Articles | Volume 20, issue 5
https://doi.org/10.5194/acp-20-3135-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-20-3135-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
16 Mar 2020
Research article |
| 16 Mar 2020
| 16 Mar 2020
Cloud condensation nuclei properties of South Asian outflow over the northern Indian Ocean during winter
Vijayakumar S. Nair
CORRESPONDING AUTHOR
Space Physics Laboratory, Vikram Sarabhai Space Centre,
Thiruvananthapuram, India
Venugopalan Nair Jayachandran
Space Physics Laboratory, Vikram Sarabhai Space Centre,
Thiruvananthapuram, India
Sobhan Kumar Kompalli
Space Physics Laboratory, Vikram Sarabhai Space Centre,
Thiruvananthapuram, India
Mukunda M. Gogoi
Space Physics Laboratory, Vikram Sarabhai Space Centre,
Thiruvananthapuram, India
S. Suresh Babu
Space Physics Laboratory, Vikram Sarabhai Space Centre,
Thiruvananthapuram, India
Related authors
Sobhan Kumar Kompalli, Surendran Nair Suresh Babu, Krishnaswamy Krishna Moorthy, Sreedharan Krishnakumari Satheesh, Mukunda Madhab Gogoi, Vijayakumar S. Nair, Venugopalan Nair Jayachandran, Dantong Liu, Michael J. Flynn, and Hugh Coe
Atmos. Chem. Phys., 21, 9173–9199, https://doi.org/10.5194/acp-21-9173-2021, https://doi.org/10.5194/acp-21-9173-2021, 2021
Short summary
Short summary
The first observations of refractory black carbon aerosol size distributions and mixing state in South Asian outflow to the northern Indian Ocean were carried out as a part of the ICARB-2018 experiment during winter. Size distributions indicated mixed sources of BC particles in the outflow, which are thickly coated. The coating thickness of BC is controlled mainly by the availability of condensable species in the outflow.
Vijayakumar Sivadasan Nair, Filippo Giorgi, and Usha Keshav Hasyagar
Atmos. Chem. Phys., 20, 14457–14471, https://doi.org/10.5194/acp-20-14457-2020, https://doi.org/10.5194/acp-20-14457-2020, 2020
Short summary
Short summary
Air pollution and wintertime fog over South Asia is a major concern due to its significant implications on air quality, visibility and health. Coupled model simulations show that hygroscopic growth of aerosols contributes significantly to the aerosol-induced cooling at the surface. Our analysis demonstrates that the aerosol–moisture interaction is the most significant contributor favouring and strengthening the high-aerosol conditions (poor air quality) prevailing over South Asia during winter.
Venugopalan Nair Jayachandran, Surendran Nair Suresh Babu, Aditya Vaishya, Mukunda M. Gogoi, Vijayakumar S. Nair, Sreedharan Krishnakumari Satheesh, and Krishnaswamy Krishna Moorthy
Atmos. Chem. Phys., 20, 561–576, https://doi.org/10.5194/acp-20-561-2020, https://doi.org/10.5194/acp-20-561-2020, 2020
Short summary
Short summary
Concurrent measurements of the altitude profiles of the concentration of cloud condensation nuclei (CCNs), as a function of supersaturation (ranging from 0.2 % to 1.0 %), and aerosol optical properties were carried out aboard an instrumented aircraft across the Indo-Gangetic Plain (IGP) just prior to the onset of the 2016 Indian summer monsoon (ISM). A high CCN concentration is observed up to 2.5 km across the IGP, indicating the significant possibility of aerosol indirect effects.
F. Solmon, V. S. Nair, and M. Mallet
Atmos. Chem. Phys., 15, 8051–8064, https://doi.org/10.5194/acp-15-8051-2015, https://doi.org/10.5194/acp-15-8051-2015, 2015
Short summary
Short summary
Using observations and a regional climate model, we suggest that
(i) dust radiative forcing over west Asia induces complex regional feedbacks on the Indian monsoon system, notably a possible enhancement of moisture convergence over southern India; and (ii) an observed AOD positive trend attributed to an increasing Arabian dust activity during 2000-2009 could be associated with, and contributing to, the observed enhancement of southern Indian summer precipitation during this decade.
R. Kumar, M. C. Barth, V. S. Nair, G. G. Pfister, S. Suresh Babu, S. K. Satheesh, K. Krishna Moorthy, G. R. Carmichael, Z. Lu, and D. G. Streets
Atmos. Chem. Phys., 15, 5415–5428, https://doi.org/10.5194/acp-15-5415-2015, https://doi.org/10.5194/acp-15-5415-2015, 2015
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We examine differences in the surface BC between the Bay of Bengal (BoB) and the Arabian Sea (AS) and identify dominant sources of BC in South Asia during ICARB. Anthropogenic emissions were the main source of BC during ICARB and had about 5 times stronger influence on the BoB compared to the AS. Regional-scale transport contributes up to 25% of BC mass concentrations in western and eastern India, suggesting that surface BC mass concentrations cannot be linked directly to the local emissions.
Mukunda M. Gogoi, S. Suresh Babu, Ryoichi Imasu, and Makiko Hashimoto
Atmos. Chem. Phys., 23, 8059–8079, https://doi.org/10.5194/acp-23-8059-2023, https://doi.org/10.5194/acp-23-8059-2023, 2023
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Considering the climate warming potential of atmospheric black carbon (BC), satellite-based retrieval is a novel idea. This study highlights the regional distribution of BC based on observations by the Cloud and Aerosol Imager-2 on board the GOSAT-2 satellite and near-surface measurements of BC in ARFINET. The satellite retrieval fairly depicts the regional and seasonal features of BC over the Indian region, which are similar to those recorded by surface observations.
Mathew Sebastian, Sobhan Kumar Kompalli, Vasudevan Anil Kumar, Sandhya Jose, S. Suresh Babu, Govindan Pandithurai, Sachchidanand Singh, Rakesh K. Hooda, Vijay K. Soni, Jeffrey R. Pierce, Ville Vakkari, Eija Asmi, Daniel M. Westervelt, Antti-Pekka Hyvärinen, and Vijay P. Kanawade
Atmos. Chem. Phys., 22, 4491–4508, https://doi.org/10.5194/acp-22-4491-2022, https://doi.org/10.5194/acp-22-4491-2022, 2022
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Characteristics of particle number size distributions and new particle formation in six locations in India were analyzed. New particle formation occurred frequently during the pre-monsoon (spring) season and it significantly modulates the shape of the particle number size distributions. The contribution of newly formed particles to cloud condensation nuclei concentrations was ~3 times higher in urban locations than in mountain background locations.
Zixia Liu, Martin Osborne, Karen Anderson, Jamie D. Shutler, Andy Wilson, Justin Langridge, Steve H. L. Yim, Hugh Coe, Suresh Babu, Sreedharan K. Satheesh, Paquita Zuidema, Tao Huang, Jack C. H. Cheng, and James Haywood
Atmos. Meas. Tech., 14, 6101–6118, https://doi.org/10.5194/amt-14-6101-2021, https://doi.org/10.5194/amt-14-6101-2021, 2021
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This paper first validates the performance of an advanced aerosol observation instrument POPS against a reference instrument and examines any biases introduced by operating it on a quadcopter drone. The results show the POPS performs relatively well on the ground. The impact of the UAV rotors on the POPS is small at low wind speeds, but when operating under higher wind speeds, larger discrepancies occur. It appears that the POPS measures sub-micron aerosol particles more accurately on the UAV.
Sobhan Kumar Kompalli, Surendran Nair Suresh Babu, Krishnaswamy Krishna Moorthy, Sreedharan Krishnakumari Satheesh, Mukunda Madhab Gogoi, Vijayakumar S. Nair, Venugopalan Nair Jayachandran, Dantong Liu, Michael J. Flynn, and Hugh Coe
Atmos. Chem. Phys., 21, 9173–9199, https://doi.org/10.5194/acp-21-9173-2021, https://doi.org/10.5194/acp-21-9173-2021, 2021
Short summary
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The first observations of refractory black carbon aerosol size distributions and mixing state in South Asian outflow to the northern Indian Ocean were carried out as a part of the ICARB-2018 experiment during winter. Size distributions indicated mixed sources of BC particles in the outflow, which are thickly coated. The coating thickness of BC is controlled mainly by the availability of condensable species in the outflow.
Vijayakumar Sivadasan Nair, Filippo Giorgi, and Usha Keshav Hasyagar
Atmos. Chem. Phys., 20, 14457–14471, https://doi.org/10.5194/acp-20-14457-2020, https://doi.org/10.5194/acp-20-14457-2020, 2020
Short summary
Short summary
Air pollution and wintertime fog over South Asia is a major concern due to its significant implications on air quality, visibility and health. Coupled model simulations show that hygroscopic growth of aerosols contributes significantly to the aerosol-induced cooling at the surface. Our analysis demonstrates that the aerosol–moisture interaction is the most significant contributor favouring and strengthening the high-aerosol conditions (poor air quality) prevailing over South Asia during winter.
