Articles | Volume 26, issue 1
https://doi.org/10.5194/acp-26-155-2026
© Author(s) 2026. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-26-155-2026
© Author(s) 2026. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Measurement report
| 
06 Jan 2026
Measurement report |
| 06 Jan 2026
| 06 Jan 2026
Measurement report: Lessons learned from the comparison and combination of fine carbonaceous aerosol source apportionment at two locations in the city of Strasbourg, France
Hasna Chebaicheb
CORRESPONDING AUTHOR
IMT Nord Europe, Institut Mines-Télécom, Université de Lille, Centre for Energy and Environment,59000, Lille, France
Institut National de l'environnement Industriel et des Risques (INERIS), 60550 Verneuil-en-Halatte, France
Laboratoire Central de Surveillance de la Qualité de l'Air (LCSQA), 60550 Verneuil-en-Halatte, France
Mélodie Chatain
CORRESPONDING AUTHOR
Atmo Grand Est, 67300 Schiltigheim, France
Olivier Favez
Institut National de l'environnement Industriel et des Risques (INERIS), 60550 Verneuil-en-Halatte, France
Laboratoire Central de Surveillance de la Qualité de l'Air (LCSQA), 60550 Verneuil-en-Halatte, France
Joel F. de Brito
IMT Nord Europe, Institut Mines-Télécom, Université de Lille, Centre for Energy and Environment,59000, Lille, France
Vincent Crenn
ADDAIR, 78530 Buc, France
Tanguy Amodeo
Institut National de l'environnement Industriel et des Risques (INERIS), 60550 Verneuil-en-Halatte, France
Laboratoire Central de Surveillance de la Qualité de l'Air (LCSQA), 60550 Verneuil-en-Halatte, France
Mohamed Gherras
Institut National de l'environnement Industriel et des Risques (INERIS), 60550 Verneuil-en-Halatte, France
Emmanuel Jantzem
Atmo Grand Est, 67300 Schiltigheim, France
Caroline Marchand
Institut National de l'environnement Industriel et des Risques (INERIS), 60550 Verneuil-en-Halatte, France
Laboratoire Central de Surveillance de la Qualité de l'Air (LCSQA), 60550 Verneuil-en-Halatte, France
Véronique Riffault
IMT Nord Europe, Institut Mines-Télécom, Université de Lille, Centre for Energy and Environment,59000, Lille, France
Laboratoire Central de Surveillance de la Qualité de l'Air (LCSQA), 60550 Verneuil-en-Halatte, France
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Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2026-490, https://doi.org/10.5194/essd-2026-490, 2026
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This work proposes a new methodology for robust, homogeneous processing of long-term datasets of aerosol mass spectrometer measurements to remedy the challenges posed by the emergence of juxtaposed data processing periods over the years. The results showed a global decrease in PM1 at a semi-urban site in the Paris region between 2011 and 2024, along with a decrease in the frequency of persistent pollution episodes. Finally, it highlights the need for Sulfate source apportionment analysis.
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Wenche Aas, Thérèse Salameh, Robert Wegener, Heidi Hellén, Jean-Luc Jaffrezo, Pontus Roldin, Elisabeth Alonso-Blanco, Andres Alastuey, Crist Amelynck, Jgor Arduini, Benjamin Bergmans, Marie Bertrand, Agnes Borbon, Efstratios Bourtsoukidis, Laetitia Bouvier, David Butterfield, Iris Buxbaum, Darius Ceburnis, Anja Claude, Augustin Colette, Aurélie Colomb, Sophie Darfeuil, James Dernie, Maximilien Desservettaz, Elías Díaz-Ramiro, Marvin Dufresne, René Dubus, Mario Duval, Marie Dury, Anna Font, Kirsten N. Fossum, Evelyn Freney, Gotzon Gangoiti, Yao Ge, Maria Carmen Gomez, Francisco J. Gómez-Moreno, Marie Gohy, Valérie Gros, Paul Hamer, Bryan Hellack, Hartmut Herrmann, Robert Holla, Adéla Holubová, Niels R. Jensen, Tuija Jokinen, Matthew Jones, Uwe Käfer, Lukas Kesper, Dieter Klemp, Dagmar Kubistin, Angela Marinoni, Martina Mazzini, Vy Ngoc Thuy Dinh, Jurgita Ovadnevaite, Tuukka Petäjä, Miguel Portillo-Estrada, Jitka Přívozníková, Jean-Philippe Putaud, Stefan Reimann, Laura Renzi, Veronique Riffault, Stuart Ritchie, Chris Robins, Begoña Artíñano Rodríguez de Torres, Laurent Poulain, Julian Rüdiger, Agnieszka Sanocka, Estibaliz Saez de Camara Oleaga, Niels Schoon, Roger Seco, Ivan Simmons, Leïla Simon, David Simpson, Sverre Solberg, Emmanuel Tison, August Thomasson, Svetlana Tsyro, Marsailidh Twigg, Toni Tykkä, Bert Verreyken, Ågot Watne, Katie Williams, Ana Maria Yáñez-Serrano, Karen Yeung, Ilona Ylivinkka, and Karl Espen Yttri
Atmos. Chem. Phys., 26, 8717–8751, https://doi.org/10.5194/acp-26-8717-2026, https://doi.org/10.5194/acp-26-8717-2026, 2026
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Atmos. Meas. Tech., 18, 7629–7649, https://doi.org/10.5194/amt-18-7629-2025, https://doi.org/10.5194/amt-18-7629-2025, 2025
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Vy Ngoc Thuy Dinh, Gaëlle Uzu, Pamela Dominutti, Stéphane Sauvage, Rhabira Elazzouzi, Sophie Darfeuil, Céline Voiron, Abdoulaye Samaké, Shouwen Zhang, Stéphane Socquet, Olivier Favez, and Jean-Luc Jaffrezo
Atmos. Meas. Tech., 18, 6817–6833, https://doi.org/10.5194/amt-18-6817-2025, https://doi.org/10.5194/amt-18-6817-2025, 2025
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Atmos. Chem. Phys., 25, 12409–12431, https://doi.org/10.5194/acp-25-12409-2025, https://doi.org/10.5194/acp-25-12409-2025, 2025
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Atmos. Chem. Phys., 25, 9451–9469, https://doi.org/10.5194/acp-25-9451-2025, https://doi.org/10.5194/acp-25-9451-2025, 2025
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Atmos. Chem. Phys., 25, 8163–8183, https://doi.org/10.5194/acp-25-8163-2025, https://doi.org/10.5194/acp-25-8163-2025, 2025
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Polycyclic aromatic hydrocarbons (PAHs), emitted from incomplete combustion, pose serious health risks due to their carcinogenic properties. This research demonstrates that viscous organic aerosol coatings significantly hinder PAH oxidation, with spatial distributions sensitive to the degradation modeling approach. Our findings emphasize the need for accurate modeling of PAH oxidation processes in risk assessments, considering both fresh and oxidized PAHs in evaluating human health risks.
Qingxiao Meng, Yunjiang Zhang, Sheng Zhong, Jie Fang, Lili Tang, Yongcai Rao, Minfeng Zhou, Jian Qiu, Xiaofeng Xu, Jean-Eudes Petit, Olivier Favez, and Xinlei Ge
Atmos. Chem. Phys., 25, 7485–7498, https://doi.org/10.5194/acp-25-7485-2025, https://doi.org/10.5194/acp-25-7485-2025, 2025
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We developed a machine-learning-based method to reconstruct missing elemental carbon (EC) data in four Chinese cities from 2013 to 2023. Using machine learning, we filled data gaps and introduced a new approach to analyze EC trends. Our findings reveal a significant decline in EC due to stricter pollution controls, though this slowed after 2020. This study provides a versatile framework for addressing data gaps and supports strategies to reduce urban air pollution and its climate impacts.
