Articles | Volume 22, issue 4
https://doi.org/10.5194/acp-22-2507-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-2507-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
24 Feb 2022
Research article |
| 24 Feb 2022
| 24 Feb 2022
Interaction between aerosol and thermodynamic stability within the planetary boundary layer during wintertime over the North China Plain: aircraft observation and WRF-Chem simulation
Advanced Science and Technology of Atmospheric Physics Group (ASAG), School of Atmospheric Sciences, Sun Yat-sen University and Southern Marine Science and Engineering Guangdong Laboratory, Zhuhai 519082, China
Li Dong
School of Electronic and Optical Engineering, Nanjing University of
Science and Technology, Nanjing 210094, China
Yichen Chen
CORRESPONDING AUTHOR
Beijing Weather Modification Center, Beijing 100089, China
Beijing Key Laboratory of Cloud, Precipitation and Atmospheric Water Resources (LCPW), Beijing Meteorological Bureau, Beijing 100089, China
Yuefeng Zhao
CORRESPONDING AUTHOR
School of Physics and Electronics, Shandong Normal University, Jinan 250014, China
Delong Zhao
Beijing Weather Modification Center, Beijing 100089, China
Beijing Key Laboratory of Cloud, Precipitation and Atmospheric Water Resources (LCPW), Beijing Meteorological Bureau, Beijing 100089, China
Mengyu Huang
Beijing Weather Modification Center, Beijing 100089, China
Beijing Key Laboratory of Cloud, Precipitation and Atmospheric Water Resources (LCPW), Beijing Meteorological Bureau, Beijing 100089, China
Deping Ding
Beijing Weather Modification Center, Beijing 100089, China
Beijing Key Laboratory of Cloud, Precipitation and Atmospheric Water Resources (LCPW), Beijing Meteorological Bureau, Beijing 100089, China
Jiayuan Liao
Advanced Science and Technology of Atmospheric Physics Group (ASAG), School of Atmospheric Sciences, Sun Yat-sen University and Southern Marine Science and Engineering Guangdong Laboratory, Zhuhai 519082, China
Tian Ma
Advanced Science and Technology of Atmospheric Physics Group (ASAG), School of Atmospheric Sciences, Sun Yat-sen University and Southern Marine Science and Engineering Guangdong Laboratory, Zhuhai 519082, China
Maohai Hu
CORRESPONDING AUTHOR
School of Electronic and Optical Engineering, Nanjing University of
Science and Technology, Nanjing 210094, China
Yong Han
CORRESPONDING AUTHOR
Advanced Science and Technology of Atmospheric Physics Group (ASAG), School of Atmospheric Sciences, Sun Yat-sen University and Southern Marine Science and Engineering Guangdong Laboratory, Zhuhai 519082, China
Key Laboratory of Tropical Atmosphere-Ocean System, Sun Yat-sen
University, Ministry of Education, Zhuhai 519082, China
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The current study explores the temporal variation of size-selected particle hygroscopicity in Delhi for the first time. Here, we report that the high volume fraction contribution of ammonium chloride to aerosol governs the high aerosol hygroscopicity and associated liquid water content based on the experimental data. The episodically high ammonium chloride present in Delhi's atmosphere could lead to haze and fog formation under high relative humidity in the region.
Yueyue Cheng, Chao Liu, Jiandong Wang, Jiaping Wang, Zhouyang Zhang, Li Chen, Dafeng Ge, Caijun Zhu, Jinbo Wang, and Aijun Ding
Atmos. Chem. Phys., 24, 3065–3078, https://doi.org/10.5194/acp-24-3065-2024, https://doi.org/10.5194/acp-24-3065-2024, 2024
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Brown carbon (BrC), a light-absorbing aerosol, plays a pivotal role in influencing global climate. However, assessing BrC radiative effects remains challenging because the required observational data are hardly accessible. Here we develop a new BrC radiative effect estimation method combining conventional observations and numerical models. Our findings reveal that BrC absorbs up to a third of the sunlight at 370 nm that black carbon does, highlighting its importance in aerosol radiative effects.
Larissa Lacher, Michael P. Adams, Kevin Barry, Barbara Bertozzi, Heinz Bingemer, Cristian Boffo, Yannick Bras, Nicole Büttner, Dimitri Castarede, Daniel J. Cziczo, Paul J. DeMott, Romy Fösig, Megan Goodell, Kristina Höhler, Thomas C. J. Hill, Conrad Jentzsch, Luis A. Ladino, Ezra J. T. Levin, Stephan Mertes, Ottmar Möhler, Kathryn A. Moore, Benjamin J. Murray, Jens Nadolny, Tatjana Pfeuffer, David Picard, Carolina Ramírez-Romero, Mickael Ribeiro, Sarah Richter, Jann Schrod, Karine Sellegri, Frank Stratmann, Benjamin E. Swanson, Erik S. Thomson, Heike Wex, Martin J. Wolf, and Evelyn Freney
Atmos. Chem. Phys., 24, 2651–2678, https://doi.org/10.5194/acp-24-2651-2024, https://doi.org/10.5194/acp-24-2651-2024, 2024
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Aerosol particles that trigger ice formation in clouds are important for the climate system but are very rare in the atmosphere, challenging measurement techniques. Here we compare three cloud chambers and seven methods for collecting aerosol particles on filters for offline analysis at a mountaintop station. A general good agreement of the methods was found when sampling aerosol particles behind a whole air inlet, supporting their use for obtaining data that can be implemented in models.
Andrea Cuesta-Mosquera, Kristina Glojek, Griša Močnik, Luka Drinovec, Asta Gregorič, Martin Rigler, Matej Ogrin, Baseerat Romshoo, Kay Weinhold, Maik Merkel, Dominik van Pinxteren, Hartmut Herrmann, Alfred Wiedensohler, Mira Pöhlker, and Thomas Müller
Atmos. Chem. Phys., 24, 2583–2605, https://doi.org/10.5194/acp-24-2583-2024, https://doi.org/10.5194/acp-24-2583-2024, 2024
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This study evaluated the air pollution and climate impacts of residential-wood-burning particle emissions from a rural European site. The authors investigate the optical and physical properties that connect the aerosol emissions with climate by evaluating atmospheric radiative impacts via simple-forcing calculations. The study contributes to reducing the lack of information on the understanding of the optical properties of air pollution from anthropogenic sources.
Xiangxinyue Meng, Zhijun Wu, Jingchuan Chen, Yanting Qiu, Taomou Zong, Mijung Song, Jiyi Lee, and Min Hu
Atmos. Chem. Phys., 24, 2399–2414, https://doi.org/10.5194/acp-24-2399-2024, https://doi.org/10.5194/acp-24-2399-2024, 2024
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Our study revealed that particles predominantly exist in a semi-solid or solid state during clean winter days with RH below 30 %. However, a non-liquid to a liquid phase transition occurred when the aerosol liquid water (ALW) mass fraction surpassed 15 % (dry mass) at transition RH thresholds ranging from 40 % to 60 %. We also provide insights into the increasingly important roles of particle phase state variation and ALW in secondary particulate growth during haze formation in Beijing, China.