Mukunda Madhab Gogoi, Venugopalan Nair Jayachandran, Aditya Vaishya, Surendran Nair Suresh Babu, Sreedharan Krishnakumari Satheesh, and Krishnaswamy Krishna Moorthy
Atmos. Chem. Phys., 20, 8593–8610, https://doi.org/10.5194/acp-20-8593-2020, https://doi.org/10.5194/acp-20-8593-2020, 2020
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Extensive airborne measurements of aerosol number–size distribution and black carbon (BC) profiles are carried out for the first time across the IGP prior to the onset of the Indian summer monsoon. These measurements, combined with spaceborne sensors and model results, provided an east–west transect of the role of mineral dust (local and transported) in the aerosol loading across the IGP, with an increase in coarse mode concentration and coarse mode mass fraction with altitude.
Venugopalan Nair Jayachandran, Mercy Varghese, Palani Murugavel, Kiran S. Todekar, Shivdas P. Bankar, Neelam Malap, Gurnule Dinesh, Pramod D. Safai, Jaya Rao, Mahen Konwar, Shivsai Dixit, and Thara V. Prabha
Atmos. Chem. Phys., 20, 7307–7334, https://doi.org/10.5194/acp-20-7307-2020, https://doi.org/10.5194/acp-20-7307-2020, 2020
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Continuous aerosol and cloud condensation nuclei (CCN) measurements carried out at the ground observational facility of a CAIPEEX campaign, situated in the rain-shadow region of the Indian subcontinent, are illustrated. The variations in CCN characteristics within the monsoon period are investigated along with the aerosol physical and optical properties. The change in the dependency of CCN activity on aerosol size and composition due to the variations in air mass and meteorology is brought out.
Sobhan Kumar Kompalli, Surendran Nair Suresh Babu, Sreedharan Krishnakumari Satheesh, Krishnaswamy Krishna Moorthy, Trupti Das, Ramasamy Boopathy, Dantong Liu, Eoghan Darbyshire, James D. Allan, James Brooks, Michael J. Flynn, and Hugh Coe
Atmos. Chem. Phys., 20, 3965–3985, https://doi.org/10.5194/acp-20-3965-2020, https://doi.org/10.5194/acp-20-3965-2020, 2020
Venugopalan Nair Jayachandran, Surendran Nair Suresh Babu, Aditya Vaishya, Mukunda M. Gogoi, Vijayakumar S. Nair, Sreedharan Krishnakumari Satheesh, and Krishnaswamy Krishna Moorthy
Atmos. Chem. Phys., 20, 561–576, https://doi.org/10.5194/acp-20-561-2020, https://doi.org/10.5194/acp-20-561-2020, 2020
Short summary
Short summary
Concurrent measurements of the altitude profiles of the concentration of cloud condensation nuclei (CCNs), as a function of supersaturation (ranging from 0.2 % to 1.0 %), and aerosol optical properties were carried out aboard an instrumented aircraft across the Indo-Gangetic Plain (IGP) just prior to the onset of the 2016 Indian summer monsoon (ISM). A high CCN concentration is observed up to 2.5 km across the IGP, indicating the significant possibility of aerosol indirect effects.
James Brooks, Dantong Liu, James D. Allan, Paul I. Williams, Jim Haywood, Ellie J. Highwood, Sobhan K. Kompalli, S. Suresh Babu, Sreedharan K. Satheesh, Andrew G. Turner, and Hugh Coe
Atmos. Chem. Phys., 19, 13079–13096, https://doi.org/10.5194/acp-19-13079-2019, https://doi.org/10.5194/acp-19-13079-2019, 2019
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Our study presents an analysis of the vertical and horizontal black carbon properties across northern India using aircraft measurements. The Indo-Gangetic Plain saw the greatest black carbon mass concentrations during the pre-monsoon season. Two black carbon modes were recorded: a small black carbon mode (traffic emissions) in the north-west and a moderately coated mode (solid-fuel emissions) in the Indo-Gangetic Plain. In the vertical profile, absorption properties increase with height.
Harshavardhana Sunil Pathak, Sreedharan Krishnakumari Satheesh, Ravi Shankar Nanjundiah, Krishnaswamy Krishna Moorthy, Sivaramakrishnan Lakshmivarahan, and Surendran Nair Suresh Babu
Atmos. Chem. Phys., 19, 11865–11886, https://doi.org/10.5194/acp-19-11865-2019, https://doi.org/10.5194/acp-19-11865-2019, 2019
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We have developed quality-enhanced, gridded datasets for aerosol optical depth (AOD) and absorption AOD by assimilating highly accurate measurements from the dense network of ground-based stations, with respective satellite-retrieved datasets. The assimilated datasets demonstrate improved accuracy and reduced uncertainties as compared to respective satellite products. Thus, these assimilated products emerge as important tools to improve the accuracy of climate impact assessment of aerosols.
James Brooks, James D. Allan, Paul I. Williams, Dantong Liu, Cathryn Fox, Jim Haywood, Justin M. Langridge, Ellie J. Highwood, Sobhan K. Kompalli, Debbie O'Sullivan, Suresh S. Babu, Sreedharan K. Satheesh, Andrew G. Turner, and Hugh Coe
Atmos. Chem. Phys., 19, 5615–5634, https://doi.org/10.5194/acp-19-5615-2019, https://doi.org/10.5194/acp-19-5615-2019, 2019
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Our study, for the first time, presents measurements of aerosol chemical composition and physical characteristics across northern India in the pre-monsoon and monsoon seasons of 2016 using the FAAM BAe-146 UK research aircraft. Across northern India, an elevated aerosol layer dominated by sulfate aerosol exists that diminishes with monsoon arrival. The Indo-Gangetic Plain (IGP) boundary layer is dominated by organics, whereas outside the IGP sulfate dominates with increased scattering aerosol.
Aditya Vaishya, Surendran Nair Suresh Babu, Venugopalan Jayachandran, Mukunda M. Gogoi, Naduparambil Bharathan Lakshmi, Krishnaswamy Krishna Moorthy, and Sreedharan Krishnakumari Satheesh
Atmos. Chem. Phys., 18, 17669–17685, https://doi.org/10.5194/acp-18-17669-2018, https://doi.org/10.5194/acp-18-17669-2018, 2018
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Aircraft-based measurements of vertical profiles of aerosol properties, across the Indo-Gangetic Plain (IGP), prior to onset of the Indian summer monsoon reveal a highly absorbing aerosol system over the IGP. Aerosols over the west IGP are mostly natural, larger in size and scatter light efficiently. Those over the central and eastern IGP are mostly anthropogenic in origin, smaller in size and absorb more light. Elevated absorbing aerosol layers may modulate regional precipitation patterns.
F. Solmon, V. S. Nair, and M. Mallet
Atmos. Chem. Phys., 15, 8051–8064, https://doi.org/10.5194/acp-15-8051-2015, https://doi.org/10.5194/acp-15-8051-2015, 2015
Short summary
Short summary
Using observations and a regional climate model, we suggest that
(i) dust radiative forcing over west Asia induces complex regional feedbacks on the Indian monsoon system, notably a possible enhancement of moisture convergence over southern India; and (ii) an observed AOD positive trend attributed to an increasing Arabian dust activity during 2000-2009 could be associated with, and contributing to, the observed enhancement of southern Indian summer precipitation during this decade.
R. Kumar, M. C. Barth, V. S. Nair, G. G. Pfister, S. Suresh Babu, S. K. Satheesh, K. Krishna Moorthy, G. R. Carmichael, Z. Lu, and D. G. Streets
Atmos. Chem. Phys., 15, 5415–5428, https://doi.org/10.5194/acp-15-5415-2015, https://doi.org/10.5194/acp-15-5415-2015, 2015
Short summary
Short summary
We examine differences in the surface BC between the Bay of Bengal (BoB) and the Arabian Sea (AS) and identify dominant sources of BC in South Asia during ICARB. Anthropogenic emissions were the main source of BC during ICARB and had about 5 times stronger influence on the BoB compared to the AS. Regional-scale transport contributes up to 25% of BC mass concentrations in western and eastern India, suggesting that surface BC mass concentrations cannot be linked directly to the local emissions.
Related subject area
Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
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From fall 2021 to summer 2023, SAIL-Net, a network of six aerosol measurement nodes, was deployed in the East River watershed (Colorado, USA) to study aerosol variability across space and time in mountainous terrain. We found that aerosol variability is influenced by elevation differences, with the most representative site in the region changing seasonally, suggesting aerosol spatial variability also varies seasonally. This work offers a blueprint for future studies in other mountainous regions.
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Clouds over the Southern Ocean are crucial to Earth's energy balance, but understanding the factors that control them is complex. Our research examines how weather patterns affect tiny particles called cloud condensation nuclei (CCN), which influence cloud properties. Using data from Kennaook / Cape Grim, we found that winter air from Antarctica brings cleaner conditions with lower CCN, while summer patterns from Australia transport more particles. Precipitation also helps reduce CCN in winter.
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Two shipborne observations in the South China Sea (SCS) in summer and winter 2021 were conducted. Our study found aerosol hygroscopicity is higher in the SCS in summer than winter, with significant influences from various terrestrial air masses. Aerosol size distribution had a stronger effect on activation ratio than aerosol hygroscopicity in summer and vice versa in winter. Our study provides valuable information to enhance our understanding of cloud condensation nuclei activities in the SCS.
