Articles | Volume 25, issue 18
https://doi.org/10.5194/acp-25-11129-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-25-11129-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
24 Sep 2025
Research article |
| 24 Sep 2025
| 24 Sep 2025
High sensitivity of simulated fog properties to parameterized aerosol activation in case studies from ParisFog
Pratapaditya Ghosh
Department of Civil and Environmental Engineering, Carnegie Mellon University, 5000 Forbes Avenue, Pittsburgh, PA 15213, United States
Center for Atmospheric Particle Studies, Carnegie Mellon University, 5000 Forbes Avenue, Pittsburgh, PA 15213, United States
Ian Boutle
Met Office, Fitzroy Road, Exeter, EX1 3PB, United Kingdom
Paul Field
Met Office, Fitzroy Road, Exeter, EX1 3PB, United Kingdom
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, United Kingdom
Adrian Hill
Met Office, Fitzroy Road, Exeter, EX1 3PB, United Kingdom
European Center for Medium-Range Weather Forecasting, Reading, UK
Anthony Jones
Met Office, Fitzroy Road, Exeter, EX1 3PB, United Kingdom
Marie Mazoyer
CNRM, Université de Toulouse, Météo-France, CNRS, Toulouse, France
Katherine J. Evans
Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
Salil Mahajan
Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
Hyun-Gyu Kang
Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
Min Xu
Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
Wei Zhang
Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
Noah Asch
Department of Civil and Environmental Engineering, Carnegie Mellon University, 5000 Forbes Avenue, Pittsburgh, PA 15213, United States
Center for Atmospheric Particle Studies, Carnegie Mellon University, 5000 Forbes Avenue, Pittsburgh, PA 15213, United States
Department of Chemical Engineering, Carnegie Mellon University, 5000 Forbes Avenue, Pittsburgh, PA 15213, United States
Center for Atmospheric Particle Studies, Carnegie Mellon University, 5000 Forbes Avenue, Pittsburgh, PA 15213, United States
Related authors
Pratapaditya Ghosh, Ian Boutle, Paul Field, Adrian Hill, Marie Mazoyer, Katherine J. Evans, Salil Mahajan, Hyun-Gyu Kang, Min Xu, Wei Zhang, and Hamish Gordon
Atmos. Chem. Phys., 25, 11157–11182, https://doi.org/10.5194/acp-25-11157-2025, https://doi.org/10.5194/acp-25-11157-2025, 2025
Short summary
Short summary
We study the life cycle of fog events in Europe using a weather and climate model. By incorporating droplet formation and growth driven by radiative cooling, our model better simulates the total liquid water in foggy atmospheric columns. We show that both adiabatic and radiative cooling play significant, often equally important, roles in driving droplet formation and growth. We discuss strategies to address droplet number overpredictions by improving model physics and addressing model artifacts.
Pratapaditya Ghosh, Katherine J. Evans, Daniel P. Grosvenor, Hyun-Gyu Kang, Salil Mahajan, Min Xu, Wei Zhang, and Hamish Gordon
Geosci. Model Dev., 18, 4899–4913, https://doi.org/10.5194/gmd-18-4899-2025, https://doi.org/10.5194/gmd-18-4899-2025, 2025
Short summary
Short summary
The most popular algorithm for calculating cloud droplet number concentrations in climate models is sensitive to parameters that control simulated aerosol particle number concentrations at different sizes. We recommend small modifications to functions in the algorithm to improve its performance. Implementing the changes in the UK Met Office climate model reduced average bias in simulated global droplet number concentrations, leading to more reflected solar radiation and a net cooling effect.
Pratapaditya Ghosh, Ian Boutle, Paul Field, Adrian Hill, Marie Mazoyer, Katherine J. Evans, Salil Mahajan, Hyun-Gyu Kang, Min Xu, Wei Zhang, and Hamish Gordon
Atmos. Chem. Phys., 25, 11157–11182, https://doi.org/10.5194/acp-25-11157-2025, https://doi.org/10.5194/acp-25-11157-2025, 2025
Short summary
Short summary
We study the life cycle of fog events in Europe using a weather and climate model. By incorporating droplet formation and growth driven by radiative cooling, our model better simulates the total liquid water in foggy atmospheric columns. We show that both adiabatic and radiative cooling play significant, often equally important, roles in driving droplet formation and growth. We discuss strategies to address droplet number overpredictions by improving model physics and addressing model artifacts.
Xuemei Wang, Kenneth S. Carslaw, Daniel P. Grosvenor, and Hamish Gordon
Atmos. Chem. Phys., 25, 9685–9717, https://doi.org/10.5194/acp-25-9685-2025, https://doi.org/10.5194/acp-25-9685-2025, 2025
Short summary
Short summary
Anthropogenic emissions can influence aerosol particle number concentrations and cloud formation. Our model simulations predict around a 10 % increase in the particle and cloud droplet number concentrations when doubling the emissions in the Manaus region in the Amazonian wet season. However, the corresponding changes in cloud water and rain mass are around 4 %. Such a weak response implies that this convective environment is not sensitive to the localized anthropogenic emission changes here.
Xu-Cheng He, Nathan Luke Abraham, Han Ding, Maria R. Russo, Daniel P. Grosvenor, Yao Ge, Xuemei Wang, Anthony C. Jones, Pedro Campuzano-Jost, Benjamin Nault, Agnieszka Kupc, Donald Blake, Jose L. Jimenez, Christina J. Williamson, Kenneth S. Carslaw, James Weber, Alexander T. Archibald, and Hamish Gordon
EGUsphere, https://doi.org/10.5194/egusphere-2025-3700, https://doi.org/10.5194/egusphere-2025-3700, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
Aerosols affect clouds and climate. However, current climate models still struggle to simulate them accurately. We used aircraft data from a global mission to evaluate how well the UK Earth System Model represents aerosols and their precursors. Our results show that the model misses key formation processes in clean ocean regions, suggesting that future improvements should focus on better representing how aerosols form naturally in the atmosphere.
Pratapaditya Ghosh, Katherine J. Evans, Daniel P. Grosvenor, Hyun-Gyu Kang, Salil Mahajan, Min Xu, Wei Zhang, and Hamish Gordon
Geosci. Model Dev., 18, 4899–4913, https://doi.org/10.5194/gmd-18-4899-2025, https://doi.org/10.5194/gmd-18-4899-2025, 2025
Short summary
Short summary
The most popular algorithm for calculating cloud droplet number concentrations in climate models is sensitive to parameters that control simulated aerosol particle number concentrations at different sizes. We recommend small modifications to functions in the algorithm to improve its performance. Implementing the changes in the UK Met Office climate model reduced average bias in simulated global droplet number concentrations, leading to more reflected solar radiation and a net cooling effect.
Neil M. Donahue, Victoria Hofbauer, Henning Finkenzeller, Dominik Stolzenburg, Paulus S. Bauer, Randall Chiu, Lubna Dada, Jonathan Duplissy, Xu-Cheng He, Martin Heinritzi, Christopher R. Hoyle, Andreas Kürten, Aleksandr Kvashnin, Katrianne Lehtipalo, Naser Mahfouz, Vladimir Makhmutov, Roy L. Mauldin III, Ugo Molteni, Lauriane L. J. Quéléver, Matti Rissanen, Siegfried Schobesberger, Mario Simon, Andrea C. Wagner, Mingyi Wang, Chao Yan, Penglin Ye, Ilona Riipinen, Hamish Gordon, Joachim Curtius, Armin Hansel, Imad El Haddad, Markku Kulmala, Douglas R. Worsnop, Rainer Volkamer, Paul M. Winkler, Jasper Kirkby, and Richard Flagan
EGUsphere, https://doi.org/10.5194/egusphere-2025-2412, https://doi.org/10.5194/egusphere-2025-2412, 2025
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
Short summary
Short summary
We describe accurate measurement of particle formation and growth in the CERN CLOUD chamber, using a suite of gas- and particle-phase instruments. The interconnected measurements establish high accuracy in key particle properties and critically important gas-phase sulfuric acid. This is a template for accurate calibration of similar experiments and thus accurate determination of aerosol nucleation and growth rates, which are an important source of uncertainty in climate science.
Forrest M. Hoffman, Birgit Hassler, Ranjini Swaminathan, Jared Lewis, Bouwe Andela, Nathaniel Collier, Dóra Hegedűs, Jiwoo Lee, Charlotte Pascoe, Mika Pflüger, Martina Stockhause, Paul Ullrich, Min Xu, Lisa Bock, Felicity Chun, Bettina K. Gier, Douglas I. Kelley, Axel Lauer, Julien Lenhardt, Manuel Schlund, Mohanan G. Sreeush, Katja Weigel, Ed Blockley, Rebecca Beadling, Romain Beucher, Demiso D. Dugassa, Valerio Lembo, Jianhua Lu, Swen Brands, Jerry Tjiputra, Elizaveta Malinina, Brian Mederios, Enrico Scoccimarro, Jeremy Walton, Philip Kershaw, André L. Marquez, Malcolm J. Roberts, Eleanor O’Rourke, Elisabeth Dingley, Briony Turner, Helene Hewitt, and John P. Dunne
EGUsphere, https://doi.org/10.5194/egusphere-2025-2685, https://doi.org/10.5194/egusphere-2025-2685, 2025
This preprint is open for discussion and under review for Geoscientific Model Development (GMD).
Short summary
Short summary
As Earth system models become more complex, rapid and comprehensive evaluation through comparison with observational data is necessary. The upcoming Assessment Fast Track for the Seventh Phase of the Coupled Model Intercomparison Project (CMIP7) will require fast analysis. This paper describes a new Rapid Evaluation Framework (REF) that was developed for the Assessment Fast Track that will be run at the Earth System Grid Federation (ESGF) to inform the community about the performance of models.
Mike Bush, David L. A. Flack, Huw W. Lewis, Sylvia I. Bohnenstengel, Chris J. Short, Charmaine Franklin, Adrian P. Lock, Martin Best, Paul Field, Anne McCabe, Kwinten Van Weverberg, Segolene Berthou, Ian Boutle, Jennifer K. Brooke, Seb Cole, Shaun Cooper, Gareth Dow, John Edwards, Anke Finnenkoetter, Kalli Furtado, Kate Halladay, Kirsty Hanley, Margaret A. Hendry, Adrian Hill, Aravindakshan Jayakumar, Richard W. Jones, Humphrey Lean, Joshua C. K. Lee, Andy Malcolm, Marion Mittermaier, Saji Mohandas, Stuart Moore, Cyril Morcrette, Rachel North, Aurore Porson, Susan Rennie, Nigel Roberts, Belinda Roux, Claudio Sanchez, Chun-Hsu Su, Simon Tucker, Simon Vosper, David Walters, James Warner, Stuart Webster, Mark Weeks, Jonathan Wilkinson, Michael Whitall, Keith D. Williams, and Hugh Zhang
Geosci. Model Dev., 18, 3819–3855, https://doi.org/10.5194/gmd-18-3819-2025, https://doi.org/10.5194/gmd-18-3819-2025, 2025
Short summary
Short summary
RAL configurations define settings for the Unified Model atmosphere and Joint UK Land Environment Simulator. The third version of the Regional Atmosphere and Land (RAL3) science configuration for kilometre- and sub-kilometre-scale modelling represents a major advance compared to previous versions (RAL2) by delivering a common science definition for applications in tropical and mid-latitude regions. RAL3 has more realistic precipitation distributions and an improved representation of clouds and visibility.
