Articles | Volume 17, issue 22
https://doi.org/10.5194/acp-17-14055-2017
https://doi.org/10.5194/acp-17-14055-2017
Research article
 | 
24 Nov 2017
Research article |  | 24 Nov 2017

Year-round record of bulk and size-segregated aerosol composition in central Antarctica (Concordia site) – Part 2: Biogenic sulfur (sulfate and methanesulfonate) aerosol

Michel Legrand, Susanne Preunkert, Rolf Weller, Lars Zipf, Christoph Elsässer, Silke Merchel, Georg Rugel, and Dietmar Wagenbach

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Cited articles

Arimoto, R., Nottingham, A. S., Webb, J., Schloesslin, C. A., and Davis, D.: Non-sea-salt sulfate and other aerosol constituents at the South Pole during ISCAT, Geophys. Res. Lett., 28, 3645–3648, 2001.
Arimoto, R., Hogan, A., Grube, P., Davis, D., Webb, J., Schloesslin, C., Sage, S., and Raccah, F.: Major ions and radionuclides in aerosol particles from the South Pole during ISCAT-2000, Atmos. Environ., 38, 5473–5484, 2004.
Arimoto, R., Zeng, T., Davis, D., Wang, Y., Khaing, H., Nesbit, C., and Huey, G.: Concentrations and sources of aerosol ions and trace elements during ANTCI-2003, Atmos. Environ., 42, 2864–2876, https://doi.org/10.1016/j.atmosenv.2007.05.054, 2008.
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Ayers, G. P., Ivey, J. P., and Gillett, R. W.: Coherence between seasonal cycles of dimethylsulphide, methanesulphonate and sulphate in marine air, Nature, 349, 404–406, 1991.
Short summary
Levels of MSA and sulfate at inland Antarctica are documented from multiple year-round records of bulk and size-segregated aerosol samplings. A striking difference in the seasonality of sulfur aerosol composition, characterized by a MSA to nssSO4 ratio reaching a minimum in summer over the Antarctic plateau (0.05) and a maximum at the coast (up to 0.40), is clearly established. An efficient chemical destruction of MSA is suggested to take place over the Antarctic plateau in summer.
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