Articles | Volume 18, issue 6
https://doi.org/10.5194/acp-18-4131-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-18-4131-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
26 Mar 2018
Research article |
| 26 Mar 2018
Measurement-based climatology of aerosol direct radiative effect, its sensitivities, and uncertainties from a background southeast US site
James P. Sherman
CORRESPONDING AUTHOR
Department of Physics and Astronomy, Appalachian State University, 525
Rivers Street, Garwood Hall Room 231, Boone, NC 28608, USA
Allison McComiskey
NOAA Earth Systems Research Laboratory, Global Monitoring Division/GMD-1, 325 Broadway, Boulder, CO 80305, USA
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Gloria Titos, María A. Burgos, Paul Zieger, Lucas Alados-Arboledas, Urs Baltensperger, Anne Jefferson, James Sherman, Ernest Weingartner, Bas Henzing, Krista Luoma, Colin O'Dowd, Alfred Wiedensohler, and Elisabeth Andrews
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This paper investigates the impact of water uptake on aerosol optical properties, in particular the aerosol light-scattering coefficient. Although in situ measurements are performed at low relative humidity (typically at
RH < 40 %), to address the climatic impact of aerosol particles it is necessary to take into account the effect that water uptake may have on the aerosol optical properties.
María A. Burgos, Elisabeth Andrews, Gloria Titos, Angela Benedetti, Huisheng Bian, Virginie Buchard, Gabriele Curci, Zak Kipling, Alf Kirkevåg, Harri Kokkola, Anton Laakso, Julie Letertre-Danczak, Marianne T. Lund, Hitoshi Matsui, Gunnar Myhre, Cynthia Randles, Michael Schulz, Twan van Noije, Kai Zhang, Lucas Alados-Arboledas, Urs Baltensperger, Anne Jefferson, James Sherman, Junying Sun, Ernest Weingartner, and Paul Zieger
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We investigate how well models represent the enhancement in scattering coefficients due to particle water uptake, and perform an evaluation of several implementation schemes used in ten Earth system models. Our results show the importance of the parameterization of hygroscopicity and model chemistry as drivers of some of the observed diversity amongst model estimates. The definition of dry conditions and the phenomena taking place in this relative humidity range also impact the model evaluation.
Paolo Laj, Alessandro Bigi, Clémence Rose, Elisabeth Andrews, Cathrine Lund Myhre, Martine Collaud Coen, Yong Lin, Alfred Wiedensohler, Michael Schulz, John A. Ogren, Markus Fiebig, Jonas Gliß, Augustin Mortier, Marco Pandolfi, Tuukka Petäja, Sang-Woo Kim, Wenche Aas, Jean-Philippe Putaud, Olga Mayol-Bracero, Melita Keywood, Lorenzo Labrador, Pasi Aalto, Erik Ahlberg, Lucas Alados Arboledas, Andrés Alastuey, Marcos Andrade, Begoña Artíñano, Stina Ausmeel, Todor Arsov, Eija Asmi, John Backman, Urs Baltensperger, Susanne Bastian, Olaf Bath, Johan Paul Beukes, Benjamin T. Brem, Nicolas Bukowiecki, Sébastien Conil, Cedric Couret, Derek Day, Wan Dayantolis, Anna Degorska, Konstantinos Eleftheriadis, Prodromos Fetfatzis, Olivier Favez, Harald Flentje, Maria I. Gini, Asta Gregorič, Martin Gysel-Beer, A. Gannet Hallar, Jenny Hand, Andras Hoffer, Christoph Hueglin, Rakesh K. Hooda, Antti Hyvärinen, Ivo Kalapov, Nikos Kalivitis, Anne Kasper-Giebl, Jeong Eun Kim, Giorgos Kouvarakis, Irena Kranjc, Radovan Krejci, Markku Kulmala, Casper Labuschagne, Hae-Jung Lee, Heikki Lihavainen, Neng-Huei Lin, Gunter Löschau, Krista Luoma, Angela Marinoni, Sebastiao Martins Dos Santos, Frank Meinhardt, Maik Merkel, Jean-Marc Metzger, Nikolaos Mihalopoulos, Nhat Anh Nguyen, Jakub Ondracek, Noemi Pérez, Maria Rita Perrone, Jean-Eudes Petit, David Picard, Jean-Marc Pichon, Veronique Pont, Natalia Prats, Anthony Prenni, Fabienne Reisen, Salvatore Romano, Karine Sellegri, Sangeeta Sharma, Gerhard Schauer, Patrick Sheridan, James Patrick Sherman, Maik Schütze, Andreas Schwerin, Ralf Sohmer, Mar Sorribas, Martin Steinbacher, Junying Sun, Gloria Titos, Barbara Toczko, Thomas Tuch, Pierre Tulet, Peter Tunved, Ville Vakkari, Fernando Velarde, Patricio Velasquez, Paolo Villani, Sterios Vratolis, Sheng-Hsiang Wang, Kay Weinhold, Rolf Weller, Margarita Yela, Jesus Yus-Diez, Vladimir Zdimal, Paul Zieger, and Nadezda Zikova
Atmos. Meas. Tech., 13, 4353–4392, https://doi.org/10.5194/amt-13-4353-2020, https://doi.org/10.5194/amt-13-4353-2020, 2020
Short summary
Short summary
The paper establishes the fiducial reference of the GAW aerosol network providing the fully characterized value chain to the provision of four climate-relevant aerosol properties from ground-based sites. Data from almost 90 stations worldwide are reported for a reference year, 2017, providing a unique and very robust view of the variability of these variables worldwide. Current gaps in the GAW network are analysed and requirements for the Global Climate Monitoring System are proposed.
Martine Collaud Coen, Elisabeth Andrews, Andrés Alastuey, Todor Petkov Arsov, John Backman, Benjamin T. Brem, Nicolas Bukowiecki, Cédric Couret, Konstantinos Eleftheriadis, Harald Flentje, Markus Fiebig, Martin Gysel-Beer, Jenny L. Hand, András Hoffer, Rakesh Hooda, Christoph Hueglin, Warren Joubert, Melita Keywood, Jeong Eun Kim, Sang-Woo Kim, Casper Labuschagne, Neng-Huei Lin, Yong Lin, Cathrine Lund Myhre, Krista Luoma, Hassan Lyamani, Angela Marinoni, Olga L. Mayol-Bracero, Nikos Mihalopoulos, Marco Pandolfi, Natalia Prats, Anthony J. Prenni, Jean-Philippe Putaud, Ludwig Ries, Fabienne Reisen, Karine Sellegri, Sangeeta Sharma, Patrick Sheridan, James Patrick Sherman, Junying Sun, Gloria Titos, Elvis Torres, Thomas Tuch, Rolf Weller, Alfred Wiedensohler, Paul Zieger, and Paolo Laj
Atmos. Chem. Phys., 20, 8867–8908, https://doi.org/10.5194/acp-20-8867-2020, https://doi.org/10.5194/acp-20-8867-2020, 2020
Short summary
Short summary
Long-term trends of aerosol radiative properties (52 stations) prove that aerosol load has significantly decreased over the last 20 years. Scattering trends are negative in Europe (EU) and North America (NA), not ss in Asia, and show a mix of positive and negative trends at polar stations. Absorption has mainly negative trends. The single scattering albedo has positive trends in Asia and eastern EU and negative in western EU and NA, leading to a global positive median trend of 0.02 % per year.
Fangqun Yu, Gan Luo, Arshad Arjunan Nair, James J. Schwab, James P. Sherman, and Yanda Zhang
Atmos. Chem. Phys., 20, 2591–2601, https://doi.org/10.5194/acp-20-2591-2020, https://doi.org/10.5194/acp-20-2591-2020, 2020
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Particle number concentration (PNC) is a key parameter important for the health and climate impacts of atmospheric aerosols. We show that, even during wintertime, regional nucleation occurs and contributes significantly to number concentrations of ultrafine particles and cloud condensation nuclei. Due to low biogenic emissions, wintertime regional nucleation is solely controlled by inorganic species, and ternary ion-mediated nucleation is able to capture the observed variations in PNC.
Amy Solomon, Gijs de Boer, Jessie M. Creamean, Allison McComiskey, Matthew D. Shupe, Maximilian Maahn, and Christopher Cox
Atmos. Chem. Phys., 18, 17047–17059, https://doi.org/10.5194/acp-18-17047-2018, https://doi.org/10.5194/acp-18-17047-2018, 2018
Short summary
Short summary
The results of this study indicate that perturbations in ice nucleating particles (INPs) dominate over cloud condensation nuclei (CCN) perturbations in Arctic mixed-phase stratocumulus; i.e., an equivalent fractional decrease in CCN and INPs results in an increase in the cloud-top longwave cooling rate, even though the droplet effective radius increases and the cloud emissivity decreases. In addition, cloud-processing causes layering of aerosols with increased concentrations of CCN at cloud top.
