Articles | Volume 22, issue 2
https://doi.org/10.5194/acp-22-1175-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-1175-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
24 Jan 2022
Research article |
| 24 Jan 2022
| 24 Jan 2022
The impact of sulfur hexafluoride (SF6) sinks on age of air climatologies and trends
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Roland Eichinger
Institut für Meteorologie, Ludwig Maximilians Universität, Munich, Germany
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Department of Atmospheric Physics, Faculty of Mathematics and Physics, Charles University, Prague, Czech Republic
Hella Garny
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Institut für Meteorologie, Ludwig Maximilians Universität, Munich, Germany
Thomas Reddmann
Institute for Meteorology and Climate Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
Frauke Fritsch
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Institut für Meteorologie, Ludwig Maximilians Universität, Munich, Germany
Stefan Versick
Steinbuch Centre for Computing (SCC), Karlsruhe Institute of Technology, Karlsruhe, Germany
Gabriele Stiller
Institute for Meteorology and Climate Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
Florian Haenel
Institute for Meteorology and Climate Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
Related authors
No articles found.
Felicia Kolonjari, Patrick E. Sheese, Kaley A. Walker, Chris D. Boone, David A. Plummer, Andreas Engel, Stephen A. Montzka, David E. Oram, Tanja Schuck, Gabriele P. Stiller, and Geoffrey C. Toon
Atmos. Meas. Tech., 17, 2429–2449, https://doi.org/10.5194/amt-17-2429-2024, https://doi.org/10.5194/amt-17-2429-2024, 2024
Short summary
Short summary
The Canadian Atmospheric Chemistry Experiment Fourier transform spectrometer (ACE-FTS) satellite instrument is currently providing the only vertically resolved chlorodifluoromethane (HCFC-22) measurements from space. This study assesses the most current ACE-FTS HCFC-22 data product in the upper troposphere and lower stratosphere, as well as modelled HCFC-22 from a 39-year run of the Canadian Middle Atmosphere Model (CMAM39) in the same region.
Hella Garny, Roland Eichinger, Johannes C. Laube, Eric A. Ray, Gabriele P. Stiller, Harald Bönisch, Laura Saunders, and Marianna Linz
Atmos. Chem. Phys., 24, 4193–4215, https://doi.org/10.5194/acp-24-4193-2024, https://doi.org/10.5194/acp-24-4193-2024, 2024
Short summary
Short summary
Transport circulation in the stratosphere is important for the distribution of tracers, but its strength is hard to measure. Mean transport times can be inferred from observations of trace gases with certain properties, such as sulfur hexafluoride (SF6). However, this gas has a chemical sink in the high atmosphere, which can lead to substantial biases in inferred transport times. In this paper we present a method to correct mean transport times derived from SF6 for the effects of chemical sinks.
Gabriele P. Stiller, Thomas von Clarmann, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Alexandra Laeng, Andrea Linden, Bernd Funke, Maya García-Comas, and Manuel López-Puertas
Atmos. Meas. Tech., 17, 1759–1789, https://doi.org/10.5194/amt-17-1759-2024, https://doi.org/10.5194/amt-17-1759-2024, 2024
Short summary
Short summary
CFC-11, CFC-12, and HCFC-22 contribute to the depletion of ozone and are potent greenhouse gases. They have been banned by the Montreal protocol. With MIPAS on Envisat the atmospheric composition could be observed between 2002 and 2012. We present here the retrieval of their atmospheric distributions for the final data version 8. We characterise the derived data by their error budget and their spatial resolution. An additional representation for direct comparison to models is also provided.
Ryan S. Williams, Michaela I. Hegglin, Patrick Jöckel, Hella Garny, and Keith P. Shine
Atmos. Chem. Phys., 24, 1389–1413, https://doi.org/10.5194/acp-24-1389-2024, https://doi.org/10.5194/acp-24-1389-2024, 2024
Short summary
Short summary
During winter, a brief but abrupt reversal of the mean stratospheric westerly flow (~30 km high) around the Arctic occurs ~6 times a decade. Using a chemistry–climate model, about half of these events are shown to induce large anomalies in Arctic ozone (>25 %) and water vapour (>±25 %) around ~8–12 km altitude for up to 2–3 months, important for weather forecasting. We also calculate a doubling to trebling of the risk in breaches of mid-latitude surface air quality (ozone) standards (~60 ppbv).
Manuel López-Puertas, Maya García-Comas, Bernd Funke, Thomas von Clarmann, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Alexandra Laeng, Andrea Linden, and Gabriele P. Stiller
Atmos. Meas. Tech., 16, 5609–5645, https://doi.org/10.5194/amt-16-5609-2023, https://doi.org/10.5194/amt-16-5609-2023, 2023
Short summary
Short summary
This paper describes a new version (V8) of ozone data from MIPAS middle-atmosphere spectra. The dataset comprises high-quality ozone profiles from 20 to 100 km, with pole-to-pole latitude coverage for the day- and nighttime, spanning 2005 until 2012. An exhaustive treatment of errors has been performed. Compared to other satellite instruments, MIPAS ozone shows a positive bias of 5 %–8 % below 70 km. In the upper mesosphere, this new version agrees much better than previous ones (within 10 %).
Maya García-Comas, Bernd Funke, Manuel López-Puertas, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Andrea Linden, Belén Martínez-Mondéjar, Gabriele P. Stiller, and Thomas von Clarmann
Atmos. Meas. Tech., 16, 5357–5386, https://doi.org/10.5194/amt-16-5357-2023, https://doi.org/10.5194/amt-16-5357-2023, 2023
Short summary
Short summary
We have released version 8 of MIPAS IMK–IAA temperatures and pointing information retrieved from MIPAS Middle and Upper Atmosphere mode version 8.03 calibrated spectra, covering 20–115 km altitude. We considered non-local thermodynamic equilibrium emission explicitly for each limb scan, essential to retrieve accurate temperatures above the mid-mesosphere. Comparisons of this temperature dataset with SABER measurements show excellent agreement, improving those of previous MIPAS versions.
Monali Borthakur, Miriam Sinnhuber, Alexandra Laeng, Thomas Reddmann, Peter Braesicke, Gabriele Stiller, Thomas von Clarmann, Bernd Funke, Ilya Usoskin, Jan Maik Wissing, and Olesya Yakovchuk
Atmos. Chem. Phys., 23, 12985–13013, https://doi.org/10.5194/acp-23-12985-2023, https://doi.org/10.5194/acp-23-12985-2023, 2023
Short summary
Short summary
Reduced ozone levels resulting from ozone depletion mean more exposure to UV radiation, which has various effects on human health. We analysed solar events to see what influence it has on the chemistry of Earth's atmosphere and how this atmospheric chemistry change can affect the ozone. To do this, we used an atmospheric model considering only chemistry and compared it with satellite data. The focus was mainly on the contribution of chlorine, and we found about 10 %–20 % ozone loss due to that.
Michael Kiefer, Dale F. Hurst, Gabriele P. Stiller, Stefan Lossow, Holger Vömel, John Anderson, Faiza Azam, Jean-Loup Bertaux, Laurent Blanot, Klaus Bramstedt, John P. Burrows, Robert Damadeo, Bianca Maria Dinelli, Patrick Eriksson, Maya García-Comas, John C. Gille, Mark Hervig, Yasuko Kasai, Farahnaz Khosrawi, Donal Murtagh, Gerald E. Nedoluha, Stefan Noël, Piera Raspollini, William G. Read, Karen H. Rosenlof, Alexei Rozanov, Christopher E. Sioris, Takafumi Sugita, Thomas von Clarmann, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 16, 4589–4642, https://doi.org/10.5194/amt-16-4589-2023, https://doi.org/10.5194/amt-16-4589-2023, 2023
Short summary
Short summary
We quantify biases and drifts (and their uncertainties) between the stratospheric water vapor measurement records of 15 satellite-based instruments (SATs, with 31 different retrievals) and balloon-borne frost point hygrometers (FPs) launched at 27 globally distributed stations. These comparisons of measurements during the period 2000–2016 are made using robust, consistent statistical methods. With some exceptions, the biases and drifts determined for most SAT–FP pairs are < 10 % and < 1 % yr−1.
Roland Eichinger, Sebastian Rhode, Hella Garny, Peter Preusse, Petr Pisoft, Aleš Kuchař, Patrick Jöckel, Astrid Kerkweg, and Bastian Kern
Geosci. Model Dev., 16, 5561–5583, https://doi.org/10.5194/gmd-16-5561-2023, https://doi.org/10.5194/gmd-16-5561-2023, 2023
Short summary
Short summary
The columnar approach of gravity wave (GW) schemes results in dynamical model biases, but parallel decomposition makes horizontal GW propagation computationally unfeasible. In the global model EMAC, we approximate it by GW redistribution at one altitude using tailor-made redistribution maps generated with a ray tracer. More spread-out GW drag helps reconcile the model with observations and close the 60°S GW gap. Polar vortex dynamics are improved, enhancing climate model credibility.
Frederik Harzer, Hella Garny, Felix Ploeger, Harald Bönisch, Peter Hoor, and Thomas Birner
Atmos. Chem. Phys., 23, 10661–10675, https://doi.org/10.5194/acp-23-10661-2023, https://doi.org/10.5194/acp-23-10661-2023, 2023
Short summary
Short summary
We study the statistical relation between year-by-year fluctuations in winter-mean ozone and the strength of the stratospheric polar vortex. In the latitude–pressure plane, regression analysis shows that anomalously weak polar vortex years are associated with three pronounced local ozone maxima over the polar cap relative to the winter climatology. These response maxima primarily reflect the non-trivial combination of different ozone transport processes with varying relative contributions.
Ales Kuchar, Maurice Öhlert, Roland Eichinger, and Christoph Jacobi
EGUsphere, https://doi.org/10.5194/egusphere-2023-1831, https://doi.org/10.5194/egusphere-2023-1831, 2023
Short summary
Short summary
Exploring the polar vortex's impact on climate, a study evaluates model simulations against the ERA5 reanalysis data. Revelations about model discrepancies in simulating disruptive stratospheric warmings and vortex behaviour highlight the need for refined model simulations of past climate. By enhancing our understanding of these dynamics, the research contributes to more reliable climate projections of the polar vortex with the impact on surface climate.
Karen De Los Ríos, Paulina Ordoñez, Gabriele P. Stiller, Piera Raspollini, Marco Gai, Kaley A. Walker, Cristina Peña-Ortiz, and Luis Acosta
EGUsphere, https://doi.org/10.5194/egusphere-2023-1348, https://doi.org/10.5194/egusphere-2023-1348, 2023
Short summary
Short summary
This study examines newer versions of H2O and HDO retrievals from Envisat/MIPAS and SCISAT/ACE-FTS. Results reveal good agreement in stratospheric H2O and HDO profiles, with biases found in specific altitudes. The tape recorder signal is consistent across databases, showing differences in climatological δD composites impacting then in the interpretation of WV transport. These findings enhance our understanding of WV dynamics and highlight the need for intercomparisons to refine our insights.
Thomas Reddmann, Miriam Sinnhuber, Jan Maik Wissing, Olesya Yakovchuk, and Ilya Usoskin
Atmos. Chem. Phys., 23, 6989–7000, https://doi.org/10.5194/acp-23-6989-2023, https://doi.org/10.5194/acp-23-6989-2023, 2023
Short summary
Short summary
Recent analyses of isotopic records of ice cores and sediments have shown that very strong explosions may occur on the Sun, perhaps about one such explosion every 1000 years. Such explosions pose a real threat to humankind. It is therefore of great interest to study the impact of such explosions on Earth. We analyzed how the explosions would affect the chemistry of the middle atmosphere and show that the related ozone loss is not dramatic and that the atmosphere will recover within 1 year.
Norbert Glatthor, Thomas von Clarmann, Bernd Funke, Maya Garcia-Comas, Udo Grabowski, Michael Höpfner, Sylvia Kellmann, Michael Kiefer, Alexandra Laeng, Andrea Linden, Manuel Lopez-Puertas, and Gabriele P. Stiller
EGUsphere, https://doi.org/10.5194/egusphere-2023-919, https://doi.org/10.5194/egusphere-2023-919, 2023
Short summary
Short summary
We present global atmospheric methane (CH4) and nitrous oxide (N2O) distributions retrieved from measurements of the MIPAS instrument onboard the ENVIronmental SATellite (ENVISAT) during 2002 to 2012. Monitoring of these gases is of scientific interest, because both of them are strong greenhouse gases. We analyse the latest, improved version of calibrated MIPAS measurements. Further, we apply a new retrieval scheme leading to an improved CH4 and N2O data product .
Bernd Funke, Maya García-Comas, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Andrea Linden, Manuel López-Puertas, Gabriele P. Stiller, and Thomas von Clarmann
Atmos. Meas. Tech., 16, 2167–2196, https://doi.org/10.5194/amt-16-2167-2023, https://doi.org/10.5194/amt-16-2167-2023, 2023
Short summary
Short summary
New global nitric oxide (NO) volume-mixing-ratio and lower-thermospheric temperature data products, retrieved from Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) spectra with the IMK-IAA MIPAS data processor, have been released. The dataset covers the entire Envisat mission lifetime and includes retrieval results from all MIPAS observation modes. The data are based on ESA version 8 calibration and were processed using an improved retrieval approach.
Michael Kiefer, Thomas von Clarmann, Bernd Funke, Maya García-Comas, Norbert Glatthor, Udo Grabowski, Michael Höpfner, Sylvia Kellmann, Alexandra Laeng, Andrea Linden, Manuel López-Puertas, and Gabriele P. Stiller
Atmos. Meas. Tech., 16, 1443–1460, https://doi.org/10.5194/amt-16-1443-2023, https://doi.org/10.5194/amt-16-1443-2023, 2023
Short summary
Short summary
A new ozone data set, derived from radiation measurements of the space-borne instrument MIPAS, is presented. It consists of more than 2 million single ozone profiles from 2002–2012, covering virtually all latitudes and altitudes between 5 and 70 km. Progress in data calibration and processing methods allowed for significant improvement of the data quality, compared to previous data versions. Hence, the data set will help to better understand e.g. the time evolution of ozone in the stratosphere.
Matthias Nützel, Sabine Brinkop, Martin Dameris, Hella Garny, Patrick Jöckel, Laura L. Pan, and Mijeong Park
Atmos. Chem. Phys., 22, 15659–15683, https://doi.org/10.5194/acp-22-15659-2022, https://doi.org/10.5194/acp-22-15659-2022, 2022
Short summary
Short summary
During the Asian summer monsoon season, a large high-pressure system is present at levels close to the tropopause above Asia. We analyse how air masses are transported from surface levels to this high-pressure system, which shows distinct features from the surrounding air masses. To this end, we employ multiannual data from two complementary models that allow us to analyse the climatology as well as the interannual and intraseasonal variability of these transport pathways.
Thomas von Clarmann, Norbert Glatthor, Udo Grabowski, Bernd Funke, Michael Kiefer, Anne Kleinert, Gabriele P. Stiller, Andrea Linden, and Sylvia Kellmann
Atmos. Meas. Tech., 15, 6991–7018, https://doi.org/10.5194/amt-15-6991-2022, https://doi.org/10.5194/amt-15-6991-2022, 2022
Short summary
Short summary
Errors of profiles of temperature and mixing ratios retrieved from spectra recorded with the Michelson Interferometer for Passive Atmospheric Sounding are estimated. All known and quantified sources of uncertainty are considered. Some ongoing uncertaities contribute to both the random and to the systematic errors. In some cases, one source of uncertainty propagates onto the error budget via multiple pathways. Problems arise when the correlations of errors to be propagated are unknown.
Ales Kuchar, Petr Sacha, Roland Eichinger, Christoph Jacobi, Petr Pisoft, and Harald Rieder
EGUsphere, https://doi.org/10.5194/egusphere-2022-474, https://doi.org/10.5194/egusphere-2022-474, 2022
Preprint archived
Short summary
Short summary
We focus on the impact of small-scale orographic gravity waves (OGWs) above the Himalayas. The interaction of GWs with the large-scale circulation in the stratosphere is not still well understood and can have implications on climate projections. We use a chemistry-climate model to show that these strong OGW events are associated with anomalously increased upward planetary-scale waves and in turn affect the circumpolar circulation and have the potential to alter ozone variability as well.
William G. Read, Gabriele Stiller, Stefan Lossow, Michael Kiefer, Farahnaz Khosrawi, Dale Hurst, Holger Vömel, Karen Rosenlof, Bianca M. Dinelli, Piera Raspollini, Gerald E. Nedoluha, John C. Gille, Yasuko Kasai, Patrick Eriksson, Christopher E. Sioris, Kaley A. Walker, Katja Weigel, John P. Burrows, and Alexei Rozanov
Atmos. Meas. Tech., 15, 3377–3400, https://doi.org/10.5194/amt-15-3377-2022, https://doi.org/10.5194/amt-15-3377-2022, 2022
Short summary
Short summary
This paper attempts to provide an assessment of the accuracy of 21 satellite-based instruments that remotely measure atmospheric humidity in the upper troposphere of the Earth's atmosphere. The instruments made their measurements from 1984 to the present time; however, most of these instruments began operations after 2000, and only a few are still operational. The objective of this study is to quantify the accuracy of each satellite humidity data set.
