Articles | Volume 21, issue 1
https://doi.org/10.5194/acp-21-357-2021
https://doi.org/10.5194/acp-21-357-2021
Research article
 | 
14 Jan 2021
Research article |  | 14 Jan 2021

Insights into the aging of biomass burning aerosol from satellite observations and 3D atmospheric modeling: evolution of the aerosol optical properties in Siberian wildfire plumes

Igor B. Konovalov, Nikolai A. Golovushkin, Matthias Beekmann, and Meinrat O. Andreae

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Cited articles

Agarwal, S., Aggarwal, S. G., Okuzawa, K., and Kawamura, K.: Size distributions of dicarboxylic acids, ketoacids, α-dicarbonyls, sugars, WSOC, OC, EC and inorganic ions in atmospheric particles over Northern Japan: implication for long-range transport of Siberian biomass burning and East Asian polluted aerosols, Atmos. Chem. Phys., 10, 5839–5858, https://doi.org/10.5194/acp-10-5839-2010, 2010. 
Ahern, A. T., Robinson, E. S., Tkacik, D. S., Saleh, R., Hatch, L. E., Barsanti, K. C., Stockwell, C. E., Yokelson, R. J., Presto, A. A., Robinson, A. L., Sullivan, R. C., and Donahue, N. M.: Production of secondary organic aerosol during aging of biomass burning smoke from fresh fuels and its relationship to VOC precursors, J. Geophys. Res., 124, 3583–3606, https://doi.org/10.1029/2018JD029068, 2019. 
Ahn, C., Torres, O., and Jethva, H.: Assessment of OMI near-U aerosol optical depth over land, J. Geophys. Res.-Atmos., 119, 2457–2473, https://doi.org/10.1002/2013JD020188, 2014. 
Akagi, S. K., Craven, J. S., Taylor, J. W., McMeeking, G. R., Yokelson, R. J., Burling, I. R., Urbanski, S. P., Wold, C. E., Seinfeld, J. H., Coe, H., Alvarado, M. J., and Weise, D. R.: Evolution of trace gases and particles emitted by a chaparral fire in California, Atmos. Chem. Phys., 12, 1397–1421, https://doi.org/10.5194/acp-12-1397-2012, 2012. 
Andreae, M. O. and Gelencsér, A.: Black carbon or brown carbon? The nature of light-absorbing carbonaceous aerosols, Atmos. Chem. Phys., 6, 3131–3148, https://doi.org/10.5194/acp-6-3131-2006, 2006. 
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Short summary
A lack of consistent observational constraints on the atmospheric evolution of the optical properties of biomass burning (BB) aerosol limits the accuracy of assessments of the aerosol radiative and climate effects. We show that useful insights into the evolution of the BB aerosol optical properties can be inferred from a combination of satellite observations and 3D modeling. We report major changes that occurred in the optical properties of Siberian BB aerosol during its long-range transport.
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