Articles | Volume 22, issue 3
https://doi.org/10.5194/acp-22-1773-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-1773-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
07 Feb 2022
Research article |
| 07 Feb 2022
| 07 Feb 2022
Data assimilation of volcanic aerosol observations using FALL3D+PDAF
Barcelona Supercomputing Center, Barcelona, Spain
Arnau Folch
Geociencias Barcelona (GEO3BCN-CSIC), Barcelona, Spain
Andrew T. Prata
Sub-department of Atmospheric, Oceanic and Planetary Physics, University of Oxford, Oxford, UK
Federica Pardini
Istituto Nazionale di Geofisica e Vulcanologia, Sezione di Pisa, Pisa, Italy
Giovanni Macedonio
Istituto Nazionale di Geofisica e Vulcanologia, Osservatorio Vesuviano, Naples, Italy
Antonio Costa
Istituto Nazionale di Geofisica e Vulcanologia, Sezione di Bologna, Bologna, Italy
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Arnau Folch, Leonardo Mingari, Natalia Gutierrez, Mauricio Hanzich, Giovanni Macedonio, and Antonio Costa
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Soledad Osores, Juan Ruiz, Arnau Folch, and Estela Collini
Geosci. Model Dev., 13, 1–22, https://doi.org/10.5194/gmd-13-1-2020, https://doi.org/10.5194/gmd-13-1-2020, 2020
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Volcanic ash dispersal forecasts are routinely used to avoid aircraft encounters with volcanic ash. However, the accuracy of these forecasts depends on the knowledge of key factors that are usually difficult to observe directly. In this work we apply an inverse methodology to improve ash concentration forecasts. Results are encouraging, showing that accurate estimations of ash emissions can be performed using the proposed approach, leading to an improvement in ash concentration forecasts.
Silvia Massaro, Antonio Costa, Roberto Sulpizio, Diego Coppola, and Lucia Capra
Solid Earth, 10, 1429–1450, https://doi.org/10.5194/se-10-1429-2019, https://doi.org/10.5194/se-10-1429-2019, 2019
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The Fuego de Colima volcano (Mexico) shows a complex eruptive history, with periods of rapid and slow lava dome growth punctuated by explosive activity. Here we reconstructed the 1998–2018 average discharge rate by means of satellite thermal data and the literature. Using spectral and wavelet analysis, we found a multi-term cyclic behavior that is in good agreement with numerical modeling, accounting for a variable magmatic feeding system composed of a single or double magma chamber system.
Matthieu Poret, Stefano Corradini, Luca Merucci, Antonio Costa, Daniele Andronico, Mario Montopoli, Gianfranco Vulpiani, and Valentin Freret-Lorgeril
Atmos. Chem. Phys., 18, 4695–4714, https://doi.org/10.5194/acp-18-4695-2018, https://doi.org/10.5194/acp-18-4695-2018, 2018
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Alejandro Marti and Arnau Folch
Atmos. Chem. Phys., 18, 4019–4038, https://doi.org/10.5194/acp-18-4019-2018, https://doi.org/10.5194/acp-18-4019-2018, 2018
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Arnau Folch, Jordi Barcons, Tomofumi Kozono, and Antonio Costa
Nat. Hazards Earth Syst. Sci., 17, 861–879, https://doi.org/10.5194/nhess-17-861-2017, https://doi.org/10.5194/nhess-17-861-2017, 2017
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Atmospheric dispersal of a gas denser than air can threat the environment and surrounding communities. In complex terrains, microscale winds and local orographic features can have a strong influence on the gas cloud behavior, potentially leading to inaccurate model results if not captured by coarser-scale simulations. We introduce a methodology for microscale wind field characterization and validate it using, as a test case, the CO2 gas dispersal from 1986 Lake Nyos eruption.
Leonardo A. Mingari, Estela A. Collini, Arnau Folch, Walter Báez, Emilce Bustos, María Soledad Osores, Florencia Reckziegel, Peter Alexander, and José G. Viramonte
Atmos. Chem. Phys., 17, 6759–6778, https://doi.org/10.5194/acp-17-6759-2017, https://doi.org/10.5194/acp-17-6759-2017, 2017
Short summary
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In this paper, we provide the first comprehensive description of
a dust episode occurred in South America in June 2015 through
observations and numerical simulations. We have investigated
the spatiotemporal distribution of aerosols and the emission
process over complex terrain to gain insight into the key role
played by the orography and the condition that triggered the
long-range transport episode.
Alejandro Marti, Arnau Folch, Oriol Jorba, and Zavisa Janjic
Atmos. Chem. Phys., 17, 4005–4030, https://doi.org/10.5194/acp-17-4005-2017, https://doi.org/10.5194/acp-17-4005-2017, 2017
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We describe and evaluate NMMB-MONARCH-ASH, a novel online multi-scale meteorological and transport model developed at the BSC-CNS capable of forecasting the dispersal and deposition of volcanic ash. The forecast skills of the model have been validated and they improve on those from traditional operational offline (decoupled) models. The results support the use of online coupled models to aid civil aviation and emergency management during a crisis such as the 2010 eruption of Eyjafjallajökull.
A. Folch, A. Costa, and G. Macedonio
Geosci. Model Dev., 9, 431–450, https://doi.org/10.5194/gmd-9-431-2016, https://doi.org/10.5194/gmd-9-431-2016, 2016
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We present FPLUME-1.0, a steady-state 1-D cross-section-averaged eruption column model based on the buoyant plume theory (BPT). The model accounts for plume bending by wind, entrainment of ambient moisture, effects of water phase changes, particle fallout and re-entrainment, a new parameterization for the air entrainment coefficients and a model for wet aggregation of ash particles in presence of liquid water or ice.
R. Tonini, L. Sandri, A. Costa, and J. Selva
Nat. Hazards Earth Syst. Sci., 15, 409–415, https://doi.org/10.5194/nhess-15-409-2015, https://doi.org/10.5194/nhess-15-409-2015, 2015
S. Biass, C. Scaini, C. Bonadonna, A. Folch, K. Smith, and A. Höskuldsson
Nat. Hazards Earth Syst. Sci., 14, 2265–2287, https://doi.org/10.5194/nhess-14-2265-2014, https://doi.org/10.5194/nhess-14-2265-2014, 2014
C. Scaini, S. Biass, A. Galderisi, C. Bonadonna, A. Folch, K. Smith, and A. Höskuldsson
Nat. Hazards Earth Syst. Sci., 14, 2289–2312, https://doi.org/10.5194/nhess-14-2289-2014, https://doi.org/10.5194/nhess-14-2289-2014, 2014
A. Folch, L. Mingari, M. S. Osores, and E. Collini
Nat. Hazards Earth Syst. Sci., 14, 119–133, https://doi.org/10.5194/nhess-14-119-2014, https://doi.org/10.5194/nhess-14-119-2014, 2014
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
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For Bucharest, Romania's capital, mobile measurements during two intensive campaigns and mixed-effect LUR (land-use regression) models to derive seasonal maps of near-surface PM10, NO2 and UFPs (ultrafine particles) have successfully been used. The model's performance was evaluated, demonstrating its potential for high-resolution mapping in other cities with well-characterized urban structures and diverse in situ monitoring stations.
Jiangtao Li, Xingqin An, Zhaobin Sun, Caihua Ye, Qing Hou, Yuxin Zhao, and Zhe Liu
Atmos. Chem. Phys., 25, 3583–3602, https://doi.org/10.5194/acp-25-3583-2025, https://doi.org/10.5194/acp-25-3583-2025, 2025
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Climate change and pollution have intensified pollen allergies. We developed a pollen emissions model using phenology and random forests. Key factors affecting annual pollen emissions include temperature, relative humidity and sunshine hours. Pollen dispersal starts around 10 August, peaks around 30 August and ends by 25 September, lasting about 45 d. Over time, annual pollen emissions exhibit significant fluctuations and a downward trend.