Martin Richard Willett, Melissa Brooks, Andrew Bushell, Paul Earnshaw, Samantha Smith, Lorenzo Tomassini, Martin Best, Ian Boutle, Jennifer Brooke, John M. Edwards, Kalli Furtado, Catherine Hardacre, Andrew J. Hartley, Alan Hewitt, Ben Johnson, Adrian Lock, Andy Malcolm, Jane Mulcahy, Eike Müller, Heather Rumbold, Gabriel G. Rooney, Alistair Sellar, Masashi Ujiie, Annelize van Niekerk, Andy Wiltshire, and Michael Whitall
EGUsphere, https://doi.org/10.5194/egusphere-2025-1829, https://doi.org/10.5194/egusphere-2025-1829, 2025
Short summary
Short summary
Global Atmosphere (GA) configurations of the Unified Model (UM) and Global Land (GL) configurations of JULES are developed for use in any global atmospheric modelling application. We describe a recent iteration of these configurations, GA8GL9, which includes improvements to the represenation of convection and other physical processes. GA8GL9 is used for operational weather prediction in the UK and forms the basis for the next GA and GL configuration.
Michael E. Kelleher and Salil Mahajan
EGUsphere, https://doi.org/10.5194/egusphere-2025-2311, https://doi.org/10.5194/egusphere-2025-2311, 2025
Short summary
Short summary
Building numerical models of the Earth is a complex task that scientists and engineers around the world work on. It's important to be able to replicate results accurately to help advance science. This study uses a statistical method to reduce false positive errors when comparing two sets of simulations to see if they agree with each other. This approach helps identify if changes made to the model's code result in unexpected effects.
August Mikkelsen, Daniel T. McCoy, Trude Eidhammer, Andrew Gettelman, Ci Song, Hamish Gordon, and Isabel L. McCoy
Atmos. Chem. Phys., 25, 4547–4570, https://doi.org/10.5194/acp-25-4547-2025, https://doi.org/10.5194/acp-25-4547-2025, 2025
Short summary
Short summary
Whether increased aerosol increases or decreases liquid cloud mass has been a longstanding question. Observed correlations suggest that aerosols thin liquid cloud, but we are able to show that observations were consistent with an increase in liquid cloud in response to aerosols by leveraging a model where causality could be traced.
Eric Giuffrida, Kate Johnson, Tyler Tatro, Paquita Zuidema, and Hamish Gordon
EGUsphere, https://doi.org/10.5194/egusphere-2025-511, https://doi.org/10.5194/egusphere-2025-511, 2025
Short summary
Short summary
Smoke aerosols emitted from summer African fires periodically travel across the ocean and interact with one of Earth’s largest permanent cloud decks. Researchers quantify the heating and cooling effects of this interaction using climate models. However, the use of different historical weather matching methods has produced a large variation in results. Here we test method variations commonly used today, and conclude on new guidelines for achieving the most accurate results.
Ashok K. Luhar, Anthony C. Jones, and Jonathan M. Wilkinson
Atmos. Chem. Phys., 24, 14005–14028, https://doi.org/10.5194/acp-24-14005-2024, https://doi.org/10.5194/acp-24-14005-2024, 2024
Short summary
Short summary
Nitrate aerosol is often omitted in global chemistry–climate models, partly due to the chemical complexity of its formation process. Using a global model, we show that including nitrate aerosol significantly impacts tropospheric composition fields, such as ozone, and radiation. Additionally, lightning-generated oxides of nitrogen influence both nitrate aerosol mass concentrations and aerosol size distribution, which has important implications for radiative fluxes and indirect aerosol effects.
Kadavathu Sreekumar Apsara, Jayakumar Aravindakshan, Anurose Theethai Jacob, Saji Mohandas, Paul Field, Hamish Gordan, Thara Prabhakaran, Mahen Konwar, and Vijapurap Srinivasa Prasad
EGUsphere, https://doi.org/10.5194/egusphere-2024-3538, https://doi.org/10.5194/egusphere-2024-3538, 2024
Short summary
Short summary
Science has made significant strides in weather prediction, especially for intense tropical rainfall that can lead to floods and landslides. Our study aims to improve monsoon rainfall forecasts by analyzing raindrop sizes. Using a new approach to model raindrop growth, we achieved a more accurate depiction of large rainfall events. These improvements can be generalized to enhance early warning systems, offering reliable predictions that help reduce risks from severe tropical weather events.
Natalie G. Ratcliffe, Claire L. Ryder, Nicolas Bellouin, Stephanie Woodward, Anthony Jones, Ben Johnson, Lisa-Maria Wieland, Maximilian Dollner, Josef Gasteiger, and Bernadett Weinzierl
Atmos. Chem. Phys., 24, 12161–12181, https://doi.org/10.5194/acp-24-12161-2024, https://doi.org/10.5194/acp-24-12161-2024, 2024
Short summary
Short summary
Large mineral dust particles are more abundant in the atmosphere than expected and have different impacts on the environment than small particles, which are better represented in climate models. We use aircraft measurements to assess a climate model representation of large-dust transport. We find that the model underestimates the amount of large dust at all stages of transport and that fast removal of the large particles increases this underestimation with distance from the Sahara.
Jim M. Haywood, Andy Jones, Anthony C. Jones, Paul Halloran, and Philip J. Rasch
Atmos. Chem. Phys., 23, 15305–15324, https://doi.org/10.5194/acp-23-15305-2023, https://doi.org/10.5194/acp-23-15305-2023, 2023
Short summary
Short summary
The difficulties in ameliorating global warming and the associated climate change via conventional mitigation are well documented, with all climate model scenarios exceeding 1.5 °C above the preindustrial level in the near future. There is therefore a growing interest in geoengineering to reflect a greater proportion of sunlight back to space and offset some of the global warming. We use a state-of-the-art Earth-system model to investigate two of the most prominent geoengineering strategies.
Denis E. Sergeev, Nathan J. Mayne, Thomas Bendall, Ian A. Boutle, Alex Brown, Iva Kavčič, James Kent, Krisztian Kohary, James Manners, Thomas Melvin, Enrico Olivier, Lokesh K. Ragta, Ben Shipway, Jon Wakelin, Nigel Wood, and Mohamed Zerroukat
Geosci. Model Dev., 16, 5601–5626, https://doi.org/10.5194/gmd-16-5601-2023, https://doi.org/10.5194/gmd-16-5601-2023, 2023
Short summary
Short summary
Three-dimensional climate models are one of the best tools we have to study planetary atmospheres. Here, we apply LFRic-Atmosphere, a new model developed by the Met Office, to seven different scenarios for terrestrial planetary climates, including four for the exoplanet TRAPPIST-1e, a primary target for future observations. LFRic-Atmosphere reproduces these scenarios within the spread of the existing models across a range of key climatic variables, justifying its use in future exoplanet studies.
Leighton A. Regayre, Lucia Deaconu, Daniel P. Grosvenor, David M. H. Sexton, Christopher Symonds, Tom Langton, Duncan Watson-Paris, Jane P. Mulcahy, Kirsty J. Pringle, Mark Richardson, Jill S. Johnson, John W. Rostron, Hamish Gordon, Grenville Lister, Philip Stier, and Ken S. Carslaw
Atmos. Chem. Phys., 23, 8749–8768, https://doi.org/10.5194/acp-23-8749-2023, https://doi.org/10.5194/acp-23-8749-2023, 2023
Short summary
Short summary
Aerosol forcing of Earth’s energy balance has persisted as a major cause of uncertainty in climate simulations over generations of climate model development. We show that structural deficiencies in a climate model are exposed by comprehensively exploring parametric uncertainty and that these deficiencies limit how much the model uncertainty can be reduced through observational constraint. This provides a future pathway towards building models with greater physical realism and lower uncertainty.
Xuemei Wang, Hamish Gordon, Daniel P. Grosvenor, Meinrat O. Andreae, and Ken S. Carslaw
Atmos. Chem. Phys., 23, 4431–4461, https://doi.org/10.5194/acp-23-4431-2023, https://doi.org/10.5194/acp-23-4431-2023, 2023
Short summary
Short summary
New particle formation in the upper troposphere is important for the global boundary layer aerosol population, and they can be transported downward in Amazonia. We use a global and a regional model to quantify the number of aerosols that are formed at high altitude and transported downward in a 1000 km region. We find that the majority of the aerosols are from outside the region. This suggests that the 1000 km region is unlikely to be a
closed loopfor aerosol formation, transport and growth.
Mike Bush, Ian Boutle, John Edwards, Anke Finnenkoetter, Charmaine Franklin, Kirsty Hanley, Aravindakshan Jayakumar, Huw Lewis, Adrian Lock, Marion Mittermaier, Saji Mohandas, Rachel North, Aurore Porson, Belinda Roux, Stuart Webster, and Mark Weeks
Geosci. Model Dev., 16, 1713–1734, https://doi.org/10.5194/gmd-16-1713-2023, https://doi.org/10.5194/gmd-16-1713-2023, 2023
Short summary
Short summary
Building on the baseline of RAL1, the RAL2 science configuration is used for regional modelling around the UM partnership and in operations at the Met Office. RAL2 has been tested in different parts of the world including Australia, India and the UK. RAL2 increases medium and low cloud amounts in the mid-latitudes compared to RAL1, leading to improved cloud forecasts and a reduced diurnal cycle of screen temperature. There is also a reduction in the frequency of heavier precipitation rates.
Danny McCulloch, Denis E. Sergeev, Nathan Mayne, Matthew Bate, James Manners, Ian Boutle, Benjamin Drummond, and Kristzian Kohary
Geosci. Model Dev., 16, 621–657, https://doi.org/10.5194/gmd-16-621-2023, https://doi.org/10.5194/gmd-16-621-2023, 2023
Short summary
Short summary
We present results from the Met Office Unified Model (UM) to study the dry Martian climate. We describe our model set-up conditions and run two scenarios, with radiatively active/inactive dust. We compare both scenarios to results from an existing Mars climate model, the planetary climate model. We find good agreement in winds and air temperatures, but dust amounts differ between models. This study highlights the importance of using the UM for future Mars research.
