Articles | Volume 10, issue 23
Atmos. Chem. Phys., 10, 11955–11968, 2010
© Author(s) 2010. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Special issue: ICIS-2007
Research article 15 Dec 2010
Research article | 15 Dec 2010
Laboratory investigations of the impact of mineral dust aerosol on cold cloud formation
K. A. Koehler et al.
Related subject area
Subject: Clouds and Precipitation | Research Activity: Laboratory Studies | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)Application of holography and automated image processing for laboratory experiments on mass and fall speed of small cloud ice crystalsReview of experimental studies of secondary ice productionExploratory experiments on pre-activated freezing nucleation on mercuric iodideThe role of contact angle and pore width on pore condensation and freezingComparative Study On Immersion Freezing Utilizing Single Droplet Levitation MethodsTechnical note: Equilibrium droplet size distributions in a turbulent cloud chamber with uniform supersaturationProtein aggregates nucleate ice: the example of apoferritinNo anomalous supersaturation in ultracold cirrus laboratory experimentsLateral facet growth of ice and snow – Part 1: Observations and applications to secondary habitsThe ice-nucleating ability of quartz immersed in water and its atmospheric importance compared to K-feldsparIce nucleation properties of K-feldspar polymorphs and plagioclase feldsparsEnhanced ice nucleation activity of coal fly ash aerosol particles initiated by ice-filled poresA comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in waterActivation of intact bacteria and bacterial fragments mixed with agar as cloud droplets and ice crystals in cloud chamber experimentsAnomalous holiday precipitation over southern ChinaCoal fly ash: linking immersion freezing behavior and physicochemical particle propertiesSurface roughness during depositional growth and sublimation of ice crystalsIce nucleation abilities of soot particles determined with the Horizontal Ice Nucleation ChamberThe efficiency of secondary organic aerosol particles acting as ice-nucleating particles under mixed-phase cloud conditionsUncertainty in counting ice nucleating particles with continuous flow diffusion chambersExperimental evidence of the rear capture of aerosol particles by raindropsRefreeze experiments with water droplets containing different types of ice nuclei interpreted by classical nucleation theoryPre-activation of aerosol particles by ice preserved in poresHeterogeneous ice nucleation on dust particles sourced from nine deserts worldwide – Part 1: Immersion freezingA comparative study of K-rich and Na/Ca-rich feldspar ice-nucleating particles in a nanoliter droplet freezing assayIce nucleation efficiency of AgI: review and new insightsThe adsorption of fungal ice-nucleating proteins on mineral dusts: a terrestrial reservoir of atmospheric ice-nucleating particlesExploring an approximation for the homogeneous freezing temperature of water dropletsCloud chamber experiments on the origin of ice crystal complexity in cirrus cloudsPhase transition observations and discrimination of small cloud particles by light polarization in expansion chamber experimentsAnalysis of isothermal and cooling-rate-dependent immersion freezing by a unifying stochastic ice nucleation modelPre-activation of ice-nucleating particles by the pore condensation and freezing mechanismInfluence of the ambient humidity on the concentration of natural deposition-mode ice-nucleating particlesComparison of measured and calculated collision efficiencies at low temperaturesInvestigating the discrepancy between wet-suspension- and dry-dispersion-derived ice nucleation efficiency of mineral particlesTechnical Note: A proposal for ice nucleation terminologyLaboratory studies of collection efficiency of sub-micrometer aerosol particles by cloud droplets on a single-droplet basisIce nucleation by combustion ash particles at conditions relevant to mixed-phase cloudsA new temperature- and humidity-dependent surface site density approach for deposition ice nucleationDeposition-mode ice nucleation reexamined at temperatures below 200 KMesoscopic surface roughness of ice crystals pervasive across a wide range of ice crystal conditionsInterpretation of freezing nucleation experiments: singular and stochastic; sites and surfacesDeposition nucleation viewed as homogeneous or immersion freezing in pores and cavitiesIce nucleation by fertile soil dusts: relative importance of mineral and biogenic componentsFeldspar minerals as efficient deposition ice nucleiImmersion freezing of birch pollen washing waterContact freezing: a review of experimental studiesGeneralisation of Levine's prediction for the distribution of freezing temperatures of droplets: a general singular model for ice nucleationImmersion freezing of ice nucleation active protein complexesState transformations and ice nucleation in amorphous (semi-)solid organic aerosol
Maximilian Weitzel, Subir K. Mitra, Miklós Szakáll, Jacob P. Fugal, and Stephan Borrmann
Atmos. Chem. Phys., 20, 14889–14901,Short summary
The properties of ice crystals smaller than 150 µm in diameter were investigated in a cold-room laboratory using digital holography and microscopy. Automated image processing has been used to determine the track of falling ice crystals, and collected crystals were melted and scanned under a microscope to infer particle mass. A parameterization relating particle size and mass was determined which describes ice crystals in this size range more accurately than existing relationships.