Ruth A. R. Digby, Knut von Salzen, Adam H. Monahan, Nathan P. Gillett, and Jiangnan Li
Atmos. Chem. Phys., 25, 3109–3130, https://doi.org/10.5194/acp-25-3109-2025, https://doi.org/10.5194/acp-25-3109-2025, 2025
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The refractive index of black carbon (BCRI), which determines how much energy black carbon absorbs and scatters, is difficult to measure, and different climate models use different values. We show that varying the BCRI across commonly used values can increase absorbing aerosol optical depth by 42 % and the warming effect from interactions between black carbon and radiation by 47 %, an appreciable fraction of the overall spread between models reported in recent literature assessments.
Hector Navarro-Barboza, Jordi Rovira, Vincenzo Obiso, Andrea Pozzer, Marta Via, Andres Alastuey, Xavier Querol, Noemi Perez, Marjan Savadkoohi, Gang Chen, Jesus Yus-Díez, Matic Ivancic, Martin Rigler, Konstantinos Eleftheriadis, Stergios Vratolis, Olga Zografou, Maria Gini, Benjamin Chazeau, Nicolas Marchand, Andre S. H. Prevot, Kaspar Dallenbach, Mikael Ehn, Krista Luoma, Tuukka Petäjä, Anna Tobler, Jaroslaw Necki, Minna Aurela, Hilkka Timonen, Jarkko Niemi, Olivier Favez, Jean-Eudes Petit, Jean-Philippe Putaud, Christoph Hueglin, Nicolas Pascal, Aurélien Chauvigné, Sébastien Conil, Marco Pandolfi, and Oriol Jorba
Atmos. Chem. Phys., 25, 2667–2694, https://doi.org/10.5194/acp-25-2667-2025, https://doi.org/10.5194/acp-25-2667-2025, 2025
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Brown carbon (BrC) absorbs ultraviolet (UV) and visible light, influencing climate. This study explores BrC's imaginary refractive index (k) using data from 12 European sites. Residential emissions are a major organic aerosol (OA) source in winter, while secondary organic aerosol (SOA) dominates in summer. Source-specific k values were derived, improving model accuracy. The findings highlight BrC's climate impact and emphasize source-specific constraints in atmospheric models.
Yuzhi Jin, Jiandong Wang, Chao Liu, David C. Wong, Golam Sarwar, Kathleen M. Fahey, Shang Wu, Jiaping Wang, Jing Cai, Zeyuan Tian, Zhouyang Zhang, Jia Xing, Aijun Ding, and Shuxiao Wang
Atmos. Chem. Phys., 25, 2613–2630, https://doi.org/10.5194/acp-25-2613-2025, https://doi.org/10.5194/acp-25-2613-2025, 2025
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Black carbon (BC) affects climate and the environment, and its aging process alters its properties. Current models, like WRF-CMAQ, lack full accounting for it. We developed the WRF-CMAQ-BCG model to better represent BC aging by introducing bare and coated BC species and their conversion. The WRF-CMAQ-BCG model introduces the capability to simulate BC mixing states and bare and coated BC wet deposition, and it improves the accuracy of BC mass concentration and aerosol optics.
Zhe Song, Shaocai Yu, Pengfei Li, Ningning Yao, Lang Chen, Yuhai Sun, Boqiong Jiang, and Daniel Rosenfeld
Atmos. Chem. Phys., 25, 2473–2494, https://doi.org/10.5194/acp-25-2473-2025, https://doi.org/10.5194/acp-25-2473-2025, 2025
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Our results with injected sea salt aerosols for five open oceans show that sea salt aerosols with low injection amounts dominate shortwave radiation, mainly through indirect effects. As indirect aerosol effects saturate with increasing injection rates, direct effects exceed indirect effects. This implies that marine cloud brightening is best implemented in areas with extensive cloud cover, while aerosol direct scattering effects remain dominant when clouds are scarce.
Danny M. Leung, Jasper F. Kok, Longlei Li, David M. Lawrence, Natalie M. Mahowald, Simone Tilmes, and Erik Kluzek
Atmos. Chem. Phys., 25, 2311–2331, https://doi.org/10.5194/acp-25-2311-2025, https://doi.org/10.5194/acp-25-2311-2025, 2025
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This study derives a gridded dust emission dataset for 1841–2000 by employing a combination of observed dust from core records and reanalyzed global dust cycle constraints. We evaluate the ability of global models to replicate the observed historical dust variability by using the emission dataset to force a historical simulation in an Earth system model. We show that prescribing our emissions forces the model to better match observations than other mechanistic models.
Hongyu Liu, Bo Zhang, Richard H. Moore, Luke D. Ziemba, Richard A. Ferrare, Hyundeok Choi, Armin Sorooshian, David Painemal, Hailong Wang, Michael A. Shook, Amy Jo Scarino, Johnathan W. Hair, Ewan C. Crosbie, Marta A. Fenn, Taylor J. Shingler, Chris A. Hostetler, Gao Chen, Mary M. Kleb, Gan Luo, Fangqun Yu, Mark A. Vaughan, Yongxiang Hu, Glenn S. Diskin, John B. Nowak, Joshua P. DiGangi, Yonghoon Choi, Christoph A. Keller, and Matthew S. Johnson
Atmos. Chem. Phys., 25, 2087–2121, https://doi.org/10.5194/acp-25-2087-2025, https://doi.org/10.5194/acp-25-2087-2025, 2025
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We use the GEOS-Chem model to simulate aerosol distributions and properties over the western North Atlantic Ocean (WNAO) during the winter and summer deployments in 2020 of the NASA ACTIVATE mission. Model results are evaluated against aircraft, ground-based, and satellite observations. The improved understanding of life cycle, composition, transport pathways, and distribution of aerosols has important implications for characterizing aerosol–cloud–meteorology interactions over WNAO.
Mingrui Ma, Jiachen Cao, Dan Tong, Bo Zheng, and Yu Zhao
Atmos. Chem. Phys., 25, 2147–2166, https://doi.org/10.5194/acp-25-2147-2025, https://doi.org/10.5194/acp-25-2147-2025, 2025
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We combined two global climate change pathways and three national emission control scenarios to analyze the future evolution of reactive nitrogen (Nr) deposition till the 2060s in China with air quality modeling. We show China’s clean air and carbon neutrality policies would overcome the adverse effects of climate change and efficiently reduce Nr deposition. The outflow of Nr fluxes from mainland China to the west Pacific would also be clearly reduced from continuous stringent emission controls.
Zhouyang Zhang, Jiandong Wang, Jiaping Wang, Nicole Riemer, Chao Liu, Yuzhi Jin, Zeyuan Tian, Jing Cai, Yueyue Cheng, Ganzhen Chen, Bin Wang, Shuxiao Wang, and Aijun Ding
Atmos. Chem. Phys., 25, 1869–1881, https://doi.org/10.5194/acp-25-1869-2025, https://doi.org/10.5194/acp-25-1869-2025, 2025
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Black carbon (BC) exerts notable warming effects. We use a particle-resolved model to investigate the long-term behavior of the BC mixing state, revealing its compositions, coating thickness distribution, and optical properties all stabilize with a characteristic time of less than 1 d. This study can effectively simplify the description of the BC mixing state, which facilitates the precise assessment of the optical properties of BC aerosols in global and chemical transport models.
Qianyi Huo, Zhicong Yin, Xiaoqing Ma, and Huijun Wang
Atmos. Chem. Phys., 25, 1711–1724, https://doi.org/10.5194/acp-25-1711-2025, https://doi.org/10.5194/acp-25-1711-2025, 2025
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Dust days during the spring seasons of 2015–2023 in North China were classified into Mongolian cyclone and cold high types depending on the presence of the Mongolian cyclone. The Mongolian cyclone type led to more frequent and severe dust weather, indicated by PM10 concentrations. To comprehensively forecast the two types of dust weather, a common predictor was established based on 500 hPa anomalous circulation systems, offering insights for dust weather forecasting and climate prediction.
