Articles | Volume 20, issue 22
https://doi.org/10.5194/acp-20-13957-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-13957-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
19 Nov 2020
Research article |
| 19 Nov 2020
| 19 Nov 2020
The effects of morphology, mobility size, and secondary organic aerosol (SOA) material coating on the ice nucleation activity of black carbon in the cirrus regime
Cuiqi Zhang
School of Energy and Power Engineering, Beihang University, Beijing, China
Department of Earth, Atmospheric, and Planetary Sciences,
Massachusetts Institute of Technology, Cambridge, MA, 02139, USA
Yue Zhang
Department of Environmental Sciences and Engineering, University of
North Carolina at Chapel Hill, Chapel Hill, NC, 27599, USA
Aerodyne Research Incorporated, Billerica, MA, 01821, USA
Department of Chemistry, Boston College, Chestnut Hill, MA, 02467,
USA
now at: Department of Atmospheric Sciences, Texas A&M University, College Station, 77843, TX, USA
Martin J. Wolf
Department of Earth, Atmospheric, and Planetary Sciences,
Massachusetts Institute of Technology, Cambridge, MA, 02139, USA
now at: Yale Center for Environmental Law and Policy, Yale Law School and Yale School of the Environment, New Haven, CT, 06511, USA
Leonid Nichman
Flight Research Laboratory, National Research Council Canada, Ottawa, ON, K1V 9B4, Canada
Chuanyang Shen
Department of Earth, Atmospheric, and Planetary Sciences,
Massachusetts Institute of Technology, Cambridge, MA, 02139, USA
Department of Atmospheric and Oceanic Sciences, School of Physics, Peking University, Beijing, China
Timothy B. Onasch
Aerodyne Research Incorporated, Billerica, MA, 01821, USA
Department of Chemistry, Boston College, Chestnut Hill, MA, 02467,
USA
Longfei Chen
CORRESPONDING AUTHOR
School of Energy and Power Engineering, Beihang University, Beijing, China
Daniel J. Cziczo
Department of Earth, Atmospheric, and Planetary Sciences,
Massachusetts Institute of Technology, Cambridge, MA, 02139, USA
Department of Civil and Environmental Engineering, Massachusetts
Institute of Technology, Cambridge, MA, 02139, USA
Department of Earth, Atmospheric, and Planetary Sciences, Purdue
University, West Lafayette, IN, 47907, USA
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- Snow particles physiochemistry: feedback on air quality, climate change, and human health R. Rangel-Alvarado et al. 10.1039/D2EA00067A
- Effect of Methyl Butyrate blending on soot formation in Jet A laminar diffusion flame X. He et al. 10.1016/j.fuel.2024.132598
- Ice-nucleating particles from multiple aerosol sources in the urban environment of Beijing under mixed-phase cloud conditions C. Zhang et al. 10.5194/acp-22-7539-2022
- Ice Nucleating Activity and Residual Particle Morphology of Bulk Seawater and Sea Surface Microlayer P. Roy et al. 10.1021/acsearthspacechem.1c00175
- Enhanced Ice Nucleation of Simulated Sea Salt Particles with the Addition of Anthropogenic Per- and Polyfluoroalkyl Substances M. Wolf et al. 10.1021/acsearthspacechem.1c00138
- Synthetic strategies for oxidation products from biogenic volatile organic compounds in the atmosphere: A review S. Gagan et al. 10.1016/j.atmosenv.2023.120017
- Soot PCF: pore condensation and freezing framework for soot aggregates C. Marcolli et al. 10.5194/acp-21-7791-2021