Felix Ploeger and Hella Garny
Atmos. Chem. Phys., 22, 5559–5576, https://doi.org/10.5194/acp-22-5559-2022, https://doi.org/10.5194/acp-22-5559-2022, 2022
Short summary
Short summary
We investigate hemispheric asymmetries in stratospheric circulation changes in the last 2 decades in model simulations and atmospheric observations. We find that observed trace gas changes can be explained by a structural circulation change related to a deepening circulation in the Northern Hemisphere relative to the Southern Hemisphere. As this asymmetric signal is small compared to internal variability observed circulation trends over the recent past are not in contradiction to climate models.
Florian Haenel, Wolfgang Woiwode, Jennifer Buchmüller, Felix Friedl-Vallon, Michael Höpfner, Sören Johansson, Farahnaz Khosrawi, Oliver Kirner, Anne Kleinert, Hermann Oelhaf, Johannes Orphal, Roland Ruhnke, Björn-Martin Sinnhuber, Jörn Ungermann, Michael Weimer, and Peter Braesicke
Atmos. Chem. Phys., 22, 2843–2870, https://doi.org/10.5194/acp-22-2843-2022, https://doi.org/10.5194/acp-22-2843-2022, 2022
Short summary
Short summary
We compare remote sensing observations of H2O, O3, HNO3 and clouds in the upper troposphere–lowermost stratosphere during an Arctic winter long-range research flight with simulations by two different state-of-the-art model systems. We find good agreement for dynamical structures, trace gas distributions and clouds. We investigate model biases and sensitivities, with the goal of aiding model development and improving our understanding of processes in the upper troposphere–lowermost stratosphere.
Michael Höpfner, Oliver Kirner, Gerald Wetzel, Björn-Martin Sinnhuber, Florian Haenel, Sören Johansson, Johannes Orphal, Roland Ruhnke, Gabriele Stiller, and Thomas von Clarmann
Atmos. Chem. Phys., 21, 18433–18464, https://doi.org/10.5194/acp-21-18433-2021, https://doi.org/10.5194/acp-21-18433-2021, 2021
Short summary
Short summary
BrONO2 is an important reservoir gas for inorganic stratospheric bromine linked to the chemical cycles of stratospheric ozone depletion. Presently infrared limb sounding is the only way to measure BrONO2 in the atmosphere. We provide global distributions of BrONO2 derived from MIPAS observations 2002–2012. Comparisons with EMAC atmospheric modelling show an overall agreement and enable us to derive an independent estimate of stratospheric bromine of 21.2±1.4pptv based on the BrONO2 measurements.
Marta Abalos, Natalia Calvo, Samuel Benito-Barca, Hella Garny, Steven C. Hardiman, Pu Lin, Martin B. Andrews, Neal Butchart, Rolando Garcia, Clara Orbe, David Saint-Martin, Shingo Watanabe, and Kohei Yoshida
Atmos. Chem. Phys., 21, 13571–13591, https://doi.org/10.5194/acp-21-13571-2021, https://doi.org/10.5194/acp-21-13571-2021, 2021
Short summary
Short summary
The stratospheric Brewer–Dobson circulation (BDC), responsible for transporting mass, tracers and heat globally in the stratosphere, is evaluated in a set of state-of-the-art climate models. The acceleration of the BDC in response to increasing greenhouse gases is most robust in the lower stratosphere. At higher levels, the well-known inconsistency between model and observational BDC trends can be partly reconciled by accounting for limited sampling and large uncertainties in the observations.
Thomas von Clarmann, Udo Grabowski, Gabriele P. Stiller, Beatriz M. Monge-Sanz, Norbert Glatthor, and Sylvia Kellmann
Atmos. Chem. Phys., 21, 8823–8843, https://doi.org/10.5194/acp-21-8823-2021, https://doi.org/10.5194/acp-21-8823-2021, 2021
Short summary
Short summary
Measurements of long-lived trace gases (SF6, CFC-11, CFC-12, HCFC-12, CCl4, N2O, CH4, H2O, and CO) performed with the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) have been used to infer the stratospheric and mesospheric meridional circulation. The MIPAS data set covers the time period from July 2002 to April 2012. The method used for this purpose was the direct inversion of the two-dimensional continuity equation. Multiannual monthly mean circulation fields are presented.
Michael Kiefer, Thomas von Clarmann, Bernd Funke, Maya García-Comas, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Anne Kleinert, Alexandra Laeng, Andrea Linden, Manuel López-Puertas, Daniel R. Marsh, and Gabriele P. Stiller
Atmos. Meas. Tech., 14, 4111–4138, https://doi.org/10.5194/amt-14-4111-2021, https://doi.org/10.5194/amt-14-4111-2021, 2021
Short summary
Short summary
An improved dataset of vertical temperature profiles of the Earth's atmosphere in the altitude range 5–70 km is presented. These profiles are derived from measurements of the MIPAS instrument onboard ESA's Envisat satellite. The overall improvements are based on upgrades in the input data and several improvements in the data processing approach. Both of these are discussed, and an extensive error discussion is included. Enhancements of the new dataset are demonstrated by means of examples.
Simone Dietmüller, Hella Garny, Roland Eichinger, and William T. Ball
Atmos. Chem. Phys., 21, 6811–6837, https://doi.org/10.5194/acp-21-6811-2021, https://doi.org/10.5194/acp-21-6811-2021, 2021
Viktoria F. Sofieva, Monika Szeląg, Johanna Tamminen, Erkki Kyrölä, Doug Degenstein, Chris Roth, Daniel Zawada, Alexei Rozanov, Carlo Arosio, John P. Burrows, Mark Weber, Alexandra Laeng, Gabriele P. Stiller, Thomas von Clarmann, Lucien Froidevaux, Nathaniel Livesey, Michel van Roozendael, and Christian Retscher
Atmos. Chem. Phys., 21, 6707–6720, https://doi.org/10.5194/acp-21-6707-2021, https://doi.org/10.5194/acp-21-6707-2021, 2021
Short summary
Short summary
The MErged GRIdded Dataset of Ozone Profiles is a long-term (2001–2018) stratospheric ozone profile climate data record with resolved longitudinal structure that combines the data from six limb satellite instruments. The dataset can be used for various analyses, some of which are discussed in the paper. In particular, regionally and vertically resolved ozone trends are evaluated, including trends in the polar regions.
Edward J. Charlesworth, Ann-Kristin Dugstad, Frauke Fritsch, Patrick Jöckel, and Felix Plöger
Atmos. Chem. Phys., 20, 15227–15245, https://doi.org/10.5194/acp-20-15227-2020, https://doi.org/10.5194/acp-20-15227-2020, 2020
Short summary
Short summary
Modeling the stratosphere requires models with good representations of chemical transport. To do this, nearly all models divide the atmosphere into boxes. This creates some unwanted problems. However, the only other option is to divide the atmosphere into balloons, and this method is very complicated. Here, we use a model which uses this balloon-like method to estimate the impacts of this method on chemical transport. We find significant differences in sensitive regions of the stratosphere.
Hella Garny, Roland Walz, Matthias Nützel, and Thomas Birner
Geosci. Model Dev., 13, 5229–5257, https://doi.org/10.5194/gmd-13-5229-2020, https://doi.org/10.5194/gmd-13-5229-2020, 2020
Short summary
Short summary
Numerical models of Earth's climate system have been gaining more and more complexity over the last decades. Therefore, it is important to establish simplified models to improve process understanding. In our study, we present and document the development of a new simplified model setup within the framework of a complex climate model system that uses the same routines to calculate atmospheric dynamics as the complex model but is simplified in the representation of clouds and radiation.
Ales Kuchar, Petr Sacha, Roland Eichinger, Christoph Jacobi, Petr Pisoft, and Harald E. Rieder
Weather Clim. Dynam., 1, 481–495, https://doi.org/10.5194/wcd-1-481-2020, https://doi.org/10.5194/wcd-1-481-2020, 2020
Short summary
Short summary
Our study focuses on the impact of topographic structures such as the Himalayas and Rocky Mountains, so-called orographic gravity-wave hotspots. These hotspots play an important role in the dynamics of the middle atmosphere, in particular in the lower stratosphere. We study intermittency and zonally asymmetric character of these hotspots and their effects on the upper stratosphere and mesosphere using a new detection method in various modeling and observational datasets.
Thomas von Clarmann, Douglas A. Degenstein, Nathaniel J. Livesey, Stefan Bender, Amy Braverman, André Butz, Steven Compernolle, Robert Damadeo, Seth Dueck, Patrick Eriksson, Bernd Funke, Margaret C. Johnson, Yasuko Kasai, Arno Keppens, Anne Kleinert, Natalya A. Kramarova, Alexandra Laeng, Bavo Langerock, Vivienne H. Payne, Alexei Rozanov, Tomohiro O. Sato, Matthias Schneider, Patrick Sheese, Viktoria Sofieva, Gabriele P. Stiller, Christian von Savigny, and Daniel Zawada
Atmos. Meas. Tech., 13, 4393–4436, https://doi.org/10.5194/amt-13-4393-2020, https://doi.org/10.5194/amt-13-4393-2020, 2020
Short summary
Short summary
Remote sensing of atmospheric state variables typically relies on the inverse solution of the radiative transfer equation. An adequately characterized retrieval provides information on the uncertainties of the estimated state variables as well as on how any constraint or a priori assumption affects the estimate. This paper summarizes related techniques and provides recommendations for unified error reporting.
Temesgen Yirdaw Berhe, Gizaw Mengistu Tsidu, Thomas Blumenstock, Frank Hase, and Gabriele P. Stiller
Atmos. Meas. Tech., 13, 4079–4096, https://doi.org/10.5194/amt-13-4079-2020, https://doi.org/10.5194/amt-13-4079-2020, 2020
Short summary
Short summary
The retrieved CH4 and N2O VMR and column amounts from Addis Ababa, tropical site, are found to exhibit very good agreement with all coincident satellite observations (MIPAS, MLS, and AIRS). Furthermore, the bias obtained from the comparison is comparable to the precision of FTIR measurement, which allows the use of data in further scientific studies as it represents a unique environment of tropical Africa, a region poorly investigated in the past.
Frauke Fritsch, Hella Garny, Andreas Engel, Harald Bönisch, and Roland Eichinger
Atmos. Chem. Phys., 20, 8709–8725, https://doi.org/10.5194/acp-20-8709-2020, https://doi.org/10.5194/acp-20-8709-2020, 2020
Short summary
Short summary
We test two methods to derive age of air as a diagnostic of the Brewer–Dobson circulation from non-linear increasing trace gases such as SF6 using a chemistry-climate model and observations. Both the model and the observations show systematic variation of the age of air trend dependent on the chosen assumptions that are required when deriving age of air from measurements. This provides insight into the differences in age of air trends of observations and models.
Markus Kunze, Tim Kruschke, Ulrike Langematz, Miriam Sinnhuber, Thomas Reddmann, and Katja Matthes
Atmos. Chem. Phys., 20, 6991–7019, https://doi.org/10.5194/acp-20-6991-2020, https://doi.org/10.5194/acp-20-6991-2020, 2020
Short summary
Short summary
Modelling the response of the atmosphere and its constituents to 11-year solar variations is subject to a certain uncertainty arising from the solar irradiance data set used in the chemistry–climate model (CCM) and the applied CCM itself.
This study reveals significant influences from both sources on the variations in the solar response in the stratosphere and mesosphere.
However, there are also regions where the random, unexplained part of the variations in the solar response is largest.
Rostislav Kouznetsov, Mikhail Sofiev, Julius Vira, and Gabriele Stiller
Atmos. Chem. Phys., 20, 5837–5859, https://doi.org/10.5194/acp-20-5837-2020, https://doi.org/10.5194/acp-20-5837-2020, 2020
Short summary
Short summary
Estimates of the age of stratospheric air (AoA), its distribution, and trends, obtained by different experimental methods, differ among each other. AoA derived form MIPAS satellite observations, the richest observational dataset on sulfur hexafluoride (SF6) in the stratosphere, are a clear outlier. With multi-decade simulations of AoA and SF6 in the stratosphere, we show that the origin of the discrepancy is in a methodology of deriving AoA from observations rather than in observational data.
Stefan Lossow, Charlotta Högberg, Farahnaz Khosrawi, Gabriele P. Stiller, Ralf Bauer, Kaley A. Walker, Sylvia Kellmann, Andrea Linden, Michael Kiefer, Norbert Glatthor, Thomas von Clarmann, Donal P. Murtagh, Jörg Steinwagner, Thomas Röckmann, and Roland Eichinger
Atmos. Meas. Tech., 13, 287–308, https://doi.org/10.5194/amt-13-287-2020, https://doi.org/10.5194/amt-13-287-2020, 2020
Maxime Prignon, Simon Chabrillat, Daniele Minganti, Simon O'Doherty, Christian Servais, Gabriele Stiller, Geoffrey C. Toon, Martin K. Vollmer, and Emmanuel Mahieu
Atmos. Chem. Phys., 19, 12309–12324, https://doi.org/10.5194/acp-19-12309-2019, https://doi.org/10.5194/acp-19-12309-2019, 2019
Short summary
Short summary
Hydrochlorofluorocarbons (HCFCs) are the first, but temporary, substitution products for the strong ozone-depleting chlorofluorocarbons (CFCs). In this work, we present and validate an improved method to retrieve the most abundant HCFC in the atmosphere, allowing its evolution to be monitored independently in the troposphere and stratosphere. These kinds of contributions are fundamental for scrutinizing the fulfilment of the Montreal Protocol on Substances that Deplete the Ozone Layer.
Andreas Chrysanthou, Amanda C. Maycock, Martyn P. Chipperfield, Sandip Dhomse, Hella Garny, Douglas Kinnison, Hideharu Akiyoshi, Makoto Deushi, Rolando R. Garcia, Patrick Jöckel, Oliver Kirner, Giovanni Pitari, David A. Plummer, Laura Revell, Eugene Rozanov, Andrea Stenke, Taichu Y. Tanaka, Daniele Visioni, and Yousuke Yamashita
Atmos. Chem. Phys., 19, 11559–11586, https://doi.org/10.5194/acp-19-11559-2019, https://doi.org/10.5194/acp-19-11559-2019, 2019
Short summary
Short summary
We perform the first multi-model comparison of the impact of nudged meteorology on the stratospheric residual circulation (RC) in chemistry–climate models. Nudging meteorology does not constrain the mean strength of RC compared to free-running simulations, and despite the lack of agreement in the mean circulation, nudging tightly constrains the inter-annual variability in the tropical upward mass flux in the lower stratosphere. In summary, nudging strongly affects the representation of RC.
Dan Weaver, Kimberly Strong, Kaley A. Walker, Chris Sioris, Matthias Schneider, C. Thomas McElroy, Holger Vömel, Michael Sommer, Katja Weigel, Alexei Rozanov, John P. Burrows, William G. Read, Evan Fishbein, and Gabriele Stiller
Atmos. Meas. Tech., 12, 4039–4063, https://doi.org/10.5194/amt-12-4039-2019, https://doi.org/10.5194/amt-12-4039-2019, 2019
Short summary
Short summary
This work assesses water vapour profiles acquired by Atmospheric Chemistry Experiment (ACE) satellite instruments in the upper troposphere and lower stratosphere (UTLS) using comparisons to radiosondes and ground-based Fourier transform infrared spectrometer measurements acquired at a Canadian high Arctic measurement site in Eureka, Nunavut. Additional comparisons are made between these Eureka measurements and other water vapour satellite datasets for context, including AIRS, MLS, and others.
Matthias Nützel, Aurélien Podglajen, Hella Garny, and Felix Ploeger
Atmos. Chem. Phys., 19, 8947–8966, https://doi.org/10.5194/acp-19-8947-2019, https://doi.org/10.5194/acp-19-8947-2019, 2019
Short summary
Short summary
We investigate the transport pathways of water vapour from the upper troposphere in the Asian monsoon region to the stratosphere. In the employed chemistry-transport model we use a tagging method, such that the impact of different source regions on the stratospheric water vapour budget can be quantified. A key finding is that the Asian monsoon (compared to other source regions) is very efficient in transporting air masses and water vapour to the tropical and extratropical stratosphere.
Petr Šácha, Roland Eichinger, Hella Garny, Petr Pišoft, Simone Dietmüller, Laura de la Torre, David A. Plummer, Patrick Jöckel, Olaf Morgenstern, Guang Zeng, Neal Butchart, and Juan A. Añel
Atmos. Chem. Phys., 19, 7627–7647, https://doi.org/10.5194/acp-19-7627-2019, https://doi.org/10.5194/acp-19-7627-2019, 2019
Short summary
Short summary
Climate models robustly project a Brewer–Dobson circulation (BDC) acceleration in the course of climate change. Analyzing mean age of stratospheric air (AoA) from a subset of climate projection simulations, we find a remarkable agreement in simulating the largest AoA trends in the extratropical stratosphere. This is shown to be related with the upward shift of the circulation, resulting in a so-called stratospheric shrinkage, which could be one of the so-far-omitted BDC acceleration drivers.