Alexei Korolev and Thomas Leisner
Atmos. Chem. Phys., 20, 11767–11797,Short summary
Secondary ice production (SIP) plays a key role in the formation of ice particles in tropospheric clouds. This work presents a critical review of the laboratory studies related to secondary ice production. It aims to identify gaps in our knowledge of SIP as well as to stimulate further laboratory studies focused on obtaining a quantitative description of efficiencies for each SIP mechanism.
Atmos. Chem. Phys. Discuss.,
Revised manuscript accepted for ACPShort summary
The freezing of water drops in clouds is the prime example for the role of ice nucleating particles (INPs). Mercuric iodide particles and a few other substances can be conditioned to become very effective INPs after previous ice formation opening a new pathway to ice formation in the atmosphere and in other systems like tissue preservation artificial snow making and more.
Robert O. David, Jonas Fahrni, Claudia Marcolli, Fabian Mahrt, Dominik Brühwiler, and Zamin A. Kanji
Atmos. Chem. Phys., 20, 9419–9440,Short summary
Ice crystal formation plays an important role in controlling the Earth's climate. However, the mechanisms responsible for ice formation in the atmosphere are still uncertain. Here we use surrogates for atmospherically relevant porous particles to determine the role of pore diameter and wettability on the ability of porous particles to nucleate ice in the atmosphere. Our results are consistent with the pore condensation and freeing mechanism.
Miklós Szakáll, Michael Debertshäuser, Christian Philipp Lackner, Amelie Mayer, Oliver Eppers, Karoline Diehl, Alexander Theis, Subir Kumar Mitra, and Stephan Borrmann
Atmos. Chem. Phys. Discuss.,
Revised manuscript accepted for ACPShort summary
A comparative study of the immersion freezing abilities of different aerosol types utilizing the Mainz vertical Wind Tunnel and the Mainz Acoustic Levitator is presented. We show that the freezing temperature of droplets containing the aerosols depends on the employed cooling rate of the instrument and the aerosol material. This finding is important not only for the intercomparison of ice nucleation instruments but also for cloud model simulations with high speed ascents of air masses.
Steven K. Krueger
Atmos. Chem. Phys., 20, 7895–7909,Short summary
When CCN are injected into a turbulent cloud chamber at a constant rate, and the rate of droplet activation is balanced by the rate of droplet fallout, a steady-state droplet size distribution (DSD) can be achieved. Analytic DSDs and PDFs of droplet radius were derived for such conditions when there is uniform supersaturation. Given the chamber height, the analytic PDF is determined by the supersaturation alone. This could allow one to infer the supersaturation that produced a measured PDF.
María Cascajo-Castresana, Robert O. David, Maiara A. Iriarte-Alonso, Alexander M. Bittner, and Claudia Marcolli
Atmos. Chem. Phys., 20, 3291–3315,Short summary
Atmospheric ice-nucleating particles are rare but relevant for cloud glaciation. A source of particles that nucleate ice above −15 °C is biological material including some proteins. Here we show that proteins of very diverse functions and structures can nucleate ice. Among these, the iron storage protein apoferritin stands out, with activity up to −4 °C. We show that its activity does not stem from correctly assembled proteins but from misfolded protein monomers or oligomers and aggregates.
Benjamin W. Clouser, Kara D. Lamb, Laszlo C. Sarkozy, Jan Habig, Volker Ebert, Harald Saathoff, Ottmar Möhler, and Elisabeth J. Moyer
Atmos. Chem. Phys., 20, 1089–1103,Short summary
Previous measurements of water vapor in the upper troposphere and lower stratosphere (UT/LS) have shown unexpectedly high concentrations of water vapor in ice clouds, which may be due to an incomplete understanding of the structure of ice and the behavior of ice growth in this part of the atmosphere. Water vapor measurements during the 2013 IsoCloud campaign at the AIDA cloud chamber show no evidence of this
anomalous supersaturationin conditions similar to the real atmosphere.