Chengzhu Zhang, Jean-Christophe Golaz, Ryan Forsyth, Tom Vo, Shaocheng Xie, Zeshawn Shaheen, Gerald L. Potter, Xylar S. Asay-Davis, Charles S. Zender, Wuyin Lin, Chih-Chieh Chen, Chris R. Terai, Salil Mahajan, Tian Zhou, Karthik Balaguru, Qi Tang, Cheng Tao, Yuying Zhang, Todd Emmenegger, Susannah Burrows, and Paul A. Ullrich
Geosci. Model Dev., 15, 9031–9056, https://doi.org/10.5194/gmd-15-9031-2022, https://doi.org/10.5194/gmd-15-9031-2022, 2022
Short summary
Short summary
Earth system model (ESM) developers run automated analysis tools on data from candidate models to inform model development. This paper introduces a new Python package, E3SM Diags, that has been developed to support ESM development and use routinely in the development of DOE's Energy Exascale Earth System Model. This tool covers a set of essential diagnostics to evaluate the mean physical climate from simulations, as well as several process-oriented and phenomenon-based evaluation diagnostics.
Leighton A. Regayre, Lucia Deaconu, Daniel P. Grosvenor, David Sexton, Christopher C. Symonds, Tom Langton, Duncan Watson-Paris, Jane P. Mulcahy, Kirsty J. Pringle, Mark Richardson, Jill S. Johnson, John Rostron, Hamish Gordon, Grenville Lister, Philip Stier, and Ken S. Carslaw
EGUsphere, https://doi.org/10.5194/egusphere-2022-1330, https://doi.org/10.5194/egusphere-2022-1330, 2022
Preprint archived
Short summary
Short summary
We show that potential structural deficiencies in a climate model can be exposed by comprehensively exploring its parametric uncertainty, and that these deficiencies limit how much the model uncertainty can be reduced through observational constraint. Combined consideration of parametric and structural uncertainties provides a future pathway towards building models that have greater physical realism and lower uncertainty.
Paul A. Barrett, Steven J. Abel, Hugh Coe, Ian Crawford, Amie Dobracki, James Haywood, Steve Howell, Anthony Jones, Justin Langridge, Greg M. McFarquhar, Graeme J. Nott, Hannah Price, Jens Redemann, Yohei Shinozuka, Kate Szpek, Jonathan W. Taylor, Robert Wood, Huihui Wu, Paquita Zuidema, Stéphane Bauguitte, Ryan Bennett, Keith Bower, Hong Chen, Sabrina Cochrane, Michael Cotterell, Nicholas Davies, David Delene, Connor Flynn, Andrew Freedman, Steffen Freitag, Siddhant Gupta, David Noone, Timothy B. Onasch, James Podolske, Michael R. Poellot, Sebastian Schmidt, Stephen Springston, Arthur J. Sedlacek III, Jamie Trembath, Alan Vance, Maria A. Zawadowicz, and Jianhao Zhang
Atmos. Meas. Tech., 15, 6329–6371, https://doi.org/10.5194/amt-15-6329-2022, https://doi.org/10.5194/amt-15-6329-2022, 2022
Short summary
Short summary
To better understand weather and climate, it is vital to go into the field and collect observations. Often measurements take place in isolation, but here we compared data from two aircraft and one ground-based site. This was done in order to understand how well measurements made on one platform compared to those made on another. Whilst this is easy to do in a controlled laboratory setting, it is more challenging in the real world, and so these comparisons are as valuable as they are rare.
Michael S. Diamond, Pablo E. Saide, Paquita Zuidema, Andrew S. Ackerman, Sarah J. Doherty, Ann M. Fridlind, Hamish Gordon, Calvin Howes, Jan Kazil, Takanobu Yamaguchi, Jianhao Zhang, Graham Feingold, and Robert Wood
Atmos. Chem. Phys., 22, 12113–12151, https://doi.org/10.5194/acp-22-12113-2022, https://doi.org/10.5194/acp-22-12113-2022, 2022
Short summary
Short summary
Smoke from southern Africa blankets the southeast Atlantic from June-October, overlying a major transition region between overcast and scattered clouds. The smoke affects Earth's radiation budget by absorbing sunlight and changing cloud properties. We investigate these effects in regional climate and large eddy simulation models based on international field campaigns. We find that large-scale circulation changes more strongly affect cloud transitions than smoke microphysical effects in our case.
Anthony C. Jones, Adrian Hill, John Hemmings, Pascal Lemaitre, Arnaud Quérel, Claire L. Ryder, and Stephanie Woodward
Atmos. Chem. Phys., 22, 11381–11407, https://doi.org/10.5194/acp-22-11381-2022, https://doi.org/10.5194/acp-22-11381-2022, 2022
Short summary
Short summary
As raindrops fall to the ground, they capture aerosol (i.e. below-cloud scavenging or BCS). Many different BCS schemes are available to climate models, and it is unclear what the impact of selecting one scheme over another is. Here, various BCS models are outlined and then applied to mineral dust in climate model simulations. We find that dust concentrations are highly sensitive to the BCS scheme, with dust atmospheric lifetimes ranging from 5 to 44 d.
Marie Mazoyer, Frédéric Burnet, and Cyrielle Denjean
Atmos. Chem. Phys., 22, 11305–11321, https://doi.org/10.5194/acp-22-11305-2022, https://doi.org/10.5194/acp-22-11305-2022, 2022
Short summary
Short summary
The evolution of the droplet size distribution during the fog life cycle remains poorly understood and progress is required to reduce the uncertainty of fog forecasts. To gain insights into the physical processes driving the microphysics, intensive field campaigns were conducted during three winters at the SIRTA site in the south of Paris. This study analyzed the variations in fog microphysical properties and their potential interactions at the different evolutionary stages of the fog events.
Haochi Che, Philip Stier, Duncan Watson-Parris, Hamish Gordon, and Lucia Deaconu
Atmos. Chem. Phys., 22, 10789–10807, https://doi.org/10.5194/acp-22-10789-2022, https://doi.org/10.5194/acp-22-10789-2022, 2022
Short summary
Short summary
Extensive stratocumulus clouds over the south-eastern Atlantic (SEA) can lead to a cooling effect on the climate. A key pathway by which aerosols affect cloud properties is by acting as cloud condensation nuclei (CCN). Here, we investigated the source attribution of CCN in the SEA as well as the cloud responses. Our results show that aerosol nucleation contributes most to CCN in the marine boundary layer. In terms of emissions, anthropogenic sources contribute most to the CCN and cloud droplets.
Ian Boutle, Wayne Angevine, Jian-Wen Bao, Thierry Bergot, Ritthik Bhattacharya, Andreas Bott, Leo Ducongé, Richard Forbes, Tobias Goecke, Evelyn Grell, Adrian Hill, Adele L. Igel, Innocent Kudzotsa, Christine Lac, Bjorn Maronga, Sami Romakkaniemi, Juerg Schmidli, Johannes Schwenkel, Gert-Jan Steeneveld, and Benoît Vié
Atmos. Chem. Phys., 22, 319–333, https://doi.org/10.5194/acp-22-319-2022, https://doi.org/10.5194/acp-22-319-2022, 2022
Short summary
Short summary
Fog forecasting is one of the biggest problems for numerical weather prediction. By comparing many models used for fog forecasting with others used for fog research, we hoped to help guide forecast improvements. We show some key processes that, if improved, will help improve fog forecasting, such as how water is deposited on the ground. We also showed that research models were not themselves a suitable baseline for comparison, and we discuss what future observations are required to improve them.
Sarah J. Doherty, Pablo E. Saide, Paquita Zuidema, Yohei Shinozuka, Gonzalo A. Ferrada, Hamish Gordon, Marc Mallet, Kerry Meyer, David Painemal, Steven G. Howell, Steffen Freitag, Amie Dobracki, James R. Podolske, Sharon P. Burton, Richard A. Ferrare, Calvin Howes, Pierre Nabat, Gregory R. Carmichael, Arlindo da Silva, Kristina Pistone, Ian Chang, Lan Gao, Robert Wood, and Jens Redemann
Atmos. Chem. Phys., 22, 1–46, https://doi.org/10.5194/acp-22-1-2022, https://doi.org/10.5194/acp-22-1-2022, 2022
Short summary
Short summary
Between July and October, biomass burning smoke is advected over the southeastern Atlantic Ocean, leading to climate forcing. Model calculations of forcing by this plume vary significantly in both magnitude and sign. This paper compares aerosol and cloud properties observed during three NASA ORACLES field campaigns to the same in four models. It quantifies modeled biases in properties key to aerosol direct radiative forcing and evaluates how these biases propagate to biases in forcing.
Anthony C. Jones, Adrian Hill, Samuel Remy, N. Luke Abraham, Mohit Dalvi, Catherine Hardacre, Alan J. Hewitt, Ben Johnson, Jane P. Mulcahy, and Steven T. Turnock
Atmos. Chem. Phys., 21, 15901–15927, https://doi.org/10.5194/acp-21-15901-2021, https://doi.org/10.5194/acp-21-15901-2021, 2021
Short summary
Short summary
Ammonium nitrate is hard to model because it forms and evaporates rapidly. One approach is to relate its equilibrium concentration to temperature, humidity, and the amount of nitric acid and ammonia gases. Using this approach, we limit the rate at which equilibrium is reached using various condensation rates in a climate model. We show that ammonium nitrate concentrations are highly sensitive to the condensation rate. Our results will help improve the representation of nitrate in climate models.
Mao Xiao, Christopher R. Hoyle, Lubna Dada, Dominik Stolzenburg, Andreas Kürten, Mingyi Wang, Houssni Lamkaddam, Olga Garmash, Bernhard Mentler, Ugo Molteni, Andrea Baccarini, Mario Simon, Xu-Cheng He, Katrianne Lehtipalo, Lauri R. Ahonen, Rima Baalbaki, Paulus S. Bauer, Lisa Beck, David Bell, Federico Bianchi, Sophia Brilke, Dexian Chen, Randall Chiu, António Dias, Jonathan Duplissy, Henning Finkenzeller, Hamish Gordon, Victoria Hofbauer, Changhyuk Kim, Theodore K. Koenig, Janne Lampilahti, Chuan Ping Lee, Zijun Li, Huajun Mai, Vladimir Makhmutov, Hanna E. Manninen, Ruby Marten, Serge Mathot, Roy L. Mauldin, Wei Nie, Antti Onnela, Eva Partoll, Tuukka Petäjä, Joschka Pfeifer, Veronika Pospisilova, Lauriane L. J. Quéléver, Matti Rissanen, Siegfried Schobesberger, Simone Schuchmann, Yuri Stozhkov, Christian Tauber, Yee Jun Tham, António Tomé, Miguel Vazquez-Pufleau, Andrea C. Wagner, Robert Wagner, Yonghong Wang, Lena Weitz, Daniela Wimmer, Yusheng Wu, Chao Yan, Penglin Ye, Qing Ye, Qiaozhi Zha, Xueqin Zhou, Antonio Amorim, Ken Carslaw, Joachim Curtius, Armin Hansel, Rainer Volkamer, Paul M. Winkler, Richard C. Flagan, Markku Kulmala, Douglas R. Worsnop, Jasper Kirkby, Neil M. Donahue, Urs Baltensperger, Imad El Haddad, and Josef Dommen
Atmos. Chem. Phys., 21, 14275–14291, https://doi.org/10.5194/acp-21-14275-2021, https://doi.org/10.5194/acp-21-14275-2021, 2021
Short summary
Short summary
Experiments at CLOUD show that in polluted environments new particle formation (NPF) is largely driven by the formation of sulfuric acid–base clusters, stabilized by amines, high ammonia concentrations or lower temperatures. While oxidation products of aromatics can nucleate, they play a minor role in urban NPF. Our experiments span 4 orders of magnitude variation of observed NPF rates in ambient conditions. We provide a framework based on NPF and growth rates to interpret ambient observations.