Stefan Lossow, Farahnaz Khosrawi, Michael Kiefer, Kaley A. Walker, Jean-Loup Bertaux, Laurent Blanot, James M. Russell, Ellis E. Remsberg, John C. Gille, Takafumi Sugita, Christopher E. Sioris, Bianca M. Dinelli, Enzo Papandrea, Piera Raspollini, Maya García-Comas, Gabriele P. Stiller, Thomas von Clarmann, Anu Dudhia, William G. Read, Gerald E. Nedoluha, Robert P. Damadeo, Joseph M. Zawodny, Katja Weigel, Alexei Rozanov, Faiza Azam, Klaus Bramstedt, Stefan Noël, John P. Burrows, Hideo Sagawa, Yasuko Kasai, Joachim Urban, Patrick Eriksson, Donal P. Murtagh, Mark E. Hervig, Charlotta Högberg, Dale F. Hurst, and Karen H. Rosenlof
Atmos. Meas. Tech., 12, 2693–2732, https://doi.org/10.5194/amt-12-2693-2019, https://doi.org/10.5194/amt-12-2693-2019, 2019
Bärbel Vogel, Rolf Müller, Gebhard Günther, Reinhold Spang, Sreeharsha Hanumanthu, Dan Li, Martin Riese, and Gabriele P. Stiller
Atmos. Chem. Phys., 19, 6007–6034, https://doi.org/10.5194/acp-19-6007-2019, https://doi.org/10.5194/acp-19-6007-2019, 2019
Short summary
Short summary
We identified the transport pathways of air masses from the region of the Asian monsoon (e.g. pollution and greenhouse gases caused by increasing population and growing industries in Asia) into the lower stratosphere. Even small changes of the chemical composition of the lower stratosphere have an impact on surface climate (e.g. surface temperatures). Therefore, it is important to identify transport pathways to the stratosphere to allow potential environmental risks to be assessed.
Marius Hauck, Frauke Fritsch, Hella Garny, and Andreas Engel
Atmos. Chem. Phys., 19, 5269–5291, https://doi.org/10.5194/acp-19-5269-2019, https://doi.org/10.5194/acp-19-5269-2019, 2019
Short summary
Short summary
The paper presents a modified method to invert mixing ratios of chemically active tracers into stratospheric age spectra. It features an imposed seasonal cycle to include transport seasonality into the spectra. An idealized set of tracers from a model is used as proof of concept and results are in good agreement with the model reference, except for the lowermost stratosphere. Applicability is studied with focus on number of tracers and error tolerance, providing a starting point for future work.
Charlotta Högberg, Stefan Lossow, Farahnaz Khosrawi, Ralf Bauer, Kaley A. Walker, Patrick Eriksson, Donal P. Murtagh, Gabriele P. Stiller, Jörg Steinwagner, and Qiong Zhang
Atmos. Chem. Phys., 19, 2497–2526, https://doi.org/10.5194/acp-19-2497-2019, https://doi.org/10.5194/acp-19-2497-2019, 2019
Short summary
Short summary
Five δD (H2O) data sets obtained from satellite observations have been evaluated using profile-to-profile and climatological comparisons. The focus is on stratospheric altitudes, but results from the upper troposphere to the lower mesosphere are also provided. There are clear quantitative differences in the δD ratio in key areas of scientific interest, resulting in difficulties drawing robust conclusions on atmospheric processes affecting the water vapour budget and distribution.
Roland Eichinger, Simone Dietmüller, Hella Garny, Petr Šácha, Thomas Birner, Harald Bönisch, Giovanni Pitari, Daniele Visioni, Andrea Stenke, Eugene Rozanov, Laura Revell, David A. Plummer, Patrick Jöckel, Luke Oman, Makoto Deushi, Douglas E. Kinnison, Rolando Garcia, Olaf Morgenstern, Guang Zeng, Kane Adam Stone, and Robyn Schofield
Atmos. Chem. Phys., 19, 921–940, https://doi.org/10.5194/acp-19-921-2019, https://doi.org/10.5194/acp-19-921-2019, 2019
Short summary
Short summary
To shed more light upon the changes in stratospheric circulation in the 21st century, climate projection simulations of 10 state-of-the-art global climate models, spanning from 1960 to 2100, are analyzed. The study shows that in addition to changes in transport, mixing also plays an important role in stratospheric circulation and that the properties of mixing vary over time. Furthermore, the influence of mixing is quantified and a dynamical framework is provided to understand the changes.
Wolfgang Woiwode, Andreas Dörnbrack, Martina Bramberger, Felix Friedl-Vallon, Florian Haenel, Michael Höpfner, Sören Johansson, Erik Kretschmer, Isabell Krisch, Thomas Latzko, Hermann Oelhaf, Johannes Orphal, Peter Preusse, Björn-Martin Sinnhuber, and Jörn Ungermann
Atmos. Chem. Phys., 18, 15643–15667, https://doi.org/10.5194/acp-18-15643-2018, https://doi.org/10.5194/acp-18-15643-2018, 2018
Short summary
Short summary
GLORIA observations during two crossings of the polar front jet stream resolve the fine mesoscale structure of a tropopause fold in high detail. Tracer–tracer correlations of H2O and O3 are presented as a function of potential temperature and reveal an active mixing region. Our study confirms conceptual models of tropopause folds, validates the high quality of ECMWF IFS forecasts, and suggests that mountain waves are capable of modulating exchange processes in the vicinity of tropopause folds.
Michael Höpfner, Terry Deshler, Michael Pitts, Lamont Poole, Reinhold Spang, Gabriele Stiller, and Thomas von Clarmann
Atmos. Meas. Tech., 11, 5901–5923, https://doi.org/10.5194/amt-11-5901-2018, https://doi.org/10.5194/amt-11-5901-2018, 2018
Short summary
Short summary
Polar stratospheric clouds (PSC) have major relevance to the processes leading to polar ozone depletion. A good understanding of these particles is a prerequisite to predict their role in a changing climate. We present the first global set of PSC volume density profiles derived from the MIPAS satellite measurements covering the entire mission period between 2002 and 2012. A comparison to CALIOP lidar measurements is provided. The dataset can serve as a basis for evaluation of atmospheric models.
Norbert Glatthor, Thomas von Clarmann, Gabriele P. Stiller, Michael Kiefer, Alexandra Laeng, Bianca M. Dinelli, Gerald Wetzel, and Johannes Orphal
Atmos. Meas. Tech., 11, 4707–4723, https://doi.org/10.5194/amt-11-4707-2018, https://doi.org/10.5194/amt-11-4707-2018, 2018
Short summary
Short summary
We report differences in ozone retrievals in channels A and AB of the space-borne Michelson Interferometer for Passive Atmospheric Sounding (MIPAS), which amount to up to 8 %. We provide strong evidence that the bias is caused by inconsistencies in different spectroscopic databases (MIPAS, HITRAN, GEISA). We show that a major part of the differences can be attributed to inconsistent air-broadening coefficients of the ozone lines contained in the databases.
Alexandra Laeng, Ellen Eckert, Thomas von Clarmann, Michael Kiefer, Daan Hubert, Gabriele Stiller, Norbert Glatthor, Manuel López-Puertas, Bernd Funke, Udo Grabowski, Johannes Plieninger, Sylvia Kellmann, Andrea Linden, Stefan Lossow, Arne Babenhauserheide, Lucien Froidevaux, and Kaley Walker
Atmos. Meas. Tech., 11, 4693–4705, https://doi.org/10.5194/amt-11-4693-2018, https://doi.org/10.5194/amt-11-4693-2018, 2018
Short summary
Short summary
MIPAS was an IR limb emission spectrometer on the Envisat platform. From 2002 to 2012, it performed pole-to-pole measurements of ozone during day and night. ESA recently released the new version 7 of Level 1 MIPAS spectra, which is expected to reduce the long-term drift of the MIPAS Level 2 data. We evaluate the long-term stability of ozone Level 2 data from the KIT IMK processor. Our results indicate that MIPAS data are now even more suited for trend studies, alone or as part of merged data.
Farahnaz Khosrawi, Stefan Lossow, Gabriele P. Stiller, Karen H. Rosenlof, Joachim Urban, John P. Burrows, Robert P. Damadeo, Patrick Eriksson, Maya García-Comas, John C. Gille, Yasuko Kasai, Michael Kiefer, Gerald E. Nedoluha, Stefan Noël, Piera Raspollini, William G. Read, Alexei Rozanov, Christopher E. Sioris, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 11, 4435–4463, https://doi.org/10.5194/amt-11-4435-2018, https://doi.org/10.5194/amt-11-4435-2018, 2018
Short summary
Short summary
Time series of stratospheric and lower mesospheric water vapour using 33 data sets from 15 satellite instruments were compared in the framework of the second SPARC water vapour assessment. We find that most data sets can be considered in observational and modelling studies addressing, e.g. stratospheric and lower mesospheric water vapour variability and trends if data-set-specific characteristics (e.g. a drift) and restrictions (e.g. temporal and spatial coverage) are taken into account.
Farahnaz Khosrawi, Oliver Kirner, Gabriele Stiller, Michael Höpfner, Michelle L. Santee, Sylvia Kellmann, and Peter Braesicke
Atmos. Chem. Phys., 18, 8873–8892, https://doi.org/10.5194/acp-18-8873-2018, https://doi.org/10.5194/acp-18-8873-2018, 2018
Short summary
Short summary
An extensive assessment of the performance of the chemistry–climate model EMAC is given for Arctic winters 2009/2010 and 2010/2011. The EMAC simulations are compared to satellite observations. The comparisons between EMAC simulations and satellite observations show that model and measurements compare well for these two Arctic winters. However, differences between model and observations are found that need improvements in the model in the future.
Stefan Lossow, Dale F. Hurst, Karen H. Rosenlof, Gabriele P. Stiller, Thomas von Clarmann, Sabine Brinkop, Martin Dameris, Patrick Jöckel, Doug E. Kinnison, Johannes Plieninger, David A. Plummer, Felix Ploeger, William G. Read, Ellis E. Remsberg, James M. Russell, and Mengchu Tao
Atmos. Chem. Phys., 18, 8331–8351, https://doi.org/10.5194/acp-18-8331-2018, https://doi.org/10.5194/acp-18-8331-2018, 2018
Short summary
Short summary
Trend estimates of lower stratospheric H2O derived from the FPH observations at Boulder and a merged zonal mean satellite data set clearly differ for the time period from the late 1980s to 2010. We investigate if a sampling bias between Boulder and the zonal mean around the Boulder latitude can explain these trend discrepancies. Typically they are small and not sufficient to explain the trend discrepancies in the observational database.
Felicia Kolonjari, David A. Plummer, Kaley A. Walker, Chris D. Boone, James W. Elkins, Michaela I. Hegglin, Gloria L. Manney, Fred L. Moore, Diane Pendlebury, Eric A. Ray, Karen H. Rosenlof, and Gabriele P. Stiller
Atmos. Chem. Phys., 18, 6801–6828, https://doi.org/10.5194/acp-18-6801-2018, https://doi.org/10.5194/acp-18-6801-2018, 2018
Short summary
Short summary
We used satellite observations and model simulations of CFC-11, CFC-12, and N2O to investigate stratospheric transport, which is important for predicting the recovery of the ozone layer and future climate. We found that sampling can impact results and that the model consistently overestimates concentrations of these gases in the lower stratosphere, consistent with a too rapid Brewer–Dobson circulation. An issue with mixing in the tropical lower stratosphere in June–July–August was also found.
Simone Dietmüller, Roland Eichinger, Hella Garny, Thomas Birner, Harald Boenisch, Giovanni Pitari, Eva Mancini, Daniele Visioni, Andrea Stenke, Laura Revell, Eugene Rozanov, David A. Plummer, John Scinocca, Patrick Jöckel, Luke Oman, Makoto Deushi, Shibata Kiyotaka, Douglas E. Kinnison, Rolando Garcia, Olaf Morgenstern, Guang Zeng, Kane Adam Stone, and Robyn Schofield
Atmos. Chem. Phys., 18, 6699–6720, https://doi.org/10.5194/acp-18-6699-2018, https://doi.org/10.5194/acp-18-6699-2018, 2018
Manuel López-Puertas, Maya García-Comas, Bernd Funke, Angela Gardini, Gabriele P. Stiller, Thomas von Clarmann, Norbert Glatthor, Alexandra Laeng, Martin Kaufmann, Viktoria F. Sofieva, Lucien Froidevaux, Kaley A. Walker, and Masato Shiotani
Atmos. Meas. Tech., 11, 2187–2212, https://doi.org/10.5194/amt-11-2187-2018, https://doi.org/10.5194/amt-11-2187-2018, 2018
Short summary
Short summary
This paper describes the inversion of O3 data from MIPAS middle atmosphere spectra which requires non-LTE. The O3 dataset comprises from 20 to 100 km, has a pole-to-pole latitude coverage, day and nighttime, and span from 2005 until 2012. A validation of the data against other satellite measurements and an overall description of O3 is also presented. This is an important dataset for the community and describes the major characteristics of stratospheric and mesospheric O3.
Neal Butchart, James A. Anstey, Kevin Hamilton, Scott Osprey, Charles McLandress, Andrew C. Bushell, Yoshio Kawatani, Young-Ha Kim, Francois Lott, John Scinocca, Timothy N. Stockdale, Martin Andrews, Omar Bellprat, Peter Braesicke, Chiara Cagnazzo, Chih-Chieh Chen, Hye-Yeong Chun, Mikhail Dobrynin, Rolando R. Garcia, Javier Garcia-Serrano, Lesley J. Gray, Laura Holt, Tobias Kerzenmacher, Hiroaki Naoe, Holger Pohlmann, Jadwiga H. Richter, Adam A. Scaife, Verena Schenzinger, Federico Serva, Stefan Versick, Shingo Watanabe, Kohei Yoshida, and Seiji Yukimoto
Geosci. Model Dev., 11, 1009–1032, https://doi.org/10.5194/gmd-11-1009-2018, https://doi.org/10.5194/gmd-11-1009-2018, 2018
Short summary
Short summary
This paper documents the numerical experiments to be used in phase 1 of the Stratosphere–troposphere Processes And their Role in Climate (SPARC) Quasi-Biennial Oscillation initiative (QBOi), which was set up to improve the representation of the QBO and tropical stratospheric variability in global climate models.
Minqiang Zhou, Bavo Langerock, Corinne Vigouroux, Pucai Wang, Christian Hermans, Gabriele Stiller, Kaley A. Walker, Geoff Dutton, Emmanuel Mahieu, and Martine De Mazière
Atmos. Meas. Tech., 11, 651–662, https://doi.org/10.5194/amt-11-651-2018, https://doi.org/10.5194/amt-11-651-2018, 2018
Short summary
Short summary
SF6 total columns are successfully retrieved from FTIR measurements (Saint Denis and Maïdo) at Reunion Island (21° S, 55° E) between 2004 and 2016 using the SFIT4 algorithm: the retrieval strategy and the error budget are discussed. The trend of SF6 is analysed based on the FTIR retrievals at Reunion Island, the in situ measurements at America Samoa (SMO) and the collocated satellite measurements (MIPAS and ACE-FTS) in the southern tropics. The results show good agreement.
Annika Günther, Michael Höpfner, Björn-Martin Sinnhuber, Sabine Griessbach, Terry Deshler, Thomas von Clarmann, and Gabriele Stiller
Atmos. Chem. Phys., 18, 1217–1239, https://doi.org/10.5194/acp-18-1217-2018, https://doi.org/10.5194/acp-18-1217-2018, 2018
Short summary
Short summary
Satellite-borne data of sulfur dioxide and a new data set of sulfate aerosol volume densities, as retrieved from MIPAS measurements, are studied in the upper-troposphere–lower-stratosphere region. General patterns of enhanced aerosol are in agreement with SO2. Via chemical transport model simulations for two volcanic eruptions in the Northern Hemisphere midlatitudes, we show that the volcanic enhancements in MIPAS SO2 and sulfate aerosol are consistent in terms of mass and transport patterns.
Miriam Sinnhuber, Uwe Berger, Bernd Funke, Holger Nieder, Thomas Reddmann, Gabriele Stiller, Stefan Versick, Thomas von Clarmann, and Jan Maik Wissing
Atmos. Chem. Phys., 18, 1115–1147, https://doi.org/10.5194/acp-18-1115-2018, https://doi.org/10.5194/acp-18-1115-2018, 2018
Short summary
Short summary
Results from global models are used to analyze the impact of energetic particle precipitation on the middle atmosphere (10–80 km). Model results agree well with observations, and show strong enhancements of NOy, long-lasting ozone loss, and a net heating in the uppermost stratosphere (~35–45 km) during polar winter which changes sign in spring. Energetic particle precipitation therefore has the potential to impact atmospheric dynamics, starting from a warmer winter-time upper stratosphere.
