Articles | Volume 24, issue 16
https://doi.org/10.5194/acp-24-9401-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-24-9401-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
15 Sep 2024
Research article |
| 15 Sep 2024
| 15 Sep 2024
The importance of an informed choice of CO2-equivalence metrics for contrail avoidance
Institut Pierre-Simon Laplace, Sorbonne Université/CNRS, Paris, France
Olivier Boucher
Institut Pierre-Simon Laplace, Sorbonne Université/CNRS, Paris, France
Keith P. Shine
Department of Meteorology, University of Reading, Reading, UK
Marc Stettler
Centre for Transport Studies, Department of Civil and Environmental Engineering, Imperial College London, London, UK
Katsumasa Tanaka
Laboratoire des Sciences du Climat et de l'Environnement (LSCE), IPSL, CEA/CNRS/UVSQ, Université Paris-Saclay, Gif-sur-Yvette, France
Earth System Division, National Institute for Environmental Studies (NIES), Tsukuba, Japan
Roger Teoh
Centre for Transport Studies, Department of Civil and Environmental Engineering, Imperial College London, London, UK
Nicolas Bellouin
Institut Pierre-Simon Laplace, Sorbonne Université/CNRS, Paris, France
Department of Meteorology, University of Reading, Reading, UK
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Tropical cyclones (TCs) are one of the most devastating natural disasters, which justifies monitoring and prediction in the context of a changing climate. In this study, we have adapted and tested a convolutional neural network (CNN) for the classification of reanalysis outputs (ERA5 and MERRA-2 labeled by HURDAT2) according to the presence or absence of TCs. We tested the impact of interpolation and of "mixing and matching" the training and test sets on the performance of the CNN.
Roger Teoh, Ulrich Schumann, Edward Gryspeerdt, Marc Shapiro, Jarlath Molloy, George Koudis, Christiane Voigt, and Marc E. J. Stettler
Atmos. Chem. Phys., 22, 10919–10935, https://doi.org/10.5194/acp-22-10919-2022, https://doi.org/10.5194/acp-22-10919-2022, 2022
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Aircraft condensation trails (contrails) contribute to over half of the climate forcing attributable to aviation. This study uses historical air traffic and weather data to simulate contrails in the North Atlantic over 5 years, from 2016 to 2021. We found large intra- and inter-year variability in contrail radiative forcing and observed a 66 % reduction due to COVID-19. Most warming contrails predominantly result from night-time flights in winter.
Irina Melnikova, Olivier Boucher, Patricia Cadule, Katsumasa Tanaka, Thomas Gasser, Tomohiro Hajima, Yann Quilcaille, Hideo Shiogama, Roland Séférian, Kaoru Tachiiri, Nicolas Vuichard, Tokuta Yokohata, and Philippe Ciais
Earth Syst. Dynam., 13, 779–794, https://doi.org/10.5194/esd-13-779-2022, https://doi.org/10.5194/esd-13-779-2022, 2022
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Zhu Deng, Philippe Ciais, Zitely A. Tzompa-Sosa, Marielle Saunois, Chunjing Qiu, Chang Tan, Taochun Sun, Piyu Ke, Yanan Cui, Katsumasa Tanaka, Xin Lin, Rona L. Thompson, Hanqin Tian, Yuanzhi Yao, Yuanyuan Huang, Ronny Lauerwald, Atul K. Jain, Xiaoming Xu, Ana Bastos, Stephen Sitch, Paul I. Palmer, Thomas Lauvaux, Alexandre d'Aspremont, Clément Giron, Antoine Benoit, Benjamin Poulter, Jinfeng Chang, Ana Maria Roxana Petrescu, Steven J. Davis, Zhu Liu, Giacomo Grassi, Clément Albergel, Francesco N. Tubiello, Lucia Perugini, Wouter Peters, and Frédéric Chevallier
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In support of the global stocktake of the Paris Agreement on climate change, we proposed a method for reconciling the results of global atmospheric inversions with data from UNFCCC national greenhouse gas inventories (NGHGIs). Here, based on a new global harmonized database that we compiled from the UNFCCC NGHGIs and a comprehensive framework presented in this study to process the results of inversions, we compared their results of carbon dioxide (CO2), methane (CH4), and nitrous oxide (N2O).
Simone Tilmes, Daniele Visioni, Andy Jones, James Haywood, Roland Séférian, Pierre Nabat, Olivier Boucher, Ewa Monica Bednarz, and Ulrike Niemeier
Atmos. Chem. Phys., 22, 4557–4579, https://doi.org/10.5194/acp-22-4557-2022, https://doi.org/10.5194/acp-22-4557-2022, 2022
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This study assesses the impacts of climate interventions, using stratospheric sulfate aerosol and solar dimming on stratospheric ozone, based on three Earth system models with interactive stratospheric chemistry. The climate interventions have been applied to a high emission (baseline) scenario in order to reach global surface temperatures of a medium emission scenario. We find significant increases and decreases in total column ozone, depending on regions and seasons.
Andy Jones, Jim M. Haywood, Adam A. Scaife, Olivier Boucher, Matthew Henry, Ben Kravitz, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Roland Séférian, Simone Tilmes, and Daniele Visioni
Atmos. Chem. Phys., 22, 2999–3016, https://doi.org/10.5194/acp-22-2999-2022, https://doi.org/10.5194/acp-22-2999-2022, 2022
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Simulations by six Earth-system models of geoengineering by introducing sulfuric acid aerosols into the tropical stratosphere are compared. A robust impact on the northern wintertime North Atlantic Oscillation is found, exacerbating precipitation reduction over parts of southern Europe. In contrast, the models show no consistency with regard to impacts on the Quasi-Biennial Oscillation, although results do indicate a risk that the oscillation could become locked into a permanent westerly phase.
Yves Balkanski, Rémy Bonnet, Olivier Boucher, Ramiro Checa-Garcia, and Jérôme Servonnat
Atmos. Chem. Phys., 21, 11423–11435, https://doi.org/10.5194/acp-21-11423-2021, https://doi.org/10.5194/acp-21-11423-2021, 2021
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Earth system models have persistent biases that impinge on our ability to make robust future regional predictions of precipitation. For the last 15 years, there has been little improvement in these biases. This work presents an accurate representation of dust absorption based upon observed dust mineralogical composition and size distribution. The striking result is that this more accurate representation improves tropical precipitations for climate models with too weak an African monsoon.
Daniele Visioni, Douglas G. MacMartin, Ben Kravitz, Olivier Boucher, Andy Jones, Thibaut Lurton, Michou Martine, Michael J. Mills, Pierre Nabat, Ulrike Niemeier, Roland Séférian, and Simone Tilmes
Atmos. Chem. Phys., 21, 10039–10063, https://doi.org/10.5194/acp-21-10039-2021, https://doi.org/10.5194/acp-21-10039-2021, 2021
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A new set of simulations is used to investigate commonalities, differences and sources of uncertainty when simulating the injection of SO2 in the stratosphere in order to mitigate the effects of climate change (solar geoengineering). The models differ in how they simulate the aerosols and how they spread around the stratosphere, resulting in differences in projected regional impacts. Overall, however, the models agree that aerosols have the potential to mitigate the warming produced by GHGs.
Ulrich Schumann, Ian Poll, Roger Teoh, Rainer Koelle, Enrico Spinielli, Jarlath Molloy, George S. Koudis, Robert Baumann, Luca Bugliaro, Marc Stettler, and Christiane Voigt
Atmos. Chem. Phys., 21, 7429–7450, https://doi.org/10.5194/acp-21-7429-2021, https://doi.org/10.5194/acp-21-7429-2021, 2021
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The roughly 70 % reduction of air traffic during the COVID-19 pandemic from March–August 2020 compared to 2019 provides a test case for the relationship between air traffic density, contrails, and their radiative forcing of climate change. This paper investigates the induced traffic and contrail changes in a model study. Besides strong weather changes, the model results indicate aviation-induced cirrus and top-of-the-atmosphere irradiance changes, which can be tested with observations.
Yuan Zhang, Olivier Boucher, Philippe Ciais, Laurent Li, and Nicolas Bellouin
Geosci. Model Dev., 14, 2029–2039, https://doi.org/10.5194/gmd-14-2029-2021, https://doi.org/10.5194/gmd-14-2029-2021, 2021
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We investigated different methods to reconstruct spatiotemporal distribution of the fraction of diffuse radiation (Fdf) to qualify the aerosol impacts on GPP using the ORCHIDEE_DF land surface model. We find that climatological-averaging methods which dampen the variability of Fdf can cause significant bias in the modeled diffuse radiation impacts on GPP. Better methods to reconstruct Fdf are recommended.
Ben Kravitz, Douglas G. MacMartin, Daniele Visioni, Olivier Boucher, Jason N. S. Cole, Jim Haywood, Andy Jones, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Alan Robock, Roland Séférian, and Simone Tilmes
Atmos. Chem. Phys., 21, 4231–4247, https://doi.org/10.5194/acp-21-4231-2021, https://doi.org/10.5194/acp-21-4231-2021, 2021
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This study investigates multi-model response to idealized geoengineering (high CO2 with solar reduction) across two different generations of climate models. We find that, with the exception of a few cases, the results are unchanged between the different generations. This gives us confidence that broad conclusions about the response to idealized geoengineering are robust.
Claudia Tebaldi, Kevin Debeire, Veronika Eyring, Erich Fischer, John Fyfe, Pierre Friedlingstein, Reto Knutti, Jason Lowe, Brian O'Neill, Benjamin Sanderson, Detlef van Vuuren, Keywan Riahi, Malte Meinshausen, Zebedee Nicholls, Katarzyna B. Tokarska, George Hurtt, Elmar Kriegler, Jean-Francois Lamarque, Gerald Meehl, Richard Moss, Susanne E. Bauer, Olivier Boucher, Victor Brovkin, Young-Hwa Byun, Martin Dix, Silvio Gualdi, Huan Guo, Jasmin G. John, Slava Kharin, YoungHo Kim, Tsuyoshi Koshiro, Libin Ma, Dirk Olivié, Swapna Panickal, Fangli Qiao, Xinyao Rong, Nan Rosenbloom, Martin Schupfner, Roland Séférian, Alistair Sellar, Tido Semmler, Xiaoying Shi, Zhenya Song, Christian Steger, Ronald Stouffer, Neil Swart, Kaoru Tachiiri, Qi Tang, Hiroaki Tatebe, Aurore Voldoire, Evgeny Volodin, Klaus Wyser, Xiaoge Xin, Shuting Yang, Yongqiang Yu, and Tilo Ziehn
Earth Syst. Dynam., 12, 253–293, https://doi.org/10.5194/esd-12-253-2021, https://doi.org/10.5194/esd-12-253-2021, 2021
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We present an overview of CMIP6 ScenarioMIP outcomes from up to 38 participating ESMs according to the new SSP-based scenarios. Average temperature and precipitation projections according to a wide range of forcings, spanning a wider range than the CMIP5 projections, are documented as global averages and geographic patterns. Times of crossing various warming levels are computed, together with benefits of mitigation for selected pairs of scenarios. Comparisons with CMIP5 are also discussed.
