Articles | Volume 21, issue 23
https://doi.org/10.5194/acp-21-17855-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-17855-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Potential new tracers and their mass fraction in the emitted PM10 from the burning of household waste in stoves
András Hoffer
CORRESPONDING AUTHOR
MTA-PE Air Chemistry Research Group, 8200, Veszprém, Hungary
Ádám Tóth
Air Chemistry Research Group, University of Pannonia, 8200,
Veszprém, Hungary
Beatrix Jancsek-Turóczi
Air Chemistry Research Group, University of Pannonia, 8200,
Veszprém, Hungary
Attila Machon
Hungarian Meteorological Service, 1181, Budapest, Hungary
Aida Meiramova
Air Chemistry Research Group, University of Pannonia, 8200,
Veszprém, Hungary
Attila Nagy
Wigner Research Centre for Physics, 1121, Budapest, Hungary
Luminita Marmureanu
Remote Sensing Department, National Institute of R&D for
Optoelectronics, 409 Atomistilor Str., Măgurele, Ilfov, Romania
András Gelencsér
MTA-PE Air Chemistry Research Group, 8200, Veszprém, Hungary
Air Chemistry Research Group, University of Pannonia, 8200,
Veszprém, Hungary
Related authors
Aino Ovaska, Daniel Holmberg, Elio Rauth, Mansour Alghamdi, Paulo Artaxo, Eija Asmi, John Backman, Benjamin Bergmans, Matthew Boyer, Liezl Bredenkamp, Maurizio Busetto, Delano Campos De Oliveira, Juan Andrés Casquero-Vera, Darius Ceburnis, Tak Chan, Tommy Chan, Sebastien Conil, Daniele Contini, Suzanne Crumeyrolle, Valentin Duflot, Kostas Eleftheriadis, Johan Esveld, Ekaterina Ezhova, Markus Fiebig, Shahzad Gani, Olga Garmash, Francisco Gómez-Moreno, Roy M. Harrison, Andras Hoffer, Rakesh Hooda, Antti Hyvärinen, Tareq Hussein, Jorma Joutsensaari, Nikos Kalivitis, Heinz Kaminski, Jutta Kesti, Radovan Krejci, Adam Kristensson, Chongai Kuang, Markku Kulmala, Lauri Laakso, Ari Leskinen, Heikki Lihavainen, Andreas Massling, Maik Merkel, Steffen Noe, Jakub Ondracek, Noemí Perez, Jean-Eudes Petit, Tuukka Petäjä, Michael Pikridas, Christopher Pöhlker, Mira Pöhlker, Jean-Philippe Putaud, Ximeng Qi, Cristina Reche, Sergio Rodríguez, Petr Roztocil, Jean Sciare, Karine Sellegri, Dongjie Shang, Ashish Singh, Mikko Sipilä, Henrik Skov, Mar Sorribas, Tamanna Subba, Junying Sun, Peter Tunved, Ville Vakkari, Pieter G. Van Zyl, Aki Virkkula, Jens Voigtländer, Kay Weinhold, Alfred Wiedensohler, Hee-Jung Yoo, Putian Zhou, Kai Puolamäki, Tuomo Nieminen, Veli-Matti Kerminen, Victoria A. Sinclair, and Pauli Paasonen
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2026-415, https://doi.org/10.5194/essd-2026-415, 2026
Preprint under review for ESSD
Short summary
Short summary
All clouds form around aerosol particles, and their abundance influences cloud properties. In turn, clouds affect climate by changing how energy moves through the atmosphere, making them important for climate change. To better understand these interactions, we need accurate information on how many aerosol particles are in the atmosphere. Therefore, we have developed a new 21-year global dataset of particle concentrations relevant for cloud formation.
András Hoffer, Aida Meiramova, Ádám Tóth, Beatrix Jancsek-Turóczi, Gyula Kiss, Ágnes Rostási, Erika Andrea Levei, Luminita Marmureanu, Attila Machon, and András Gelencsér
Atmos. Chem. Phys., 24, 1659–1671, https://doi.org/10.5194/acp-24-1659-2024, https://doi.org/10.5194/acp-24-1659-2024, 2024
Short summary
Short summary
Specific tracer compounds identified previously in controlled test burnings of different waste types in the laboratory were detected and quantified in ambient PM10 samples collected in five Hungarian and four Romanian settlements. Back-of-the-envelope calculations based on the relative emission factors of individual tracers suggested that the contribution of solid waste burning particulate emissions to ambient PM10 mass concentrations may be as high as a few percent.