Gerald E. Nedoluha, Michael Kiefer, Stefan Lossow, R. Michael Gomez, Niklaus Kämpfer, Martin Lainer, Peter Forkman, Ole Martin Christensen, Jung Jin Oh, Paul Hartogh, John Anderson, Klaus Bramstedt, Bianca M. Dinelli, Maya Garcia-Comas, Mark Hervig, Donal Murtagh, Piera Raspollini, William G. Read, Karen Rosenlof, Gabriele P. Stiller, and Kaley A. Walker
Atmos. Chem. Phys., 17, 14543–14558, https://doi.org/10.5194/acp-17-14543-2017, https://doi.org/10.5194/acp-17-14543-2017, 2017
Short summary
Short summary
As part of the second SPARC (Stratosphere–troposphere Processes And their Role in Climate) water vapor assessment (WAVAS-II), we present measurements taken from or coincident with seven sites from which ground-based microwave instruments measure water vapor in the middle atmosphere. In the lower mesosphere, we quantify instrumental differences in the observed trends and annual variations at six sites. We then present a range of observed trends in water vapor over the past 20 years.
Viktoria F. Sofieva, Erkki Kyrölä, Marko Laine, Johanna Tamminen, Doug Degenstein, Adam Bourassa, Chris Roth, Daniel Zawada, Mark Weber, Alexei Rozanov, Nabiz Rahpoe, Gabriele Stiller, Alexandra Laeng, Thomas von Clarmann, Kaley A. Walker, Patrick Sheese, Daan Hubert, Michel van Roozendael, Claus Zehner, Robert Damadeo, Joseph Zawodny, Natalya Kramarova, and Pawan K. Bhartia
Atmos. Chem. Phys., 17, 12533–12552, https://doi.org/10.5194/acp-17-12533-2017, https://doi.org/10.5194/acp-17-12533-2017, 2017
Short summary
Short summary
We present a merged dataset of ozone profiles from several satellite instruments: SAGE II, GOMOS, SCIAMACHY, MIPAS, OSIRIS, ACE-FTS and OMPS. For merging, we used the latest versions of the original ozone datasets.
The merged SAGE–CCI–OMPS dataset is used for evaluating ozone trends in the stratosphere through multiple linear regression. Negative ozone trends in the upper stratosphere are observed before 1997 and positive trends are found after 1997.
Stefan Lossow, Hella Garny, and Patrick Jöckel
Atmos. Chem. Phys., 17, 11521–11539, https://doi.org/10.5194/acp-17-11521-2017, https://doi.org/10.5194/acp-17-11521-2017, 2017
Roland Eichinger, Gary Shaffer, Nelson Albarrán, Maisa Rojas, and Fabrice Lambert
Geosci. Model Dev., 10, 3481–3498, https://doi.org/10.5194/gmd-10-3481-2017, https://doi.org/10.5194/gmd-10-3481-2017, 2017
Short summary
Short summary
We reformulate the land biosphere of the reduced-complexity DCESS model by introducing three vegetation types and relating their latitudinal borders to global temperature change. This enhancement yields more realistic estimates of biosphere carbon cycling for cold conditions like the Last Glacial Maximum. As a first application we conduct transient simulations across the last glacial termination to estimate the importance of different processes on temperature, pCO2 and carbon isotope ratios.
Gabriele P. Stiller, Federico Fierli, Felix Ploeger, Chiara Cagnazzo, Bernd Funke, Florian J. Haenel, Thomas Reddmann, Martin Riese, and Thomas von Clarmann
Atmos. Chem. Phys., 17, 11177–11192, https://doi.org/10.5194/acp-17-11177-2017, https://doi.org/10.5194/acp-17-11177-2017, 2017
Short summary
Short summary
The discrepancy between modelled and observed 25-year trends of the strength of the stratospheric Brewer–Dobson circulation (BDC) is still not resolved. With our paper we trace the observed hemispheric dipole structure of age of air trends back to natural variability in shorter-term (decadal) time frames. Beyond this we demonstrate that after correction for the decadal natural variability the remaining trend for the first decade of the 21st century is consistent with model simulations.
Wolfgang Steinbrecht, Lucien Froidevaux, Ryan Fuller, Ray Wang, John Anderson, Chris Roth, Adam Bourassa, Doug Degenstein, Robert Damadeo, Joe Zawodny, Stacey Frith, Richard McPeters, Pawan Bhartia, Jeannette Wild, Craig Long, Sean Davis, Karen Rosenlof, Viktoria Sofieva, Kaley Walker, Nabiz Rahpoe, Alexei Rozanov, Mark Weber, Alexandra Laeng, Thomas von Clarmann, Gabriele Stiller, Natalya Kramarova, Sophie Godin-Beekmann, Thierry Leblanc, Richard Querel, Daan Swart, Ian Boyd, Klemens Hocke, Niklaus Kämpfer, Eliane Maillard Barras, Lorena Moreira, Gerald Nedoluha, Corinne Vigouroux, Thomas Blumenstock, Matthias Schneider, Omaira García, Nicholas Jones, Emmanuel Mahieu, Dan Smale, Michael Kotkamp, John Robinson, Irina Petropavlovskikh, Neil Harris, Birgit Hassler, Daan Hubert, and Fiona Tummon
Atmos. Chem. Phys., 17, 10675–10690, https://doi.org/10.5194/acp-17-10675-2017, https://doi.org/10.5194/acp-17-10675-2017, 2017
Short summary
Short summary
Thanks to the 1987 Montreal Protocol and its amendments, ozone-depleting chlorine (and bromine) in the stratosphere has declined slowly since the late 1990s. Improved and extended long-term ozone profile observations from satellites and ground-based stations confirm that ozone is responding as expected and has increased by about 2 % per decade since 2000 in the upper stratosphere, around 40 km altitude. At lower altitudes, however, ozone has not changed significantly since 2000.
Ellen Eckert, Thomas von Clarmann, Alexandra Laeng, Gabriele P. Stiller, Bernd Funke, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Michael Kiefer, Andrea Linden, Arne Babenhauserheide, Gerald Wetzel, Christopher Boone, Andreas Engel, Jeremy J. Harrison, Patrick E. Sheese, Kaley A. Walker, and Peter F. Bernath
Atmos. Meas. Tech., 10, 2727–2743, https://doi.org/10.5194/amt-10-2727-2017, https://doi.org/10.5194/amt-10-2727-2017, 2017
Short summary
Short summary
We retrieved vertical profiles of CCl4 from MIPAS Envisat IMK/IAA data. A detailed description of all characteristics is included in the paper as well as comparisons with historical measurements and comparisons with collocated measurements of instruments covering the same time span as MIPAS Envisat. A particular focus also lies on the usage of a new CCl4 spectroscopic dataset introduced recently, which leads to more realistic CCl4 volume mixing ratios.
Michael Weimer, Jennifer Schröter, Johannes Eckstein, Konrad Deetz, Marco Neumaier, Garlich Fischbeck, Lu Hu, Dylan B. Millet, Daniel Rieger, Heike Vogel, Bernhard Vogel, Thomas Reddmann, Oliver Kirner, Roland Ruhnke, and Peter Braesicke
Geosci. Model Dev., 10, 2471–2494, https://doi.org/10.5194/gmd-10-2471-2017, https://doi.org/10.5194/gmd-10-2471-2017, 2017
Short summary
Short summary
In this paper, the recently developed module for trace gas emissions in the online coupled modelling framework ICON-ART for atmospheric chemistry is presented. Algorithms for offline and online calculation of the emissions are described. The module is validated with ground-based as well as airborne measurements of acetone. It is shown that the module performs well and allows the simulation of annual cycles of emission-driven trace gases.
Simone Dietmüller, Hella Garny, Felix Plöger, Patrick Jöckel, and Duy Cai
Atmos. Chem. Phys., 17, 7703–7719, https://doi.org/10.5194/acp-17-7703-2017, https://doi.org/10.5194/acp-17-7703-2017, 2017
Katja Matthes, Bernd Funke, Monika E. Andersson, Luke Barnard, Jürg Beer, Paul Charbonneau, Mark A. Clilverd, Thierry Dudok de Wit, Margit Haberreiter, Aaron Hendry, Charles H. Jackman, Matthieu Kretzschmar, Tim Kruschke, Markus Kunze, Ulrike Langematz, Daniel R. Marsh, Amanda C. Maycock, Stergios Misios, Craig J. Rodger, Adam A. Scaife, Annika Seppälä, Ming Shangguan, Miriam Sinnhuber, Kleareti Tourpali, Ilya Usoskin, Max van de Kamp, Pekka T. Verronen, and Stefan Versick
Geosci. Model Dev., 10, 2247–2302, https://doi.org/10.5194/gmd-10-2247-2017, https://doi.org/10.5194/gmd-10-2247-2017, 2017
Short summary
Short summary
The solar forcing dataset for climate model experiments performed for the upcoming IPCC report is described. This dataset provides the radiative and particle input of solar variability on a daily basis from 1850 through to 2300. With this dataset a better representation of natural climate variability with respect to the output of the Sun is provided which provides the most sophisticated and comprehensive respresentation of solar variability that has been used in climate model simulations so far.
Alexandra Laeng, Thomas von Clarmann, Gabriele Stiller, Bianca Maria Dinelli, Anu Dudhia, Piera Raspollini, Norbert Glatthor, Udo Grabowski, Viktoria Sofieva, Lucien Froidevaux, Kaley A. Walker, and Claus Zehner
Atmos. Meas. Tech., 10, 1511–1518, https://doi.org/10.5194/amt-10-1511-2017, https://doi.org/10.5194/amt-10-1511-2017, 2017
Short summary
Short summary
A MIPAS instrument was flown in 2002–2012 on the Envisat satellite and measured atmospheric composition. There exist four processors retrieving atmospheric profiles from MIPAS spectra. We performed a mathematically clean merging of 2007–2008 datasets of ozone from these four processors. The merged product was compared with ozone datasets from ACE-FTS and MLS instruments. The advantages and the shortcomings of this merged product are discussed.
Stefan Lossow, Farahnaz Khosrawi, Gerald E. Nedoluha, Faiza Azam, Klaus Bramstedt, John. P. Burrows, Bianca M. Dinelli, Patrick Eriksson, Patrick J. Espy, Maya García-Comas, John C. Gille, Michael Kiefer, Stefan Noël, Piera Raspollini, William G. Read, Karen H. Rosenlof, Alexei Rozanov, Christopher E. Sioris, Gabriele P. Stiller, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 10, 1111–1137, https://doi.org/10.5194/amt-10-1111-2017, https://doi.org/10.5194/amt-10-1111-2017, 2017
Bernd Funke, William Ball, Stefan Bender, Angela Gardini, V. Lynn Harvey, Alyn Lambert, Manuel López-Puertas, Daniel R. Marsh, Katharina Meraner, Holger Nieder, Sanna-Mari Päivärinta, Kristell Pérot, Cora E. Randall, Thomas Reddmann, Eugene Rozanov, Hauke Schmidt, Annika Seppälä, Miriam Sinnhuber, Timofei Sukhodolov, Gabriele P. Stiller, Natalia D. Tsvetkova, Pekka T. Verronen, Stefan Versick, Thomas von Clarmann, Kaley A. Walker, and Vladimir Yushkov
Atmos. Chem. Phys., 17, 3573–3604, https://doi.org/10.5194/acp-17-3573-2017, https://doi.org/10.5194/acp-17-3573-2017, 2017
Short summary
Short summary
Simulations from eight atmospheric models have been compared to tracer and temperature observations from seven satellite instruments in order to evaluate the energetic particle indirect effect (EPP IE) during the perturbed northern hemispheric (NH) winter 2008/2009. Models are capable to reproduce the EPP IE in dynamically and geomagnetically quiescent NH winter conditions. The results emphasize the need for model improvements in the dynamical representation of elevated stratopause events.
Norbert Glatthor, Michael Höpfner, Adrian Leyser, Gabriele P. Stiller, Thomas von Clarmann, Udo Grabowski, Sylvia Kellmann, Andrea Linden, Björn-Martin Sinnhuber, Gisèle Krysztofiak, and Kaley A. Walker
Atmos. Chem. Phys., 17, 2631–2652, https://doi.org/10.5194/acp-17-2631-2017, https://doi.org/10.5194/acp-17-2631-2017, 2017
Short summary
Short summary
To date, information on the global distribution of atmospheric carbonyl sulfide (OCS) is still rather sparse.
However, detailed knowledge of the OCS distribution is of scientific interest, because this trace gas is on one of the major sources of atmospheric sulfur, which is a prerequisite of the stratospheric aerosol layer. Under this aspect we present a comprehensive space-borne data set of global OCS concentrations covering the period from June 2002 to April 2012.
Tamás Kovács, Wuhu Feng, Anna Totterdill, John M. C. Plane, Sandip Dhomse, Juan Carlos Gómez-Martín, Gabriele P. Stiller, Florian J. Haenel, Christopher Smith, Piers M. Forster, Rolando R. García, Daniel R. Marsh, and Martyn P. Chipperfield
Atmos. Chem. Phys., 17, 883–898, https://doi.org/10.5194/acp-17-883-2017, https://doi.org/10.5194/acp-17-883-2017, 2017
Short summary
Short summary
Sulfur hexafluoride (SF6) is a very potent greenhouse gas, which is present in the atmosphere only through its industrial use, for example as an electrical insulator. To estimate accurately the impact of SF6 emissions on climate we need to know how long it persists in the atmosphere before being removed. Previous estimates of the SF6 lifetime indicate a large degree of uncertainty. Here we use a detailed atmospheric model to calculate a current best estimate of the SF6 lifetime.
Á. Aythami Jurado-Navarro, Manuel López-Puertas, Bernd Funke, Maya García-Comas, Angela Gardini, Francisco González-Galindo, Gabriele P. Stiller, Thomas von Clarmann, Udo Grabowski, and Andrea Linden
Atmos. Meas. Tech., 9, 6081–6100, https://doi.org/10.5194/amt-9-6081-2016, https://doi.org/10.5194/amt-9-6081-2016, 2016
Short summary
Short summary
We present global distributions of CO2 concentrations in the upper atmosphere (70–140 km) derived from high-resolution 4.3 µm MIPAS spectra from 2005 to 2012. CO2 relative abundances have been measured at 120–140 km for the first time. The data have an unprecedented accuracy. CO2 shows a strong seasonal behaviour. CO2 largely controls the temperature of the upper atmosphere and its measurement is very important for understanding the impact of climate change in this region.
Bastiaan Jonkheid, Thomas Röckmann, Norbert Glatthor, Christof Janssen, Gabriele Stiller, and Thomas von Clarmann
Atmos. Meas. Tech., 9, 6069–6079, https://doi.org/10.5194/amt-9-6069-2016, https://doi.org/10.5194/amt-9-6069-2016, 2016
Bärbel Vogel, Gebhard Günther, Rolf Müller, Jens-Uwe Grooß, Armin Afchine, Heiko Bozem, Peter Hoor, Martina Krämer, Stefan Müller, Martin Riese, Christian Rolf, Nicole Spelten, Gabriele P. Stiller, Jörn Ungermann, and Andreas Zahn
Atmos. Chem. Phys., 16, 15301–15325, https://doi.org/10.5194/acp-16-15301-2016, https://doi.org/10.5194/acp-16-15301-2016, 2016
Short summary
Short summary
The identification of transport pathways from the Asian monsoon anticyclone into the lower stratosphere is unclear. Global simulations with the CLaMS model demonstrate that source regions in Asia and in the Pacific Ocean have a significant impact on the chemical composition of the lower stratosphere of the Northern Hemisphere by flooding the extratropical lower stratosphere with young moist air masses. Two main horizontal transport pathways from the Asian monsoon anticyclone are identified.
Matthias Nützel, Martin Dameris, and Hella Garny
Atmos. Chem. Phys., 16, 14755–14774, https://doi.org/10.5194/acp-16-14755-2016, https://doi.org/10.5194/acp-16-14755-2016, 2016
Short summary
Short summary
Using seven reanalyses, we study the movement and drivers of the upper tropospheric–lower stratospheric anticyclone (AC) that forms during the Asian summer monsoon and is debated to be an important pathway for air masses to the stratosphere. We find that the distribution of the AC's centre position, and especially the so-called bimodality, largely depends on the reanalysis. Furthermore, we can connect shifts of the AC to precipitation and convection anomalies over India and the western Pacific.