Camilla W. Stjern, Bjørn H. Samset, Olivier Boucher, Trond Iversen, Jean-François Lamarque, Gunnar Myhre, Drew Shindell, and Toshihiko Takemura
Atmos. Chem. Phys., 20, 13467–13480, https://doi.org/10.5194/acp-20-13467-2020, https://doi.org/10.5194/acp-20-13467-2020, 2020
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The span between the warmest and coldest temperatures over a day is a climate parameter that influences both agriculture and human health. Using data from 10 models, we show how individual climate drivers such as greenhouse gases and aerosols produce distinctly different responses in this parameter in high-emission regions. Given the high uncertainty in future aerosol emissions, this improved understanding of the temperature responses may ultimately help these regions prepare for future changes.
Yuan Zhang, Ana Bastos, Fabienne Maignan, Daniel Goll, Olivier Boucher, Laurent Li, Alessandro Cescatti, Nicolas Vuichard, Xiuzhi Chen, Christof Ammann, M. Altaf Arain, T. Andrew Black, Bogdan Chojnicki, Tomomichi Kato, Ivan Mammarella, Leonardo Montagnani, Olivier Roupsard, Maria J. Sanz, Lukas Siebicke, Marek Urbaniak, Francesco Primo Vaccari, Georg Wohlfahrt, Will Woodgate, and Philippe Ciais
Geosci. Model Dev., 13, 5401–5423, https://doi.org/10.5194/gmd-13-5401-2020, https://doi.org/10.5194/gmd-13-5401-2020, 2020
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We improved the ORCHIDEE LSM by distinguishing diffuse and direct light in canopy and evaluated the new model with observations from 159 sites. Compared with the old model, the new model has better sunny GPP and reproduced the diffuse light fertilization effect observed at flux sites. Our simulations also indicate different mechanisms causing the observed GPP enhancement under cloudy conditions at different times. The new model has the potential to study large-scale impacts of aerosol changes.
Zebedee R. J. Nicholls, Malte Meinshausen, Jared Lewis, Robert Gieseke, Dietmar Dommenget, Kalyn Dorheim, Chen-Shuo Fan, Jan S. Fuglestvedt, Thomas Gasser, Ulrich Golüke, Philip Goodwin, Corinne Hartin, Austin P. Hope, Elmar Kriegler, Nicholas J. Leach, Davide Marchegiani, Laura A. McBride, Yann Quilcaille, Joeri Rogelj, Ross J. Salawitch, Bjørn H. Samset, Marit Sandstad, Alexey N. Shiklomanov, Ragnhild B. Skeie, Christopher J. Smith, Steve Smith, Katsumasa Tanaka, Junichi Tsutsui, and Zhiang Xie
Geosci. Model Dev., 13, 5175–5190, https://doi.org/10.5194/gmd-13-5175-2020, https://doi.org/10.5194/gmd-13-5175-2020, 2020
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Computational limits mean that we cannot run our most comprehensive climate models for all applications of interest. In such cases, reduced complexity models (RCMs) are used. Here, researchers working on 15 different models present the first systematic community effort to evaluate and compare RCMs: the Reduced Complexity Model Intercomparison Project (RCMIP). Our research ensures that users of RCMs can more easily evaluate the strengths, weaknesses and limitations of their tools.
Vivek K. Arora, Anna Katavouta, Richard G. Williams, Chris D. Jones, Victor Brovkin, Pierre Friedlingstein, Jörg Schwinger, Laurent Bopp, Olivier Boucher, Patricia Cadule, Matthew A. Chamberlain, James R. Christian, Christine Delire, Rosie A. Fisher, Tomohiro Hajima, Tatiana Ilyina, Emilie Joetzjer, Michio Kawamiya, Charles D. Koven, John P. Krasting, Rachel M. Law, David M. Lawrence, Andrew Lenton, Keith Lindsay, Julia Pongratz, Thomas Raddatz, Roland Séférian, Kaoru Tachiiri, Jerry F. Tjiputra, Andy Wiltshire, Tongwen Wu, and Tilo Ziehn
Biogeosciences, 17, 4173–4222, https://doi.org/10.5194/bg-17-4173-2020, https://doi.org/10.5194/bg-17-4173-2020, 2020
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Since the preindustrial period, land and ocean have taken up about half of the carbon emitted into the atmosphere by humans. Comparison of different earth system models with the carbon cycle allows us to assess how carbon uptake by land and ocean differs among models. This yields an estimate of uncertainty in our understanding of how land and ocean respond to increasing atmospheric CO2. This paper summarizes results from two such model intercomparison projects that use an idealized scenario.
Christopher J. Smith, Ryan J. Kramer, Gunnar Myhre, Kari Alterskjær, William Collins, Adriana Sima, Olivier Boucher, Jean-Louis Dufresne, Pierre Nabat, Martine Michou, Seiji Yukimoto, Jason Cole, David Paynter, Hideo Shiogama, Fiona M. O'Connor, Eddy Robertson, Andy Wiltshire, Timothy Andrews, Cécile Hannay, Ron Miller, Larissa Nazarenko, Alf Kirkevåg, Dirk Olivié, Stephanie Fiedler, Anna Lewinschal, Chloe Mackallah, Martin Dix, Robert Pincus, and Piers M. Forster
Atmos. Chem. Phys., 20, 9591–9618, https://doi.org/10.5194/acp-20-9591-2020, https://doi.org/10.5194/acp-20-9591-2020, 2020
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The spread in effective radiative forcing for both CO2 and aerosols is narrower in the latest CMIP6 (Coupled Model Intercomparison Project) generation than in CMIP5. For the case of CO2 it is likely that model radiation parameterisations have improved. Tropospheric and stratospheric radiative adjustments to the forcing behave differently for different forcing agents, and there is still significant diversity in how clouds respond to forcings, particularly for total anthropogenic forcing.
Prodromos Zanis, Dimitris Akritidis, Aristeidis K. Georgoulias, Robert J. Allen, Susanne E. Bauer, Olivier Boucher, Jason Cole, Ben Johnson, Makoto Deushi, Martine Michou, Jane Mulcahy, Pierre Nabat, Dirk Olivié, Naga Oshima, Adriana Sima, Michael Schulz, Toshihiko Takemura, and Konstantinos Tsigaridis
Atmos. Chem. Phys., 20, 8381–8404, https://doi.org/10.5194/acp-20-8381-2020, https://doi.org/10.5194/acp-20-8381-2020, 2020
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In this work, we use Coupled Model Intercomparison Project Phase 6 (CMIP6) simulations from 10 Earth system models (ESMs) and general circulation models (GCMs) to study the fast climate responses on pre-industrial climate, due to present-day aerosols. All models carried out two sets of simulations: a control experiment with all forcings set to the year 1850 and a perturbation experiment with all forcings identical to the control, except for aerosols with precursor emissions set to the year 2014.
Nicolas Bellouin, Will Davies, Keith P. Shine, Johannes Quaas, Johannes Mülmenstädt, Piers M. Forster, Chris Smith, Lindsay Lee, Leighton Regayre, Guy Brasseur, Natalia Sudarchikova, Idir Bouarar, Olivier Boucher, and Gunnar Myhre
Earth Syst. Sci. Data, 12, 1649–1677, https://doi.org/10.5194/essd-12-1649-2020, https://doi.org/10.5194/essd-12-1649-2020, 2020
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Quantifying the imbalance in the Earth's energy budget caused by human activities is important to understand and predict climate changes. This study presents new estimates of the imbalance caused by changes in atmospheric concentrations of carbon dioxide, methane, ozone, and particles of pollution. Over the period 2003–2017, the overall imbalance has been positive, indicating that the climate system has gained energy and will warm further.
Pierre Sepulchre, Arnaud Caubel, Jean-Baptiste Ladant, Laurent Bopp, Olivier Boucher, Pascale Braconnot, Patrick Brockmann, Anne Cozic, Yannick Donnadieu, Jean-Louis Dufresne, Victor Estella-Perez, Christian Ethé, Frédéric Fluteau, Marie-Alice Foujols, Guillaume Gastineau, Josefine Ghattas, Didier Hauglustaine, Frédéric Hourdin, Masa Kageyama, Myriam Khodri, Olivier Marti, Yann Meurdesoif, Juliette Mignot, Anta-Clarisse Sarr, Jérôme Servonnat, Didier Swingedouw, Sophie Szopa, and Delphine Tardif
Geosci. Model Dev., 13, 3011–3053, https://doi.org/10.5194/gmd-13-3011-2020, https://doi.org/10.5194/gmd-13-3011-2020, 2020
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Our paper describes IPSL-CM5A2, an Earth system model that can be integrated for long (several thousands of years) climate simulations. We describe the technical aspects, assess the model computing performance and evaluate the strengths and weaknesses of the model, by comparing pre-industrial and historical runs to the previous-generation model simulations and to observations. We also present a Cretaceous simulation as a case study to show how the model simulates deep-time paleoclimates.
Jonathan Elsey, Marc D. Coleman, Tom D. Gardiner, Kaah P. Menang, and Keith P. Shine
Atmos. Meas. Tech., 13, 2335–2361, https://doi.org/10.5194/amt-13-2335-2020, https://doi.org/10.5194/amt-13-2335-2020, 2020
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Water vapour is an important component in trying to understand the flows of energy between the Sun and Earth, since it is opaque to radiation emitted by both the surface and the Sun. In this paper, we study how it absorbs sunlight by way of its
continuum, a property which is poorly understood and with few measurements. Our results indicate that this continuum absorption may be more significant than previously thought, potentially impacting satellite observations and climate studies.
Samuel Rémy, Zak Kipling, Johannes Flemming, Olivier Boucher, Pierre Nabat, Martine Michou, Alessio Bozzo, Melanie Ades, Vincent Huijnen, Angela Benedetti, Richard Engelen, Vincent-Henri Peuch, and Jean-Jacques Morcrette
Geosci. Model Dev., 12, 4627–4659, https://doi.org/10.5194/gmd-12-4627-2019, https://doi.org/10.5194/gmd-12-4627-2019, 2019
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This article describes the IFS-AER aerosol module used operationally in the Integrated Forecasting System (IFS) cycle 45R1, operated by the ECMWF in the framework of the Copernicus Atmospheric Monitoring Services (CAMS). We describe the different parameterizations for aerosol sources, sinks, and how the aerosols are integrated in the larger atmospheric composition forecasting system. The skill of PM and AOD simulations against observations is improved compared to the older cycle 40R2.