Aino Ovaska, Daniel Holmberg, Elio Rauth, Mansour Alghamdi, Paulo Artaxo, Eija Asmi, John Backman, Benjamin Bergmans, Matthew Boyer, Liezl Bredenkamp, Maurizio Busetto, Delano Campos De Oliveira, Juan Andrés Casquero-Vera, Darius Ceburnis, Tak Chan, Tommy Chan, Sebastien Conil, Daniele Contini, Suzanne Crumeyrolle, Valentin Duflot, Kostas Eleftheriadis, Johan Esveld, Ekaterina Ezhova, Markus Fiebig, Shahzad Gani, Olga Garmash, Francisco Gómez-Moreno, Roy M. Harrison, Andras Hoffer, Rakesh Hooda, Antti Hyvärinen, Tareq Hussein, Jorma Joutsensaari, Nikos Kalivitis, Heinz Kaminski, Jutta Kesti, Radovan Krejci, Adam Kristensson, Chongai Kuang, Markku Kulmala, Lauri Laakso, Ari Leskinen, Heikki Lihavainen, Andreas Massling, Maik Merkel, Steffen Noe, Jakub Ondracek, Noemí Perez, Jean-Eudes Petit, Tuukka Petäjä, Michael Pikridas, Christopher Pöhlker, Mira Pöhlker, Jean-Philippe Putaud, Ximeng Qi, Cristina Reche, Sergio Rodríguez, Petr Roztocil, Jean Sciare, Karine Sellegri, Dongjie Shang, Ashish Singh, Mikko Sipilä, Henrik Skov, Mar Sorribas, Tamanna Subba, Junying Sun, Peter Tunved, Ville Vakkari, Pieter G. Van Zyl, Aki Virkkula, Jens Voigtländer, Kay Weinhold, Alfred Wiedensohler, Hee-Jung Yoo, Putian Zhou, Kai Puolamäki, Tuomo Nieminen, Veli-Matti Kerminen, Victoria A. Sinclair, and Pauli Paasonen
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2026-415, https://doi.org/10.5194/essd-2026-415, 2026
Preprint under review for ESSD
Short summary
Short summary
All clouds form around aerosol particles, and their abundance influences cloud properties. In turn, clouds affect climate by changing how energy moves through the atmosphere, making them important for climate change. To better understand these interactions, we need accurate information on how many aerosol particles are in the atmosphere. Therefore, we have developed a new 21-year global dataset of particle concentrations relevant for cloud formation.
András Hoffer, Aida Meiramova, Ádám Tóth, Beatrix Jancsek-Turóczi, Gyula Kiss, Ágnes Rostási, Erika Andrea Levei, Luminita Marmureanu, Attila Machon, and András Gelencsér
Atmos. Chem. Phys., 24, 1659–1671, https://doi.org/10.5194/acp-24-1659-2024, https://doi.org/10.5194/acp-24-1659-2024, 2024
Short summary
Short summary
Specific tracer compounds identified previously in controlled test burnings of different waste types in the laboratory were detected and quantified in ambient PM10 samples collected in five Hungarian and four Romanian settlements. Back-of-the-envelope calculations based on the relative emission factors of individual tracers suggested that the contribution of solid waste burning particulate emissions to ambient PM10 mass concentrations may be as high as a few percent.
Cited articles
Al-Naiema, I. M. and Stone, E. A.: Evaluation of anthropogenic secondary organic aerosol tracers from aromatic hydrocarbons, Atmos. Chem. Phys., 17, 2053–2065, https://doi.org/10.5194/acp-17-2053-2017, 2017.
Bajpai, P.: Pulp and paper industry: Chemicals, Elsevier, https://doi.org/10.1016/C2014-0-02795-5, 2015.
Fabbri, D., Torri, C., Simonei, B. R. T., Marynowski, L., Rushdi, A. I., and
Fabianska, M. J.: Levoglucosan and other cellulose and lignin markers in
emissions from burning of Miocene lignites, Atmos. Environ., 43,
2286–2295, https://doi.org/10.1016/j.atmosenv.2009.01.030, 2009.
Ferre-Huguet, N., Nadal, M., Schuhmacher, M., and Domingo, J. L.:
Environmental impact and human health risks of polychlorinated
dibenzo-p-dioxins and dibenzofurans in the vicinity of a new hazardous waste
incinerator: A case study, Environ. Sci. Technol., 40, 61–66, https://doi.org/10.1021/es051630+, 2006.
Fiedler, H.: Sources of PCDD/PCDF and impact on the environment,
Chemosphere, 32, 55–64, https://doi.org/10.1016/0045-6535(95)00228-6, 1996.
Fine, P. M., Chakrabarti, B., Krudysz, M., Schauer, J. J., and Sioutas, C.:
Diurnal variations of individual organic compound constituents of ultrafine
and accumulation mode particulate matter in the Los Angeles basin,
Environ. Sci. Technol., 38, 1296–1304, https://doi.org/10.1021/es0348389,
2004.
