Articles | Volume 17, issue 14
https://doi.org/10.5194/acp-17-8999-2017
https://doi.org/10.5194/acp-17-8999-2017
Research article
 | 
27 Jul 2017
Research article |  | 27 Jul 2017

Subtropical subsidence and surface deposition of oxidized mercury produced in the free troposphere

Viral Shah and Lyatt Jaeglé

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Cited articles

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Ambrose, J. L., Gratz, L. E., Jaffe, D. A., Campos, T., Flocke, F. M., Knapp, D. J., Stechman, D. M., Stell, M., Weinheimer, A. J., Cantrell, C. A., and Mauldin, R. L.: Mercury Emission Ratios from Coal-Fired Power Plants in the Southeastern United States during NOMADSS, Environ. Sci. Technol., 49, 10389–10397, https://doi.org/10.1021/acs.est.5b01755, 2015.
Angot, H., Barret, M., Magand, O., Ramonet, M., and Dommergue, A.: A 2-year record of atmospheric mercury species at a background Southern Hemisphere station on Amsterdam Island, Atmos. Chem. Phys., 14, 11461–11473, https://doi.org/10.5194/acp-14-11461-2014, 2014.
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Short summary
We use a model of mercury chemistry and transport in the atmosphere, along with ground- and aircraft-based mercury observations, to learn that oxidized mercury chemically produced in the free troposphere descends in the subtropical anticyclones and makes up much of the mercury depositing to the Earth's surface. Our findings imply that mercury chemistry in the free troposphere and transport in the subtropics are important links between global emissions and surface deposition of mercury.
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