Jessie M. Creamean, Maximilian Maahn, Gijs de Boer, Allison McComiskey, Arthur J. Sedlacek, and Yan Feng
Atmos. Chem. Phys., 18, 555–570, https://doi.org/10.5194/acp-18-555-2018, https://doi.org/10.5194/acp-18-555-2018, 2018
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Short summary
We report on airborne observations from the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) program's Fifth Airborne Carbon Measurements (ACME-V) campaign along the North Slope of Alaska during the summer of 2015. We show how local oil extraction activities, 2015's central Alaskan wildfires, and, to a lesser extent, long-range transport introduce aerosols and trace gases higher in concentration than previously reported in Arctic haze measurements to the North Slope.
Lauren Schmeisser, Elisabeth Andrews, John A. Ogren, Patrick Sheridan, Anne Jefferson, Sangeeta Sharma, Jeong Eun Kim, James P. Sherman, Mar Sorribas, Ivo Kalapov, Todor Arsov, Christo Angelov, Olga L. Mayol-Bracero, Casper Labuschagne, Sang-Woo Kim, András Hoffer, Neng-Huei Lin, Hao-Ping Chia, Michael Bergin, Junying Sun, Peng Liu, and Hao Wu
Atmos. Chem. Phys., 17, 12097–12120, https://doi.org/10.5194/acp-17-12097-2017, https://doi.org/10.5194/acp-17-12097-2017, 2017
Short summary
Short summary
Three methods are used to classify aerosol type from aerosol optical properties measured in situ at 24 surface sites. Classification methods work best at sites with stable, homogenous aerosol at particularly polluted and dust-prone continental and marine sites. Classification methods are poor at remote marine and Arctic sites. Using these methods to extrapolate aerosol type from optical properties can help determine aerosol radiative forcing and improve aerosol satellite retrieval algorithms.
Lauren M. Zamora, Ralph A. Kahn, Sabine Eckhardt, Allison McComiskey, Patricia Sawamura, Richard Moore, and Andreas Stohl
Atmos. Chem. Phys., 17, 7311–7332, https://doi.org/10.5194/acp-17-7311-2017, https://doi.org/10.5194/acp-17-7311-2017, 2017
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Short summary
Clouds have a major but uncertain effect on Arctic surface temperatures. Here, we used remote sensing observations to better understand aerosol effects on one type of Arctic cloud. By modifying a variety of cloud properties, aerosols in this type of cloud indirectly reduced the net warming effect of these clouds on the surface by ~ 10 % of the clean-background cloud effect, not including changes in cloud fraction. This work will improve our ability to predict future Arctic surface temperatures.
Elisa T. Sena, Allison McComiskey, and Graham Feingold
Atmos. Chem. Phys., 16, 11301–11318, https://doi.org/10.5194/acp-16-11301-2016, https://doi.org/10.5194/acp-16-11301-2016, 2016
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A new method for assessing aerosol effects on clouds is proposed. For the first time, 14 years of collocated, coincident ground-based observations have been used to study cloud–aerosol–meteorology–radiation interactions in the USA. For this site, the results indicate that the influence of the aerosol on cloud radiative effect and cloud albedo is weak, and that macroscopic cloud properties play a much larger role in determining the cloud radiative effect compared to aerosol effects.
J. P. Sherman, P. J. Sheridan, J. A. Ogren, E. Andrews, D. Hageman, L. Schmeisser, A. Jefferson, and S. Sharma
Atmos. Chem. Phys., 15, 12487–12517, https://doi.org/10.5194/acp-15-12487-2015, https://doi.org/10.5194/acp-15-12487-2015, 2015
Short summary
Short summary
Variability in aerosol optical properties relevant to radiative forcing were studied on several timescales at four continental North American NOAA-ESRL sites. Light scattering and intensive properties varied most on seasonal scales while absorption variability on weekly and diurnal timescales was comparable to its seasonal variability. Large reductions in light scattering were observed at the two long-term sites (relative to late 1990s), along with a smaller contribution by sub-1µm particles.
Related subject area
Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
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Black carbon content of traffic emissions significantly impacts black carbon mass size distributions and mixing states
Impact of desert dust on new particle formation events and cloud condensation nuclei budget in dust-influenced areas
Measurement Report: Wintertime new particle formation in the rural area of the North China Plain – influencing factors and possible formation mechanism
Measurement report: Rapid decline of aerosol absorption coefficient and aerosol optical property effects on radiative forcing in an urban area of Beijing from 2018 to 2021
Aerosol first indirect effect of African smoke at the cloud base of marine cumulus clouds over Ascension Island, southern Atlantic Ocean
Increase in precipitation scavenging contributes to long-term reductions of black carbon in the Arctic
Measurement report: Atmospheric fluorescent bioaerosol concentrations measured during 18 months in a coniferous forest in the south of Sweden
Measurement report: High Arctic aerosol hygroscopicity at sub- and supersaturated conditions during spring and summer
Examining the vertical heterogeneity of aerosols over the Southern Great Plains
Ice-nucleating particles in northern Greenland: annual cycles, biological contribution and parameterizations
Aerosol deposition to the boreal forest in the vicinity of the Alberta Oil Sands
The density of ambient black carbon retrieved by a new method: implications for cloud condensation nuclei prediction
Two-year measurements of Black Carbon properties at the high-altitude mountain site of Pic du Midi Observatory in the French Pyrenees
Long-range transported continental aerosol in the eastern North Atlantic: three multiday event regimes influence cloud condensation nuclei
Measurement report: Understanding the seasonal cycle of Southern Ocean aerosols
Elucidating ozone and PM2.5 pollution in the Fenwei Plain reveals the co-benefits of controlling precursor gas emissions in winter haze
Quantifying particle-to-particle heterogeneity in aerosol hygroscopicity
Measurement report: Black carbon properties and concentrations in southern Sweden urban and rural air – the importance of long-range transport
Markku Kulmala, Anna Lintunen, Hanna Lappalainen, Annele Virtanen, Chao Yan, Ekaterina Ezhova, Tuomo Nieminen, Ilona Riipinen, Risto Makkonen, Johanna Tamminen, Anu-Maija Sundström, Antti Arola, Armin Hansel, Kari Lehtinen, Timo Vesala, Tuukka Petäjä, Jaana Bäck, Tom Kokkonen, and Veli-Matti Kerminen
Atmos. Chem. Phys., 23, 14949–14971, https://doi.org/10.5194/acp-23-14949-2023, https://doi.org/10.5194/acp-23-14949-2023, 2023
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To be able to meet global grand challenges, we need comprehensive open data with proper metadata. In this opinion paper, we describe the SMEAR (Station for Measuring Earth surface – Atmosphere Relations) concept and include several examples (cases), such as new particle formation and growth, feedback loops and the effect of COVID-19, and what has been learned from these investigations. The future needs and the potential of comprehensive observations of the environment are summarized.
Weilun Zhao, Ying Li, Gang Zhao, Song Guo, Nan Ma, Shuya Hu, and Chunsheng Zhao
Atmos. Chem. Phys., 23, 14889–14902, https://doi.org/10.5194/acp-23-14889-2023, https://doi.org/10.5194/acp-23-14889-2023, 2023
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Studies have concentrated on particles containing black carbon (BC) smaller than 700 nm because of technical limitations. In this study, BC-containing particles larger than 700 nm (BC>700) were measured, highlighting their importance to total BC mass and absorption. The contribution of BC>700 to the BC direct radiative effect was estimated, highlighting the necessity to consider the whole size range of BC-containing particles in the model estimation of BC radiative effects.
Alessandro Bigi, Giorgio Veratti, Elisabeth Andrews, Martine Collaud Coen, Lorenzo Guerrieri, Vera Bernardoni, Dario Massabò, Luca Ferrero, Sergio Teggi, and Grazia Ghermandi
Atmos. Chem. Phys., 23, 14841–14869, https://doi.org/10.5194/acp-23-14841-2023, https://doi.org/10.5194/acp-23-14841-2023, 2023
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Atmospheric particles include compounds that play a key role in the greenhouse effect and air toxicity. Concurrent observations of these compounds by multiple instruments are presented, following deployment within an urban environment in the Po Valley, one of Europe's pollution hotspots. The study compares these data, highlighting the impact of ground emissions, mainly vehicular traffic and biomass burning, on the absorption of sun radiation and, ultimately, on climate change and air quality.
