Articles | Volume 26, issue 10
https://doi.org/10.5194/acp-26-6929-2026
© Author(s) 2026. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-26-6929-2026
© Author(s) 2026. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Measurement report
| 
22 May 2026
Measurement report |
| 22 May 2026
| 22 May 2026
Measurement report: Insights into the high temporal variability of atmospheric carbon dioxide (CO2) at a suburban station in the Indo-Gangetic Plain
Vimal Jose Vazhathara
CORRESPONDING AUTHOR
Centre for Atmospheric Sciences, Indian Institute of Technology Delhi, New Delhi, India
Ravi Kumar Kunchala
Centre for Atmospheric Sciences, Indian Institute of Technology Delhi, New Delhi, India
Sajeev Philip
Centre for Atmospheric Sciences, Indian Institute of Technology Delhi, New Delhi, India
Jaswant Rathore
Centre for Atmospheric Sciences, Indian Institute of Technology Delhi, New Delhi, India
Dilip Ganguly
Centre for Atmospheric Sciences, Indian Institute of Technology Delhi, New Delhi, India
Sagnik Dey
Centre for Atmospheric Sciences, Indian Institute of Technology Delhi, New Delhi, India
Centre of Excellence for Research on Clean Air, Indian Institute of Technology Delhi, New Delhi, India
Tomoki Nakayama
Graduate School of Integrated Science and Technology, Nagasaki University, 1–14 Bunkyo-machi, Nagasaki, Nagasaki, 852–8521, Japan
Yutaka Matsumi
Research Institute for Humanity and Nature, Kyoto, Japan
Institute for Space-Earth Environmental Research, Nagoya University, Nagoya, Japan
Prabir K. Patra
Research Institute for Humanity and Nature, Kyoto, Japan
Japan Agency for Marine-Earth Science and Technology (JAMSTEC), Yokohama, Japan
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Christopher R. Oxford, Haihui Zhu, Maya Mehrotra, Xuan Liu, Yuxuan Ren, Maya Arnott, Isaac Abionum Adimula, Taiye Benjamin Ajibolataiye, Clement Akoshile, Omar Amador-Munoz, Araya Asfaw, Rachel Ying-Wen Chang, Sagnik Dey, Ann M. Dillner, David J. Diner, Connor J. Flynn, Diana Francis, Paterne Gahungu, Rebecca M. Garland, Michel Grutter, Sina Hasheminassab, Fahad Imam, Jhoon Kim, Kristy Langerman, Pei-Chen Lee, Puji Lestari, Po-Hsiung Lin, S. Marcela Loria-Salazar, Tesfaye Mamo, Olga L. Mayol-Bracero, Mogesh Naidoo, Narendra Nelli, Sang Seo Park, Abdus Salam, Bighnaraj Sarangi, Trailokya Saud, Robyn Schofield, Yoav Schechner, Sachchida N. Tripathi, Emily K. West, Eli Windwer, Ming-Tsang Wu, Qiang Zhang, Michael Brauer, Yinon Rudich, Jay R. Turner, and Randall V. Martin
EGUsphere, https://doi.org/10.5194/egusphere-2026-3224, https://doi.org/10.5194/egusphere-2026-3224, 2026
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
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A high-sensitivity balance, controlled temperature and relative humidity chamber, and filter samples collected around the world were used to develop a mass as a function of relative humidity relationship. We subsequently measured the chemical composition of these same samples. A relationship between the chemical composition and water mass was created and used to calculate aerosol water content showing how composition and water content varies worldwide.
Gaurav K. Srivastav, Aasif A. Wagay, Janne Lampilahti, Jaswant Rathore, Ravi K. Kunchala, Dilip Ganguly, Markku Kulmala, Tuukka Petäjä, Pauli Paasonen, Roseline C. Thakur, and Shahzad Gani
EGUsphere, https://doi.org/10.5194/egusphere-2026-2212, https://doi.org/10.5194/egusphere-2026-2212, 2026
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Particle formation events affect climate and air quality. Using measurements of particle number concentrations down to very small particles (~3 nm) in polluted northern India, we show that these events occur frequently in summer under reduced background particle load. However, in this environment, emissions and changing air masses can mask or distort these events, making them difficult to detect. Such environments require adaptation of standard analytical methods used in cleaner regions.