Ananth Ranjithkumar, Hamish Gordon, Christina Williamson, Andrew Rollins, Kirsty Pringle, Agnieszka Kupc, Nathan Luke Abraham, Charles Brock, and Ken Carslaw
Atmos. Chem. Phys., 21, 4979–5014, https://doi.org/10.5194/acp-21-4979-2021, https://doi.org/10.5194/acp-21-4979-2021, 2021
Short summary
Short summary
The effect aerosols have on climate can be better understood by studying their vertical and spatial distribution throughout the atmosphere. We use observation data from the ATom campaign and evaluate the vertical profile of aerosol number concentration, sulfur dioxide and condensation sink using the UKESM (UK Earth System Model). We identify uncertainties in key atmospheric processes that help improve their theoretical representation in global climate models.
Andy Jones, Jim M. Haywood, Anthony C. Jones, Simone Tilmes, Ben Kravitz, and Alan Robock
Atmos. Chem. Phys., 21, 1287–1304, https://doi.org/10.5194/acp-21-1287-2021, https://doi.org/10.5194/acp-21-1287-2021, 2021
Short summary
Short summary
Two different methods of simulating a geoengineering scenario are compared using data from two different Earth system models. One method is very idealised while the other includes details of a plausible mechanism. The results from both models agree that the idealised approach does not capture an impact found when detailed modelling is included, namely that geoengineering induces a positive phase of the North Atlantic Oscillation which leads to warmer, wetter winters in northern Europe.
Jim M. Haywood, Steven J. Abel, Paul A. Barrett, Nicolas Bellouin, Alan Blyth, Keith N. Bower, Melissa Brooks, Ken Carslaw, Haochi Che, Hugh Coe, Michael I. Cotterell, Ian Crawford, Zhiqiang Cui, Nicholas Davies, Beth Dingley, Paul Field, Paola Formenti, Hamish Gordon, Martin de Graaf, Ross Herbert, Ben Johnson, Anthony C. Jones, Justin M. Langridge, Florent Malavelle, Daniel G. Partridge, Fanny Peers, Jens Redemann, Philip Stier, Kate Szpek, Jonathan W. Taylor, Duncan Watson-Parris, Robert Wood, Huihui Wu, and Paquita Zuidema
Atmos. Chem. Phys., 21, 1049–1084, https://doi.org/10.5194/acp-21-1049-2021, https://doi.org/10.5194/acp-21-1049-2021, 2021
Short summary
Short summary
Every year, the seasonal cycle of biomass burning from agricultural practices in Africa creates a huge plume of smoke that travels many thousands of kilometres over the Atlantic Ocean. This study provides an overview of a measurement campaign called the cloud–aerosol–radiation interaction and forcing for year 2017 (CLARIFY-2017) and documents the rationale, deployment strategy, observations, and key results from the campaign which utilized the heavily equipped FAAM atmospheric research aircraft.
Benjamin J. Murray, Kenneth S. Carslaw, and Paul R. Field
Atmos. Chem. Phys., 21, 665–679, https://doi.org/10.5194/acp-21-665-2021, https://doi.org/10.5194/acp-21-665-2021, 2021
Short summary
Short summary
The balance between the amounts of ice and supercooled water in clouds over the world's oceans strongly influences how much these clouds can dampen or amplify global warming. Aerosol particles which catalyse ice formation can dramatically reduce the amount of supercooled water in clouds; hence we argue that we need a concerted effort to improve our understanding of these ice-nucleating particles if we are to improve our predictions of climate change.
Haochi Che, Philip Stier, Hamish Gordon, Duncan Watson-Parris, and Lucia Deaconu
Atmos. Chem. Phys., 21, 17–33, https://doi.org/10.5194/acp-21-17-2021, https://doi.org/10.5194/acp-21-17-2021, 2021
Short summary
Short summary
The south-eastern Atlantic is semi-permanently covered by some of the largest stratocumulus clouds and is influenced by one-third of the biomass burning emissions from African fires. A UKEMS1 model simulation shows that the absorption effect of biomass burning aerosols is the most significant on clouds and radiation. The dominate cooling and rapid adjustments induced by the radiative effects of biomass burning aerosols result in an overall cooling in the south-eastern Atlantic.
Martin Heinritzi, Lubna Dada, Mario Simon, Dominik Stolzenburg, Andrea C. Wagner, Lukas Fischer, Lauri R. Ahonen, Stavros Amanatidis, Rima Baalbaki, Andrea Baccarini, Paulus S. Bauer, Bernhard Baumgartner, Federico Bianchi, Sophia Brilke, Dexian Chen, Randall Chiu, Antonio Dias, Josef Dommen, Jonathan Duplissy, Henning Finkenzeller, Carla Frege, Claudia Fuchs, Olga Garmash, Hamish Gordon, Manuel Granzin, Imad El Haddad, Xucheng He, Johanna Helm, Victoria Hofbauer, Christopher R. Hoyle, Juha Kangasluoma, Timo Keber, Changhyuk Kim, Andreas Kürten, Houssni Lamkaddam, Tiia M. Laurila, Janne Lampilahti, Chuan Ping Lee, Katrianne Lehtipalo, Markus Leiminger, Huajun Mai, Vladimir Makhmutov, Hanna Elina Manninen, Ruby Marten, Serge Mathot, Roy Lee Mauldin, Bernhard Mentler, Ugo Molteni, Tatjana Müller, Wei Nie, Tuomo Nieminen, Antti Onnela, Eva Partoll, Monica Passananti, Tuukka Petäjä, Joschka Pfeifer, Veronika Pospisilova, Lauriane L. J. Quéléver, Matti P. Rissanen, Clémence Rose, Siegfried Schobesberger, Wiebke Scholz, Kay Scholze, Mikko Sipilä, Gerhard Steiner, Yuri Stozhkov, Christian Tauber, Yee Jun Tham, Miguel Vazquez-Pufleau, Annele Virtanen, Alexander L. Vogel, Rainer Volkamer, Robert Wagner, Mingyi Wang, Lena Weitz, Daniela Wimmer, Mao Xiao, Chao Yan, Penglin Ye, Qiaozhi Zha, Xueqin Zhou, Antonio Amorim, Urs Baltensperger, Armin Hansel, Markku Kulmala, António Tomé, Paul M. Winkler, Douglas R. Worsnop, Neil M. Donahue, Jasper Kirkby, and Joachim Curtius
Atmos. Chem. Phys., 20, 11809–11821, https://doi.org/10.5194/acp-20-11809-2020, https://doi.org/10.5194/acp-20-11809-2020, 2020
Short summary
Short summary
With experiments performed at CLOUD, we show how isoprene interferes in monoterpene oxidation via RO2 termination at atmospherically relevant concentrations. This interference shifts the distribution of highly oxygenated organic molecules (HOMs) away from C20 class dimers towards C15 class dimers, which subsequently reduces both biogenic nucleation and early growth rates. Our results may help to understand the absence of new-particle formation in isoprene-rich environments.
Yohei Shinozuka, Pablo E. Saide, Gonzalo A. Ferrada, Sharon P. Burton, Richard Ferrare, Sarah J. Doherty, Hamish Gordon, Karla Longo, Marc Mallet, Yan Feng, Qiaoqiao Wang, Yafang Cheng, Amie Dobracki, Steffen Freitag, Steven G. Howell, Samuel LeBlanc, Connor Flynn, Michal Segal-Rosenhaimer, Kristina Pistone, James R. Podolske, Eric J. Stith, Joseph Ryan Bennett, Gregory R. Carmichael, Arlindo da Silva, Ravi Govindaraju, Ruby Leung, Yang Zhang, Leonhard Pfister, Ju-Mee Ryoo, Jens Redemann, Robert Wood, and Paquita Zuidema
Atmos. Chem. Phys., 20, 11491–11526, https://doi.org/10.5194/acp-20-11491-2020, https://doi.org/10.5194/acp-20-11491-2020, 2020
Short summary
Short summary
In the southeast Atlantic, well-defined smoke plumes from Africa advect over marine boundary layer cloud decks; both are most extensive around September, when most of the smoke resides in the free troposphere. A framework is put forth for evaluating the performance of a range of global and regional atmospheric composition models against observations made during the NASA ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) airborne mission in September 2016.
Hamish Gordon, Paul R. Field, Steven J. Abel, Paul Barrett, Keith Bower, Ian Crawford, Zhiqiang Cui, Daniel P. Grosvenor, Adrian A. Hill, Jonathan Taylor, Jonathan Wilkinson, Huihui Wu, and Ken S. Carslaw
Atmos. Chem. Phys., 20, 10997–11024, https://doi.org/10.5194/acp-20-10997-2020, https://doi.org/10.5194/acp-20-10997-2020, 2020
Short summary
Short summary
The Met Office's Unified Model is widely used both for weather forecasting and climate prediction. We present the first version of the model in which both aerosol and cloud particle mass and number concentrations are allowed to evolve separately and independently, which is important for studying how aerosols affect weather and climate. We test the model against aircraft observations near Ascension Island in the Atlantic, focusing on how aerosols can "activate" to become cloud droplets.