Mariya Petrenko, Ralph Kahn, Mian Chin, Susanne E. Bauer, Tommi Bergman, Huisheng Bian, Gabriele Curci, Ben Johnson, Johannes W. Kaiser, Zak Kipling, Harri Kokkola, Xiaohong Liu, Keren Mezuman, Tero Mielonen, Gunnar Myhre, Xiaohua Pan, Anna Protonotariou, Samuel Remy, Ragnhild Bieltvedt Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Hailong Wang, Duncan Watson-Parris, and Kai Zhang
Atmos. Chem. Phys., 25, 1545–1567, https://doi.org/10.5194/acp-25-1545-2025, https://doi.org/10.5194/acp-25-1545-2025, 2025
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We compared smoke plume simulations from 11 global models to each other and to satellite smoke amount observations aimed at constraining smoke source strength. In regions where plumes are thick and background aerosol is low, models and satellites compare well. However, the input emission inventory tends to underestimate in many places, and particle property and loss rate assumptions vary enormously among models, causing uncertainties that require systematic in situ measurements to resolve.
Yongqing Bai, Tianliang Zhao, Kai Meng, Yue Zhou, Jie Xiong, Xiaoyun Sun, Lijuan Shen, Yanyu Yue, Yan Zhu, Weiyang Hu, and Jingyan Yao
Atmos. Chem. Phys., 25, 1273–1287, https://doi.org/10.5194/acp-25-1273-2025, https://doi.org/10.5194/acp-25-1273-2025, 2025
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We proposed a composite statistical method to identify the quasi-weekly oscillation (QWO) of regional PM2.5 transport over China in winter from 2015 to 2019. The QWO of regional PM2.5 transport is constrained by synoptic-scale disturbances of the East Asian winter monsoon circulation with the periodic activities of the Siberian high, providing a new insight into the understanding of regional pollutant transport with meteorological drivers in atmospheric environment changes.
Léo Clauzel, Sandrine Anquetin, Christophe Lavaysse, Gilles Bergametti, Christel Bouet, Guillaume Siour, Rémy Lapere, Béatrice Marticorena, and Jennie Thomas
Atmos. Chem. Phys., 25, 997–1021, https://doi.org/10.5194/acp-25-997-2025, https://doi.org/10.5194/acp-25-997-2025, 2025
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Solar energy production in West Africa is set to rise and needs accurate solar radiation estimates which are affected by desert dust. This work analyses a March 2021 dust event using a modelling strategy incorporating desert dust. Results show that considering desert dust cuts errors in solar radiation estimates by 75 % and reduces surface solar radiation by 18 %. This highlights the importance of incorporating dust aerosols into solar forecasting for better accuracy.
Pan Wang, Yue Zhao, Jiandong Wang, Veli-Matti Kerminen, Jingkun Jiang, and Chenxi Li
EGUsphere, https://doi.org/10.5194/egusphere-2024-3666, https://doi.org/10.5194/egusphere-2024-3666, 2025
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We developed a numerical model to explore how the charge state of newly formed atmospheric particles evolves during growth and how this relates to ion-induced nucleation rates. We identify the governing factors of particle charging and further apply neural networks to predict particle charge states and estimate ion induced nucleation rates. This study offers insights into particle charging dynamics and introduces new methods for assessing ion induced nucleation in atmospheric research.
Ross J. Herbert, Alberto Sanchez-Marroquin, Daniel P. Grosvenor, Kirsty J. Pringle, Stephen R. Arnold, Benjamin J. Murray, and Kenneth S. Carslaw
Atmos. Chem. Phys., 25, 291–325, https://doi.org/10.5194/acp-25-291-2025, https://doi.org/10.5194/acp-25-291-2025, 2025
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Aerosol particles that help form ice in clouds vary in number and type around the world and with time. However, in many weather and climate models cloud ice is not linked to aerosols that are known to nucleate ice. Here we report the first steps towards representing ice-nucleating particles within the UK Earth System Model. We conclude that in addition to ice nucleation by sea spray and mineral components of soil dust, we also need to represent ice nucleation by the organic components of soils.
Ryan Schmedding and Andreas Zuend
Atmos. Chem. Phys., 25, 327–346, https://doi.org/10.5194/acp-25-327-2025, https://doi.org/10.5194/acp-25-327-2025, 2025
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Four different approaches for computing the interfacial tension between liquid phases in aerosol particles were tested for particles with diameters from 10 nm to more than 5 μm. Antonov's rule led to the strongest reductions in the onset relative humidity of liquid–liquid phase separation and reproduced measured interfacial tensions for highly immiscible systems. A modified form of the Butler equation was able to best reproduce measured interfacial tensions in more miscible systems.
Masaru Yoshioka, Daniel P. Grosvenor, Ben B. B. Booth, Colin P. Morice, and Ken S. Carslaw
Atmos. Chem. Phys., 24, 13681–13692, https://doi.org/10.5194/acp-24-13681-2024, https://doi.org/10.5194/acp-24-13681-2024, 2024
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A 2020 regulation has reduced sulfur emissions from shipping by about 80 %, leading to a decrease in atmospheric aerosols that have a cooling effect primarily by affecting cloud properties and amounts. Our climate model simulations predict a global temperature increase of 0.04 K over the next 3 decades as a result, which could contribute to surpassing the Paris Agreement's 1.5 °C target. Reduced aerosols may have also contributed to the recent temperature spikes.
Alcide Zhao, Laura J. Wilcox, and Claire L. Ryder
Atmos. Chem. Phys., 24, 13385–13402, https://doi.org/10.5194/acp-24-13385-2024, https://doi.org/10.5194/acp-24-13385-2024, 2024
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Climate models include desert dust aerosols, which cause atmospheric heating and can change circulation patterns. We assess the effect of dust on the Indian and east Asian summer monsoons through multi-model experiments isolating the effect of dust in current climate models for the first time. Dust atmospheric heating results in a southward shift of western Pacific equatorial rainfall and an enhanced Indian summer monsoon. This shows the importance of accurate dust representation in models.
Ragnhild Bieltvedt Skeie, Rachael Byrom, Øivind Hodnebrog, Caroline Jouan, and Gunnar Myhre
Atmos. Chem. Phys., 24, 13361–13370, https://doi.org/10.5194/acp-24-13361-2024, https://doi.org/10.5194/acp-24-13361-2024, 2024
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In 2020, new regulations by the International Maritime Organization regarding sulfur emissions came into force, reducing emissions of SO2 from the shipping sector by approximately 80 %. In this study, we use multiple models to calculate how much the Earth energy balance changed due to the emission reduction or the so-called effective radiative forcing. The calculated effective radiative forcing is weak, comparable to the effect of the increase in CO2 over the last 2 to 3 years.
Ge Yu, Yueya Wang, Zhe Wang, and Xiaoming Shi
EGUsphere, https://doi.org/10.5194/egusphere-2024-3581, https://doi.org/10.5194/egusphere-2024-3581, 2024
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Studying the cloud-forming capacity of aerosols is crucial in climate research. The PartMC model can provide detailed particle information and help these studies. This model is integrated with the ideal meteorological Cloud Model 1 (CM1) to simulate the aerosols at cloud-forming locations. Significant changes are revealed in the hygroscopicity distribution of aerosols within ascending air parcels. Additionally, different ascent times also affect aerosol aging processes.
Mingxu Liu, Hitoshi Matsui, Douglas S. Hamilton, Sagar D. Rathod, Kara D. Lamb, and Natalie M. Mahowald
Atmos. Chem. Phys., 24, 13115–13127, https://doi.org/10.5194/acp-24-13115-2024, https://doi.org/10.5194/acp-24-13115-2024, 2024
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Atmospheric aerosol deposition provides bioavailable iron to promote marine primary production, yet the estimates of its fluxes remain highly uncertain. This study, by performing global aerosol simulations, demonstrates that iron-containing particle size upon emission is a critical factor in regulating soluble iron input to open oceans. Further observational constraints on this are needed to reduce modeling uncertainties.
