Articles | Volume 14, issue 24
Atmos. Chem. Phys., 14, 13601–13629, 2014
Atmos. Chem. Phys., 14, 13601–13629, 2014
Research article
19 Dec 2014
Research article | 19 Dec 2014

A physically based framework for modeling the organic fractionation of sea spray aerosol from bubble film Langmuir equilibria

S. M. Burrows et al.

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Cited articles

Adamson, A. W. and Gast, A. P.: Physical chemistry of surfaces, Wiley Interscience, New York, 808 pp., 1997.
Albert, M. F. M. A., Schaap, M., Manders, A. M. M., Scannell, C., O'Dowd, C. D., and de Leeuw, G.: Uncertainties in the determination of global sub-micron marine organic matter emissions, Atmos. Environ., 57, 289–300, 2012.
Alexander, D. M., Barnes, G. T., McGregor, M. A., and Walker, K.: The penetration of monolayers by surfactants, edited by: Scamehorn, J., in: vol. 311 of ACS Symposium Series, chap. 10, 133–142, American Chemical Society, Washington, DC,, 1986.
Amon, R. M. W. and Benner, R.: Bacterial utilization of different size classes of dissolved organic matter, Limnol. Oceanogr., 41, 41–51, 1996.
Armstrong, R. A., Lee, C., Hedges, J. I., Honjo, S., and Wakeham, S. G.: A new, mechanistic model for organic carbon fluxes in the ocean based on the quantitative association of POC with ballast minerals, Deep Sea Research Part II: Topical Studies in Oceanography, 49, 219–236, 2001.
Short summary
The air over the ocean is full of sea spray particles ejected by bubbles that burst in the wake of breaking waves. The smallest of such particles, less than a micrometer in diameter, include organic matter derived from ocean biota. This paper introduces a method to calculate the chemical composition of spray particles. Ocean organic matter is divided into several classes using a global model. Basic chemistry relationships predict the amount of organic material in emitted spray.
Final-revised paper