Jon Nelson and Brian D. Swanson
Atmos. Chem. Phys., 19, 15285–15320,Short summary
Ice crystals in clouds have a wide variety. But many crystal forms are inexplicable using the common approach of modeling the growth rates normal to the crystal faces. Instead of using only this normal-growth approach, we suggest including lateral facet growth processes. Using such lateral processes, backed up by new experiments, we give explanations for some of these puzzling forms. The forms include the center droxtal in stellar crystals, scrolls, capped columns, sheath bundles, and trigonals.
Alexander D. Harrison, Katherine Lever, Alberto Sanchez-Marroquin, Mark A. Holden, Thomas F. Whale, Mark D. Tarn, James B. McQuaid, and Benjamin J. Murray
Atmos. Chem. Phys., 19, 11343–11361,Short summary
Mineral dusts are a source of ice-nucleating particles (INPs) in the atmosphere. Here we present a comprehensive survey of the ice-nucleating ability of naturally occurring quartz. We show the ice-nucleating variability of quartz and its sensitivity to time spent in water and air. We propose four new parameterizations for the minerals quartz, K feldspar, albite and plagioclase to predict INP concentrations in the atmosphere and show that K-feldspar is the dominant INP type in mineral dusts.
André Welti, Ulrike Lohmann, and Zamin A. Kanji
Atmos. Chem. Phys., 19, 10901–10918,Short summary
The ice nucleation ability of singly immersed feldspar particles in suspended water droplets relevant for ice crystal formation under mixed-phase cloud conditions is presented. The effects of particle size, crystal structure, trace metal and mineralogical composition are discussed by testing up to five different diameters in the submicron range and nine different feldspar samples at conditions relevant for ice nucleation in mixed-phase clouds.
Nsikanabasi Silas Umo, Robert Wagner, Romy Ullrich, Alexei Kiselev, Harald Saathoff, Peter G. Weidler, Daniel J. Cziczo, Thomas Leisner, and Ottmar Möhler
Atmos. Chem. Phys., 19, 8783–8800,Short summary
Annually, over 600 Tg of coal fly ash (CFA) is produced; a significant proportion of this amount is injected into the atmosphere, which could significantly contribute to heterogeneous ice formation in clouds. This study presents an improved understanding of CFA particles' behaviour in forming ice in clouds, especially when exposed to lower temperatures before being re-circulated in the upper troposphere or entrained into the lower troposphere.
Naruki Hiranuma, Kouji Adachi, David M. Bell, Franco Belosi, Hassan Beydoun, Bhaskar Bhaduri, Heinz Bingemer, Carsten Budke, Hans-Christian Clemen, Franz Conen, Kimberly M. Cory, Joachim Curtius, Paul J. DeMott, Oliver Eppers, Sarah Grawe, Susan Hartmann, Nadine Hoffmann, Kristina Höhler, Evelyn Jantsch, Alexei Kiselev, Thomas Koop, Gourihar Kulkarni, Amelie Mayer, Masataka Murakami, Benjamin J. Murray, Alessia Nicosia, Markus D. Petters, Matteo Piazza, Michael Polen, Naama Reicher, Yinon Rudich, Atsushi Saito, Gianni Santachiara, Thea Schiebel, Gregg P. Schill, Johannes Schneider, Lior Segev, Emiliano Stopelli, Ryan C. Sullivan, Kaitlyn Suski, Miklós Szakáll, Takuya Tajiri, Hans Taylor, Yutaka Tobo, Romy Ullrich, Daniel Weber, Heike Wex, Thomas F. Whale, Craig L. Whiteside, Katsuya Yamashita, Alla Zelenyuk, and Ottmar Möhler
Atmos. Chem. Phys., 19, 4823–4849,Short summary
A total of 20 ice nucleation measurement techniques contributed to investigate the immersion freezing behavior of cellulose particles – natural polymers. Our data showed several types of cellulose are able to nucleate ice as efficiently as some mineral dust samples and cellulose has the potential to be an important atmospheric ice-nucleating particle. Continued investigation/collaboration is necessary to obtain further insight into consistency or diversity of ice nucleation measurements.
