the characterization of irradiance variability with very high spatiotemporal resolution. We use 1 Hz irradiance data recorded by as many as 99 pyranometers and show mixed sky conditions to differ substantially from clear and overcast skies. For example, the probabilities of strong fluctuations and their respective spatial autocorrelation structures are appreciably distinct under mixed conditions.
John H. Marsham, Douglas J. Parker, Martin C. Todd, Jamie R. Banks, Helen E. Brindley, Luis Garcia-Carreras, Alexander J. Roberts, and Claire L. Ryder
Atmos. Chem. Phys., 16, 3563–3575, https://doi.org/10.5194/acp-16-3563-2016, https://doi.org/10.5194/acp-16-3563-2016, 2016
Short summary
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The roles of water, clouds and airborne dust in controlling the heating of the Sahara are uncertain, which has major implications for the West African monsoon. Observations from the Fennec project, with satellite data, show that total atmospheric water content provides a far stronger control on total radiative heating than dust does, but dust provides the stronger control on surface heating. Therefore major heating errors in global models are likely due to known errors in water transport.
Adel Imamovic, Katsumasa Tanaka, Doris Folini, and Martin Wild
Atmos. Chem. Phys., 16, 2719–2725, https://doi.org/10.5194/acp-16-2719-2016, https://doi.org/10.5194/acp-16-2719-2016, 2016
Short summary
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Systematic measurements of surface solar radiation revealed a worldwide decrease from the 1960s to the mid-1980s. The role of urbanization for this so called global dimming is still under debate. We developed a set of population-data based urbanization indicators and found no correlation between urbanization and global dimming for Europe and Japan, while an urbanization impact can't be precluded for Asia. It is thus called into question whether the global dimming was mainly a local phenomenon.
Ilias Fountoulakis, Alkiviadis F. Bais, Konstantinos Fragkos, Charickleia Meleti, Kleareti Tourpali, and Melina Maria Zempila
Atmos. Chem. Phys., 16, 2493–2505, https://doi.org/10.5194/acp-16-2493-2016, https://doi.org/10.5194/acp-16-2493-2016, 2016
Short summary
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Short- and long-term variability of spectral UV irradiance at Thessaloniki, Greece, is discussed in association with changes in total ozone column, aerosols and cloudiness. The UV data set from two Brewer spectrophotometers is used for the analysis. For the entire period 1994–2014, positive, statistically significant increases of UV irradiance were found, mainly attributable to changes in aerosols. UV irradiance is mainly increased from 1994 to 2006 and remains relatively stable thereafter.
Costas A. Varotsos, Chris G. Tzanis, and Nicholas V. Sarlis
Atmos. Chem. Phys., 16, 2007–2011, https://doi.org/10.5194/acp-16-2007-2016, https://doi.org/10.5194/acp-16-2007-2016, 2016
Short summary
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It has been recently reported that the current 2015–2016 El Niño could become "one of the strongest on record". To further explore this claim, we performed a new analysis that allows the detection of precursory signals of the strong El Niño events by using a recently developed non-linear dynamics tool. The analysis of the SOI time series shows that the 2015–2016 El Niño would be rather a "moderate to strong" or even a "strong” event and not "one of the strongest on record", as that of 1997–1998.
X. Guan, J. Huang, R. Guo, H. Yu, P. Lin, and Y. Zhang
Atmos. Chem. Phys., 15, 13777–13786, https://doi.org/10.5194/acp-15-13777-2015, https://doi.org/10.5194/acp-15-13777-2015, 2015
Short summary
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Dynamical adjustment methodology has been applied to the raw surface air temperature and has successfully identified and separated the contribution of dynamically induced temperature (DIT) and radiatively forced temperature (RFT). It found that regional anthropogenic radiative forcing caused the enhanced warming in the semi-arid region, which may be closely associated with local human activities.
C.-M. Gan, J. Pleim, R. Mathur, C. Hogrefe, C. N. Long, J. Xing, D. Wong, R. Gilliam, and C. Wei
Atmos. Chem. Phys., 15, 12193–12209, https://doi.org/10.5194/acp-15-12193-2015, https://doi.org/10.5194/acp-15-12193-2015, 2015
Short summary
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This study attempts to determine the consequences of the changes in tropospheric aerosol burden arising from substantial reductions in emissions of SO2 and NOx associated with control measures under the Clean Air Act especially on trends in solar radiation. Comparisons of model results with observations of aerosol optical depth, aerosol concentration, and radiation demonstrate that the coupled WRF-CMAQ model is capable of replicating the trends well even though it tends to underestimate the AOD.
G. Bernhard, A. Arola, A. Dahlback, V. Fioletov, A. Heikkilä, B. Johnsen, T. Koskela, K. Lakkala, T. Svendby, and J. Tamminen
Atmos. Chem. Phys., 15, 7391–7412, https://doi.org/10.5194/acp-15-7391-2015, https://doi.org/10.5194/acp-15-7391-2015, 2015
Short summary
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Surface erythemal UV data from the Ozone Monitoring Instrument (OMI) are validated for high northern latitudes (Arctic and Scandinavia) using ground-based measurements. The bias in OMI data caused by incorrect assumptions of the surface albedo are quantified and the mechanism that causes this bias is discussed. Methods to improve the accuracy of OMI data products are presented.
S. R. Wilson
Atmos. Chem. Phys., 15, 7337–7349, https://doi.org/10.5194/acp-15-7337-2015, https://doi.org/10.5194/acp-15-7337-2015, 2015
Short summary
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Measurements of the photolysis rates which drive production of OH from ozone are reported for Cape Grim, a "clean-air" site in the southern midlatitudes. This remote maritime site sits in the Southern Ocean, a region of the globe which is little studied. From the 6 years of data the dependence of this photolysis on solar zenith angle and stratospheric ozone is determined. Included with the reported values is an estimate of the uncertainties in these measurements.
C. A. Varotsos, S. Lovejoy, N. V. Sarlis, C. G. Tzanis, and M. N. Efstathiou
Atmos. Chem. Phys., 15, 7301–7306, https://doi.org/10.5194/acp-15-7301-2015, https://doi.org/10.5194/acp-15-7301-2015, 2015
Short summary
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Varotsos et al. (Theor. Appl. Climatol., 114, 725–727, 2013) found that the solar ultraviolet (UV) wavelengths exhibit 1/f-type power-law correlations. In this study, we show that the residues of the spectral solar incident flux with respect to the Planck law over a wider range of wavelengths (i.e. UV-visible) have a scaling regime too.
P. Wang, M. Allaart, W. H. Knap, and P. Stammes
Atmos. Chem. Phys., 15, 4131–4144, https://doi.org/10.5194/acp-15-4131-2015, https://doi.org/10.5194/acp-15-4131-2015, 2015
Short summary
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A green light sensor has been developed at KNMI to measure actinic flux profiles together with an ozonesonde. The impact of clouds on the actinic flux is clearly detected. Good agreement is found between the DAK-simulated actinic flux profiles and the observations for single-layer clouds in fully overcast scenes. The instrument is suitable for operational balloon measurements because of its simplicity and low cost.
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Short summary
The present-day land energy balance over East Asia is estimated for the first time. Results indicate that high aerosol loadings, clouds, and the Tibet Plateau (TP) over East Asia play vital roles in the shortwave budgets, while the TP is responsible for the longwave budgets during this regional energy budget assessment. This study provides a perspective to understand fully how the potential factors influence the diversifying regional energy budget assessments.
The present-day land energy balance over East Asia is estimated for the first time. Results...
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