Yiming Wang, Haolin Wang, Yujie Qin, Xinqi Xu, Guowen He, Nanxi Liu, Shengjie Miao, Xiao Lu, Haichao Wang, and Shaojia Fan
Atmos. Chem. Phys., 24, 2267–2285, https://doi.org/10.5194/acp-24-2267-2024, https://doi.org/10.5194/acp-24-2267-2024, 2024
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We conducted a vertical measurement of winter PM2.5 using a mobile multi-lidar system in four cities. Combined with the surface PM2.5 data, the ERA5 reanalysis data, and GEOS-Chem simulations during Dec 2018–Feb 2019, we found that transport nocturnal PM2.5 enhancement by subsidence (T-NPES) events widely occurred with high frequencies in plains regions in eastern China but happened less often in basin regions like Xi’an and Chengdu. We propose a conceptual model of the T-NPES events.
Dominic Heslin-Rees, Peter Tunved, Johan Ström, Roxana Cremer, Paul Zieger, Ilona Riipinen, Annica M. L. Ekman, Konstantinos Eleftheriadis, and Radovan Krejci
Atmos. Chem. Phys., 24, 2059–2075, https://doi.org/10.5194/acp-24-2059-2024, https://doi.org/10.5194/acp-24-2059-2024, 2024
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Light-absorbing atmospheric particles (e.g. black carbon – BC) exert a warming effect on the Arctic climate. We show that the amount of particle light absorption decreased from 2002 to 2023. We conclude that in addition to reductions in emissions of BC, wet removal plays a role in the long-term reduction of BC in the Arctic, given the increase in surface precipitation experienced by air masses arriving at the site. The potential impact of biomass burning events is shown to have increased.
Julika Zinke, Ernst Douglas Nilsson, Piotr Markuszewski, Paul Zieger, Eva Monica Mårtensson, Anna Rutgersson, Erik Nilsson, and Matthew Edward Salter
Atmos. Chem. Phys., 24, 1895–1918, https://doi.org/10.5194/acp-24-1895-2024, https://doi.org/10.5194/acp-24-1895-2024, 2024
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We conducted two research campaigns in the Baltic Sea, during which we combined laboratory sea spray simulation experiments with flux measurements on a nearby island. To combine these two methods, we scaled the laboratory measurements to the flux measurements using three different approaches. As a result, we derived a parameterization that is dependent on wind speed and wave state for particles with diameters 0.015–10 μm. This parameterization is applicable to low-salinity waters.
Sarah Tinorua, Cyrielle Denjean, Pierre Nabat, Thierry Bourrianne, Véronique Pont, François Gheusi, and Emmanuel Leclerc
Atmos. Chem. Phys., 24, 1801–1824, https://doi.org/10.5194/acp-24-1801-2024, https://doi.org/10.5194/acp-24-1801-2024, 2024
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At a French high-altitude site, where many complex interactions between black carbon (BC), radiation, clouds and snow impact climate, 2 years of refractive BC (rBC) and aerosol optical and microphysical measurements have been made. We observed strong seasonal rBC properties variations, with an enhanced absorption in summer compared to winter. The combination of rBC emission sources, transport pathways, atmospheric dynamics and chemical processes explains the rBC light absorption seasonality.
Wenwen Ma, Rong Sun, Xiaoping Wang, Zheng Zong, Shizhen Zhao, Zeyu Sun, Chongguo Tian, Jianhui Tang, Song Cui, Jun Li, and Gan Zhang
Atmos. Chem. Phys., 24, 1509–1523, https://doi.org/10.5194/acp-24-1509-2024, https://doi.org/10.5194/acp-24-1509-2024, 2024
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This is the first report of long-term atmospheric PAH monitoring around the Bohai Sea. The results showed that the concentrations of PAHs in the atmosphere around the Bohai Sea decreased from June 2014 to May 2019, especially the concentrations of highly toxic PAHs. This indicates that the contributions from PAH sources changed to a certain extent in different areas, and it also led to reductions in the related health risk and medical costs following pollution prevention and control.
Marco A. Franco, Rafael Valiati, Bruna A. Holanda, Bruno B. Meller, Leslie A. Kremper, Luciana V. Rizzo, Samara Carbone, Fernando G. Morais, Janaína P. Nascimento, Meinrat O. Andreae, Micael A. Cecchini, Luiz A. T. Machado, Milena Ponczek, Ulrich Pöschl, David Walter, Christopher Pöhlker, and Paulo Artaxo
EGUsphere, https://doi.org/10.5194/egusphere-2023-2607, https://doi.org/10.5194/egusphere-2023-2607, 2024
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The Amazon wet season atmosphere was studied at the Amazon Tall Tower Observatory site, revealing vertical variations (between 60 and 325 m height) in natural aerosols. Daytime mixing contrasted with nighttime stratification, with distinct rain-induced changes in aerosol populations. Notably, optical properties recovery at higher levels was faster, while near-canopy aerosols showed higher scattering efficiency. These findings enhance our understanding of aerosol impacts on climate dynamics.
Julius Seidler, Markus N. Friedrich, Christoph K. Thomas, and Anke C. Nölscher
Atmos. Chem. Phys., 24, 137–153, https://doi.org/10.5194/acp-24-137-2024, https://doi.org/10.5194/acp-24-137-2024, 2024
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Here, we study the transport of ultrafine particles (UFPs) from an airport to two new adjacent measuring sites for 1 year. The number of UFPs in the air and the diurnal variation are typical urban. Winds from the airport show increased number concentrations. Additionally, considering wind frequencies, we estimate that, from all UFPs measured at the two sites, 10 %–14 % originate from the airport and/or other UFP sources from between the airport and site.
Andreas Aktypis, Christos Kaltsonoudis, David Patoulias, Panayiotis Kalkavouras, Angeliki Matrali, Christina N. Vasilakopoulou, Evangelia Kostenidou, Kalliopi Florou, Nikos Kalivitis, Aikaterini Bougiatioti, Konstantinos Eleftheriadis, Stergios Vratolis, Maria I. Gini, Athanasios Kouras, Constantini Samara, Mihalis Lazaridis, Sofia-Eirini Chatoutsidou, Nikolaos Mihalopoulos, and Spyros N. Pandis
Atmos. Chem. Phys., 24, 65–84, https://doi.org/10.5194/acp-24-65-2024, https://doi.org/10.5194/acp-24-65-2024, 2024
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Extensive continuous particle number size distribution measurements took place during two summers (2020 and 2021) at 11 sites in Greece for the investigation of the frequency and the spatial extent of new particle formation. The frequency during summer varied from close to zero in southwestern Greece to more than 60 % in the northern, central, and eastern regions. The spatial variability can be explained by the proximity of the sites to coal-fired power plants and agricultural areas.
Juan Andrés Casquero-Vera, Daniel Pérez-Ramírez, Hassan Lyamani, Fernando Rejano, Andrea Casans, Gloria Titos, Francisco José Olmo, Lubna Dada, Simo Hakala, Tareq Hussein, Katrianne Lehtipalo, Pauli Paasonen, Antti Hyvärinen, Noemí Pérez, Xavier Querol, Sergio Rodríguez, Nikos Kalivitis, Yenny González, Mansour A. Alghamdi, Veli-Matti Kerminen, Andrés Alastuey, Tuukka Petäjä, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 23, 15795–15814, https://doi.org/10.5194/acp-23-15795-2023, https://doi.org/10.5194/acp-23-15795-2023, 2023
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Here we present the first study of the effect of mineral dust on the inhibition/promotion of new particle formation (NPF) events in different dust-influenced areas. Unexpectedly, we show that the occurrence of NPF events is highly frequent during mineral dust outbreaks, occurring even during extreme dust outbreaks. We also show that the occurrence of NPF events during mineral dust outbreaks significantly affects the potential cloud condensation nuclei budget.