Øivind Hodnebrog, Gunnar Myhre, Bjørn H. Samset, Kari Alterskjær, Timothy Andrews, Olivier Boucher, Gregory Faluvegi, Dagmar Fläschner, Piers M. Forster, Matthew Kasoar, Alf Kirkevåg, Jean-Francois Lamarque, Dirk Olivié, Thomas B. Richardson, Dilshad Shawki, Drew Shindell, Keith P. Shine, Philip Stier, Toshihiko Takemura, Apostolos Voulgarakis, and Duncan Watson-Parris
Atmos. Chem. Phys., 19, 12887–12899, https://doi.org/10.5194/acp-19-12887-2019, https://doi.org/10.5194/acp-19-12887-2019, 2019
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Different greenhouse gases (e.g. CO2) and aerosols (e.g. black carbon) impact the Earth’s water cycle differently. Here we investigate how various gases and particles impact atmospheric water vapour and its lifetime, i.e., the average number of days that water vapour stays in the atmosphere after evaporation and before precipitation. We find that this lifetime could increase substantially by the end of this century, indicating that important changes in precipitation patterns are excepted.
Sauvik Santra, Shubha Verma, Koji Fujita, Indrajit Chakraborty, Olivier Boucher, Toshihiko Takemura, John F. Burkhart, Felix Matt, and Mukesh Sharma
Atmos. Chem. Phys., 19, 2441–2460, https://doi.org/10.5194/acp-19-2441-2019, https://doi.org/10.5194/acp-19-2441-2019, 2019
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The present study provided information on specific glaciers over the Hindu Kush Himalayan region identified as being vulnerable to BC-induced impacts (affected by high BC-induced snow albedo reduction in addition to being sensitive to BC-induced impacts), thus impacting the downstream hydrology. The source-specific contribution to atmospheric BC aerosols by emission sources led to identifying the potential emission source, which was distinctive over south and north to 30° N.
Jeronimo Escribano, Alessio Bozzo, Philippe Dubuisson, Johannes Flemming, Robin J. Hogan, Laurent C.-Labonnote, and Olivier Boucher
Geosci. Model Dev., 12, 805–827, https://doi.org/10.5194/gmd-12-805-2019, https://doi.org/10.5194/gmd-12-805-2019, 2019
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Accurate shortwave radiance computations are becoming increasingly important for some applications in atmospheric composition. In this work we propose a benchmark protocol and dataset to asses the accuracy and computing runtime of radiance calculations of radiative transfer models. It is applied to four models, showing the potential of this benchmark to evaluate the model performance under a variety of atmospheric conditions, viewing geometries, aerosol loading, and optical properties.
Ben Kravitz, Philip J. Rasch, Hailong Wang, Alan Robock, Corey Gabriel, Olivier Boucher, Jason N. S. Cole, Jim Haywood, Duoying Ji, Andy Jones, Andrew Lenton, John C. Moore, Helene Muri, Ulrike Niemeier, Steven Phipps, Hauke Schmidt, Shingo Watanabe, Shuting Yang, and Jin-Ho Yoon
Atmos. Chem. Phys., 18, 13097–13113, https://doi.org/10.5194/acp-18-13097-2018, https://doi.org/10.5194/acp-18-13097-2018, 2018
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Marine cloud brightening has been proposed as a means of geoengineering/climate intervention, or deliberately altering the climate system to offset anthropogenic climate change. In idealized simulations that highlight contrasts between land and ocean, we find that the globe warms, including the ocean due to transport of heat from land. This study reinforces that no net energy input into the Earth system does not mean that temperature will necessarily remain unchanged.
Angela Benedetti, Jeffrey S. Reid, Peter Knippertz, John H. Marsham, Francesca Di Giuseppe, Samuel Rémy, Sara Basart, Olivier Boucher, Ian M. Brooks, Laurent Menut, Lucia Mona, Paolo Laj, Gelsomina Pappalardo, Alfred Wiedensohler, Alexander Baklanov, Malcolm Brooks, Peter R. Colarco, Emilio Cuevas, Arlindo da Silva, Jeronimo Escribano, Johannes Flemming, Nicolas Huneeus, Oriol Jorba, Stelios Kazadzis, Stefan Kinne, Thomas Popp, Patricia K. Quinn, Thomas T. Sekiyama, Taichu Tanaka, and Enric Terradellas
Atmos. Chem. Phys., 18, 10615–10643, https://doi.org/10.5194/acp-18-10615-2018, https://doi.org/10.5194/acp-18-10615-2018, 2018
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Numerical prediction of aerosol particle properties has become an important activity at many research and operational weather centers. This development is due to growing interest from a diverse set of stakeholders, such as air quality regulatory bodies, aviation authorities, solar energy plant managers, climate service providers, and health professionals. This paper describes the advances in the field and sets out requirements for observations for the sustainability of these activities.
Tao Tang, Drew Shindell, Bjørn H. Samset, Oliviér Boucher, Piers M. Forster, Øivind Hodnebrog, Gunnar Myhre, Jana Sillmann, Apostolos Voulgarakis, Timothy Andrews, Gregory Faluvegi, Dagmar Fläschner, Trond Iversen, Matthew Kasoar, Viatcheslav Kharin, Alf Kirkevåg, Jean-Francois Lamarque, Dirk Olivié, Thomas Richardson, Camilla W. Stjern, and Toshihiko Takemura
Atmos. Chem. Phys., 18, 8439–8452, https://doi.org/10.5194/acp-18-8439-2018, https://doi.org/10.5194/acp-18-8439-2018, 2018
Christoph Kleinschmitt, Olivier Boucher, and Ulrich Platt
Atmos. Chem. Phys., 18, 2769–2786, https://doi.org/10.5194/acp-18-2769-2018, https://doi.org/10.5194/acp-18-2769-2018, 2018
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We use a state-of-the-art stratospheric aerosol model to study geoengineering through stratospheric sulfur injections. We find that the efficiency may decrease more drastically for larger injections than previously estimated and that injections at higher altitude are not more effective. This study may provide additional evidence that this proposed geoengineering technique is still more complicated, probably less effective, and may implicate stronger side effects than initially thought.
Roland Séférian, Sunghye Baek, Olivier Boucher, Jean-Louis Dufresne, Bertrand Decharme, David Saint-Martin, and Romain Roehrig
Geosci. Model Dev., 11, 321–338, https://doi.org/10.5194/gmd-11-321-2018, https://doi.org/10.5194/gmd-11-321-2018, 2018
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This paper presents a new interactive scheme for ocean surface albedo suited for the current generation of Earth system models. This scheme computes the ocean surface albedo accounting for the spectral dependence (across a range of wavelengths between 200 and 4000 nm), the characteristics of incident solar radiation (direct of diffuse), the effects of surface winds, chlorophyll content and whitecaps in addition to the canonical solar zenith angle dependence.
Camilla W. Stjern, Helene Muri, Lars Ahlm, Olivier Boucher, Jason N. S. Cole, Duoying Ji, Andy Jones, Jim Haywood, Ben Kravitz, Andrew Lenton, John C. Moore, Ulrike Niemeier, Steven J. Phipps, Hauke Schmidt, Shingo Watanabe, and Jón Egill Kristjánsson
Atmos. Chem. Phys., 18, 621–634, https://doi.org/10.5194/acp-18-621-2018, https://doi.org/10.5194/acp-18-621-2018, 2018
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Marine cloud brightening (MCB) has been proposed to help limit global warming. We present here the first multi-model assessment of idealized MCB simulations from the Geoengineering Model Intercomparison Project. While all models predict a global cooling as intended, there is considerable spread between the models both in terms of radiative forcing and the climate response, largely linked to the substantial differences in the models' representation of clouds.
Borgar Aamaas, Terje K. Berntsen, Jan S. Fuglestvedt, Keith P. Shine, and William J. Collins
Atmos. Chem. Phys., 17, 10795–10809, https://doi.org/10.5194/acp-17-10795-2017, https://doi.org/10.5194/acp-17-10795-2017, 2017
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The climate impacts for emissions of different pollutants can be made comparable with weighting factors. This article estimates these weights based on temperature change for short-lived pollutants, such as methane and black carbon. Emissions from different seasons and regions are compared, for instance Europe and East Asia. The responses are calculated for four regions, where we see that the responses can be much higher in the Arctic than globally in some cases.
Christoph Kleinschmitt, Olivier Boucher, Slimane Bekki, François Lott, and Ulrich Platt
Geosci. Model Dev., 10, 3359–3378, https://doi.org/10.5194/gmd-10-3359-2017, https://doi.org/10.5194/gmd-10-3359-2017, 2017
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Stratospheric aerosols play an important role in the climate system by affecting the Earth's radiative budget. In this article we present the newly developed LMDZ-S3A model and assess its performance against observations in periods of low and high aerosol loading. The model may serve as a tool to study the climate impacts of volcanic eruptions, as well as the deliberate injection of aerosols into the stratosphere, which has been proposed as a method of geoengineering to abate global warming.
Marianne T. Lund, Borgar Aamaas, Terje Berntsen, Lisa Bock, Ulrike Burkhardt, Jan S. Fuglestvedt, and Keith P. Shine
Earth Syst. Dynam., 8, 547–563, https://doi.org/10.5194/esd-8-547-2017, https://doi.org/10.5194/esd-8-547-2017, 2017
Jerónimo Escribano, Olivier Boucher, Frédéric Chevallier, and Nicolás Huneeus
Atmos. Chem. Phys., 17, 7111–7126, https://doi.org/10.5194/acp-17-7111-2017, https://doi.org/10.5194/acp-17-7111-2017, 2017
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Top-down estimates of mineral dust flux usually rely on a single observational dataset whose observational errors propagate onto the emission estimates. Aerosol optical depth from five satellites are assimilated one by one into a source inversion system over northern Africa. We find a relatively large dispersion in flux estimates among the five experiments, which can likely be attributed to differences in the assimilated observational datasets and their associated error statistics.
William J. Collins, Jean-François Lamarque, Michael Schulz, Olivier Boucher, Veronika Eyring, Michaela I. Hegglin, Amanda Maycock, Gunnar Myhre, Michael Prather, Drew Shindell, and Steven J. Smith
Geosci. Model Dev., 10, 585–607, https://doi.org/10.5194/gmd-10-585-2017, https://doi.org/10.5194/gmd-10-585-2017, 2017
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We have designed a set of climate model experiments called the Aerosol Chemistry Model Intercomparison Project (AerChemMIP). These are designed to quantify the climate and air quality impacts of aerosols and chemically reactive gases in the climate models that are used to simulate past and future climate. We hope that many climate modelling centres will choose to run these experiments to help understand the contribution of aerosols and chemistry to climate change.