Bighnaraj Sarangi, Darrel Baumgardner, Ana Isabel Calvo, Benjamin Bolaños-Rosero, Roberto Fraile, Alberto Rodríguez-Fernández, Delia Fernández-González, Carlos Blanco-Alegre, Cátia Gonçalves, Estela D. Vicente, and Olga L. Mayol-Bracero
Atmos. Chem. Phys., 25, 843–865, https://doi.org/10.5194/acp-25-843-2025, https://doi.org/10.5194/acp-25-843-2025, 2025
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Measurements of fluorescing aerosol particle properties have been made during two major African dust events, one over the island of Puerto Rico and the other over the city of León, Spain. The measurements were made with two wideband integrated bioaerosol spectrometers. A significant change in the background aerosol properties, at both locations, is observed when the dust is in the respective regions.
Lijing Chen, Lei Zhang, Yong She, Zhaoliang Zeng, Yu Zheng, Biao Tian, Wenqian Zhang, Zhaohui Liu, Huizheng Che, and Minghu Ding
Atmos. Chem. Phys., 25, 727–739, https://doi.org/10.5194/acp-25-727-2025, https://doi.org/10.5194/acp-25-727-2025, 2025
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Aerosol optical depth (AOD) at Zhongshan Station varies seasonally, with lower values in summer and higher values in winter. Winter and spring AOD increases due to reduced fine-mode particles, while summer and autumn increases are linked to particle growth. Diurnal AOD variation correlates positively with temperature but negatively with wind speed and humidity. Backward trajectories show that aerosols on high-AOD (low-AOD) days primarily originate from the ocean (interior Antarctica).
Shravan Deshmukh, Laurent Poulain, Birgit Wehner, Silvia Henning, Jean-Eudes Petit, Pauline Fombelle, Olivier Favez, Hartmut Herrmann, and Mira Pöhlker
Atmos. Chem. Phys., 25, 741–758, https://doi.org/10.5194/acp-25-741-2025, https://doi.org/10.5194/acp-25-741-2025, 2025
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Aerosol hygroscopicity has been investigated at a sub-urban site in Paris; analysis shows the sub-saturated regime's measured hygroscopicity and the chemically derived hygroscopic growth, shedding light on the large effect of external particle mixing and its influence on predicting hygroscopicity.
Takeshi Kinase, Fumikazu Taketani, Masayuki Takigawa, Chunmao Zhu, Yongwon Kim, Petr Mordovskoi, and Yugo Kanaya
Atmos. Chem. Phys., 25, 143–156, https://doi.org/10.5194/acp-25-143-2025, https://doi.org/10.5194/acp-25-143-2025, 2025
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Boreal forest wildfires in interior Alaska represent an important black carbon (BC) source for the Arctic and surrounding regions. We observed BC and carbon monoxide (CO) concentrations in the Poker Flat Research Range since 2016 and found a positive correlation between the observed BC / ∆CO ratio and fire radiative power (FRP) observed in Alaska and Canada. Our finding suggests the BC emission factor and/or inventory could be potentially improved by using FRP.
Erin N. Raif, Sarah L. Barr, Mark D. Tarn, James B. McQuaid, Martin I. Daily, Steven J. Abel, Paul A. Barrett, Keith N. Bower, Paul R. Field, Kenneth S. Carslaw, and Benjamin J. Murray
Atmos. Chem. Phys., 24, 14045–14072, https://doi.org/10.5194/acp-24-14045-2024, https://doi.org/10.5194/acp-24-14045-2024, 2024
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Ice-nucleating particles (INPs) allow ice to form in clouds at temperatures warmer than −35°C. We measured INP concentrations over the Norwegian and Barents seas in weather events where cold air is ejected from the Arctic. These concentrations were among the highest measured in the Arctic. It is likely that the INPs were transported to the Arctic from distant regions. These results show it is important to consider hemispheric-scale INP processes to understand INP concentrations in the Arctic.
Fernando Rejano, Andrea Casans, Marta Via, Juan Andrés Casquero-Vera, Sonia Castillo, Hassan Lyamani, Alberto Cazorla, Elisabeth Andrews, Daniel Pérez-Ramírez, Andrés Alastuey, Francisco Javier Gómez-Moreno, Lucas Alados-Arboledas, Francisco José Olmo, and Gloria Titos
Atmos. Chem. Phys., 24, 13865–13888, https://doi.org/10.5194/acp-24-13865-2024, https://doi.org/10.5194/acp-24-13865-2024, 2024
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This study provides valuable insights to improve cloud condensation nuclei (CCN) estimations at a high-altitude remote site which is influenced by nearby urban pollution. Understanding the factors that affect CCN estimations is essential to improve the CCN data coverage worldwide and assess aerosol–cloud interactions on a global scale. This is crucial for improving climate models, since aerosol–cloud interactions are the most important source of uncertainty in climate projections.
Lu Zhang, Michal Segal-Rozenhaimer, Haochi Che, Caroline Dang, Junying Sun, Ye Kuang, Paola Formenti, and Steven G. Howell
Atmos. Chem. Phys., 24, 13849–13864, https://doi.org/10.5194/acp-24-13849-2024, https://doi.org/10.5194/acp-24-13849-2024, 2024
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Using airborne measurements over the southeast Atlantic Ocean, we examined how much moisture aerosols take up during Africa’s biomass burning season. Our study revealed the important role of organic aerosols and introduced a predictive model for moisture uptake, accounting for organics, sulfate, and black carbon, summarizing results from various campaigns. These findings improve our understanding of aerosol–moisture interactions and their radiative effects in this climatically critical region.
Mary C. Robinson, Kaitlin Schueth, and Karin Ardon-Dryer
Atmos. Chem. Phys., 24, 13733–13750, https://doi.org/10.5194/acp-24-13733-2024, https://doi.org/10.5194/acp-24-13733-2024, 2024
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On 26 February 2023, New Mexico and West Texas were impacted by a severe dust storm. To analyze this storm, 28 meteorological stations and 19 PM2.5 and PM10 stations were used. Dust particles were in the air for 16 h, and dust storm conditions lasted for up to 120 min. Hourly PM2.5 and PM10 concentrations were up to 518 and 9983 µg m−3, respectively. For Lubbock, Texas, the maximum PM2.5 concentrations were the highest ever recorded.
Jerome D. Fast, Adam C. Varble, Fan Mei, Mikhail Pekour, Jason Tomlinson, Alla Zelenyuk, Art J. Sedlacek III, Maria Zawadowicz, and Louisa Emmons
Atmos. Chem. Phys., 24, 13477–13502, https://doi.org/10.5194/acp-24-13477-2024, https://doi.org/10.5194/acp-24-13477-2024, 2024
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Aerosol property measurements recently collected on the ground and by a research aircraft in central Argentina during the Cloud, Aerosol, and Complex Terrain Interactions (CACTI) campaign exhibit large spatial and temporal variability. These measurements coupled with coincident meteorological information provide a valuable data set needed to evaluate and improve model predictions of aerosols in a traditionally data-sparse region of South America.
Julika Zinke, Gabriel Pereira Freitas, Rachel Ann Foster, Paul Zieger, Ernst Douglas Nilsson, Piotr Markuszewski, and Matthew Edward Salter
Atmos. Chem. Phys., 24, 13413–13428, https://doi.org/10.5194/acp-24-13413-2024, https://doi.org/10.5194/acp-24-13413-2024, 2024
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Bioaerosols, which can influence climate and human health, were studied in the Baltic Sea. In May and August 2021, we used a sea spray simulation chamber during two ship-based campaigns to collect and measure these aerosols. We found that microbes were enriched in air compared to seawater. Bacterial diversity was analysed using DNA sequencing. Our methods provided consistent estimates of microbial emission fluxes, aligning with previous studies.
Chimurkar Navinya, Taveen Singh Kapoor, Gupta Anurag, Chandra Venkataraman, Harish C. Phuleria, and Rajan K. Chakrabarty
Atmos. Chem. Phys., 24, 13285–13297, https://doi.org/10.5194/acp-24-13285-2024, https://doi.org/10.5194/acp-24-13285-2024, 2024
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Brown carbon (BrC) aerosols show an order-of-magnitude variation in their light absorption strength. Our understanding of BrC from real-world biomass burning remains limited, complicating the determination of its radiative impact. Our study reports absorption properties of BrC emitted from four major biomass burning sources using field measurements in India. It develops an absorption parameterization for BrC and examines the spatial variability in BrC's absorption strength across India.
Yao Song, Jing Wei, Wenlong Zhao, Jinmei Ding, Xiangyu Pei, Fei Zhang, Zhengning Xu, Ruifang Shi, Ya Wei, Lu Zhang, Lingling Jin, and Zhibin Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-3298, https://doi.org/10.5194/egusphere-2024-3298, 2024
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This study investigates the size-resolved effective density (ρeff) of aerosol particles in Hangzhou using an AAC-SMPS. The ρeff values ranged from 1.47 to 1.63 g/cm3, increasing with particle diameter. Smaller particles showed significant diurnal density variations. The relationship between ρeff and particle diameter varies due to differences in the chemical composition of the particles. A new method to derive size-resolved chemical composition of particles from ρeff was proposed.
