Articles | Volume 19, issue 5
https://doi.org/10.5194/acp-19-2917-2019
https://doi.org/10.5194/acp-19-2917-2019
Research article
 | 
07 Mar 2019
Research article |  | 07 Mar 2019

Accounting for the effects of nonideal minor structures on the optical properties of black carbon aerosols

Shiwen Teng, Chao Liu, Martin Schnaiter, Rajan K. Chakrabarty, and Fengshan Liu

Related authors

Inversion algorithm of black carbon mixing state based on machine learning
Zeyuan Tian, Jiandong Wang, Jiaping Wang, Chao Liu, Jia Xing, Jinbo Wang, Zhouyang Zhang, Yuzhi Jin, Sunan Shen, Bin Wang, Wei Nie, Xin Huang, and Aijun Ding
Atmos. Meas. Tech., 18, 1149–1162, https://doi.org/10.5194/amt-18-1149-2025,https://doi.org/10.5194/amt-18-1149-2025, 2025
Short summary
Accounting for the black carbon aging process in a two-way coupled meteorology–air quality model
Yuzhi Jin, Jiandong Wang, Chao Liu, David C. Wong, Golam Sarwar, Kathleen M. Fahey, Shang Wu, Jiaping Wang, Jing Cai, Zeyuan Tian, Zhouyang Zhang, Jia Xing, Aijun Ding, and Shuxiao Wang
Atmos. Chem. Phys., 25, 2613–2630, https://doi.org/10.5194/acp-25-2613-2025,https://doi.org/10.5194/acp-25-2613-2025, 2025
Short summary
Steady-state mixing state of black carbon aerosols from a particle-resolved model
Zhouyang Zhang, Jiandong Wang, Jiaping Wang, Nicole Riemer, Chao Liu, Yuzhi Jin, Zeyuan Tian, Jing Cai, Yueyue Cheng, Ganzhen Chen, Bin Wang, Shuxiao Wang, and Aijun Ding
Atmos. Chem. Phys., 25, 1869–1881, https://doi.org/10.5194/acp-25-1869-2025,https://doi.org/10.5194/acp-25-1869-2025, 2025
Short summary
Optimal estimation of cloud properties from thermal infrared observations with a combination of deep learning and radiative transfer simulation
He Huang, Quan Wang, Chao Liu, and Chen Zhou
Atmos. Meas. Tech., 17, 7129–7141, https://doi.org/10.5194/amt-17-7129-2024,https://doi.org/10.5194/amt-17-7129-2024, 2024
Short summary
A revised ocean mixed layer model for better simulating the diurnal variation in ocean skin temperature
Eui-Jong Kang, Byung-Ju Sohn, Sang-Woo Kim, Wonho Kim, Young-Cheol Kwon, Seung-Bum Kim, Hyoung-Wook Chun, and Chao Liu
Geosci. Model Dev., 17, 8553–8568, https://doi.org/10.5194/gmd-17-8553-2024,https://doi.org/10.5194/gmd-17-8553-2024, 2024
Short summary