Ghislain Motos, Gabriel Freitas, Paraskevi Georgakaki, Jörg Wieder, Guangyu Li, Wenche Aas, Chris Lunder, Radovan Krejci, Julie Thérèse Pasquier, Jan Henneberger, Robert Oscar David, Christoph Ritter, Claudia Mohr, Paul Zieger, and Athanasios Nenes
Atmos. Chem. Phys., 23, 13941–13956, https://doi.org/10.5194/acp-23-13941-2023, https://doi.org/10.5194/acp-23-13941-2023, 2023
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Low-altitude clouds play a key role in regulating the climate of the Arctic, a region that suffers from climate change more than any other on the planet. We gathered meteorological and aerosol physical and chemical data over a year and utilized them for a parameterization that help us unravel the factors driving and limiting the efficiency of cloud droplet formation. We then linked this information to the sources of aerosol found during each season and to processes of cloud glaciation.
Alberto Sanchez-Marroquin, Sarah L. Barr, Ian T. Burke, James B. McQuaid, and Benjamin J. Murray
Atmos. Chem. Phys., 23, 13819–13834, https://doi.org/10.5194/acp-23-13819-2023, https://doi.org/10.5194/acp-23-13819-2023, 2023
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The sources and concentrations of ice-nucleating particles (INPs) in the Arctic are still poorly understood. Here we report aircraft-based INP concentrations and aerosol composition in the western North American Arctic. The concentrations of INPs and all aerosol particles were low. The aerosol samples contained mostly sea salt and dust particles. Dust particles were more relevant for the INP concentrations than sea salt. However, dust alone cannot account for all of the measured INPs.
Katherine L. Ackerman, Alison D. Nugent, and Chung Taing
Atmos. Chem. Phys., 23, 13735–13753, https://doi.org/10.5194/acp-23-13735-2023, https://doi.org/10.5194/acp-23-13735-2023, 2023
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Sea salt aerosol is an important marine aerosol that may be produced in greater quantities in coastal regions than over the open ocean. This study observed these particles along the windward coastline of O'ahu, Hawai'i, to understand how wind and waves influence their production and dispersal. Overall, wave heights were the strongest variable correlated with changes in aerosol concentrations, while wind speeds played an important role in their horizontal dispersal and vertical mixing.
Jiyeon Park, Hyojin Kang, Yeontae Gim, Eunho Jang, Ki-Tae Park, Sangjong Park, Chang Hoon Jung, Darius Ceburnis, Colin O'Dowd, and Young Jun Yoon
Atmos. Chem. Phys., 23, 13625–13646, https://doi.org/10.5194/acp-23-13625-2023, https://doi.org/10.5194/acp-23-13625-2023, 2023
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We measured the number size distribution of 2.5–300 nm particles and cloud condensation nuclei (CCN) number concentrations at King Sejong Station on the Antarctic Peninsula continuously from 1 January to 31 December 2018. During the pristine and clean periods, 97 new particle formation (NPF) events were detected. For 83 of these, CCN concentrations increased by 2 %–268 % (median 44 %) following 1 to 36 h (median 8 h) after NPF events.
Aodong Du, Jiaxing Sun, Hang Liu, Weiqi Xu, Wei Zhou, Yuting Zhang, Lei Li, Xubing Du, Yan Li, Xiaole Pan, Zifa Wang, and Yele Sun
Atmos. Chem. Phys., 23, 13597–13611, https://doi.org/10.5194/acp-23-13597-2023, https://doi.org/10.5194/acp-23-13597-2023, 2023
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We characterized the impacts of emission controls on particle mixing state and density during the Beijing Olympic Winter Games using a SPAMS in tandem with a DMA and an AAC. OC and sulfate-containing particles increased, while those from primary emissions decreased. The effective particle densities increased and varied largely for different particles, highlighting the impacts of aging and formation processes on the changes of particle density and mixing state.
Karine Sellegri, Theresa Barthelmeß, Jonathan Trueblood, Antonia Cristi, Evelyn Freney, Clémence Rose, Neill Barr, Mike Harvey, Karl Safi, Stacy Deppeler, Karen Thompson, Wayne Dillon, Anja Engel, and Cliff Law
Atmos. Chem. Phys., 23, 12949–12964, https://doi.org/10.5194/acp-23-12949-2023, https://doi.org/10.5194/acp-23-12949-2023, 2023
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The amount of sea spray emitted to the atmosphere depends on the ocean temperature, but this dependency is not well understood, especially when ocean biology is involved. In this study, we show that sea spray emissions are increased by up to a factor of 4 at low seawater temperatures compared to moderate temperatures, and we quantify the temperature dependence as a function of the ocean biogeochemistry.
Albert Ansmann, Kevin Ohneiser, Ronny Engelmann, Martin Radenz, Hannes Griesche, Julian Hofer, Dietrich Althausen, Jessie M. Creamean, Matthew C. Boyer, Daniel A. Knopf, Sandro Dahlke, Marion Maturilli, Henriette Gebauer, Johannes Bühl, Cristofer Jimenez, Patric Seifert, and Ulla Wandinger
Atmos. Chem. Phys., 23, 12821–12849, https://doi.org/10.5194/acp-23-12821-2023, https://doi.org/10.5194/acp-23-12821-2023, 2023
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The 1-year MOSAiC (2019–2020) expedition with the German ice breaker Polarstern was the largest polar field campaign ever conducted. The Polarstern, with our lidar aboard, drifted with the pack ice north of 85° N for more than 7 months (October 2019 to mid-May 2020). We measured the full annual cycle of aerosol conditions in terms of aerosol optical and cloud-process-relevant properties. We observed a strong contrast between polluted winter and clean summer aerosol conditions.
Nair Krishnan Kala, Narayana Sarma Anand, Mohanan R. Manoj, Srinivasan Prasanth, Harshavardhana S. Pathak, Thara Prabhakaran, Pramod D. Safai, Krishnaswamy K. Moorthy, and Sreedharan K. Satheesh
Atmos. Chem. Phys., 23, 12801–12819, https://doi.org/10.5194/acp-23-12801-2023, https://doi.org/10.5194/acp-23-12801-2023, 2023
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We present a 3D data set of aerosol black carbon over the Indian mainland by assimilating data from surface, aircraft, and balloon measurements, along with multi-satellite observations. Radiative transfer computations using height-resolved aerosol absorption show higher warming in the free troposphere and will have large implications for atmospheric stability. This data set will help reduce the uncertainty in aerosol radiative effects in climate model simulations over the Indian region.
Sujan Shrestha, Shan Zhou, Manisha Mehra, Meghan Guagenti, Subin Yoon, Sergio L. Alvarez, Fangzhou Guo, Chun-Ying Chao, James H. Flynn III, Yuxuan Wang, Robert J. Griffin, Sascha Usenko, and Rebecca J. Sheesley
Atmos. Chem. Phys., 23, 10845–10867, https://doi.org/10.5194/acp-23-10845-2023, https://doi.org/10.5194/acp-23-10845-2023, 2023
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We evaluated different methods for assessing the influence of long-range transport of biomass burning (BB) plumes at a coastal site in Texas, USA. We show that the aerosol composition and optical properties exhibited good agreement, while CO and acetonitrile trends were less specific for assessing BB source influence. Our results demonstrate that the network of aerosol optical measurements can be useful for identifying the influence of aged BB plumes in anthropogenically influenced areas.
Guangyu Li, Elise K. Wilbourn, Zezhen Cheng, Jörg Wieder, Allison Fagerson, Jan Henneberger, Ghislain Motos, Rita Traversi, Sarah D. Brooks, Mauro Mazzola, Swarup China, Athanasios Nenes, Ulrike Lohmann, Naruki Hiranuma, and Zamin A. Kanji
Atmos. Chem. Phys., 23, 10489–10516, https://doi.org/10.5194/acp-23-10489-2023, https://doi.org/10.5194/acp-23-10489-2023, 2023
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In this work, we present results from an Arctic field campaign (NASCENT) in Ny-Ålesund, Svalbard, on the abundance, variability, physicochemical properties, and potential sources of ice-nucleating particles (INPs) relevant for mixed-phase cloud formation. This work improves the data coverage of Arctic INPs and aerosol properties, allowing for the validation of models predicting cloud microphysical and radiative properties of mixed-phase clouds in the rapidly warming Arctic.
Jun Shi, Jinpei Yan, Shanshan Wang, Shuhui Zhao, Miming Zhang, Suqing Xu, Qi Lin, Hang Yang, and Siying Dai
Atmos. Chem. Phys., 23, 10349–10359, https://doi.org/10.5194/acp-23-10349-2023, https://doi.org/10.5194/acp-23-10349-2023, 2023
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An underway aerosol-monitoring system was used to determine the Na+ concentration during different cyclone periods in the Southern Ocean in order to assess the potential effects of cyclones on sea spray aerosol (SSA) emissions. It was estimated that more than 23 % of SSAs were transported upwards during cyclone periods. Vertically transported SSAs can be regarded as an important source of CCN and hence have an effect on climate in the middle and high latitudes of the Southern Hemisphere.