Sami D. Harni, Minna Aurela, Sanna Saarikoski, Jarkko V. Niemi, Harri Portin, Hanna Manninen, Ville Leinonen, Pasi Aalto, Phil K. Hopke, Tuukka Petäjä, Topi Rönkkö, and Hilkka Timonen
Atmos. Chem. Phys., 24, 12143–12160, https://doi.org/10.5194/acp-24-12143-2024, https://doi.org/10.5194/acp-24-12143-2024, 2024
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In this study, particle number size distribution data were used in a novel way in positive matrix factorization analysis to find aerosol source profiles in the area. Measurements were made in Helsinki at a street canyon and urban background sites between February 2015 and June 2019. Five different aerosol sources were identified. These sources underline the significance of traffic-related emissions in urban environments despite recent improvements in emission reduction technologies.
Natalie G. Ratcliffe, Claire L. Ryder, Nicolas Bellouin, Stephanie Woodward, Anthony Jones, Ben Johnson, Lisa-Maria Wieland, Maximilian Dollner, Josef Gasteiger, and Bernadett Weinzierl
Atmos. Chem. Phys., 24, 12161–12181, https://doi.org/10.5194/acp-24-12161-2024, https://doi.org/10.5194/acp-24-12161-2024, 2024
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Large mineral dust particles are more abundant in the atmosphere than expected and have different impacts on the environment than small particles, which are better represented in climate models. We use aircraft measurements to assess a climate model representation of large-dust transport. We find that the model underestimates the amount of large dust at all stages of transport and that fast removal of the large particles increases this underestimation with distance from the Sahara.
Sergio Rodríguez and Jessica López-Darias
Atmos. Chem. Phys., 24, 12031–12053, https://doi.org/10.5194/acp-24-12031-2024, https://doi.org/10.5194/acp-24-12031-2024, 2024
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Extreme Saharan dust events expanded northward to the Atlantic and Europe, prompting record-breaking PM10 and PM2.5 events. These episodes are caused by low-to-high dipole meteorology during hemispheric anomalies characterized by subtropical anticyclones shifting to higher latitudes, anomalous low pressures beyond the tropics and amplified Rossby waves. Extreme dust events occur in a paradoxical context of a multidecadal decrease in dust emissions, a topic that requires further investigation.
Valeria Mardoñez-Balderrama, Griša Močnik, Marco Pandolfi, Robin L. Modini, Fernando Velarde, Laura Renzi, Angela Marinoni, Jean-Luc Jaffrezo, Isabel Moreno R., Diego Aliaga, Federico Bianchi, Claudia Mohr, Martin Gysel-Beer, Patrick Ginot, Radovan Krejci, Alfred Wiedensohler, Gaëlle Uzu, Marcos Andrade, and Paolo Laj
Atmos. Chem. Phys., 24, 12055–12077, https://doi.org/10.5194/acp-24-12055-2024, https://doi.org/10.5194/acp-24-12055-2024, 2024
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Levels of black carbon (BC) are scarcely reported in the Southern Hemisphere, especially in high-altitude conditions. This study provides insight into the concentration level, variability, and optical properties of BC in La Paz and El Alto and at the Chacaltaya Global Atmosphere Watch Station. Two methods of source apportionment of absorption were tested and compared showing traffic as the main contributor to absorption in the urban area, in addition to biomass and open waste burning.
Krishnakant Budhavant, Mohanan Remani Manoj, Hari Ram Chandrika Rajendran Nair, Samuel Mwaniki Gaita, Henry Holmstrand, Abdus Salam, Ahmed Muslim, Sreedharan Krishnakumari Satheesh, and Örjan Gustafsson
Atmos. Chem. Phys., 24, 11911–11925, https://doi.org/10.5194/acp-24-11911-2024, https://doi.org/10.5194/acp-24-11911-2024, 2024
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The South Asian Pollution Experiment 2018 used access to three strategically located receptor observatories. Observational constraints revealed opposing trends in the mass absorption cross sections of black carbon (BC MAC) and brown carbon (BrC MAC) during long-range transport. Models estimating the climate effects of BC aerosols may have underestimated the ambient BC MAC over distant receptor areas, leading to discrepancies in aerosol absorption predicted by observation-constrained models.
Jieyao Liu, Fang Zhang, Jingye Ren, and Lu Chen
EGUsphere, https://doi.org/10.5194/egusphere-2024-2999, https://doi.org/10.5194/egusphere-2024-2999, 2024
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The particles mixing states and aging time scale are important for the evaluation of aerosols climate effects, but they are poorly parameterized in current models. We unravel the evolution of real-time mixing states and aging time scale of size-resolved particles based on field measurement in urban Beijing. This study provides observational basis for accurately parameterizing the aging time scale of aerosol particles in climate models.
Abigail S. Williams, Jeramy L. Dedrick, Lynn M. Russell, Florian Tornow, Israel Silber, Ann M. Fridlind, Benjamin Swanson, Paul J. DeMott, Paul Zieger, and Radovan Krejci
Atmos. Chem. Phys., 24, 11791–11805, https://doi.org/10.5194/acp-24-11791-2024, https://doi.org/10.5194/acp-24-11791-2024, 2024
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The measured aerosol size distribution modes reveal distinct properties characteristic of cold-air outbreaks in the Norwegian Arctic. We find higher sea spray number concentrations, smaller Hoppel minima, lower effective supersaturations, and accumulation-mode particle scavenging during cold-air outbreaks. These results advance our understanding of cold-air outbreak aerosol–cloud interactions in order to improve their accurate representation in models.
Franziska Vogel, Michael P. Adams, Larissa Lacher, Polly B. Foster, Grace C. E. Porter, Barbara Bertozzi, Kristina Höhler, Julia Schneider, Tobias Schorr, Nsikanabasi S. Umo, Jens Nadolny, Zoé Brasseur, Paavo Heikkilä, Erik S. Thomson, Nicole Büttner, Martin I. Daily, Romy Fösig, Alexander D. Harrison, Jorma Keskinen, Ulrike Proske, Jonathan Duplissy, Markku Kulmala, Tuukka Petäjä, Ottmar Möhler, and Benjamin J. Murray
Atmos. Chem. Phys., 24, 11737–11757, https://doi.org/10.5194/acp-24-11737-2024, https://doi.org/10.5194/acp-24-11737-2024, 2024
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Primary ice formation in clouds strongly influences their properties; hence, it is important to understand the sources of ice-nucleating particles (INPs) and their variability. We present 2 months of INP measurements in a Finnish boreal forest using a new semi-autonomous INP counting device based on gas expansion. These results show strong variability in INP concentrations, and we present a case that the INPs we observe are, at least some of the time, of biological origin.
Xiaojing Shen, Quan Liu, Junying Sun, Wanlin Kong, Qianli Ma, Bing Qi, Lujie Han, Yangmei Zhang, Linlin Liang, Lei Liu, Shuo Liu, Xinyao Hu, Jiayuan Lu, Aoyuan Yu, Huizheng Che, and Xiaoye Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2024-2850, https://doi.org/10.5194/egusphere-2024-2850, 2024
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In this work, an automatic switched inlet system was developed and employed to investigate the aerosols and cloud droplets at a mountain site with frequent cloud processes. It showed different characteristics of cloud residual and interstitial particles. Stronger particle hygroscopicity reduced liquid water content and smaller cloud droplet diameters. This investigation contributes to understanding aerosol-cloud interactions by assessing the impact of aerosol particles on cloud microphysics.
Rebecca Dischl, Daniel Sauer, Christiane Voigt, Theresa Harlaß, Felicitas Sakellariou, Raphael Märkl, Ulrich Schumann, Monika Scheibe, Stefan Kaufmann, Anke Roiger, Andreas Dörnbrack, Charles Renard, Maxime Gauthier, Peter Swann, Paul Madden, Darren Luff, Mark Johnson, Denise Ahrens, Reetu Sallinen, Tobias Schripp, Georg Eckel, Uwe Bauder, and Patrick Le Clercq
Atmos. Chem. Phys., 24, 11255–11273, https://doi.org/10.5194/acp-24-11255-2024, https://doi.org/10.5194/acp-24-11255-2024, 2024
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In-flight measurements of aircraft emissions burning 100 % sustainable aviation fuel (SAF) show reduced particle number concentrations up to 41 % compared to conventional jet fuel. Particle emissions are dependent on engine power setting, flight altitude, and fuel composition. Engine models show a good correlation with measurement results. Future increased prevalence of SAF can positively influence the climate impact of aviation.
Zoé Brasseur, Julia Schneider, Janne Lampilahti, Ville Vakkari, Victoria A. Sinclair, Christina J. Williamson, Carlton Xavier, Dmitri Moisseev, Markus Hartmann, Pyry Poutanen, Markus Lampimäki, Markku Kulmala, Tuukka Petäjä, Katrianne Lehtipalo, Erik S. Thomson, Kristina Höhler, Ottmar Möhler, and Jonathan Duplissy
Atmos. Chem. Phys., 24, 11305–11332, https://doi.org/10.5194/acp-24-11305-2024, https://doi.org/10.5194/acp-24-11305-2024, 2024
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Ice-nucleating particles (INPs) strongly influence the formation of clouds by initiating the formation of ice crystals. However, very little is known about the vertical distribution of INPs in the atmosphere. Here, we present aircraft measurements of INP concentrations above the Finnish boreal forest. Results show that near-surface INPs are efficiently transported and mixed within the boundary layer and occasionally reach the free troposphere.