Mengze Li, Robert B. Jackson, Marielle Saunois, Philippe Ciais, Ben Poulter, Josep G. Canadell, Prabir K. Patra, Hanqin Tian, Zhen Zhang, Etienne Fluet-Chouinard, Zutao Ouyang, Ting Zhang, David J. Beerling, Dmitry A. Belikov, Philippe Bousquet, Danilo Custodio, Naveen Chandra, Xinyu Dou, Nicola Gedney, Peter O. Hopcroft, Alison M. Hoyt, Kazuhito Ichii, Akihito Ito, Atul K. Jain, Katherine Jensen, Fortunat Joos, Thomas Kleinen, Masayuki Kondo, Fa Li, Tingting Li, Xiangyu Liu, Shamil Maksyutov, Avni Malhotra, Adrien Martinez, Kyle McDonald, Joe R. Melton, Jurek Müller, Yosuke Niwa, Shufen Pan, Shushi Peng, Changhui Peng, Zhangcai Qin, Peter Raymond, William Riley, Arjo Segers, Rona L. Thompson, Aki Tsuruta, Yi Xi, Kunxiaojia Yuan, Wenxin Zhang, Bo Zheng, Qing Zhu, Qiuan Zhu, and Qianlai Zhuang
Earth Syst. Sci. Data, 18, 3507–3524, https://doi.org/10.5194/essd-18-3507-2026, https://doi.org/10.5194/essd-18-3507-2026, 2026
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We proposed a framework that combines machine-learning and climate data to predict global natural vegetated wetland methane emissions for 2000–2025. We found that although total global emissions remained stable in the post-2020s, Northern Hemisphere emissions surged whilst tropical emissions fell. This approach allows us to rapidly monitor emissions and provides early warnings for climate impacts.
Vasu Singh, Dilip Ganguly, Jaswant Rathore, Lokesh Kumar Sahu, Ravi K. Kunchala, and Sagnik Dey
EGUsphere, https://doi.org/10.5194/egusphere-2026-1428, https://doi.org/10.5194/egusphere-2026-1428, 2026
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Each post-monsoon season, northern India faces severe air pollution, especially around Delhi, largely linked to crop residue burning and stagnant weather. We measured air pollution in Sonipat, northwest of Delhi, along the pathway of incoming smoke. Fine particle levels were extremely high and mainly made of carbon-rich particles from crop burning and solid fuels. Much of this pollution formed before reaching Delhi, showing regional sources drive the city’s severe haze.
Yuming Jin, Britton B. Stephens, Matthew C. Long, Naveen Chandra, Frédéric Chevallier, Joram J. D. Hooghiem, Ingrid T. Luijkx, Shamil Maksyutov, Eric J. Morgan, Yosuke Niwa, Prabir K. Patra, Christian Rödenbeck, and Jesse Vance
Geosci. Model Dev., 18, 5937–5969, https://doi.org/10.5194/gmd-18-5937-2025, https://doi.org/10.5194/gmd-18-5937-2025, 2025
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We carry out a comprehensive atmospheric transport model (ATM) intercomparison project. This project aims to evaluate errors in ATMs and three air-sea O2 flux products by comparing model simulations with observations collected from surface stations, ships, and aircraft. We also present a model evaluation framework to independently quantify transport-related and flux-related biases that contribute to model-observation discrepancies in atmospheric tracer distributions.
Mizuo Kajino, Kentaro Ishijima, Joseph Ching, Kazuyo Yamaji, Rio Ishikawa, Tomoki Kajikawa, Tanbir Singh, Tomoki Nakayama, Yutaka Matsumi, Koyo Kojima, Taisei Machida, Takashi Maki, Prabir K. Patra, and Sachiko Hayashida
Atmos. Chem. Phys., 25, 7137–7160, https://doi.org/10.5194/acp-25-7137-2025, https://doi.org/10.5194/acp-25-7137-2025, 2025
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Air pollution in Delhi during the post-monsoon period is severe, and association with intensive crop residue burning (CRB) over Punjab state has attracted attention. However, the relationship has been unclear as the CRB emissions conventionally derived from satellites were underestimated due to clouds or thick smoke/haze over the region. We evaluated the impact of CRB on PM2.5 to be about 50 %, based on a combination of numerical modeling and an observation network using low-cost sensors we installed.
Marielle Saunois, Adrien Martinez, Benjamin Poulter, Zhen Zhang, Peter A. Raymond, Pierre Regnier, Josep G. Canadell, Robert B. Jackson, Prabir K. Patra, Philippe Bousquet, Philippe Ciais, Edward J. Dlugokencky, Xin Lan, George H. Allen, David Bastviken, David J. Beerling, Dmitry A. Belikov, Donald R. Blake, Simona Castaldi, Monica Crippa, Bridget R. Deemer, Fraser Dennison, Giuseppe Etiope, Nicola Gedney, Lena Höglund-Isaksson, Meredith A. Holgerson, Peter O. Hopcroft, Gustaf Hugelius, Akihiko Ito, Atul K. Jain, Rajesh Janardanan, Matthew S. Johnson, Thomas Kleinen, Paul B. Krummel, Ronny Lauerwald, Tingting Li, Xiangyu Liu, Kyle C. McDonald, Joe R. Melton, Jens Mühle, Jurek Müller, Fabiola Murguia-Flores, Yosuke Niwa, Sergio Noce, Shufen Pan, Robert J. Parker, Changhui Peng, Michel Ramonet, William J. Riley, Gerard Rocher-Ros, Judith A. Rosentreter, Motoki Sasakawa, Arjo Segers, Steven J. Smith, Emily H. Stanley, Joël Thanwerdas, Hanqin Tian, Aki Tsuruta, Francesco N. Tubiello, Thomas S. Weber, Guido R. van der Werf, Douglas E. J. Worthy, Yi Xi, Yukio Yoshida, Wenxin Zhang, Bo Zheng, Qing Zhu, Qiuan Zhu, and Qianlai Zhuang
Earth Syst. Sci. Data, 17, 1873–1958, https://doi.org/10.5194/essd-17-1873-2025, https://doi.org/10.5194/essd-17-1873-2025, 2025
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Methane (CH4) is the second most important human-influenced greenhouse gas in terms of climate forcing after carbon dioxide (CO2). A consortium of multi-disciplinary scientists synthesise and update the budget of the sources and sinks of CH4. This edition benefits from important progress in estimating emissions from lakes and ponds, reservoirs, and streams and rivers. For the 2010s decade, global CH4 emissions are estimated at 575 Tg CH4 yr-1, including ~65 % from anthropogenic sources.