Kaitlyn J. Suski, David M. Bell, Naruki Hiranuma, Ottmar Möhler, Dan Imre, and Alla Zelenyuk
Atmos. Chem. Phys., 18, 17497–17513,Short summary
This work investigates the cloud condensation nuclei and ice nucleation activity of bacteria using cloud chamber data and a single particle mass spectrometer. The size and chemical composition of the cloud residuals show that bacterial fragments mixed with agar growth media activate preferentially over intact bacteria cells as cloud condensation nuclei. Intact bacteria cells do not make it into cloud droplets; they thus cannot serve as immersion-mode ice nucleating particles.
Jiahui Zhang, Dao-Yi Gong, Rui Mao, Jing Yang, Ziyin Zhang, and Yun Qian
Atmos. Chem. Phys., 18, 16775–16791,Short summary
The Chinese Spring Festival (also known as the Chinese New Year or Lunar New Year) is the most important festival in China. This paper reports that during the Chinese Spring Festival, the precipitation over southern China has been significantly reduced. The precipitation reduction is due to anomalous northerly winds. We suppose that anomalous atmospheric circulation is likely related to the human activity during holidays. It is an interesting phenomenon.
Sarah Grawe, Stefanie Augustin-Bauditz, Hans-Christian Clemen, Martin Ebert, Stine Eriksen Hammer, Jasmin Lubitz, Naama Reicher, Yinon Rudich, Johannes Schneider, Robert Staacke, Frank Stratmann, André Welti, and Heike Wex
Atmos. Chem. Phys., 18, 13903–13923,Short summary
In this study, coal fly ash particles immersed in supercooled cloud droplets were analyzed concerning their freezing behavior. Additionally, physico-chemical particle properties (morphology, chemical composition, crystallography) were investigated. In combining both aspects, components that potentially contribute to the observed freezing behavior of the ash could be identified. Interactions at the particle-water interface, that depend on suspension time and influence freezing, are discussed.
Jens Voigtländer, Cedric Chou, Henner Bieligk, Tina Clauss, Susan Hartmann, Paul Herenz, Dennis Niedermeier, Georg Ritter, Frank Stratmann, and Zbigniew Ulanowski
Atmos. Chem. Phys., 18, 13687–13702,Short summary
Surface roughness of ice crystals has recently been acknowledged to strongly influence the radiative properties of cold clouds such as cirrus, but it is unclear how this roughness arises. The study investigates the origins of ice surface roughness under a variety of atmospherically relevant conditions, using a novel method to measure roughness quantitatively. It is found that faster growth leads to stronger roughness. Roughness also increases following repeated growth–sublimation cycles.
Fabian Mahrt, Claudia Marcolli, Robert O. David, Philippe Grönquist, Eszter J. Barthazy Meier, Ulrike Lohmann, and Zamin A. Kanji
Atmos. Chem. Phys., 18, 13363–13392,Short summary
The ice nucleation ability of different soot particles in the cirrus and mixed-phase cloud temperature regime is presented. The impact of aerosol particle size, particle morphology, organic matter and hydrophilicity on ice nucleation is examined. We propose ice nucleation proceeds via a pore condensation freezing mechanism for soot particles with the necessary physicochemical properties that nucleated ice well below water saturation.
Wiebke Frey, Dawei Hu, James Dorsey, M. Rami Alfarra, Aki Pajunoja, Annele Virtanen, Paul Connolly, and Gordon McFiggans
Atmos. Chem. Phys., 18, 9393–9409,Short summary
The coupled system of the Manchester Aerosol Chamber and Manchester Ice Cloud Chamber was used to study the ice-forming abilities of secondary organic aerosol particles under mixed-phase cloud conditions. Given the vast abundance of secondary organic particles in the atmosphere, they might present an important contribution to ice-nucleating particles. However, we find that in the studied temperature range (20 to 28 °C) the secondary organic particles do not nucleate ice particles.
Sarvesh Garimella, Daniel A. Rothenberg, Martin J. Wolf, Robert O. David, Zamin A. Kanji, Chien Wang, Michael Rösch, and Daniel J. Cziczo
Atmos. Chem. Phys., 17, 10855–10864,Short summary
This study investigates systematic and variable low bias in the measurement of ice nucleating particle concentration using continuous flow diffusion chambers. We find that non-ideal instrument behavior exposes particles to different humidities and/or temperatures than predicted from theory. We use a machine learning approach to quantify and minimize the uncertainty associated with this measurement bias.