Jingmin Li, Mattia Righi, Johannes Hendricks, Christof G. Beer, Ulrike Burkhardt, and Anja Schmidt
Atmos. Chem. Phys., 24, 12727–12747, https://doi.org/10.5194/acp-24-12727-2024, https://doi.org/10.5194/acp-24-12727-2024, 2024
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Aiming to understand underlying patterns and trends in aerosols, we characterize the spatial patterns and long-term evolution of lower tropospheric aerosols by clustering multiple aerosol properties from preindustrial times to the year 2050 under three Shared
Socioeconomic Pathway scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Socioeconomic Pathway scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Bishuo He and Chunsheng Zhao
EGUsphere, https://doi.org/10.5194/egusphere-2024-3441, https://doi.org/10.5194/egusphere-2024-3441, 2024
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Factor-uncertainty analysis helps us understand their impacts on complex systems. Traditional methods have many limitations. This study introduces a new method to measure how each factor contributes to uncertainty. It gains insights into the role of each variable and works for all multi-factor systems. As an application, we analyzed how aerosols affect solar radiation and identified the key factors. These analyses can improve our understanding of the role of aerosols in climate change.
Yueming Cheng, Tie Dai, Junji Cao, Daisuke Goto, Jianbing Jin, Teruyuki Nakajima, and Guangyu Shi
Atmos. Chem. Phys., 24, 12643–12659, https://doi.org/10.5194/acp-24-12643-2024, https://doi.org/10.5194/acp-24-12643-2024, 2024
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In March 2021, east Asia experienced an outbreak of severe dust storms after an absence of 1.5 decades. Here, we innovatively used the time-lagged ground-based aerosol size information with the fixed-lag ensemble Kalman smoother to optimize dust emission and reproduce the dust storm. This work is valuable for not only the quantification of health damage, aviation risks, and profound impacts on the Earth's system but also revealing the climatic driving force and the process of desertification.
Marc Mallet, Aurore Voldoire, Fabien Solmon, Pierre Nabat, Thomas Drugé, and Romain Roehrig
Atmos. Chem. Phys., 24, 12509–12535, https://doi.org/10.5194/acp-24-12509-2024, https://doi.org/10.5194/acp-24-12509-2024, 2024
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This study investigates the interactions between smoke aerosols and climate in tropical Africa using a coupled ocean–atmosphere–aerosol climate model. The work shows that smoke plumes have a significant impact by increasing the low-cloud fraction, decreasing the ocean and continental surface temperature and reducing the precipitation of coastal western Africa. It also highlights the role of the ocean temperature response and its feedbacks for the September–November season.
Jia Liu, Cancan Zhu, Donghui Zhou, and Jinbao Han
Atmos. Chem. Phys., 24, 12341–12354, https://doi.org/10.5194/acp-24-12341-2024, https://doi.org/10.5194/acp-24-12341-2024, 2024
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The hydrophilic coatings of aged black carbon (BC) particles absorb moisture during the hygroscopic growth process, but it is difficult to characterize how much water is absorbed under different relative humidities (RHs). In this study, we propose a method to obtain the water content in the coatings based on the equivalent complex refractive index retrieved from optical properties. This method is verified from a theoretical perspective, and it performs well for thickly coated BC at high RHs.
Mizuo Kajino, Kentaro Ishijima, Joseph Ching, Kazuyo Yamaji, Rio Ishikawa, Tomoki Kajikawa, Tanbir Singh, Tomoki Nakayama, Yutaka Matsumi, Koyo Kojima, Prabir K. Patra, and Sachiko Hayashida
EGUsphere, https://doi.org/10.5194/egusphere-2024-1811, https://doi.org/10.5194/egusphere-2024-1811, 2024
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Air pollution in Delhi during post monsoon period is severe and association with intensive crop residue burning (CRB) over Punjab state has attracted attention. However, the relationship has been unclear as the CRB emissions conventionally derived from satellites were underestimated due to clouds and haze over the region. We evaluated the impact of CRB on PM2.5 as about 50 %, based on a combination of numerical modeling and high-density observation network using low-cost sensors we installed.
Zijun Li, Angela Buchholz, and Noora Hyttinen
Atmos. Chem. Phys., 24, 11717–11725, https://doi.org/10.5194/acp-24-11717-2024, https://doi.org/10.5194/acp-24-11717-2024, 2024
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Evaluating organosulfur (OS) hygroscopicity is important for assessing aerosol–cloud climate interactions in the post-fossil-fuel future, when SO2 emissions decrease and OS compounds become increasingly important. Here a state-of-the-art quantum-chemistry-based method was used to predict the hygroscopic growth factors (HGFs) of a group of atmospherically relevant OS compounds and their mixtures with (NH4)2SO4. A good agreement was observed between their model-estimated and experimental HGFs.
Jamie R. Banks, Bernd Heinold, and Kerstin Schepanski
Atmos. Chem. Phys., 24, 11451–11475, https://doi.org/10.5194/acp-24-11451-2024, https://doi.org/10.5194/acp-24-11451-2024, 2024
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The Aralkum is a new desert in Central Asia formed by the desiccation of the Aral Sea. This has created a source of atmospheric dust, with implications for the balance of solar and thermal radiation. Simulating these effects using a dust transport model, we find that Aralkum dust adds radiative cooling effects to the surface and atmosphere on average but also adds heating events. Increases in surface pressure due to Aralkum dust strengthen the Siberian High and weaken the summer Asian heat low.
Xinyue Shao, Minghuai Wang, Xinyi Dong, Yaman Liu, Wenxiang Shen, Stephen R. Arnold, Leighton A. Regayre, Meinrat O. Andreae, Mira L. Pöhlker, Duseong S. Jo, Man Yue, and Ken S. Carslaw
Atmos. Chem. Phys., 24, 11365–11389, https://doi.org/10.5194/acp-24-11365-2024, https://doi.org/10.5194/acp-24-11365-2024, 2024
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Highly oxygenated organic molecules (HOMs) play an important role in atmospheric new particle formation (NPF). By semi-explicitly coupling the chemical mechanism of HOMs and a comprehensive nucleation scheme in a global climate model, the updated model shows better agreement with measurements of nucleation rate, growth rate, and NPF event frequency. Our results reveal that HOM-driven NPF leads to a considerable increase in particle and cloud condensation nuclei burden globally.
Anderson Da Silva, Louis Marelle, Jean-Christophe Raut, Yvette Gramlich, Karolina Siegel, Sophie L. Haslett, Claudia Mohr, and Jennie L. Thomas
EGUsphere, https://doi.org/10.5194/egusphere-2024-2839, https://doi.org/10.5194/egusphere-2024-2839, 2024
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Particles sources in polar climates are unclear, affecting climate representation in models. This study introduces an evaluated method for tracking particles with backtrajectory modeling. Tests on simulated particles allowed to show that traditional detection methods often misidentify sources. An improved method that accurately traces origins of aerosol particles in the Arctic is presented. The study recommends using this enhanced method for better source identification of atmospheric species.
Stuart Evans
EGUsphere, https://doi.org/10.5194/egusphere-2024-2820, https://doi.org/10.5194/egusphere-2024-2820, 2024
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This study of the North American Great Plains identifies the various weather patterns responsible for blowing dust in all parts of the region using a weather pattern classification. In the southwest plains passing cold fronts are the primary cause of dust; in the understudied northern plains, summertime patterns and southerly pre-frontal winds are most important in the west and east, respectively. These results are valuable to understanding and forecasting dust in this complex source region.
Falei Xu, Shuang Wang, Yan Li, and Juan Feng
Atmos. Chem. Phys., 24, 10689–10705, https://doi.org/10.5194/acp-24-10689-2024, https://doi.org/10.5194/acp-24-10689-2024, 2024
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This study examines how the winter North Atlantic Oscillation (NAO) and El Niño–Southern Oscillation (ENSO) affect dust activities in North China during the following spring. The results show that the NAO and ENSO, particularly in their negative phases, greatly influence dust activities. When both are negative, their combined effect on dust activities is even greater. This research highlights the importance of these climate patterns in predicting spring dust activities in North China.