Ashutosh K. Shukla, Sachchida N. Tripathi, Shamitaksha Talukdar, Vishnu Murari, Sreenivas Gaddamidi, Manousos-Ioannis Manousakas, Vipul Lalchandani, Kuldeep Dixit, Vinayak M. Ruge, Peeyush Khare, Mayank Kumar, Vikram Singh, Neeraj Rastogi, Suresh Tiwari, Atul K. Srivastava, Dilip Ganguly, Kaspar Rudolf Daellenbach, and André S. H. Prévôt
Atmos. Chem. Phys., 25, 3765–3784, https://doi.org/10.5194/acp-25-3765-2025, https://doi.org/10.5194/acp-25-3765-2025, 2025
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Our study delves into the elemental composition of aerosols at three sites across the Indo-Gangetic Plain (IGP), revealing distinct patterns during pollution episodes. We found significant increases in chlorine (Cl)-rich and solid fuel combustion (SFC) sources, indicating dynamic emission sources, agricultural burning impacts, and meteorological influences. Surges in Cl-rich particles during cold periods highlight their role in particle growth under high-relative-humidity conditions.
Chiranjit Das, Ravi Kumar Kunchala, Prabir K. Patra, Naveen Chandra, Kentaro Ishijima, and Toshinobu Machida
EGUsphere, https://doi.org/10.5194/egusphere-2024-3976, https://doi.org/10.5194/egusphere-2024-3976, 2025
Preprint archived
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Our study compares model CO2 with aircraft and OCO-2 data to identify transport model errors to better policy-related flux estimation. The model align better with aircraft data than satellite data, especially over oceans, but struggles near the surface due to inaccurate CO2 estimates. Over the Amazon and Asian megacities, differences arise from limited measurements and coarse model resolution, highlighting the need for improved monitoring and higher-resolution data to capture emissions better.
Zhen Zhang, Benjamin Poulter, Joe R. Melton, William J. Riley, George H. Allen, David J. Beerling, Philippe Bousquet, Josep G. Canadell, Etienne Fluet-Chouinard, Philippe Ciais, Nicola Gedney, Peter O. Hopcroft, Akihiko Ito, Robert B. Jackson, Atul K. Jain, Katherine Jensen, Fortunat Joos, Thomas Kleinen, Sara H. Knox, Tingting Li, Xin Li, Xiangyu Liu, Kyle McDonald, Gavin McNicol, Paul A. Miller, Jurek Müller, Prabir K. Patra, Changhui Peng, Shushi Peng, Zhangcai Qin, Ryan M. Riggs, Marielle Saunois, Qing Sun, Hanqin Tian, Xiaoming Xu, Yuanzhi Yao, Yi Xi, Wenxin Zhang, Qing Zhu, Qiuan Zhu, and Qianlai Zhuang
Biogeosciences, 22, 305–321, https://doi.org/10.5194/bg-22-305-2025, https://doi.org/10.5194/bg-22-305-2025, 2025
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This study assesses global methane emissions from wetlands between 2000 and 2020 using multiple models. We found that wetland emissions increased by 6–7 Tg CH4 yr-1 in the 2010s compared to the 2000s. Rising temperatures primarily drove this increase, while changes in precipitation and CO2 levels also played roles. Our findings highlight the importance of wetlands in the global methane budget and the need for continuous monitoring to understand their impact on climate change.
Ana Maria Roxana Petrescu, Glen P. Peters, Richard Engelen, Sander Houweling, Dominik Brunner, Aki Tsuruta, Bradley Matthews, Prabir K. Patra, Dmitry Belikov, Rona L. Thompson, Lena Höglund-Isaksson, Wenxin Zhang, Arjo J. Segers, Giuseppe Etiope, Giancarlo Ciotoli, Philippe Peylin, Frédéric Chevallier, Tuula Aalto, Robbie M. Andrew, David Bastviken, Antoine Berchet, Grégoire Broquet, Giulia Conchedda, Stijn N. C. Dellaert, Hugo Denier van der Gon, Johannes Gütschow, Jean-Matthieu Haussaire, Ronny Lauerwald, Tiina Markkanen, Jacob C. A. van Peet, Isabelle Pison, Pierre Regnier, Espen Solum, Marko Scholze, Maria Tenkanen, Francesco N. Tubiello, Guido R. van der Werf, and John R. Worden
Earth Syst. Sci. Data, 16, 4325–4350, https://doi.org/10.5194/essd-16-4325-2024, https://doi.org/10.5194/essd-16-4325-2024, 2024
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This study provides an overview of data availability from observation- and inventory-based CH4 emission estimates. It systematically compares them and provides recommendations for robust comparisons, aiming to steadily engage more parties in using observational methods to complement their UNFCCC submissions. Anticipating improvements in atmospheric modelling and observations, future developments need to resolve knowledge gaps in both approaches and to better quantify remaining uncertainty.