Diana L. Pereira, Chiara Giorio, Aline Gratien, Alexander Zherebker, Gael Noyalet, Servanne Chevaillier, Stéphanie Alage, Elie Almarj, Antonin Bergé, Thomas Bertin, Mathieu Cazaunau, Patrice Coll, Ludovico Di Antonio, Sergio Harb, Johannes Heuser, Cécile Gaimoz, Oscar Guillemant, Brigitte Language, Olivier Lauret, Camilo Macias, Franck Maisonneuve, Bénédicte Picquet-Varrault, Raquel Torres, Sylvain Triquet, Pascal Zapf, Lelia Hawkins, Drew Pronovost, Sydney Riley, Pierre-Marie Flaud, Emilie Perraudin, Pauline Pouyes, Eric Villenave, Alexandre Albinet, Olivier Favez, Robin Aujay-Plouzeau, Vincent Michoud, Christopher Cantrell, Manuela Cirtog, Claudia Di Biagio, Jean-François Doussin, and Paola Formenti
Atmos. Chem. Phys., 25, 4885–4905, https://doi.org/10.5194/acp-25-4885-2025, https://doi.org/10.5194/acp-25-4885-2025, 2025
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In order to study aerosols in environments influenced by anthropogenic and biogenic emissions, we performed analyses of samples collected during the ACROSS (Atmospheric Chemistry Of the Suburban Forest) campaign in summer 2022 in the greater Paris area. After analysis of the chemical composition by means of total carbon determination and high-resolution mass spectrometry, this work highlights the influence of anthropogenic inputs on the chemical composition of both urban and forested areas.
Ludovico Di Antonio, Matthias Beekmann, Guillaume Siour, Vincent Michoud, Christopher Cantrell, Astrid Bauville, Antonin Bergé, Mathieu Cazaunau, Servanne Chevaillier, Manuela Cirtog, Joel F. de Brito, Paola Formenti, Cecile Gaimoz, Olivier Garret, Aline Gratien, Valérie Gros, Martial Haeffelin, Lelia N. Hawkins, Simone Kotthaus, Gael Noyalet, Diana L. Pereira, Jean-Eudes Petit, Eva Drew Pronovost, Véronique Riffault, Chenjie Yu, Gilles Foret, Jean-François Doussin, and Claudia Di Biagio
Atmos. Chem. Phys., 25, 4803–4831, https://doi.org/10.5194/acp-25-4803-2025, https://doi.org/10.5194/acp-25-4803-2025, 2025
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The summer of 2022 has been considered a proxy for future climate scenarios due to its hot and dry conditions. In this paper, we use the measurements from the Atmospheric Chemistry of the Suburban Forest (ACROSS) campaign, conducted in the Paris area in June–July 2022, along with observations from existing networks, to evaluate a 3D chemistry transport model (WRF–CHIMERE) simulation. Results are shown to be satisfactory, allowing us to explain the gas and aerosol variability at the campaign sites.
Soo-Jin Park, Lya Lugon, Oscar Jacquot, Youngseob Kim, Alexia Baudic, Barbara D'Anna, Ludovico Di Antonio, Claudia Di Biagio, Fabrice Dugay, Olivier Favez, Véronique Ghersi, Aline Gratien, Julien Kammer, Jean-Eudes Petit, Olivier Sanchez, Myrto Valari, Jérémy Vigneron, and Karine Sartelet
Atmos. Chem. Phys., 25, 3363–3387, https://doi.org/10.5194/acp-25-3363-2025, https://doi.org/10.5194/acp-25-3363-2025, 2025
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To accurately represent the population exposure to outdoor concentrations of pollutants of interest to health (NO2, PM2.5, black carbon, and ultrafine particles), multi-scale modelling down to the street scale is set up and evaluated using measurements from field campaigns. An exposure scaling factor is defined, allowing regional-scale simulations to be corrected to evaluate population exposure. Urban heterogeneities strongly influence NO2, black carbon, and ultrafine particles but less strongly PM2.5.
Ludovico Di Antonio, Claudia Di Biagio, Paola Formenti, Aline Gratien, Vincent Michoud, Christopher Cantrell, Astrid Bauville, Antonin Bergé, Mathieu Cazaunau, Servanne Chevaillier, Manuela Cirtog, Patrice Coll, Barbara D'Anna, Joel F. de Brito, David O. De Haan, Juliette R. Dignum, Shravan Deshmukh, Olivier Favez, Pierre-Marie Flaud, Cecile Gaimoz, Lelia N. Hawkins, Julien Kammer, Brigitte Language, Franck Maisonneuve, Griša Močnik, Emilie Perraudin, Jean-Eudes Petit, Prodip Acharja, Laurent Poulain, Pauline Pouyes, Eva Drew Pronovost, Véronique Riffault, Kanuri I. Roundtree, Marwa Shahin, Guillaume Siour, Eric Villenave, Pascal Zapf, Gilles Foret, Jean-François Doussin, and Matthias Beekmann
Atmos. Chem. Phys., 25, 3161–3189, https://doi.org/10.5194/acp-25-3161-2025, https://doi.org/10.5194/acp-25-3161-2025, 2025
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The spectral complex refractive index (CRI) and single scattering albedo were retrieved from submicron aerosol measurements at three sites within the greater Paris area during the ACROSS field campaign (June–July 2022). Measurements revealed urban emission impact on surrounding areas. CRI full period averages at 520 nm were 1.41 – 0.037i (urban), 1.52 – 0.038i (peri-urban), and 1.50 – 0.025i (rural). Organic aerosols dominated the aerosol mass and contributed up to 22 % of absorption at 370 nm.
Hector Navarro-Barboza, Jordi Rovira, Vincenzo Obiso, Andrea Pozzer, Marta Via, Andres Alastuey, Xavier Querol, Noemi Perez, Marjan Savadkoohi, Gang Chen, Jesus Yus-Díez, Matic Ivancic, Martin Rigler, Konstantinos Eleftheriadis, Stergios Vratolis, Olga Zografou, Maria Gini, Benjamin Chazeau, Nicolas Marchand, Andre S. H. Prevot, Kaspar Dallenbach, Mikael Ehn, Krista Luoma, Tuukka Petäjä, Anna Tobler, Jaroslaw Necki, Minna Aurela, Hilkka Timonen, Jarkko Niemi, Olivier Favez, Jean-Eudes Petit, Jean-Philippe Putaud, Christoph Hueglin, Nicolas Pascal, Aurélien Chauvigné, Sébastien Conil, Marco Pandolfi, and Oriol Jorba
Atmos. Chem. Phys., 25, 2667–2694, https://doi.org/10.5194/acp-25-2667-2025, https://doi.org/10.5194/acp-25-2667-2025, 2025
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Brown carbon (BrC) absorbs ultraviolet (UV) and visible light, influencing climate. This study explores BrC's imaginary refractive index (k) using data from 12 European sites. Residential emissions are a major organic aerosol (OA) source in winter, while secondary organic aerosol (SOA) dominates in summer. Source-specific k values were derived, improving model accuracy. The findings highlight BrC's climate impact and emphasize source-specific constraints in atmospheric models.
Gabriel Chesnoiu, Isabelle Chiapello, Nicolas Ferlay, Pierre Nabat, Marc Mallet, and Véronique Riffault
Atmos. Chem. Phys., 25, 1307–1331, https://doi.org/10.5194/acp-25-1307-2025, https://doi.org/10.5194/acp-25-1307-2025, 2025
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The ALADIN regional climate model at 12.5 km resolution allows us to study the evolution of surface solar radiation (SSR) and key associated atmospheric parameters. Over northern France and Benelux, influenced by anthropogenic aerosols and cloudy conditions, regional evaluation of recent hindcast simulations shows satisfying results and high spatial variability. Future SSR evolution by the end of the century for two contrasting CMIP6 scenarios highlights large decreases in SSR for SSP3-7.0.
