Articles | Volume 20, issue 22
https://doi.org/10.5194/acp-20-13957-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-13957-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
19 Nov 2020
Research article |
| 19 Nov 2020
| 19 Nov 2020
The effects of morphology, mobility size, and secondary organic aerosol (SOA) material coating on the ice nucleation activity of black carbon in the cirrus regime
Cuiqi Zhang
School of Energy and Power Engineering, Beihang University, Beijing, China
Department of Earth, Atmospheric, and Planetary Sciences,
Massachusetts Institute of Technology, Cambridge, MA, 02139, USA
Yue Zhang
Department of Environmental Sciences and Engineering, University of
North Carolina at Chapel Hill, Chapel Hill, NC, 27599, USA
Aerodyne Research Incorporated, Billerica, MA, 01821, USA
Department of Chemistry, Boston College, Chestnut Hill, MA, 02467,
USA
now at: Department of Atmospheric Sciences, Texas A&M University, College Station, 77843, TX, USA
Martin J. Wolf
Department of Earth, Atmospheric, and Planetary Sciences,
Massachusetts Institute of Technology, Cambridge, MA, 02139, USA
now at: Yale Center for Environmental Law and Policy, Yale Law School and Yale School of the Environment, New Haven, CT, 06511, USA
Leonid Nichman
Flight Research Laboratory, National Research Council Canada, Ottawa, ON, K1V 9B4, Canada
Chuanyang Shen
Department of Earth, Atmospheric, and Planetary Sciences,
Massachusetts Institute of Technology, Cambridge, MA, 02139, USA
Department of Atmospheric and Oceanic Sciences, School of Physics, Peking University, Beijing, China
Timothy B. Onasch
Aerodyne Research Incorporated, Billerica, MA, 01821, USA
Department of Chemistry, Boston College, Chestnut Hill, MA, 02467,
USA
Longfei Chen
CORRESPONDING AUTHOR
School of Energy and Power Engineering, Beihang University, Beijing, China
Daniel J. Cziczo
Department of Earth, Atmospheric, and Planetary Sciences,
Massachusetts Institute of Technology, Cambridge, MA, 02139, USA
Department of Civil and Environmental Engineering, Massachusetts
Institute of Technology, Cambridge, MA, 02139, USA
Department of Earth, Atmospheric, and Planetary Sciences, Purdue
University, West Lafayette, IN, 47907, USA
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Julia Perim de Faria, Ulrich Bundke, Andrew Freedman, Timothy B. Onasch, and Andreas Petzold
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Weilun Zhao, Wangshu Tan, Gang Zhao, Chuanyang Shen, Yingli Yu, and Chunsheng Zhao
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Chuanyang Shen, Gang Zhao, and Chunsheng Zhao
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Chuanyang Shen, Gang Zhao, Weilun Zhao, Ping Tian, and Chunsheng Zhao
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Michael Rösch and Daniel J. Cziczo
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Martin J. Wolf, Megan Goodell, Eric Dong, Lilian A. Dove, Cuiqi Zhang, Lesly J. Franco, Chuanyang Shen, Emma G. Rutkowski, Domenic N. Narducci, Susan Mullen, Andrew R. Babbin, and Daniel J. Cziczo
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Gourihar Kulkarni, Naruki Hiranuma, Ottmar Möhler, Kristina Höhler, Swarup China, Daniel J. Cziczo, and Paul J. DeMott
Atmos. Meas. Tech., 13, 6631–6643, https://doi.org/10.5194/amt-13-6631-2020, https://doi.org/10.5194/amt-13-6631-2020, 2020
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This study presents a new continuous-flow-diffusion-chamber-style operated ice chamber (Modified Compact Ice Chamber, MCIC) to measure the immersion-freezing efficiency of atmospheric particles. MCIC allowed us to obtain maximum droplet-freezing efficiency at higher time resolution without droplet breakthrough ambiguity. Its evaluation was performed by reproducing published data from the recent ice nucleation workshop and past laboratory data for standard and airborne ice-nucleating particles.
Lawrence I. Kleinman, Arthur J. Sedlacek III, Kouji Adachi, Peter R. Buseck, Sonya Collier, Manvendra K. Dubey, Anna L. Hodshire, Ernie Lewis, Timothy B. Onasch, Jeffery R. Pierce, John Shilling, Stephen R. Springston, Jian Wang, Qi Zhang, Shan Zhou, and Robert J. Yokelson
Atmos. Chem. Phys., 20, 13319–13341, https://doi.org/10.5194/acp-20-13319-2020, https://doi.org/10.5194/acp-20-13319-2020, 2020
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Aerosols from wildfires affect the Earth's temperature by absorbing light or reflecting it back into space. This study investigates time-dependent chemical, microphysical, and optical properties of aerosols generated by wildfires in the Pacific Northwest, USA. Wildfire smoke plumes were traversed by an instrumented aircraft at locations near the fire and up to 3.5 h travel time downwind. Although there was no net aerosol production, aerosol particles grew and became more efficient scatters.
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Short summary
Black carbon (BC) is considered the second most important global warming agent. However, the role of BC aerosol–cloud–climate interactions in the cirrus formation remains uncertain. Our study of selected BC types and sizes suggests that increases in diameter, compactness, and/or surface oxidation of BC particles lead to more efficient ice nucleation (IN) via pore condensation freezing (PCF) pathways，and that coatings of common secondary organic aerosol (SOA) materials can inhibit ice formation.
Black carbon (BC) is considered the second most important global warming agent. However, the...
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