Michael Höpfner, Rainer Volkamer, Udo Grabowski, Michel Grutter, Johannes Orphal, Gabriele Stiller, Thomas von Clarmann, and Gerald Wetzel
Atmos. Chem. Phys., 16, 14357–14369, https://doi.org/10.5194/acp-16-14357-2016, https://doi.org/10.5194/acp-16-14357-2016, 2016
Short summary
Short summary
Ammonia (NH3) in the atmosphere is important because of its influence on aerosol and cloud formation and its increasing anthropogenic emissions. We report the first detection of NH3 in the upper troposphere by the analysis of infrared limb emission spectra measured by the MIPAS instrument on Envisat. We have found enhanced values of NH3 within the Asian summer monsoon upper troposphere, where it might contribute to the composition of the Asian tropopause aerosol layer.
Duy Cai, Martin Dameris, Hella Garny, Felix Bunzel, Patrick Jöckel, and Phoebe Graf
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-870, https://doi.org/10.5194/acp-2016-870, 2016
Revised manuscript not accepted
Short summary
Short summary
Reliable information on weather and climate are of increasing interest for economy, politics and society.
In particular decadal timescales become more and more important. This study focuses on stratospheric processes relevant for the dynamical variability on intra decadal timescale. We apply a so called power spectra analysis. With this method and further analyses we could determine a minimum vertical resolution for numerical models, which is required to capture these processes.
Andreas Ostler, Ralf Sussmann, Prabir K. Patra, Sander Houweling, Marko De Bruine, Gabriele P. Stiller, Florian J. Haenel, Johannes Plieninger, Philippe Bousquet, Yi Yin, Marielle Saunois, Kaley A. Walker, Nicholas M. Deutscher, David W. T. Griffith, Thomas Blumenstock, Frank Hase, Thorsten Warneke, Zhiting Wang, Rigel Kivi, and John Robinson
Atmos. Meas. Tech., 9, 4843–4859, https://doi.org/10.5194/amt-9-4843-2016, https://doi.org/10.5194/amt-9-4843-2016, 2016
Short summary
Short summary
Our evaluation of column-averaged methane (XCH4) in models and TCCON reveals latitudinal biases between 0.4 % and 2.1 % originating from an inter-model spread in stratospheric CH4. Substituting model stratospheric CH4 fields by satellite data significantly reduces the large XCH4 bias observed for one model. For other models, showing only minor biases, the impact is ambiguous; i.e., the satellite uncertainty range hinders a more accurate model evaluation needed to improve inverse modeling.
E. Eckert, A. Laeng, S. Lossow, S. Kellmann, G. Stiller, T. von Clarmann, N. Glatthor, M. Höpfner, M. Kiefer, H. Oelhaf, J. Orphal, B. Funke, U. Grabowski, F. Haenel, A. Linden, G. Wetzel, W. Woiwode, P. F. Bernath, C. Boone, G. S. Dutton, J. W. Elkins, A. Engel, J. C. Gille, F. Kolonjari, T. Sugita, G. C. Toon, and K. A. Walker
Atmos. Meas. Tech., 9, 3355–3389, https://doi.org/10.5194/amt-9-3355-2016, https://doi.org/10.5194/amt-9-3355-2016, 2016
Short summary
Short summary
We investigate the accuracy, precision and long-term stability of the MIPAS Envisat IMK/IAA CFC-11 (CCl3F) and CFC-12 (CCl2F2) products.
For comparisons we use several data products from satellite, airplane and balloon-borne instruments as well as ground-based data.
MIPAS Envisat CFC-11 has a slight high bias at the lower end of the profile.
CFC-12 agrees well with other data products.
The temporal stability is good up to ~ 30 km, but still leaves room for improvement.
Markus Kunze, Peter Braesicke, Ulrike Langematz, and Gabriele Stiller
Atmos. Chem. Phys., 16, 8695–8714, https://doi.org/10.5194/acp-16-8695-2016, https://doi.org/10.5194/acp-16-8695-2016, 2016
Bernd Funke, Manuel López-Puertas, Gabriele P. Stiller, Stefan Versick, and Thomas von Clarmann
Atmos. Chem. Phys., 16, 8667–8693, https://doi.org/10.5194/acp-16-8667-2016, https://doi.org/10.5194/acp-16-8667-2016, 2016
Short summary
Short summary
We present a semi-empirical model for the reconstruction of polar winter descent of reactive nitrogen (NOy) produced by energetic particle precipitation (EPP) into the stratosphere. It can be used to prescribe NOy in chemistry climate models with an upper lid below the EPP source region. We also found a significant reduction of the EPP-generated NOy during the last 30 years, likely affecting the long-term NOy trend by counteracting the expected increase caused by growing N2O emission.
Khalil Karami, Peter Braesicke, Miriam Sinnhuber, and Stefan Versick
Atmos. Chem. Phys., 16, 8447–8460, https://doi.org/10.5194/acp-16-8447-2016, https://doi.org/10.5194/acp-16-8447-2016, 2016
Short summary
Short summary
We introduce a diagnostic tool to assess in a climatological framework the optimal propagation conditions for stationary planetary waves. Analyzing 50 winters using NCEP/NCAR reanalysis data we demonstrate several problematic features of the refractive index of Rossby waves. We introduced the Rossby waves membership value function to calculate the optimal propagation conditions for Rossby waves. Sensitivity of our diagnostic tool to strong and weak vortex regimes are examined.
Sabine Brinkop, Martin Dameris, Patrick Jöckel, Hella Garny, Stefan Lossow, and Gabriele Stiller
Atmos. Chem. Phys., 16, 8125–8140, https://doi.org/10.5194/acp-16-8125-2016, https://doi.org/10.5194/acp-16-8125-2016, 2016
Short summary
Short summary
This study investigates the water vapour decline in the stratosphere beginning in the year 2000 and other similarly strong stratospheric water vapour reductions. The driving forces are tropical sea surface temperature (SST) changes due to coincidence with a preceding ENSO event and supported by the west to east change of the QBO.
There are indications that both SSTs and the specific dynamical state of the atmosphere contribute to the long period of low water vapour values from 2001 to 2006.
Maya García-Comas, Manuel López-Puertas, Bernd Funke, Á. Aythami Jurado-Navarro, Angela Gardini, Gabriele P. Stiller, Thomas von Clarmann, and Michael Höpfner
Atmos. Chem. Phys., 16, 6701–6719, https://doi.org/10.5194/acp-16-6701-2016, https://doi.org/10.5194/acp-16-6701-2016, 2016
Short summary
Short summary
We have analysed IR measurements of PMCs in the NH and SH from 2005 to 2012. This technique is sensitive to the total ice volume independent of particle size. For the first time, we have measured the total ice volume from the midlatitudes to the poles. The data indicate a layer of ice from 81 to 89 km and from the poles to 50–60º in each hemisphere, increasing near the poles. The ice density is larger in the NH than in the SH and located 1 km lower. PMCs also show a diurnal variation.
Patrick Jöckel, Holger Tost, Andrea Pozzer, Markus Kunze, Oliver Kirner, Carl A. M. Brenninkmeijer, Sabine Brinkop, Duy S. Cai, Christoph Dyroff, Johannes Eckstein, Franziska Frank, Hella Garny, Klaus-Dirk Gottschaldt, Phoebe Graf, Volker Grewe, Astrid Kerkweg, Bastian Kern, Sigrun Matthes, Mariano Mertens, Stefanie Meul, Marco Neumaier, Matthias Nützel, Sophie Oberländer-Hayn, Roland Ruhnke, Theresa Runde, Rolf Sander, Dieter Scharffe, and Andreas Zahn
Geosci. Model Dev., 9, 1153–1200, https://doi.org/10.5194/gmd-9-1153-2016, https://doi.org/10.5194/gmd-9-1153-2016, 2016
Short summary
Short summary
With an advanced numerical global chemistry climate model (CCM) we performed several detailed
combined hind-cast and projection simulations of the period 1950 to 2100 to assess the
past, present, and potential future dynamical and chemical state of the Earth atmosphere.
The manuscript documents the model and the various applied model set-ups and provides
a first evaluation of the simulation results from a global perspective as a quality check of the data.
M. Chirkov, G. P. Stiller, A. Laeng, S. Kellmann, T. von Clarmann, C. D. Boone, J. W. Elkins, A. Engel, N. Glatthor, U. Grabowski, C. M. Harth, M. Kiefer, F. Kolonjari, P. B. Krummel, A. Linden, C. R. Lunder, B. R. Miller, S. A. Montzka, J. Mühle, S. O'Doherty, J. Orphal, R. G. Prinn, G. Toon, M. K. Vollmer, K. A. Walker, R. F. Weiss, A. Wiegele, and D. Young
Atmos. Chem. Phys., 16, 3345–3368, https://doi.org/10.5194/acp-16-3345-2016, https://doi.org/10.5194/acp-16-3345-2016, 2016
Short summary
Short summary
HCFC-22 global distributions from MIPAS measurements for 2005 to 2012 are presented. Tropospheric trends are in good agreement with ground-based observations. A layer of enhanced HCFC-22 in the upper tropospheric tropics and northern subtropics is identified to come from Asian sources uplifted in the Asian monsoon. Stratospheric distributions provide show seasonal, semi-annual, and QBO-related variations. Hemispheric asymmetries of trends hint towards a change in the stratospheric circulation.
Hella Garny and William J. Randel
Atmos. Chem. Phys., 16, 2703–2718, https://doi.org/10.5194/acp-16-2703-2016, https://doi.org/10.5194/acp-16-2703-2016, 2016
Short summary
Short summary
We investigate the fate of air that originates in the monsoon region in the upper troposphere, where it was transported to by convection. We find that almost half of the air parcels released in the monsoon region in the upper troposphere reach the stratosphere within 60 days, and most ascend to the tropical lower stratosphere. This suggests that trace gases, including pollutants, that are transported into the stratosphere via the Asian monsoon are in a position to enter the deep stratosphere.
Johannes Plieninger, Alexandra Laeng, Stefan Lossow, Thomas von Clarmann, Gabriele P. Stiller, Sylvia Kellmann, Andrea Linden, Michael Kiefer, Kaley A. Walker, Stefan Noël, Mark E. Hervig, Martin McHugh, Alyn Lambert, Joachim Urban, James W. Elkins, and Donal Murtagh
Atmos. Meas. Tech., 9, 765–779, https://doi.org/10.5194/amt-9-765-2016, https://doi.org/10.5194/amt-9-765-2016, 2016
Short summary
Short summary
We compare concentration profiles of methane and nitrous oxide measured from MIPAS-ENVISAT and derived with a new retrieval setup to those measured by other satellite instruments and to surface measurements. For methane we use profiles measured by ACE-FTS, HALOE and SCIAMACHY; for nitrous oxide we use profiles measured by ACE-FTS, Aura-MLS and Odin-SMR for the comparisons. We give a quantitative bias estimation and compare the estimated errors provided by the instruments.
K. Weigel, A. Rozanov, F. Azam, K. Bramstedt, R. Damadeo, K.-U. Eichmann, C. Gebhardt, D. Hurst, M. Kraemer, S. Lossow, W. Read, N. Spelten, G. P. Stiller, K. A. Walker, M. Weber, H. Bovensmann, and J. P. Burrows
Atmos. Meas. Tech., 9, 133–158, https://doi.org/10.5194/amt-9-133-2016, https://doi.org/10.5194/amt-9-133-2016, 2016
Short summary
Short summary
The SCanning Imaging Absorption spectroMeter for Atmospheric CHartographY (SCIAMACHY) aboard the Envisat satellite provided measurements between 2002 and 2012 with different viewing geometries. The limb viewing geometry allows the retrieval of water vapour profiles in the UTLS (upper troposphere and lower stratosphere) from the near-infrared spectral range (1353–1410 nm). Here, we present data version 3.01 and compare it to other water vapour data.
Roland Eichinger, Gary Shaffer, Nelson Albarrán, Maisa Rojas, and Fabrice Lambert
Clim. Past Discuss., https://doi.org/10.5194/cp-2015-190, https://doi.org/10.5194/cp-2015-190, 2016
Revised manuscript not accepted
Short summary
Short summary
We apply the DCESS ESM to assess the process of Southern Ocean deep water upwelling as to whether it can explain the climate change between 17.5 and 14.5 kaBP. From a glacial climate state, which was generated under the guidance of proxy data records, transient climate simulations are conducted to analyse the impact of various parameters. This approach can explain parts but not all of the observed atmospheric variations in temperatures, carbon dioxide and carbon isotopes across that period.
F. Khosrawi, J. Urban, S. Lossow, G. Stiller, K. Weigel, P. Braesicke, M. C. Pitts, A. Rozanov, J. P. Burrows, and D. Murtagh
Atmos. Chem. Phys., 16, 101–121, https://doi.org/10.5194/acp-16-101-2016, https://doi.org/10.5194/acp-16-101-2016, 2016
Short summary
Short summary
Our sensitivity studies based on air parcel trajectories confirm that Polar stratospheric cloud (PSC) formation is quite sensitive to water vapour and temperature changes. Considering water vapour time series from satellite measurements we do not find a consistent, significant trend in water vapour in the lower stratosphere during the past 15 years (2000–2014). Thus, the severe dentrification observed in 2010/2011 cannot be directly related to increases in stratospheric water vapour.
A. Laeng, J. Plieninger, T. von Clarmann, U. Grabowski, G. Stiller, E. Eckert, N. Glatthor, F. Haenel, S. Kellmann, M. Kiefer, A. Linden, S. Lossow, L. Deaver, A. Engel, M. Hervig, I. Levin, M. McHugh, S. Noël, G. Toon, and K. Walker
Atmos. Meas. Tech., 8, 5251–5261, https://doi.org/10.5194/amt-8-5251-2015, https://doi.org/10.5194/amt-8-5251-2015, 2015
F. J. Haenel, G. P. Stiller, T. von Clarmann, B. Funke, E. Eckert, N. Glatthor, U. Grabowski, S. Kellmann, M. Kiefer, A. Linden, and T. Reddmann
Atmos. Chem. Phys., 15, 13161–13176, https://doi.org/10.5194/acp-15-13161-2015, https://doi.org/10.5194/acp-15-13161-2015, 2015
Short summary
Short summary
Stratospheric circulation is thought to change as a consequence of climate change. Empirical evidence, however, is sparse. In this paper we present latitude- and altitude-resolved trends of the mean age of stratospheric air as derived from SF6 measurements performed by the MIPAS satellite instrument. The mean of the age of stratospheric air is a measure of the intensity of the Brewer-Dobson circulation. In this paper we discuss differences with respect to a preceding analysis by Stiller et al.
K. Karami, P. Braesicke, M. Kunze, U. Langematz, M. Sinnhuber, and S. Versick
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-15-33283-2015, https://doi.org/10.5194/acpd-15-33283-2015, 2015
Revised manuscript has not been submitted
J. Plieninger, T. von Clarmann, G. P. Stiller, U. Grabowski, N. Glatthor, S. Kellmann, A. Linden, F. Haenel, M. Kiefer, M. Höpfner, A. Laeng, and S. Lossow
Atmos. Meas. Tech., 8, 4657–4670, https://doi.org/10.5194/amt-8-4657-2015, https://doi.org/10.5194/amt-8-4657-2015, 2015
Short summary
Short summary
We present our revised CH4 and N2O profiles derived from MIPAS-ENVISAT spectra, which are now available for the entire measurement period. We describe the retrieval of the profiles and discuss the improvements compared to earlier versions and their effect on the mixing ratios. We analyse the averaging kernels and the resolution of the profiles. An error discussion for both gases is given.
N. Rahpoe, M. Weber, A. V. Rozanov, K. Weigel, H. Bovensmann, J. P. Burrows, A. Laeng, G. Stiller, T. von Clarmann, E. Kyrölä, V. F. Sofieva, J. Tamminen, K. Walker, D. Degenstein, A. E. Bourassa, R. Hargreaves, P. Bernath, J. Urban, and D. P. Murtagh
Atmos. Meas. Tech., 8, 4369–4381, https://doi.org/10.5194/amt-8-4369-2015, https://doi.org/10.5194/amt-8-4369-2015, 2015
Short summary
Short summary
The analyses among six satellite instruments measuring ozone reveals that the relative drift between the sensors is not significant in the stratosphere and we conclude that merging of data from these instruments is possible. The merged ozone profiles can then be ingested in global climate models for long-term forecasts of ozone and climate change in the atmosphere. The added drift uncertainty is estimated at about 3% per decade (1 sigma) and should be applied in the calculation of ozone trends.
S. Bender, M. Sinnhuber, T. von Clarmann, G. Stiller, B. Funke, M. López-Puertas, J. Urban, K. Pérot, K. A. Walker, and J. P. Burrows
Atmos. Meas. Tech., 8, 4171–4195, https://doi.org/10.5194/amt-8-4171-2015, https://doi.org/10.5194/amt-8-4171-2015, 2015
Short summary
Short summary
We compare the nitric oxide (NO) daily zonal mean number density data sets in the mesosphere and lower thermosphere (MLT, 60km to 150km) from four instruments: ACE-FTS (2004--2010), MIPAS (2005--2012), SCIAMACHY (2008--2012), and SMR (2003--2012). We find that these data sets from different instruments consistently constrain NO in the MLT. Thus, they offer reliable forcing inputs for climate and chemistry climate models as an initial step to include solar and geomagnetic activity.