Related subject area

Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Characterization of brown carbon absorption in different European environments through source contribution analysis
Hector Navarro-Barboza, Jordi Rovira, Vincenzo Obiso, Andrea Pozzer, Marta Via, Andres Alastuey, Xavier Querol, Noemi Perez, Marjan Savadkoohi, Gang Chen, Jesus Yus-Díez, Matic Ivancic, Martin Rigler, Konstantinos Eleftheriadis, Stergios Vratolis, Olga Zografou, Maria Gini, Benjamin Chazeau, Nicolas Marchand, Andre S. H. Prevot, Kaspar Dallenbach, Mikael Ehn, Krista Luoma, Tuukka Petäjä, Anna Tobler, Jaroslaw Necki, Minna Aurela, Hilkka Timonen, Jarkko Niemi, Olivier Favez, Jean-Eudes Petit, Jean-Philippe Putaud, Christoph Hueglin, Nicolas Pascal, Aurélien Chauvigné, Sébastien Conil, Marco Pandolfi, and Oriol Jorba
Atmos. Chem. Phys., 25, 2667–2694, https://doi.org/10.5194/acp-25-2667-2025,https://doi.org/10.5194/acp-25-2667-2025, 2025
Short summary
Accounting for the black carbon aging process in a two-way coupled meteorology–air quality model
Yuzhi Jin, Jiandong Wang, Chao Liu, David C. Wong, Golam Sarwar, Kathleen M. Fahey, Shang Wu, Jiaping Wang, Jing Cai, Zeyuan Tian, Zhouyang Zhang, Jia Xing, Aijun Ding, and Shuxiao Wang
Atmos. Chem. Phys., 25, 2613–2630, https://doi.org/10.5194/acp-25-2613-2025,https://doi.org/10.5194/acp-25-2613-2025, 2025
Short summary
The effectiveness of solar radiation management using fine sea spray across multiple climatic regions
Zhe Song, Shaocai Yu, Pengfei Li, Ningning Yao, Lang Chen, Yuhai Sun, Boqiong Jiang, and Daniel Rosenfeld
Atmos. Chem. Phys., 25, 2473–2494, https://doi.org/10.5194/acp-25-2473-2025,https://doi.org/10.5194/acp-25-2473-2025, 2025
Short summary
A global dust emission dataset for estimating dust radiative forcings in climate models
Danny M. Leung, Jasper F. Kok, Longlei Li, David M. Lawrence, Natalie M. Mahowald, Simone Tilmes, and Erik Kluzek
Atmos. Chem. Phys., 25, 2311–2331, https://doi.org/10.5194/acp-25-2311-2025,https://doi.org/10.5194/acp-25-2311-2025, 2025
Short summary
Tropospheric aerosols over the western North Atlantic Ocean during the winter and summer deployments of ACTIVATE 2020: life cycle, transport, and distribution
Hongyu Liu, Bo Zhang, Richard H. Moore, Luke D. Ziemba, Richard A. Ferrare, Hyundeok Choi, Armin Sorooshian, David Painemal, Hailong Wang, Michael A. Shook, Amy Jo Scarino, Johnathan W. Hair, Ewan C. Crosbie, Marta A. Fenn, Taylor J. Shingler, Chris A. Hostetler, Gao Chen, Mary M. Kleb, Gan Luo, Fangqun Yu, Mark A. Vaughan, Yongxiang Hu, Glenn S. Diskin, John B. Nowak, Joshua P. DiGangi, Yonghoon Choi, Christoph A. Keller, and Matthew S. Johnson
Atmos. Chem. Phys., 25, 2087–2121, https://doi.org/10.5194/acp-25-2087-2025,https://doi.org/10.5194/acp-25-2087-2025, 2025
Short summary

Cited articles

Alexander, D. T. L., Crozier, P. A., and Anderson, J. R.: Brown carbon spheres in East Asian outflow and their optical properties, Science, 321, 833–836, 2008. 
Andreae, M. O. and Gelencsér, A.: Black carbon or brown carbon? The nature of light-absorbing carbonaceous aerosols, Atmos. Chem. Phys., 6, 3131–3148, https://doi.org/10.5194/acp-6-3131-2006, 2006. 
Bescond, A., Yon, J., Girasole, T., Jouen, C., Rozé, C., and Coppalle, A.: Numerical investigation of the possibility to determine the primary particle size of fractal aggregates by measuring light depolarization, J. Quant. Spectrosc. Ra., 126, 130–139, 2013. 
Bescond, A., Yon, J., Ouf, F. X., Ferry, D., Delhaye, D., Gaffié, D., Coppalle, A., and Rozé, C.: Automated determination of aggregate primary particle size distribution by TEM image analysis: Application to soot, Aerosol Sci. Tech., 48, 831–841, 2014. 
Bond, T. C. and Bergstrom, R. W.: Light absorption by carbonaceous particles: An investigative review, Aerosol Sci. Tech., 40, 27–67, 2006. 
Download
Short summary
Black carbon (BC) possesses complex minor structures besides the overall aggregate geometry, thus altering their optical properties. This study introduces volume variation to quantify and unify different minor structures and develops an empirical relation to account for their effects on BC optical properties. We find the effects of minor structures are mainly contributed by their influence on particle volume/mass, and a relative difference of 5 % is noticed after removing volume differences.
Share
Altmetrics
Final-revised paper
Preprint