Kevin R. Barry, Thomas C. J. Hill, Marina Nieto-Caballero, Thomas A. Douglas, Sonia M. Kreidenweis, Paul J. DeMott, and Jessie M. Creamean
Atmos. Chem. Phys., 23, 15783–15793, https://doi.org/10.5194/acp-23-15783-2023, https://doi.org/10.5194/acp-23-15783-2023, 2023
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Ice-nucleating particles (INPs) are important for the climate due to their influence on cloud properties. To understand potential land-based sources of them in the Arctic, we carried out a survey near the northernmost point of Alaska, a landscape connected to the permafrost (thermokarst). Permafrost contained high concentrations of INPs, with the largest values near the coast. The thermokarst lakes were found to emit INPs, and the water contained elevated concentrations.
Yang Wang, Chanakya Bagya Ramesh, Scott E. Giangrande, Jerome Fast, Xianda Gong, Jiaoshi Zhang, Ahmet Tolga Odabasi, Marcus Vinicius Batista Oliveira, Alyssa Matthews, Fan Mei, John E. Shilling, Jason Tomlinson, Die Wang, and Jian Wang
Atmos. Chem. Phys., 23, 15671–15691, https://doi.org/10.5194/acp-23-15671-2023, https://doi.org/10.5194/acp-23-15671-2023, 2023
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We report the vertical profiles of aerosol properties over the Southern Great Plains (SGP), a region influenced by shallow convective clouds, land–atmosphere interactions, boundary layer turbulence, and the aerosol life cycle. We examined the processes that drive the aerosol population and distribution in the lower troposphere over the SGP. This study helps improve our understanding of aerosol–cloud interactions and the model representation of aerosol processes.
Stefania Gilardoni, Dominic Heslin-Rees, Mauro Mazzola, Vito Vitale, Michael Sprenger, and Radovan Krejci
Atmos. Chem. Phys., 23, 15589–15607, https://doi.org/10.5194/acp-23-15589-2023, https://doi.org/10.5194/acp-23-15589-2023, 2023
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Models still fail in reproducing black carbon (BC) temporal variability in the Arctic. Analysis of equivalent BC concentrations in the European Arctic shows that BC seasonal variability is modulated by the efficiency of removal by precipitation during transport towards high latitudes. Short-term variability is controlled by synoptic-scale circulation patterns. The advection of warm air from lower latitudes is an effective pollution transport pathway during summer.
Markku Kulmala, Anna Lintunen, Hanna Lappalainen, Annele Virtanen, Chao Yan, Ekaterina Ezhova, Tuomo Nieminen, Ilona Riipinen, Risto Makkonen, Johanna Tamminen, Anu-Maija Sundström, Antti Arola, Armin Hansel, Kari Lehtinen, Timo Vesala, Tuukka Petäjä, Jaana Bäck, Tom Kokkonen, and Veli-Matti Kerminen
Atmos. Chem. Phys., 23, 14949–14971, https://doi.org/10.5194/acp-23-14949-2023, https://doi.org/10.5194/acp-23-14949-2023, 2023
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To be able to meet global grand challenges, we need comprehensive open data with proper metadata. In this opinion paper, we describe the SMEAR (Station for Measuring Earth surface – Atmosphere Relations) concept and include several examples (cases), such as new particle formation and growth, feedback loops and the effect of COVID-19, and what has been learned from these investigations. The future needs and the potential of comprehensive observations of the environment are summarized.
Weilun Zhao, Ying Li, Gang Zhao, Song Guo, Nan Ma, Shuya Hu, and Chunsheng Zhao
Atmos. Chem. Phys., 23, 14889–14902, https://doi.org/10.5194/acp-23-14889-2023, https://doi.org/10.5194/acp-23-14889-2023, 2023
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Studies have concentrated on particles containing black carbon (BC) smaller than 700 nm because of technical limitations. In this study, BC-containing particles larger than 700 nm (BC>700) were measured, highlighting their importance to total BC mass and absorption. The contribution of BC>700 to the BC direct radiative effect was estimated, highlighting the necessity to consider the whole size range of BC-containing particles in the model estimation of BC radiative effects.
Alessandro Bigi, Giorgio Veratti, Elisabeth Andrews, Martine Collaud Coen, Lorenzo Guerrieri, Vera Bernardoni, Dario Massabò, Luca Ferrero, Sergio Teggi, and Grazia Ghermandi
Atmos. Chem. Phys., 23, 14841–14869, https://doi.org/10.5194/acp-23-14841-2023, https://doi.org/10.5194/acp-23-14841-2023, 2023
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Atmospheric particles include compounds that play a key role in the greenhouse effect and air toxicity. Concurrent observations of these compounds by multiple instruments are presented, following deployment within an urban environment in the Po Valley, one of Europe's pollution hotspots. The study compares these data, highlighting the impact of ground emissions, mainly vehicular traffic and biomass burning, on the absorption of sun radiation and, ultimately, on climate change and air quality.
Kristina Pistone, Eric M. Wilcox, Paquita Zuidema, Marco Giordano, James Podolske, Samuel E. LeBlanc, Meloë Kacenelenbogen, Steven G. Howell, and Steffen Freitag
EGUsphere, https://doi.org/10.5194/egusphere-2023-2412, https://doi.org/10.5194/egusphere-2023-2412, 2023
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The springtime southeast Atlantic atmosphere contains lots of smoke from continental fires. This smoke also contains water vapor; more smoke means more humidity. We use aircraft observations and models to describe how these values change through the season and over the region. We then sort the atmosphere into different profile types, by vertical structure and amount of smoke and humidity. Since they both absorb solar energy, our work helps to better quantify the heating effects in this region.
Ghislain Motos, Gabriel Freitas, Paraskevi Georgakaki, Jörg Wieder, Guangyu Li, Wenche Aas, Chris Lunder, Radovan Krejci, Julie Thérèse Pasquier, Jan Henneberger, Robert Oscar David, Christoph Ritter, Claudia Mohr, Paul Zieger, and Athanasios Nenes
Atmos. Chem. Phys., 23, 13941–13956, https://doi.org/10.5194/acp-23-13941-2023, https://doi.org/10.5194/acp-23-13941-2023, 2023
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Low-altitude clouds play a key role in regulating the climate of the Arctic, a region that suffers from climate change more than any other on the planet. We gathered meteorological and aerosol physical and chemical data over a year and utilized them for a parameterization that help us unravel the factors driving and limiting the efficiency of cloud droplet formation. We then linked this information to the sources of aerosol found during each season and to processes of cloud glaciation.
Alberto Sanchez-Marroquin, Sarah L. Barr, Ian T. Burke, James B. McQuaid, and Benjamin J. Murray
Atmos. Chem. Phys., 23, 13819–13834, https://doi.org/10.5194/acp-23-13819-2023, https://doi.org/10.5194/acp-23-13819-2023, 2023
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The sources and concentrations of ice-nucleating particles (INPs) in the Arctic are still poorly understood. Here we report aircraft-based INP concentrations and aerosol composition in the western North American Arctic. The concentrations of INPs and all aerosol particles were low. The aerosol samples contained mostly sea salt and dust particles. Dust particles were more relevant for the INP concentrations than sea salt. However, dust alone cannot account for all of the measured INPs.