Wenwen Ma, Rong Sun, Xiaoping Wang, Zheng Zong, Shizhen Zhao, Zeyu Sun, Chongguo Tian, Jianhui Tang, Song Cui, Jun Li, and Gan Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2023-1995, https://doi.org/10.5194/egusphere-2023-1995, 2023
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This is the first report of long-term atmospheric PAHs monitoring around the Bohai Sea. The results showed that the concentrations of PAHs in the atmosphere of Bohai Sea was decreasing from June 2014 to May 2019, especially the high toxic PAHs concentrations. This indicated that the contribution of PAHs sources had been changed by some certain extent at different areas, and it also led to the reduction of the related health risk and medical costs during pollution prevention and control.
Jean-Philippe Putaud, Enrico Pisoni, Alexander Mangold, Christoph Hueglin, Jean Sciare, Michael Pikridas, Chrysanthos Savvides, Jakub Ondracek, Saliou Mbengue, Alfred Wiedensohler, Kay Weinhold, Maik Merkel, Laurent Poulain, Dominik van Pinxteren, Hartmut Herrmann, Andreas Massling, Claus Nordstroem, Andrés Alastuey, Cristina Reche, Noemí Pérez, Sonia Castillo, Mar Sorribas, Jose Antonio Adame, Tuukka Petaja, Katrianne Lehtipalo, Jarkko Niemi, Véronique Riffault, Joel F. de Brito, Augustin Colette, Olivier Favez, Jean-Eudes Petit, Valérie Gros, Maria I. Gini, Stergios Vratolis, Konstantinos Eleftheriadis, Evangelia Diapouli, Hugo Denier van der Gon, Karl Espen Yttri, and Wenche Aas
Atmos. Chem. Phys., 23, 10145–10161, https://doi.org/10.5194/acp-23-10145-2023, https://doi.org/10.5194/acp-23-10145-2023, 2023
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Many European people are still exposed to levels of air pollution that can affect their health. COVID-19 lockdowns in 2020 were used to assess the impact of the reduction in human mobility on air pollution across Europe by comparing measurement data with values that would be expected if no lockdown had occurred. We show that lockdown measures did not lead to consistent decreases in the concentrations of fine particulate matter suspended in the air, and we investigate why.
Qian Xiao, Jiaoshi Zhang, Yang Wang, Luke D. Ziemba, Ewan Crosbie, Edward L. Winstead, Claire E. Robinson, Joshua P. DiGangi, Glenn S. Diskin, Jeffrey S. Reid, K. Sebastian Schmidt, Armin Sorooshian, Miguel Ricardo A. Hilario, Sarah Woods, Paul Lawson, Snorre A. Stamnes, and Jian Wang
Atmos. Chem. Phys., 23, 9853–9871, https://doi.org/10.5194/acp-23-9853-2023, https://doi.org/10.5194/acp-23-9853-2023, 2023
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Using recent airborne measurements, we show that the influences of anthropogenic emissions, transport, convective clouds, and meteorology lead to new particle formation (NPF) under a variety of conditions and at different altitudes in tropical marine environments. NPF is enhanced by fresh urban emissions in convective outflow but is suppressed in air masses influenced by aged urban emissions where reactive precursors are mostly consumed while particle surface area remains relatively high.
Andreas Aktypis, Christos Kaltsonoudis, David Patoulias, Panayiotis Kalkavouras, Angeliki Matrali, Christina N. Vasilakopoulou, Evangelia Kostenidou, Kalliopi Florou, Nikos Kalivitis, Aikaterini Bougiatioti, Konstantinos Eleftheriadis, Stergios Vratolis, Maria I. Gini, Athanasios Kouras, Constantini Samara, Mihalis Lazaridis, Sofia-Eirini Chatoutsidou, Nikolaos Mihalopoulos, and Spyros N. Pandis
EGUsphere, https://doi.org/10.5194/egusphere-2023-1899, https://doi.org/10.5194/egusphere-2023-1899, 2023
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Extensive continuous particle number size distribution measurements took place during two summers (2020 and 2021) in 11 sites in Greece for the investigation of the frequency and the spatial extent of new particle formation. The frequency during summer varied from close to zero in southwestern Greece to more than 60 % in the northern, central, and eastern regions. The spatial variability can be explained by the proximity of the sites to coal-fired power plants and agricultural areas.
Simo Hakala, Ville Vakkari, Heikki Lihavainen, Antti-Pekka Hyvärinen, Kimmo Neitola, Jenni Kontkanen, Veli-Matti Kerminen, Markku Kulmala, Tuukka Petäjä, Tareq Hussein, Mamdouh I. Khoder, Mansour A. Alghamdi, and Pauli Paasonen
Atmos. Chem. Phys., 23, 9287–9321, https://doi.org/10.5194/acp-23-9287-2023, https://doi.org/10.5194/acp-23-9287-2023, 2023
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Things are not always as they first seem in ambient aerosol measurements. Observations of decreasing particle sizes are often interpreted as resulting from particle evaporation. We show that such observations can counterintuitively be explained by particles that are constantly growing in size. This requires one to account for the previous movements of the observed air. Our explanation implies a larger number of larger particles, meaning more significant effects of aerosols on climate and health.
Julius Seidler, Markus Norbert Friedrich, Christoph Karl Thomas, and Anke Christine Nölscher
EGUsphere, https://doi.org/10.5194/egusphere-2023-1696, https://doi.org/10.5194/egusphere-2023-1696, 2023
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Here we study the transport of ultrafine particles (UFP) from an airport to two new adjacent measuring sites for one year. The number of UFP in the air and the diurnal variation is typical urban. Winds from the airport show increased number concentrations. Additionally, considering wind frequencies, we estimate that from all UFP measured at the two sites 10–14 % originate from the airport and/or other UFP sources from between airport and site.
Akriti Masoom, Ilias Fountoulakis, Stelios Kazadzis, Ioannis-Panagiotis Raptis, Anna Kampouri, Basil E. Psiloglou, Dimitra Kouklaki, Kyriakoula Papachristopoulou, Eleni Marinou, Stavros Solomos, Anna Gialitaki, Dimitra Founda, Vasileios Salamalikis, Dimitris Kaskaoutis, Natalia Kouremeti, Nikolaos Mihalopoulos, Vassilis Amiridis, Andreas Kazantzidis, Alexandros Papayannis, Christos S. Zerefos, and Kostas Eleftheratos
Atmos. Chem. Phys., 23, 8487–8514, https://doi.org/10.5194/acp-23-8487-2023, https://doi.org/10.5194/acp-23-8487-2023, 2023
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We analyse the spatial and temporal aerosol spectral optical properties during the extreme wildfires of August 2021 in Greece and assess their effects on air quality and solar radiation quantities related to health, agriculture, and energy. Different aerosol conditions are identified (pure smoke, pure dust, dust–smoke together); the largest impact on solar radiation quantities is found for cases with mixed dust–smoke aerosols. Such situations are expected to occur more frequently in the future.
Xiaojing Shen, Junying Sun, Huizheng Che, Yangmei Zhang, Chunhong Zhou, Ke Gui, Wanyun Xu, Quan Liu, Junting Zhong, Can Xia, Xinyao Hu, Sinan Zhang, Jialing Wang, Shuo Liu, Jiayuan Lu, Aoyuan Yu, and Xiaoye Zhang
Atmos. Chem. Phys., 23, 8241–8257, https://doi.org/10.5194/acp-23-8241-2023, https://doi.org/10.5194/acp-23-8241-2023, 2023
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New particle formation (NPF) events occur when the dust episodes' fade is analysed based on long-term measurement of particle number size distribution. Analysis shows that the observed formation and growth rates are approximately 50 % of and 30 % lower than those of other NPF events. As a consequence of the uptake of precursor gases on mineral dust, the physical and chemical properties of submicron particles, as well as the ability to be cloud condensation nuclei, can be changed.
Marco Zanatta, Stephan Mertes, Olivier Jourdan, Regis Dupuy, Emma Järvinen, Martin Schnaiter, Oliver Eppers, Johannes Schneider, Zsófia Jurányi, and Andreas Herber
Atmos. Chem. Phys., 23, 7955–7973, https://doi.org/10.5194/acp-23-7955-2023, https://doi.org/10.5194/acp-23-7955-2023, 2023
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Black carbon (BC) particles influence the Arctic radiative balance. Vertical measurements of black carbon were conducted during the ACLOUD campaign in the European Arctic to study the interaction of BC with clouds. This study shows that clouds influence the vertical variability of BC properties across the inversion layer and that multiple activation and transformation mechanisms of BC may occur in the presence of low-level, persistent, mixed-phase clouds.
