Articles | Volume 21, issue 9
https://doi.org/10.5194/acp-21-6799-2021
https://doi.org/10.5194/acp-21-6799-2021
Research article
 | 
05 May 2021
Research article |  | 05 May 2021

Impact of regional Northern Hemisphere mid-latitude anthropogenic sulfur dioxide emissions on local and remote tropospheric oxidants

Daniel M. Westervelt, Arlene M. Fiore, Colleen B. Baublitz, and Gustavo Correa

Related authors

Interactions between atmospheric composition and climate change – progress in understanding and future opportunities from AerChemMIP, PDRMIP, and RFMIP
Stephanie Fiedler, Vaishali Naik, Fiona M. O'Connor, Christopher J. Smith, Paul Griffiths, Ryan J. Kramer, Toshihiko Takemura, Robert J. Allen, Ulas Im, Matthew Kasoar, Angshuman Modak, Steven Turnock, Apostolos Voulgarakis, Duncan Watson-Parris, Daniel M. Westervelt, Laura J. Wilcox, Alcide Zhao, William J. Collins, Michael Schulz, Gunnar Myhre, and Piers M. Forster
Geosci. Model Dev., 17, 2387–2417, https://doi.org/10.5194/gmd-17-2387-2024,https://doi.org/10.5194/gmd-17-2387-2024, 2024
Short summary
The Regional Aerosol Model Intercomparison Project (RAMIP)
Laura J. Wilcox, Robert J. Allen, Bjørn H. Samset, Massimo A. Bollasina, Paul T. Griffiths, James Keeble, Marianne T. Lund, Risto Makkonen, Joonas Merikanto, Declan O'Donnell, David J. Paynter, Geeta G. Persad, Steven T. Rumbold, Toshihiko Takemura, Kostas Tsigaridis, Sabine Undorf, and Daniel M. Westervelt
Geosci. Model Dev., 16, 4451–4479, https://doi.org/10.5194/gmd-16-4451-2023,https://doi.org/10.5194/gmd-16-4451-2023, 2023
Short summary
AMORE-Isoprene v1.0: a new reduced mechanism for gas-phase isoprene oxidation
Forwood Wiser, Bryan K. Place, Siddhartha Sen, Havala O. T. Pye, Benjamin Yang, Daniel M. Westervelt, Daven K. Henze, Arlene M. Fiore, and V. Faye McNeill
Geosci. Model Dev., 16, 1801–1821, https://doi.org/10.5194/gmd-16-1801-2023,https://doi.org/10.5194/gmd-16-1801-2023, 2023
Short summary
Observations of particle number size distributions and new particle formation in six Indian locations
Mathew Sebastian, Sobhan Kumar Kompalli, Vasudevan Anil Kumar, Sandhya Jose, S. Suresh Babu, Govindan Pandithurai, Sachchidanand Singh, Rakesh K. Hooda, Vijay K. Soni, Jeffrey R. Pierce, Ville Vakkari, Eija Asmi, Daniel M. Westervelt, Antti-Pekka Hyvärinen, and Vijay P. Kanawade
Atmos. Chem. Phys., 22, 4491–4508, https://doi.org/10.5194/acp-22-4491-2022,https://doi.org/10.5194/acp-22-4491-2022, 2022
Short summary
Climate and air quality impacts due to mitigation of non-methane near-term climate forcers
Robert J. Allen, Steven Turnock, Pierre Nabat, David Neubauer, Ulrike Lohmann, Dirk Olivié, Naga Oshima, Martine Michou, Tongwen Wu, Jie Zhang, Toshihiko Takemura, Michael Schulz, Kostas Tsigaridis, Susanne E. Bauer, Louisa Emmons, Larry Horowitz, Vaishali Naik, Twan van Noije, Tommi Bergman, Jean-Francois Lamarque, Prodromos Zanis, Ina Tegen, Daniel M. Westervelt, Philippe Le Sager, Peter Good, Sungbo Shim, Fiona O'Connor, Dimitris Akritidis, Aristeidis K. Georgoulias, Makoto Deushi, Lori T. Sentman, Jasmin G. John, Shinichiro Fujimori, and William J. Collins
Atmos. Chem. Phys., 20, 9641–9663, https://doi.org/10.5194/acp-20-9641-2020,https://doi.org/10.5194/acp-20-9641-2020, 2020