Shravan Deshmukh, Laurent Poulain, Birgit Wehner, Silvia Henning, Jean-Eudes Petit, Pauline Fombelle, Olivier Favez, Hartmut Herrmann, and Mira Pöhlker
Atmos. Chem. Phys., 25, 741–758, https://doi.org/10.5194/acp-25-741-2025, https://doi.org/10.5194/acp-25-741-2025, 2025
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Aerosol hygroscopicity has been investigated at a sub-urban site in Paris; analysis shows the sub-saturated regime's measured hygroscopicity and the chemically derived hygroscopic growth, shedding light on the large effect of external particle mixing and its influence on predicting hygroscopicity.
Hasna Chebaicheb, Joel F. de Brito, Tanguy Amodeo, Florian Couvidat, Jean-Eudes Petit, Emmanuel Tison, Gregory Abbou, Alexia Baudic, Mélodie Chatain, Benjamin Chazeau, Nicolas Marchand, Raphaële Falhun, Florie Francony, Cyril Ratier, Didier Grenier, Romain Vidaud, Shouwen Zhang, Gregory Gille, Laurent Meunier, Caroline Marchand, Véronique Riffault, and Olivier Favez
Earth Syst. Sci. Data, 16, 5089–5109, https://doi.org/10.5194/essd-16-5089-2024, https://doi.org/10.5194/essd-16-5089-2024, 2024
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Long-term (2015–2021) quasi-continuous measurements have been obtained at 13 French urban sites using online mass spectrometry, to acquire the comprehensive chemical composition of submicron particulate matter. The results show their spatial and temporal differences and confirm the predominance of organics in France (40–60 %). These measurements can be used for many future studies, such as trend and epidemiological analyses, or comparisons with chemical transport models.
Matthieu Vida, Gilles Foret, Guillaume Siour, Florian Couvidat, Olivier Favez, Gaelle Uzu, Arineh Cholakian, Sébastien Conil, Matthias Beekmann, and Jean-Luc Jaffrezo
Atmos. Chem. Phys., 24, 10601–10615, https://doi.org/10.5194/acp-24-10601-2024, https://doi.org/10.5194/acp-24-10601-2024, 2024
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We simulate 2 years of atmospheric fungal spores over France and use observations of polyols and primary biogenic factors from positive matrix factorisation. The representation of emissions taking into account a proxy for vegetation surface and specific humidity enables us to reproduce very accurately the seasonal cycle of fungal spores. Furthermore, we estimate that fungal spores can account for 20 % of PM10 and 40 % of the organic fraction of PM10 over vegetated areas in summer.
Vy Dinh Ngoc Thuy, Jean-Luc Jaffrezo, Ian Hough, Pamela A. Dominutti, Guillaume Salque Moreton, Grégory Gille, Florie Francony, Arabelle Patron-Anquez, Olivier Favez, and Gaëlle Uzu
Atmos. Chem. Phys., 24, 7261–7282, https://doi.org/10.5194/acp-24-7261-2024, https://doi.org/10.5194/acp-24-7261-2024, 2024
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The capacity of particulate matter (PM) to generate reactive oxygen species in vivo is represented by oxidative potential (OP). This study focuses on finding the appropriate model to evaluate the oxidative character of PM sources in six sites using the PM sources and OP. Eight regression techniques are introduced to assess the OP of PM. The study highlights the importance of selecting a model according to the input data characteristics and establishes some recommendations for the procedure.
Alejandra Velazquez-Garcia, Joel F. de Brito, Suzanne Crumeyrolle, Isabelle Chiapello, and Véronique Riffault
Aerosol Research, 2, 107–122, https://doi.org/10.5194/ar-2-107-2024, https://doi.org/10.5194/ar-2-107-2024, 2024
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Multi-annual in situ observations were combined with back trajectory and emissions inventories to study black and brown carbon (BC, BrC) sources in the north of France. Results show BC to be mainly originated from vehicular traffic (31 %), shipping (25 %), and residential heating (21 %). Also, a significant decrease of the BrC component from residential heating is observed after 24 h of atmospheric aging. These results should lead to better climate and air pollution mitigation strategies.
Abd El Rahman El Mais, Barbara D'Anna, Luka Drinovec, Andrew T. Lambe, Zhe Peng, Jean-Eudes Petit, Olivier Favez, Selim Aït-Aïssa, and Alexandre Albinet
Atmos. Chem. Phys., 23, 15077–15096, https://doi.org/10.5194/acp-23-15077-2023, https://doi.org/10.5194/acp-23-15077-2023, 2023
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Polycyclic aromatic hydrocarbons (PAHS) and furans are key precursors of secondary organic aerosols (SOAs) related to biomass burning emissions. We evaluated and compared the formation yields, and the physical and light absorption properties, of laboratory-generated SOAs from the oxidation of such compounds for both, day- and nighttime reactivities. The results illustrate that PAHs are large SOA precursors and may contribute significantly to the biomass burning brown carbon in the atmosphere.
Jean-Philippe Putaud, Enrico Pisoni, Alexander Mangold, Christoph Hueglin, Jean Sciare, Michael Pikridas, Chrysanthos Savvides, Jakub Ondracek, Saliou Mbengue, Alfred Wiedensohler, Kay Weinhold, Maik Merkel, Laurent Poulain, Dominik van Pinxteren, Hartmut Herrmann, Andreas Massling, Claus Nordstroem, Andrés Alastuey, Cristina Reche, Noemí Pérez, Sonia Castillo, Mar Sorribas, Jose Antonio Adame, Tuukka Petaja, Katrianne Lehtipalo, Jarkko Niemi, Véronique Riffault, Joel F. de Brito, Augustin Colette, Olivier Favez, Jean-Eudes Petit, Valérie Gros, Maria I. Gini, Stergios Vratolis, Konstantinos Eleftheriadis, Evangelia Diapouli, Hugo Denier van der Gon, Karl Espen Yttri, and Wenche Aas
Atmos. Chem. Phys., 23, 10145–10161, https://doi.org/10.5194/acp-23-10145-2023, https://doi.org/10.5194/acp-23-10145-2023, 2023
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Many European people are still exposed to levels of air pollution that can affect their health. COVID-19 lockdowns in 2020 were used to assess the impact of the reduction in human mobility on air pollution across Europe by comparing measurement data with values that would be expected if no lockdown had occurred. We show that lockdown measures did not lead to consistent decreases in the concentrations of fine particulate matter suspended in the air, and we investigate why.
Frédéric Ledoux, Cloé Roche, Gilles Delmaire, Gilles Roussel, Olivier Favez, Marc Fadel, and Dominique Courcot
Atmos. Chem. Phys., 23, 8607–8622, https://doi.org/10.5194/acp-23-8607-2023, https://doi.org/10.5194/acp-23-8607-2023, 2023
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We quantify the emissions from the marine sector in northern France, whether from natural or human-made sources. Therefore, a 1-year PM10 sampling campaign was conducted at a French coastal site. Results showed that sea salts contributed 37 %, while secondary nitrate and sulfate contributed 42 %, biomass burning 8 %, and heavy-fuel-oil combustion from shipping emissions 5 %. Sources contributing more than 80 % of PM10 are of regional and/or long-range origin.
Leïla Simon, Valérie Gros, Jean-Eudes Petit, François Truong, Roland Sarda-Estève, Carmen Kalalian, Alexia Baudic, Caroline Marchand, and Olivier Favez
Earth Syst. Sci. Data, 15, 1947–1968, https://doi.org/10.5194/essd-15-1947-2023, https://doi.org/10.5194/essd-15-1947-2023, 2023
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Long-term measurements of volatile organic compounds (VOCs) have been set up to better characterize the atmospheric chemistry at the SIRTA national facility (Paris area, France). Results obtained from the first 2 years (2020–2021) confirm the importance of local sources for short-lived compounds and the role played by meteorology and air mass origins in the long-term analysis of VOCs. They also point to a substantial influence of anthropogenic on the monoterpene loadings.
