Articles | Volume 26, issue 16
https://doi.org/10.5194/acp-26-11967-2026
https://doi.org/10.5194/acp-26-11967-2026
Research article
 | 
24 Aug 2026
Research article |  | 24 Aug 2026

Improved representation of isoprene-derived secondary organic aerosol in CAM6-Chem reveals regional contrasts in its long-term changes over China

Wenxin Zhang, Man Yue, Xinyue Shao, Xinyi Dong, and Minghuai Wang

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Cited articles

Bardakov, R., Thornton, J. A., Riipinen, I., Krejci, R., and Ekman, A. M. L.: Transport and chemistry of isoprene and its oxidation products in deep convective clouds, Tellus B, 73, 1979856, https://doi.org/10.1080/16000889.2021.1979856, 2021. 
Birdsall, A. W., Miner, C. R., Mael, L. E., and Elrod, M. J.: Mechanistic study of secondary organic aerosol components formed from nucleophilic addition reactions of methacrylic acid epoxide, Atmos. Chem. Phys., 14, 12951–12964, https://doi.org/10.5194/acp-14-12951-2014, 2014. 
Budisulistiorini, S. H., Li, X., Bairai, S. T., Renfro, J., Liu, Y., Liu, Y. J., McKinney, K. A., Martin, S. T., McNeill, V. F., Pye, H. O. T., Nenes, A., Neff, M. E., Stone, E. A., Mueller, S., Knote, C., Shaw, S. L., Zhang, Z., Gold, A., and Surratt, J. D.: Examining the effects of anthropogenic emissions on isoprene-derived secondary organic aerosol formation during the 2013 Southern Oxidant and Aerosol Study (SOAS) at the Look Rock, Tennessee ground site, Atmos. Chem. Phys., 15, 8871–8888, https://doi.org/10.5194/acp-15-8871-2015, 2015. 
Budisulistiorini, S. H., Nenes, A., Carlton, A. G., Surratt, J. D., McNeill, V. F., and Pye, H. O. T.: Simulating aqueous-phase isoprene-epoxydiol (IEPOX) secondary organic aerosol production during the 2013 Southern Oxidant and Aerosol Study (SOAS), Environ. Sci. Technol., 51, 5026–5034, https://doi.org/10.1021/acs.est.6b05750, 2017. 
Carlton, A. G., Wiedinmyer, C., and Kroll, J. H.: A review of Secondary Organic Aerosol (SOA) formation from isoprene, Atmos. Chem. Phys., 9, 4987–5005, https://doi.org/10.5194/acp-9-4987-2009, 2009. 
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Short summary
Isoprene-derived secondary organic aerosol (ISOA) remains poorly represented in models, creating uncertainty in its changes and drivers. An improved model better matches observations and shows that low-NOx formation dominates. Overall ISOA changed little from 2000 to 2019 because opposite regional trends offset each other: increases in Southwest China were driven by stronger isoprene emissions, while decreases in Shaanxi–Gansu–Ningxia were driven by changes in anthropogenic emissions.
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