Piotr Markuszewski, E. Douglas Nilsson, Julika Zinke, E. Monica Mårtensson, Matthew Salter, Przemysław Makuch, Małgorzata Kitowska, Iwona Niedźwiecka-Wróbel, Violetta Drozdowska, Dominik Lis, Tomasz Petelski, Luca Ferrero, and Jacek Piskozub
Atmos. Chem. Phys., 24, 11227–11253, https://doi.org/10.5194/acp-24-11227-2024, https://doi.org/10.5194/acp-24-11227-2024, 2024
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Our research provides new insights into the study of sea spray aerosol (SSA) emissions in the Baltic Sea and North Atlantic. We observed that SSA flux is suppressed during increased marine biological activity in the Baltic Sea. At the same time, the influence of wave age showed higher SSA emissions in the Baltic Sea for younger waves compared to the Atlantic Ocean. These insights underscore the complex interplay between biological activity and physical dynamics in regulating SSA emissions.
Heather Guy, Andrew S. Martin, Erik Olson, Ian M. Brooks, and Ryan R. Neely III
Atmos. Chem. Phys., 24, 11103–11114, https://doi.org/10.5194/acp-24-11103-2024, https://doi.org/10.5194/acp-24-11103-2024, 2024
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Aerosol particles impact cloud properties which influence Greenland Ice Sheet melt. Understanding the aerosol population that interacts with clouds is important for constraining future melt. Measurements of aerosols at cloud height over Greenland are rare, and surface measurements are often used to investigate cloud–aerosol interactions. We use a tethered balloon to measure aerosols up to cloud base and show that surface measurements are often not equivalent to those just below the cloud.
Kouji Adachi, Jack E. Dibb, Joseph M. Katich, Joshua P. Schwarz, Hongyu Guo, Pedro Campuzano-Jost, Jose L. Jimenez, Jeff Peischl, Christopher D. Holmes, and James Crawford
Atmos. Chem. Phys., 24, 10985–11004, https://doi.org/10.5194/acp-24-10985-2024, https://doi.org/10.5194/acp-24-10985-2024, 2024
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We examined aerosol particles from wildfires and identified tarballs (TBs) from the Fire Influence on Regional to Global Environments and Air Quality (FIREX-AQ) campaign. This study reveals the compositions, abundance, sizes, and mixing states of TBs and shows that TBs formed as the smoke aged for up to 5 h. This study provides measurements of TBs from various biomass-burning events and ages, enhancing our knowledge of TB emissions and our understanding of their climate impact.
Sihan Liu, Honglei Wang, Delong Zhao, Wei Zhou, Yuanmou Du, Zhengguo Zhang, Peng Cheng, Tianliang Zhao, Yue Ke, Zihao Wu, and Mengyu Huang
EGUsphere, https://doi.org/10.5194/egusphere-2024-2756, https://doi.org/10.5194/egusphere-2024-2756, 2024
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To understand the effect of aerosols on the vertical distribution of stratocumulus microphysical quantities in southwest China, the daily variation characteristics and formation mechanism of the vertical profiles of stratocumulus microphysical characteristics in this region were described by using the data of 9 cloud-crossing aircraft observations over Guangxi from October 10 to November 3, 2020.
Jia Sun, Markus Hermann, Kay Weinhold, Maik Merkel, Wolfram Birmili, Yifan Yang, Thomas Tuch, Harald Flentje, Björn Briel, Ludwig Ries, Cedric Couret, Michael Elsasser, Ralf Sohmer, Klaus Wirtz, Frank Meinhardt, Maik Schütze, Olaf Bath, Bryan Hellack, Veli-Matti Kerminen, Markku Kulmala, Nan Ma, and Alfred Wiedensohler
Atmos. Chem. Phys., 24, 10667–10687, https://doi.org/10.5194/acp-24-10667-2024, https://doi.org/10.5194/acp-24-10667-2024, 2024
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We investigated the characteristics of new particle formation (NPF) for various environments from urban background to high Alpine and the impacts of NPF on cloud condensation nuclei and aerosol radiative forcing. NPF features differ between site categories, implying the crucial role of local environmental factors such as the degree of emissions and meteorological conditions. The results also underscore the importance of local environments when assessing the impact of NPF on climate in models.
Baptiste Testa, Lukas Durdina, Jacinta Edebeli, Curdin Spirig, and Zamin A. Kanji
Atmos. Chem. Phys., 24, 10409–10424, https://doi.org/10.5194/acp-24-10409-2024, https://doi.org/10.5194/acp-24-10409-2024, 2024
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Aviation soot residuals released from contrails can become compacted upon sublimation of the ice crystals, generating new voids in the aggregates where ice nucleation can occur. Here we show that contrail-processed soot is highly compact but that it remains unable to form ice at a relative humidity different from that required for the formation of background cirrus from the more ubiquitous aqueous solution droplets, suggesting that it will not perturb cirrus cloud formation via ice nucleation.
Roman Pohorsky, Andrea Baccarini, Natalie Brett, Brice Barret, Slimane Bekki, Gianluca Pappaccogli, Elsa Dieudonné, Brice Temime-Roussel, Barbara D'Anna, Meeta Cesler-Maloney, Antonio Donateo, Stefano Decesari, Kathy S. Law, William R. Simpson, Javier Fochesatto, Steve R. Arnold, and Julia Schmale
EGUsphere, https://doi.org/10.5194/egusphere-2024-2863, https://doi.org/10.5194/egusphere-2024-2863, 2024
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This study presents an analysis of vertical measurements of pollution in an Alaskan city during winter. It investigates the relationship between the atmospheric structure and the layering of aerosols and trace gases. Results indicate an overall very shallow surface mixing layer. The height of this layer is strongly influenced by a local shallow wind. The study also provides information on the pollution chemical composition at different altitudes, including pollution signatures from power plants.
Lingjun Li, Mengren Li, Xiaolong Fan, Yuping Chen, Ziyi Lin, Anqi Hou, Siqing Zhang, Ronghua Zheng, and Jinsheng Chen
EGUsphere, https://doi.org/10.5194/egusphere-2024-2376, https://doi.org/10.5194/egusphere-2024-2376, 2024
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Aerosol hygroscopicity has a great impact on regional and global climate, air quality. Here, we show differences and variations in f(RH) between NPF and Non-NPF days and the effect of aerosol chemical compositions on f(RH) in Xiamen, the coastal city of southeast China by in situ observations. The findings are helpful for the further understanding about aerosol hygroscopicity in the coastal city, and the use of hygroscopic growth factors in the models of air quality and climate change.
Kunfeng Gao, Franziska Vogel, Romanos Foskinis, Stergios Vratolis, Maria I. Gini, Konstantinos Granakis, Anne-Claire Billault-Roux, Paraskevi Georgakaki, Olga Zografou, Prodromos Fetfatzis, Alexis Berne, Alexandros Papayannis, Konstantinos Eleftheridadis, Ottmar Möhler, and Athanasios Nenes
Atmos. Chem. Phys., 24, 9939–9974, https://doi.org/10.5194/acp-24-9939-2024, https://doi.org/10.5194/acp-24-9939-2024, 2024
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Ice nucleating particle (INP) concentrations are required for correct predictions of clouds and precipitation in a changing climate, but they are poorly constrained in climate models. We unravel source contributions to INPs in the eastern Mediterranean and find that biological particles are important, regardless of their origin. The parameterizations developed exhibit superior performance and enable models to consider biological-particle effects on INPs.
Alexandra Kuwano, Amato T. Evan, Blake Walkowiak, and Robert Frouin
Atmos. Chem. Phys., 24, 9843–9868, https://doi.org/10.5194/acp-24-9843-2024, https://doi.org/10.5194/acp-24-9843-2024, 2024
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The dust direct radiative effect is highly uncertain. Here we used new measurements collected over 3 years and during dust storms at a field site in a desert region in the southwestern United States to estimate the regional dust direct radiative effect. We also used novel soil mineralogy retrieved from an airborne spectrometer to estimate this parameter with model output. We find that, in this region, dust has a minimal net cooling effect on this region's climate.
Denghui Ji, Mathias Palm, Matthias Buschmann, Kerstin Ebell, Marion Maturilli, Xiaoyu Sun, and Justus Notholt
EGUsphere, https://doi.org/10.5194/egusphere-2024-2241, https://doi.org/10.5194/egusphere-2024-2241, 2024
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Our study explores how certain aerosols, like sea salt, affect infrared heat radiation in the Arctic, potentially speeding up warming. We used advanced technology to measure aerosol composition and found that these particles grow with humidity, significantly increasing their heat-trapping effect in the infrared region, especially in winter. Our findings suggest these aerosols could be a key factor in Arctic warming, emphasizing the importance of understanding aerosols for climate prediction.