Cited articles
Ackerman, A. S., Kirkpatrick, M. P., Stevens, D., and Toon, O. B.: The impact of humidity above stratiform clouds on indirect aerosol climate forcing, Nature, 432, 1014–1017, 2004. a
Archibald, A. T., O'Connor, F. M., Abraham, N. L., Archer-Nicholls, S., Chipperfield, M. P., Dalvi, M., Folberth, G. A., Dennison, F., Dhomse, S. S., Griffiths, P. T., Hardacre, C., Hewitt, A. J., Hill, R. S., Johnson, C. E., Keeble, J., Köhler, M. O., Morgenstern, O., Mulcahy, J. P., Ordóñez, C., Pope, R. J., Rumbold, S. T., Russo, M. R., Savage, N. H., Sellar, A., Stringer, M., Turnock, S. T., Wild, O., and Zeng, G.: Description and evaluation of the UKCA stratosphere–troposphere chemistry scheme (StratTrop vn 1.0) implemented in UKESM1, Geosci. Model Dev., 13, 1223–1266, https://doi.org/10.5194/gmd-13-1223-2020, 2020. a
Árnason, G. and Brown, P. S.: Growth of Cloud Droplets by Condensation: A Problem in Computational Stability, J. Atmos. Sci., 28, 72–77, https://doi.org/10.1175/1520-0469(1971)028<0072:GOCDBC>2.0.CO;2, 1971. a
Baranizadeh, E., Murphy, B. N., Julin, J., Falahat, S., Reddington, C. L., Arola, A., Ahlm, L., Mikkonen, S., Fountoukis, C., Patoulias, D., Minikin, A., Hamburger, T., Laaksonen, A., Pandis, S. N., Vehkamäki, H., Lehtinen, K. E. J., and Riipinen, I.: Implementation of state-of-the-art ternary new-particle formation scheme to the regional chemical transport model PMCAMx-UF in Europe, Geosci. Model Dev., 9, 2741–2754, https://doi.org/10.5194/gmd-9-2741-2016, 2016. a
Bergot, T.: Small-scale structure of radiation fog: A large-eddy simulation study, Q. J. Roy. Meteor. Soc., 139, 1099–1112, https://doi.org/10.1002/qj.2051, 2013. a
Bergot, T., Carrer, D., Noilhan, J., and Bougeault, P.: Improved Site-Specific Numerical Prediction of Fog and Low Clouds: A Feasibility Study, Weather Forecast., 20, 627–646, https://doi.org/10.1175/WAF873.1, 2005. a
Boutle, I., Angevine, W., Bao, J.-W., Bergot, T., Bhattacharya, R., Bott, A., Ducongé, L., Forbes, R., Goecke, T., Grell, E., Hill, A., Igel, A. L., Kudzotsa, I., Lac, C., Maronga, B., Romakkaniemi, S., Schmidli, J., Schwenkel, J., Steeneveld, G.-J., and Vié, B.: Demistify: a large-eddy simulation (LES) and single-column model (SCM) intercomparison of radiation fog, Atmos. Chem. Phys., 22, 319–333, https://doi.org/10.5194/acp-22-319-2022, 2022. a
Boutle, I. A., Eyre, J. E. J., and Lock, A. P.: Seamless Stratocumulus Simulation across the Turbulent Gray Zone, Mon. Weather Rev., 142, 1655–1668, https://doi.org/10.1175/MWR-D-13-00229.1, 2014. a, b
Boutle, I. A., Finnenkoetter, A., Lock, A. P., and Wells, H.: The London Model: forecasting fog at 333 m resolution, Q. J. Roy. Meteor. Soc., 142, 360–371, https://doi.org/10.1002/qj.2656, 2016. a, b, c
Bretherton, C. S., Blossey, P. N., and Uchida, J.: Cloud droplet sedimentation, entrainment efficiency, and subtropical stratocumulus albedo, Geophys. Res. Lett., 34, https://doi.org/10.1029/2006GL027648, 2007. a
Bush, M., Boutle, I., Edwards, J., Finnenkoetter, A., Franklin, C., Hanley, K., Jayakumar, A., Lewis, H., Lock, A., Mittermaier, M., Mohandas, S., North, R., Porson, A., Roux, B., Webster, S., and Weeks, M.: The second Met Office Unified Model–JULES Regional Atmosphere and Land configuration, RAL2, Geosci. Model Dev., 16, 1713–1734, https://doi.org/10.5194/gmd-16-1713-2023, 2023. a
Bush, M., Flack, D. L. A., Lewis, H. W., Bohnenstengel, S. I., Short, C. J., Franklin, C., Lock, A. P., Best, M., Field, P., McCabe, A., Van Weverberg, K., Berthou, S., Boutle, I., Brooke, J. K., Cole, S., Cooper, S., Dow, G., Edwards, J., Finnenkoetter, A., Furtado, K., Halladay, K., Hanley, K., Hendry, M. A., Hill, A., Jayakumar, A., Jones, R. W., Lean, H., Lee, J. C. K., Malcolm, A., Mittermaier, M., Mohandas, S., Moore, S., Morcrette, C., North, R., Porson, A., Rennie, S., Roberts, N., Roux, B., Sanchez, C., Su, C.-H., Tucker, S., Vosper, S., Walters, D., Warner, J., Webster, S., Weeks, M., Wilkinson, J., Whitall, M., Williams, K. D., and Zhang, H.: The third Met Office Unified Model–JULES Regional Atmosphere and Land Configuration, RAL3, Geosci. Model Dev., 18, 3819–3855, https://doi.org/10.5194/gmd-18-3819-2025, 2025. a, b
Chapman, E. G., Gustafson Jr., W. I., Easter, R. C., Barnard, J. C., Ghan, S. J., Pekour, M. S., and Fast, J. D.: Coupling aerosol-cloud-radiative processes in the WRF-Chem model: Investigating the radiative impact of elevated point sources, Atmos. Chem. Phys., 9, 945–964, https://doi.org/10.5194/acp-9-945-2009, 2009. a
Chiriaco, M., Dupont, J.-C., Bastin, S., Badosa, J., Lopez, J., Haeffelin, M., Chepfer, H., and Guzman, R.: ReOBS: a new approach to synthesize long-term multi-variable dataset and application to the SIRTA supersite, Earth Syst. Sci. Data, 10, 919–940, https://doi.org/10.5194/essd-10-919-2018, 2018. a, b, c
Clark, P. A., Harcourt, S. A., Macpherson, B., Mathison, C. T., Cusack, S., and Naylor, M.: Prediction of visibility and aerosol within the operational Met Office Unified Model. I: Model formulation and variational assimilation, Q. J. Roy. Meteor. Soc., 134, 1801–1816, https://doi.org/10.1002/qj.318, 2008. a
Clark, T. L.: A Study in Cloud Phase Parameterization Using the Gamma Distribution, J. Atmos. Sci., 31, 142–155, https://doi.org/10.1175/1520-0469(1974)031<0142:ASICPP>2.0.CO;2, 1974. a
Crippa, M., DeCarlo, P. F., Slowik, J. G., Mohr, C., Heringa, M. F., Chirico, R., Poulain, L., Freutel, F., Sciare, J., Cozic, J., Di Marco, C. F., Elsasser, M., Nicolas, J. B., Marchand, N., Abidi, E., Wiedensohler, A., Drewnick, F., Schneider, J., Borrmann, S., Nemitz, E., Zimmermann, R., Jaffrezo, J.-L., Prévôt, A. S. H., and Baltensperger, U.: Wintertime aerosol chemical composition and source apportionment of the organic fraction in the metropolitan area of Paris, Atmos. Chem. Phys., 13, 961–981, https://doi.org/10.5194/acp-13-961-2013, 2013. a, b, c, d
Denjean, C., Formenti, P., Picquet-Varrault, B., Katrib, Y., Pangui, E., Zapf, P., and Doussin, J. F.: A new experimental approach to study the hygroscopic and optical properties of aerosols: application to ammonium sulfate particles, Atmos. Meas. Tech., 7, 183–197, https://doi.org/10.5194/amt-7-183-2014, 2014. a
Duplessis, P., Bhatia, S., Hartery, S., Wheeler, M. J., and Chang, R. Y.-W.: Microphysics of aerosol, fog and droplet residuals on the Canadian Atlantic coast, Atmos. Res., 264, 105859, https://doi.org/10.1016/j.atmosres.2021.105859, 2021. a
Dupont, J.-C., Haeffelin, M., Stolaki, S., and Elias, T.: Analysis of Dynamical and Thermal Processes Driving Fog and Quasi-Fog Life Cycles Using the 2010–2013 ParisFog Dataset, Pure Appl. Geophys., 173, https://doi.org/10.1007/s00024-015-1159-x, 2016. a
Edwards, J. M. and Slingo, A.: Studies with a flexible new radiation code. I: Choosing a configuration for a large-scale model, Q. J. Roy. Meteor. Soc., 122, 689–719, https://doi.org/10.1002/qj.49712253107, 1996. a
Elias, T., Dupont, J.-C., Hammer, E., Hoyle, C. R., Haeffelin, M., Burnet, F., and Jolivet, D.: Enhanced extinction of visible radiation due to hydrated aerosols in mist and fog, Atmos. Chem. Phys., 15, 6605–6623, https://doi.org/10.5194/acp-15-6605-2015, 2015. a, b, c, d
Fanourgakis, G. S., Kanakidou, M., Nenes, A., Bauer, S. E., Bergman, T., Carslaw, K. S., Grini, A., Hamilton, D. S., Johnson, J. S., Karydis, V. A., Kirkevåg, A., Kodros, J. K., Lohmann, U., Luo, G., Makkonen, R., Matsui, H., Neubauer, D., Pierce, J. R., Schmale, J., Stier, P., Tsigaridis, K., van Noije, T., Wang, H., Watson-Parris, D., Westervelt, D. M., Yang, Y., Yoshioka, M., Daskalakis, N., Decesari, S., Gysel-Beer, M., Kalivitis, N., Liu, X., Mahowald, N. M., Myriokefalitakis, S., Schrödner, R., Sfakianaki, M., Tsimpidi, A. P., Wu, M., and Yu, F.: Evaluation of global simulations of aerosol particle and cloud condensation nuclei number, with implications for cloud droplet formation, Atmos. Chem. Phys., 19, 8591–8617, https://doi.org/10.5194/acp-19-8591-2019, 2019. a
Feng, L., Smith, S. J., Braun, C., Crippa, M., Gidden, M. J., Hoesly, R., Klimont, Z., van Marle, M., van den Berg, M., and van der Werf, G. R.: The generation of gridded emissions data for CMIP6, Geosci. Model Dev., 13, 461–482, https://doi.org/10.5194/gmd-13-461-2020, 2020. a, b, c
Field, P. R., Hill, A., Shipway, B., Furtado, K., Wilkinson, J., Miltenberger, A., Gordon, H., Grosvenor, D. P., Stevens, R., and Van Weverberg, K.: Implementation of a Double Moment Cloud Microphysics Scheme in the UK Met Office Regional Numerical Weather Prediction Model, Q. J. Roy. Meteor. Soc., 149, 703–739, 2023. a, b, c, d, e, f