T. Schieferdecker, S. Lossow, G. P. Stiller, and T. von Clarmann
Atmos. Chem. Phys., 15, 9851–9863, https://doi.org/10.5194/acp-15-9851-2015, https://doi.org/10.5194/acp-15-9851-2015, 2015
Short summary
Short summary
A merged data set of HALOE and MIPAS lower stratospheric water vapour has been constructed. Multivariate linear regression shows that the merged time series can best be explained if a proxy for the 11-year solar cycle is considered. The amplitude of the solar cycle signal in water vapour is slightly higher than that which can be explained by the known solar cycle variation of cold-point temperatures.
R. Eichinger, P. Jöckel, and S. Lossow
Atmos. Chem. Phys., 15, 7003–7015, https://doi.org/10.5194/acp-15-7003-2015, https://doi.org/10.5194/acp-15-7003-2015, 2015
M. Höpfner, C. D. Boone, B. Funke, N. Glatthor, U. Grabowski, A. Günther, S. Kellmann, M. Kiefer, A. Linden, S. Lossow, H. C. Pumphrey, W. G. Read, A. Roiger, G. Stiller, H. Schlager, T. von Clarmann, and K. Wissmüller
Atmos. Chem. Phys., 15, 7017–7037, https://doi.org/10.5194/acp-15-7017-2015, https://doi.org/10.5194/acp-15-7017-2015, 2015
L. E. Revell, F. Tummon, A. Stenke, T. Sukhodolov, A. Coulon, E. Rozanov, H. Garny, V. Grewe, and T. Peter
Atmos. Chem. Phys., 15, 5887–5902, https://doi.org/10.5194/acp-15-5887-2015, https://doi.org/10.5194/acp-15-5887-2015, 2015
Short summary
Short summary
We have examined the effects of ozone precursor emissions and climate change on the tropospheric ozone budget. Under RCP 6.0, ozone in the future is governed primarily by changes in nitrogen oxides (NOx). Methane is also important, and induces an increase in tropospheric ozone that is approximately one-third of that caused by NOx. This study highlights the critical role that emission policies globally have to play in determining tropospheric ozone evolution through the 21st century.
R. Eichinger, P. Jöckel, S. Brinkop, M. Werner, and S. Lossow
Atmos. Chem. Phys., 15, 5537–5555, https://doi.org/10.5194/acp-15-5537-2015, https://doi.org/10.5194/acp-15-5537-2015, 2015
T. Fytterer, M. G. Mlynczak, H. Nieder, K. Pérot, M. Sinnhuber, G. Stiller, and J. Urban
Atmos. Chem. Phys., 15, 3327–3338, https://doi.org/10.5194/acp-15-3327-2015, https://doi.org/10.5194/acp-15-3327-2015, 2015
Short summary
Short summary
Energetic particles from the sun produce NOx (=N+NO+NO2) in the mesosphere/lower thermosphere. The NOx can be transported downward in the stratosphere during polar winter where NOx eventually depletes O3. This entire chain is the so-called energetic particle precipitation (EPP) indirect effect.
Here we show downward propagating negative stratospheric O3 anomalies during Antarctic polar winter. The O3 anomalies are caused by geomagnetic activity and show strong hints of the EPP indirect effect.
N. Glatthor, M. Höpfner, G. P. Stiller, T. von Clarmann, B. Funke, S. Lossow, E. Eckert, U. Grabowski, S. Kellmann, A. Linden, K. A. Walker, and A. Wiegele
Atmos. Chem. Phys., 15, 563–582, https://doi.org/10.5194/acp-15-563-2015, https://doi.org/10.5194/acp-15-563-2015, 2015
A. Laeng, U. Grabowski, T. von Clarmann, G. Stiller, N. Glatthor, M. Höpfner, S. Kellmann, M. Kiefer, A. Linden, S. Lossow, V. Sofieva, I. Petropavlovskikh, D. Hubert, T. Bathgate, P. Bernath, C. D. Boone, C. Clerbaux, P. Coheur, R. Damadeo, D. Degenstein, S. Frith, L. Froidevaux, J. Gille, K. Hoppel, M. McHugh, Y. Kasai, J. Lumpe, N. Rahpoe, G. Toon, T. Sano, M. Suzuki, J. Tamminen, J. Urban, K. Walker, M. Weber, and J. Zawodny
Atmos. Meas. Tech., 7, 3971–3987, https://doi.org/10.5194/amt-7-3971-2014, https://doi.org/10.5194/amt-7-3971-2014, 2014
M. García-Comas, B. Funke, A. Gardini, M. López-Puertas, A. Jurado-Navarro, T. von Clarmann, G. Stiller, M. Kiefer, C. D. Boone, T. Leblanc, B. T. Marshall, M. J. Schwartz, and P. E. Sheese
Atmos. Meas. Tech., 7, 3633–3651, https://doi.org/10.5194/amt-7-3633-2014, https://doi.org/10.5194/amt-7-3633-2014, 2014
Short summary
Short summary
We present the new vM21 MIPAS temperatures from 20 to 102km for all of its 2005-2012 MA, UA and NLC measurements. The main upgrades are the update of ESA L1b spectra, spectroscopic database and O and CO2 climatologies, and improvement in Tk-gradient and offset regularizations and apodization accuracy. The vM21 Tk's correct the main systematic errors of previous versions and lead to remarkable improvement in their comparisons with ACE-FTS, MLS, OSIRIS, SABER and SOFIE and the MLO and TMF lidars.
M. Sinnhuber, B. Funke, T. von Clarmann, M. Lopez-Puertas, G. P. Stiller, and A. Seppälä
Atmos. Chem. Phys., 14, 7681–7692, https://doi.org/10.5194/acp-14-7681-2014, https://doi.org/10.5194/acp-14-7681-2014, 2014
R. Eichinger and P. Jöckel
Geosci. Model Dev., 7, 1573–1582, https://doi.org/10.5194/gmd-7-1573-2014, https://doi.org/10.5194/gmd-7-1573-2014, 2014
B. Hassler, I. Petropavlovskikh, J. Staehelin, T. August, P. K. Bhartia, C. Clerbaux, D. Degenstein, M. De Mazière, B. M. Dinelli, A. Dudhia, G. Dufour, S. M. Frith, L. Froidevaux, S. Godin-Beekmann, J. Granville, N. R. P. Harris, K. Hoppel, D. Hubert, Y. Kasai, M. J. Kurylo, E. Kyrölä, J.-C. Lambert, P. F. Levelt, C. T. McElroy, R. D. McPeters, R. Munro, H. Nakajima, A. Parrish, P. Raspollini, E. E. Remsberg, K. H. Rosenlof, A. Rozanov, T. Sano, Y. Sasano, M. Shiotani, H. G. J. Smit, G. Stiller, J. Tamminen, D. W. Tarasick, J. Urban, R. J. van der A, J. P. Veefkind, C. Vigouroux, T. von Clarmann, C. von Savigny, K. A. Walker, M. Weber, J. Wild, and J. M. Zawodny
Atmos. Meas. Tech., 7, 1395–1427, https://doi.org/10.5194/amt-7-1395-2014, https://doi.org/10.5194/amt-7-1395-2014, 2014
S. Meul, U. Langematz, S. Oberländer, H. Garny, and P. Jöckel
Atmos. Chem. Phys., 14, 2959–2971, https://doi.org/10.5194/acp-14-2959-2014, https://doi.org/10.5194/acp-14-2959-2014, 2014
E. Eckert, T. von Clarmann, M. Kiefer, G. P. Stiller, S. Lossow, N. Glatthor, D. A. Degenstein, L. Froidevaux, S. Godin-Beekmann, T. Leblanc, S. McDermid, M. Pastel, W. Steinbrecht, D. P. J. Swart, K. A. Walker, and P. F. Bernath
Atmos. Chem. Phys., 14, 2571–2589, https://doi.org/10.5194/acp-14-2571-2014, https://doi.org/10.5194/acp-14-2571-2014, 2014
J.-U. Grooß, I. Engel, S. Borrmann, W. Frey, G. Günther, C. R. Hoyle, R. Kivi, B. P. Luo, S. Molleker, T. Peter, M. C. Pitts, H. Schlager, G. Stiller, H. Vömel, K. A. Walker, and R. Müller
Atmos. Chem. Phys., 14, 1055–1073, https://doi.org/10.5194/acp-14-1055-2014, https://doi.org/10.5194/acp-14-1055-2014, 2014
V. Grewe, C. Frömming, S. Matthes, S. Brinkop, M. Ponater, S. Dietmüller, P. Jöckel, H. Garny, E. Tsati, K. Dahlmann, O. A. Søvde, J. Fuglestvedt, T. K. Berntsen, K. P. Shine, E. A. Irvine, T. Champougny, and P. Hullah
Geosci. Model Dev., 7, 175–201, https://doi.org/10.5194/gmd-7-175-2014, https://doi.org/10.5194/gmd-7-175-2014, 2014
V. F. Sofieva, N. Rahpoe, J. Tamminen, E. Kyrölä, N. Kalakoski, M. Weber, A. Rozanov, C. von Savigny, A. Laeng, T. von Clarmann, G. Stiller, S. Lossow, D. Degenstein, A. Bourassa, C. Adams, C. Roth, N. Lloyd, P. Bernath, R. J. Hargreaves, J. Urban, D. Murtagh, A. Hauchecorne, F. Dalaudier, M. van Roozendael, N. Kalb, and C. Zehner
Earth Syst. Sci. Data, 5, 349–363, https://doi.org/10.5194/essd-5-349-2013, https://doi.org/10.5194/essd-5-349-2013, 2013
P. Braesicke, J. Keeble, X. Yang, G. Stiller, S. Kellmann, N. L. Abraham, A. Archibald, P. Telford, and J. A. Pyle
Atmos. Chem. Phys., 13, 10677–10688, https://doi.org/10.5194/acp-13-10677-2013, https://doi.org/10.5194/acp-13-10677-2013, 2013
M. Höpfner, N. Glatthor, U. Grabowski, S. Kellmann, M. Kiefer, A. Linden, J. Orphal, G. Stiller, T. von Clarmann, B. Funke, and C. D. Boone
Atmos. Chem. Phys., 13, 10405–10423, https://doi.org/10.5194/acp-13-10405-2013, https://doi.org/10.5194/acp-13-10405-2013, 2013
Y. Kasai, H. Sagawa, D. Kreyling, E. Dupuy, P. Baron, J. Mendrok, K. Suzuki, T. O. Sato, T. Nishibori, S. Mizobuchi, K. Kikuchi, T. Manabe, H. Ozeki, T. Sugita, M. Fujiwara, Y. Irimajiri, K. A. Walker, P. F. Bernath, C. Boone, G. Stiller, T. von Clarmann, J. Orphal, J. Urban, D. Murtagh, E. J. Llewellyn, D. Degenstein, A. E. Bourassa, N. D. Lloyd, L. Froidevaux, M. Birk, G. Wagner, F. Schreier, J. Xu, P. Vogt, T. Trautmann, and M. Yasui
Atmos. Meas. Tech., 6, 2311–2338, https://doi.org/10.5194/amt-6-2311-2013, https://doi.org/10.5194/amt-6-2311-2013, 2013
H. Garny, G. E. Bodeker, D. Smale, M. Dameris, and V. Grewe
Atmos. Chem. Phys., 13, 7279–7300, https://doi.org/10.5194/acp-13-7279-2013, https://doi.org/10.5194/acp-13-7279-2013, 2013
B. Tschanz, C. Straub, D. Scheiben, K. A. Walker, G. P. Stiller, and N. Kämpfer
Atmos. Meas. Tech., 6, 1725–1745, https://doi.org/10.5194/amt-6-1725-2013, https://doi.org/10.5194/amt-6-1725-2013, 2013
G. Wetzel, H. Oelhaf, G. Berthet, A. Bracher, C. Cornacchia, D. G. Feist, H. Fischer, A. Fix, M. Iarlori, A. Kleinert, A. Lengel, M. Milz, L. Mona, S. C. Müller, J. Ovarlez, G. Pappalardo, C. Piccolo, P. Raspollini, J.-B. Renard, V. Rizi, S. Rohs, C. Schiller, G. Stiller, M. Weber, and G. Zhang
Atmos. Chem. Phys., 13, 5791–5811, https://doi.org/10.5194/acp-13-5791-2013, https://doi.org/10.5194/acp-13-5791-2013, 2013
F. Khosrawi, R. Müller, J. Urban, M. H. Proffitt, G. Stiller, M. Kiefer, S. Lossow, D. Kinnison, F. Olschewski, M. Riese, and D. Murtagh
Atmos. Chem. Phys., 13, 3619–3641, https://doi.org/10.5194/acp-13-3619-2013, https://doi.org/10.5194/acp-13-3619-2013, 2013
F. Friederich, T. von Clarmann, B. Funke, H. Nieder, J. Orphal, M. Sinnhuber, G. P. Stiller, and J. M. Wissing
Atmos. Chem. Phys., 13, 2531–2539, https://doi.org/10.5194/acp-13-2531-2013, https://doi.org/10.5194/acp-13-2531-2013, 2013
S. Takele Kenea, G. Mengistu Tsidu, T. Blumenstock, F. Hase, T. von Clarmann, and G. P. Stiller
Atmos. Meas. Tech., 6, 495–509, https://doi.org/10.5194/amt-6-495-2013, https://doi.org/10.5194/amt-6-495-2013, 2013
S. Kellmann, T. von Clarmann, G. P. Stiller, E. Eckert, N. Glatthor, M. Höpfner, M. Kiefer, J. Orphal, B. Funke, U. Grabowski, A. Linden, G. S. Dutton, and J. W. Elkins
Atmos. Chem. Phys., 12, 11857–11875, https://doi.org/10.5194/acp-12-11857-2012, https://doi.org/10.5194/acp-12-11857-2012, 2012
Related subject area
Subject: Dynamics | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Stratosphere | Science Focus: Physics (physical properties and processes)
Crucial role of obliquely propagating gravity waves in the quasi-biennial oscillation dynamics
Technical note: Multi-year changes in the Brewer–Dobson circulation from Halogen Occultation Experiment (HALOE) methane
Exploring the ENSO modulation of the QBO periods with GISS E2.2 models
The impact of ENSO and NAO initial conditions and anomalies on the modeled response to Pinatubo-sized volcanic forcing
Stratospherically induced circulation changes under the extreme conditions of the no-Montreal-Protocol scenario
Vortex preconditioning of the 2021 sudden stratospheric warming: barotropic–baroclinic instability associated with the double westerly jets
On the pattern of interannual polar vortex–ozone co-variability during northern hemispheric winter
A mountain ridge model for quantifying oblique mountain wave propagation and distribution
QBO modulation of the Asian Monsoon water vapour
Weakening of the tropical tropopause layer cold trap with global warming
On the magnitude and sensitivity of the quasi-biennial oscillation response to a tropical volcanic eruption
The response of the North Pacific jet and stratosphere-to-troposphere transport of ozone over western North America to RCP8.5 climate forcing
The Holton–Tan mechanism under stratospheric aerosol intervention
Very-long-period oscillations in the atmosphere (0–110 km) – Part 2: Latitude– longitude comparisons and trends
Driving mechanisms for the El Niño–Southern Oscillation impact on stratospheric ozone
Exploring the link between austral stratospheric polar vortex anomalies and surface climate in chemistry-climate models
The impact of improved spatial and temporal resolution of reanalysis data on Lagrangian studies of the tropical tropopause layer
Dynamics of ENSO-driven stratosphere-to-troposphere transport of ozone over North America
Ozone–gravity wave interaction in the upper stratosphere/lower mesosphere
How can Brewer–Dobson circulation trends be estimated from changes in stratospheric water vapour and methane?
The semi-annual oscillation (SAO) in the upper troposphere and lower stratosphere (UTLS)
Interactions between the stratospheric polar vortex and Atlantic circulation on seasonal to multi-decadal timescales
Impacts of three types of solar geoengineering on the Atlantic Meridional Overturning Circulation
Enhanced upward motion through the troposphere over the tropical western Pacific and its implications for the transport of trace gases from the troposphere to the stratosphere
Evolution of the intensity and duration of the Southern Hemisphere stratospheric polar vortex edge for the period 1979–2020
Characterization of transport from the Asian summer monsoon anticyclone into the UTLS via shedding of low potential vorticity cutoffs
Long-range prediction and the stratosphere
Weakening of Antarctic stratospheric planetary wave activities in early austral spring since the early 2000s: a response to sea surface temperature trends
Specified dynamics scheme impacts on wave-mean flow dynamics, convection, and tracer transport in CESM2 (WACCM6)
Propagation paths and source distributions of resolved gravity waves in ECMWF-IFS analysis fields around the southern polar night jet
Observation and modeling of high-7Be concentration events at the surface in northern Europe associated with the instability of the Arctic polar vortex in early 2003
Eastward-propagating planetary waves in the polar middle atmosphere
The Brewer–Dobson circulation in CMIP6
Climate impact of volcanic eruptions: the sensitivity to eruption season and latitude in MPI-ESM ensemble experiments
Contributions of equatorial waves and small-scale convective gravity waves to the 2019/20 quasi-biennial oscillation (QBO) disruption
Differences in the quasi-biennial oscillation response to stratospheric aerosol modification depending on injection strategy and species
The advective Brewer–Dobson circulation in the ERA5 reanalysis: climatology, variability, and trends
Is our dynamical understanding of the circulation changes associated with the Antarctic ozone hole sensitive to the choice of reanalysis dataset?