Matthew S. Johnson, Sajeev Philip, Scott Meech, Rajesh Kumar, Meytar Sorek-Hamer, Yoichi P. Shiga, and Jia Jung
Atmos. Chem. Phys., 24, 10363–10384, https://doi.org/10.5194/acp-24-10363-2024, https://doi.org/10.5194/acp-24-10363-2024, 2024
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Satellites, like the Ozone Monitoring Instrument (OMI), retrieve proxy species of ozone (O3) formation (formaldehyde and nitrogen dioxide) and the ratios (FNRs) which can define O3 production sensitivity regimes. Here we investigate trends of OMI FNRs from 2005 to 2021, and they have increased in major cities, suggesting a transition from radical- to NOx-limited regimes. OMI also observed the impact of reduced emissions during the 2020 COVID-19 lockdown that resulted in increased FNRs.
Hanqin Tian, Naiqing Pan, Rona L. Thompson, Josep G. Canadell, Parvadha Suntharalingam, Pierre Regnier, Eric A. Davidson, Michael Prather, Philippe Ciais, Marilena Muntean, Shufen Pan, Wilfried Winiwarter, Sönke Zaehle, Feng Zhou, Robert B. Jackson, Hermann W. Bange, Sarah Berthet, Zihao Bian, Daniele Bianchi, Alexander F. Bouwman, Erik T. Buitenhuis, Geoffrey Dutton, Minpeng Hu, Akihiko Ito, Atul K. Jain, Aurich Jeltsch-Thömmes, Fortunat Joos, Sian Kou-Giesbrecht, Paul B. Krummel, Xin Lan, Angela Landolfi, Ronny Lauerwald, Ya Li, Chaoqun Lu, Taylor Maavara, Manfredi Manizza, Dylan B. Millet, Jens Mühle, Prabir K. Patra, Glen P. Peters, Xiaoyu Qin, Peter Raymond, Laure Resplandy, Judith A. Rosentreter, Hao Shi, Qing Sun, Daniele Tonina, Francesco N. Tubiello, Guido R. van der Werf, Nicolas Vuichard, Junjie Wang, Kelley C. Wells, Luke M. Western, Chris Wilson, Jia Yang, Yuanzhi Yao, Yongfa You, and Qing Zhu
Earth Syst. Sci. Data, 16, 2543–2604, https://doi.org/10.5194/essd-16-2543-2024, https://doi.org/10.5194/essd-16-2543-2024, 2024
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Atmospheric concentrations of nitrous oxide (N2O), a greenhouse gas 273 times more potent than carbon dioxide, have increased by 25 % since the preindustrial period, with the highest observed growth rate in 2020 and 2021. This rapid growth rate has primarily been due to a 40 % increase in anthropogenic emissions since 1980. Observed atmospheric N2O concentrations in recent years have exceeded the worst-case climate scenario, underscoring the importance of reducing anthropogenic N2O emissions.
Wei Huang, Cheng Wu, Linyu Gao, Yvette Gramlich, Sophie L. Haslett, Joel Thornton, Felipe D. Lopez-Hilfiker, Ben H. Lee, Junwei Song, Harald Saathoff, Xiaoli Shen, Ramakrishna Ramisetty, Sachchida N. Tripathi, Dilip Ganguly, Feng Jiang, Magdalena Vallon, Siegfried Schobesberger, Taina Yli-Juuti, and Claudia Mohr
Atmos. Chem. Phys., 24, 2607–2624, https://doi.org/10.5194/acp-24-2607-2024, https://doi.org/10.5194/acp-24-2607-2024, 2024
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We present distinct molecular composition and volatility of oxygenated organic aerosol particles in different rural, urban, and mountain environments. We do a comprehensive investigation of the relationship between the chemical composition and volatility of oxygenated organic aerosol particles across different systems and environments. This study provides implications for volatility descriptions of oxygenated organic aerosol particles in different model frameworks.
Astrid Müller, Hiroshi Tanimoto, Takafumi Sugita, Prabir K. Patra, Shin-ichiro Nakaoka, Toshinobu Machida, Isamu Morino, André Butz, and Kei Shiomi
Atmos. Meas. Tech., 17, 1297–1316, https://doi.org/10.5194/amt-17-1297-2024, https://doi.org/10.5194/amt-17-1297-2024, 2024
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Satellite CH4 observations with high accuracy are needed to understand changes in atmospheric CH4 concentrations. But over oceans, reference data are limited. We combine various ship and aircraft observations with the help of atmospheric chemistry models to derive observation-based column-averaged mixing ratios of CH4 (obs. XCH4). We discuss three different approaches and demonstrate the applicability of the new reference dataset for carbon cycle studies and satellite evaluation.