Ghan, S. J., Abdul-Razzak, H., Nenes, A., Ming, Y., Liu, X., Ovchinnikov, M., Shipway, B., Meskhidze, N., Xu, J., and Shi, X.: Droplet nucleation: Physically-based parameterizations and comparative evaluation, J. Adv. Model. Earth Sy., 3, https://doi.org/10.1029/2011MS000074, 2011. a, b
Ghosh, P., Evans, K. J., Grosvenor, D. P., Kang, H.-G., Mahajan, S., Xu, M., Zhang, W., and Gordon, H.: Assessing modifications to the Abdul-Razzak and Ghan aerosol activation parameterization (version ARG2000) to improve simulated aerosol–cloud radiative effects in the UK Met Office Unified Model (UM version 13.0), Geosci. Model Dev., 18, 4899–4913, https://doi.org/10.5194/gmd-18-4899-2025, 2025a. a, b, c
Ghosh, P., Boutle, I., Field, P., Hill, A., Jones, A., Mazoyer, M., Evans, K., Salil, M., Kang, H.-G., Zhang, W., Xu, M., Asch, N., and Gordon, H.: High sensitivity of simulated fog properties to parameterized aerosol activation in case studies from ParisFog, Zenodo [code], https://doi.org/10.5281/zenodo.15671189, 2025b. a
Ghosh, P., Boutle, I., Field, P., Hill, A., Mazoyer, M., Evans, K. J., Mahajan, S., Kang, H.-G., Xu, M., Zhang, W., and Gordon, H.: Adiabatic and radiative cooling are both important causes of aerosol activation in simulated fog events in Europe, Atmos. Chem. Phys., 25, 11157–11182, https://doi.org/10.5194/acp-25-11157-2025, 2025c. a
Ghude, S., Bhat, G., Prabha, T., Jenamani, R., Chate, D., Safai, P., Karipot, A., Konwar, M., Pithani, P., Sinha, V., Pasumarti, R., Dixit, S., Tiwari, S., Todekar, K., Varpe, S., Srivastava, A., Bisht, D., Murugavel, P., Ali, K., and Rajeevan, M.: Winter Fog Experiment Over the Indo-Gangetic Plains of India, Curr. Sci. India, 112, 767, https://doi.org/10.18520/cs/v112/i04/767-784, 2017. a
Glassmeier, F., Hoffmann, F., Johnson, J. S., Yamaguchi, T., Carslaw, K. S., and Feingold, G.: Aerosol-cloud-climate cooling overestimated by ship-track data, Science, 371, 485–489, https://doi.org/10.1126/science.abd3980, 2021. a
Goodman, C. J. and Griswold, J. D. S.: Meteorological Impacts on Commercial Aviation Delays and Cancellations in the Continental United States, J. Appl. Meteorol. Clim., 58, 479–494, https://doi.org/10.1175/JAMC-D-17-0277.1, 2019. a
Gordon, H., Field, P. R., Abel, S. J., Barrett, P., Bower, K., Crawford, I., Cui, Z., Grosvenor, D. P., Hill, A. A., Taylor, J., Wilkinson, J., Wu, H., and Carslaw, K. S.: Development of aerosol activation in the double-moment Unified Model and evaluation with CLARIFY measurements, Atmos. Chem. Phys., 20, 10997–11024, https://doi.org/10.5194/acp-20-10997-2020, 2020. a, b, c, d, e
Gordon, H., Carslaw, K. S., Hill, A. A., Field, P. R., Abraham, N. L., Beyersdorf, A., Corr-Limoges, C., Ghosh, P., Hemmings, J., Jones, A. C., Sánchez, C., Wang, X., and Wilkinson, J.: NUMAC: Description of the Nested Unified Model With Aerosols and Chemistry, and Evaluation With KORUS-AQ Data, J. Adv. Model. Earth Sy., 15, e2022MS003457, https://doi.org/10.1029/2022MS003457, 2023. a, b, c, d, e
Grosvenor, D. P. and Wood, R.: The effect of solar zenith angle on MODIS cloud optical and microphysical retrievals within marine liquid water clouds, Atmos. Chem. Phys., 14, 7291–7321, https://doi.org/10.5194/acp-14-7291-2014, 2014. a
Grosvenor, D. P., Field, P. R., Hill, A. A., and Shipway, B. J.: The relative importance of macrophysical and cloud albedo changes for aerosol-induced radiative effects in closed-cell stratocumulus: insight from the modelling of a case study, Atmos. Chem. Phys., 17, 5155–5183, https://doi.org/10.5194/acp-17-5155-2017, 2017. a
Grosvenor, D. P., Sourdeval, O., Zuidema, P., Ackerman, A., Alexandrov, M. D., Bennartz, R., Boers, R., Cairns, B., Chiu, J. C., Christensen, M., Deneke, H., Diamond, M., Feingold, G., Fridlind, A., Hünerbein, A., Knist, C., Kollias, P., Marshak, A., McCoy, D., Merk, D., Painemal, D., Rausch, J., Rosenfeld, D., Russchenberg, H., Seifert, P., Sinclair, K., Stier, P., van Diedenhoven, B., Wendisch, M., Werner, F., Wood, R., Zhang, Z., and Quaas, J.: Remote Sensing of Droplet Number Concentration in Warm Clouds: A Review of the Current State of Knowledge and Perspectives, Rev. Geophys., 56, 409–453, https://doi.org/10.1029/2017RG000593, 2018. a, b
Gultepe, I., Müller, M. D., and Boybeyi, Z.: A new visibility parameterization for warm-fog applications in numerical weather prediction models, J. Appl. Meteorol. Clim., 45, 1469–1480, 2006. a
Gultepe, I., Tardif, R., Michaelides, S., Cermak, J., Bott, A., Muller, M., Pagowski, M., Hansen, B., Ellrod, G., Jacobs, W., Toth, G., and Cober, S.: Fog research: A review of past achievements and future perspectives, Pure Appl. Geophys., 164, 1121–1159, 2007. a
Haeffelin, M., Barthès, L., Bock, O., Boitel, C., Bony, S., Bouniol, D., Chepfer, H., Chiriaco, M., Cuesta, J., Delanoë, J., Drobinski, P., Dufresne, J.-L., Flamant, C., Grall, M., Hodzic, A., Hourdin, F., Lapouge, F., Lemaître, Y., Mathieu, A., Morille, Y., Naud, C., Noël, V., O'Hirok, W., Pelon, J., Pietras, C., Protat, A., Romand, B., Scialom, G., and Vautard, R.: SIRTA, a ground-based atmospheric observatory for cloud and aerosol research, Ann. Geophys., 23, 253–275, https://doi.org/10.5194/angeo-23-253-2005, 2005. a
Haeffelin, M., Bergot, T., Elias, T., Tardif, R., Carrer, D., Chazette, P., Colomb, M., Drobinski, P., Dupont, E., Dupont, J.-C., Gomes, L., Musson-Genon, L., Pietras, C., Plana-Fattori, A., Protat, A., Rangognio, J., Raut, J.-C., Rémy, S., Richard, D., Sciare, J., and Zhang, X.: Parisfog: Shedding new Light on Fog Physical Processes, B. Am. Meteorol. Soc., 91, 767–783, https://doi.org/10.1175/2009BAMS2671.1, 2010. a
Hammer, E., Gysel, M., Roberts, G. C., Elias, T., Hofer, J., Hoyle, C. R., Bukowiecki, N., Dupont, J.-C., Burnet, F., Baltensperger, U., and Weingartner, E.: Size-dependent particle activation properties in fog during the ParisFog 2012/13 field campaign, Atmos. Chem. Phys., 14, 10517–10533, https://doi.org/10.5194/acp-14-10517-2014, 2014. a, b
Heim, M., Mullins, B. J., Umhauer, H., and Kasper, G.: Performance evaluation of three optical particle counters with an efficient “multimodal” calibration method, J. Aerosol Sci., 39, 1019–1031, https://doi.org/10.1016/j.jaerosci.2008.07.006, 2008. a
Hill, A. A., Feingold, G., and Jiang, H.: The Influence of Entrainment and Mixing Assumption on Aerosol–Cloud Interactions in Marine Stratocumulus, J. Atmos. Sci., 66, 1450–1464, https://doi.org/10.1175/2008JAS2909.1, 2009. a
Hulst, H. C. and van de Hulst, H. C.: Light scattering by small particles, Courier Corporation, edited by: van de Hulst, H. C., Dover Publication Inc., New York, ISBN 0-486-64228-3, 1981. a
Janssens-Maenhout, G., Crippa, M., Guizzardi, D., Dentener, F., Muntean, M., Pouliot, G., Keating, T., Zhang, Q., Kurokawa, J., Wankmüller, R., Denier van der Gon, H., Kuenen, J. J. P., Klimont, Z., Frost, G., Darras, S., Koffi, B., and Li, M.: HTAP_v2.2: a mosaic of regional and global emission grid maps for 2008 and 2010 to study hemispheric transport of air pollution, Atmos. Chem. Phys., 15, 11411–11432, https://doi.org/10.5194/acp-15-11411-2015, 2015. a, b
Jayakumar, A., Gordon, H., Francis, T., Hill, A. A., Mohandas, S., Sandeepan, B. S., Mitra, A. K., and Beig, G.: Delhi Model with Chemistry and aerosol framework (DM-Chem) for high-resolution fog forecasting, Q. J. Roy. Meteor. Soc., 147, 3957–3978, https://doi.org/10.1002/qj.4163, 2021. a, b, c, d
Jia, X., Quan, J., Zheng, Z., Liu, X., Liu, Q., He, H., and Liu, Y.: Impacts of Anthropogenic Aerosols on Fog in North China Plain, J. Geophys. Res.-Atmos., 124, https://doi.org/10.1029/2018JD029437, 2019. a, b, c, d
Jones, A. C., Hill, A., Remy, S., Abraham, N. L., Dalvi, M., Hardacre, C., Hewitt, A. J., Johnson, B., Mulcahy, J. P., and Turnock, S. T.: Exploring the sensitivity of atmospheric nitrate concentrations to nitric acid uptake rate using the Met Office's Unified Model, Atmos. Chem. Phys., 21, 15901–15927, https://doi.org/10.5194/acp-21-15901-2021, 2021. a, b
Lock, A. P., Brown, A. R., Bush, M. R., Martin, G. M., and Smith, R. N. B.: A New Boundary Layer Mixing Scheme. Part I: Scheme Description and Single-Column Model Tests, Mon. Weather Rev., 128, 3187–3199, https://doi.org/10.1175/1520-0493(2000)128<3187:ANBLMS>2.0.CO;2, 2000. a, b
Lohmann, U.: Possible Aerosol Effects on Ice Clouds via Contact Nucleation, J. Atmos. Sci., 59, 647–656, https://doi.org/10.1175/1520-0469(2001)059<0647:PAEOIC>2.0.CO;2, 2002. a, b
Maalick, Z., Kühn, T., Korhonen, H., Kokkola, H., Laaksonen, A., and Romakkaniemi, S.: Effect of aerosol concentration and absorbing aerosol on the radiation fog life cycle, Atmos. Environ., 133, 26–33, https://doi.org/10.1016/j.atmosenv.2016.03.018, 2016. a