Katherine L. Ackerman, Alison D. Nugent, and Chung Taing
Atmos. Chem. Phys., 23, 13735–13753, https://doi.org/10.5194/acp-23-13735-2023, https://doi.org/10.5194/acp-23-13735-2023, 2023
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Sea salt aerosol is an important marine aerosol that may be produced in greater quantities in coastal regions than over the open ocean. This study observed these particles along the windward coastline of O'ahu, Hawai'i, to understand how wind and waves influence their production and dispersal. Overall, wave heights were the strongest variable correlated with changes in aerosol concentrations, while wind speeds played an important role in their horizontal dispersal and vertical mixing.
Jiyeon Park, Hyojin Kang, Yeontae Gim, Eunho Jang, Ki-Tae Park, Sangjong Park, Chang Hoon Jung, Darius Ceburnis, Colin O'Dowd, and Young Jun Yoon
Atmos. Chem. Phys., 23, 13625–13646, https://doi.org/10.5194/acp-23-13625-2023, https://doi.org/10.5194/acp-23-13625-2023, 2023
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We measured the number size distribution of 2.5–300 nm particles and cloud condensation nuclei (CCN) number concentrations at King Sejong Station on the Antarctic Peninsula continuously from 1 January to 31 December 2018. During the pristine and clean periods, 97 new particle formation (NPF) events were detected. For 83 of these, CCN concentrations increased by 2 %–268 % (median 44 %) following 1 to 36 h (median 8 h) after NPF events.
Aodong Du, Jiaxing Sun, Hang Liu, Weiqi Xu, Wei Zhou, Yuting Zhang, Lei Li, Xubing Du, Yan Li, Xiaole Pan, Zifa Wang, and Yele Sun
Atmos. Chem. Phys., 23, 13597–13611, https://doi.org/10.5194/acp-23-13597-2023, https://doi.org/10.5194/acp-23-13597-2023, 2023
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We characterized the impacts of emission controls on particle mixing state and density during the Beijing Olympic Winter Games using a SPAMS in tandem with a DMA and an AAC. OC and sulfate-containing particles increased, while those from primary emissions decreased. The effective particle densities increased and varied largely for different particles, highlighting the impacts of aging and formation processes on the changes of particle density and mixing state.
Karine Sellegri, Theresa Barthelmeß, Jonathan Trueblood, Antonia Cristi, Evelyn Freney, Clémence Rose, Neill Barr, Mike Harvey, Karl Safi, Stacy Deppeler, Karen Thompson, Wayne Dillon, Anja Engel, and Cliff Law
Atmos. Chem. Phys., 23, 12949–12964, https://doi.org/10.5194/acp-23-12949-2023, https://doi.org/10.5194/acp-23-12949-2023, 2023
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The amount of sea spray emitted to the atmosphere depends on the ocean temperature, but this dependency is not well understood, especially when ocean biology is involved. In this study, we show that sea spray emissions are increased by up to a factor of 4 at low seawater temperatures compared to moderate temperatures, and we quantify the temperature dependence as a function of the ocean biogeochemistry.
Albert Ansmann, Kevin Ohneiser, Ronny Engelmann, Martin Radenz, Hannes Griesche, Julian Hofer, Dietrich Althausen, Jessie M. Creamean, Matthew C. Boyer, Daniel A. Knopf, Sandro Dahlke, Marion Maturilli, Henriette Gebauer, Johannes Bühl, Cristofer Jimenez, Patric Seifert, and Ulla Wandinger
Atmos. Chem. Phys., 23, 12821–12849, https://doi.org/10.5194/acp-23-12821-2023, https://doi.org/10.5194/acp-23-12821-2023, 2023
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The 1-year MOSAiC (2019–2020) expedition with the German ice breaker Polarstern was the largest polar field campaign ever conducted. The Polarstern, with our lidar aboard, drifted with the pack ice north of 85° N for more than 7 months (October 2019 to mid-May 2020). We measured the full annual cycle of aerosol conditions in terms of aerosol optical and cloud-process-relevant properties. We observed a strong contrast between polluted winter and clean summer aerosol conditions.
Nair Krishnan Kala, Narayana Sarma Anand, Mohanan R. Manoj, Srinivasan Prasanth, Harshavardhana S. Pathak, Thara Prabhakaran, Pramod D. Safai, Krishnaswamy K. Moorthy, and Sreedharan K. Satheesh
Atmos. Chem. Phys., 23, 12801–12819, https://doi.org/10.5194/acp-23-12801-2023, https://doi.org/10.5194/acp-23-12801-2023, 2023
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We present a 3D data set of aerosol black carbon over the Indian mainland by assimilating data from surface, aircraft, and balloon measurements, along with multi-satellite observations. Radiative transfer computations using height-resolved aerosol absorption show higher warming in the free troposphere and will have large implications for atmospheric stability. This data set will help reduce the uncertainty in aerosol radiative effects in climate model simulations over the Indian region.
Sujan Shrestha, Shan Zhou, Manisha Mehra, Meghan Guagenti, Subin Yoon, Sergio L. Alvarez, Fangzhou Guo, Chun-Ying Chao, James H. Flynn III, Yuxuan Wang, Robert J. Griffin, Sascha Usenko, and Rebecca J. Sheesley
Atmos. Chem. Phys., 23, 10845–10867, https://doi.org/10.5194/acp-23-10845-2023, https://doi.org/10.5194/acp-23-10845-2023, 2023
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We evaluated different methods for assessing the influence of long-range transport of biomass burning (BB) plumes at a coastal site in Texas, USA. We show that the aerosol composition and optical properties exhibited good agreement, while CO and acetonitrile trends were less specific for assessing BB source influence. Our results demonstrate that the network of aerosol optical measurements can be useful for identifying the influence of aged BB plumes in anthropogenically influenced areas.
Guangyu Li, Elise K. Wilbourn, Zezhen Cheng, Jörg Wieder, Allison Fagerson, Jan Henneberger, Ghislain Motos, Rita Traversi, Sarah D. Brooks, Mauro Mazzola, Swarup China, Athanasios Nenes, Ulrike Lohmann, Naruki Hiranuma, and Zamin A. Kanji
Atmos. Chem. Phys., 23, 10489–10516, https://doi.org/10.5194/acp-23-10489-2023, https://doi.org/10.5194/acp-23-10489-2023, 2023
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In this work, we present results from an Arctic field campaign (NASCENT) in Ny-Ålesund, Svalbard, on the abundance, variability, physicochemical properties, and potential sources of ice-nucleating particles (INPs) relevant for mixed-phase cloud formation. This work improves the data coverage of Arctic INPs and aerosol properties, allowing for the validation of models predicting cloud microphysical and radiative properties of mixed-phase clouds in the rapidly warming Arctic.
Jun Shi, Jinpei Yan, Shanshan Wang, Shuhui Zhao, Miming Zhang, Suqing Xu, Qi Lin, Hang Yang, and Siying Dai
Atmos. Chem. Phys., 23, 10349–10359, https://doi.org/10.5194/acp-23-10349-2023, https://doi.org/10.5194/acp-23-10349-2023, 2023
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An underway aerosol-monitoring system was used to determine the Na+ concentration during different cyclone periods in the Southern Ocean in order to assess the potential effects of cyclones on sea spray aerosol (SSA) emissions. It was estimated that more than 23 % of SSAs were transported upwards during cyclone periods. Vertically transported SSAs can be regarded as an important source of CCN and hence have an effect on climate in the middle and high latitudes of the Southern Hemisphere.