Guangdong Niu, Ximeng Qi, Liangduo Chen, Lian Xue, Shiyi Lai, Xin Huang, Jiaping Wang, Xuguang Chi, Wei Nie, Veli-Matti Kerminen, Tuukka Petäjä, Markku Kulmala, and Aijun Ding
Atmos. Chem. Phys., 23, 7521–7534, https://doi.org/10.5194/acp-23-7521-2023, https://doi.org/10.5194/acp-23-7521-2023, 2023
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The reported below-cloud wet-scavenging coefficients (BWSCs) are much higher than theoretical data, but the reason remains unclear. Based on long-term observation, we find that air mass changing during rainfall events causes the overestimation of BWSCs. Thus, the discrepancy in BWSCs between observation and theory is not as large as currently believed. To obtain reasonable BWSCs and parameterizations from field observations, the effect of air mass changes needs to be considered.
Antonio Donateo, Gianluca Pappaccogli, Daniela Famulari, Mauro Mazzola, Federico Scoto, and Stefano Decesari
Atmos. Chem. Phys., 23, 7425–7445, https://doi.org/10.5194/acp-23-7425-2023, https://doi.org/10.5194/acp-23-7425-2023, 2023
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This work aims to measure the turbulent fluxes and the dry deposition velocity for size-segregated particles (from ultrafine to quasi-coarse range) at an Arctic site (Svalbard). Aiming to characterize the effect of surface properties on dry deposition, continuous observations were performed from the coldest months (on snow surface) to the snow melting period and throughout the summer (snow-free surface). A data fit of the deposition velocity as a function of particle diameters will be provided.
Hang Liu, Xiaole Pan, Shandong Lei, Yuting Zhang, Aodong Du, Weijie Yao, Guiqian Tang, Tao Wang, Jinyuan Xin, Jie Li, Yele Sun, Junji Cao, and Zifa Wang
Atmos. Chem. Phys., 23, 7225–7239, https://doi.org/10.5194/acp-23-7225-2023, https://doi.org/10.5194/acp-23-7225-2023, 2023
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We provide the average vertical profiles of black carbon (BC) concentration, size distribution and coating thickness at different times of the day in an urban area based on 112 vertical profiles. In addition, it is found that BC in the residual layer generally has a thicker coating, higher absorption enhancement and hygroscopicity than on the surface. Such aged BC could enter into the boundary layer and influence the BC properties in the early morning.
Cristina González-Flórez, Martina Klose, Andrés Alastuey, Sylvain Dupont, Jerónimo Escribano, Vicken Etyemezian, Adolfo Gonzalez-Romero, Yue Huang, Konrad Kandler, George Nikolich, Agnesh Panta, Xavier Querol, Cristina Reche, Jesús Yus-Díez, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 23, 7177–7212, https://doi.org/10.5194/acp-23-7177-2023, https://doi.org/10.5194/acp-23-7177-2023, 2023
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Atmospheric mineral dust consists of tiny mineral particles that are emitted by wind erosion from arid regions. Its particle size distribution (PSD) affects its impact on the Earth's system. Nowadays, there is an incomplete understanding of the emitted dust PSD and a lot of debate about its variability. Here, we try to address these issues based on the measurements performed during a wind erosion and dust emission field campaign in the Moroccan Sahara within the framework of FRAGMENT project.
Kevin R. Barry, Thomas C. J. Hill, Marina Nieto-Caballero, Thomas A. Douglas, Sonia M. Kreidenweis, Paul J. DeMott, and Jessie M. Creamean
EGUsphere, https://doi.org/10.5194/egusphere-2023-1208, https://doi.org/10.5194/egusphere-2023-1208, 2023
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Ice nucleating particles (INPs) are important for the climate due to their influence on cloud properties. To understand potential land-based sources of them in the Arctic, we carried out a source survey near the northernmost point of Alaska, a landscape connected to the changing permafrost (thermokarst). Permafrost contained high concentrations of INPs, with the largest values near the coast. The thermokarst lakes were found to emit INPs, and its water contained elevated concentrations.
Stefania Gilardoni, Dominic Heslin-Rees, Mauro Mazzola, Vito Vitale, Michael Sprenger, and Radovan Krejci
EGUsphere, https://doi.org/10.5194/egusphere-2023-1376, https://doi.org/10.5194/egusphere-2023-1376, 2023
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Models still fail in reproducing black carbon (BC) temporal variability in the Arctic. Analysis of equivalent BC concentration in the European Arctic shows that BC seasonal variability is modulated by the efficiency of removal by precipitation during transport towards high latitudes. Short-term variability is controlled by synoptic-scale circulation patterns. The advection of warm air from lower latitudes is an effective pollution transport pathway during summer.
Stergios Vratolis, Evangelia Diapouli, Manousos I. Manousakas, Susana Marta Almeida, Ivan Beslic, Zsofia Kertesz, Lucyna Samek, and Konstantinos Eleftheriadis
Atmos. Chem. Phys., 23, 6941–6961, https://doi.org/10.5194/acp-23-6941-2023, https://doi.org/10.5194/acp-23-6941-2023, 2023
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Using a dataset from 16 European and Asian cities we develop a new method so as to identify and quantify the emission fluxes from each geographic grid cell for secondary sulfate and dust aerosol. The information provided by the new method allows the implementation of targeted mitigation measures. The new method could be applied to several other pollutants (e.g., black carbon).
Yishuo Guo, Chenjuan Deng, Aino Ovaska, Feixue Zheng, Chenjie Hua, Junlei Zhan, Yiran Li, Jin Wu, Zongcheng Wang, Jiali Xie, Ying Zhang, Tingyu Liu, Yusheng Zhang, Boying Song, Wei Ma, Yongchun Liu, Chao Yan, Jingkun Jiang, Veli-Matti Kerminen, Men Xia, Tuomo Nieminen, Wei Du, Tom Kokkonen, and Markku Kulmala
Atmos. Chem. Phys., 23, 6663–6690, https://doi.org/10.5194/acp-23-6663-2023, https://doi.org/10.5194/acp-23-6663-2023, 2023
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Using the comprehensive datasets, we investigated the long-term variations of air pollutants during winter in Beijing from 2019 to 2022 and analyzed the characteristics of atmospheric pollution cocktail during different short-term special events (e.g., Beijing Winter Olympics, COVID lockdown and Chinese New Year) associated with substantial emission reductions. Our results are useful in planning more targeted and sustainable long-term pollution control plans.
Julika Zinke, E. Douglas Nilsson, Piotr Markuszewski, Paul Zieger, E. Monica Mårtensson, Anna Rutgersson, Erik Nilsson, and Matthew E. Salter
EGUsphere, https://doi.org/10.5194/egusphere-2023-966, https://doi.org/10.5194/egusphere-2023-966, 2023
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We conducted two research campaigns in the Baltic Sea, during which we combined laboratory sea spray simulation experiments with flux measurements on a nearby island. To combine these two methods, we scaled the laboratory measurements to the flux measurements using three different approaches. As a result, we derived a parameterization that is dependent on wind speed and wave state for particles with diameters 0.015–10 μm. This parameterization is applicable to low-salinity waters.
Fei Li, Biao Luo, Miaomiao Zhai, Li Liu, Gang Zhao, Hanbing Xu, Tao Deng, Xuejiao Deng, Haobo Tan, Ye Kuang, and Jun Zhao
Atmos. Chem. Phys., 23, 6545–6558, https://doi.org/10.5194/acp-23-6545-2023, https://doi.org/10.5194/acp-23-6545-2023, 2023
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A field campaign was conducted to study black carbon (BC) mass size distributions and mixing states connected to traffic emissions using a system that combines a differential mobility analyzer and single-particle soot photometer. Results showed that the black carbon content of traffic emissions has a considerable influence on both BC mass size distributions and mixing states, which has crucial implications for accurately representing BC from various sources in regional and climate models.