Hengheng Zhang, Wei Huang, Xiaoli Shen, Ramakrishna Ramisetty, Junwei Song, Olga Kiseleva, Christopher Claus Holst, Basit Khan, Thomas Leisner, and Harald Saathoff
Atmos. Chem. Phys., 24, 10617–10637, https://doi.org/10.5194/acp-24-10617-2024, https://doi.org/10.5194/acp-24-10617-2024, 2024
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Our study unravels how stagnant winter conditions elevate aerosol levels in Stuttgart. Cloud cover at night plays a pivotal role, impacting morning air quality. Validating a key model, our findings aid accurate air quality predictions, crucial for effective pollution mitigation in urban areas.
Giorgio Veratti, Alessandro Bigi, Michele Stortini, Sergio Teggi, and Grazia Ghermandi
Atmos. Chem. Phys., 24, 10475–10512, https://doi.org/10.5194/acp-24-10475-2024, https://doi.org/10.5194/acp-24-10475-2024, 2024
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In a study of two consecutive winter seasons, we used measurements and modelling tools to identify the levels and sources of black carbon pollution in a medium-sized urban area of the Po Valley, Italy. Our findings show that biomass burning and traffic-related emissions (especially from Euro 4 diesel cars) significantly contribute to BC concentrations. This research offers crucial insights for policymakers and urban planners aiming to improve air quality in cities.
Steven Soon-Kai Kong, Joshua S. Fu, Neng-Huei Lin, Guey-Rong Sheu, and Wei-Syun Huang
EGUsphere, https://doi.org/10.5194/egusphere-2024-2549, https://doi.org/10.5194/egusphere-2024-2549, 2024
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The accuracy of the chemical transport model, a key focus of our research, is strongly dependent on the dry deposition parameterization. Our finding shows that the refined CMAQ dust model correlated well with the ground and high altitude in-situ measurements by implementing the suggested dry deposition schemes. Furthermore, we reveal the mixing state of two types of aerosols at the upper level, a finding supported by both the optimized model and measurement.
Pascal Lemaitre, Arnaud Quérel, Alexis Dépée, Alice Guerra Devigne, Marie Monier, Thibault Hiron, Chloé Soto Minguez, Daniel Hardy, and Andrea Flossmann
Atmos. Chem. Phys., 24, 9713–9732, https://doi.org/10.5194/acp-24-9713-2024, https://doi.org/10.5194/acp-24-9713-2024, 2024
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A new in-cloud scavenging scheme is proposed. It is based on a microphysical model of cloud formation and may be applied to long-distance atmospheric transport models (> 100 km) and climatic models. This model is applied to the two most extreme precipitating cloud types in terms of both relative humidity and vertical extension: cumulonimbus and stratus.
Alex Rowell, James Brean, David C. S. Beddows, Tuukka Petäjä, Máté Vörösmarty, Imre Salma, Jarkko V. Niemi, Hanna E. Manninen, Dominik van Pinxteren, Thomas Tuch, Kay Weinhold, Zongbo Shi, and Roy M. Harrison
Atmos. Chem. Phys., 24, 9515–9531, https://doi.org/10.5194/acp-24-9515-2024, https://doi.org/10.5194/acp-24-9515-2024, 2024
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Different sources of airborne particles in the atmospheres of four European cities were distinguished by recognising their particle size distributions using a statistical procedure, positive matrix factorisation. The various sources responded differently to the changes in emissions associated with COVID-19 lockdowns, and the reasons are investigated. While traffic emissions generally decreased, particles formed from reactions of atmospheric gases decreased in some cities but increased in others.
Amy H. Peace, Ying Chen, George Jordan, Daniel G. Partridge, Florent Malavelle, Eliza Duncan, and Jim M. Haywood
Atmos. Chem. Phys., 24, 9533–9553, https://doi.org/10.5194/acp-24-9533-2024, https://doi.org/10.5194/acp-24-9533-2024, 2024
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Natural aerosols from volcanic eruptions can help us understand how anthropogenic aerosols modify climate. We use observations and model simulations of the 2014–2015 Holuhraun eruption plume to examine aerosol–cloud interactions in September 2014. We find a shift to clouds with smaller, more numerous cloud droplets in the first 2 weeks of the eruption. In the third week, the background meteorology and previous conditions experienced by air masses modulate the aerosol perturbation to clouds.
Hua Lu, Min Xie, Bingliang Zhuang, Danyang Ma, Bojun Liu, Yangzhihao Zhan, Tijian Wang, Shu Li, Mengmeng Li, and Kuanguang Zhu
Atmos. Chem. Phys., 24, 8963–8982, https://doi.org/10.5194/acp-24-8963-2024, https://doi.org/10.5194/acp-24-8963-2024, 2024
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To identify cloud, aerosol, and planetary boundary layer (PBL) interactions from an air quality perspective, we summarized two pollution patterns characterized by denser liquid cloud and by obvious cloud radiation interaction (CRI). Numerical simulation experiments showed CRI could cause a 50 % reduction in aerosol radiation interaction (ARI) under a low-trough system. The results emphasized the nonnegligible role of CRI and its inhibition of ARI under wet and cloudy pollution synoptic patterns.
Huiyun Du, Jie Li, Xueshun Chen, Gabriele Curci, Fangqun Yu, Yele Sun, Xu Dao, Song Guo, Zhe Wang, Wenyi Yang, Lianfang Wei, and Zifa Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-1432, https://doi.org/10.5194/egusphere-2024-1432, 2024
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Inadequate consideration of mixing state and coatings on BC hinders aerosol radiation forcing quantification. While core-shell mixing results match observations closely, partial internal mixing and coating are more realistic. The fraction of embedded BC and coating aerosols resolved by a microphysics module were used to constrain the mixing state. This led to a 30~43 % absorption enhancement decrease over Northern China, offering valuable insights for the assessment of BC's radiative effects.
Emilie Fons, Ann Kristin Naumann, David Neubauer, Theresa Lang, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 8653–8675, https://doi.org/10.5194/acp-24-8653-2024, https://doi.org/10.5194/acp-24-8653-2024, 2024
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Aerosols can modify the liquid water path (LWP) of stratocumulus and, thus, their radiative effect. We compare storm-resolving model and satellite data that disagree on the sign of LWP adjustments and diagnose this discrepancy with causal inference. We find that strong precipitation, the absence of wet scavenging, and cloud deepening under a weak inversion contribute to positive LWP adjustments to aerosols in the model, despite weak negative effects from cloud-top entrainment enhancement.
Muhammed Irfan, Thomas Kühn, Taina Yli-Juuti, Anton Laakso, Eemeli Holopainen, Douglas R. Worsnop, Annele Virtanen, and Harri Kokkola
Atmos. Chem. Phys., 24, 8489–8506, https://doi.org/10.5194/acp-24-8489-2024, https://doi.org/10.5194/acp-24-8489-2024, 2024
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The study examines how the volatility of semi-volatile organic compounds affects secondary organic aerosol (SOA) formation and climate. Our simulations show that uncertainties in these volatilities influence aerosol mass and climate impacts. Accurate representation of these compounds in climate models is crucial for predicting global climate patterns.
Zhixin Xue, Nair Udaysankar, and Sundar Christopher
EGUsphere, https://doi.org/10.5194/egusphere-2024-1781, https://doi.org/10.5194/egusphere-2024-1781, 2024
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Canadian wildfires degrade US air quality through long-range smoke transport. This study uses surface, satellite, and numerical models to assess the PM2.5 increase due to Canadian fires during 2018 fire season. Satellite data, often limited by cloud cover, was supplemented with high-resolution simulated data to fill gaps. Weather systems significantly influenced smoke movement. Canadian fires led to a notable rise in PM2.5 levels across various US regions during the 2018 summer wildfire events.