Jean-Philippe Putaud, Enrico Pisoni, Alexander Mangold, Christoph Hueglin, Jean Sciare, Michael Pikridas, Chrysanthos Savvides, Jakub Ondracek, Saliou Mbengue, Alfred Wiedensohler, Kay Weinhold, Maik Merkel, Laurent Poulain, Dominik van Pinxteren, Hartmut Herrmann, Andreas Massling, Claus Nordstroem, Andrés Alastuey, Cristina Reche, Noemí Pérez, Sonia Castillo, Mar Sorribas, Jose Antonio Adame, Tuukka Petaja, Katrianne Lehtipalo, Jarkko Niemi, Véronique Riffault, Joel F. de Brito, Augustin Colette, Olivier Favez, Jean-Eudes Petit, Valérie Gros, Maria I. Gini, Stergios Vratolis, Konstantinos Eleftheriadis, Evangelia Diapouli, Hugo Denier van der Gon, Karl Espen Yttri, and Wenche Aas
Atmos. Chem. Phys., 23, 10145–10161, https://doi.org/10.5194/acp-23-10145-2023, https://doi.org/10.5194/acp-23-10145-2023, 2023
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Many European people are still exposed to levels of air pollution that can affect their health. COVID-19 lockdowns in 2020 were used to assess the impact of the reduction in human mobility on air pollution across Europe by comparing measurement data with values that would be expected if no lockdown had occurred. We show that lockdown measures did not lead to consistent decreases in the concentrations of fine particulate matter suspended in the air, and we investigate why.
Qian Xiao, Jiaoshi Zhang, Yang Wang, Luke D. Ziemba, Ewan Crosbie, Edward L. Winstead, Claire E. Robinson, Joshua P. DiGangi, Glenn S. Diskin, Jeffrey S. Reid, K. Sebastian Schmidt, Armin Sorooshian, Miguel Ricardo A. Hilario, Sarah Woods, Paul Lawson, Snorre A. Stamnes, and Jian Wang
Atmos. Chem. Phys., 23, 9853–9871, https://doi.org/10.5194/acp-23-9853-2023, https://doi.org/10.5194/acp-23-9853-2023, 2023
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Using recent airborne measurements, we show that the influences of anthropogenic emissions, transport, convective clouds, and meteorology lead to new particle formation (NPF) under a variety of conditions and at different altitudes in tropical marine environments. NPF is enhanced by fresh urban emissions in convective outflow but is suppressed in air masses influenced by aged urban emissions where reactive precursors are mostly consumed while particle surface area remains relatively high.
Simo Hakala, Ville Vakkari, Heikki Lihavainen, Antti-Pekka Hyvärinen, Kimmo Neitola, Jenni Kontkanen, Veli-Matti Kerminen, Markku Kulmala, Tuukka Petäjä, Tareq Hussein, Mamdouh I. Khoder, Mansour A. Alghamdi, and Pauli Paasonen
Atmos. Chem. Phys., 23, 9287–9321, https://doi.org/10.5194/acp-23-9287-2023, https://doi.org/10.5194/acp-23-9287-2023, 2023
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Things are not always as they first seem in ambient aerosol measurements. Observations of decreasing particle sizes are often interpreted as resulting from particle evaporation. We show that such observations can counterintuitively be explained by particles that are constantly growing in size. This requires one to account for the previous movements of the observed air. Our explanation implies a larger number of larger particles, meaning more significant effects of aerosols on climate and health.
Akriti Masoom, Ilias Fountoulakis, Stelios Kazadzis, Ioannis-Panagiotis Raptis, Anna Kampouri, Basil E. Psiloglou, Dimitra Kouklaki, Kyriakoula Papachristopoulou, Eleni Marinou, Stavros Solomos, Anna Gialitaki, Dimitra Founda, Vasileios Salamalikis, Dimitris Kaskaoutis, Natalia Kouremeti, Nikolaos Mihalopoulos, Vassilis Amiridis, Andreas Kazantzidis, Alexandros Papayannis, Christos S. Zerefos, and Kostas Eleftheratos
Atmos. Chem. Phys., 23, 8487–8514, https://doi.org/10.5194/acp-23-8487-2023, https://doi.org/10.5194/acp-23-8487-2023, 2023
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We analyse the spatial and temporal aerosol spectral optical properties during the extreme wildfires of August 2021 in Greece and assess their effects on air quality and solar radiation quantities related to health, agriculture, and energy. Different aerosol conditions are identified (pure smoke, pure dust, dust–smoke together); the largest impact on solar radiation quantities is found for cases with mixed dust–smoke aerosols. Such situations are expected to occur more frequently in the future.
Xiaojing Shen, Junying Sun, Huizheng Che, Yangmei Zhang, Chunhong Zhou, Ke Gui, Wanyun Xu, Quan Liu, Junting Zhong, Can Xia, Xinyao Hu, Sinan Zhang, Jialing Wang, Shuo Liu, Jiayuan Lu, Aoyuan Yu, and Xiaoye Zhang
Atmos. Chem. Phys., 23, 8241–8257, https://doi.org/10.5194/acp-23-8241-2023, https://doi.org/10.5194/acp-23-8241-2023, 2023
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New particle formation (NPF) events occur when the dust episodes' fade is analysed based on long-term measurement of particle number size distribution. Analysis shows that the observed formation and growth rates are approximately 50 % of and 30 % lower than those of other NPF events. As a consequence of the uptake of precursor gases on mineral dust, the physical and chemical properties of submicron particles, as well as the ability to be cloud condensation nuclei, can be changed.
Marco Zanatta, Stephan Mertes, Olivier Jourdan, Regis Dupuy, Emma Järvinen, Martin Schnaiter, Oliver Eppers, Johannes Schneider, Zsófia Jurányi, and Andreas Herber
Atmos. Chem. Phys., 23, 7955–7973, https://doi.org/10.5194/acp-23-7955-2023, https://doi.org/10.5194/acp-23-7955-2023, 2023
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Black carbon (BC) particles influence the Arctic radiative balance. Vertical measurements of black carbon were conducted during the ACLOUD campaign in the European Arctic to study the interaction of BC with clouds. This study shows that clouds influence the vertical variability of BC properties across the inversion layer and that multiple activation and transformation mechanisms of BC may occur in the presence of low-level, persistent, mixed-phase clouds.
Guangdong Niu, Ximeng Qi, Liangduo Chen, Lian Xue, Shiyi Lai, Xin Huang, Jiaping Wang, Xuguang Chi, Wei Nie, Veli-Matti Kerminen, Tuukka Petäjä, Markku Kulmala, and Aijun Ding
Atmos. Chem. Phys., 23, 7521–7534, https://doi.org/10.5194/acp-23-7521-2023, https://doi.org/10.5194/acp-23-7521-2023, 2023
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The reported below-cloud wet-scavenging coefficients (BWSCs) are much higher than theoretical data, but the reason remains unclear. Based on long-term observation, we find that air mass changing during rainfall events causes the overestimation of BWSCs. Thus, the discrepancy in BWSCs between observation and theory is not as large as currently believed. To obtain reasonable BWSCs and parameterizations from field observations, the effect of air mass changes needs to be considered.
Antonio Donateo, Gianluca Pappaccogli, Daniela Famulari, Mauro Mazzola, Federico Scoto, and Stefano Decesari
Atmos. Chem. Phys., 23, 7425–7445, https://doi.org/10.5194/acp-23-7425-2023, https://doi.org/10.5194/acp-23-7425-2023, 2023
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This work aims to measure the turbulent fluxes and the dry deposition velocity for size-segregated particles (from ultrafine to quasi-coarse range) at an Arctic site (Svalbard). Aiming to characterize the effect of surface properties on dry deposition, continuous observations were performed from the coldest months (on snow surface) to the snow melting period and throughout the summer (snow-free surface). A data fit of the deposition velocity as a function of particle diameters will be provided.