Mounia Mostefaoui, Philippe Ciais, Matthew J. McGrath, Philippe Peylin, Prabir K. Patra, and Yolandi Ernst
Earth Syst. Sci. Data, 16, 245–275, https://doi.org/10.5194/essd-16-245-2024, https://doi.org/10.5194/essd-16-245-2024, 2024
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Our aim is to assess African anthropogenic greenhouse gas emissions and removals by using different data products, including inventories and process-based models, and to compare their relative merits with inversion data coming from satellites. We show a good match among the various estimates in terms of overall trends at a regional level and on a decadal basis, but large differences exist even among similar data types, which is a limit to the possibility of verification of country-reported data.
Nofel Lagrosas, Kosuke Okubo, Hitoshi Irie, Yutaka Matsumi, Tomoki Nakayama, Yutaka Sugita, Takashi Okada, and Tatsuo Shiina
Atmos. Meas. Tech., 16, 5937–5951, https://doi.org/10.5194/amt-16-5937-2023, https://doi.org/10.5194/amt-16-5937-2023, 2023
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This work examines the near-ground aerosol–weather relationship from 7-month continuous lidar and weather observations in Chiba, Japan. Optical parameters from lidar data are compared with weather parameters to understand and quantify the aerosol–weather relationship and how these optical parameters are affected by the weather and season. The results provide insights into analyzing optical properties of radioactive aerosols when the lidar system is continuously operated in a radioactive area.
Sophie L. Haslett, David M. Bell, Varun Kumar, Jay G. Slowik, Dongyu S. Wang, Suneeti Mishra, Neeraj Rastogi, Atinderpal Singh, Dilip Ganguly, Joel Thornton, Feixue Zheng, Yuanyuan Li, Wei Nie, Yongchun Liu, Wei Ma, Chao Yan, Markku Kulmala, Kaspar R. Daellenbach, David Hadden, Urs Baltensperger, Andre S. H. Prevot, Sachchida N. Tripathi, and Claudia Mohr
Atmos. Chem. Phys., 23, 9023–9036, https://doi.org/10.5194/acp-23-9023-2023, https://doi.org/10.5194/acp-23-9023-2023, 2023
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In Delhi, some aspects of daytime and nighttime atmospheric chemistry are inverted, and parodoxically, vehicle emissions may be limiting other forms of particle production. This is because the nighttime emissions of nitrogen oxide (NO) by traffic and biomass burning prevent some chemical processes that would otherwise create even more particles and worsen the urban haze.
Matthew S. Johnson, Amir H. Souri, Sajeev Philip, Rajesh Kumar, Aaron Naeger, Jeffrey Geddes, Laura Judd, Scott Janz, Heesung Chong, and John Sullivan
Atmos. Meas. Tech., 16, 2431–2454, https://doi.org/10.5194/amt-16-2431-2023, https://doi.org/10.5194/amt-16-2431-2023, 2023
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Satellites provide vital information for studying the processes controlling ozone formation. Based on the abundance of particular gases in the atmosphere, ozone formation is sensitive to specific human-induced and natural emission sources. However, errors and biases in satellite retrievals hinder this data source’s application for studying ozone formation sensitivity. We conducted a thorough statistical evaluation of two commonly applied satellites for investigating ozone formation sensitivity.
Jagat S. H. Bisht, Prabir K. Patra, Masayuki Takigawa, Takashi Sekiya, Yugo Kanaya, Naoko Saitoh, and Kazuyuki Miyazaki
Geosci. Model Dev., 16, 1823–1838, https://doi.org/10.5194/gmd-16-1823-2023, https://doi.org/10.5194/gmd-16-1823-2023, 2023
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In this study, we estimated CH4 fluxes using an advanced 4D-LETKF method. The system was tested and optimized using observation system simulation experiments (OSSEs), where a known surface emission distribution is retrieved from synthetic observations. The availability of satellite measurements has increased, and there are still many missions focused on greenhouse gas observations that have not yet launched. The technique being referred to has the potential to improve estimates of CH4 fluxes.