Alkiviadis Kalisoras, Aristeidis K. Georgoulias, Dimitris Akritidis, Robert J. Allen, Vaishali Naik, Chaincy Kuo, Sophie Szopa, Pierre Nabat, Dirk Olivié, Twan van Noije, Philippe Le Sager, David Neubauer, Naga Oshima, Jane Mulcahy, Larry W. Horowitz, and Prodromos Zanis
Atmos. Chem. Phys., 24, 7837–7872, https://doi.org/10.5194/acp-24-7837-2024, https://doi.org/10.5194/acp-24-7837-2024, 2024
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Effective radiative forcing (ERF) is a metric for estimating how human activities and natural agents change the energy flow into and out of the Earth’s climate system. We investigate the anthropogenic aerosol ERF, and we estimate the contribution of individual processes to the total ERF using simulations from Earth system models within the Coupled Model Intercomparison Project Phase 6 (CMIP6). Our findings highlight that aerosol–cloud interactions drive ERF variability during the last 150 years.
Qianqian Song, Paul Ginoux, María Gonçalves Ageitos, Ron L. Miller, Vincenzo Obiso, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 7421–7446, https://doi.org/10.5194/acp-24-7421-2024, https://doi.org/10.5194/acp-24-7421-2024, 2024
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We implement and simulate the distribution of eight dust minerals in the GFDL AM4.0 model. We found that resolving the eight minerals reduces dust absorption compared to the homogeneous dust used in the standard GFDL AM4.0 model that assumes a globally uniform hematite content of 2.7 % by volume. Resolving dust mineralogy results in significant impacts on radiation, land surface temperature, surface winds, and precipitation over North Africa in summer.
Senyi Kong, Zheng Wang, and Lei Bi
Atmos. Chem. Phys., 24, 6911–6935, https://doi.org/10.5194/acp-24-6911-2024, https://doi.org/10.5194/acp-24-6911-2024, 2024
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The retrieval of refractive indices of dust aerosols from laboratory optical measurements is commonly done assuming spherical particles. This paper aims to investigate the uncertainties in the shortwave refractive indices and corresponding optical properties by considering non-spherical and inhomogeneous models for dust samples. The study emphasizes the significance of using non-spherical models for simulating dust aerosols.
Wenxuan Hua, Sijia Lou, Xin Huang, Lian Xue, Ke Ding, Zilin Wang, and Aijun Ding
Atmos. Chem. Phys., 24, 6787–6807, https://doi.org/10.5194/acp-24-6787-2024, https://doi.org/10.5194/acp-24-6787-2024, 2024
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In this study, we diagnose uncertainties in carbon monoxide and organic carbon emissions from four inventories for seven major wildfire-prone regions. Uncertainties in vegetation classification methods, fire detection products, and cloud obscuration effects lead to bias in these biomass burning (BB) emission inventories. By comparing simulations with measurements, we provide certain inventory recommendations. Our study has implications for reducing uncertainties in emissions in further studies.
Chandrakala Bharali, Mary Barth, Rajesh Kumar, Sachin D. Ghude, Vinayak Sinha, and Baerbel Sinha
Atmos. Chem. Phys., 24, 6635–6662, https://doi.org/10.5194/acp-24-6635-2024, https://doi.org/10.5194/acp-24-6635-2024, 2024
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This study examines the role of atmospheric aerosols in winter fog over the Indo-Gangetic Plains of India using WRF-Chem. The increase in RH with aerosol–radiation feedback (ARF) is found to be important for fog formation as it promotes the growth of aerosols in the polluted environment. Aqueous-phase chemistry in the fog increases PM2.5 concentration, further affecting ARF. ARF and aqueous-phase chemistry affect the fog intensity and the timing of fog formation by ~1–2 h.
Cited articles
Amezcua, J. and Van Leeuwen, P. J.: Gaussian anamorphosis in the analysis step
of the EnKF: a joint state-variable/observation approach, Tellus A, 66,
23493, https://doi.org/10.3402/tellusa.v66.23493, 2014. a
Anderson, J., Hoar, T., Raeder, K., Liu, H., Collins, N., Torn, R., and
Avellano, A.: The data assimilation research testbed: A community facility,
B. Am. Meteorol. Soc., 90, 1283–1296, 2009. a
Anderson, J. L. and Anderson, S. L.: A Monte Carlo Implementation of the
Nonlinear Filtering Problem to Produce Ensemble Assimilations and Forecasts,
Mon. Weather Rev., 127, 2741–2758,
https://doi.org/10.1175/1520-0493(1999)127<2741:AMCIOT>2.0.CO;2, 1999. a
Beckett, F. M., Witham, C. S., Leadbetter, S. J., Crocker, R., Webster, H. N.,
Hort, M. C., Jones, A. R., Devenish, B. J., and Thomson, D. J.: Atmospheric
Dispersion Modelling at the London VAAC: A Review of Developments since the
2010 Eyjafjallajökull Volcano Ash Cloud, Atmosphere, 11, 352,
https://doi.org/10.3390/atmos11040352, 2020. a
Bessho, K., Date, K., Hayashi, M., Ikeda, A., Imai, T., Inoue, H., Kumagai, Y.,
Miyakawa, T., Murata, H., Ohno, T., et al.: An introduction to
Himawari-8/9–Japan's new-generation geostationary meteorological satellites,
J. Meteorol. Soc. Jpn., 94, 151–183,
https://doi.org/10.2151/jmsj.2016-009, 2016. a
Bishop, C. H.: The GIGG-EnKF: ensemble Kalman filtering for highly skewed
non-negative uncertainty distributions, Q. J. Roy. Meteor. Soc., 142,
1395–1412, https://doi.org/10.1002/qj.2742, 2016. a
Bishop, C. H., Etherton, B. J., and Majumdar, S. J.: Adaptive Sampling with the
Ensemble Transform Kalman Filter. Part I: Theoretical Aspects, Mon. Weather
Rev., 129, 420–436, https://doi.org/10.1175/1520-0493(2001)129<0420:ASWTET>2.0.CO;2,
2001. a, b
Bonadonna, C., Folch, A., Loughlin, S., and Puempel, H.: Future developments
in modelling and monitoring of volcanic ash clouds: outcomes from the first
IAVCEI-WMO workshop on Ash Dispersal Forecast and Civil Aviation, Bull.
Volcanol., 74, 1–10, https://doi.org/10.1007/s00445-011-0508-6, 2012. a
Bonavita, M., Hólm, E., Isaksen, L., and Fisher, M.: The evolution of the
ECMWF hybrid data assimilation system, Q. J. Roy. Meteor. Soc., 142,
287–303, https://doi.org/10.1002/qj.2652, 2016. a
Burgers, G., Jan van Leeuwen, P., and Evensen, G.: Analysis Scheme in the
Ensemble Kalman Filter, Mon. Weather Rev., 126, 1719–1724,
https://doi.org/10.1175/1520-0493(1998)126<1719:ASITEK>2.0.CO;2, 1998. a, b
Carrassi, A., Bocquet, M., Bertino, L., and Evensen, G.: Data assimilation in
the geosciences: An overview of methods, issues, and perspectives, WIREs
Climate Change, 9, e535, https://doi.org/10.1002/wcc.535, 2018. a, b, c, d
Clarkson, R. J., Majewicz, E. J., and Mack, P.: A re-evaluation of the 2010
quantitative understanding of the effects volcanic ash has on gas turbine
engines, Proceedings of the Institution of Mechanical Engineers, Part G:
J. Aero. Eng., 230, 2274–2291,
https://doi.org/10.1177/0954410015623372, 2016. a
Costa, A., Pioli, L., and Bonadonna, C.: Assessing tephra total grain-size
distribution: Insights from field data analysis, Earth Planet. Sc. Lett.,
443, 90–107, https://doi.org/10.1016/j.epsl.2016.02.040, 2016a. a, b
Costa, A., Suzuki, Y., Cerminara, M., Devenish, B., Ongaro, T. E., Herzog, M.,
Eaton, A. V., Denby, L., Bursik, M., de' Michieli Vitturi, M., Engwell, S.,
Neri, A., Barsotti, S., Folch, A., Macedonio, G., Girault, F., Carazzo, G.,
Tait, S., Kaminski, E., Mastin, L., Woodhouse, M., Phillips, J., Hogg, A.,
Degruyter, W., and Bonadonna, C.: Results of the eruptive column model
inter-comparison study, J. Volcanol. Geoth. Res., 326, 2–25,
https://doi.org/10.1016/j.jvolgeores.2016.01.017, 2016b. a, b
Degruyter, W. and Bonadonna, C.: Improving on mass flow rate estimates of
volcanic eruptions, Geophys. Res. Lett., 39, , L16308, https://doi.org/10.1029/2012GL052566,
2012. a, b
Eckhardt, S., Prata, A. J., Seibert, P., Stebel, K., and Stohl, A.: Estimation of the vertical profile of sulfur dioxide injection into the atmosphere by a volcanic eruption using satellite column measurements and inverse transport modeling, Atmos. Chem. Phys., 8, 3881–3897, https://doi.org/10.5194/acp-8-3881-2008, 2008. a
Evensen, G.: Sequential data assimilation with a nonlinear quasi-geostrophic
model using Monte Carlo methods to forecast error statistics, J. Geophys.