Malavelle, F. F., Haywood, J. M., Field, P. R., Hill, A. A., Abel, S. J., Lock, A. P., Shipway, B. J., and McBeath, K.: A method to represent subgrid-scale updraft velocity in kilometer-scale models: Implication for aerosol activation, J. Geophys. Res.-Atmos., 119, 4149–4173, https://doi.org/10.1002/2013JD021218, 2014. a
Mann, G. W., Carslaw, K. S., Spracklen, D. V., Ridley, D. A., Manktelow, P. T., Chipperfield, M. P., Pickering, S. J., and Johnson, C. E.: Description and evaluation of GLOMAP-mode: a modal global aerosol microphysics model for the UKCA composition-climate model, Geosci. Model Dev., 3, 519–551, https://doi.org/10.5194/gmd-3-519-2010, 2010. a, b, c, d
Mann, G. W., Carslaw, K. S., Ridley, D. A., Spracklen, D. V., Pringle, K. J., Merikanto, J., Korhonen, H., Schwarz, J. P., Lee, L. A., Manktelow, P. T., Woodhouse, M. T., Schmidt, A., Breider, T. J., Emmerson, K. M., Reddington, C. L., Chipperfield, M. P., and Pickering, S. J.: Intercomparison of modal and sectional aerosol microphysics representations within the same 3-D global chemical transport model, Atmos. Chem. Phys., 12, 4449–4476, https://doi.org/10.5194/acp-12-4449-2012, 2012. a, b, c, d
Martinet, P., Cimini, D., Burnet, F., Ménétrier, B., Michel, Y., and Unger, V.: Improvement of numerical weather prediction model analysis during fog conditions through the assimilation of ground-based microwave radiometer observations: a 1D-Var study, Atmos. Meas. Tech., 13, 6593–6611, https://doi.org/10.5194/amt-13-6593-2020, 2020. a
Mazoyer, M., Lac, C., Thouron, O., Bergot, T., Masson, V., and Musson-Genon, L.: Large eddy simulation of radiation fog: impact of dynamics on the fog life cycle, Atmos. Chem. Phys., 17, 13017–13035, https://doi.org/10.5194/acp-17-13017-2017, 2017. a, b, c, d
Mazoyer, M., Burnet, F., and Denjean, C.: Experimental study on the evolution of droplet size distribution during the fog life cycle, Atmos. Chem. Phys., 22, 11305–11321, https://doi.org/10.5194/acp-22-11305-2022, 2022. a, b, c
McCaul, E. W., Goodman, S. J., LaCasse, K. M., and Cecil, D. J.: Forecasting Lightning Threat Using Cloud-Resolving Model Simulations, Weather Forecast., 24, 709–729, https://doi.org/10.1175/2008WAF2222152.1, 2009. a
Menut, L., Mailler, S., Dupont, J.-C., Laurant, O., Piriou, B., Haeffelin, P., Siour, M., Elias, T., Puygrenier, G., Colomb, A., Bresson, Y., Delbarre, O., and Augustin, P.: Predictability of the Meteorological Conditions Favourable to Radiative Fog Formation During the 2011 ParisFog Campaign, Bound.-Lay. Meteorol., 150, 277–297, https://doi.org/10.1007/s10546-013-9875-1, 2014. a
Morales Betancourt, R. and Nenes, A.: Droplet activation parameterization: the population-splitting concept revisited, Geosci. Model Dev., 7, 2345–2357, https://doi.org/10.5194/gmd-7-2345-2014, 2014. a, b
Mulcahy, J. P., Jones, C., Sellar, A., Johnson, B., Boutle, I. A., Jones, A., Andrews, T., Rumbold, S. T., Mollard, J., Bellouin, N., Johnson, C. E., Williams, K. D., Grosvenor, D. P., and McCoy, D. T.: Improved Aerosol Processes and Effective Radiative Forcing in HadGEM3 and UKESM1, J. Adv. Model. Earth Sy., 10, 2786–2805, https://doi.org/10.1029/2018MS001464, 2018. a
Mulcahy, J. P., Johnson, C., Jones, C. G., Povey, A. C., Scott, C. E., Sellar, A., Turnock, S. T., Woodhouse, M. T., Abraham, N. L., Andrews, M. B., Bellouin, N., Browse, J., Carslaw, K. S., Dalvi, M., Folberth, G. A., Glover, M., Grosvenor, D. P., Hardacre, C., Hill, R., Johnson, B., Jones, A., Kipling, Z., Mann, G., Mollard, J., O'Connor, F. M., Palmiéri, J., Reddington, C., Rumbold, S. T., Richardson, M., Schutgens, N. A. J., Stier, P., Stringer, M., Tang, Y., Walton, J., Woodward, S., and Yool, A.: Description and evaluation of aerosol in UKESM1 and HadGEM3-GC3.1 CMIP6 historical simulations, Geosci. Model Dev., 13, 6383–6423, https://doi.org/10.5194/gmd-13-6383-2020, 2020. a, b, c, d, e
Mulcahy, J. P., Jones, C. G., Rumbold, S. T., Kuhlbrodt, T., Dittus, A. J., Blockley, E. W., Yool, A., Walton, J., Hardacre, C., Andrews, T., Bodas-Salcedo, A., Stringer, M., de Mora, L., Harris, P., Hill, R., Kelley, D., Robertson, E., and Tang, Y.: UKESM1.1: development and evaluation of an updated configuration of the UK Earth System Model, Geosci. Model Dev., 16, 1569–1600, https://doi.org/10.5194/gmd-16-1569-2023, 2023. a, b
Nenes, A., Ghan, S., Abdul-Razzak, H., Chuang, P. Y., and Seinfeld, J. H.: Kinetic limitations on cloud droplet formation and impact on cloud albedo, Tellus B, 53, 133–149, https://doi.org/10.1034/j.1600-0889.2001.d01-12.x, 2001. a
Oliver, H. J., Shin, M., Sanders, O., Fitzpatrick, B., Clark, A., Kinoshita, B. P., Dutta, R., Pillinger, T., Bartholomew, S. L., Hall, M., Valters, D., Sutherland, D., Trzeciak, T., challurip, Gaist, S., Matthews, D., Wales, S., ColemanTom, Menezes, G., Haiducek, J., Williams, J., lhuggett, Osprey, A., at BoM, J., Hatcher, R., Veselov, D., Reinecke, A., Andrew, Pulo, K., and Dix, M.: cylc/cylc-flow: cylc-7.8.8, Zenodo [code], https://doi.org/10.5281/zenodo.4638360, 2021. a
Oliver, H. J., Sanders, O., Shin, M., Pillinger, T., Dutta, R., Fitzpatrick, B., Clark, A., Kinoshita, B. P., Hall, M., Bartholomew, S. L., Sutherland, D., Valters, D., Trzeciak, T., challurip, Matthews, D., Gaist, S., Coleman, T., Dawson, M., Menezes, G., Haiducek, J., Wales, S., Huggett, L., Osprey, A., at BoM, J., Hatcher, R., Da, C., Veselov, D., Diquan-BOM, and Andrew: cylc/cylc-flow: cylc-flow-8.3.3, Zenodo [code], https://doi.org/10.5281/zenodo.12801923, 2024. a
Petters, M. D. and Kreidenweis, S. M.: A single parameter representation of hygroscopic growth and cloud condensation nucleus activity, Atmos. Chem. Phys., 7, 1961–1971, https://doi.org/10.5194/acp-7-1961-2007, 2007. a, b, c
Phinney, L. A., Lohmann, U., and Leaitch, W. R.: Limitations of using an equilibrium approximation in an aerosol activation parameterization, J. Geophys. Res.-Atmos., 108, https://doi.org/10.1029/2002JD002391, 2003. a
Poku, C., Ross, A., Blyth, A., Hill, A., and Price, J.: How important are aerosol-fog interactions for the successful modelling of nocturnal radiation fog?, Weather, 74, https://doi.org/10.1002/wea.3503, 2019. a, b, c
Poku, C., Ross, A. N., Hill, A. A., Blyth, A. M., and Shipway, B.: Is a more physical representation of aerosol activation needed for simulations of fog?, Atmos. Chem. Phys., 21, 7271–7292, https://doi.org/10.5194/acp-21-7271-2021, 2021. a, b, c
Price, J. D., Lane, S., Boutle, I. A., Smith, D. K. E., Bergot, T., Lac, C., Duconge, L., McGregor, J., Kerr-Munslow, A., Pickering, M., and Clark, R.: LANFEX: A Field and Modeling Study to Improve Our Understanding and Forecasting of Radiation Fog, B. Am. Meteorol. Soc., 99, 2061–2077, https://doi.org/10.1175/BAMS-D-16-0299.1, 2018. a, b
Ranjithkumar, A., Gordon, H., Williamson, C., Rollins, A., Pringle, K., Kupc, A., Abraham, N. L., Brock, C., and Carslaw, K.: Constraints on global aerosol number concentration, SO2 and condensation sink in UKESM1 using ATom measurements, Atmos. Chem. Phys., 21, 4979–5014, https://doi.org/10.5194/acp-21-4979-2021, 2021. a
Roig Rodelas, R., Chakraborty, A., Perdrix, E., Tison, E., and Riffault, V.: Real-time assessment of wintertime organic aerosol characteristics and sources at a suburban site in northern France, Atmos. Environ., 203, 48–61, https://doi.org/10.1016/j.atmosenv.2019.01.035, 2019. a, b
Roquelaure, S. and Bergot, T.: Contributions from a Local Ensemble Prediction System (LEPS) for improving fog and low cloud forecasts at airports, Weather Forecast., 24, 39–52, 2009. a
Rothenberg, D. and Wang, C.: Metamodeling of Droplet Activation for Global Climate Models, J. Atmos. Sci., 73, 1255–1272, https://doi.org/10.1175/JAS-D-15-0223.1, 2016. a
Saleeby, S. M. and Cotton, W. R.: A Large-Droplet Mode and Prognostic Number Concentration of Cloud Droplets in the Colorado State University Regional Atmospheric Modeling System (RAMS). Part I: Module Descriptions and Supercell Test Simulations, J. Appl. Meteorol., 43, 182–195, https://doi.org/10.1175/1520-0450(2004)043<0182:ALMAPN>2.0.CO;2, 2004. a
Schmale, J., Henning, S., Decesari, S., Henzing, B., Keskinen, H., Sellegri, K., Ovadnevaite, J., Pöhlker, M. L., Brito, J., Bougiatioti, A., Kristensson, A., Kalivitis, N., Stavroulas, I., Carbone, S., Jefferson, A., Park, M., Schlag, P., Iwamoto, Y., Aalto, P., Äijälä, M., Bukowiecki, N., Ehn, M., Frank, G., Fröhlich, R., Frumau, A., Herrmann, E., Herrmann, H., Holzinger, R., Kos, G., Kulmala, M., Mihalopoulos, N., Nenes, A., O'Dowd, C., Petäjä, T., Picard, D., Pöhlker, C., Pöschl, U., Poulain, L., Prévôt, A. S. H., Swietlicki, E., Andreae, M. O., Artaxo, P., Wiedensohler, A., Ogren, J., Matsuki, A., Yum, S. S., Stratmann, F., Baltensperger, U., and Gysel, M.: Long-term cloud condensation nuclei number concentration, particle number size distribution and chemical composition measurements at regionally representative observatories, Atmos. Chem. Phys., 18, 2853–2881, https://doi.org/10.5194/acp-18-2853-2018, 2018. a, b