Pascal Lemaitre, Arnaud Querel, Marie Monier, Thibault Menard, Emmanuel Porcheron, and Andrea I. Flossmann
Atmos. Chem. Phys., 17, 4159–4176,Short summary
We present new measurements of the efficiency with which aerosol particles are collected by raindrops. These measurements provide the link to reconcile the scavenging coefficients obtained from theoretical approaches with those from experimental studies. We provide proof of the rear capture that is a fundamental effect on submicroscopic particles. Finally, we propose an expression to take into account this mechanism to calculate the collection efficiency for drops within the rain size range.
Lukas Kaufmann, Claudia Marcolli, Beiping Luo, and Thomas Peter
Atmos. Chem. Phys., 17, 3525–3552,Short summary
To improve the understanding of heterogeneous ice nucleation, we have subjected different ice nuclei to repeated freezing cycles and evaluated the freezing temperatures with different parameterizations of classical nucleation theory. It was found that two fit parameters were necessary to describe the temperature dependence of the nucleation rate.
Atmos. Chem. Phys., 17, 1595–1622,Short summary
Laboratory studies from the last century have shown that some types of particles are susceptible to pre-activation, i.e. they are able to develop macroscopic ice at warmer temperatures or lower relative humidities after they had been involved in an ice nucleation event before. This review analyses these works under the presumption that pre-activation occurs by ice preserved in pores, and it discusses atmospheric scenarios for which pre-activation might be important.
Yvonne Boose, André Welti, James Atkinson, Fabiola Ramelli, Anja Danielczok, Heinz G. Bingemer, Michael Plötze, Berko Sierau, Zamin A. Kanji, and Ulrike Lohmann
Atmos. Chem. Phys., 16, 15075–15095,Short summary
We compare the immersion freezing behavior of four airborne to 11 surface-collected dust samples to investigate the role of different minerals for atmospheric ice nucleation on desert dust. We find that present K-feldspars dominate at T > 253 K, while quartz does at colder temperatures, and surface-collected dust samples are not necessarily representative for airborne dust. For improved ice cloud prediction, modeling of quartz and feldspar emission and transport are key.
Andreas Peckhaus, Alexei Kiselev, Thibault Hiron, Martin Ebert, and Thomas Leisner
Atmos. Chem. Phys., 16, 11477–11496,Short summary
The precipitation in midlatitude clouds proceeds predominantly via nucleation of ice in the supercooled droplets containing foreign inclusions, like feldspar mineral dust, that have been recently identified as one of the most active ice nucleating agents in the atmosphere. We have built an apparatus to observe the freezing of feldspar immersed in up to 1500 identical droplets simultaneously. With this setup we investigated four feldspar samples and show that it can induce freezing at −5 °C.
Claudia Marcolli, Baban Nagare, André Welti, and Ulrike Lohmann
Atmos. Chem. Phys., 16, 8915–8937,Short summary
Silver iodide is one of the best-investigated ice nuclei. It has relevance for the atmosphere since it is used for glaciogenic cloud seeding. Nevertheless, many open questions remain. This paper gives an overview of silver iodide as an ice nucleus and tries to identify the factors that influence the ice nucleation ability of silver iodide.
Daniel O'Sullivan, Benjamin J. Murray, James F. Ross, and Michael E. Webb
Atmos. Chem. Phys., 16, 7879–7887,Short summary
In the absence of particles which can trigger freezing, cloud droplets can exist in a supercooled liquid state well below the melting point. However, the sources of efficient ice-nucleating particles in the atmosphere are uncertain. Here we show that ice-nucleating proteins produced by soil fungi can bind to clay particles in soils. Hence, the subsequent dispersion of soil particles into the atmosphere acts as a route through which biological ice nucleators can influence clouds.
Kuan-Ting O and Robert Wood
Atmos. Chem. Phys., 16, 7239–7249,Short summary
In this work, based on the well-known formulae of classical nucleation theory (CNT), the temperature at which the mean number of critical embryos inside a droplet is unity is derived from the Boltzmann distribution function and explored as a new simplified approximation for homogeneous freezing temperature. It thus appears that the simplicity of this approximation makes it potentially useful for predicting homogeneous freezing temperatures of water droplets in the atmosphere.