Ana Maria Roxana Petrescu, Chunjing Qiu, Matthew J. McGrath, Philippe Peylin, Glen P. Peters, Philippe Ciais, Rona L. Thompson, Aki Tsuruta, Dominik Brunner, Matthias Kuhnert, Bradley Matthews, Paul I. Palmer, Oksana Tarasova, Pierre Regnier, Ronny Lauerwald, David Bastviken, Lena Höglund-Isaksson, Wilfried Winiwarter, Giuseppe Etiope, Tuula Aalto, Gianpaolo Balsamo, Vladislav Bastrikov, Antoine Berchet, Patrick Brockmann, Giancarlo Ciotoli, Giulia Conchedda, Monica Crippa, Frank Dentener, Christine D. Groot Zwaaftink, Diego Guizzardi, Dirk Günther, Jean-Matthieu Haussaire, Sander Houweling, Greet Janssens-Maenhout, Massaer Kouyate, Adrian Leip, Antti Leppänen, Emanuele Lugato, Manon Maisonnier, Alistair J. Manning, Tiina Markkanen, Joe McNorton, Marilena Muntean, Gabriel D. Oreggioni, Prabir K. Patra, Lucia Perugini, Isabelle Pison, Maarit T. Raivonen, Marielle Saunois, Arjo J. Segers, Pete Smith, Efisio Solazzo, Hanqin Tian, Francesco N. Tubiello, Timo Vesala, Guido R. van der Werf, Chris Wilson, and Sönke Zaehle
Earth Syst. Sci. Data, 15, 1197–1268, https://doi.org/10.5194/essd-15-1197-2023, https://doi.org/10.5194/essd-15-1197-2023, 2023
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This study updates the state-of-the-art scientific overview of CH4 and N2O emissions in the EU27 and UK in Petrescu et al. (2021a). Yearly updates are needed to improve the different respective approaches and to inform on the development of formal verification systems. It integrates the most recent emission inventories, process-based model and regional/global inversions, comparing them with UNFCCC national GHG inventories, in support to policy to facilitate real-time verification procedures.
Brendan Byrne, David F. Baker, Sourish Basu, Michael Bertolacci, Kevin W. Bowman, Dustin Carroll, Abhishek Chatterjee, Frédéric Chevallier, Philippe Ciais, Noel Cressie, David Crisp, Sean Crowell, Feng Deng, Zhu Deng, Nicholas M. Deutscher, Manvendra K. Dubey, Sha Feng, Omaira E. García, David W. T. Griffith, Benedikt Herkommer, Lei Hu, Andrew R. Jacobson, Rajesh Janardanan, Sujong Jeong, Matthew S. Johnson, Dylan B. A. Jones, Rigel Kivi, Junjie Liu, Zhiqiang Liu, Shamil Maksyutov, John B. Miller, Scot M. Miller, Isamu Morino, Justus Notholt, Tomohiro Oda, Christopher W. O'Dell, Young-Suk Oh, Hirofumi Ohyama, Prabir K. Patra, Hélène Peiro, Christof Petri, Sajeev Philip, David F. Pollard, Benjamin Poulter, Marine Remaud, Andrew Schuh, Mahesh K. Sha, Kei Shiomi, Kimberly Strong, Colm Sweeney, Yao Té, Hanqin Tian, Voltaire A. Velazco, Mihalis Vrekoussis, Thorsten Warneke, John R. Worden, Debra Wunch, Yuanzhi Yao, Jeongmin Yun, Andrew Zammit-Mangion, and Ning Zeng
Earth Syst. Sci. Data, 15, 963–1004, https://doi.org/10.5194/essd-15-963-2023, https://doi.org/10.5194/essd-15-963-2023, 2023
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Changes in the carbon stocks of terrestrial ecosystems result in emissions and removals of CO2. These can be driven by anthropogenic activities (e.g., deforestation), natural processes (e.g., fires) or in response to rising CO2 (e.g., CO2 fertilization). This paper describes a dataset of CO2 emissions and removals derived from atmospheric CO2 observations. This pilot dataset informs current capabilities and future developments towards top-down monitoring and verification systems.
Amir H. Souri, Matthew S. Johnson, Glenn M. Wolfe, James H. Crawford, Alan Fried, Armin Wisthaler, William H. Brune, Donald R. Blake, Andrew J. Weinheimer, Tijl Verhoelst, Steven Compernolle, Gaia Pinardi, Corinne Vigouroux, Bavo Langerock, Sungyeon Choi, Lok Lamsal, Lei Zhu, Shuai Sun, Ronald C. Cohen, Kyung-Eun Min, Changmin Cho, Sajeev Philip, Xiong Liu, and Kelly Chance
Atmos. Chem. Phys., 23, 1963–1986, https://doi.org/10.5194/acp-23-1963-2023, https://doi.org/10.5194/acp-23-1963-2023, 2023
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We have rigorously characterized different sources of error in satellite-based HCHO / NO2 tropospheric columns, a widely used metric for diagnosing near-surface ozone sensitivity. Specifically, the errors were categorized/quantified into (i) an inherent chemistry error, (ii) the decoupled relationship between columns and the near-surface concentration, (iii) the spatial representativeness error of ground satellite pixels, and (iv) the satellite retrieval errors.