Suzanne Crumeyrolle, Jenni S. S. Kontkanen, Clémence Rose, Alejandra Velazquez Garcia, Eric Bourrianne, Maxime Catalfamo, Véronique Riffault, Emmanuel Tison, Joel Ferreira de Brito, Nicolas Visez, Nicolas Ferlay, Frédérique Auriol, and Isabelle Chiapello
Atmos. Chem. Phys., 23, 183–201, https://doi.org/10.5194/acp-23-183-2023, https://doi.org/10.5194/acp-23-183-2023, 2023
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Ultrafine particles (UFPs) are particles with an aerodynamic diameter of 100 nm or less and negligible mass concentration but are the dominant contributor to the total particle number concentration. The present study aims to better understand the environmental factors favoring or inhibiting atmospheric new particle formation (NPF) over Lille, a large city in the north of France, and to analyze the impact of such an event on urban air quality using a long-term dataset (3 years).
Marta Via, Gang Chen, Francesco Canonaco, Kaspar R. Daellenbach, Benjamin Chazeau, Hasna Chebaicheb, Jianhui Jiang, Hannes Keernik, Chunshui Lin, Nicolas Marchand, Cristina Marin, Colin O'Dowd, Jurgita Ovadnevaite, Jean-Eudes Petit, Michael Pikridas, Véronique Riffault, Jean Sciare, Jay G. Slowik, Leïla Simon, Jeni Vasilescu, Yunjiang Zhang, Olivier Favez, André S. H. Prévôt, Andrés Alastuey, and María Cruz Minguillón
Atmos. Meas. Tech., 15, 5479–5495, https://doi.org/10.5194/amt-15-5479-2022, https://doi.org/10.5194/amt-15-5479-2022, 2022
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This work presents the differences resulting from two techniques (rolling and seasonal) of the positive matrix factorisation model that can be run for organic aerosol source apportionment. The current state of the art suggests that the rolling technique is more accurate, but no proof of its effectiveness has been provided yet. This paper tackles this issue in the context of a synthetic dataset and a multi-site real-world comparison.
Lucille Joanna Borlaza, Samuël Weber, Anouk Marsal, Gaëlle Uzu, Véronique Jacob, Jean-Luc Besombes, Mélodie Chatain, Sébastien Conil, and Jean-Luc Jaffrezo
Atmos. Chem. Phys., 22, 8701–8723, https://doi.org/10.5194/acp-22-8701-2022, https://doi.org/10.5194/acp-22-8701-2022, 2022
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A 9-year dataset of the chemical and oxidative potential (OP) of PM10 was investigated at a rural background site. Extensive source apportionment led to identification of differences in source impacts between mass and OP, underlining the importance of PM redox activity when considering health effects. The influence of mixing and ageing processes was also tackled. Traffic contributions have decreased here over the years, attributed to regulations limiting vehicular emissions in bigger cities.
Adam Brighty, Véronique Jacob, Gaëlle Uzu, Lucille Borlaza, Sébastien Conil, Christoph Hueglin, Stuart K. Grange, Olivier Favez, Cécile Trébuchon, and Jean-Luc Jaffrezo
Atmos. Chem. Phys., 22, 6021–6043, https://doi.org/10.5194/acp-22-6021-2022, https://doi.org/10.5194/acp-22-6021-2022, 2022
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With an revised analytical method and long-term sampling strategy, we have been able to elucidate much more information about atmospheric plant debris, a poorly understood class of particulate matter. We found weaker seasonal patterns at urban locations compared to rural locations and significant interannual variability in concentrations between previous years and 2020, during the COVID-19 pandemic. This suggests a possible man-made influence on plant debris concentration and source strength.
Petra Pokorná, Naděžda Zíková, Petr Vodička, Radek Lhotka, Saliou Mbengue, Adéla Holubová Šmejkalová, Véronique Riffault, Jakub Ondráček, Jaroslav Schwarz, and Vladimír Ždímal
Atmos. Chem. Phys., 22, 5829–5858, https://doi.org/10.5194/acp-22-5829-2022, https://doi.org/10.5194/acp-22-5829-2022, 2022
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By examining individual episodes of high mass and number concentrations, we show that the seasonality in the physicochemical properties of aerosol particles was caused by the sources' diversity and was related to the different air masses and meteorology. We also confirmed the relation between particle size and age that is reflected in oxidation state and shape (difference in densities; effective vs. material). The results have general validity and thus transcend the study regional character.
Marco A. Franco, Florian Ditas, Leslie A. Kremper, Luiz A. T. Machado, Meinrat O. Andreae, Alessandro Araújo, Henrique M. J. Barbosa, Joel F. de Brito, Samara Carbone, Bruna A. Holanda, Fernando G. Morais, Janaína P. Nascimento, Mira L. Pöhlker, Luciana V. Rizzo, Marta Sá, Jorge Saturno, David Walter, Stefan Wolff, Ulrich Pöschl, Paulo Artaxo, and Christopher Pöhlker
Atmos. Chem. Phys., 22, 3469–3492, https://doi.org/10.5194/acp-22-3469-2022, https://doi.org/10.5194/acp-22-3469-2022, 2022
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In Central Amazonia, new particle formation in the planetary boundary layer is rare. Instead, there is the appearance of sub-50 nm aerosols with diameters larger than about 20 nm that eventually grow to cloud condensation nuclei size range. Here, 254 growth events were characterized which have higher predominance in the wet season. About 70 % of them showed direct relation to convective downdrafts, while 30 % occurred partly under clear-sky conditions, evidencing still unknown particle sources.
Adrien Deroubaix, Laurent Menut, Cyrille Flamant, Peter Knippertz, Andreas H. Fink, Anneke Batenburg, Joel Brito, Cyrielle Denjean, Cheikh Dione, Régis Dupuy, Valerian Hahn, Norbert Kalthoff, Fabienne Lohou, Alfons Schwarzenboeck, Guillaume Siour, Paolo Tuccella, and Christiane Voigt
Atmos. Chem. Phys., 22, 3251–3273, https://doi.org/10.5194/acp-22-3251-2022, https://doi.org/10.5194/acp-22-3251-2022, 2022
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During the summer monsoon in West Africa, pollutants emitted in urbanized areas modify cloud cover and precipitation patterns. We analyze these patterns with the WRF-CHIMERE model, integrating the effects of aerosols on meteorology, based on the numerous observations provided by the Dynamics-Aerosol-Climate-Interactions campaign. This study adds evidence to recent findings that increased pollution levels in West Africa delay the breakup time of low-level clouds and reduce precipitation.
Jean-Eudes Petit, Jean-Charles Dupont, Olivier Favez, Valérie Gros, Yunjiang Zhang, Jean Sciare, Leila Simon, François Truong, Nicolas Bonnaire, Tanguy Amodeo, Robert Vautard, and Martial Haeffelin
Atmos. Chem. Phys., 21, 17167–17183, https://doi.org/10.5194/acp-21-17167-2021, https://doi.org/10.5194/acp-21-17167-2021, 2021
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The COVID-19 outbreak led to lockdowns at national scales in spring 2020. Large cuts in emissions occurred, but the quantitative assessment of their role from observations is hindered by weather and interannual variability. That is why we developed an innovative methodology in order to best characterize the impact of lockdown on atmospheric chemistry. We find that a local decrease in traffic-related pollutants triggered a decrease of secondary aerosols and an increase in ozone.