Fraser, M. P., Cass, G. R., and Simoneit, B. R. T.: Air quality model
evaluation data for organics. 6. C3–C24 organic acids, Environ.
Sci. Technol., 37, 446–453, https://doi.org/10.1021/es0209262, 2003.
Fu, P. Q. and Kawamura, K.: Ubiquity of bisphenol A in the atmosphere,
Environ. Pollut., 158, 3138–3143, https://doi.org/10.1016/j.envpol.2010.06.040, 2010.
Giri, B., Patel, K. S., Jaiswal, N. K., Sharma, S., Ambade, B., Wang, W. T.,
Simonich, S. L. M., and Simoneit, B. R. T.: Composition and sources of
organic tracers in aerosol particles of industrial central India,
Atmos. Res., 120, 312–324, https://doi.org/10.1016/j.atmosres.2012.09.016, 2013.
Gu, Z. P., Feng, J. L., Han, W. L., Wu, M. H., Fu, J. M., and Sheng, G. Y.:
Characteristics of organic matter in PM2.5 from an e-waste dismantling area
in Taizhou, China, Chemosphere, 80, 800–806, https://doi.org/10.1016/j.chemosphere.2010.04.078, 2010.
Guillen, M. D., Sopelana, P., and Partearroyo, M. A.: Polycyclic aromatic
hydrocarbons in liquid smoke flavorings obtained from different types of
wood. Effect of storage in polyethylene flasks on their concentrations,
J. Agr. Food Chem., 48, 5083–5087, https://doi.org/10.1021/jf000371z, 2000.
Hagiopol, C. and Johnston, J. W.: Chemistry of modern papermaking. CRC Press,
Taylor & Francis Group, https://doi.org/10.1201/b11011, 2012.
He, X., Huang, X. H. H., Chow, K. S., Wang, Q. Q., Zhang, T., Wu, D., and
Yu, J. Z.: Abundance and Sources of Phthalic Acids, Benzene-Tricarboxylic
Acids, and Phenolic Acids in PM2.5 at Urban and Suburban Sites in Southern
China, Acs Earth and Space Chemistry, 2, 147–158, https://doi.org/10.1021/acsearthspacechem.7b00131, 2018.
Hermabessiere, L., Receveur, J., Himber, C., Mazurais, D., Huvet, A.,
Lagarde, F., Lambert, C., Paul-Pont, I., Dehaut, A., Jezequel, R., Soudant,
P., and Duflos, G.: An Irgafos® 168 story: When the ubiquity of an
additive prevents studying its leaching from plastics, Sci. Total
Environ., 749, 141651, https://doi.org/10.1016/j.scitotenv.2020.141651, 2020.
Hoffer, A., Jancsek-Turóczi, B., Tóth, Á., Kiss, G., Naghiu, A., Levei, E. A., Marmureanu, L., Machon, A., and Gelencsér, A.: Emission factors for PM10 and polycyclic aromatic hydrocarbons (PAHs) from illegal burning of different types of municipal waste in households, Atmos. Chem. Phys., 20, 16135–16144, https://doi.org/10.5194/acp-20-16135-2020, 2020.
Hoornweg, D. and Bhada-Tata, P.: What a Waste: A Global Review of Solid Waste
Management, Urban development series;knowledge papers no. 15, World Bank,
Washington, DC, © World Bank, available at:
https://openknowledge.worldbank.org/handle/10986/17388 (last access: 18 November 2021), License: CC BY 3.0
IGO, 2012.
Jayarathne, T., Stockwell, C. E., Bhave, P. V., Praveen, P. S., Rathnayake, C. M., Islam, Md. R., Panday, A. K., Adhikari, S., Maharjan, R., Goetz, J. D., DeCarlo, P. F., Saikawa, E., Yokelson, R. J., and Stone, E. A.: Nepal Ambient Monitoring and Source Testing Experiment (NAMaSTE): emissions of particulate matter from wood- and dung-fueled cooking fires, garbage and crop residue burning, brick kilns, and other sources, Atmos. Chem. Phys., 18, 2259–2286, https://doi.org/10.5194/acp-18-2259-2018, 2018.
Keyte, I. J., Albinet, A., and Harrison, R. M.: On-road traffic emissions of
polycyclic aromatic hydrocarbons and their oxy- and nitro-derivative
compounds measured in road tunnel environments, Sci. Total
Environ., 566, 1131–1142, https://doi.org/10.1016/j.scitotenv.2016.05.152, 2016.
Kumar, S., Aggarwal, S. G., Gupta, P. K., and Kawamura, K.: Investigation of
the tracers for plastic-enriched waste burning aerosols, Atmos.