Sudipta Ghosh, Sagnik Dey, Sushant Das, Nicole Riemer, Graziano Giuliani, Dilip Ganguly, Chandra Venkataraman, Filippo Giorgi, Sachchida Nand Tripathi, Srikanthan Ramachandran, Thazhathakal Ayyappen Rajesh, Harish Gadhavi, and Atul Kumar Srivastava
Geosci. Model Dev., 16, 1–15, https://doi.org/10.5194/gmd-16-1-2023, https://doi.org/10.5194/gmd-16-1-2023, 2023
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Accurate representation of aerosols in climate models is critical for minimizing the uncertainty in climate projections. Here, we implement region-specific emission fluxes and a more accurate scheme for carbonaceous aerosol ageing processes in a regional climate model (RegCM4) and show that it improves model performance significantly against in situ, reanalysis, and satellite data over the Indian subcontinent. We recommend improving the model performance before using them for climate studies.
Brendan Byrne, Junjie Liu, Yonghong Yi, Abhishek Chatterjee, Sourish Basu, Rui Cheng, Russell Doughty, Frédéric Chevallier, Kevin W. Bowman, Nicholas C. Parazoo, David Crisp, Xing Li, Jingfeng Xiao, Stephen Sitch, Bertrand Guenet, Feng Deng, Matthew S. Johnson, Sajeev Philip, Patrick C. McGuire, and Charles E. Miller
Biogeosciences, 19, 4779–4799, https://doi.org/10.5194/bg-19-4779-2022, https://doi.org/10.5194/bg-19-4779-2022, 2022
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Plants draw CO2 from the atmosphere during the growing season, while respiration releases CO2 to the atmosphere throughout the year, driving seasonal variations in atmospheric CO2 that can be observed by satellites, such as the Orbiting Carbon Observatory 2 (OCO-2). Using OCO-2 XCO2 data and space-based constraints on plant growth, we show that permafrost-rich northeast Eurasia has a strong seasonal release of CO2 during the autumn, hinting at an unexpectedly large respiration signal from soils.
Naveen Chandra, Prabir K. Patra, Yousuke Niwa, Akihiko Ito, Yosuke Iida, Daisuke Goto, Shinji Morimoto, Masayuki Kondo, Masayuki Takigawa, Tomohiro Hajima, and Michio Watanabe
Atmos. Chem. Phys., 22, 9215–9243, https://doi.org/10.5194/acp-22-9215-2022, https://doi.org/10.5194/acp-22-9215-2022, 2022
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This paper is intended to accomplish two goals: (1) quantify mean and uncertainty in non-fossil-fuel CO2 fluxes estimated by inverse modeling and (2) provide in-depth analyses of regional CO2 fluxes in support of emission mitigation policymaking. CO2 flux variability and trends are discussed concerning natural climate variability and human disturbances using multiple lines of evidence.
Varun Kumar, Stamatios Giannoukos, Sophie L. Haslett, Yandong Tong, Atinderpal Singh, Amelie Bertrand, Chuan Ping Lee, Dongyu S. Wang, Deepika Bhattu, Giulia Stefenelli, Jay S. Dave, Joseph V. Puthussery, Lu Qi, Pawan Vats, Pragati Rai, Roberto Casotto, Rangu Satish, Suneeti Mishra, Veronika Pospisilova, Claudia Mohr, David M. Bell, Dilip Ganguly, Vishal Verma, Neeraj Rastogi, Urs Baltensperger, Sachchida N. Tripathi, André S. H. Prévôt, and Jay G. Slowik
Atmos. Chem. Phys., 22, 7739–7761, https://doi.org/10.5194/acp-22-7739-2022, https://doi.org/10.5194/acp-22-7739-2022, 2022
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Here we present source apportionment results from the first field deployment in Delhi of an extractive electrospray ionization time-of-flight mass spectrometer (EESI-TOF). The EESI-TOF is a recently developed instrument capable of providing uniquely detailed online chemical characterization of organic aerosol (OA), in particular the secondary OA (SOA) fraction. Here, we are able to apportion not only primary OA but also SOA to specific sources, which is performed for the first time in Delhi.
Pawan Gupta, Prakash Doraiswamy, Jashwanth Reddy, Palak Balyan, Sagnik Dey, Ryan Chartier, Adeel Khan, Karmann Riter, Brandon Feenstra, Robert C. Levy, Nhu Nguyen Minh Tran, Olga Pikelnaya, Kurinji Selvaraj, Tanushree Ganguly, and Karthik Ganesan
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2022-140, https://doi.org/10.5194/amt-2022-140, 2022
Revised manuscript not accepted
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The use of low-cost sensors in air quality monitoring has been gaining interest across all walks of society. We present the results of evaluations of the PurpleAir against regulatory-grade PM2.5. The results indicate that with proper calibration, we can achieve bias-corrected PM2.5 data using PA sensors. Our study also suggests that pre-deployment calibrations developed at local or regional scales are required for the PA sensors to correct data from the field for scientific data analysis.