Cited articles
An, Z., Huang, R.-J., Zhang, R., Tie, X., Li, G., Cao, J., Zhou, W., Shi,
Z., Han, Y., Gu, Z., and Ji, Y.: Severe haze in northern China: A synergy of
anthropogenic emissions and atmospheric processes, P.
Natl. Acad. Sci. USA, 116, 8657–8666, https://doi.org/10.1073/pnas.1900125116, 2019.
Barnard, J. C., Fast, J. D., Paredes-Miranda, G., Arnott, W. P., and Laskin,
A.: Technical Note: Evaluation of the WRF-Chem “Aerosol Chemical to Aerosol
Optical Properties” Module using data from the MILAGRO campaign, Atmos.
Chem. Phys., 10, 7325–7340, https://doi.org/10.5194/acp-10-7325-2010, 2010.
Chan, C. K. and Yao, X.: Air pollution in mega cities in China, Atmos.
Environ., 42, 1–42, https://doi.org/10.1016/j.atmosenv.2007.09.003, 2008.
Che, H., Gui, K., Xia, X., Wang, Y., Holben, B. N., Goloub, P.,
Cuevas-Agulló, E., Wang, H., Zheng, Y., Zhao, H., and Zhang, X.: Large
contribution of meteorological factors to inter-decadal changes in regional
aerosol optical depth, Atmos. Chem. Phys., 19, 10497–10523,
https://doi.org/10.5194/acp-19-10497-2019, 2019.
Chi, X., Winderlich, J., Mayer, J. C., Panov, A. V., Heimann, M., Birmili,
W., Heintzenberg, J., Cheng, Y., and Andreae, M. O.: Long-term measurements
of aerosol and carbon monoxide at the ZOTTO tall tower to characterize
polluted and pristine air in the Siberian taiga, Atmos. Chem. Phys., 13,
12271–12298, https://doi.org/10.5194/acp-13-12271-2013, 2013.
CNEMC: air pollution data [data set], available at: https://www.http://www.cnemc.cn, last access: 20 November 2020.
Ding, A. J., Fu, C. B., Yang, X. Q., Sun, J. N., Petäjä, T.,
Kerminen, V. M., Wang, T., Xie, Y., Herrmann, E., Zheng, L. F., Nie, W.,
Liu, Q., Wei, X. L., and Kulmala, M.: Intense atmospheric pollution modifies
weather: a case of mixed biomass burning with fossil fuel combustion
pollution in eastern China, Atmos. Chem. Phys., 13, 10545–10554,
https://doi.org/10.5194/acp-13-10545-2013, 2013.
Ding, A. J., Huang, X., Nie, W., Sun, J. N., Kerminen, V.-M.,
Petäjä, T., Su, H., Cheng, Y. F., Yang, X.-Q., Wang, M. H., Chi, X.
G., Wang, J. P., Virkkula, A., Guo, W. D., Yuan, J., Wang, S. Y., Zhang, R.
J., Wu, Y. F., Song, Y., Zhu, T., Zilitinkevich, S., Kulmala, M., and Fu, C.
B.: Enhanced haze pollution by black carbon in megacities in China,
Geophys. Res. Lett., 43, 2873–2879, https://doi.org/10.1002/2016GL067745, 2016.
Du, H., Li, J., Wang, Z., Dao, X., Guo, S., Wang, L., Ma, S., Wu, J., Yang,
W., Chen, X., and Sun, Y.: Effects of Regional Transport on Haze in the
North China Plain: Transport of Precursors or Secondary Inorganic Aerosols,
Geophys. Res. Lett., 47, e2020GL087461, https://doi.org/10.1029/2020GL087461, 2020.
ECWMF: ERA5 data [data set], https://www.ecmwf.int/en/forecasts/datasets/reanalysis-datasets/era5, last access: 20 November 2020.
Ek, M. B., Mitchell, K. E., Lin, Y., Rogers, E., Grunmann, P., Koren, V.,
Gayno, G., and Tarpley, J. D.: Implementation of Noah land surface model
advances in the National Centers for Environmental Prediction operational
mesoscale Eta model, J. Geophys. Res.-Atmos., 108, 8851,
https://doi.org/10.1029/2002JD003296, 2003.
Fan, H., Zhao, C., and Yang, Y.: A comprehensive analysis of the
spatio-temporal variation of urban air pollution in China during 2014–2018,
Atmos. Environ., 220, 117066, https://doi.org/10.1016/j.atmosenv.2019.117066, 2020.
Fast, J. D., Gustafson Jr., W. I., Easter, R. C., Zaveri, R. A., Barnard, J.
C., Chapman, E. G., Grell, G. A., and Peckham, S. E.: Evolution of ozone,
particulates, and aerosol direct radiative forcing in the vicinity of
Houston using a fully coupled meteorology-chemistry-aerosol model, J. Geophys. Res.-Atmos.s, 111, D21305,
https://doi.org/10.1029/2005JD006721, 2006.
Granella, F., Aleluia Reis, L., Bosetti, V., and Tavoni, M.: COVID-19
lockdown only partially alleviates health impacts of air pollution in
Northern Italy, Environ. Res. Lett., 16, 035012,
https://doi.org/10.1088/1748-9326/abd3d2, 2021.
Grell, G. A., Peckham, S. E., Schmitz, R., McKeen, S. A., Frost, G.,
Skamarock, W. C., and Eder, B.: Fully coupled “online” chemistry within
the WRF model, Atmos. Environ.t, 39, 6957–6975,
https://doi.org/10.1016/j.atmosenv.2005.04.027, 2005.
Guenther, A., Karl, T., Harley, P., Wiedinmyer, C., Palmer, P. I., and
Geron, C.: Estimates of global terrestrial isoprene emissions using MEGAN
(Model of Emissions of Gases and Aerosols from Nature), Atmos. Chem. Phys.,
6, 3181–3210, https://doi.org/10.5194/acp-6-3181-2006, 2006.
Hu, X.-M., Li, X., Xue, M., Wu, D., and Fuentes, J. D.: The Formation of
Barrier Winds East of the Loess Plateau and Their Effects on Dispersion
Conditions in the North China Plains, Bound.-Lay. Meteorol., 161,
145–163, https://doi.org/10.1007/s10546-016-0159-4, 2016.
Huang, X., Wang, Z., and Ding, A.: Impact of Aerosol-PBL Interaction on Haze
Pollution: Multiyear Observational Evidences in North China, Geophys. Res. Lett., 45, 8596–8603, https://doi.org/10.1029/2018GL079239, 2018.
Hung, W.-T., Lu, C.-H., Alessandrini, S., Kumar, R., and Lin, C.-A.: The
impacts of transported wildfire smoke aerosols on surface air quality in New
York State: A multi-year study using machine learning, Atmos.
Environ., 259, 118513, https://doi.org/10.1016/j.atmosenv.2021.118513, 2021.
Iacono, M. J., Delamere, J. S., Mlawer, E. J., Shephard, M. W., Clough, S.
A., and Collins, W. D.: Radiative forcing by long-lived greenhouse gases:
Calculations with the AER radiative transfer models, J. Geophys.
Res.-Atmos., 113, D13103, https://doi.org/10.1029/2008JD009944, 2008.