Thomas Gasser, Philippe Ciais, Olivier Boucher, Yann Quilcaille, Maxime Tortora, Laurent Bopp, and Didier Hauglustaine
Geosci. Model Dev., 10, 271–319, https://doi.org/10.5194/gmd-10-271-2017, https://doi.org/10.5194/gmd-10-271-2017, 2017
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Simple models of the Earth system are useful, especially because of their high computing efficiency. This work describes the OSCAR model: a new simple Earth system model calibrated on state-of-the-art complex models. It will add to the pool of the few simple models currently used by the community, and it will therefore improve the robustness of future studies. Its source code is available upon request.
Katsumasa Tanaka, Atsumu Ohmura, Doris Folini, Martin Wild, and Nozomu Ohkawara
Atmos. Chem. Phys., 16, 13969–14001, https://doi.org/10.5194/acp-16-13969-2016, https://doi.org/10.5194/acp-16-13969-2016, 2016
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Surface solar radiation observed in Japan generally shows a strong decline until the end of the 1980s and then a recovery up until around 2000. A substantial number of measurement stations are located close to populated areas and are speculated to have been influenced by air pollution. However, data obtained at 14 meteorological observatories suggest that the large decadal variations in surface solar radiation occur on a large scale and not limited to urban areas.
Borgar Aamaas, Terje K. Berntsen, Jan S. Fuglestvedt, Keith P. Shine, and Nicolas Bellouin
Atmos. Chem. Phys., 16, 7451–7468, https://doi.org/10.5194/acp-16-7451-2016, https://doi.org/10.5194/acp-16-7451-2016, 2016
Adel Imamovic, Katsumasa Tanaka, Doris Folini, and Martin Wild
Atmos. Chem. Phys., 16, 2719–2725, https://doi.org/10.5194/acp-16-2719-2016, https://doi.org/10.5194/acp-16-2719-2016, 2016
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Systematic measurements of surface solar radiation revealed a worldwide decrease from the 1960s to the mid-1980s. The role of urbanization for this so called global dimming is still under debate. We developed a set of population-data based urbanization indicators and found no correlation between urbanization and global dimming for Europe and Japan, while an urbanization impact can't be precluded for Asia. It is thus called into question whether the global dimming was mainly a local phenomenon.
H. Eskes, V. Huijnen, A. Arola, A. Benedictow, A.-M. Blechschmidt, E. Botek, O. Boucher, I. Bouarar, S. Chabrillat, E. Cuevas, R. Engelen, H. Flentje, A. Gaudel, J. Griesfeller, L. Jones, J. Kapsomenakis, E. Katragkou, S. Kinne, B. Langerock, M. Razinger, A. Richter, M. Schultz, M. Schulz, N. Sudarchikova, V. Thouret, M. Vrekoussis, A. Wagner, and C. Zerefos
Geosci. Model Dev., 8, 3523–3543, https://doi.org/10.5194/gmd-8-3523-2015, https://doi.org/10.5194/gmd-8-3523-2015, 2015
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The MACC project is preparing the operational atmosphere service of the European Copernicus Programme, and uses data assimilation to combine atmospheric models with available observations. Our paper provides an overview of the aerosol and trace gas validation activity of MACC. Topics are the validation requirements, the measurement data, the assimilation systems, the upgrade procedure, operational aspects and the scoring methods. A summary is provided of recent results, including special events.
B. Kravitz, A. Robock, S. Tilmes, O. Boucher, J. M. English, P. J. Irvine, A. Jones, M. G. Lawrence, M. MacCracken, H. Muri, J. C. Moore, U. Niemeier, S. J. Phipps, J. Sillmann, T. Storelvmo, H. Wang, and S. Watanabe
Geosci. Model Dev., 8, 3379–3392, https://doi.org/10.5194/gmd-8-3379-2015, https://doi.org/10.5194/gmd-8-3379-2015, 2015
A. Stohl, B. Aamaas, M. Amann, L. H. Baker, N. Bellouin, T. K. Berntsen, O. Boucher, R. Cherian, W. Collins, N. Daskalakis, M. Dusinska, S. Eckhardt, J. S. Fuglestvedt, M. Harju, C. Heyes, Ø. Hodnebrog, J. Hao, U. Im, M. Kanakidou, Z. Klimont, K. Kupiainen, K. S. Law, M. T. Lund, R. Maas, C. R. MacIntosh, G. Myhre, S. Myriokefalitakis, D. Olivié, J. Quaas, B. Quennehen, J.-C. Raut, S. T. Rumbold, B. H. Samset, M. Schulz, Ø. Seland, K. P. Shine, R. B. Skeie, S. Wang, K. E. Yttri, and T. Zhu
Atmos. Chem. Phys., 15, 10529–10566, https://doi.org/10.5194/acp-15-10529-2015, https://doi.org/10.5194/acp-15-10529-2015, 2015
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This paper presents a summary of the findings of the ECLIPSE EU project. The project has investigated the climate and air quality impacts of short-lived climate pollutants (especially methane, ozone, aerosols) and has designed a global mitigation strategy that maximizes co-benefits between air quality and climate policy. Transient climate model simulations allowed quantifying the impacts on temperature (e.g., reduction in global warming by 0.22K for the decade 2041-2050) and precipitation.
E. A. Irvine and K. P. Shine
Earth Syst. Dynam., 6, 555–568, https://doi.org/10.5194/esd-6-555-2015, https://doi.org/10.5194/esd-6-555-2015, 2015
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Aviation impacts on climate via contrails, which are often clearly visible in the sky. Contrail formation requires particular cold/moist atmospheric conditions at aircraft cruise altitudes. Climate change is expected to change these conditions. Using simulations from several climate models we conclude that, by 2100, the probability of contrail formation could decrease from 11 to 7%, mostly due to changing conditions in the tropics. There is no consensus on the likely change in mid-latitudes.
K. P. Shine, R. P. Allan, W. J. Collins, and J. S. Fuglestvedt
Earth Syst. Dynam., 6, 525–540, https://doi.org/10.5194/esd-6-525-2015, https://doi.org/10.5194/esd-6-525-2015, 2015
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Emissions due to human activity impact on rainfall. This impact depends on the properties of the gases or particles that are emitted. This paper uses improved understanding of relevant processes to produce a new measure, called the Global Precipitation-change Potential, which allows a direct comparison of the effect of different emissions on global-mean rainfall. Carbon dioxide, in the years following its emission, is shown to be less effective than methane emissions at causing rainfall change.
V. N. Aswathy, O. Boucher, M. Quaas, U. Niemeier, H. Muri, J. Mülmenstädt, and J. Quaas
Atmos. Chem. Phys., 15, 9593–9610, https://doi.org/10.5194/acp-15-9593-2015, https://doi.org/10.5194/acp-15-9593-2015, 2015
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Simulations conducted in the GeoMIP and IMPLICC model intercomparison studies for climate engineering by stratospheric sulfate injection and marine cloud brightening via sea salt are analysed and compared to the reference scenario RCP4.5. The focus is on extremes in surface temperature and precipitation. It is found that the extreme changes mostly follow the mean changes and that extremes are also in general well mitigated, except for in polar regions.
R. Wang, Y. Balkanski, O. Boucher, L. Bopp, A. Chappell, P. Ciais, D. Hauglustaine, J. Peñuelas, and S. Tao
Atmos. Chem. Phys., 15, 6247–6270, https://doi.org/10.5194/acp-15-6247-2015, https://doi.org/10.5194/acp-15-6247-2015, 2015
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This study makes a first attempt to estimate the temporal trend of Fe emissions from anthropogenic and natural combustion sources from 1960 to 2007 and the emissions of Fe from mineral dust based on a recent mineralogical database. The new emission inventory is introduced into a global aerosol model. The simulated total Fe and soluble Fe concentrations in surface air as well as the deposition of total Fe are evaluated by observations over major continental and oceanic regions globally.
C. R. MacIntosh, K. P. Shine, and W. J. Collins
Atmos. Chem. Phys., 15, 3957–3969, https://doi.org/10.5194/acp-15-3957-2015, https://doi.org/10.5194/acp-15-3957-2015, 2015
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This study examines quantitatively the impact of methodological choices, in particular of averaging of multi-model ensembles, on climate metrics for ozone precursors.
Estimates of the standard deviation of radiative forcing (RF), global warming and temperature potential (GWP, GTP) from ensemble-mean input fields generally overestimate the true value.
The multi-model average fields are appropriate for calculating mean metrics, but are not a reliable method for calculating the uncertainty.
M. Ménégoz, G. Krinner, Y. Balkanski, O. Boucher, A. Cozic, S. Lim, P. Ginot, P. Laj, H. Gallée, P. Wagnon, A. Marinoni, and H. W. Jacobi
Atmos. Chem. Phys., 14, 4237–4249, https://doi.org/10.5194/acp-14-4237-2014, https://doi.org/10.5194/acp-14-4237-2014, 2014
V. Grewe, C. Frömming, S. Matthes, S. Brinkop, M. Ponater, S. Dietmüller, P. Jöckel, H. Garny, E. Tsati, K. Dahlmann, O. A. Søvde, J. Fuglestvedt, T. K. Berntsen, K. P. Shine, E. A. Irvine, T. Champougny, and P. Hullah
Geosci. Model Dev., 7, 175–201, https://doi.org/10.5194/gmd-7-175-2014, https://doi.org/10.5194/gmd-7-175-2014, 2014
N. Huneeus, O. Boucher, and F. Chevallier
Atmos. Chem. Phys., 13, 6555–6573, https://doi.org/10.5194/acp-13-6555-2013, https://doi.org/10.5194/acp-13-6555-2013, 2013
P. Stier, N. A. J. Schutgens, N. Bellouin, H. Bian, O. Boucher, M. Chin, S. Ghan, N. Huneeus, S. Kinne, G. Lin, X. Ma, G. Myhre, J. E. Penner, C. A. Randles, B. Samset, M. Schulz, T. Takemura, F. Yu, H. Yu, and C. Zhou
Atmos. Chem. Phys., 13, 3245–3270, https://doi.org/10.5194/acp-13-3245-2013, https://doi.org/10.5194/acp-13-3245-2013, 2013
F. Joos, R. Roth, J. S. Fuglestvedt, G. P. Peters, I. G. Enting, W. von Bloh, V. Brovkin, E. J. Burke, M. Eby, N. R. Edwards, T. Friedrich, T. L. Frölicher, P. R. Halloran, P. B. Holden, C. Jones, T. Kleinen, F. T. Mackenzie, K. Matsumoto, M. Meinshausen, G.-K. Plattner, A. Reisinger, J. Segschneider, G. Shaffer, M. Steinacher, K. Strassmann, K. Tanaka, A. Timmermann, and A. J. Weaver
Atmos. Chem. Phys., 13, 2793–2825, https://doi.org/10.5194/acp-13-2793-2013, https://doi.org/10.5194/acp-13-2793-2013, 2013
M. T. Woodhouse, G. W. Mann, K. S. Carslaw, and O. Boucher
Atmos. Chem. Phys., 13, 2723–2733, https://doi.org/10.5194/acp-13-2723-2013, https://doi.org/10.5194/acp-13-2723-2013, 2013
N. Bellouin, J. Quaas, J.-J. Morcrette, and O. Boucher
Atmos. Chem. Phys., 13, 2045–2062, https://doi.org/10.5194/acp-13-2045-2013, https://doi.org/10.5194/acp-13-2045-2013, 2013
Related subject area
Subject: Climate and Earth System | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Contrasting the roles of regional anthropogenic aerosols from the western and eastern hemispheres in driving the 1980–2020 Pacific multi-decadal variations
A new method for diagnosing effective radiative forcing from aerosol–cloud interactions in climate models
Climate variability can outweigh the influence of climate mean changes for extreme precipitation under global warming
Using a region-specific ice-nucleating particle parameterization improves the representation of Arctic clouds in a global climate model
Small emission sources in aggregate disproportionately account for a large majority of total methane emissions from the US oil and gas sector
Technical note: Recommendations for diagnosing cloud feedbacks and rapid cloud adjustments using cloud radiative kernels
Satellite quantification of methane emissions from South American countries: a high-resolution inversion of TROPOMI and GOSAT observations
To what extent does the CO2 diurnal cycle impact flux estimates derived from global and regional inversions?