Martin Schnaiter, Emma Järvinen, Paul Vochezer, Ahmed Abdelmonem, Robert Wagner, Olivier Jourdan, Guillaume Mioche, Valery N. Shcherbakov, Carl G. Schmitt, Ugo Tricoli, Zbigniew Ulanowski, and Andrew J. Heymsfield
Atmos. Chem. Phys., 16, 5091–5110,
Leonid Nichman, Claudia Fuchs, Emma Järvinen, Karoliina Ignatius, Niko Florian Höppel, Antonio Dias, Martin Heinritzi, Mario Simon, Jasmin Tröstl, Andrea Christine Wagner, Robert Wagner, Christina Williamson, Chao Yan, Paul James Connolly, James Robert Dorsey, Jonathan Duplissy, Sebastian Ehrhart, Carla Frege, Hamish Gordon, Christopher Robert Hoyle, Thomas Bjerring Kristensen, Gerhard Steiner, Neil McPherson Donahue, Richard Flagan, Martin William Gallagher, Jasper Kirkby, Ottmar Möhler, Harald Saathoff, Martin Schnaiter, Frank Stratmann, and António Tomé
Atmos. Chem. Phys., 16, 3651–3664,Short summary
Processes in the atmosphere are often governed by the physical and chemical properties of small cloud particles. Ice, water, and mixed clouds, as well as viscous aerosols, were formed under controlled conditions at the CLOUD-CERN facility. The experimental results show a link between cloud particle properties and their unique optical fingerprints. The classification map presented here allows easier discrimination between various particles such as viscous organic aerosol, salt, ice, and liquid.
Peter A. Alpert and Daniel A. Knopf
Atmos. Chem. Phys., 16, 2083–2107,Short summary
A stochastic immersion freezing model is introduced capable of reproducing laboratory data for a variety of experimental methods using a time and surface area dependent ice nucleation process. The assumption that droplets contain identical surface area is evaluated. A quantitative uncertainty analysis of the laboratory observed freezing process is presented. Our results imply that ice nuclei surface area assumptions are crucial for interpretation of experimental immersion freezing results.
Robert Wagner, Alexei Kiselev, Ottmar Möhler, Harald Saathoff, and Isabelle Steinke
Atmos. Chem. Phys., 16, 2025–2042,Short summary
We have investigated the enhancement of the ice nucleation ability of well-known and abundant ice nucleating particles like dust grains due to pre-activation. Temporary exposure to a low temperature (228 K) provokes that pores and surface cracks of the particles are filled with ice, which makes them better nuclei for the growth of macroscopic ice crystals at high temperatures (245–260 K).
M. L. López and E. E. Ávila
Atmos. Chem. Phys., 16, 927–932,Short summary
This work deals with the origin and nature of atmospheric ice-nucleating particles (INPs). An accurate determination of the atmospheric INP concentration is relevant since INPs induce freezing in clouds, thus initiating an efficient mechanism for cloud particles to reach a precipitating size. The effect of relative humidity on the INP concentration at ground level was analyzed and discussed.
B. Nagare, C. Marcolli, O. Stetzer, and U. Lohmann
Atmos. Chem. Phys., 15, 13759–13776,Short summary
We determined collision efficiencies of cloud droplets with aerosol particles experimentally and found that they were around 1 order of magnitude higher than theoretical formulations that include Brownian diffusion, impaction, interception, thermophoretic, diffusiophoretic and electric forces. This is most probably due to uncertainties and inaccuracies in the theoretical formulations of thermophoretic and diffusiophoretic processes.
C. Emersic, P. J. Connolly, S. Boult, M. Campana, and Z. Li
Atmos. Chem. Phys., 15, 11311–11326,
G. Vali, P. J. DeMott, O. Möhler, and T. F. Whale
Atmos. Chem. Phys., 15, 10263–10270,Short summary
Clarification is needed in the terminology used to discuss ice nucleation in the literature. Conflicting interpretations coupled with uncertainties about the details of the processes have led to difficulties in the clear communication of results and ideas. This paper contains a proposal for future usage. This proposed terminology was arrived at as a result of a year-long exchange of suggestions by a number of scientists.