Jutta Kesti, Ewan J. O'Connor, Anne Hirsikko, John Backman, Maria Filioglou, Anu-Maija Sundström, Juha Tonttila, Heikki Lihavainen, Hannele Korhonen, and Eija Asmi
Atmos. Chem. Phys., 24, 9369–9386, https://doi.org/10.5194/acp-24-9369-2024, https://doi.org/10.5194/acp-24-9369-2024, 2024
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The study combines aerosol particle measurements at the surface and vertical profiling of the atmosphere with a scanning Doppler lidar to investigate how particle transportation together with boundary layer evolution can affect particle and SO2 concentrations at the surface in the Arabian Peninsula region. The instrumentation enabled us to see elevated nucleation mode particle and SO2 concentrations at the surface when air masses transported from polluted areas are mixed in the boundary layer.
Jiangchuan Tao, Biao Luo, Weiqi Xu, Gang Zhao, Hanbin Xu, Biao Xue, Miaomiao Zhai, Wanyun Xu, Huarong Zhao, Sanxue Ren, Guangsheng Zhou, Li Liu, Ye Kuang, and Yele Sun
Atmos. Chem. Phys., 24, 9131–9154, https://doi.org/10.5194/acp-24-9131-2024, https://doi.org/10.5194/acp-24-9131-2024, 2024
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Using simultaneous measurements of DMA–CCNC, H(/V)TDMA, and DMA–SP2, impacts of primary emissions and secondary aerosol formations on changes in aerosol physicochemical properties were comprehensively investigated. It was found that intercomparisons among aerosol mixing-state parameters derived from different techniques can help us gain more insight into aerosol physical properties which, in turn, will aid the investigation of emission characteristics and secondary aerosol formation pathways.
Haibiao Chen, Caiqing Yan, Liubin Huang, Lin Du, Yang Yue, Xinfeng Wang, Qingcai Chen, Mingjie Xie, Junwen Liu, Fengwen Wang, Shuhong Fang, Qiaoyun Yang, Hongya Niu, Mei Zheng, Yan Wu, and Likun Xue
EGUsphere, https://doi.org/10.5194/egusphere-2024-2416, https://doi.org/10.5194/egusphere-2024-2416, 2024
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A comprehensive understanding of the optical properties of brown carbon (BrC) is essential to accurately assess its climatic effects. Based on multi-site spectroscopic measurements, this study demonstrated the significant spatial heterogeneity in the optical and structural properties of water-soluble BrC (WS-BrC) in different regions of China, and revealed factors affecting WS-BrC light absorption and the relationship between fluorophores and light absorption of WS-BrC.
Elena Bazo, Daniel Perez-Ramirez, Antonio Valenzuela, Vanderlei Martins, Gloria Titos, Alberto Cazorla, Fernando Rejano, Diego Patrón, Arlett Diaz-Zurita, Francisco Jose Garcia-Izquierdo, David Fuertes, Lucas Alados-Arboledas, and Francisco Jose Olmo
EGUsphere, https://doi.org/10.5194/egusphere-2024-2080, https://doi.org/10.5194/egusphere-2024-2080, 2024
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This works analyses aerosol scattering phase function for transported Saharan dust to the city of Granada – located in southwestern Europe. We use the novel technique polar imaging nephelometry that helps to determine the phase functions using a CCD camara. The capability of measuring with polarized light helps to inferr new properties about the mixture of Saharan dust particles with other of anthropogenic origin.
Marco A. Franco, Rafael Valiati, Bruna A. Holanda, Bruno B. Meller, Leslie A. Kremper, Luciana V. Rizzo, Samara Carbone, Fernando G. Morais, Janaína P. Nascimento, Meinrat O. Andreae, Micael A. Cecchini, Luiz A. T. Machado, Milena Ponczek, Ulrich Pöschl, David Walter, Christopher Pöhlker, and Paulo Artaxo
Atmos. Chem. Phys., 24, 8751–8770, https://doi.org/10.5194/acp-24-8751-2024, https://doi.org/10.5194/acp-24-8751-2024, 2024
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The Amazon wet-season atmosphere was studied at the Amazon Tall Tower Observatory site, revealing vertical variations (between 60 and 325 m) in natural aerosols. Daytime mixing contrasted with nighttime stratification, with distinct rain-induced changes in aerosol populations. Notably, optical property recovery at higher levels was faster, while near-canopy aerosols showed higher scattering efficiency. These findings enhance our understanding of aerosol impacts on climate dynamics.
Kristina Pistone, Eric M. Wilcox, Paquita Zuidema, Marco Giordano, James Podolske, Samuel E. LeBlanc, Meloë Kacenelenbogen, Steven G. Howell, and Steffen Freitag
Atmos. Chem. Phys., 24, 7983–8005, https://doi.org/10.5194/acp-24-7983-2024, https://doi.org/10.5194/acp-24-7983-2024, 2024
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The springtime southeast Atlantic atmosphere contains lots of smoke from continental fires. This smoke travels with water vapor; more smoke means more humidity. We use aircraft observations and models to describe how the values change through the season and over the region. We sort the atmosphere into different types by vertical structure and amount of smoke and humidity. Since our work shows how frequently these components coincide, it helps to better quantify heating effects over this region.
Haifeng Yu, Yunhua Chang, Lin Cheng, Yusen Duan, and Jianlin Hu
EGUsphere, https://doi.org/10.5194/egusphere-2024-1488, https://doi.org/10.5194/egusphere-2024-1488, 2024
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This study presents long-term measurements and comprehensive analysis of carbonaceous aerosols in PM2.5 in Shanghai. We further estimated POC and SOC levels, examining their temporal variations on interannual, monthly, seasonal, and diurnal scales. Through rigorous statistical analysis and correlation studies with meteorological parameters and pollutant concentrations, the origins, formation mechanisms, and spatial distribution patterns of SOC were elucidated.
Yange Deng, Hiroshi Tanimoto, Kohei Ikeda, Sohiko Kameyama, Sachiko Okamoto, Jinyoung Jung, Young Jun Yoon, Eun Jin Yang, and Sung-Ho Kang
Atmos. Chem. Phys., 24, 6339–6357, https://doi.org/10.5194/acp-24-6339-2024, https://doi.org/10.5194/acp-24-6339-2024, 2024
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Black carbon (BC) aerosols play important roles in Arctic climate change, yet they are not well understood because of limited observational data. We observed BC mass concentrations (mBC) in the western Arctic Ocean during summer and early autumn 2016–2020. The mean mBC in 2019 was much higher than in other years. Biomass burning was likely the dominant BC source. Boreal fire BC transport occurring near the surface and/or in the mid-troposphere contributed to high-BC events in the Arctic Ocean.
Máté Vörösmarty, Philip K. Hopke, and Imre Salma
Atmos. Chem. Phys., 24, 5695–5712, https://doi.org/10.5194/acp-24-5695-2024, https://doi.org/10.5194/acp-24-5695-2024, 2024
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The World Health Organization identified ultrafine particles, which make up most of the particle number concentrations, as a potential risk factor for humans. The sources of particle numbers are very different from those of the particulate matter mass. We performed source apportionment of size-segregated particle number concentrations over the diameter range of 6–1000 nm in Budapest for 11 full years. Six source types were identified, characterized and quantified.
Cited articles
Ackerman, A. S., Toon, O. B., Stevens, D. E., Heymsfield, A. J., Ramanathan,
V., and Welton, E. J.: Reduction of tropical cloudiness by soot, Science, 288,
1042–1047, https://doi.org/10.1126/science.288.5468.1042, 2000.
Andreae, M. O.: Correlation between cloud condensation nuclei concentration and aerosol optical thickness in remote and polluted regions, Atmos. Chem. Phys., 9, 543–556, https://doi.org/10.5194/acp-9-543-2009, 2009.
Bharali, C., Nair, V. S., Chutia, L., and Babu, S. S.: Modeling of the effects of
wintertime aerosols on boundary layer properties over the Indo Gangetic
Plain, J. Geophys. Res.-Atmos., 124, 4141–4157,
https://doi.org/10.1029/2018JD029758, 2019.
Burkart, J., Steiner, G., Reischl, G., and Hitzenberger, R.: Long-term study of
cloud condensation nuclei (CCN) activation of the atmospheric aerosol in
Vienna, Atmos. Environ., 45, 5751–5759, 2011.
Cantrell, W., Shaw, G., Leck, C., Granat, L., and Cachier, H.: Relationships
between cloud condensation nuclei spectra and aerosol particles on a
south-north transect of the Indian Ocean, J. Geophys. Res., 105, 15313–15320, 2000.
Cantrell, W., Shaw, G., Cass, G., Chowdhury, Z., Hughes, L., Prather, K.,
Guazzotti, S., and Coffee, K.: Closure between aerosol particles and cloud
condensation nuclei at Kaashidhoo Climate Observatory, J. Geophys. Res.,
106, 28711–28718, 2001.
Chylek, P., Dubey, M. K., Lohmann, U., Ramanathan, V., Kaufman, Y. J.,
Lesins, G., Hudson, J., Altmann, G., and Olsen, S. C.: Aerosol indirect
effect over the Indian Ocean, Geophys. Res. Lett., 33, L06806,
https://doi.org/10.1029/2005GL025397, 2006.