Environ., 108, 49–58, https://doi.org/10.1016/j.atmosenv.2015.02.066, 2015.
Lavric, E. D., Konnov, A. A., and De Ruyck, J.: Dioxin levels in wood
combustion – a review, Biomass Bioenerg., 26, 115–145, https://doi.org/10.1016/s0961-9534(03)00104-1, 2004.
Lee, H., Wang, L., and Shih, J. F.: Mutagenicity of particulates from the
laboratory combustion of plastics, Mutat. Res. Lett., 346, 135–144, https://doi.org/10.1016/0165-7992(95)90045-4, 1995.
Liu, R. Z. and Mabury, S. A.: Unexpectedly High Concentrations of a Newly
Identified Organophosphate Ester, Tris(2,4-di-tert-butylphenyl) Phosphate,
in Indoor Dust from Canada, Environ. Sci. Technol., 52,
9677–9683, https://doi.org/10.1021/acs.est.8b03061, 2018.
Manisalidis, I., Stavropoulou, E., Stavropoulos, A., and Bezirtzoglou, E.:
Environmental and Health Impacts of Air Pollution: A Review, Frontiers in
Public Health, 8, 14, https://doi.org/10.3389/fpubh.2020.00014, 2020.
Ni, Y. W., Zhang, H. J., Fan, S., Zhang, X. P., Zhang, Q., and Chen, J. P.:
Emissions of PCDD/Fs from municipal solid waste incinerators in China,
Chemosphere, 75, 1153–1158, https://doi.org/10.1016/j.chemosphere.2009.02.051, 2009.
Reuters 2021: Crime networks suspected of burning tech waste for scrap metal in Romania, available at: https://www.reuters.com/business/environment/crime-networks-suspected-burning-tech-waste-scrap-metal-romania-2021-04-16/, last access: 21 June 2021.
Romania Insider 2020: Minister: Waste illegally brought from the UK to Romania could cause the high pollution in Bucharest, available at:
https://www.romania-insider.com/romania-waste-uk-pollution-bucharest, last
access: 21 June 2021.
Simoneit, B. R. T.: Biomass burning – A review of organic tracers for smoke
from incomplete combustion, Appl. Geochem., 17, 129–162,
https://doi.org/10.1016/S0883-2927(01)00061-0, 2002.
Simoneit, B. R. T., Medeiros, P. M., and Didyk, B. M.: Combustion products
of plastics as indicators for refuse burning in the atmosphere,
Environ. Sci. Technol., 39, 6961–6970, https://doi.org/10.1021/es050767x,
2005.
Simoneit, B. R. T.: Triphenylbenzene in Urban Atmospheres, a New PAH Source
Tracer, Polycycl. Aromat. Comp., 35, 3–15, https://doi.org/10.1080/10406638.2014.883417, 2015.
Tomsej, T., Horak, J., Tomsejova, S., Krpec, K., Klanova, J., Dej, M., and
Hopan, F.: The impact of co-combustion of polyethylene plastics and wood in
a small residential boiler on emissions of gaseous pollutants, particulate
matter, PAHs and 1,3,5-triphenylbenzene, Chemosphere, 196, 18–24, https://doi.org/10.1016/j.chemosphere.2017.12.127, 2018.
Tsuge, S., Ohtani, H., and Watanabe, C.: Pyrolysis-GC/MS data book of
synthetic polymers: pyrograms, thermograms and MS of pyrolyzates, Elsevier,
available at: https://www.elsevier.com/books/pyrolysis-gc-ms-data-book-of-synthetic-polymers/tsuge/978-0-444-53892-5 (last access: 22 November 2021), 2011.
Wiedinmyer, C., Yokelson, R. J., and Gullett, B. K.: Global Emissions of
Trace Gases, Particulate Matter, and Hazardous Air Pollutants from Open
Burning of Domestic Waste, Environ. Sci. Technol., 48,
9523–9530, https://doi.org/10.1021/es502250z, 2014.
Zaman, A. U.: A comprehensive study
of the environmental and economic benefits of resource recovery from global
waste management systems, J. Clean. Prod., 124, 41-50, https://doi.org/10.1016/j.jclepro.2016.02.086, 2016.
Short summary
Due to the widespread use of plastics high amounts of waste are burned in households worldwide, emitting vast amounts of PM10 and PAHs into the atmosphere. In this work different types of common plastics were burned in the laboratory with a view to identifying potentially specific tracer compounds and determining their emission factors. The compounds found were also successfully identified in atmospheric PM10 samples, indicating their potential use as ambient tracers for illegal waste burning.
Due to the widespread use of plastics high amounts of waste are burned in households worldwide,...
Altmetrics
Final-revised paper
Preprint