Can general circulation models (GCMs) represent cloud liquid water path adjustments to aerosol–cloud interactions?
Constraining net long-term climate feedback from satellite-observed internal variability possible by the mid-2030s
Investigating the limiting aircraft design-dependent and environmental factors of persistent contrail formation
Effects of 2010–2045 climate change on ozone levels in China under carbon neutrality scenario: Key meteorological parameters and processes
Highly-resolved satellite remote sensing based land-use change inventory yields weaker surface albedo-induced global cooling
Measurement report: Can Zenith Wet Delay from GNSS "see" atmospheric turbulence? Insights from case studies across diverse climate zones
Investigation of the characteristics of low-level jets over North America in a convection-permitting Weather Research and Forecasting simulation
Impacts of tropical cyclone–heat wave compound events on surface ozone in eastern China: comparison between the Yangtze River and Pearl River deltas
The 2023 global warming spike was driven by the El Niño–Southern Oscillation
Present-day methane shortwave absorption mutes surface warming relative to preindustrial conditions
A novel method for detecting tropopause structures based on the bi-Gaussian function
Too cold, too saturated? Evaluating climate models at the gateway to the Arctic
Unraveling the discrepancies between Eulerian and Lagrangian moisture tracking models in monsoon- and westerly-dominated basins of the Tibetan Plateau
Increasing aerosol direct effect despite declining global emissions in MPI-ESM1.2
Multi-scale variability of southeastern Australian wind resources
Parameterizations for global thundercloud corona discharge distributions
Relative humidity over ice as a key variable for Northern Hemisphere midlatitude tropopause inversion layers
Modelled surface climate response to Icelandic effusive volcanic eruptions: Sensitivity to season and size
Technical note: Posterior uncertainty estimation via a Monte Carlo procedure specialized for 4D-Var data assimilation
Understanding the role of contrails and contrail cirrus in climate change: a global perspective
Interannual variations in Siberian carbon uptake and carbon release period
Using historical temperature to constrain the climate sensitivity, the transient climate response, and aerosol-induced cooling
Weak surface temperature effects of recent reductions in shipping SO2 emissions, with quantification confounded by internal variability
Future reduction of cold extremes over East Asia due to thermodynamic and dynamic warming
General circulation models simulate negative liquid water path–droplet number correlations, but anthropogenic aerosols still increase simulated liquid water path
Global scenarios of anthropogenic mercury emissions
Impact of Asian aerosols on the summer monsoon strongly modulated by regional precipitation biases
Opinion: Optimizing climate models with process knowledge, resolution, and artificial intelligence
Assessing methane emissions from collapsing Venezuelan oil production using TROPOMI
Simulation of ozone–vegetation coupling and feedback in China using multiple ozone damage schemes
Opinion: Can uncertainty in climate sensitivity be narrowed further?
Emission Inventory Development for Spatiotemporal Release of Vanadium from Anthropogenic Sources in China
Significant human health co-benefits of mitigating African emissions
Water vapour exchange between the atmospheric boundary layer and free troposphere over eastern China: seasonal characteristics and the El Niño–Southern Oscillation anomaly
Strong aerosol cooling alone does not explain cold-biased mid-century temperatures in CMIP6 models
Air pollution reductions caused by the COVID-19 lockdown open up a way to preserve the Himalayan glaciers
Modeling atmosphere–land interactions at a rainforest site – a case study using Amazon Tall Tower Observatory (ATTO) measurements and reanalysis data
Chenrui Diao, Yangyang Xu, Aixue Hu, and Zhili Wang
Atmos. Chem. Phys., 25, 2167–2180, https://doi.org/10.5194/acp-25-2167-2025, https://doi.org/10.5194/acp-25-2167-2025, 2025
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Industrial aerosol increases in Asia and reductions in North America and Europe in 1980–2020 influenced climate changes over the Pacific Ocean differently. Asian aerosols caused El Niño-like temperature patterns and slightly weakened the natural variation in the North Pacific, while reduced emissions of western countries led to extensive warming in middle–high latitudes of the North Pacific. Human impacts on the Pacific climate may change when emission reduction occurs over Asia in the future.
Brandon M. Duran, Casey J. Wall, Nicholas J. Lutsko, Takuro Michibata, Po-Lun Ma, Yi Qin, Margaret L. Duffy, Brian Medeiros, and Matvey Debolskiy
Atmos. Chem. Phys., 25, 2123–2146, https://doi.org/10.5194/acp-25-2123-2025, https://doi.org/10.5194/acp-25-2123-2025, 2025
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We use satellite simulator data generated by global climate models to investigate how aerosol particles impact the radiative properties of liquid clouds. Specifically, we quantify the radiative perturbations arising from aerosol-driven changes in the number density of cloud droplets, the vertically integrated cloud water mass, and the cloud amount. Our results show that, in models, aerosol effects on the number density of cloud droplets contribute the most to anthropogenic climate forcing.
Kalle Nordling, Nora L. S. Fahrenbach, and Bjørn H. Samset
Atmos. Chem. Phys., 25, 1659–1684, https://doi.org/10.5194/acp-25-1659-2025, https://doi.org/10.5194/acp-25-1659-2025, 2025
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People experience daily weather, not changes in monthly averages. We investigate the likelihood of events, which occurred once every 10 years in the pre-industrial era. We analyze how summertime precipitation and daily maximum temperature events evolve. Our focus is on understanding the role of day-to-day variability in the change in the number of extreme weather days. We find that in most regions, a change in variability is the primary driver for change in summertime extreme precipitation.
Astrid B. Gjelsvik, Robert O. David, Tim Carlsen, Franziska Hellmuth, Stefan Hofer, Zachary McGraw, Harald Sodemann, and Trude Storelvmo
Atmos. Chem. Phys., 25, 1617–1637, https://doi.org/10.5194/acp-25-1617-2025, https://doi.org/10.5194/acp-25-1617-2025, 2025
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Ice formation in clouds has a substantial impact on radiation and precipitation and must be realistically simulated in order to understand present and future Arctic climate. Rare aerosols known as ice-nucleating particles can play an important role in cloud ice formation, but their representation in global climate models is not well suited for the Arctic. In this study, the simulation of cloud phase is improved when the representation of these particles is constrained by Arctic observations.
James P. Williams, Mark Omara, Anthony Himmelberger, Daniel Zavala-Araiza, Katlyn MacKay, Joshua Benmergui, Maryann Sargent, Steven C. Wofsy, Steven P. Hamburg, and Ritesh Gautam
Atmos. Chem. Phys., 25, 1513–1532, https://doi.org/10.5194/acp-25-1513-2025, https://doi.org/10.5194/acp-25-1513-2025, 2025
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We utilize peer-reviewed facility-level oil and gas methane emission rate data gathered in prior work to estimate the relative contributions of methane sources emitting at different emission rates in the United States. We find that the majority of total methane emissions in the US oil and gas sector stem from a large number of small sources emitting in aggregate, corroborating findings from several other studies.
Mark D. Zelinka, Li-Wei Chao, Timothy A. Myers, Yi Qin, and Stephen A. Klein
Atmos. Chem. Phys., 25, 1477–1495, https://doi.org/10.5194/acp-25-1477-2025, https://doi.org/10.5194/acp-25-1477-2025, 2025
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Clouds lie at the heart of uncertainty in both climate sensitivity and radiative forcing, making it imperative to properly diagnose their radiative effects. Here we provide a recommended methodology and code base for the community to use in performing such diagnoses using cloud radiative kernels. We show that properly accounting for changes in obscuration of lower-level clouds by upper-level clouds is important for accurate diagnosis and attribution of cloud feedbacks and adjustments.
Sarah E. Hancock, Daniel J. Jacob, Zichong Chen, Hannah Nesser, Aaron Davitt, Daniel J. Varon, Melissa P. Sulprizio, Nicholas Balasus, Lucas A. Estrada, María Cazorla, Laura Dawidowski, Sebastián Diez, James D. East, Elise Penn, Cynthia A. Randles, John Worden, Ilse Aben, Robert J. Parker, and Joannes D. Maasakkers
Atmos. Chem. Phys., 25, 797–817, https://doi.org/10.5194/acp-25-797-2025, https://doi.org/10.5194/acp-25-797-2025, 2025
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We quantify 2021 methane emissions in South America at up to 25 km × 25 km resolution using satellite methane observations. We find a 55 % upward adjustment to anthropogenic emission inventories, including those reported to the UN Framework Convention on Climate Change under the Paris Agreement. Our estimates match inventories for Brazil, Bolivia, and Paraguay but are much higher for other countries. Livestock emissions (65 % of anthropogenic emissions) show the largest discrepancies.