Clémence Rose, Martine Collaud Coen, Elisabeth Andrews, Yong Lin, Isaline Bossert, Cathrine Lund Myhre, Thomas Tuch, Alfred Wiedensohler, Markus Fiebig, Pasi Aalto, Andrés Alastuey, Elisabeth Alonso-Blanco, Marcos Andrade, Begoña Artíñano, Todor Arsov, Urs Baltensperger, Susanne Bastian, Olaf Bath, Johan Paul Beukes, Benjamin T. Brem, Nicolas Bukowiecki, Juan Andrés Casquero-Vera, Sébastien Conil, Konstantinos Eleftheriadis, Olivier Favez, Harald Flentje, Maria I. Gini, Francisco Javier Gómez-Moreno, Martin Gysel-Beer, Anna Gannet Hallar, Ivo Kalapov, Nikos Kalivitis, Anne Kasper-Giebl, Melita Keywood, Jeong Eun Kim, Sang-Woo Kim, Adam Kristensson, Markku Kulmala, Heikki Lihavainen, Neng-Huei Lin, Hassan Lyamani, Angela Marinoni, Sebastiao Martins Dos Santos, Olga L. Mayol-Bracero, Frank Meinhardt, Maik Merkel, Jean-Marc Metzger, Nikolaos Mihalopoulos, Jakub Ondracek, Marco Pandolfi, Noemi Pérez, Tuukka Petäjä, Jean-Eudes Petit, David Picard, Jean-Marc Pichon, Veronique Pont, Jean-Philippe Putaud, Fabienne Reisen, Karine Sellegri, Sangeeta Sharma, Gerhard Schauer, Patrick Sheridan, James Patrick Sherman, Andreas Schwerin, Ralf Sohmer, Mar Sorribas, Junying Sun, Pierre Tulet, Ville Vakkari, Pieter Gideon van Zyl, Fernando Velarde, Paolo Villani, Stergios Vratolis, Zdenek Wagner, Sheng-Hsiang Wang, Kay Weinhold, Rolf Weller, Margarita Yela, Vladimir Zdimal, and Paolo Laj
Atmos. Chem. Phys., 21, 17185–17223, https://doi.org/10.5194/acp-21-17185-2021, https://doi.org/10.5194/acp-21-17185-2021, 2021
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Aerosol particles are a complex component of the atmospheric system the effects of which are among the most uncertain in climate change projections. Using data collected at 62 stations, this study provides the most up-to-date picture of the spatial distribution of particle number concentration and size distribution worldwide, with the aim of contributing to better representation of aerosols and their interactions with clouds in models and, therefore, better evaluation of their impact on climate.
Cited articles
Aiken, A. C., DeCarlo, P. F., Kroll, J. H., Worsnop, D. R., Huffman, J. A., Docherty, K. S., Ulbrich, I. M., Mohr, C., Kimmel, J. R., Sueper, D., Sun, Y., Zhang, Q., Trimborn, A., Northway, M., Ziemann, P. J., Canagaratna, M. R., Onasch, T. B., Alfarra, M. R., Prevot, A. S. H., Dommen, J., Duplissy, J., Metzger, A., Baltensperger, U., and Jimenez, J. L.: O/C and OM/OC Ratios of Primary, Secondary, and Ambient Organic Aerosols with High-Resolution Time-of-Flight Aerosol Mass Spectrometry, Environ. Sci. Technol., 42, 4478–4485, https://doi.org/10.1021/es703009q, 2008.
ATMO Grand Est: Le bilan annuel 2022 de la qualité de l'air dans le Grand Est, https://www.atmo-grandest.eu/actualite/le-bilan-annuel-2022-de-la-qualite-de-lair-dans-le-grand-est, last access: 31 July 2023.
Allan, J. D., Delia, A. E., Coe, H., Bower, K. N., Alfarra, M. R., Jimenez, J. L., Middlebrook, A. M., Drewnick, F., Onasch, T. B., Canagaratna, M. R., Jayne, J. T., and Worsnop, D. R.: A generalised method for the extraction of chemically resolved mass spectra from Aerodyne aerosol mass spectrometer data, Journal of Aerosol Science, 35, 909–922, https://doi.org/10.1016/j.jaerosci.2004.02.007, 2004.
Bressi, M., Cavalli, F., Putaud, J. P., Fröhlich, R., Petit, J.-E., Aas, W., Äijälä, M., Alastuey, A., Allan, J. D., Aurela, M., Berico, M., Bougiatioti, A., Bukowiecki, N., Canonaco, F., Crenn, V., Dusanter, S., Ehn, M., Elsasser, M., Flentje, H., Graf, P., Green, D. C., Heikkinen, L., Hermann, H., Holzinger, R., Hueglin, C., Keernik, H., Kiendler-Scharr, A., Kubelová, L., Lunder, C., Maasikmets, M., Makeš, O., Malaguti, A., Mihalopoulos, N., Nicolas, J. B., O'Dowd, C., Ovadnevaite, J., Petralia, E., Poulain, L., Priestman, M., Riffault, V., Ripoll, A., Schlag, P., Schwarz, J., Sciare, J., Slowik, J., Sosedova, Y., Stavroulas, I., Teinemaa, E., Via, M., Vodička, P., Williams, P. I., Wiedensohler, A., Young, D. E., Zhang, S., Favez, O., Minguillón, M. C., and Prevot, A. S. H.: A European aerosol phenomenology – 7: High-time resolution chemical characteristics of submicron particulate matter across Europe, Atmospheric Environment, 10, 100108, https://doi.org/10.1016/j.aeaoa.2021.100108, 2021.
Cavalli, F., Viana, M., Yttri, K. E., Genberg, J., and Putaud, J.-P.: Toward a standardised thermal-optical protocol for measuring atmospheric organic and elemental carbon: the EUSAAR protocol, Atmos. Meas. Tech., 3, 79–89, https://doi.org/10.5194/amt-3-79-2010, 2010.
Chatain, M., Alvarez, R., Ustache, A., Rivière, E., Favez, O., and Pallares, C.: Simultaneous Roadside and Urban Background Measurements of Submicron Aerosol Number Concentration and Size Distribution (in the Range 20–800 nm), along with Chemical Composition in Strasbourg, France, Atmosphere, 12, 71, https://doi.org/10.3390/atmos12010071, 2021.
Chebaicheb, H., F. de Brito, J., Chen, G., Tison, E., Marchand, C., Prévôt, A. S. H., Favez, O., and Riffault, V.: Investigation of four-year chemical composition and organic aerosol sources of submicron particles at the ATOLL site in northern France, Environ. Pollut., 330, 121805, https://doi.org/10.1016/j.envpol.2023.121805, 2023.
Chebaicheb, H., de Brito, J. F., Amodeo, T., Couvidat, F., Petit, J.-E., Tison, E., Abbou, G., Baudic, A., Chatain, M., Chazeau, B., Marchand, N., Falhun, R., Francony, F., Ratier, C., Grenier, D., Vidaud, R., Zhang, S., Gille, G., Meunier, L., Marchand, C., Riffault, V., and Favez, O.: Multiyear high-temporal-resolution measurements of submicron aerosols at 13 French urban sites: data processing and chemical composition, Earth Syst. Sci. Data, 16, 5089–5109, https://doi.org/10.5194/essd-16-5089-2024, 2024a.
Chebaicheb, H., Ferreira de Brito, J., Amodeo, T., Couvidat, F., Petit, J.-E., Tison, E., Abbou, G., Alexia, B., Chatain, M., Chazeau, B., Marchand, N., Falhun, R., Francony, F., Ratier, C., Grenier, D., Vidaud, R., Zhang, S., Gille, G., Meunier, L., Marchand, C., Riffault, V., and Favez, O.: Multi-year high time resolution measurements of fine PM at 13 sites of the French Operational Network (CARA program), In Earth System Science Data, Zenodo [data set], https://doi.org/10.5281/zenodo.13318298, 2024b.
Chebaicheb, H., Chatain, M., Favez, O., Ferreira de Brito, J., Crenn, V., Amodeo, T., Gherras, M., Jantzem, E., Marchand, C., and Riffault, V.: Lessons learned from the comparison and combination of fine carbonaceous aerosol source apportionment at two locations in the city of Strasbourg, France, In Atmospheric Chemistry and Physics (ACP), Zenodo [data set], https://doi.org/10.5281/zenodo.14855186, 2025.