Related subject area

Subject: Gases | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
MIXv2: a long-term mosaic emission inventory for Asia (2010–2017)
Meng Li, Junichi Kurokawa, Qiang Zhang, Jung-Hun Woo, Tazuko Morikawa, Satoru Chatani, Zifeng Lu, Yu Song, Guannan Geng, Hanwen Hu, Jinseok Kim, Owen R. Cooper, and Brian C. McDonald
Atmos. Chem. Phys., 24, 3925–3952, https://doi.org/10.5194/acp-24-3925-2024,https://doi.org/10.5194/acp-24-3925-2024, 2024
Short summary
Organosulfate produced from consumption of SO3 speeds up sulfuric acid–dimethylamine atmospheric nucleation
Xiaomeng Zhang, Yongjian Lian, Shendong Tan, and Shi Yin
Atmos. Chem. Phys., 24, 3593–3612, https://doi.org/10.5194/acp-24-3593-2024,https://doi.org/10.5194/acp-24-3593-2024, 2024
Short summary
Contribution of expanded marine sulfur chemistry to the seasonal variability of dimethyl sulfide oxidation products and size-resolved sulfate aerosol
Linia Tashmim, William C. Porter, Qianjie Chen, Becky Alexander, Charles H. Fite, Christopher D. Holmes, Jeffrey R. Pierce, Betty Croft, and Sakiko Ishino
Atmos. Chem. Phys., 24, 3379–3403, https://doi.org/10.5194/acp-24-3379-2024,https://doi.org/10.5194/acp-24-3379-2024, 2024
Short summary
Spatial disparities of ozone pollution in the Sichuan Basin spurred by extreme, hot weather
Nan Wang, Yunsong Du, Dongyang Chen, Haiyan Meng, Xi Chen, Li Zhou, Guangming Shi, Yu Zhan, Miao Feng, Wei Li, Mulan Chen, Zhenliang Li, and Fumo Yang
Atmos. Chem. Phys., 24, 3029–3042, https://doi.org/10.5194/acp-24-3029-2024,https://doi.org/10.5194/acp-24-3029-2024, 2024
Short summary
Global impacts of aviation on air quality evaluated at high resolution
Sebastian D. Eastham, Guillaume P. Chossière, Raymond L. Speth, Daniel J. Jacob, and Steven R. H. Barrett
Atmos. Chem. Phys., 24, 2687–2703, https://doi.org/10.5194/acp-24-2687-2024,https://doi.org/10.5194/acp-24-2687-2024, 2024
Short summary

Cited articles

Abbatt, J. P. D., Lee, A. K. Y., and Thornton, J. A.: Quantifying trace gas uptake to tropospheric aerosol: Recent advances and remaining challenges, Chem. Soc. Rev., 41, 6555–6581, https://doi.org/10.1039/c2cs35052a, 2012. 
Bian, H. and Zender, C. S.: Mineral dust and global tropospheric chemistry: Relative roles of photolysis and heterogeneous uptake, J. Geophys. Res.-Atmos., 108, D21, https://doi.org/10.1029/2002jd003143, 2003. 
Bian, H., Prather, M. J. and Takemura, T.: Tropospheric aerosol impacts on trace gas budgets through photolysis, J. Geophys. Res.-Atmos., 108, D8, https://doi.org/10.1029/2002jd002743, 2003. 
Chang, W. L., Bhave, P. V, Brown, S. S., Riemer, N., Stutz, J. and Dabdub, D.: Heterogeneous Atmospheric Chemistry, Ambient Measurements, and Model Calculations of N2O5: A Review, Aerosol Sci. Technol., 45, 665–695, https://doi.org/10.1080/02786826.2010.551672, 2011. 
Dentener, F. J. and Crutzen, P. J.: Reaction of N2O5 on tropospheric aerosols: impact on the global distributions of NOx, O3, and OH, J. Geophys. Res., 98, 7149–7163, https://doi.org/10.1029/92JD02979, 1993. 
Download
Short summary
Particulate air pollution in the atmosphere can impact the availability of gas-phase chemical constituents, which can then have feedbacks on gas-phase air pollutants. We use a chemistry–climate computer model to simulate the impact of particulate pollution from three major world regions on gas-phase chemical constituents. We find that surface-level ozone air pollution decreases by up to 5 ppbv over China in response to Chinese particulate air pollution, which has implications for policy.
Altmetrics
Final-revised paper
Preprint