Accounting for the effects of nonideal minor structures on the optical properties of black carbon aerosols
Shiwen Teng,Chao Liu,Martin Schnaiter,Rajan K. Chakrabarty,and Fengshan Liu
Shiwen Teng
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Nanjing University of Information Science &
Technology, Nanjing 210044, China
Key Laboratory for Aerosol-Cloud-Precipitation of the China Meteorological
Administration, School of Atmospheric Physics, Nanjing University of
Information Science & Technology, Nanjing 210044, China
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Nanjing University of Information Science &
Technology, Nanjing 210044, China
Key Laboratory for Aerosol-Cloud-Precipitation of the China Meteorological
Administration, School of Atmospheric Physics, Nanjing University of
Information Science & Technology, Nanjing 210044, China
Center for Aerosol Science and Engineering, Department of Energy,
Environmental and Chemical Engineering, Washington University in St. Louis, St. Louis,
Missouri 63130, USA
Fengshan Liu
Black Carbon Metrology, Measurement Science and Standards, National
Research Council, Ottawa, Ontario K1A 0R6, Canada
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Black carbon (BC) possesses complex minor structures besides the overall aggregate geometry, thus altering their optical properties. This study introduces volume variation to quantify and unify different minor structures and develops an empirical relation to account for their effects on BC optical properties. We find the effects of minor structures are mainly contributed by their influence on particle volume/mass, and a relative difference of 5 % is noticed after removing volume differences.
Black carbon (BC) possesses complex minor structures besides the overall aggregate geometry,...