Chen, G., Sosedova, Y., Canonaco, F., Fröhlich, R., Tobler, A., Vlachou, A., Daellenbach, K. R., Bozzetti, C., Hueglin, C., Graf, P., Baltensperger, U., Slowik, J. G., El Haddad, I., and Prévôt, A. S. H.: Time-dependent source apportionment of submicron organic aerosol for a rural site in an alpine valley using a rolling positive matrix factorisation (PMF) window, Atmos. Chem. Phys., 21, 15081–15101, https://doi.org/10.5194/acp-21-15081-2021, 2021.
Chen, G., Canonaco, F., Tobler, A., Aas, W., Alastuey, A., Allan, J., Atabakhsh, S., Aurela, M., Baltensperger, U., Bougiatioti, A., De Brito, J. F., Ceburnis, D., Chazeau, B., Chebaicheb, H., Daellenbach, K. R., Ehn, M., El Haddad, I., Eleftheriadis, K., Favez, O., Flentje, H., Font, A., Fossum, K., Freney, E., Gini, M., Green, D. C., Heikkinen, L., Herrmann, H., Kalogridis, A.-C., Keernik, H., Lhotka, R., Lin, C., Lunder, C., Maasikmets, M., Manousakas, M. I., Marchand, N., Marin, C., Marmureanu, L., Mihalopoulos, N., Močnik, G., Nęcki, J., O'Dowd, C., Ovadnevaite, J., Peter, T., Petit, J.-E., Pikridas, M., Matthew Platt, S., Pokorná, P., Poulain, L., Priestman, M., Riffault, V., Rinaldi, M., Różański, K., Schwarz, J., Sciare, J., Simon, L., Skiba, A., Slowik, J. G., Sosedova, Y., Stavroulas, I., Styszko, K., Teinemaa, E., Timonen, H., Tremper, A., Vasilescu, J., Via, M., Vodička, P., Wiedensohler, A., Zografou, O., Cruz Minguillón, M., and Prévôt, A. S. H.: European aerosol phenomenology – 8: Harmonised source apportionment of organic aerosol using 22 Year-long ACSM/AMS datasets, Environ. Int., 166, 107325, https://doi.org/10.1016/j.envint.2022.107325, 2022.
Crippa, M., DeCarlo, P. F., Slowik, J. G., Mohr, C., Heringa, M. F., Chirico, R., Poulain, L., Freutel, F., Sciare, J., Cozic, J., Di Marco, C. F., Elsasser, M., Nicolas, J. B., Marchand, N., Abidi, E., Wiedensohler, A., Drewnick, F., Schneider, J., Borrmann, S., Nemitz, E., Zimmermann, R., Jaffrezo, J.-L., Prévôt, A. S. H., and Baltensperger, U.: Wintertime aerosol chemical composition and source apportionment of the organic fraction in the metropolitan area of Paris, Atmos. Chem. Phys., 13, 961–981, https://doi.org/10.5194/acp-13-961-2013, 2013.
Drinovec, L., Močnik, G., Zotter, P., Prévôt, A. S. H., Ruckstuhl, C., Coz, E., Rupakheti, M., Sciare, J., Müller, T., Wiedensohler, A., and Hansen, A. D. A.: The ”dual-spot” Aethalometer: an improved measurement of aerosol black carbon with real-time loading compensation, Atmos. Meas. Tech., 8, 1965–1979, https://doi.org/10.5194/amt-8-1965-2015, 2015.
Duarte, R. M. B. O. and Duarte, A. C.: Health Effects of Urban Atmospheric Aerosols, Atmosphere, 14, 309, https://doi.org/10.3390/atmos14020309, 2023.
EEA: Air quality in Europe 2022: https://www.eea.europa.eu/publications/air-quality-in-europe-2022, last access: 31 July 2023.
Favez, O., El Haddad, I., Piot, C., Boréave, A., Abidi, E., Marchand, N., Jaffrezo, J.-L., Besombes, J.-L., Personnaz, M.-B., Sciare, J., Wortham, H., George, C., and D’Anna, B.: Inter-comparison of source apportionment models for the estimation of wood burning aerosols during wintertime in an Alpine city (Grenoble, France), Atmospheric Chemistry and Physics, 10, 5295–5314, https://doi.org/10.5194/acp-10-5295-2010, 2010.
Favez, O., Weber, S., Petit, J.-E., Alleman, L., Albinet, A., Riffault, V., Chazeau, B., Amodeo, T., Salameh, D., Zhang, Y., Srivastava, D., Samaké, A., Aujay, R., Papin, A., Bonnaire, N., Boullanger, C., Chatain, M., Chevrier, F., Detournay, A., and Leoz-Garziandia, E.: Overview of the French Operational Network for In Situ Observation of PM Chemical Composition and Sources in Urban Unvironments (CARA Program), Atmosphere, https://doi.org/10.20944/preprints202101.0182.v1, 2021.
Freutel, F., Schneider, J., Drewnick, F., von der Weiden-Reinmüller, S.-L., Crippa, M., Prévôt, A. S. H., Baltensperger, U., Poulain, L., Wiedensohler, A., Sciare, J., Sarda-Estève, R., Burkhart, J. F., Eckhardt, S., Stohl, A., Gros, V., Colomb, A., Michoud, V., Doussin, J. F., Borbon, A., Haeffelin, M., Morille, Y., Beekmann, M., and Borrmann, S.: Aerosol particle measurements at three stationary sites in the megacity of Paris during summer 2009: meteorology and air mass origin dominate aerosol particle composition and size distribution, Atmospheric Chemistry and Physics, 13, 933–959, https://doi.org/10.5194/acp-13-933-2013, 2013.
Fröhlich, R., Crenn, V., Setyan, A., Belis, C. A., Canonaco, F., Favez, O., Riffault, V., Slowik, J. G., Aas, W., Aijälä, M., Alastuey, A., Artiñano, B., Bonnaire, N., Bozzetti, C., Bressi, M., Carbone, C., Coz, E., Croteau, P. L., Cubison, M. J., Esser-Gietl, J. K., Green, D. C., Gros, V., Heikkinen, L., Herrmann, H., Jayne, J. T., Lunder, C. R., Minguillón, M. C., Močnik, G., O’Dowd, C. D., Ovadnevaite, J., Petralia, E., Poulain, L., Priestman, M., Ripoll, A., Sarda-Estève, R., Wiedensohler, A., Baltensperger, U., Sciare, J., and Prévôt, A. S. H.: ACTRIS ACSM intercomparison – Part 2: Intercomparison of ME-2 organic source apportionment results from 15 individual, co-located aerosol mass spectrometers, Atmospheric Measurement Techniques, 8, 2555–2576, https://doi.org/10.5194/amt-8-2555-2015, 2015.
Hildebrandt, L., Kostenidou, E., Lanz, V. A., Prevot, A. S. H., Baltensperger, U., Mihalopoulos, N., Laaksonen, A., Donahue, N. M., and Pandis, S. N.: Sources and atmospheric processing of organic aerosol in the Mediterranean: insights from aerosol mass spectrometer factor analysis, Atmos. Chem. Phys., 11, 12499–12515, https://doi.org/10.5194/acp-11-12499-2011, 2011.
Hopke, P. K., Dai, Q., Li, L., and Feng, Y.: Global review of recent source apportionments for airborne particulate matter, Sci. Total Environ., 740, 140091, https://doi.org/10.1016/j.scitotenv.2020.140091, 2020.