Itahashi, S., Hayami, H., and Uno, I.: Comprehensive study of emission
source contributions for tropospheric ozone formation over East Asia,
J. Geophys. Res.-Atmos., 120, 331–358,
https://doi.org/10.1002/2014JD022117, 2015.
Jiménez, P. A., Dudhia, J., González-Rouco, J. F., Montávez, J.
P., García-Bustamante, E., Navarro, J., Vilà-Guerau de Arellano,
J., and Muñoz-Roldán, A.: An evaluation of WRF's ability to
reproduce the surface wind over complex terrain based on typical circulation
patterns, J. Geophys. Res.-Atmos., 118, 7651–7669,
https://doi.org/10.1002/jgrd.50585, 2013.
Letu, H., Nakajima, T. Y., Wang, T., Shang, H., Ma, R., Yang, K., Baran, A.
J., Riedi, J., Ishimoto, H., Yoshida, M., Shi, C., Khatri, P., Du, Y., Chen,
L., and Shi, J.: A new benchmark for surface radiation products over the
East Asia-Pacific region retrieved from the Himawari-8/AHI next-generation
geostationary satellite, Bull. Am. Meteorol. Soc.,
1–40, https://doi.org/10.1175/bams-d-20-0148.1, 2021.
Li, M., Liu, H., Geng, G., Hong, C., Liu, F., Song, Y., Tong, D., Zheng, B.,
Cui, H., Man, H., Zhang, Q., and He, K.: Anthropogenic emission inventories
in China: a review, Natl. Sci. Rev., 4, 834–866, https://doi.org/10.1093/nsr/nwx150,
2017.
Li, M., Wang, T., Xie, M., Li, S., Zhuang, B., Fu, Q., Zhao, M., Wu, H.,
Liu, J., Saikawa, E., and Liao, K.: Drivers for the poor air quality
conditions in North China Plain during the COVID-19 outbreak, Atmos.
Environ., 246, 118103, https://doi.org/10.1016/j.atmosenv.2020.118103, 2021.
Li, Q., Zhang, H., Cai, X., Song, Y., and Zhu, T.: The impacts of the
atmospheric boundary layer on regional haze in North China, npj Clim.
Atmos. Sci., 4, 9, https://doi.org/10.1038/s41612-021-00165-y, 2021.
Li, Z., Guo, J., Ding, A., Liao, H., Liu, J., Sun, Y., Wang, T., Xue, H.,
Zhang, H., and Zhu, B.: Aerosol and boundary-layer interactions and impact
on air quality, Natl. Sci. Rev., 4, 810–833, https://doi.org/10.1093/nsr/nwx117,
2017.
Luo, H., Han, Y., Lu, C., Yang, J., and Wu, Y.: Characteristics of Surface
Solar Radiation under Different Air Pollution Conditions over Nanjing,
China: Observation and Simulation, Adv. Atmos. Sci., 36,
1047–1059, https://doi.org/10.1007/s00376-019-9010-4, 2019.
Luo, H., Han, Y., Cheng, X., Lu, C., and Wu, Y.: Spatiotemporal Variations
in Particulate Matter and Air Quality over China: National, Regional and
Urban Scales, Atmosphere, 12, 43, https://doi.org/10.3390/atmos12010043, 2021.
Ma, Y., Ye, J., Xin, J., Zhang, W., Vilà-Guerau de Arellano, J., Wang,
S., Zhao, D., Dai, L., Ma, Y., Wu, X., Xia, X., Tang, G., Wang, Y., Shen,
P., Lei, Y., and Martin, S. T.: The Stove, Dome, and Umbrella Effects of
Atmospheric Aerosol on the Development of the Planetary Boundary Layer in
Hazy Regions, Geophys. Res. Lett., 47, e2020GL087373,
https://doi.org/10.1029/2020GL087373, 2020.
Menon, S., Hansen, J., Nazarenko, L., and Luo, Y.: Climate Effects of Black
Carbon Aerosols in China and India, Science, 297, 2250–2253,
https://doi.org/10.1126/science.1075159, 2002.
Miao, Y., Liu, S., and Huang, S.: Synoptic pattern and planetary boundary
layer structure associated with aerosol pollution during winter in Beijing,
China, Sci. Total Environ., 682, 464–474,
https://doi.org/10.1016/j.scitotenv.2019.05.199, 2019.
Miao, Y., Che, H., Zhang, X., and Liu, S.: Integrated impacts of synoptic
forcing and aerosol radiative effect on boundary layer and pollution in the
Beijing–Tianjin–Hebei region, China, Atmos. Chem. Phys., 20, 5899–5909,
https://doi.org/10.5194/acp-20-5899-2020, 2020.
Morrison, H., Curry, J. A., and Khvorostyanov, V. I.: A New Double-Moment
Microphysics Parameterization for Application in Cloud and Climate Models,
Part I: Description, J. Atmos. Sci., 62, 1665,
https://doi.org/10.1175/jas3446.1, 2005.
NCAR: NCEP FNL Operational Model Global Tropospheric Analyses, continuing from July 1999, Research Data Archive at the National Center for Atmospheric Research, Computational and Information Systems Laboratory [data set], https://doi.org/10.5065/D6M043C6, 2000.
NCAR: WRF-Chem Version 3.9 [code], https://www2.mmm.ucar.edu/wrf/users/download/get_source.html, last access: 20 November 2020.
Niu, F., Li, Z., Li, C., Lee, K.-H., and Wang, M.: Increase of wintertime
fog in China: Potential impacts of weakening of the Eastern Asian monsoon
circulation and increasing aerosol loading, J. Geophys. Res.-Atmos., 115, D00K20, https://doi.org/10.1029/2009JD013484, 2010.
Noh, Y., Cheon, W. G., Hong, S. Y., and Raasch, S.: Improvement of the
K-profile Model for the Planetary Boundary Layer based on Large Eddy
Simulation Data, Bound.-Lay. Meteorol., 107, 401–427,
https://doi.org/10.1023/a:1022146015946, 2003.
Qu, Y., Han, Y., Wu, Y., Gao, P., and Wang, T.: Study of PBLH and Its
Correlation with Particulate Matter from One-Year Observation over Nanjing,
Southeast China, Remote Sens., 9, 668, https://doi.org/10.3390/rs9070668, 2017.
Ran, L., Deng, Z. Z., Wang, P. C., and Xia, X. A.: Black carbon and
wavelength-dependent aerosol absorption in the North China Plain based on
two-year aethalometer measurements, Atmos. Environ., 142, 132–144,
https://doi.org/10.1016/j.atmosenv.2016.07.014, 2016.
Rosenfeld, D., Sherwood, S., Wood, R., and Donner, L.: Climate Effects of
Aerosol-Cloud Interactions, Science, 343, 379–380, https://doi.org/10.1126/science.1247490,
2014.
Shen, L. and Zhao, C.: Dominance of Shortwave Radiative Heating in the
Sea-Land Breeze Amplitude and its Impacts on Atmospheric Visibility in
Tokyo, Japan, J. Geophys. Res.-Atmos., 125,
e2019JD031541, https://doi.org/10.1029/2019JD031541, 2020.
Su, T., Li, Z., and Kahn, R.: Relationships between the planetary boundary
layer height and surface pollutants derived from lidar observations over
China: regional pattern and influencing factors, Atmos. Chem. Phys., 18,
15921–15935, https://doi.org/10.5194/acp-18-15921-2018, 2018.