K. Ardon-Dryer, Y.-W. Huang, and D. J. Cziczo
Atmos. Chem. Phys., 15, 9159–9171,Short summary
The collection between aerosol and a water droplet is an important mechanism for removing particles from the atmosphere, and has an influence on cloud dynamics, precipitation processes and cloud lifetime. In this experiment, the collection process was studied on a single-droplet basis, with atmospherically relevant conditions (droplet sizes, charges and flow). Collection efficiency values were found to be in agreement with previous experimental and theoretical studies.
N. S. Umo, B. J. Murray, M. T. Baeza-Romero, J. M. Jones, A. R. Lea-Langton, T. L. Malkin, D. O'Sullivan, L. Neve, J. M. C. Plane, and A. Williams
Atmos. Chem. Phys., 15, 5195–5210,Short summary
Combustion ash particles nucleate ice in the immersion mode at conditions relevant to mixed-phase clouds. Hence, combustion ashes could play an important role in primary ice formation in mixed-phase clouds, especially in clouds that are formed near the emission source of these aerosol particles. From this study, there is a need to quantify the atmospheric abundance of combustion ashes in order to quantitatively assess the impact of combustion ashes on mixed-phase clouds.
I. Steinke, C. Hoose, O. Möhler, P. Connolly, and T. Leisner
Atmos. Chem. Phys., 15, 3703–3717,Short summary
Ice nucleation in clouds has a significant influence on the global radiative budget and the hydrological cycle. Several studies have investigated the ice formation in droplets and parameterizations have been developed in order to include immersion freezing in climate models. In contrast, there are fewer studies regarding the conversion of water vapor into ice (so-called deposition nucleation) which is the topic of this paper which investigates deposition nucleation by Arizona Test dust in detail
E. S. Thomson, X. Kong, P. Papagiannakopoulos, and J. B. C. Pettersson
Atmos. Chem. Phys., 15, 1621–1632,Short summary
We present new observations of ice nucleation on substrate surfaces that affirm the ``puzzle'' of very high supersaturations required for nucleation from the vapor phase. To explain the observations, the kinetics and thermodynamics of nucleation theory are explored. The results explicitly connect the nucleation to the substrate material's surface binding energy and demonstrate that an improved fundamental understanding must include a strict understanding of the relevant microphysics.
N. B. Magee, A. Miller, M. Amaral, and A. Cumiskey
Atmos. Chem. Phys., 14, 12357–12371,Short summary
High-resolution images of ice crystals acquired by environmental scanning electron microscope reveal a wide array of surface complexities at scales from 100 nm to greater than 10 microns. These observations include ice crystals grown in the low-pressure microscope chamber and crystals grown externally under cirrus cloud conditions and then transferred for imaging. The results suggest that accounting for microscale complexity is critical for understanding cirrus interactions with radiation.
Atmos. Chem. Phys., 14, 5271–5294,
Atmos. Chem. Phys., 14, 2071–2104,
D. O'Sullivan, B. J. Murray, T. L. Malkin, T. F. Whale, N. S. Umo, J. D. Atkinson, H. C. Price, K. J. Baustian, J. Browse, and M. E. Webb
Atmos. Chem. Phys., 14, 1853–1867,
J. D. Yakobi-Hancock, L. A. Ladino, and J. P. D. Abbatt
Atmos. Chem. Phys., 13, 11175–11185,
S. Augustin, H. Wex, D. Niedermeier, B. Pummer, H. Grothe, S. Hartmann, L. Tomsche, T. Clauss, J. Voigtländer, K. Ignatius, and F. Stratmann
Atmos. Chem. Phys., 13, 10989–11003,
L. A. Ladino Moreno, O. Stetzer, and U. Lohmann
Atmos. Chem. Phys., 13, 9745–9769,
R. P. Sear
Atmos. Chem. Phys., 13, 7215–7223,
S. Hartmann, S. Augustin, T. Clauss, H. Wex, T. Šantl-Temkiv, J. Voigtländer, D. Niedermeier, and F. Stratmann
Atmos. Chem. Phys., 13, 5751–5766,
K. J. Baustian, M. E. Wise, E. J. Jensen, G. P. Schill, M. A. Freedman, and M. A. Tolbert
Atmos. Chem. Phys., 13, 5615–5628,
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