Dusek, U., Frank, G. P., Hildebrandt, L., Curtius, J., Schneider, J.,
Walter, S., Chand, D., Drewnick, F., Hings, S., Jung, D., Borrmann, S., and
Andreae, M. O.: Size matters more than chemistry for cloud-nucleating
ability of aerosol particles, Science, 312, 1375–1378, 2006a.
Dusek, U., Reischl, G. P., and Hitzenberger, R.: CCN Activation of Pure and
Coated Carbon Black Particles, Environ. Sci. Technol., 40,
1223–1230, 2006b.
Fang, S., Han, Y., Chen, K., Lu, C., Yin, Y., Tan, H., and Wang, J.:
Parameterization and comparative evaluation of the CCN number concentration
on Mt. Huang, China, Atmos. Res., 181, 300–311, 2016.
Furutani, H., Dall'osto, M., Roberts, G. C., and Prather, K. A.: Assessment
of the relative importance of atmospheric aging on CCN activity derived from
field observations, Atmos. Environ., 42, 3130–3142, 2008.
Gunthe, S. S., King, S. M., Rose, D., Chen, Q., Roldin, P., Farmer, D. K., Jimenez, J. L., Artaxo, P., Andreae, M. O., Martin, S. T., and Pöschl, U.: Cloud condensation nuclei in pristine tropical rainforest air of Amazonia: size-resolved measurements and modeling of atmospheric aerosol composition and CCN activity, Atmos. Chem. Phys., 9, 7551–7575, https://doi.org/10.5194/acp-9-7551-2009, 2009.
Hudson, J. G.: Variability of the relationship between particle size and
cloud-nucleating ability, Geophys. Res. Lett., 34, L08801,
https://doi.org/10.1029/2006GL028850, 2007.
Hudson, J. G. and Yum, S. S.: Cloud condensation nuclei spectra and
polluted and clean clouds over the Indian Ocean, J. Geophys. Res., 107,
8022, https://doi.org/10.1029/2001JD000829, 2002.
Hudson, J. G., Noble, S., and Tabor, S.: Cloud supersaturations from CCN
spectra Hoppel minima, J. Geophys. Res.-Atmos., 120,
3436–3452, https://doi.org/10.1002/2014JD022669, 2015.
IPCC: Climate Change 2013: The Physical Science Basis, in: Contribution of
Working Group I to the Fifth Assessment Report of the Intergovernmental
Panel on Climate Change, Cambridge University Press, Cambridge, UK and New
York, NY, USA, 2013.
Jayachandran, V., Nair, V. S., and Babu, S. S.: CCN characteristics over a
tropical coastal station during south-west monsoon: observations and closure
studies, Atmos. Environ. 164, 299–308,
https://doi.org/10.1016/j.atmosenv.2017.06.012, 2017.
Jayachandran, V., Nair, V. S., and Babu, S. S.: CCN activation properties at
a tropical hill station during south-west summer monsoon: Vertical
heterogeneity, Atmos. Res., 214, 36–45, https://doi.org/10.1016/j.atmosres.2018.07.018, 2018.
Jayachandran, V. N., Suresh Babu, S. N., Vaishya, A., Gogoi, M. M., Nair, V. S., Satheesh, S. K., and Krishna Moorthy, K.: Altitude profiles of cloud condensation nuclei characteristics across the Indo-Gangetic Plain prior to the onset of the Indian summer monsoon, Atmos. Chem. Phys., 20, 561–576, https://doi.org/10.5194/acp-20-561-2020, 2020.
Jefferson, A.: Empirical estimates of CCN from aerosol optical properties at four remote sites, Atmos. Chem. Phys., 10, 6855–6861, https://doi.org/10.5194/acp-10-6855-2010, 2010.
Jurányi, Z., Gysel, M., Weingartner, E., DeCarlo, P. F., Kammermann, L., and Baltensperger, U.: Measured and modelled cloud condensation nuclei number concentration at the high alpine site Jungfraujoch, Atmos. Chem. Phys., 10, 7891–7906, https://doi.org/10.5194/acp-10-7891-2010, 2010.
Kalivitis, N., Kerminen, V.-M., Kouvarakis, G., Stavroulas, I., Bougiatioti, A., Nenes, A., Manninen, H. E., Petäjä, T., Kulmala, M., and Mihalopoulos, N.: Atmospheric new particle formation as a source of CCN in the eastern Mediterranean marine boundary layer, Atmos. Chem. Phys., 15, 9203–9215, https://doi.org/10.5194/acp-15-9203-2015, 2015.
Kerminen, V.-M., Paramonov, M., Anttila, T., Riipinen, I., Fountoukis, C., Korhonen, H., Asmi, E., Laakso, L., Lihavainen, H., Swietlicki, E., Svenningsson, B., Asmi, A., Pandis, S. N., Kulmala, M., and Petäjä, T.: Cloud condensation nuclei production associated with atmospheric nucleation: a synthesis based on existing literature and new results, Atmos. Chem. Phys., 12, 12037–12059, https://doi.org/10.5194/acp-12-12037-2012, 2012.
Kim, J. H., Yum, S. S., Shim, S., Kim, W. J., Park, M., Kim, J.-H., Kim, M.-H., and Yoon, S.-C.: On the submicron aerosol distributions and CCN number concentrations in and around the Korean Peninsula, Atmos. Chem. Phys., 14, 8763–8779, https://doi.org/10.5194/acp-14-8763-2014, 2014.
Kim, N., Park, M., Yum, S. S., Park, J. S., Shin, H. J., and Ahn, J. Y.: Impact
of urban aerosol properties on cloud condensation nuclei (CCN) activity
during the KORUS-AQ field campaign, Atmos. Enviro., 185, 221–236,
2018.
Lelieveld, J., Crutzen, P. J., Ramanathan, V., Andreae, M. O.,
Brennikmeijer, C. A. M., Campos, T., Cass, G. R., Dickerson, R., Fischer,
H., De Gouw, J. A., Hansel, A., Jefferson, A., Kley, D., DeLaat, A. T. J.,
Lal, S., Lawrence, M. G., Lobert, J. M., Mayol-Bracero, O. L., Mitra, A. P.,
Novakov, T., Oltmans, S. J.,Prather, K. A., Rodhe, H., Scheeren, H. A.,
Sikka, D., and Williams, J.: The Indian Ocean Experiment: Widespread air
pollution from South and South East Asia, Science, 292, 1031–1036, 2001.
Li, Z., Lau, W. K.-M., Ramanathan, V., Wu, G., Ding, Y., Manoj, M. G., Liu, J., Qian, Y., Li, J., Zhou, T., Fan, J., Rosenfeld, D., Ming, Y., Wang, Y., Huang, J., Wang, B., Xu, X., Lee, S.-S., Cribb, M., Zhang, F., Yang, X., Zhao, C., Takemura, T., Wang, K., Xia, X., Yin, Y., Zhang, H., Guo, J., Zhai, P. M., Sugimoto, N., Babu, S. S., and Brasseur, G. P.: Aerosol and monsoon climate interactions
over Asia, Rev. Geophys., 54, 866–929, https://doi.org/10.1002/2015RG000500, 2016.
Mayol-Bracero, O. L., Gabriel, R., Andreae, M. O., Kirchstetter, T. W.,
Novakov, T., Ogren, J., Sheridan, P., and Streets, D. G.: Carbonaceous
aerosols over the Indian Ocean during the Indian Ocean Experiment (INDOEX):
Chemical characterization, optical properties, and probable sources, J.
Geophys. Res., 107, 8030, https://doi.org/10.1029/2000JD000039, 2002.
Meng, J. W., Yeung, M. C., Li, Y. J., Lee, B. Y. L., and Chan, C. K.: Size-resolved cloud condensation nuclei (CCN) activity and closure analysis at the HKUST Supersite in Hong Kong, Atmos. Chem. Phys., 14, 10267–10282, https://doi.org/10.5194/acp-14-10267-2014, 2014.
Merikanto, J., Spracklen, D. V., Mann, G. W., Pickering, S. J., and Carslaw, K. S.: Impact of nucleation on global CCN, Atmos. Chem. Phys., 9, 8601–8616, https://doi.org/10.5194/acp-9-8601-2009, 2009.
Moorthy K. K., Nair, V. S., Babu S. S., and Satheesh, S. K.: Spatial and
vertical heterogeneities of aerosol radiative forcing over the oceanic
regions surrounding the Indian peninsula: climate implications, Q.
J. Roy. Meteor. Soc., 135, 2131–2145, 2009.
Nair, V. S., Moorthy, K. K., Alappattu, D. P., Kunhikrishnan, P. K., George,
S. K., Nair, P. R., Babu, S. S., Abish, B., Satheesh, S. K., Tripathy, S.
N., Niranjan, K., Madhavan, B. L., Srikant, V., Dutt, C. B. S., Badarinath,
K. V. S., and Reddy, R. R.: Wintertime aerosol characteristics over the
Indo-Gangetic Plain (IGP): Impacts of local boundary layer processes and
long range transport, J. Geophys. Res.-Atmos., 112,
D13205, https://doi.org/10.1029/2006JD008099, 2007.