The impact of increasing stratospheric radiative damping on the quasi-biennial oscillation period
Analysis of recent lower-stratospheric ozone trends in chemistry climate models
Asymmetry and pathways of inter-hemispheric transport in the upper troposphere and lower stratosphere
Effects of prescribed CMIP6 ozone on simulating the Southern Hemisphere atmospheric circulation response to ozone depletion
Reanalysis intercomparison of potential vorticity and potential-vorticity-based diagnostics
Influence of the El Niño–Southern Oscillation on entry stratospheric water vapor in coupled chemistry–ocean CCMI and CMIP6 models
Reappraising the appropriate calculation of a common meteorological quantity: potential temperature
Impact of Lagrangian transport on lower-stratospheric transport timescales in a climate model
Role of equatorial waves and convective gravity waves in the 2015/16 quasi-biennial oscillation disruption
Sensitivity of the Southern Hemisphere circumpolar jet response to Antarctic ozone depletion: prescribed versus interactive chemistry
Characterizing quasi-biweekly variability of the Asian monsoon anticyclone using potential vorticity and large-scale geopotential height field
Climatological impact of the Brewer–Dobson circulation on the N2O budget in WACCM, a chemical reanalysis and a CTM driven by four dynamical reanalyses
Young-Ha Kim, Georg Sebastian Voelker, Gergely Bölöni, Günther Zängl, and Ulrich Achatz
Atmos. Chem. Phys., 24, 3297–3308, https://doi.org/10.5194/acp-24-3297-2024, https://doi.org/10.5194/acp-24-3297-2024, 2024
Short summary
Short summary
The quasi-biennial oscillation, which governs the tropical stratospheric circulation, is driven primarily by small-scale wave processes. We employ a novel method to realistically represent these wave processes in a global model, thereby revealing an aspect of the oscillation that has not been identified before. We find that the oblique propagation of waves, a process neglected by existing climate models, plays a pivotal role in the stratospheric circulation and its oscillation.
Ellis Remsberg
Atmos. Chem. Phys., 24, 1691–1697, https://doi.org/10.5194/acp-24-1691-2024, https://doi.org/10.5194/acp-24-1691-2024, 2024
Short summary
Short summary
CH4 data from the Halogen Occultation Experiment show clear changes in the deep and shallow branches of the Brewer–Dobson circulation (BDC) from 1992 to 2005. CH4 decreased in the upper stratosphere in the early 1990s following the Pinatubo eruption. There was also meridional transport of CH4 from the tropics to mid-latitudes in both hemispheres in the late 1990s. CH4 trends in the shallow branch agree with the tropospheric CH4 trends from 1996 to 2005.
Tiehan Zhou, Kevin J. DallaSanta, Clara Orbe, David H. Rind, Jeffrey A. Jonas, Larissa Nazarenko, Gavin A. Schmidt, and Gary Russell
Atmos. Chem. Phys., 24, 509–532, https://doi.org/10.5194/acp-24-509-2024, https://doi.org/10.5194/acp-24-509-2024, 2024
Short summary
Short summary
The El Niño–Southern Oscillation (ENSO) tends to speed up and slow down the phase speed of the Quasi-Biennial Oscillation (QBO) during El Niño and La Niña, respectively. The ENSO modulation of the QBO does not show up in the climate models with parameterized but temporally constant gravity wave sources. We show that the GISS E2.2 models can capture the observed ENSO modulation of the QBO period with a horizontal resolution of 2° by 2.5° and its gravity wave sources parameterized interactively.
Helen Weierbach, Allegra N. LeGrande, and Kostas Tsigaridis
Atmos. Chem. Phys., 23, 15491–15505, https://doi.org/10.5194/acp-23-15491-2023, https://doi.org/10.5194/acp-23-15491-2023, 2023
Short summary
Short summary
Volcanic aerosols impact global and regional climate conditions but can vary depending on pre-existing initial climate conditions. We ran an ensemble of volcanic aerosol simulations under varying ENSO and NAO initial conditions to understand how initial climate states impact the modeled response to volcanic forcing. Overall we found that initial NAO conditions can impact the strength of the first winter post-eruptive response but are also affected by the choice of anomaly and sampling routine.
Franziska Zilker, Timofei Sukhodolov, Gabriel Chiodo, Marina Friedel, Tatiana Egorova, Eugene Rozanov, Jan Sedlacek, Svenja Seeber, and Thomas Peter
Atmos. Chem. Phys., 23, 13387–13411, https://doi.org/10.5194/acp-23-13387-2023, https://doi.org/10.5194/acp-23-13387-2023, 2023
Short summary
Short summary
The Montreal Protocol (MP) has successfully reduced the Antarctic ozone hole by banning chlorofluorocarbons (CFCs) that destroy the ozone layer. Moreover, CFCs are strong greenhouse gases (GHGs) that would have strengthened global warming. In this study, we investigate the surface weather and climate in a world without the MP at the end of the 21st century, disentangling ozone-mediated and GHG impacts of CFCs. Overall, we avoided 1.7 K global surface warming and a poleward shift in storm tracks.
Ji-Hee Yoo, Hye-Yeong Chun, and Min-Jee Kang
Atmos. Chem. Phys., 23, 10869–10881, https://doi.org/10.5194/acp-23-10869-2023, https://doi.org/10.5194/acp-23-10869-2023, 2023
Short summary
Short summary
The January 2021 sudden stratospheric warming was preceded by unusual double westerly jets with polar stratospheric and subtropical mesospheric cores. This wind structure promotes anomalous dissipation of tropospheric planetary waves between the two maxima, leading to unusually strong shear instability. Shear instability generates the westward-propagating planetary waves with zonal wavenumber 2 in situ, thereby splitting the polar vortex just before the onset.
Frederik Harzer, Hella Garny, Felix Ploeger, Harald Bönisch, Peter Hoor, and Thomas Birner
Atmos. Chem. Phys., 23, 10661–10675, https://doi.org/10.5194/acp-23-10661-2023, https://doi.org/10.5194/acp-23-10661-2023, 2023
Short summary
Short summary
We study the statistical relation between year-by-year fluctuations in winter-mean ozone and the strength of the stratospheric polar vortex. In the latitude–pressure plane, regression analysis shows that anomalously weak polar vortex years are associated with three pronounced local ozone maxima over the polar cap relative to the winter climatology. These response maxima primarily reflect the non-trivial combination of different ozone transport processes with varying relative contributions.
Sebastian Rhode, Peter Preusse, Manfred Ern, Jörn Ungermann, Lukas Krasauskas, Julio Bacmeister, and Martin Riese
Atmos. Chem. Phys., 23, 7901–7934, https://doi.org/10.5194/acp-23-7901-2023, https://doi.org/10.5194/acp-23-7901-2023, 2023
Short summary
Short summary
Gravity waves (GWs) transport energy vertically and horizontally within the atmosphere and thereby affect wind speeds far from their sources. Here, we present a model that identifies orographic GW sources and predicts the pathways of the excited GWs through the atmosphere for a better understanding of horizontal GW propagation. We use this model to explain physical patterns in satellite observations (e.g., low GW activity above the Himalaya) and predict seasonal patterns of GW propagation.
Cristina Peña-Ortiz, Nurial Pilar Plaza, David Gallego, and Felix Plöger
EGUsphere, https://doi.org/10.5194/egusphere-2023-1432, https://doi.org/10.5194/egusphere-2023-1432, 2023
Short summary
Short summary
Although water vapour (H2O) in the lower stratosphere is only a few molecules among 1 million air molecules, atmospheric radiative forcing and surface temperature are particularly sensible to small changes in its concentration. Monsoon regions play a key role in H2O transport and in its concentration in the lower stratosphere. We show how the QBO has a major impact on H2O over the Asian monsoon during August through changes in temperature caused by the QBO modulation of convection.
Stephen Bourguet and Marianna Linz
Atmos. Chem. Phys., 23, 7447–7460, https://doi.org/10.5194/acp-23-7447-2023, https://doi.org/10.5194/acp-23-7447-2023, 2023
Short summary
Short summary
Here, we show how projected changes to tropical circulation will impact the water vapor concentration in the lower stratosphere, which has implications for surface climate and stratospheric chemistry. In our transport scenarios with slower east–west winds, air parcels ascending into the stratosphere do not experience the same cold temperatures that they would today. This effect could act in concert with previously modeled changes to stratospheric water vapor to amplify surface warming.
Flossie Brown, Lauren Marshall, Peter H. Haynes, Rolando R. Garcia, Thomas Birner, and Anja Schmidt
Atmos. Chem. Phys., 23, 5335–5353, https://doi.org/10.5194/acp-23-5335-2023, https://doi.org/10.5194/acp-23-5335-2023, 2023
Short summary
Short summary
Large-magnitude volcanic eruptions have the potential to alter large-scale circulation patterns, such as the quasi-biennial oscillation (QBO). The QBO is an oscillation of the tropical stratospheric zonal winds between easterly and westerly directions. Using a climate model, we show that large-magnitude eruptions can delay the progression of the QBO, with a much longer delay when the shear is easterly than when it is westerly. Such delays may affect weather and transport of atmospheric gases.
Dillon Elsbury, Amy H. Butler, John R. Albers, Melissa L. Breeden, and Andrew O'Neil Langford
Atmos. Chem. Phys., 23, 5101–5117, https://doi.org/10.5194/acp-23-5101-2023, https://doi.org/10.5194/acp-23-5101-2023, 2023
Short summary
Short summary
One of the global hotspots where stratosphere-to-troposphere transport (STT) of ozone takes place is over Pacific North America (PNA). However, we do not know how or if STT over PNA will change in response to climate change. Using climate model experiments forced with
worst-casescenario Representative Concentration Pathway 8.5 climate change, we find that changes in net chemical production and transport of ozone in the lower stratosphere increase STT of ozone over PNA in the future.
Khalil Karami, Rolando Garcia, Christoph Jacobi, Jadwiga H. Richter, and Simone Tilmes
Atmos. Chem. Phys., 23, 3799–3818, https://doi.org/10.5194/acp-23-3799-2023, https://doi.org/10.5194/acp-23-3799-2023, 2023
Short summary
Short summary
Alongside mitigation and adaptation efforts, stratospheric aerosol intervention (SAI) is increasingly considered a third pillar to combat dangerous climate change. We investigate the teleconnection between the quasi-biennial oscillation in the equatorial stratosphere and the Arctic stratospheric polar vortex under a warmer climate and an SAI scenario. We show that the Holton–Tan relationship weakens under both scenarios and discuss the physical mechanisms responsible for such changes.
Dirk Offermann, Christoph Kalicinsky, Ralf Koppmann, and Johannes Wintel
Atmos. Chem. Phys., 23, 3267–3278, https://doi.org/10.5194/acp-23-3267-2023, https://doi.org/10.5194/acp-23-3267-2023, 2023
Short summary
Short summary
Atmospheric oscillations with periods between 5 and more than 200 years are believed to be self-excited (internal) in the atmosphere, i.e. non-anthropogenic. They are found at all altitudes up to 110 km and at four very different geographical locations (75° N, 70° E; 75° N, 280° E; 50° N, 7° E; 50° S, 7° E). Therefore, they hint at a global-oscillation mode. Their amplitudes are on the order of present-day climate trends, and it is therefore difficult to disentangle them.
Samuel Benito-Barca, Natalia Calvo, and Marta Abalos
Atmos. Chem. Phys., 22, 15729–15745, https://doi.org/10.5194/acp-22-15729-2022, https://doi.org/10.5194/acp-22-15729-2022, 2022
Short summary
Short summary
The impact of different El Niño flavors (eastern (EP) and central (CP) Pacific El Niño) and La Niña on the stratospheric ozone is studied in a state-of-the-art chemistry–climate model. Ozone reduces in the tropics and increases in the extratropics when an EP El Niño event occurs, the opposite of La Niña. However, CP El Niño has no impact on extratropical ozone. These ozone variations are driven by changes in the stratospheric transport circulation, with an important contribution of mixing.
Nora Bergner, Marina Friedel, Daniela I. V. Domeisen, Darryn Waugh, and Gabriel Chiodo
Atmos. Chem. Phys., 22, 13915–13934, https://doi.org/10.5194/acp-22-13915-2022, https://doi.org/10.5194/acp-22-13915-2022, 2022
Short summary
Short summary
Polar vortex extremes, particularly situations with an unusually weak cyclonic circulation in the stratosphere, can influence the surface climate in the spring–summer time in the Southern Hemisphere. Using chemistry-climate models and observations, we evaluate the robustness of the surface impacts. While models capture the general surface response, they do not show the observed climate patterns in midlatitude regions, which we trace back to biases in the models' circulations.
Stephen Bourguet and Marianna Linz
Atmos. Chem. Phys., 22, 13325–13339, https://doi.org/10.5194/acp-22-13325-2022, https://doi.org/10.5194/acp-22-13325-2022, 2022
Short summary
Short summary
Here, we tested the impact of spatial and temporal resolution on Lagrangian trajectory studies in a key region of interest for climate feedbacks and stratospheric chemistry. Our analysis shows that new higher-resolution input data provide an opportunity for a better understanding of physical processes that control how air moves from the troposphere to the stratosphere. Future studies of how these processes will change in a warming climate will benefit from these results.
John R. Albers, Amy H. Butler, Andrew O. Langford, Dillon Elsbury, and Melissa L. Breeden
Atmos. Chem. Phys., 22, 13035–13048, https://doi.org/10.5194/acp-22-13035-2022, https://doi.org/10.5194/acp-22-13035-2022, 2022
Short summary
Short summary
Ozone transported from the stratosphere contributes to background ozone concentrations in the free troposphere and to surface ozone exceedance events that affect human health. The physical processes whereby the El Niño–Southern Oscillation (ENSO) modulates North American stratosphere-to-troposphere ozone transport during spring are documented, and the usefulness of ENSO for predicting ozone events that may cause exceedances in surface air quality standards are assessed.
Axel Gabriel
Atmos. Chem. Phys., 22, 10425–10441, https://doi.org/10.5194/acp-22-10425-2022, https://doi.org/10.5194/acp-22-10425-2022, 2022
Short summary
Short summary
Recent measurements show some evidence that the amplitudes of atmospheric gravity waves (horizontal wavelengths of 100–2000 km), which propagate from the troposphere (0–10 km) to the stratosphere and mesosphere (10–100 km), increase more strongly with height during daytime than during nighttime. This study shows that ozone–temperature coupling in the upper stratosphere can principally produce such an amplification. The results will help to improve atmospheric circulation models.
Liubov Poshyvailo-Strube, Rolf Müller, Stephan Fueglistaler, Michaela I. Hegglin, Johannes C. Laube, C. Michael Volk, and Felix Ploeger
Atmos. Chem. Phys., 22, 9895–9914, https://doi.org/10.5194/acp-22-9895-2022, https://doi.org/10.5194/acp-22-9895-2022, 2022
Short summary
Short summary
Brewer–Dobson circulation (BDC) controls the composition of the stratosphere, which in turn affects radiation and climate. As the BDC cannot be measured directly, it is necessary to infer its strength and trends indirectly. In this study, we test in the
model worlddifferent methods for estimating the mean age of air trends based on a combination of stratospheric water vapour and methane data. We also provide simple practical advice of a more reliable estimation of the mean age of air trends.
Ming Shangguan and Wuke Wang
Atmos. Chem. Phys., 22, 9499–9511, https://doi.org/10.5194/acp-22-9499-2022, https://doi.org/10.5194/acp-22-9499-2022, 2022
Short summary
Short summary
Skilful predictions of weather and climate on subseasonal to seasonal scales are valuable for decision makers. Here we show the global spatiotemporal variation of the temperature SAO in the UTLS with GNSS RO and reanalysis data. The formation of the SAO is explained by an energy budget analysis. The results show that the SAO in the UTLS is partly modified by the SSTs according to model simulations. The results may provide an important source for seasonal predictions of the surface weather.
Oscar Dimdore-Miles, Lesley Gray, Scott Osprey, Jon Robson, Rowan Sutton, and Bablu Sinha
Atmos. Chem. Phys., 22, 4867–4893, https://doi.org/10.5194/acp-22-4867-2022, https://doi.org/10.5194/acp-22-4867-2022, 2022
Short summary
Short summary
This study examines interactions between variations in the strength of polar stratospheric winds and circulation in the North Atlantic in a climate model simulation. It finds that the Atlantic Meridional Overturning Circulation (AMOC) responds with oscillations to sets of consecutive Northern Hemisphere winters, which show all strong or all weak polar vortex conditions. The study also shows that a set of strong vortex winters in the 1990s contributed to the recent slowdown in the observed AMOC.