Yange Deng, Hiroaki Fujinari, Hikari Yai, Kojiro Shimada, Yuzo Miyazaki, Eri Tachibana, Dhananjay K. Deshmukh, Kimitaka Kawamura, Tomoki Nakayama, Shiori Tatsuta, Mingfu Cai, Hanbing Xu, Fei Li, Haobo Tan, Sho Ohata, Yutaka Kondo, Akinori Takami, Shiro Hatakeyama, and Michihiro Mochida
Atmos. Chem. Phys., 22, 5515–5533, https://doi.org/10.5194/acp-22-5515-2022, https://doi.org/10.5194/acp-22-5515-2022, 2022
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Offline analyses of the hygroscopicity and composition of atmospheric aerosols are complementary to online analyses in view of the applicability to broader sizes, specific compound groups, and investigations at remote sites. This offline study characterized the composition of water-soluble matter in aerosols and their humidity-dependent hygroscopicity on Okinawa, a receptor site of East Asian outflow. Further, comparison with online analyses showed the appropriateness of the offline method.
Philippe Ciais, Ana Bastos, Frédéric Chevallier, Ronny Lauerwald, Ben Poulter, Josep G. Canadell, Gustaf Hugelius, Robert B. Jackson, Atul Jain, Matthew Jones, Masayuki Kondo, Ingrid T. Luijkx, Prabir K. Patra, Wouter Peters, Julia Pongratz, Ana Maria Roxana Petrescu, Shilong Piao, Chunjing Qiu, Celso Von Randow, Pierre Regnier, Marielle Saunois, Robert Scholes, Anatoly Shvidenko, Hanqin Tian, Hui Yang, Xuhui Wang, and Bo Zheng
Geosci. Model Dev., 15, 1289–1316, https://doi.org/10.5194/gmd-15-1289-2022, https://doi.org/10.5194/gmd-15-1289-2022, 2022
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The second phase of the Regional Carbon Cycle Assessment and Processes (RECCAP) will provide updated quantification and process understanding of CO2, CH4, and N2O emissions and sinks for ten regions of the globe. In this paper, we give definitions, review different methods, and make recommendations for estimating different components of the total land–atmosphere carbon exchange for each region in a consistent and complete approach.
Hélène Peiro, Sean Crowell, Andrew Schuh, David F. Baker, Chris O'Dell, Andrew R. Jacobson, Frédéric Chevallier, Junjie Liu, Annmarie Eldering, David Crisp, Feng Deng, Brad Weir, Sourish Basu, Matthew S. Johnson, Sajeev Philip, and Ian Baker
Atmos. Chem. Phys., 22, 1097–1130, https://doi.org/10.5194/acp-22-1097-2022, https://doi.org/10.5194/acp-22-1097-2022, 2022
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Satellite CO2 observations are constantly improved. We study an ensemble of different atmospheric models (inversions) from 2015 to 2018 using separate ground-based data or two versions of the OCO-2 satellite. Our study aims to determine if different satellite data corrections can yield different estimates of carbon cycle flux. A difference in the carbon budget between the two versions is found over tropical Africa, which seems to show the impact of corrections applied in satellite data.
Shohei Nomura, Manish Naja, M. Kawser Ahmed, Hitoshi Mukai, Yukio Terao, Toshinobu Machida, Motoki Sasakawa, and Prabir K. Patra
Atmos. Chem. Phys., 21, 16427–16452, https://doi.org/10.5194/acp-21-16427-2021, https://doi.org/10.5194/acp-21-16427-2021, 2021
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Long-term measurements of greenhouse gases (GHGs) in India and Bangladesh unveiled specific characteristics in their variations in these regions. Plants including rice cultivated in winter and summer strongly affected seasonal variations and levels in CO2 and CH4. Long-term variability of GHGs showed quite different features in their growth rates from those in Mauna Loa. GHG trends in this region seemed to be hardly affected by El Niño–Southern Oscillation (ENSO).
Jun Zhou, Kei Sato, Yu Bai, Yukiko Fukusaki, Yuka Kousa, Sathiyamurthi Ramasamy, Akinori Takami, Ayako Yoshino, Tomoki Nakayama, Yasuhiro Sadanaga, Yoshihiro Nakashima, Jiaru Li, Kentaro Murano, Nanase Kohno, Yosuke Sakamoto, and Yoshizumi Kajii
Atmos. Chem. Phys., 21, 12243–12260, https://doi.org/10.5194/acp-21-12243-2021, https://doi.org/10.5194/acp-21-12243-2021, 2021
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HO2 radicals play key roles in tropospheric chemistry, their levels in ambient air not yet fully explained by sophisticated models. Here we measured HO2 uptake kinetics onto ambient aerosols in real time using a self-built online system and investigated the impacting factors on such processes by coupling with other instrumentations. The role of the HO2 uptake process in O3 formation is also discussed. Results give useful information for coordinated control of aerosol and ozone pollutants.
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To address the lack of continuous ground-based CO2 measurements in the Indo-Gangetic Plain, we started ground-based measurements of atmospheric CO2 concentrations, for the very first time at Sonipat within the IGP. Based on these measurements, we examined the seasonal and diurnal patterns of atmospheric CO2. We found that the interplay of anthropogenic emissions, biospheric fluxes, and prevailing meteorology contributes to the observed high seasonal and diurnal variability of atmospheric CO2.
To address the lack of continuous ground-based CO2 measurements in the Indo-Gangetic Plain, we...
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