Schmetz, J., Pili, P., Tjemkes, S., Just, D., Kerkmann, J., Rota, S., and Ratier, A.: An introduction to Meteosat Second Generation (MSG), B. Am. Meteorol. Soc., 83, 977–992, 2002. a
Schutgens, N., Tsyro, S., Gryspeerdt, E., Goto, D., Weigum, N., Schulz, M., and Stier, P.: On the spatio-temporal representativeness of observations, Atmos. Chem. Phys., 17, 9761–9780, https://doi.org/10.5194/acp-17-9761-2017, 2017. a
Schwenkel, J. and Maronga, B.: Large-eddy simulation of radiation fog with comprehensive two-moment bulk microphysics: impact of different aerosol activation and condensation parameterizations, Atmos. Chem. Phys., 19, 7165–7181, https://doi.org/10.5194/acp-19-7165-2019, 2019. a
Seinfeld, J. H. and Pandis, S. N.: Atmospheric chemistry and physics. From air pollution to climate change, John Wiley and Sons, inc., New York, ISBN 9781118947401, 1998. a
Sellar, A. A., Walton, J., Jones, C. G., Wood, R., Abraham, N. L., Andrejczuk, M., Andrews, M. B., Andrews, T., Archibald, A. T., de Mora, L., Dyson, H., Elkington, M., Ellis, R., Florek, P., Good, P., Gohar, L., Haddad, S., Hardiman, S. C., Hogan, E., Iwi, A., Jones, C. D., Johnson, B., Kelley, D. I., Kettleborough, J., Knight, J. R., Köhler, M. O., Kuhlbrodt, T., Liddicoat, S., Linova-Pavlova, I., Mizielinski, M. S., Morgenstern, O., Mulcahy, J., Neininger, E., O'Connor, F. M., Petrie, R., Ridley, J., Rioual, J.-C., Roberts, M., Robertson, E., Rumbold, S., Seddon, J., Shepherd, H., Shim, S., Stephens, A., Teixiera, J. C., Tang, Y., Williams, J., Wiltshire, A., and Griffiths, P. T.: Implementation of U. K. Earth System Models for CMIP6, J. Adv. Model. Earth Sy., 12, e2019MS001946, https://doi.org/10.1029/2019MS001946, 2020. a
Shin, M., Fitzpatrick, B., Clark, A., Sanders, O., Bartholomew, S. L., Whitehouse, S., Pillinger, T., Wardle, S., Matthews, D., Oxley, S., Trzeciak, T., Valters, D., Kinoshita, B. P., Mancell, J., harry shepherd, Oliver, H. J., Wales, S., Hall, M., Seddon, J., Osprey, A., Dix, M., Sharp, R., and Cresswell, P.: metomi/rose: 2019.01.3, Zenodo [code], https://doi.org/10.5281/zenodo.3800775, 2020. a
Shipway, B. J. and Hill, A. A.: Diagnosis of systematic differences between multiple parametrizations of warm rain microphysics using a kinematic framework, Q. J. Roy. Meteor. Soc., 138, 2196–2211, https://doi.org/10.1002/qj.1913, 2012. a
Smith, R. N. B.: A scheme for predicting layer clouds and their water content in a general circulation model, Q. J. Roy. Meteor. Soc., 116, 435–460, https://doi.org/10.1002/qj.49711649210, 1990. a, b
Steeneveld, G., Ronda, R., and Holtslag, A.: The challenge of forecasting the onset and development of radiation fog using mesoscale atmospheric models, Bound.-Lay. Meteorol., 154, 265–289, 2015. a
Stolaki, S., Haeffelin, M., Lac, C., Dupont, J.-C., Elias, T., and Masson, V.: Influence of aerosols on the life cycle of a radiation fog event. A numerical and observational study, Atmos. Res., 151, 146–161, https://doi.org/10.1016/j.atmosres.2014.04.013, 2015. a, b, c, d
Thuburn, J.: ENDGame: The New Dynamical Core of the Met Office Weather and Climate Prediction Model, Springer, 27–33, https://doi.org/10.1007/978-3-319-25454-8_4, 2016. a
Van Weverberg, K. and Morcrette, C. J.: Sensitivity of cloud-radiative effects to cloud fraction parametrizations in tropical, midlatitude, and arctic kilometre-scale simulations, Q. J. Roy. Meteor. Soc., 148, 2563–2586, https://doi.org/10.1002/qj.4325, 2022. a
Van Weverberg, K., Morcrette, C. J., Boutle, I., Furtado, K., and Field, P. R.: A Bimodal Diagnostic Cloud Fraction Parameterization. Part I: Motivating Analysis and Scheme Description, Mon. Weather Rev., 149, 841–857, https://doi.org/10.1175/MWR-D-20-0224.1, 2021. a
Velde, I., Steeneveld, G.-J., Wichers Schreur, B., and Holtslag, B.: Modeling and Forecasting the Onset and Duration of Severe Radiation Fog under Frost Conditions, Mon. Weather Rev., 138, 4237–4253, https://doi.org/10.1175/2010MWR3427.1, 2010. a
Vié, B., Ducongé, L., Lac, C., Bergot, T., and Price, J.: Importance of CCN activation for fog forecasting and its representation in the two-moment microphysical scheme LIMA, Q. J. Roy. Meteor. Soc., 150, 4217–4234, https://doi.org/10.1002/qj.4812, 2024. a
Wainwright, C., Chang, R. Y.-W., and Richter, D.: Aerosol Activation in Radiation Fog at the Atmospheric Radiation Program Southern Great Plains Site, J. Geophys. Res.-Atmos., 126, e2021JD035358, https://doi.org/10.1029/2021JD035358, 2021. a
Wærsted, E. G., Haeffelin, M., Dupont, J.-C., Delanoë, J., and Dubuisson, P.: Radiation in fog: quantification of the impact on fog liquid water based on ground-based remote sensing, Atmos. Chem. Phys., 17, 10811–10835, https://doi.org/10.5194/acp-17-10811-2017, 2017. a
Walters, D., Baran, A. J., Boutle, I., Brooks, M., Earnshaw, P., Edwards, J., Furtado, K., Hill, P., Lock, A., Manners, J., Morcrette, C., Mulcahy, J., Sanchez, C., Smith, C., Stratton, R., Tennant, W., Tomassini, L., Van Weverberg, K., Vosper, S., Willett, M., Browse, J., Bushell, A., Carslaw, K., Dalvi, M., Essery, R., Gedney, N., Hardiman, S., Johnson, B., Johnson, C., Jones, A., Jones, C., Mann, G., Milton, S., Rumbold, H., Sellar, A., Ujiie, M., Whitall, M., Williams, K., and Zerroukat, M.: The Met Office Unified Model Global Atmosphere 7.0/7.1 and JULES Global Land 7.0 configurations, Geosci. Model Dev., 12, 1909–1963, https://doi.org/10.5194/gmd-12-1909-2019, 2019. a, b, c
Williamson, C. J., Kupc, A., Axisa, D., Bilsback, K. R., Bui, T., Campuzano-Jost, P., Dollner, M., Froyd, K. D., Hodshire, A. L., Jimenez, J. L., Kodros, J. K., Luo, G., Murphy, D. M., Nault, B. A., Ray, E. A., Weinzierl, B., Wilson, J. C., Yu, F., Yu, P., Pierce, J. R., and Brock, C. A.: A large source of cloud condensation nuclei from new particle formation in the tropics, Nature, 574, 399–403, https://doi.org/10.1038/s41586-019-1638-9, 2019. a
Wilson, D. R. and Ballard, S. P.: A microphysically based precipitation scheme for the UK meteorological office unified model, Q. J. Roy. Meteor. Soc., 125, 1607–1636, https://doi.org/10.1002/qj.49712555707, 1999. a, b, c
Wilson, D. R., Bushell, A. C., Kerr-Munslow, A. M., Price, J. D., and Morcrette, C. J.: PC2: A prognostic cloud fraction and condensation scheme. I: Scheme description, Q. J. Roy. Meteor. Soc., 134, 2093–2107, https://doi.org/10.1002/qj.333, 2008. a, b
Wood, N., Staniforth, A., White, A., Allen, T., Diamantakis, M., Gross, M., Melvin, T., Smith, C., Vosper, S., Zerroukat, M., and Thuburn, J.: An inherently mass-conserving semi-implicit semi-Lagrangian discretization of the deep-atmosphere global non-hydrostatic equations, Q. J. Roy. Meteor. Soc., 140, 1505–1520, https://doi.org/10.1002/qj.2235, 2014. a
Woodward, S.: Modeling the atmospheric life cycle and radiative impact of mineral dust in the Hadley Centre climate model, J. Geophys. Res.-Atmos., 106, 18155–18166, https://doi.org/10.1029/2000JD900795, 2001. a
Yan, S., Zhu, B., Zhu, T., Shi, C., Liu, D., Kang, H., Lu, W., and Lu, C.: The Effect of Aerosols on Fog Lifetime: Observational Evidence and Model Simulations, Geophys. Res. Lett., 48, https://doi.org/10.1029/2020GL091156, 2021. a, b, c
Yang, F., Hoffmann, F., Shaw, R. A., Ovchinnikov, M., and Vogelmann, A. M.: An Intercomparison of Large-Eddy Simulations of a Convection Cloud Chamber Using Haze-Capable Bin and Lagrangian Cloud Microphysics Schemes, J. Adv. Model. Earth Sy., 15, e2022MS003270, https://doi.org/10.1029/2022MS003270, 2023. a
Zhang, X., Musson-Genon, L., Dupont, E., Milliez, M., and Carissimo, B.: On the influence of a simple microphysics parametrization on radiation fog modelling: A case study during parisfog, Bound.-Lay. Meteorol., 151, 293–315, 2014. a
Zhou, B. and Ferrier, B.: Asymptotic Analysis of Equilibrium in Radiation Fog, J. Appl. Meteorol. Clim., 47, 1704–1722, https://doi.org/10.1175/2007JAMC1685.1, 2008. a
Short summary
We study aerosol–fog interactions near Paris using a weather and climate model with high spatial resolution. We show that our model can simulate the fog life cycle effectively. We find that the fog droplet number concentrations, the amount of liquid water in the fog, and the vertical structure of the fog are highly sensitive to the parameterization that simulates droplet formation and growth. The changes we propose could improve fog forecasts significantly without increasing computational costs.
We study aerosol–fog interactions near Paris using a weather and climate model with high spatial...
Altmetrics
Final-revised paper
Preprint