Katz, E. F., Guo, H., Campuzano-Jost, P., Day, D. A., Brown, W. L., Boedicker, E., Pothier, M., Lunderberg, D. M., Patel, S., Patel, K., Hayes, P. L., Avery, A., Hildebrandt Ruiz, L., Goldstein, A. H., Vance, M. E., Farmer, D. K., Jimenez, J. L., and DeCarlo, P. F.: Quantification of cooking organic aerosol in the indoor environment using aerodyne aerosol mass spectrometers, Aerosol Science and Technology, 55, 1099–1114, https://doi.org/10.1080/02786826.2021.1931013, 2021.
Kim, B. M., Cassmassi, J., Hogo, H., and Zeldin, M. D.: Positive Organic Carbon Artifacts on Filter Medium During PM2.5 Sampling in the South Coast Air Basin, Aerosol Science and Technology, 34, 35–41, https://doi.org/10.1080/02786820118227, 2001.
Laj, P., Myhre, C. L., Riffault, V., Amiridis, V., Fuchs, H., Eleftheriadis, K., Petäjä, T., Salameh, T., Kivekäs, N., Juurola, E., Saponaro, G., Philippin, S., Cornacchia, C., Arboledas, L. A., Baars, H., Claude, A., Mazière, M. D., Dils, B., Dufresne, M., Evangeliou, N., Favez, O., Fiebig, M., Haeffelin, M., Herrmann, H., Höhler, K., Illmann, N., Kreuter, A., Ludewig, E., Marinou, E., Möhler, O., Mona, L., Murberg, L. E., Nicolae, D., Novelli, A., O'Connor, E., Ohneiser, K., Altieri, R. M. P., Picquet-Varrault, B., Pinxteren, D. van, Pospichal, B., Putaud, J.-P., Reimann, S., Siomos, N., Stachlewska, I., Tillmann, R., Voudouri, K. A., Wandinger, U., Wiedensohler, A., Apituley, A., Comerón, A., Gysel-Beer, M., Mihalopoulos, N., Nikolova, N., Pietruczuk, A., Sauvage, S., Sciare, J., Skov, H., Svendby, T., Swietlicki, E., Tonev, D., Vaughan, G., Zdimal, V., Baltensperger, U., Doussin, J.-F., Kulmala, M., Pappalardo, G., Sundet, S. S., and Vana, M.: Aerosol, Clouds and Trace Gases Research Infrastructure (ACTRIS): The European Research Infrastructure Supporting Atmospheric Science, Bulletin of the American Meteorological Society, 105, E1098–E1136, https://doi.org/10.1175/BAMS-D-23-0064.1, 2024.
Li, S., Chen, C., Yang, G., Fang, J., Sun, Y., Tang, L., Wang, H., Xiang, W., Zhang, H., Croteau, P. L., Jayne, J. T., Liao, H., Ge, X., Favez, O., and Zhang, Y.: Sources and processes of organic aerosol in non-refractory PM1 and PM2.5 during foggy and haze episodes in an urban environment of the Yangtze River Delta, China, Environmental Research, 212, 113557, https://doi.org/10.1016/j.envres.2022.113557, 2022.
Liu, P. S. K., Deng, R., Smith, K. A., Williams, L. R., Jayne, J. T., Canagaratna, M. R., Moore, K., Onasch, T. B., Worsnop, D. R., and Deshler, T.: Transmission Efficiency of an Aerodynamic Focusing Lens System: Comparison of Model Calculations and Laboratory Measurements for the Aerodyne Aerosol Mass Spectrometer, Aerosol Science and Technology, 41, 721–733, https://doi.org/10.1080/02786820701422278, 2007.
Middlebrook, A. M., Bahreini, R., Jimenez, J. L., and Canagaratna, M. R.: Evaluation of Composition-Dependent Collection Efficiencies for the Aerodyne Aerosol Mass Spectrometer using Field Data, Aerosol Science and Technology, 46, 258–271, https://doi.org/10.1080/02786826.2011.620041, 2011.
Mooibroek, D., Schaap, M., Weijers, E. P., and Hoogerbrugge, R.: Source apportionment and spatial variability of PM2.5 using measurements at five sites in the Netherlands, Atmos. Environ., 45, 4180–4191, https://doi.org/10.1016/j.atmosenv.2011.05.017, 2011.
Mooibroek, D., Staelens, J., Cordell, R., Panteliadis, P., Delaunay, T., Weijers, E., Vercauteren, J., Hoogerbrugge, R., Dijkema, M., Monks, P. S., and Roekens, E.: PM10 Source Apportionment in Five North Western European Cities–Outcome of the Joaquin Project, Special Collection: 2016 ebook collection, ECCC Environmental eBooks 1968-2022, 264–292 pp., https://doi.org/10.1039/9781782626589-00264, 2016.
Nault, B. A., Croteau, P., Jayne, J., Williams, A., Williams, L., Worsnop, D., Katz, E. F., DeCarlo, P. F., and Canagaratna, M.: Laboratory evaluation of organic aerosol relative ionization efficiencies in the aerodyne aerosol mass spectrometer and aerosol chemical speciation monitor, Aerosol Science and Technology, 57, 981–997, https://doi.org/10.1080/02786826.2023.2223249, 2023.
Ng, N. L., Herndon, S. C., Trimborn, A., Canagaratna, M. R., Croteau, P. L., Onasch, T. B., Sueper, D., Worsnop, D. R., Zhang, Q., Sun, Y. L., and Jayne, J. T.: An Aerosol Chemical Speciation Monitor (ACSM) for Routine Monitoring of the Composition and Mass Concentrations of Ambient Aerosol, Aerosol Sci. Technol., 45, 780–794, https://doi.org/10.1080/02786826.2011.560211, 2011.
Paatero, P. and Tapper, U.: Positive matrix factorization: a non-negative factor model with optimal utilization of error estimates of data values, Environmetrics, 5, 111–126, https://doi.org/10.1002/env.3170050203, 1994
Pandolfi, M., Mooibroek, D., Hopke, P., van Pinxteren, D., Querol, X., Herrmann, H., Alastuey, A., Favez, O., Hüglin, C., Perdrix, E., Riffault, V., Sauvage, S., van der Swaluw, E., Tarasova, O., and Colette, A.: Long-range and local air pollution: what can we learn from chemical speciation of particulate matter at paired sites?, Atmos. Chem. Phys., 20, 409–429, https://doi.org/10.5194/acp-20-409-2020, 2020.
Petit, J.-E., Favez, O., Albinet, A., and Canonaco, F.: A user-friendly tool for comprehensive evaluation of the geographical origins of atmospheric pollution: Wind and trajectory analyses, Environmental Modelling & Software, 88, 183–187, https://doi.org/10.1016/j.envsoft.2016.11.022, 2017.
Petit, J.-E., Favez, O., Sciare, J., Canonaco, F., Croteau, P., Močnik, G., Jayne, J., Worsnop, D., and Leoz-Garziandia, E.: Submicron aerosol source apportionment of wintertime pollution in Paris, France by double positive matrix factorization (PMF2) using an aerosol chemical speciation monitor (ACSM) and a multi-wavelength Aethalometer, Atmos. Chem. Phys., 14, 13773–13787, https://doi.org/10.5194/acp-14-13773-2014, 2014.
Pieber, S. M., El Haddad, I., Slowik, J. G., Canagaratna, M. R., Jayne, J. T., Platt, S. M., Bozzetti, C., Daellenbach, K. R., Fröhlich, R., Vlachou, A., Klein, F., Dommen, J., Miljevic, B., Jiménez, J. L., Worsnop, D. R., Baltensperger, U., and Prévôt, A. S. H.: Inorganic Salt Interference on CO2+ in Aerodyne AMS and ACSM Organic Aerosol Composition Studies, Environ. Sci. Technol., 50, 10494–10503, https://doi.org/10.1021/acs.est.6b01035, 2016.