- Heterogeneous Ice Nucleation in Model Crystalline Porous Organic Polymers: Influence of Pore Size on Immersion Freezing L. Nandy et al. 10.1021/acs.jpca.3c00071
- Simulated contrail-processed aviation soot aerosols are poor ice-nucleating particles at cirrus temperatures B. Testa et al. 10.5194/acp-24-10409-2024
- Microfluidic platform for coupled studies of freezing behavior and final effloresced particle morphology in Snomax ® containing aqueous droplets M. House & C. Dutcher 10.1080/02786826.2023.2233574
- Soot aerosols from commercial aviation engines are poor ice-nucleating particles at cirrus cloud temperatures B. Testa et al. 10.5194/acp-24-4537-2024
- Enhanced soot particle ice nucleation ability induced by aggregate compaction and densification K. Gao et al. 10.5194/acp-22-4985-2022
- The dependence of soot particle ice nucleation ability on its volatile content K. Gao et al. 10.1039/D2EM00158F
- The Role of Mineral Dust Aerosol Particles in Aviation Soot‐Cirrus Interactions B. Kärcher et al. 10.1029/2022JD037881
- The effects of photochemical aging and interactions with secondary organic aerosols on cellular toxicity of combustion particles R. Attah et al. 10.1016/j.jaerosci.2024.106473
- Particle emissions from a modern heavy-duty diesel engine as ice nuclei in immersion freezing mode: a laboratory study on fossil and renewable fuels K. Korhonen et al. 10.5194/acp-22-1615-2022
- Physicochemical properties of charcoal aerosols derived from biomass pyrolysis affect their ice-nucleating abilities at cirrus and mixed-phase cloud conditions F. Mahrt et al. 10.5194/acp-23-1285-2023
- Experimental Determination of the Relationship Between Organic Aerosol Viscosity and Ice Nucleation at Upper Free Tropospheric Conditions S. Kasparoglu et al. 10.1029/2021JD036296
- Cloud Activation via Formation of Water and Ice on Various Types of Porous Aerosol Particles E. Jantsch & T. Koop 10.1021/acsearthspacechem.0c00330
- Quantifying the contributions of diesel fuel and lubricating oil to the SVOC emissions from a diesel engine using GC × GC-ToFMS Z. Liang et al. 10.1016/j.fuel.2021.122409
- Impacts of Cloud‐Processing on Ice Nucleation of Soot Particles Internally Mixed With Sulfate and Organics K. Gao & Z. Kanji 10.1029/2022JD037146
- Characteristics of ice-nucleating particles in Beijing during spring: A comparison study of measurements between the suburban and a nearby mountain area Y. Hu et al. 10.1016/j.atmosenv.2022.119451
- Measurements and calculations of enhanced side- and back-scattering of visible radiation by black carbon aggregates C. Haspel et al. 10.5194/acp-23-10091-2023
- The Relationship of Aerosol Properties and Ice‐Nucleating Particle Concentrations in Beijing Y. Ren et al. 10.1029/2022JD037383
- Laboratory studies of ice nucleation onto bare and internally mixed soot–sulfuric acid particles K. Gao et al. 10.5194/acp-22-5331-2022
- Inter-annual variability of ice nucleating particles in Mexico city D. Cabrera-Segoviano et al. 10.1016/j.atmosenv.2022.118964
- Process-oriented analysis of aircraft soot-cirrus interactions constrains the climate impact of aviation B. Kärcher et al. 10.1038/s43247-021-00175-x
26 citations as recorded by crossref.