Su, T., Li, Z., Li, C., Li, J., Han, W., Shen, C., Tan, W., Wei, J., and
Guo, J.: The significant impact of aerosol vertical structure on lower
atmosphere stability and its critical role in aerosol–planetary boundary
layer (PBL) interactions, Atmos. Chem. Phys., 20, 3713–3724,
https://doi.org/10.5194/acp-20-3713-2020, 2020.
Sun, Y., Jiang, Q., Wang, Z., Fu, P., Li, J., Yang, T., and Yin, Y.:
Investigation of the sources and evolution processes of severe haze
pollution in Beijing in January 2013, J. Geophys. Res.-Atmos., 119, 4380–4398, https://doi.org/10.1002/2014JD021641, 2014.
Twohy, C. H., Petters, M. D., Snider, J. R., Stevens, B., Tahnk, W., Wetzel,
M., Russell, L., and Burnet, F.: Evaluation of the aerosol indirect effect
in marine stratocumulus clouds: Droplet number, size, liquid water path, and
radiative impact, J. Geophys. Res.-Atmos., 110, D08203,
https://doi.org/10.1029/2004JD005116, 2005.
Wang, H., Shi, G. Y., Zhang, X. Y., Gong, S. L., Tan, S. C., Chen, B., Che,
H. Z., and Li, T.: Mesoscale modelling study of the interactions between
aerosols and PBL meteorology during a haze episode in China Jing–Jin–Ji
and its near surrounding region – Part 2: Aerosols' radiative feedback
effects, Atmos. Chem. Phys., 15, 3277–3287, https://doi.org/10.5194/acp-15-3277-2015, 2015.
Wang, Z., Huang, X., Ding, K., Ren, C., Cao, L., Zhou, D., Gao, J., and
Ding, A.: Weakened Aerosol-PBL Interaction During COVID-19 Lockdown in
Northern China, Geophys. Res. Lett., 48, e2020GL090542,
https://doi.org/10.1029/2020GL090542, 2021.
Wu, B. and Wang, J.: Winter Arctic Oscillation, Siberian High and East
Asian Winter Monsoon, Geophys. Res. Lett., 29, 3-1–3-4,
https://doi.org/10.1029/2002GL015373, 2002.
Wu, Y., Wang, X., Tao, J., Huang, R., Tian, P., Cao, J., Zhang, L., Ho, K.
F., Han, Z., and Zhang, R.: Size distribution and source of black carbon
aerosol in urban Beijing during winter haze episodes, Atmos. Chem. Phys.,
17, 7965–7975, https://doi.org/10.5194/acp-17-7965-2017, 2017.
Yang, X., Zhao, C., Guo, J., and Wang, Y.: Intensification of aerosol
pollution associated with its feedback with surface solar radiation and
winds in Beijing, J. Geophys. Res.-Atmos., 121,
4093–4099, https://doi.org/10.1002/2015JD024645, 2016.
Ye, X., Song, Y., Cai, X., and Zhang, H.: Study on the synoptic flow
patterns and boundary layer process of the severe haze events over the North
China Plain in January 2013, Atmos. Environ., 124, 129–145,
https://doi.org/10.1016/j.atmosenv.2015.06.011, 2016.
Zaveri, R. A., Easter, R. C., Fast, J. D., and Peters, L. K.: Model for
Simulating Aerosol Interactions and Chemistry (MOSAIC), J. Geophys. Res.-Atmos., 113, D13204, https://doi.org/10.1029/2007JD008782, 2008.
Zhang, J. P., Zhu, T., Zhang, Q. H., Li, C. C., Shu, H. L., Ying, Y., Dai,
Z. P., Wang, X., Liu, X. Y., Liang, A. M., Shen, H. X., and Yi, B. Q.: The
impact of circulation patterns on regional transport pathways and air
quality over Beijing and its surroundings, Atmos. Chem. Phys., 12,
5031–5053, https://doi.org/10.5194/acp-12-5031-2012, 2012.
Zhang, Q., Ma, X., Tie, X., Huang, M., and Zhao, C.: Vertical distributions
of aerosols under different weather conditions: Analysis of in-situ aircraft
measurements in Beijing, China, Atmos. Environ., 43, 5526–5535,
https://doi.org/10.1016/j.atmosenv.2009.05.037, 2009.
Zhang, Q., Zheng, Y., Tong, D., Shao, M., Wang, S., Zhang, Y., Xu, X., Wang,
J., He, H., Liu, W., Ding, Y., Lei, Y., Li, J., Wang, Z., Zhang, X., Wang,
Y., Cheng, J., Liu, Y., Shi, Q., Yan, L., Geng, G., Hong, C., Li, M., Liu,
F., Zheng, B., Cao, J., Ding, A., Gao, J., Fu, Q., Huo, J., Liu, B., Liu,
Z., Yang, F., He, K., and Hao, J.: Drivers of improved PM2.5 air
quality in China from 2013 to 2017, P. Natl. Acad.
Sci. USA, 116, 24463–24469, https://doi.org/10.1073/pnas.1907956116, 2019.
Zhang, W., Guo, J., Miao, Y., Liu, H., Song, Y., Fang, Z., He, J., Lou, M.,
Yan, Y., Li, Y., and Zhai, P.: On the Summertime Planetary Boundary Layer
with Different Thermodynamic Stability in China: A Radiosonde Perspective,
J. Clim., 31, 1451–1465, https://doi.org/10.1175/jcli-d-17-0231.1, 2018.
Zhang, X., Xu, X., Ding, Y., Liu, Y., Zhang, H., Wang, Y., and Zhong, J.:
The impact of meteorological changes from 2013 to 2017 on PM2.5 mass
reduction in key regions in China, Sci. China Earth Sci., 62,
1885–1902, https://doi.org/10.1007/s11430-019-9343-3, 2019.
Zhang, Y., Ding, A., Mao, H., Nie, W., Zhou, D., Liu, L., Huang, X., and Fu,
C.: Impact of synoptic weather patterns and inter-decadal climate
variability on air quality in the North China Plain during 1980–2013,
Atmos. Environ., 124, 119–128, https://doi.org/10.1016/j.atmosenv.2015.05.063, 2016.
Zhao, C., Yang, Y., Fan, H., Huang, J., Fu, Y., Zhang, X., Kang, S., Cong,
Z., Letu, H., and Menenti, M.: Aerosol characteristics and impacts on
weather and climate over the Tibetan Plateau, Natl. Sci. Rev., 7,
492–495, https://doi.org/10.1093/nsr/nwz184, 2019.
Zheng, B., Tong, D., Li, M., Liu, F., Hong, C., Geng, G., Li, H., Li, X.,
Peng, L., Qi, J., Yan, L., Zhang, Y., Zhao, H., Zheng, Y., He, K., and
Zhang, Q.: Trends in China's anthropogenic emissions since 2010 as the
consequence of clean air actions, Atmos. Chem. Phys., 18, 14095–14111,
https://doi.org/10.5194/acp-18-14095-2018, 2018.
Short summary
Aerosol–planetary boundary layer (PBL) interaction is a key mechanism for stabilizing the atmosphere and exacerbating surface air pollution. Using aircraft measurements and WRF-Chem simulations, we find that the aerosol–PBL interaction of different aerosols under contrasting synoptic patterns, PBL structures, and aerosol vertical distributions vary significantly. We attempt to determine which pollutants to target in different synoptic conditions to attain more precise air pollution control.
Aerosol–planetary boundary layer (PBL) interaction is a key mechanism for stabilizing the...
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