Juan Andrés Casquero-Vera, Daniel Pérez-Ramírez, Hassan Lyamani, Fernando Rejano, Andrea Casans, Gloria Titos, Francisco José Olmo, Lubna Dada, Simo Hakala, Tareq Hussein, Katrianne Lehtipalo, Pauli Paasonen, Antti Hyvärinen, Noemí Pérez, Xavier Querol, Sergio Rodríguez, Nikos Kalivitis, Yenny González, Mansour A. Alghamdi, Veli-Matti Kerminen, Andrés Alastuey, Tuukka Petäjä, and Lucas Alados-Arboledas
EGUsphere, https://doi.org/10.5194/egusphere-2023-1238, https://doi.org/10.5194/egusphere-2023-1238, 2023
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Here we present the first study of the effect of mineral dust on the inhibition/promotion of new particle formation (NPF) events in different dust-influenced areas. Unexpectedly, we show that the occurrence of NPF events is highly frequent during mineral dust outbreaks, occurring even during extreme dust outbreaks. We also show that the occurrence of NPF events during mineral dust outbreaks significantly affects the potential cloud condensation nuclei budget.
Juan Hong, Min Tang, Qiaoqiao Wang, Nan Ma, Shaowen Zhu, Shaobin Zhang, Xihao Pan, Linhong Xie, Guo Li, Uwe Kuhn, Chao Yan, Jiangchuan Tao, Ye Kuang, Yao He, Wanyun Xu, Runlong Cai, Yaqing Zhou, Zhibin Wang, Guangsheng Zhou, Bin Yuan, Yafang Cheng, and Hang Su
Atmos. Chem. Phys., 23, 5699–5713, https://doi.org/10.5194/acp-23-5699-2023, https://doi.org/10.5194/acp-23-5699-2023, 2023
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A comprehensive investigation of the characteristics of new particle formation (NPF) events was conducted at a rural site on the North China Plain (NCP), China, during the wintertime of 2018 by covering the particle number size distribution down to sub–3 nm. Potential mechanisms for NPF under the current environment were explored, followed by a further discussion on the factors governing the occurrence of NPF at this rural site compared with other regions (e.g., urban areas) in the NCP region.
Xinyao Hu, Junying Sun, Can Xia, Xiaojing Shen, Yangmei Zhang, Quan Liu, Zhaodong Liu, Sinan Zhang, Jialing Wang, Aoyuan Yu, Jiayuan Lu, Shuo Liu, and Xiaoye Zhang
Atmos. Chem. Phys., 23, 5517–5531, https://doi.org/10.5194/acp-23-5517-2023, https://doi.org/10.5194/acp-23-5517-2023, 2023
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The simultaneous measurements under dry conditions of aerosol optical properties were conducted at three wavelengths for PM1 and PM10 in urban Beijing from 2018 to 2021. Considerable reductions in aerosol absorption coefficient and increased single scattering albedo demonstrated that absorbing aerosols were more effectively controlled than scattering aerosols due to pollution control measures. The aerosol radiative effect and the transport's impact on aerosol optical properties were analysed.
Martin de Graaf, Karolina Sarna, Jessica Brown, Elma V. Tenner, Manon Schenkels, and David P. Donovan
Atmos. Chem. Phys., 23, 5373–5391, https://doi.org/10.5194/acp-23-5373-2023, https://doi.org/10.5194/acp-23-5373-2023, 2023
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Clouds over the oceans reflect sunlight and cool the earth. Simultaneous measurements were performed of cloud droplet sizes and smoke particles in and near the cloud base over Ascension Island, a remote island in the Atlantic Ocean, to determine the sensitivity of cloud droplets to smoke from the African continent. The smoke was found to reduce cloud droplet sizes, which makes the cloud droplets more susceptible to evaporation, reducing cloud lifetime.
Dominic Heslin-Rees, Peter Tunved, Johan Ström, Roxana Cremer, Paul Zieger, Ilona Riipinen, Annica Ekman, Konstantinos Eleftheriadis, and Radovan Krejci
EGUsphere, https://doi.org/10.5194/egusphere-2023-940, https://doi.org/10.5194/egusphere-2023-940, 2023
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Light-absorbing atmospheric particles (e.g. black carbon (BC)) exert a warming effect on the Arctic climate. We show that the amount of particle light absorption decreased from 2002 to 2022. We conclude that in addition to reductions in emissions of BC, wet removal plays a role in the long-term reduction of BC in the Arctic, given the increase in surface precipitation experienced by air masses arriving at the site. The potential impact of biomass-burning events is shown to have increased.
Madeleine Petersson Sjögren, Malin Alsved, Tina Šantl-Temkiv, Thomas Bjerring Kristensen, and Jakob Löndahl
Atmos. Chem. Phys., 23, 4977–4992, https://doi.org/10.5194/acp-23-4977-2023, https://doi.org/10.5194/acp-23-4977-2023, 2023
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Biological aerosol particles (bioaerosols) affect human health by spreading diseases and may be important agents for atmospheric processes, but their abundance and size distributions are largely unknown. We measured bioaerosols for 18 months in the south of Sweden to investigate bioaerosol temporal variations and their couplings to meteorology. Our results showed that the bioaerosols emissions were coupled to meteorological parameters and depended strongly on the season.
Andreas Massling, Robert Lange, Jakob Boyd Pernov, Ulrich Gosewinkel, Lise-Lotte Sørensen, and Henrik Skov
Atmos. Chem. Phys., 23, 4931–4953, https://doi.org/10.5194/acp-23-4931-2023, https://doi.org/10.5194/acp-23-4931-2023, 2023
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The effect of anthropogenic activities on cloud formation introduces the highest uncertainties with respect to climate change. Data on Arctic aerosols and their corresponding cloud-forming properties are very scarce and most important as the Arctic is warming about 2 times as fast as the rest of the globe. Our studies investigate aerosols in the remote Arctic and suggest relatively high cloud-forming potential, although differences are observed between the Arctic spring and summer.
Yang Wang, Chanakya Bagya Ramesh, Scott Giangrande, Jerome Fast, Xianda Gong, Jiaoshi Zhang, Alyssa Matthews, Fan Mei, Ahmet Tolga Odabasi, John Shilling, Jason Tomlinson, Die Wang, and Jian Wang
EGUsphere, https://doi.org/10.5194/egusphere-2023-830, https://doi.org/10.5194/egusphere-2023-830, 2023
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We report the vertical profiles of aerosol properties over the Southern Great Plains (SGP), a region influenced by shallow convective clouds, land-atmosphere interactions, boundary layer turbulence, and the aerosol life cycle. We examined the processes that drive the aerosol population and distribution in the lower troposphere over the SGP. This study helps improve our understanding of aerosol-cloud interactions and the model representation of aerosol processes.
Kevin C. H. Sze, Heike Wex, Markus Hartmann, Henrik Skov, Andreas Massling, Diego Villanueva, and Frank Stratmann
Atmos. Chem. Phys., 23, 4741–4761, https://doi.org/10.5194/acp-23-4741-2023, https://doi.org/10.5194/acp-23-4741-2023, 2023
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Ice-nucleating particles (INPs) play an important role in cloud formation and thus in our climate. But little is known about the abundance and properties of INPs, especially in the Arctic, where the temperature increases almost 4 times as fast as that of the rest of the globe. We observe higher INP concentrations and more biological INPs in summer than in winter, likely from local sources. We also provide three equations for estimating INP concentrations in models at different times of the year.
Timothy Jiang, Mark Gordon, Paul A. Makar, Ralf M. Staebler, and Michael Wheeler
Atmos. Chem. Phys., 23, 4361–4372, https://doi.org/10.5194/acp-23-4361-2023, https://doi.org/10.5194/acp-23-4361-2023, 2023
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Measurements of submicron aerosols (particles smaller than 1 / 1000 of a millimeter) were made in a forest downwind of oil sands mining and production facilities in northern Alberta. These measurements tell us how quickly aerosols are absorbed by the forest (known as deposition rate) and how the deposition rate depends on the size of the aerosol. The measurements show good agreement with a parameterization developed from a recent study for deposition of aerosols to a similar pine forest.
Jingye Ren, Lu Chen, Jieyao Liu, and Fang Zhang
Atmos. Chem. Phys., 23, 4327–4342, https://doi.org/10.5194/acp-23-4327-2023, https://doi.org/10.5194/acp-23-4327-2023, 2023
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The density of black carbon (BC) is linked to its morphology and mixing state and could cause uncertainty in evaluating cloud condensation nuclei (CCN) activity. A method for retrieving the mixing state and density of BC in the urban atmosphere is developed. The mean retrieval density of internally mixed BC was lower, assuming void-free spherical structures. Our study suggests the importance of accounting for variable BC density in models when assessing its climate effect in urban atmosphere.
Sarah Tinorua, Cyrielle Denjean, Pierre Nabat, Thierry Bourrianne, Véronique Pont, François Gheusi, and Emmanuel Leclerc
EGUsphere, https://doi.org/10.5194/egusphere-2023-570, https://doi.org/10.5194/egusphere-2023-570, 2023
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Two years of Black Carbon (BC) and aerosols optical and microphysical measurements have been conducted at a french high-altitude site, where numerous complex interactions between BC, radiation, clouds and snow impact climate. We observed strong seasonal BC properties variations, with a higher absorption enhancement in summer compared to winter. The combination of BC emission sources, transport pathways, atmospheric dynamics and chemical processes explains the BC light absorption seasonality.