Res.-Oceans, 99, 10143–10162, https://doi.org/10.1029/94JC00572, 1994. a, b
Evensen, G.: The ensemble Kalman filter: Theoretical formulation and practical
implementation, Ocean Dynam., 53, 343–367, 2003. a
Folch, A.: A review of tephra transport and dispersal models: Evolution,
current status, and future perspectives, J. Volcanol. Geoth. Res., 235,
96–115, https://doi.org/10.1016/j.jvolgeores.2012.05.020, 2012. a
Folch, A., Costa, A., and Macedonio, G.: FALL3D: A computational model for
transport and deposition of volcanic ash, Comput. Geosci., 35, 1334–1342,
https://doi.org/10.1016/j.cageo.2008.08.008, 2009. a
Folch, A., Mingari, L., Gutierrez, N., Hanzich, M., Macedonio, G., and Costa, A.: FALL3D-8.0: a computational model for atmospheric transport and deposition of particles, aerosols and radionuclides – Part 1: Model physics and numerics, Geosci. Model Dev., 13, 1431–1458, https://doi.org/10.5194/gmd-13-1431-2020, 2020. a, b, c
Folch, A., Mingari, L. and Prata, A. T.: Ensemble-Based Forecast of Volcanic Clouds Using FALL3D-8.1, Front. Earth Sci., 9, 741841, https://doi.org/10.3389/feart.2021.741841, 2021. a, b, c, d
Fu, G., Lin, H., Heemink, A., Segers, A., Lu, S., and Palsson, T.: Assimilating
aircraft-based measurements to improve forecast accuracy of volcanic ash
transport, Atmos. Environ., 115, 170–184,
https://doi.org/10.1016/j.atmosenv.2015.05.061, 2015. a
Fu, G., Heemink, A., Lu, S., Segers, A., Weber, K., and Lin, H.-X.: Model-based aviation advice on distal volcanic ash clouds by assimilating aircraft in situ measurements, Atmos. Chem. Phys., 16, 9189–9200, https://doi.org/10.5194/acp-16-9189-2016, 2016. a
Fu, G., Lin, H. X., Heemink, A., Lu, S., Segers, A., van Velzen, N., Lu, T., and Xu, S.: Accelerating volcanic ash data assimilation using a mask-state algorithm based on an ensemble Kalman filter: a case study with the LOTOS-EUROS model (version 1.10), Geosci. Model Dev., 10, 1751–1766, https://doi.org/10.5194/gmd-10-1751-2017, 2017a. a
Fu, G., Prata, F., Lin, H. X., Heemink, A., Segers, A., and Lu, S.: Data assimilation for volcanic ash plumes using a satellite observational operator: a case study on the 2010 Eyjafjallajökull volcanic eruption, Atmos. Chem. Phys., 17, 1187–1205, https://doi.org/10.5194/acp-17-1187-2017, 2017b. a
Gordon, N. J., Salmond, D. J., and Smith, A. F.: Novel approach to
nonlinear/non-Gaussian Bayesian state estimation, in: IEE Proc.-F, Vol. 140,
107–113, 1993. a
Hodyss, D.: Accounting for skewness in ensemble data assimilation, Mon. Weather
Rev., 140, 2346–2358, 2012. a
Hodyss, D. and Campbell, W. F.: Square root and perturbed observation ensemble
generation techniques in Kalman and quadratic ensemble filtering algorithms,
Mon. Weather Rev., 141, 2561–2573, 2013. a
Houtekamer, P. L. and Zhang, F.: Review of the Ensemble Kalman Filter for
Atmospheric Data Assimilation, Mon. Weather Rev., 144, 4489–4532,
https://doi.org/10.1175/MWR-D-15-0440.1, 2016. a, b
Kalman, R. E.: A New Approach to Linear Filtering and Prediction Problems,
Journal of Basic Engineering, 82, 35–45, https://doi.org/10.1115/1.3662552, 1960. a, b
Kalnay, E.: Atmospheric modeling, data assimilation and predictability,
Cambridge university press, 2003. a
Kleist, D. T., Parrish, D. F., Derber, J. C., Treadon, R., Wu, W.-S., and Lord,
S.: Introduction of the GSI into the NCEP global data assimilation system,
Weather Forecast., 24, 1691–1705, 2009. a
Kloss, C., Berthet, G., Sellitto, P., Ploeger, F., Taha, G., Tidiga, M., Eremenko, M., Bossolasco, A., Jégou, F., Renard, J.-B., and Legras, B.: Stratospheric aerosol layer perturbation caused by the 2019 Raikoke and Ulawun eruptions and their radiative forcing, Atmos. Chem. Phys., 21, 535–560, https://doi.org/10.5194/acp-21-535-2021, 2021. a
Kristiansen, N. I., Stohl, A., Prata, A. J., Richter, A., Eckhardt, S.,
Seibert, P., Hoffmann, A., Ritter, C., Bitar, L., Duck, T. J., and Stebel,
K.: Remote sensing and inverse transport modeling of the Kasatochi eruption
sulfur dioxide cloud, J. Geophys. Res.-Atmos., 115, D00L16,
https://doi.org/10.1029/2009JD013286, 2010. a
Lu, S., Lin, H., Heemink, A., Fu, G., and Segers, A.: Estimation of volcanic
ash emissions using trajectory-based 4D-Var data assimilation, Mon. Weather
Rev., 144, 575–589, 2016a. a
Lu, S., Lin, H. X., Heemink, A., Segers, A., and Fu, G.: Estimation of volcanic
ash emissions through assimilating satellite data and ground-based
observations, J. Geophys. Res.-Atmos., 121, 10971–10994,
https://doi.org/10.1002/2016JD025131, 2016b. a
McKay, M. D., Beckman, R. J., and Conover, W. J.: A Comparison of Three Methods
for Selecting Values of Input Variables in the Analysis of Output from a
Computer Code, Technometrics, 21, 239–245, 1979. a
Mingari, L., Folch, A., Dominguez, L., and Bonadonna, C.: Volcanic Ash
Resuspension in Patagonia: Numerical Simulations and Observations,
Atmosphere, 11, 977, https://doi.org/10.3390/atmos11090977, 2020. a
Muser, L. O., Hoshyaripour, G. A., Bruckert, J., Horváth, Á., Malinina, E., Wallis, S., Prata, F. J., Rozanov, A., von Savigny, C., Vogel, H., and Vogel, B.: Particle aging and aerosol–radiation interaction affect volcanic plume dispersion: evidence from the Raikoke 2019 eruption, Atmos. Chem. Phys., 20, 15015–15036, https://doi.org/10.5194/acp-20-15015-2020, 2020. a
Nerger, L., Hiller, W., and Schröter, J.: PDAF - The Parallel Data
Assimilation Framework: Experiences with Kalman filtering, in: Use of High
Performance Computing in Meteorology, 63–83, World Scientific,
https://doi.org/10.1142/9789812701831_0006, 2005. a, b, c
Nerger, L., Janjić, T., Schröter, J., and Hiller, W.: A Unification of
Ensemble Square Root Kalman Filters, Mon. Weather Rev., 140, 2335–2345,
https://doi.org/10.1175/MWR-D-11-00102.1, 2012. a, b, c, d
Osores, S., Ruiz, J., Folch, A., and Collini, E.: Volcanic ash forecast using ensemble-based data assimilation: an ensemble transform Kalman filter coupled with the FALL3D-7.2 model (ETKF–FALL3D version 1.0), Geosci. Model Dev., 13, 1–22, https://doi.org/10.5194/gmd-13-1-2020, 2020. a
Ott, E., Hunt, B. R., Szunyogh, I., Zimin, A. V., Kostelich, E. J., Corazza,
M., Kalnay, E., Patil, D., and Yorke, J. A.: A local ensemble Kalman filter
for atmospheric data assimilation, Tellus A, 56, 415–428, https://doi.org/10.3402/tellusa.v56i5.14462, 2004. a
Pardini, F., Corradini, S., Costa, A., Esposti Ongaro, T., Merucci, L., Neri, A., Stelitano, D., and de' Michieli Vitturi, M.: Ensemble-Based Data Assimilation of Volcanic Ash
Clouds from Satellite Observations: Application to the 24 December 2018 Mt.