Potier, E., Waked, A., Bourin, A., Minvielle, F., Péré, J. C., Perdrix, E., Michoud, V., Riffault, V., Alleman, L. Y., and Sauvage, S.: Characterizing the regional contribution to PM10 pollution over northern France using two complementary approaches: Chemistry transport and trajectory-based receptor models, Atmospheric Research, 223, 1–14, https://doi.org/10.1016/j.atmosres.2019.03.002, 2019.
Sandradewi, J., Prevot, A., Weingartner, E., Schmidhauser, R., Gysel, M., and Baltensperger, U.: A study of wood burning and traffic aerosols in an Alpine valley using a multi-wavelength Aethalometer, Atmos. Environ., 42, 101–112, https://doi.org/10.1016/j.atmosenv.2007.09.034, 2008.
Savadkoohi, M., Gherras, M., Favez, O., Petit, J.-E., Rovira, J., Chen, G. I., Via, M., Platt, S., Aurela, M., Chazeau, B., de Brito, J. F., Riffault, V., Eleftheriadis, K., Flentje, H., Gysel-Beer, M., Hueglin, C., Rigler, M., Gregorič, A., Ivančič, M., Keernik, H., Maasikmets, M., Liakakou, E., Stavroulas, I., Luoma, K., Marchand, N., Mihalopoulos, N., Petäjä, T., Prevot, A. S. H., Daellenbach, K. R., Vodička, P., Timonen, H., Tobler, A., Vasilescu, J., Dandocsi, A., Mbengue, S., Vratolis, S., Zografou, O., Chauvigné, A., Hopke, P. K., Querol, X., Alastuey, A., and Pandolfi, M.: Addressing the advantages and limitations of using Aethalometer data to determine the optimal absorption Ångström exponents (AAEs) values for eBC source apportionment, Atmospheric Environment, 349, 121121, https://doi.org/10.1016/j.atmosenv.2025.121121, 2025.
Savadkoohi, M., Pandolfi, M., Reche, C., Niemi, J. V., Mooibroek, D., Titos, G., Green, D. C., Tremper, A. H., Hueglin, C., Liakakou, E., Mihalopoulos, N., Stavroulas, I., Artiñano, B., Coz, E., Alados-Arboledas, L., Beddows, D., Riffault, V., De Brito, J. F., Bastian, S., Baudic, A., Colombi, C., Costabile, F., Chazeau, B., Marchand, N., Gómez-Amo, J. L., Estellés, V., Matos, V., van der Gaag, E., Gille, G., Luoma, K., Manninen, H. E., Norman, M., Silvergren, S., Petit, J.-E., Putaud, J.-P., Rattigan, O. V., Timonen, H., Tuch, T., Merkel, M., Weinhold, K., Vratolis, S., Vasilescu, J., Favez, O., Harrison, R. M., Laj, P., Wiedensohler, A., Hopke, P. K., Petäjä, T., Alastuey, A., and Querol, X.: The variability of mass concentrations and source apportionment analysis of equivalent black carbon across urban Europe, Environ Int, 178, 108081, https://doi.org/10.1016/j.envint.2023.108081, 2023.
Schmid, P., Bogdal, C., Wang, Z., Azara, V., Haag, R., and von Arx, U.: Releases of chlorobenzenes, chlorophenols and dioxins during fireworks, Chemosphere, 114, 158–164, https://doi.org/10.1016/j.chemosphere.2014.03.088, 2014.
Tobler, A. K., Skiba, A., Canonaco, F., Močnik, G., Rai, P., Chen, G., Bartyzel, J., Zimnoch, M., Styszko, K., Nęcki, J., Furger, M., Różański, K., Baltensperger, U., Slowik, J. G., and Prevot, A. S. H.: Characterization of non-refractory (NR) PM1 and source apportionment of organic aerosol in Kraków, Poland, Atmos. Chem. Phys., 21, 14893–14906, https://doi.org/10.5194/acp-21-14893-2021, 2021.
Via, M., Minguillón, M. C., Reche, C., Querol, X., and Alastuey, A.: Increase in secondary organic aerosol in an urban environment, Atmos. Chem. Phys., 21, 8323–8339, https://doi.org/10.5194/acp-21-8323-2021, 2021.
Waked, A., Bourin, A., Michoud, V., Perdrix, E., Alleman, L. Y., Sauvage, S., Delaunay, T., Vermeesch, S., Petit, J.-E., and Riffault, V.: Investigation of the geographical origins of PM10 based on long, medium and short-range air mass back-trajectories impacting Northern France during the period 2009–2013, Atmospheric Environment, 193, 143–152, https://doi.org/10.1016/j.atmosenv.2018.08.015, 2018.
WHO: Air Quality Guidelines, https://www.c40knowledgehub.org/s/article/WHO-Air-Quality-Guidelines?language=en_US (last access: 23 January 2023), 2022.
Xu, W., Lambe, A., Silva, P., Hu, W., Onasch, T., Williams, L., Croteau, P., Zhang, X., Renbaum-Wolff, L., Fortner, E., Jimenez, J. L., Jayne, J., Worsnop, D., and Canagaratna, M.: Laboratory evaluation of species-dependent relative ionization efficiencies in the Aerodyne Aerosol Mass Spectrometer, Aerosol Sci. Technol., 52, 626–641, https://doi.org/10.1080/02786826.2018.1439570, 2018.
Zhang, S., Tison, E., Dusanter, S., Beaugard, C., Gengembre, C., Augustin, P., Fourmentin, M., Delbarre, H., and Riffault, V.: Near real-time PM1 chemical composition measurements at a French urban background and coastal site under industrial influence over more than a year: Temporal variability and assessment of sulfur-containing emissions, Atmospheric Environment, 244, 117960, https://doi.org/10.1016/j.atmosenv.2020.117960, 2021.
Zhang, Y., Favez, O., Petit, J.-E., Canonaco, F., Truong, F., Bonnaire, N., Crenn, V., Amodeo, T., Prévôt, A. S. H., Sciare, J., Gros, V., and Albinet, A.: Six-year source apportionment of submicron organic aerosols from near-continuous highly time-resolved measurements at SIRTA (Paris area, France), Atmos. Chem. Phys., 19, 14755–14776, https://doi.org/10.5194/acp-19-14755-2019, 2019.
Zhang, Y., Albinet, A., Petit, J.-E., Jacob, V., Chevrier, F., Gille, G., Pontet, S., Chrétien, E., Dominik-Sègue, M., Levigoureux, G., Močnik, G., Gros, V., Jaffrezo, J.-L., and Favez, O.: Substantial brown carbon emissions from wintertime residential wood burning over France, Science of The Total Environment, 743, 140752, https://doi.org/10.1016/j.scitotenv.2020.140752, 2020.
Zhou, W., Xu, W., Kim, H., Zhang, Q., Fu, P., Worsnop, D. R., and Sun, Y.: A review of aerosol chemistry in Asia: insights from aerosol mass spectrometer measurements, Environ. Sci.: Processes Impacts, 22, 1616–1653, https://doi.org/10.1039/D0EM00212G, 2020.
Zotter, P., Herich, H., Gysel, M., El-Haddad, I., Zhang, Y., Močnik, G., Hüglin, C., Baltensperger, U., Szidat, S., and Prévôt, A. S. H.: Evaluation of the absorption Ångström exponents for traffic and wood burning in the Aethalometer-based source apportionment using radiocarbon measurements of ambient aerosol, Atmospheric Chemistry and Physics, 17, 4229–4249, https://doi.org/10.5194/acp-17-4229-2017, 2017.
Short summary
This study compares carbonaceous aerosols source apportionment at paired traffic and background locations in urban environment (Strasbourg, France). Positive matrix factorization was applied (individually and in a combined input dataset) to aerosol mass spectrometry measurements at both sites, providing notably insights into the challenges of attributing real sources to organic aerosol (OA) factors and the impact of instrumental result specificities leading to differences in OA mass spectra.
This study compares carbonaceous aerosols source apportionment at paired traffic and background...
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