Francesca Gallo, Janek Uin, Kevin J. Sanchez, Richard H. Moore, Jian Wang, Robert Wood, Fan Mei, Connor Flynn, Stephen Springston, Eduardo B. Azevedo, Chongai Kuang, and Allison C. Aiken
Atmos. Chem. Phys., 23, 4221–4246, https://doi.org/10.5194/acp-23-4221-2023, https://doi.org/10.5194/acp-23-4221-2023, 2023
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This study provides a summary statistic of multiday aerosol plume transport event influences on aerosol physical properties and the cloud condensation nuclei budget at the U.S. Department of Energy Atmospheric Radiation Measurement Facility in the eastern North Atlantic (ENA). An algorithm that integrates aerosol properties is developed and applied to identify multiday aerosol transport events. The influence of the aerosol plumes on aerosol populations at the ENA is successively assessed.
Ruhi S. Humphries, Melita D. Keywood, Jason P. Ward, James Harnwell, Simon P. Alexander, Andrew R. Klekociuk, Keiichiro Hara, Ian M. McRobert, Alain Protat, Joel Alroe, Luke T. Cravigan, Branka Miljevic, Zoran D. Ristovski, Robyn Schofield, Stephen R. Wilson, Connor J. Flynn, Gourihar R. Kulkarni, Gerald G. Mace, Greg M. McFarquhar, Scott D. Chambers, Alastair G. Williams, and Alan D. Griffiths
Atmos. Chem. Phys., 23, 3749–3777, https://doi.org/10.5194/acp-23-3749-2023, https://doi.org/10.5194/acp-23-3749-2023, 2023
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Observations of aerosols in pristine regions are rare but are vital to constraining the natural baseline from which climate simulations are calculated. Here we present recent seasonal observations of aerosols from the Southern Ocean and contrast them with measurements from Antarctica, Australia and regionally relevant voyages. Strong seasonal cycles persist, but striking differences occur at different latitudes. This study highlights the need for more long-term observations in remote regions.
Chunshui Lin, Ru-Jin Huang, Haobin Zhong, Jing Duan, Zixi Wang, Wei Huang, and Wei Xu
Atmos. Chem. Phys., 23, 3595–3607, https://doi.org/10.5194/acp-23-3595-2023, https://doi.org/10.5194/acp-23-3595-2023, 2023
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The complex interaction between O3 and PM2.5, coupled with the topology of the Fenwei Plain and the evolution of the boundary layer height, highlights the challenges in further reducing particulate pollution in winter despite years of efforts to reduce emissions. Through scenario analysis in a chemical box model constrained by observation, we show the co-benefits of reducing NOx and VOCs simultaneously in reducing ozone and SOA.
Liang Yuan and Chunsheng Zhao
Atmos. Chem. Phys., 23, 3195–3205, https://doi.org/10.5194/acp-23-3195-2023, https://doi.org/10.5194/acp-23-3195-2023, 2023
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Chemical compositions vary between and within particles due to the complex sources and aging processes, causing particle-to-particle heterogeneity in aerosol hygroscopicity, which is of great importance to aerosol climatic and environmental effects. This study proposes an algorithm to quantify the heterogeneity from in situ measurements, sheds light on the reanalysis of the existing H-TDMA datasets, and could have a large impact on how we use and think about these datasets.
Erik Ahlberg, Stina Ausmeel, Lovisa Nilsson, Mårten Spanne, Julija Pauraite, Jacob Klenø Nøjgaard, Michele Bertò, Henrik Skov, Pontus Roldin, Adam Kristensson, Erik Swietlicki, and Axel Eriksson
Atmos. Chem. Phys., 23, 3051–3064, https://doi.org/10.5194/acp-23-3051-2023, https://doi.org/10.5194/acp-23-3051-2023, 2023
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To investigate the properties and origin of black carbon particles in southern Sweden during late summer, we performed measurements both at a rural site and the nearby city of Malmö. We found that local traffic emissions of black carbon led to concentrations around twice as high as those at the rural site. Modeling show that these emissions are not clearly distinguishable at the rural site, unless meteorology was favourable, which shows the importance of long-range transport and processing.
Cited articles
Alston E. and Sokolik, I.: A first-order assessment of direct aerosol radiative effect in the southeastern US using over a decade long multi-satellite data record, Air, Soil Water Res., 9, 97–112, https://doi.org/10.4137/ASWR.S39226, 2016.
Andreae, M. O., Jones, C. D., and Cox, P. M.: Strong present-day aerosol cooling implies a hot future, Nature, 435, 1187–1190, 2005.
Andrews, E., Sheridan, P. J., Fiebig, M., McComiskey, A., Ogren, J. A., Arnott, P., Covert, D., Elleman, R., Gasparini, R., Collins, D., Jonsson, H., Schmid, B., and Wang, J.: Comparison of methods for deriving aerosol asymmetry parameter, J. Geophys. Res, 111, D05S04, https://doi.org/10.1029/2004JD005734, 2006.
Brem, B. T., Mena Gonzalez, F. C., Meyers, S. R., Bond, T. C., and Rood, M. J.: Laboratory-Measured Optical Properties of Inorganic and Organic Aerosols at Relative Humidities up to 95 %, Aerosol Sci. Tech., 46, 178–190, https://doi.org/10.1080/02786826.2011.617794, 2012.
Carrico, C. M., Bergin, M. H., Xu, J., Baumann, K., and Maring, H.: Urban aerosol radiative properties: Measurements during the 1999 Atlanta Supersite Experiment, J. Geophys. Res., 108, 8422, https://doi.org/10.1029/2001JD001222, 2003.
Chung, C. E.: Aerosol Direct Radiative Forcing: A Review, Atmospheric Aerosols – Regional Characteristics – Chemistry and Physics, edited by: Abdul-Razzak, H., InTech, 379–393 https://doi.org/10.5772/50248, 2012.
Delene, D. J. and Ogren, J. A.: Variability of aerosol optical properties at four North American surface monitoring sites, J. Atmos. Sci., 59, 1135–1150, 2002.
Dubovik, O., Smirnov, A., Holben, B. N., King, M. D., Kaufman, Y. J., Eck, T. F., and Slutsker, I.: Accuracy assessments of aerosol optical properties retrieved from Aerosol Robotic Network (AERONET) Sun and sky radiance measurements, J. Geophys. Res., 105, 9791–9806, 2000.
Eck, T. F., Holben, B. N., Reid, J. S., Dubovik, O., Smirnov, A., O'Neill, N. T., Slutsker, I., and Kinne, S.: Wavelength dependence of the optical depth of biomass burning, urban and desert dust aerosols, J. Geophys. Res., 104, 31333–31350, 1999.
EMEP: Aerosol measurements, available at: http://ebas.nilu.no/Default.aspx, last access: 27 February 2018.
Gadhavi, H. and Jayaraman A.: Aerosol characteristics and aerosol radiative forcing over Maitri, Antarctica, Current Sci. India, 86, 296–304, 2004.
Goldstein, A. H., Koven, C. D., Heald, C. L., and Fung, I. Y.: Biogenic carbon and anthropogenic pollutants combine to form a cooling haze over the southeastern United States, P. Natl. Acad. Sci. USA, 106, 8835–8840, https://doi.org/10.1073/pnas.0904128106, 2009.
GSFC: AERONET Level 2 aerosol optical depth data, available at: https://aeronet.gsfc.nasa.gov/cgi-bin/webtool_opera_v2_new, last access: 27 February 2018.
Haywood, J. M. and Shine K. P.: The effect of anthropogenic sulfate and soot aerosol on the clear sky planetary radiation budget, Geophys Res Lett., 22, 603–606, 1995.
Henyey, L. C. and Greenstein, J. L.: Diffuse radiation in the galaxy, Astrophys. J., 93, 70–83, 1941.
Holben, B. N., Eck, T. F., Slutsker, I., Tanre, D., Buis, J. P., Setzer, A., Vermote, E., Reagan, J. A., Kaufman, Y. J., Nakajima, T., Lavenu, F., Janowiak, I., and Smirnov, A.: AERONET – A federated instrument network and data archive for aerosol characterization, Remote Sens. Environ., 66, 1–16, 1998.