Saqr Munassar, Christian Rödenbeck, Michał Gałkowski, Frank-Thomas Koch, Kai U. Totsche, Santiago Botía, and Christoph Gerbig
Atmos. Chem. Phys., 25, 639–656, https://doi.org/10.5194/acp-25-639-2025, https://doi.org/10.5194/acp-25-639-2025, 2025
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CO2 mole fractions simulated over a global set of stations showed an overestimation of CO2 if the diurnal cycle is missing in biogenic fluxes. This leads to biases in the estimated fluxes derived from the regional-scale inversions. Interannual variability of estimated biogenic fluxes is also affected by the exclusion of the CO2 diurnal cycle. The findings point to the importance of including the diurnal variations of CO2 in the biogenic fluxes used as priors in global and regional inversions.
Johannes Mülmenstädt, Andrew S. Ackerman, Ann M. Fridlind, Meng Huang, Po-Lun Ma, Naser Mahfouz, Susanne E. Bauer, Susannah M. Burrows, Matthew W. Christensen, Sudhakar Dipu, Andrew Gettelman, L. Ruby Leung, Florian Tornow, Johannes Quaas, Adam C. Varble, Hailong Wang, Kai Zhang, and Youtong Zheng
Atmos. Chem. Phys., 24, 13633–13652, https://doi.org/10.5194/acp-24-13633-2024, https://doi.org/10.5194/acp-24-13633-2024, 2024
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Stratocumulus clouds play a large role in Earth's climate by reflecting incoming solar energy back to space. Turbulence at stratocumulus cloud top mixes in dry, warm air, which can lead to cloud dissipation. This process is challenging for coarse-resolution global models to represent. We show that global models nevertheless agree well with our process understanding. Global models also think the process is less important for the climate than other lines of evidence have led us to conclude.
Alejandro Uribe, Frida A.-M. Bender, and Thorsten Mauritsen
Atmos. Chem. Phys., 24, 13371–13384, https://doi.org/10.5194/acp-24-13371-2024, https://doi.org/10.5194/acp-24-13371-2024, 2024
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Our study explores climate feedbacks, vital for understanding global warming. It links them to shifts in Earth's energy balance at the atmosphere's top due to natural temperature variations. It takes roughly 50 years to establish this connection. Combined satellite observations and reanalysis suggest that Earth cools more than expected under carbon dioxide influence. However, continuous satellite data until at least the mid-2030s are crucial for refining our understanding of climate feedbacks.
Liam Megill and Volker Grewe
EGUsphere, https://doi.org/10.5194/egusphere-2024-3398, https://doi.org/10.5194/egusphere-2024-3398, 2024
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This study uses ERA5 data to better understand the relative importance of the factors limiting persistent contrail formation. We develop climatological relationships to estimate potential persistent contrail formation for existing as well as future aircraft and propulsion system designs. We identify latitudes and pressure levels where the introduction of novel aircraft designs would result in significant changes in potential persistent contrail formation compared to conventional aircraft.
Ling Kang, Hong Liao, Ke Li, Xu Yue, Yang Yang, and Ye Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-3470, https://doi.org/10.5194/egusphere-2024-3470, 2024
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Climate change over 2010–2045 under carbon neutrality scenario is simulated to increase ozone levels in China in the model of Global Change and Air Pollution version 2.0. Future climate change increases summertime MDA8 O3 levels by 2.3, 4.7, and 3.0 ppbv in eastern China, North China Plain, and Yangtze River Delta, respectively. Temperature, radiation, and RH are the key meteorological parameters and net chemical production is the key process for climate-driven ozone increases in eastern China.
Xiaohu Jian, Xiaodong Zhang, Xinrui Liu, Kaijie Chen, Tao Huang, Shu Tao, Junfeng Liu, Hong Gao, Yuan Zhao, Ruiyu Zhugu, and Jianmin Ma
EGUsphere, https://doi.org/10.5194/egusphere-2024-1497, https://doi.org/10.5194/egusphere-2024-1497, 2024
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We implemented a new global land use change (LUC) dataset on a 5 km×5 km resolution from 1982 to 2010 into a compact earth system model OSCAR and carried out extensive multiple model scenario simulations. Our result reveals that the global radiative forcing (RF) induced by LUC driving surface albedo change is -0.12 W m-2, 20 % lower than IPCC, and vegetation changes play a key role in RF evolution, which provides an important references for the assessment of earth energy balance.
Gael Kermarrec, Xavier Calbet, Zhiguo Deng, and Cintia Carbajal Henken
EGUsphere, https://doi.org/10.5194/egusphere-2024-2680, https://doi.org/10.5194/egusphere-2024-2680, 2024
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Microwave signals from Global Navigation Satellite Systems are delayed as they travel through the troposphere, Whereas the hydrostatic delay is predictable, the wet delay, tied to atmospheric moisture, is highly variable. This study introduces a method to analyze small-scale zenith wet delay variations, showing specific daily and seasonal turbulence-influenced patterns in various climate zones. These findings can improve weather forecasting and the accuracy of satellite positioning systems.
Xiao Ma, Yanping Li, Zhenhua Li, and Fei Huo
Atmos. Chem. Phys., 24, 12013–12030, https://doi.org/10.5194/acp-24-12013-2024, https://doi.org/10.5194/acp-24-12013-2024, 2024
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This study uses 4 km Weather Research and Forecasting simulations to investigate the features of low-level jets (LLJs) in North America. It identifies significant LLJ systems, such as the Great Plains LLJ. It also provides insight into LLJs poorly captured in coarser models, such as the northerly Quebec LLJ and the small-scale, low-level wind maxima around the Rocky Mountains. Furthermore, the study examines different physical mechanisms of forming three distinct types of LLJs.
Cuini Qi, Pinya Wang, Yang Yang, Huimin Li, Hui Zhang, Lili Ren, Xipeng Jin, Chenchao Zhan, Jianping Tang, and Hong Liao
Atmos. Chem. Phys., 24, 11775–11789, https://doi.org/10.5194/acp-24-11775-2024, https://doi.org/10.5194/acp-24-11775-2024, 2024
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We investigate extremely hot weather impacts on surface ozone over the southeastern coast of China with and without tropical cyclones. Compared to hot days alone, ozone concentration decreased notably in the Yangtze River Delta (YRD) but increased in the Pearl River Delta (PRD) during tropical cyclones and hot days. The YRD benefited from strong and clean sea winds aiding ozone elimination. In contrast, the PRD experienced strong northeasterly winds that potentially transport ozone pollution.
Shiv Priyam Raghuraman, Brian Soden, Amy Clement, Gabriel Vecchi, Sofia Menemenlis, and Wenchang Yang
Atmos. Chem. Phys., 24, 11275–11283, https://doi.org/10.5194/acp-24-11275-2024, https://doi.org/10.5194/acp-24-11275-2024, 2024
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The rapid global warming of 2023 has led to concerns that it could be externally driven. Here we show that climate models subject only to internal variability predict such warming spikes but rarely (p~1.6 %). However, when a prolonged La Niña immediately precedes an El Niño, as occurred leading up to 2023, such spikes are not uncommon (p~10.3 %). Virtually all of the spikes occur during an El Niño, strongly suggesting that internal variability drove the 2023 warming.
Robert J. Allen, Xueying Zhao, Cynthia A. Randles, Ryan J. Kramer, Bjørn H. Samset, and Christopher J. Smith
Atmos. Chem. Phys., 24, 11207–11226, https://doi.org/10.5194/acp-24-11207-2024, https://doi.org/10.5194/acp-24-11207-2024, 2024
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Present-day methane shortwave absorption mutes 28% (7–55%) of the surface warming associated with its longwave absorption. The precipitation increase associated with the longwave radiative effects of the present-day methane perturbation is also muted by shortwave absorption but not significantly so. Methane shortwave absorption also impacts the magnitude of its climate feedback parameter, largely through the cloud feedback.
Kun Zhang, Tao Luo, Xuebin Li, Shengcheng Cui, Ningquan Weng, Yinbo Huang, and Yingjian Wang
Atmos. Chem. Phys., 24, 11157–11173, https://doi.org/10.5194/acp-24-11157-2024, https://doi.org/10.5194/acp-24-11157-2024, 2024
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In order to deeply understand the formation mechanisms and evolution processes associated with vertical tropopause structures, this study proposes a new method for identifying the multiple characteristic parameters of vertical tropopause structures by fitting temperature profiles using the bi-Gaussian function. The identification results from the bi-Gaussian method are more reasonable and more consistent with the evolution process of atmospheric thermal stratifications.
Felix Pithan, Ann Kristin Naumann, and Marion Maturilli
EGUsphere, https://doi.org/10.5194/egusphere-2024-2961, https://doi.org/10.5194/egusphere-2024-2961, 2024
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Representing the exchange of air masses between the Arctic and mid-latitudes and associated cloud formation is difficult for climate models. We compare climate model output to temperature and humidity measurements from weather balloons to provide suggestions for model improvements. Cold biases mostly occur in air that is exported from the Arctic. Models that compute the number of ice particles in a cloud better represent humidity than models that assume a fixed number of ice particles.
Ying Li, Chenghao Wang, Qiuhong Tang, Shibo Yao, Bo Sun, Hui Peng, and Shangbin Xiao
Atmos. Chem. Phys., 24, 10741–10758, https://doi.org/10.5194/acp-24-10741-2024, https://doi.org/10.5194/acp-24-10741-2024, 2024
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For moisture tracking over the Tibetan Plateau, we recommend using high-resolution forcing datasets, prioritizing temporal resolution over spatial resolution for WAM2layers, while for FLEXPART coupled with WaterSip, we suggest applying bias corrections to optimize the filtering of precipitation particles and adjust evaporation estimates.
Antoine Hermant, Linnea Huusko, and Thorsten Mauritsen
Atmos. Chem. Phys., 24, 10707–10715, https://doi.org/10.5194/acp-24-10707-2024, https://doi.org/10.5194/acp-24-10707-2024, 2024
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Aerosol particles, from natural and human sources, have a cooling effect on the climate, partially offsetting global warming. They do this through direct (sunlight reflection) and indirect (cloud property alteration) mechanisms. Using a global climate model, we found that, despite declining emissions, the direct effect of human aerosols has increased while the indirect effect has decreased, which is attributed to the shift in emissions from North America and Europe to Southeast Asia.
Claire L. Vincent and Andrew J. Dowdy
Atmos. Chem. Phys., 24, 10209–10223, https://doi.org/10.5194/acp-24-10209-2024, https://doi.org/10.5194/acp-24-10209-2024, 2024
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We investigate how wind speed at the height of a wind turbine changes during El Niño and La Niña years and with season and time of day in southeastern Australia. We found that El Niño and La Niña can cause average wind speed differences of around 1 m s-1 in some regions. The highest wind speeds occur in the afternoon or evening around mountains or the coast and during the night for inland areas. The results help show how placement of wind turbines can help balance electricity generation.