Nair, V. S., Moorthy, K. K., and Babu, S. S.: Influence of continental outflow
and ocean biogeochemistry on the distribution of fine and ultrafine particles
in the marine atmospheric boundary layer over Arabian Sea and Bay of Bengal,
J. Geophys. Res.-Atmos., 118, 7321–7337, https://doi.org/10.1002/jgrd.50541,
2013.
Noble, S. R. and Hudson, J. G.: Effects of continental clouds on surface
Aitken and accumulation modes, J. Geophys. Res.-Atmos.,
124, 5479–5502, https://doi.org/10.1029/2019JD030297, 2019.
Paramonov, M., Kerminen, V.-M., Gysel, M., Aalto, P. P., Andreae, M. O., Asmi, E., Baltensperger, U., Bougiatioti, A., Brus, D., Frank, G. P., Good, N., Gunthe, S. S., Hao, L., Irwin, M., Jaatinen, A., Jurányi, Z., King, S. M., Kortelainen, A., Kristensson, A., Lihavainen, H., Kulmala, M., Lohmann, U., Martin, S. T., McFiggans, G., Mihalopoulos, N., Nenes, A., O'Dowd, C. D., Ovadnevaite, J., Petäjä, T., Pöschl, U., Roberts, G. C., Rose, D., Svenningsson, B., Swietlicki, E., Weingartner, E., Whitehead, J., Wiedensohler, A., Wittbom, C., and Sierau, B.: A synthesis of cloud condensation nuclei counter (CCNC) measurements within the EUCAARI network, Atmos. Chem. Phys., 15, 12211–12229, https://doi.org/10.5194/acp-15-12211-2015, 2015.
Petters, M. D. and Kreidenweis, S. M.: A single parameter representation of hygroscopic growth and cloud condensation nucleus activity, Atmos. Chem. Phys., 7, 1961–1971, https://doi.org/10.5194/acp-7-1961-2007, 2007.
Pierce, J. R. and Adams, P. J.: Efficiency of cloud condensation nuclei formation from ultrafine particles, Atmos. Chem. Phys., 7, 1367–1379, https://doi.org/10.5194/acp-7-1367-2007, 2007.
Pöhlker, M. L., Pöhlker, C., Ditas, F., Klimach, T., Hrabe de Angelis, I., Araújo, A., Brito, J., Carbone, S., Cheng, Y., Chi, X., Ditz, R., Gunthe, S. S., Kesselmeier, J., Könemann, T., Lavrič, J. V., Martin, S. T., Mikhailov, E., Moran-Zuloaga, D., Rose, D., Saturno, J., Su, H., Thalman, R., Walter, D., Wang, J., Wolff, S., Barbosa, H. M. J., Artaxo, P., Andreae, M. O., and Pöschl, U.: Long-term observations of cloud condensation nuclei in the Amazon rain forest – Part 1: Aerosol size distribution, hygroscopicity, and new model parametrizations for CCN prediction, Atmos. Chem. Phys., 16, 15709–15740, https://doi.org/10.5194/acp-16-15709-2016, 2016.
Quinn, P. K., Bates, T. S., Coffman, D. J., and Covert, D. S.: Influence of particle size and chemistry on the cloud nucleating properties of aerosols, Atmos. Chem. Phys., 8, 1029–1042, https://doi.org/10.5194/acp-8-1029-2008, 2008.
Ramanathan, V., Crutzen, P. J., Lelieveld, J., Mitra, A. P., Althausen, D., Anderson, J., Andreae, M. O., Cantrell, W., Cass, G. R., Chung, C. E., Clarke, A. D., Coakley, J. A., Collins, W. D., Conant, W. C., Dulac, F., Heintzenberg, J., Heymsfield, A. J., Holben, B., Howell, S., Hudson, J., Jayaraman, A., Kiehl, J. T., Krishnamurti, T. N., Lubin, D., McFarquhar, G., Novakov, T., Ogren, J. A., Podgorny, I. A., Prather, K., Priestley, K., Prospero, J. M., Quinn, P. K., Rajeev, K., Rasch, P., Rupert, S., Sadourny, R., Satheesh, S. K., Shaw, G. E., Sheridan, P., and Valero, F. P. J.: Indian Ocean Experiment: an integrated analysis of
the climate forcing and effects of the great Indo-Asian haze, J. Geophys.
Res., 106, 28371–28398, 2001.
Reutter, P., Su, H., Trentmann, J., Simmel, M., Rose, D., Gunthe, S. S., Wernli, H., Andreae, M. O., and Pöschl, U.: Aerosol- and updraft-limited regimes of cloud droplet formation: influence of particle number, size and hygroscopicity on the activation of cloud condensation nuclei (CCN), Atmos. Chem. Phys., 9, 7067–7080, https://doi.org/10.5194/acp-9-7067-2009, 2009.
Roberts, G. C. and Nenes, A.: A continuous-flow streamwise thermal-gradient CCN
chamber for atmospheric measurements., Aerosol Sci. Tech., 39,
206–221, 2005.
Rose, D., Nowak, A., Achtert, P., Wiedensohler, A., Hu, M., Shao, M., Zhang, Y., Andreae, M. O., and Pöschl, U.: Cloud condensation nuclei in polluted air and biomass burning smoke near the mega-city Guangzhou, China – Part 1: Size-resolved measurements and implications for the modeling of aerosol particle hygroscopicity and CCN activity, Atmos. Chem. Phys., 10, 3365–3383, https://doi.org/10.5194/acp-10-3365-2010, 2010.
Rose, D., Gunthe, S. S., Su, H., Garland, R. M., Yang, H., Berghof, M., Cheng, Y. F., Wehner, B., Achtert, P., Nowak, A., Wiedensohler, A., Takegawa, N., Kondo, Y., Hu, M., Zhang, Y., Andreae, M. O., and Pöschl, U.: Cloud condensation nuclei in polluted air and biomass burning smoke near the mega-city Guangzhou, China – Part 2: Size-resolved aerosol chemical composition, diurnal cycles, and externally mixed weakly CCN-active soot particles, Atmos. Chem. Phys., 11, 2817–2836, https://doi.org/10.5194/acp-11-2817-2011, 2011.
Rosenfeld, D., Andreae, M. O., Asmi, A., Chin, M., de Leeuw, G., Donovan, D.
P., Kahn, R., Kinne, S., Kivekäs, N., Kulmala, M., Lau, W., Schmidt, S.,
Suni, T., Wagner, T., Wild, M., and Quaas, J.: Global observations of
aerosol–cloud– precipitation–climate interactions, Rev. Geophys., 52,
750–808, https://doi.org/10.1002/2013RG000441, 2014.
Schmale, J., Henning, S., Decesari, S., Henzing, B., Keskinen, H., Sellegri, K., Ovadnevaite, J., Pöhlker, M. L., Brito, J., Bougiatioti, A., Kristensson, A., Kalivitis, N., Stavroulas, I., Carbone, S., Jefferson, A., Park, M., Schlag, P., Iwamoto, Y., Aalto, P., Äijälä, M., Bukowiecki, N., Ehn, M., Frank, G., Fröhlich, R., Frumau, A., Herrmann, E., Herrmann, H., Holzinger, R., Kos, G., Kulmala, M., Mihalopoulos, N., Nenes, A., O'Dowd, C., Petäjä, T., Picard, D., Pöhlker, C., Pöschl, U., Poulain, L., Prévôt, A. S. H., Swietlicki, E., Andreae, M. O., Artaxo, P., Wiedensohler, A., Ogren, J., Matsuki, A., Yum, S. S., Stratmann, F., Baltensperger, U., and Gysel, M.: Long-term cloud condensation nuclei number concentration, particle number size distribution and chemical composition measurements at regionally representative observatories, Atmos. Chem. Phys., 18, 2853–2881, https://doi.org/10.5194/acp-18-2853-2018, 2018.
Snider, J. R. and Brenguier, J. L.: Cloud condensation nuclei and cloud
droplet measurements during ACE-2, Tellus, 52B, 828–842, 2000.
Ueda, S., Miura, K., Kawata, R., Furutani, H., Uematsu, M., Omori, Y., and
Tanimoto, H.: Number-size distribution of aerosol particles and new particle
formation events in tropical and subtropical Pacific Oceans, Atmos.
Environ., 142, 324–339, 2016.
Wang, S. C. and Flagan, R. C.: Scanning electrical mobility spectrometer, Aerosol
Sci. Tech., 13, 2230–2240, https://doi.org/10.1080/02786829008959441,
1990.
Yum, S. S., Roberts, G., Kim, J. H., Song, K., and Kim, D.: Submicron
aerosol size distributions and cloud condensation nuclei concentrations
measured at Gosan, Korea, during the Atmospheric Brown Clouds–East Asian
Regional Experiment 2005, J. Geophys. Res., 112, D22S32,
https://doi.org/10.1029/2006JD008212, 2007.
Short summary
Extensive measurements of the aerosol and cloud condensation nuclei (CCN) properties in South Asian outflow to the northern Indian Ocean were carried out as a part of the ICARB-2018 experiment during winter. At high supersaturations, most of the aerosols in the South Asian outflow become activated as CCN, whereas the aerosol system over the equatorial Indian Ocean is less CCN efficient even at higher supersaturations.
Extensive measurements of the aerosol and cloud condensation nuclei (CCN) properties in South...
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