Hyer, E. J., Reid, J. S., and Zhang, J.: An over-land aerosol optical depth data set for data assimilation by filtering, correction, and aggregation of MODIS Collection 5 optical depth retrievals, Atmos. Meas. Tech., 4, 379–408, https://doi.org/10.5194/amt-4-379-2011, 2011.
Justice, C. O., Townshend, J. R. G., Vermote, E. F., Masuoka, E., Wolfe, R. E., Saleous, N., Roy, D. P., and Morisette, J. T.: An overview of MODIS Land data processing and product status, Remote Sens. Environ., 83, 3–15, 2002.
Kaufman, Y. J., Boucher, O., Tanre, D., Chin, M., Remer, L. A., and Takemura, T.: Aerosol anthropogenic component estimated from satellite data, Geophys. Res. Lett., 32, L17804, https://doi.org/10.1029/2005gl023125, 2005.
Levy, R. C., Remer, L. A., Kleidman, R. G., Mattoo, S., Ichoku, C., Kahn, R., and Eck, T. F.: Global evaluation of the Collection 5 MODIS dark-target aerosol products over land, Atmos. Chem. Phys., 10, 10399–10420, https://doi.org/10.5194/acp-10-10399-2010, 2010.
Levy, R. C., Mattoo, S., Munchak, L. A., Remer, L. A., Sayer, A. M., Patadia, F., and Hsu, N. C.: The Collection 6 MODIS aerosol products over land and ocean, Atmos. Meas. Tech., 6, 2989–3034, https://doi.org/10.5194/amt-6-2989-2013, 2013.
Link, M. F., Zhou, Y., Taubman, B. F., Sherman, J. P., Sive, B. C., Morrow, H., Krintz, I., Robertson, L., Cook, R., Stocks, J., and West, M.: A characterization of volatile organic compounds and secondary organic aerosol at a mountain site in the southeastern United States Estimating background secondary organic aerosol in the southeastern United States from a regionally representative site, J. Atmos. Chem, 72, 81–104, https://doi.org/10.1007/s10874-015- 9305-5, 2015.
McClatchey, R. A., Fenn, R. W., Selby, J. E. A., Volz, F. E., and Garing, J. S.: Optical properties of the atmosphere, 3rd edn., AFCRL Environ. Res. Papers, 411, 108 pp., 1972.
McComiskey, A., Schwartz, S. E., Schmid, B., Guan, H., Lewis, E. R., Ricchiazzi, P., and Ogren, J. A.: Direct aerosol forcing: Calculation from observables and sensitivities to inputs, J. Geophys. Res., 113, D09202, https://doi.org/10.1029/2007JD009170, 2008.
Menne, M. J., Williams C. N., and Vose, R. S.: The US historical climatology network monthly temperature data, Version 2, B. Am. Meteorol. Soc., 90, 993–1007, 2009.
Michalsky, J. J., Anderson, G. P., Barnard, J., Delamere, J., Gueymard, C., Kato, S., Kiedron, P., McComiskey, A., and Ricchiazzi, P.: Shortwave radiative closure studies for clear skies during the Atmospheric Radiation Measurement 2003 Aerosol Intensive Observation Period, J. Geophys. Res., 111, D14S90, https://doi.org/10.1029/2005JD006341, 2006.
NOAA: APP Statistical Summary Plot Page, available at: https://www.esrl.noaa.gov/gmd/aero/net/status_plot.php?sta=app, last access: 27 February 2018.
Ogren, J. A., Wendell, J. Sheridan, P. J., Hageman, D., and Jefferson, A.: Continuous light absorption photometer performance, ASR Science Team Meeting, Potomac, MD, USA, 18–21 March 2013, available at: http://asr.science.energy.gov/meetings/stm/posters/view?id=781 (last access: 11 April 2017), 2013.
Remer, L. A., Chin, M., DeCola, P., Feingold, G., Halthore, R., Kahn, R. A., Quinn, P. K., Rind, D., Schwartz, S. E., Streets, D., and Yu, H.: Executive Summary, in: Atmospheric Aerosol Properties and Climate Impacts, A Report by the US Climate Change Science Program and the Subcommittee on Global Change Research, edited by: Chin, M., Kahn, R. A., and Schwartz, S. E., National Aeronautics and Space Administration, Washington, DC, USA, 2009.
Ricchiazzi, P., Yang, S. R., Gautier, C., and Sowle, D.: SBDART: A research and teaching software tool for plane-parallel radiative transfer in the Earth's atmosphere, B. Am. Meteorol. Soc., 79, 2101–2114, 1998.
Sheridan, P. J., Delene, D. J., and Ogren, J. A.: Four years of continuous surface aerosol measurements from the Department of Energy's Atmospheric Radiation Measurement Program Southern Great Plains Cloud and Radiation Testbed site, J. Geophys. Res., 106, 20735–20747, https://doi.org/10.1029/2001JD000785, 2001.
Sherman, J. P., Sheridan, P. J., Ogren, J. A., Andrews, E., Hageman, D., Schmeisser, L., Jefferson, A., and Sharma, S.: A multi-year study of lower tropospheric aerosol variability and systematic relationships from four North American regions, Atmos. Chem. Phys., 15, 12487–12517, https://doi.org/10.5194/acp-15-12487-2015, 2015.
Sherman, J. P., Gupta, P., Levy, R. C., and Sherman, P.: An evaluation of MODIS-retrieved aerosol optical depth over a mountainous AERONET site in the southeastern US, Aerosol Air Qual. Res., 16, 3243–3255, https://doi.org/10.4209/aaqr.2015.09.0568, 2016a.
Sherman, J. P., Link, M. F., and Zhou, Y.: Relationships amongst lower tropospheric and column-averaged aerosol properties and composition from co-located NOAA and NASA monitoring sites at Appalachian State University, NOAA ESRL Global Monitoring Annual Conference, Boulder, CO, USA, 17–18 May 2016, available at: https://www.esrl.noaa.gov/gmd/publications/annual_meetings/2016/slides/25-Sherman.pdf (last access: 11 April 2017), 2016b.
Titos, G., Cazorla, A., Zieger, P., Andrews, E., Lyamani, H., Granados-Munoz, M. J., Olmo, F. J., and Alados-Arboledas, L.: Effect of hygroscopic growth on the aerosol light-scattering coefficient: A review of measurements, techniques, and error sources, Atmos. Environ., 141, 494–507, 2016.
US Census Bureau: 2006–2010 American Community Survey, available at: http://www.census.gov/acs/www/ (last access: 3 January 2012), 2010.
Vermote, E. F. and Kotchenova, S.: Atmospheric correction for the monitoring of land surfaces, J. Geophys. Res., 113, D23590, https://doi.org/10.1029/2007JD009662, 2008.
Vermote, E. F. and Saleous, N. Z.: Operational atmospheric correction of MODIS visible to middle land surface data in the case of an infinite Lambertian target, Earth Science Satellite Remote Sensing, Volume 1: Science and Instruments, edited by: Qu, J. J., Gao, W., Kafatos, M., Murphy, R. E., and Salomonson, V. V. Chapter 8, 123–153, Springer, Berlin Heidelberg, Germany, ISBN 978-3-540-35606-6, 2006.
Welton, E. J., Campbell, J. R., Spinhirne, J. D., and Scott, V. S.: Global monitoring of clouds and aerosols using a network of micro-pulse lidar systems, in: Lidar Remote Sensing for Industry and Environmental Monitoring, edited by: Singh, U. N., Itabe, T., and Sugimoto, N., Proc. SPIE, 4153, 151–158, 2001.
Yu, H., Kaufman, Y. J., Chin, M., Feingold, G., Remer, L. A., Anderson, T. L., Balkanski, Y., Bellouin, N., Boucher, O., Christopher, S., DeCola, P., Kahn, R., Koch, D., Loeb, N., Reddy, M. S., Schulz, M., Takemura, T., and Zhou, M.: A review of measurement-based assessments of the aerosol direct radiative effect and forcing, Atmos. Chem. Phys., 6, 613–666, https://doi.org/10.5194/acp-6-613-2006, 2006.
Yu, S., Zender, C. S., and Saxena, V. K.: Direct radiative forcing and atmospheric absorption by boundary layer aerosols in the southeastern US: model estimates on the basis of new observations, Atmos. Environ., 35, 3967–3977, 2001.
Short summary
This paper highlights the first multi-year ground-based climatology of aerosol direct radiative effect (DRE) in the southeastern US Aerosol DRE at the co-located NOAA and NASA aerosol monitoring sites at Appalachian State University is approximately five times more negative during summer than winter. Aerosol DRE is most sensitive to aerosol optical depth (AOD). Use of MODIS-measured increases DRE uncertainty by a factor of 2.5 to 5.
This paper highlights the first multi-year ground-based climatology of aerosol direct radiative...
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