Sergio Soler, Francisco J. Gordillo-Vázquez, Francisco J. Pérez-Invernón, Patrick Jöckel, Torsten Neubert, Olivier Chanrion, Victor Reglero, and Nikolai Østgaard
Atmos. Chem. Phys., 24, 10225–10243, https://doi.org/10.5194/acp-24-10225-2024, https://doi.org/10.5194/acp-24-10225-2024, 2024
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Sudden local ozone (O3) enhancements have been reported in different regions of the world since the 1970s. While the hot channel of lightning strokes directly produce significant amounts of nitrogen oxide, no direct emission of O3 is expected. Corona discharges in convective active regions could explain local O3 increases, which remains unexplained. We present the first mathematical functions that relate the global annual frequency of in-cloud coronas with four sets of meteorological variables.
Daniel Köhler, Philipp Reutter, and Peter Spichtinger
Atmos. Chem. Phys., 24, 10055–10072, https://doi.org/10.5194/acp-24-10055-2024, https://doi.org/10.5194/acp-24-10055-2024, 2024
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In this work, the influence of humidity on the properties of the tropopause is studied. The tropopause is the interface between the troposphere and the stratosphere and represents a barrier for the transport of air masses between the troposphere and the stratosphere. We consider not only the tropopause itself, but also a layer around it called the tropopause inversion layer (TIL). It is shown that the moister the underlying atmosphere is, the more this layer acts as a barrier.
Tómas Zoëga, Trude Storelvmo, and Kirstin Krüger
EGUsphere, https://doi.org/10.5194/egusphere-2024-2651, https://doi.org/10.5194/egusphere-2024-2651, 2024
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We use an Earth system model to systematically investigate the climate response to high-latitude, effusive volcanic eruptions as a function of eruption season and size with a special focus on the Arctic. We find that different seasons strongly modulate the climate response with Arctic surface warming in winter and cooling in summer. Also, as eruptions become larger in terms of sulfur dioxide emissions, the climate response becomes increasingly insensitive to variations in the emission strength.
Michael Stanley, Mikael Kuusela, Brendan Byrne, and Junjie Liu
Atmos. Chem. Phys., 24, 9419–9433, https://doi.org/10.5194/acp-24-9419-2024, https://doi.org/10.5194/acp-24-9419-2024, 2024
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To serve the uncertainty quantification (UQ) needs of 4D-Var data assimilation (DA) practitioners, we describe and justify a UQ algorithm from carbon flux inversion and incorporate its sampling uncertainty into the final reported UQ. The algorithm is mathematically proved, and its performance is shown for a carbon flux observing system simulation experiment. These results legitimize and generalize this algorithm's current use and make available this effective algorithm to new DA domains.
Dharmendra Kumar Singh, Swarnali Sanyal, and Donald J. Wuebbles
Atmos. Chem. Phys., 24, 9219–9262, https://doi.org/10.5194/acp-24-9219-2024, https://doi.org/10.5194/acp-24-9219-2024, 2024
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Radiative forcing of contrails could triple by 2050 due to increased air traffic and potential changes in flight altitudes. Factors like air traffic patterns, fuel efficiency, alternative fuels, and climate change further influence this impact. By highlighting gaps in knowledge and uncertainties, this research helps set priorities for future studies and assess strategies to mitigate the environmental impact of aviation emissions.
Dieu Anh Tran, Christoph Gerbig, Christian Rödenbeck, and Sönke Zaehle
Atmos. Chem. Phys., 24, 8413–8440, https://doi.org/10.5194/acp-24-8413-2024, https://doi.org/10.5194/acp-24-8413-2024, 2024
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The analysis of the atmospheric CO2 record from the Zotino Tall Tower Observatory (ZOTTO) in central Siberia shows significant increases in the length and amplitude of the CO2 uptake and release in the 2010–2021 period. The trend shows a stronger increase in carbon release amplitude compared to the uptake, suggesting that, despite enhanced growing season uptake, during this period climate warming did not elevate the annual net CO2 uptake as cold-season respirations also responded to the warming.
Olaf Morgenstern
Atmos. Chem. Phys., 24, 8105–8123, https://doi.org/10.5194/acp-24-8105-2024, https://doi.org/10.5194/acp-24-8105-2024, 2024
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I use errors in climate model simulations to derive correction factors for the impacts of greenhouse gases and particles that bring these simulated temperature fields into agreement with an observational reconstruction of the Earth's temperature. On average across eight models, a reduction by about one-half of the particle-induced cooling would be required, causing only 0.24 K of cooling since 1850–1899. The greenhouse gas warming simulated by several highly sensitive models would also reduce.
Duncan Watson-Parris, Laura J. Wilcox, Camilla W. Stjern, Robert J. Allen, Geeta Persad, Massimo A. Bollasina, Annica M. L. Ekman, Carley E. Iles, Manoj Joshi, Marianne T. Lund, Daniel McCoy, Daniel Westervelt, Andrew Williams, and Bjørn H. Samset
EGUsphere, https://doi.org/10.5194/egusphere-2024-1946, https://doi.org/10.5194/egusphere-2024-1946, 2024
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In 2020, regulations by the International Maritime Organization aimed to reduce aerosol emissions from ships. These aerosols previously had a cooling effect, which the regulations might reduce, revealing more greenhouse gas warming. Here we find that while there is regional warming, the global 2020–2040 temperature rise is only +0.03°C. This small change is difficult to distinguish from natural climate variability, indicating the regulations have had a limited effect on observed warming to date.
Donghuan Li, Tianjun Zhou, Youcun Qi, Liwei Zou, Chao Li, Wenxia Zhang, and Xiaolong Chen
Atmos. Chem. Phys., 24, 7347–7358, https://doi.org/10.5194/acp-24-7347-2024, https://doi.org/10.5194/acp-24-7347-2024, 2024
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Two sets of climate model simulations are used to investigate the dynamic and thermodynamic factors of future change in cold extremes in East Asia. Dynamic factor accounted for over 80 % of cold-month temperature anomalies in past 50 years. The intensity of cold extreme is expected to decrease by 5 ℃, with thermodynamic factor contributing ~ 75 % by the end of the 21st century. Changes in dynamic factor are driven by an upward trend of positive Arctic Oscillation-like sea level pressure pattern.
Johannes Mülmenstädt, Edward Gryspeerdt, Sudhakar Dipu, Johannes Quaas, Andrew S. Ackerman, Ann M. Fridlind, Florian Tornow, Susanne E. Bauer, Andrew Gettelman, Yi Ming, Youtong Zheng, Po-Lun Ma, Hailong Wang, Kai Zhang, Matthew W. Christensen, Adam C. Varble, L. Ruby Leung, Xiaohong Liu, David Neubauer, Daniel G. Partridge, Philip Stier, and Toshihiko Takemura
Atmos. Chem. Phys., 24, 7331–7345, https://doi.org/10.5194/acp-24-7331-2024, https://doi.org/10.5194/acp-24-7331-2024, 2024
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Human activities release copious amounts of small particles called aerosols into the atmosphere. These particles change how much sunlight clouds reflect to space, an important human perturbation of the climate, whose magnitude is highly uncertain. We found that the latest climate models show a negative correlation but a positive causal relationship between aerosols and cloud water. This means we need to be very careful when we interpret observational studies that can only see correlation.
Flora Maria Brocza, Peter Rafaj, Robert Sander, Fabian Wagner, and Jenny Marie Jones
Atmos. Chem. Phys., 24, 7385–7404, https://doi.org/10.5194/acp-24-7385-2024, https://doi.org/10.5194/acp-24-7385-2024, 2024
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To understand how atmospheric mercury levels will change in the future, we model how anthropogenic Hg releases will change following developments in human energy use and mercury use and efforts to reduce pollution and battle climate change. Overall, the findings emphasize that it will be necessary to implement targeted Hg control measures in addition to stringent climate and clean air policies to achieve significant reductions in Hg emissions.
Zhen Liu, Massimo A. Bollasina, and Laura J. Wilcox
Atmos. Chem. Phys., 24, 7227–7252, https://doi.org/10.5194/acp-24-7227-2024, https://doi.org/10.5194/acp-24-7227-2024, 2024
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The aerosol impact on monsoon precipitation and circulation is strongly influenced by a model-simulated spatio-temporal variability in the climatological monsoon precipitation across Asia, which critically modulates the efficacy of aerosol–cloud–precipitation interactions, the predominant driver of the total aerosol response. There is a strong interplay between South Asia and East Asia monsoon precipitation biases and their relative predominance in driving the overall monsoon response.
Tapio Schneider, L. Ruby Leung, and Robert C. J. Wills
Atmos. Chem. Phys., 24, 7041–7062, https://doi.org/10.5194/acp-24-7041-2024, https://doi.org/10.5194/acp-24-7041-2024, 2024
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Climate models are crucial for predicting climate change in detail. This paper proposes a balanced approach to improving their accuracy by combining traditional process-based methods with modern artificial intelligence (AI) techniques while maximizing the resolution to allow for ensemble simulations. The authors propose using AI to learn from both observational and simulated data while incorporating existing physical knowledge to reduce data demands and improve climate prediction reliability.
Brian Nathan, Joannes D. Maasakkers, Stijn Naus, Ritesh Gautam, Mark Omara, Daniel J. Varon, Melissa P. Sulprizio, Lucas A. Estrada, Alba Lorente, Tobias Borsdorff, Robert J. Parker, and Ilse Aben
Atmos. Chem. Phys., 24, 6845–6863, https://doi.org/10.5194/acp-24-6845-2024, https://doi.org/10.5194/acp-24-6845-2024, 2024
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Venezuela's Lake Maracaibo region is notoriously hard to observe from space and features intensive oil exploitation, although production has strongly decreased in recent years. We estimate methane emissions using 2018–2020 TROPOMI satellite observations with national and regional transport models. Despite the production decrease, we find relatively constant emissions from Lake Maracaibo between 2018 and 2020, indicating that there could be large emissions from abandoned infrastructure.
Jiachen Cao, Xu Yue, and Mingrui Ma
Atmos. Chem. Phys., 24, 3973–3987, https://doi.org/10.5194/acp-24-3973-2024, https://doi.org/10.5194/acp-24-3973-2024, 2024
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We implemented two widely used ozone damage schemes into a same regional model. Although the two schemes yielded distinct ozone vegetation damages, they predicted similar feedbacks to surface air temperature and ozone air quality in China. Our results highlighted the significance of ozone pollution control given its detrimental impacts on ecosystem functions, contributions to global warming, and amplifications of ozone pollution through ozone–vegetation coupling.