- Snow particles physiochemistry: feedback on air quality, climate change, and human health R. Rangel-Alvarado et al. 10.1039/D2EA00067A
- Effect of Methyl Butyrate blending on soot formation in Jet A laminar diffusion flame X. He et al. 10.1016/j.fuel.2024.132598
- Ice-nucleating particles from multiple aerosol sources in the urban environment of Beijing under mixed-phase cloud conditions C. Zhang et al. 10.5194/acp-22-7539-2022
- Ice Nucleating Activity and Residual Particle Morphology of Bulk Seawater and Sea Surface Microlayer P. Roy et al. 10.1021/acsearthspacechem.1c00175
- Enhanced Ice Nucleation of Simulated Sea Salt Particles with the Addition of Anthropogenic Per- and Polyfluoroalkyl Substances M. Wolf et al. 10.1021/acsearthspacechem.1c00138
- Synthetic strategies for oxidation products from biogenic volatile organic compounds in the atmosphere: A review S. Gagan et al. 10.1016/j.atmosenv.2023.120017
- Soot PCF: pore condensation and freezing framework for soot aggregates C. Marcolli et al. 10.5194/acp-21-7791-2021
- Heterogeneous Ice Nucleation in Model Crystalline Porous Organic Polymers: Influence of Pore Size on Immersion Freezing L. Nandy et al. 10.1021/acs.jpca.3c00071
- Simulated contrail-processed aviation soot aerosols are poor ice-nucleating particles at cirrus temperatures B. Testa et al. 10.5194/acp-24-10409-2024
- Microfluidic platform for coupled studies of freezing behavior and final effloresced particle morphology in Snomax ® containing aqueous droplets M. House & C. Dutcher 10.1080/02786826.2023.2233574
- Soot aerosols from commercial aviation engines are poor ice-nucleating particles at cirrus cloud temperatures B. Testa et al. 10.5194/acp-24-4537-2024
- Enhanced soot particle ice nucleation ability induced by aggregate compaction and densification K. Gao et al. 10.5194/acp-22-4985-2022
- The dependence of soot particle ice nucleation ability on its volatile content K. Gao et al. 10.1039/D2EM00158F
- The Role of Mineral Dust Aerosol Particles in Aviation Soot‐Cirrus Interactions B. Kärcher et al. 10.1029/2022JD037881
- The effects of photochemical aging and interactions with secondary organic aerosols on cellular toxicity of combustion particles R. Attah et al. 10.1016/j.jaerosci.2024.106473
- Particle emissions from a modern heavy-duty diesel engine as ice nuclei in immersion freezing mode: a laboratory study on fossil and renewable fuels K. Korhonen et al. 10.5194/acp-22-1615-2022
- Physicochemical properties of charcoal aerosols derived from biomass pyrolysis affect their ice-nucleating abilities at cirrus and mixed-phase cloud conditions F. Mahrt et al. 10.5194/acp-23-1285-2023
- Experimental Determination of the Relationship Between Organic Aerosol Viscosity and Ice Nucleation at Upper Free Tropospheric Conditions S. Kasparoglu et al. 10.1029/2021JD036296
- Cloud Activation via Formation of Water and Ice on Various Types of Porous Aerosol Particles E. Jantsch & T. Koop 10.1021/acsearthspacechem.0c00330
- Quantifying the contributions of diesel fuel and lubricating oil to the SVOC emissions from a diesel engine using GC × GC-ToFMS Z. Liang et al. 10.1016/j.fuel.2021.122409
- Impacts of Cloud‐Processing on Ice Nucleation of Soot Particles Internally Mixed With Sulfate and Organics K. Gao & Z. Kanji 10.1029/2022JD037146
- Characteristics of ice-nucleating particles in Beijing during spring: A comparison study of measurements between the suburban and a nearby mountain area Y. Hu et al. 10.1016/j.atmosenv.2022.119451
- Measurements and calculations of enhanced side- and back-scattering of visible radiation by black carbon aggregates C. Haspel et al. 10.5194/acp-23-10091-2023
- The Relationship of Aerosol Properties and Ice‐Nucleating Particle Concentrations in Beijing Y. Ren et al. 10.1029/2022JD037383
- Laboratory studies of ice nucleation onto bare and internally mixed soot–sulfuric acid particles K. Gao et al. 10.5194/acp-22-5331-2022
- Inter-annual variability of ice nucleating particles in Mexico city D. Cabrera-Segoviano et al. 10.1016/j.atmosenv.2022.118964
Latest update: 23 Nov 2024
Short summary
Black carbon (BC) is considered the second most important global warming agent. However, the role of BC aerosol–cloud–climate interactions in the cirrus formation remains uncertain. Our study of selected BC types and sizes suggests that increases in diameter, compactness, and/or surface oxidation of BC particles lead to more efficient ice nucleation (IN) via pore condensation freezing (PCF) pathways，and that coatings of common secondary organic aerosol (SOA) materials can inhibit ice formation.
Black carbon (BC) is considered the second most important global warming agent. However, the...
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