Etna Explosive Eruption, Atmosphere, 11, 359, https://doi.org/10.3390/atmos11040359, 2020. a, b
Pfeiffer, T., Costa, A., and Macedonio, G.: A model for the numerical
simulation of tephra fall deposits, J. Volcanol. Geoth. Res., 140, 273–294, https://doi.org/10.1016/j.jvolgeores.2004.09.001, 2005. a, b
Poulidis, A. P. and Iguchi, M.: Model sensitivities in the case of
high-resolution Eulerian simulations of local tephra transport and
deposition, Atmos. Res., 247, 105136, https://doi.org/10.1016/j.atmosres.2020.105136,
2021. a
Prata, A., Rose, W., Self, S., and O'Brien, D.: Global, Long-Term Sulphur
Dioxide Measurements from TOVS Data: A New Tool for Studying Explosive
Volcanism and Climate, in: Volcanism and the Earth's Atmosphere, edited by:
Robock, A. and Oppenheimer, C., American Geophysical Union (AGU), 75–92,
https://doi.org/10.1029/139GM05, 2004. a
Prata, A. J. and Prata, A. T.: Eyjafjallajökull volcanic ash concentrations
determined using Spin Enhanced Visible and Infrared Imager measurements, J.
Geophys. Res.-Atmos., 117, D00U23, https://doi.org/10.1029/2011JD016800, 2012. a
Prata, A. T., Mingari, L., Folch, A., Macedonio, G., and Costa, A.: FALL3D-8.0: a computational model for atmospheric transport and deposition of particles, aerosols and radionuclides – Part 2: Model validation, Geosci. Model Dev., 14, 409–436, https://doi.org/10.5194/gmd-14-409-2021, 2021. a, b, c, d, e
Schmetz, J., Pili, P., Tjemkes, S., Just, D., Kerkmann, J., Rota, S., and
Ratier, A.: An introduction to Meteosat Second Generation (MSG), B. Am. Meteorol. Soc., 83, 977–992,
https://doi.org/10.1175/1520-0477(2002)083<0977:AITMSG>2.3.CO;2, 2002. a
Sulpizio, R., Folch, A., Costa, A., Scaini, C., and Dellino, P.: Hazard
assessment of far-range volcanic ash dispersal from a violent Strombolian
eruption at Somma-Vesuvius volcano, Naples, Italy: Implications on civil
aviation, Bull. Volcanol., 74, 2205–2218, https://doi.org/10.1007/s00445-012-0656-3,
2012. a
Suzuki, Y., Costa, A., Cerminara, M., Esposti Ongaro, T., Herzog, M., Van
Eaton, A., and Denby, L.: Inter-comparison of three-dimensional models of
volcanic plumes, J. Volcanol. Geoth. Res., 326, 26–42,
https://doi.org/10.1016/j.jvolgeores.2016.06.011, 2016a. a
Suzuki, Y., Costa, A., and Koyaguchi, T.: On the relationship between eruption
intensity and volcanic plume height: Insights from three-dimensional
numerical simulations, J. Volcanol. Geoth. Res., 326, 120–126,
https://doi.org/10.1016/j.jvolgeores.2016.04.016, 2016b. a, b
Tödter, J. and Ahrens, B.: A Second-Order Exact Ensemble Square Root Filter
for Nonlinear Data Assimilation, Mon. Weather Rev., 143, 1347–1367,
https://doi.org/10.1175/MWR-D-14-00108.1, 2015. a, b, c, d
van Leeuwen, P. J. and Ades, M.: Efficient fully nonlinear data assimilation
for geophysical fluid dynamics, Comput. Geosci., 55, 16–27,
https://doi.org/10.1016/j.cageo.2012.04.015, 2013. a
Whitaker, J. S., Hamill, T. M., Wei, X., Song, Y., and Toth, Z.: Ensemble data
assimilation with the NCEP Global Forecast System, Mon. Weather Rev., 136,
463–482, 2008. a
Wilkins, K., Western, L., and Watson, I.: Simulating atmospheric transport of
the 2011 Grímsvötn ash cloud using a data insertion update scheme, Atmos.
Environ., 141, 48–59, https://doi.org/10.1016/j.atmosenv.2016.06.045,
2016a. a
Wilkins, K. L., Mackie, S., Watson, M., Webster, H. N., Thomson, D. J., and
Dacre, H. F.: Data insertion in volcanic ash cloud forecasting, Ann.
Geophys., 57, https://doi.org/10.4401/ag-6624, 2015. a
Wilkins, K. L., Watson, I. M., Kristiansen, N. I., Webster, H. N., Thomson,
D. J., Dacre, H. F., and Prata, A. J.: Using data insertion with the NAME
model to simulate the 8 May 2010 Eyjafjallajökull volcanic ash cloud, J.
Geophys. Res.-Atmos., 121, 306–323, https://doi.org/10.1002/2015JD023895,
2016b. a
Wilson, G., Wilson, T., Deligne, N., and Cole, J.: Volcanic hazard impacts to
critical infrastructure: A review, J. Volcanol. Geoth. Res., 286, 148–182,
https://doi.org/10.1016/j.jvolgeores.2014.08.030, 2014. a
Zhou, H., Gómez-Hernández, J. J., Hendricks Franssen, H.-J., and Li, L.: An
approach to handling non-Gaussianity of parameters and state variables in
ensemble Kalman filtering, Adv. Water Res., 34, 844–864,
https://doi.org/10.1016/j.advwatres.2011.04.014, 2011. a
Zidikheri, M. J. and Lucas, C.: Using Satellite Data to Determine Empirical
Relationships between Volcanic Ash Source Parameters, Atmosphere, 11, 342,
https://doi.org/10.3390/atmos11040342, 2020. a
Zidikheri, M. J. and Lucas, C.: A Computationally Efficient Ensemble Filtering
Scheme for Quantitative Volcanic Ash Forecasts, J. Geophys. Res.-Atmos., 126,
e2020JD033094, https://doi.org/10.1029/2020JD033094, 2021a. a, b
Zidikheri, M. J. and Lucas, C.: Improving Ensemble Volcanic Ash Forecasts by
Direct Insertion of Satellite Data and Ensemble Filtering, Atmosphere, 12,
https://doi.org/10.3390/atmos12091215, 2021b. a
Short summary
We present a new implementation of an ensemble-based data assimilation method to improve forecasting of volcanic aerosols. This system can be efficiently integrated into operational workflows by exploiting high-performance computing resources. We found a dramatic improvement of forecast quality when satellite retrievals are continuously assimilated. Management of volcanic risk and reduction of aviation impacts can strongly benefit from this research.
We present a new implementation of an ensemble-based data assimilation method to improve...
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