Steven C. Sherwood and Chris E. Forest
Atmos. Chem. Phys., 24, 2679–2686, https://doi.org/10.5194/acp-24-2679-2024, https://doi.org/10.5194/acp-24-2679-2024, 2024
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The most fundamental parameter used to gauge the severity of future climate change is the so-called equilibrium climate sensitivity, which measures the warming that would ultimately occur due to a doubling of atmospheric carbon dioxide levels. Due to recent advances it is now thought to probably lie in the range 2.5–4 °C. We discuss this and the issues involved in evaluating and using the number, pointing to some pitfalls in current efforts but also possibilities for further progress.
Han Zhang, Baogang Zhang, Bo Jiang, Qimin Li, Xuewen Hu, and Yi Xing
EGUsphere, https://doi.org/10.5194/egusphere-2024-10, https://doi.org/10.5194/egusphere-2024-10, 2024
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We developed the vanadium emission inventories of anthropogenic sources in China during 2015–2019. We identified five major emission sources, including coal combustion, oil burning, transportation, industrial manufacture, and waste handling. Emission outputs were calculated by integrating the emission factors and activity levels of vanadium related processes. Our results identified the key emitters and highlighted the spatial and temporal patterns of vanadium releases.
Christopher D. Wells, Matthew Kasoar, Majid Ezzati, and Apostolos Voulgarakis
Atmos. Chem. Phys., 24, 1025–1039, https://doi.org/10.5194/acp-24-1025-2024, https://doi.org/10.5194/acp-24-1025-2024, 2024
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Human-driven emissions of air pollutants, mostly caused by burning fossil fuels, impact both the climate and human health. Millions of deaths each year are caused by air pollution globally, and the future trends are uncertain. Here, we use a global climate model to study the effect of African pollutant emissions on surface level air pollution, and resultant impacts on human health, in several future emission scenarios. We find much lower health impacts under cleaner, lower-emission futures.
Xipeng Jin, Xuhui Cai, Xuesong Wang, Qianqian Huang, Yu Song, Ling Kang, Hongsheng Zhang, and Tong Zhu
Atmos. Chem. Phys., 24, 259–274, https://doi.org/10.5194/acp-24-259-2024, https://doi.org/10.5194/acp-24-259-2024, 2024
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This work presents a climatology of water vapour exchange flux between the atmospheric boundary layer (ABL) and free troposphere (FT) over eastern China. The water vapour exchange maintains ABL humidity in cold months and moistens the FT in warm seasons, and its distribution has terrain-dependent features. The exchange flux is correlated with the El Niño–Southern Oscillation (ENSO) index and precipitation pattern. The study provides new insight into moisture transport and extreme weather.
Clare Marie Flynn, Linnea Huusko, Angshuman Modak, and Thorsten Mauritsen
Atmos. Chem. Phys., 23, 15121–15133, https://doi.org/10.5194/acp-23-15121-2023, https://doi.org/10.5194/acp-23-15121-2023, 2023
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The latest-generation climate models show surprisingly cold mid-20th century global-mean temperatures, often despite exhibiting more realistic late 20th/early 21st century temperatures. A too-strong aerosol forcing in many models was thought to the be primary cause of these too-cold mid-century temperatures, but this was found to only be a partial explanation. This also partly undermines the hope to construct a strong relationship between the mid-century temperatures and aerosol forcing.
Suvarna Fadnavis, Bernd Heinold, T. P. Sabin, Anne Kubin, Katty Huang, Alexandru Rap, and Rolf Müller
Atmos. Chem. Phys., 23, 10439–10449, https://doi.org/10.5194/acp-23-10439-2023, https://doi.org/10.5194/acp-23-10439-2023, 2023
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The influence of the COVID-19 lockdown on the Himalayas caused increases in snow cover and a decrease in runoff, ultimately leading to an enhanced snow water equivalent. Our findings highlight that, out of the two processes causing a retreat of Himalayan glaciers – (1) slow response to global climate change and (2) fast response to local air pollution – a policy action on the latter is more likely to be within the reach of possible policy action to help billions of people in southern Asia.
Amelie U. Schmitt, Felix Ament, Alessandro C. de Araújo, Marta Sá, and Paulo Teixeira
Atmos. Chem. Phys., 23, 9323–9346, https://doi.org/10.5194/acp-23-9323-2023, https://doi.org/10.5194/acp-23-9323-2023, 2023
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Tall vegetation in forests affects the exchange of heat and moisture between the atmosphere and the land surface. We compared measurements from the Amazon Tall Tower Observatory to results from a land surface model to identify model shortcomings. Our results suggest that soil temperatures in the model could be improved by incorporating a separate canopy layer which represents the heat storage within the forest.
Cited articles
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Allen, M. R., Peters, G. P., Shine, K. P., Azar, C., Balcombe, P., Boucher, O., Cain, M., Ciais, P., Collins, W., Forster, P. M., Frame, D. J., Friedlingstein, P., Fyson, C., Gasser, T., Hare, B., Jenkins, S., Hamburg, S. P., Johansson, D. J. A., Lynch, J., Macey, A., Morfeldt, J., Nauels, A., Ocko, I., Oppenheimer, M., Pacala, S. W., Pierrehumbert, R., Rogelj, J., Schaeffer, M., Schleussner, C. F., Shindell, D., Skeie, R. B., Smith, S. M., and Tanaka, K.: Indicate separate contributions of long-lived and short-lived greenhouse gases in emission targets, npj Clim. Atmos. Sci., 5, 1–4, https://doi.org/10.1038/s41612-021-00226-2, 2022.
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Bickel, M., Ponater, M., Bock, L., Burkhardt, U., and Reineke, S.: Estimating the effective radiative forcing of contrail cirrus, J. Climate, 33, 1991–2005, https://doi.org/10.1175/JCLI-D-19-0467.1, 2020.
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Deuber, O., Matthes, S., Sausen, R., Ponater, M., and Ling, L.: A physical metric-based framework for evaluating the climate trade-off between CO2 and contrails – the case of lowering aircraft flight trajectories, Environ. Sci. Policy, 25, 176–185, https://doi.org/10.1016/j.envsci.2012.10.004, 2013.
Dhakal, S., Minx, J. C., Toth, F. L., Abdel-Aziz, A., Figueroa Meza, M. J., Hubacek, K., Jonckheere, I. G. C., Kim, Y.-G., Nemet, G. F., Pachauri, S., Tan, X. C., and Wiedmann, T.: 2022: Emissions Trends and Drivers, in: IPCC, 2022: Climate Change 2022: Mitigation of Climate Change. Contribution of Working Group III to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Shukla, P. R., Skea, J., Slade, R., Al Khourdajie, A., van Diemen, R., McCollum, D., Pathak, M., Some, S., Vyas, P., Fradera, R., Belkacemi, M., Hasija, A., Lisboa, G., Luz, S., and Malley, J., Cambridge University Press, Cambridge, UK and New York, NY, USA, https://doi.org/10.1017/9781009157926.004, 2022.
Dietmüller, S., Jöckel, P., Tost, H., Kunze, M., Gellhorn, C., Brinkop, S., Frömming, C., Ponater, M., Steil, B., Lauer, A., and Hendricks, J.: A new radiation infrastructure for the Modular Earth Submodel System (MESSy, based on version 2.51), Geosci. Model Dev., 9, 2209–2222, https://doi.org/10.5194/gmd-9-2209-2016, 2016.
EASA: Updated analysis of the non-CO2 climate impacts of aviation and potential policy measures pursuant to the EU Emissions Trading System Directive Article 30(4), European Union Aviation Safety Agency, https://www.easa.europa.eu/en/document-library/research-reports/report-commission-european-parliament-and-council (last access: 17 October 2023), 192 pp, 2020.
Emmerling, J., Drouet, L., van der Wijst, K.-I., van Vuuren, D., Bosetti, V., and Tavoni, M.: The role of the discount rate for emission pathways and negative emissions, Environ. Res. Lett., 14, 104008, https://doi.org/10.1088/1748-9326/ab3cc9, 2019.
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Forster, P., Storelvmo, T., Armour, K., Collins, W., Dufresne, J.-L., Frame, D., Lunt, D. J., Mauritsen, T., Palmer, M. D., Watanabe, M., Wild, M., and Zhang, H.: The Earth's Energy Budget, Climate Feedbacks, and Climate Sensitivity, in: Climate Change 2021: The Physical Science Basis. Contribution of Working Group I to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Masson-Delmotte, V., Zhai, P., Pirani, A., Connors, S. L., Péan, C., Berger, S., Caud, N., Chen, Y., Goldfarb, L., Gomis, M. I., Huang, M., Leitzell, K., Lonnoy, E., Matthews, J. B. R., Maycock, T. K., Waterfield, T., Yelekçi, O., Yu, R., and Zhou, B., Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, https://doi.org/10.1017/9781009157896.009, pp. 923–1054, 2021.
Fuglestvedt, J. S., Berntsen, T. K., Godal, O., Sausen, R., Shine, K. P., and Skodvin, T.: Metrics of Climate Change: Assessing Radiative Forcing and Emission Indices, Climatic Change, 58, 267–33, https://doi.org/10.1023/A:1023905326842, 2003.
Fuglestvedt, J. S., Shine, K. P., Berntsen, T., Cook, J., Lee, D. S., Stenke, A., Skeie, R. B., Velders, G. J. M. M., and Waitz, I. A.: Transport impacts on atmosphere and climate: metrics, Atmos. Environ., 44, 4648–4677, https://doi.org/10.1016/j.atmosenv.2009.04.044, 2010.
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Gasser, T., Peters, G. P., Fuglestvedt, J. S., Collins, W. J., Shindell, D. T., and Ciais, P.: Accounting for the climate–carbon feedback in emission metrics, Earth Syst. Dynam., 8, 235–253, https://doi.org/10.5194/esd-8-235-2017, 2017b.
Gasser, T., Crepin, L., Quilcaille, Y., Houghton, R. A., Ciais, P., and Obersteiner, M.: Historical CO2 emissions from land use and land cover change and their uncertainty, Biogeosciences, 17, 4075–4101, https://doi.org/10.5194/bg-17-4075-2020, 2020.
Gierens, K., Schumann, U., Helten, M., Smit, H., and Marenco, A.: A distribution law for relative humidity in the upper troposphere and lower stratosphere derived from three years of MOZAIC measurements, Ann. Geophys., 17, 1218–1226, https://doi.org/10.1007/s00585-999-1218-7, 1999.
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Short summary
This work studies how to compare the climate impact of the CO2 emitted and contrails formed by a flight. This is applied to contrail avoidance strategies that would decrease climate impact of flights by changing the trajectory of aircraft to avoid persistent contrail formation, at the risk of increasing CO2 emissions. We find that different comparison methods lead to different quantification of the total climate impact of a flight but lead to similar decisions of whether to reroute an aircraft.
This work studies how to compare the climate impact of the CO2 emitted and contrails formed by a...
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