Mengdie Xie, John C. Moore, Liyun Zhao, Michael Wolovick, and Helene Muri
Atmos. Chem. Phys., 22, 4581–4597, https://doi.org/10.5194/acp-22-4581-2022, https://doi.org/10.5194/acp-22-4581-2022, 2022
Short summary
Short summary
We use data from six Earth system models to estimate Atlantic meridional overturning circulation (AMOC) changes and its drivers under four different solar geoengineering methods. Solar dimming seems relatively more effective than marine cloud brightening or stratospheric aerosol injection at reversing greenhouse-gas-driven declines in AMOC. Geoengineering-induced AMOC amelioration is due to better maintenance of air–sea temperature differences and reduced loss of Arctic summer sea ice.
Kai Qie, Wuke Wang, Wenshou Tian, Rui Huang, Mian Xu, Tao Wang, and Yifeng Peng
Atmos. Chem. Phys., 22, 4393–4411, https://doi.org/10.5194/acp-22-4393-2022, https://doi.org/10.5194/acp-22-4393-2022, 2022
Short summary
Short summary
We identify a significantly intensified upward motion over the tropical western Pacific (TWP) and an enhanced tropical upwelling in boreal winter during 1958–2017 due to the warming of global sea surface temperatures (SSTs). Our results suggest that more tropospheric trace gases over the TWP could be elevated to the lower stratosphere, which implies that the emission from the maritime continent plays a more important role in the stratospheric processes and the global climate.
Audrey Lecouffe, Sophie Godin-Beekmann, Andrea Pazmiño, and Alain Hauchecorne
Atmos. Chem. Phys., 22, 4187–4200, https://doi.org/10.5194/acp-22-4187-2022, https://doi.org/10.5194/acp-22-4187-2022, 2022
Short summary
Short summary
This study uses a model developped at LATMOS (France) to analyze the behavior of the Antarctic polar vortex from 1979 to 2020 at 675 K, 550 K, and 475 K isentropic levels. We found that the vortex edge intensity is stronger during the September–October–November period, while its edge position is less extended during this period. The polar vortex is stronger and lasts longer during solar minimum years. Breakup dates of the polar vortex are linked to the ozone hole and maximum wind speed.
Jan Clemens, Felix Ploeger, Paul Konopka, Raphael Portmann, Michael Sprenger, and Heini Wernli
Atmos. Chem. Phys., 22, 3841–3860, https://doi.org/10.5194/acp-22-3841-2022, https://doi.org/10.5194/acp-22-3841-2022, 2022
Short summary
Short summary
Highly polluted air flows from the surface to higher levels of the atmosphere during the Asian summer monsoon. At high levels, the air is trapped within eddies. Here, we study how air masses can leave the eddy within its cutoff, how they distribute, and how their chemical composition changes. We found evidence for transport from the eddy to higher latitudes over the North Pacific and even Alaska. During transport, trace gas concentrations within cutoffs changed gradually, showing steady mixing.
Adam A. Scaife, Mark P. Baldwin, Amy H. Butler, Andrew J. Charlton-Perez, Daniela I. V. Domeisen, Chaim I. Garfinkel, Steven C. Hardiman, Peter Haynes, Alexey Yu Karpechko, Eun-Pa Lim, Shunsuke Noguchi, Judith Perlwitz, Lorenzo Polvani, Jadwiga H. Richter, John Scinocca, Michael Sigmond, Theodore G. Shepherd, Seok-Woo Son, and David W. J. Thompson
Atmos. Chem. Phys., 22, 2601–2623, https://doi.org/10.5194/acp-22-2601-2022, https://doi.org/10.5194/acp-22-2601-2022, 2022
Short summary
Short summary
Great progress has been made in computer modelling and simulation of the whole climate system, including the stratosphere. Since the late 20th century we also gained a much clearer understanding of how the stratosphere interacts with the lower atmosphere. The latest generation of numerical prediction systems now explicitly represents the stratosphere and its interaction with surface climate, and here we review its role in long-range predictions and projections from weeks to decades ahead.
Yihang Hu, Wenshou Tian, Jiankai Zhang, Tao Wang, and Mian Xu
Atmos. Chem. Phys., 22, 1575–1600, https://doi.org/10.5194/acp-22-1575-2022, https://doi.org/10.5194/acp-22-1575-2022, 2022
Short summary
Short summary
Antarctic stratospheric wave activities in September have been weakening significantly since the 2000s. Further analysis supports the finding that sea surface temperature (SST) trends over 20° N–70° S lead to the weakening of stratospheric wave activities, while the response of stratospheric wave activities to ozone recovery is weak. Thus, the SST trend should be taken into consideration when exploring the mechanism for the climate transition in the southern hemispheric stratosphere around 2000.
Nicholas A. Davis, Patrick Callaghan, Isla R. Simpson, and Simone Tilmes
Atmos. Chem. Phys., 22, 197–214, https://doi.org/10.5194/acp-22-197-2022, https://doi.org/10.5194/acp-22-197-2022, 2022
Short summary
Short summary
Specified dynamics schemes attempt to constrain the atmospheric circulation in a climate model to isolate the role of transport in chemical variability, evaluate model physics, and interpret field campaign observations. We show that the specified dynamics scheme in CESM2 erroneously suppresses convection and induces circulation errors that project onto errors in tracers, even using the most optimal settings. Development of a more sophisticated scheme is necessary for future progress.
Cornelia Strube, Peter Preusse, Manfred Ern, and Martin Riese
Atmos. Chem. Phys., 21, 18641–18668, https://doi.org/10.5194/acp-21-18641-2021, https://doi.org/10.5194/acp-21-18641-2021, 2021
Short summary
Short summary
High gravity wave (GW) momentum fluxes in the lower stratospheric southern polar vortex around 60° S are still poorly understood. Few GW sources are found at these latitudes. We present a ray tracing case study on waves resolved in high-resolution global model temperatures southeast of New Zealand. We show that lateral propagation of more than 1000 km takes place below 20 km altitude, and a variety of orographic and non-orographic sources located north of 50° S generate the wave field.
Erika Brattich, Hongyu Liu, Bo Zhang, Miguel Ángel Hernández-Ceballos, Jussi Paatero, Darko Sarvan, Vladimir Djurdjevic, Laura Tositti, and Jelena Ajtić
Atmos. Chem. Phys., 21, 17927–17951, https://doi.org/10.5194/acp-21-17927-2021, https://doi.org/10.5194/acp-21-17927-2021, 2021
Short summary
Short summary
In this study we analyse the output of a chemistry and transport model together with observations of different meteorological and compositional variables to demonstrate the link between sudden stratospheric warming and transport of stratospheric air to the surface in the subpolar regions of Europe during the cold season. Our findings have particular implications for atmospheric composition since climate projections indicate more frequent sudden stratospheric warming under a warmer climate.
Liang Tang, Sheng-Yang Gu, and Xian-Kang Dou
Atmos. Chem. Phys., 21, 17495–17512, https://doi.org/10.5194/acp-21-17495-2021, https://doi.org/10.5194/acp-21-17495-2021, 2021
Short summary
Short summary
Our study explores the variation in the occurrence date, peak amplitude and wave period for eastward waves and the role of instability, background wind structure and the critical layer in eastward wave propagation and amplification.
Marta Abalos, Natalia Calvo, Samuel Benito-Barca, Hella Garny, Steven C. Hardiman, Pu Lin, Martin B. Andrews, Neal Butchart, Rolando Garcia, Clara Orbe, David Saint-Martin, Shingo Watanabe, and Kohei Yoshida
Atmos. Chem. Phys., 21, 13571–13591, https://doi.org/10.5194/acp-21-13571-2021, https://doi.org/10.5194/acp-21-13571-2021, 2021
Short summary
Short summary
The stratospheric Brewer–Dobson circulation (BDC), responsible for transporting mass, tracers and heat globally in the stratosphere, is evaluated in a set of state-of-the-art climate models. The acceleration of the BDC in response to increasing greenhouse gases is most robust in the lower stratosphere. At higher levels, the well-known inconsistency between model and observational BDC trends can be partly reconciled by accounting for limited sampling and large uncertainties in the observations.
Zhihong Zhuo, Ingo Kirchner, Stephan Pfahl, and Ulrich Cubasch
Atmos. Chem. Phys., 21, 13425–13442, https://doi.org/10.5194/acp-21-13425-2021, https://doi.org/10.5194/acp-21-13425-2021, 2021
Short summary
Short summary
The impact of volcanic eruptions varies with eruption season and latitude. This study simulated eruptions at different latitudes and in different seasons with a fully coupled climate model. The climate impacts of northern and southern hemispheric eruptions are reversed but are insensitive to eruption season. Results suggest that the regional climate impacts are due to the dynamical response of the climate system to radiative effects of volcanic aerosols and the subsequent regional feedbacks.
Min-Jee Kang and Hye-Yeong Chun
Atmos. Chem. Phys., 21, 9839–9857, https://doi.org/10.5194/acp-21-9839-2021, https://doi.org/10.5194/acp-21-9839-2021, 2021
Short summary
Short summary
In winter 2019/20, the westerly quasi-biennial oscillation (QBO) phase was disrupted again by easterly winds. It is found that strong Rossby waves from the Southern Hemisphere weaken the jet core in early stages, and strong mixed Rossby–gravity waves reverse the wind in later stages. Inertia–gravity waves and small-scale convective gravity waves also provide negative forcing. These strong waves are attributed to an anomalous wind profile, barotropic instability, and slightly strong convection.
Henning Franke, Ulrike Niemeier, and Daniele Visioni
Atmos. Chem. Phys., 21, 8615–8635, https://doi.org/10.5194/acp-21-8615-2021, https://doi.org/10.5194/acp-21-8615-2021, 2021
Short summary
Short summary
Stratospheric aerosol modification (SAM) can alter the quasi-biennial oscillation (QBO). Our simulations with two different models show that the characteristics of the QBO response are primarily determined by the meridional structure of the aerosol-induced heating. Therefore, the QBO response to SAM depends primarily on the location of injection, while injection type and rate act to scale the specific response. Our results have important implications for evaluating adverse side effects of SAM.
Mohamadou Diallo, Manfred Ern, and Felix Ploeger
Atmos. Chem. Phys., 21, 7515–7544, https://doi.org/10.5194/acp-21-7515-2021, https://doi.org/10.5194/acp-21-7515-2021, 2021
Short summary
Short summary
Despite good agreement in the spatial structure, there are substantial differences in the strength of the Brewer–Dobson circulation (BDC) and its modulations in the UTLS and upper stratosphere. The tropical upwelling is generally weaker in ERA5 than in ERAI due to weaker planetary and gravity wave breaking in the UTLS. Analysis of the BDC trend shows an acceleration of the BDC of about 1.5 % decade-1 due to the long-term intensification in wave breaking, consistent with climate predictions.
Andrew Orr, Hua Lu, Patrick Martineau, Edwin P. Gerber, Gareth J. Marshall, and Thomas J. Bracegirdle
Atmos. Chem. Phys., 21, 7451–7472, https://doi.org/10.5194/acp-21-7451-2021, https://doi.org/10.5194/acp-21-7451-2021, 2021
Short summary
Short summary
Reanalysis datasets combine observations and weather forecast simulations to create our best estimate of the state of the atmosphere and are important for climate monitoring. Differences in the technical details of these products mean that they may give different results. This study therefore examined how changes associated with the so-called Antarctic ozone hole are represented, which is one of the most important climate changes in recent decades, and showed that they were broadly consistent.
Tiehan Zhou, Kevin DallaSanta, Larissa Nazarenko, Gavin A. Schmidt, and Zhonghai Jin
Atmos. Chem. Phys., 21, 7395–7407, https://doi.org/10.5194/acp-21-7395-2021, https://doi.org/10.5194/acp-21-7395-2021, 2021
Short summary
Short summary
Stratospheric radiative damping increases with rising CO2. Sensitivity experiments using the one-dimensional mechanistic models of the quasi-biennial oscillation (QBO) indicate a shortening of the simulated QBO period due to the enhancing of the radiative damping. This result suggests that increasing radiative damping may play a role in determining the QBO period in a warming climate along with wave momentum flux entering the stratosphere and tropical vertical residual velocity.
Simone Dietmüller, Hella Garny, Roland Eichinger, and William T. Ball
Atmos. Chem. Phys., 21, 6811–6837, https://doi.org/10.5194/acp-21-6811-2021, https://doi.org/10.5194/acp-21-6811-2021, 2021
Xiaolu Yan, Paul Konopka, Marius Hauck, Aurélien Podglajen, and Felix Ploeger
Atmos. Chem. Phys., 21, 6627–6645, https://doi.org/10.5194/acp-21-6627-2021, https://doi.org/10.5194/acp-21-6627-2021, 2021
Short summary
Short summary
Inter-hemispheric transport is important for understanding atmospheric tracers because of the asymmetry in emissions between the Southern Hemisphere (SH) and Northern Hemisphere (NH). This study finds that the air masses from the NH extratropics to the atmosphere are about 5 times larger than those from the SH extratropics. The interplay between the Asian summer monsoon and westerly ducts triggers the cross-Equator transport from the NH to the SH in boreal summer and fall.
Ioana Ivanciu, Katja Matthes, Sebastian Wahl, Jan Harlaß, and Arne Biastoch
Atmos. Chem. Phys., 21, 5777–5806, https://doi.org/10.5194/acp-21-5777-2021, https://doi.org/10.5194/acp-21-5777-2021, 2021
Short summary
Short summary
The Antarctic ozone hole has driven substantial dynamical changes in the Southern Hemisphere atmosphere over the past decades. This study separates the historical impacts of ozone depletion from those of rising levels of greenhouse gases and investigates how these impacts are captured in two types of climate models: one using interactive atmospheric chemistry and one prescribing the CMIP6 ozone field. The effects of ozone depletion are more pronounced in the model with interactive chemistry.
Luis F. Millán, Gloria L. Manney, and Zachary D. Lawrence
Atmos. Chem. Phys., 21, 5355–5376, https://doi.org/10.5194/acp-21-5355-2021, https://doi.org/10.5194/acp-21-5355-2021, 2021
Short summary
Short summary
We assess how consistently reanalyses represent potential vorticity (PV) among each other. PV helps describe dynamical processes in the stratosphere because it acts approximately as a tracer of the movement of air parcels; it is extensively used to identify the location of the tropopause and to identify and characterize the stratospheric polar vortex. Overall, PV from all reanalyses agrees well with the reanalysis ensemble mean.
Chaim I. Garfinkel, Ohad Harari, Shlomi Ziskin Ziv, Jian Rao, Olaf Morgenstern, Guang Zeng, Simone Tilmes, Douglas Kinnison, Fiona M. O'Connor, Neal Butchart, Makoto Deushi, Patrick Jöckel, Andrea Pozzer, and Sean Davis
Atmos. Chem. Phys., 21, 3725–3740, https://doi.org/10.5194/acp-21-3725-2021, https://doi.org/10.5194/acp-21-3725-2021, 2021
Short summary
Short summary
Water vapor is the dominant greenhouse gas in the atmosphere, and El Niño is the dominant mode of variability in the ocean–atmosphere system. The connection between El Niño and water vapor above ~ 17 km is unclear, with single-model studies reaching a range of conclusions. This study examines this connection in 12 different models. While there are substantial differences among the models, all models appear to capture the fundamental physical processes correctly.
Manuel Baumgartner, Ralf Weigel, Allan H. Harvey, Felix Plöger, Ulrich Achatz, and Peter Spichtinger
Atmos. Chem. Phys., 20, 15585–15616, https://doi.org/10.5194/acp-20-15585-2020, https://doi.org/10.5194/acp-20-15585-2020, 2020
Short summary
Short summary
The potential temperature is routinely used in atmospheric science. We review its derivation and suggest a new potential temperature, based on a temperature-dependent parameterization of the dry air's specific heat capacity. Moreover, we compare the new potential temperature to the common one and discuss the differences which become more important at higher altitudes. Finally, we indicate some consequences of using the new potential temperature in typical applications.
Edward J. Charlesworth, Ann-Kristin Dugstad, Frauke Fritsch, Patrick Jöckel, and Felix Plöger
Atmos. Chem. Phys., 20, 15227–15245, https://doi.org/10.5194/acp-20-15227-2020, https://doi.org/10.5194/acp-20-15227-2020, 2020
Short summary
Short summary
Modeling the stratosphere requires models with good representations of chemical transport. To do this, nearly all models divide the atmosphere into boxes. This creates some unwanted problems. However, the only other option is to divide the atmosphere into balloons, and this method is very complicated. Here, we use a model which uses this balloon-like method to estimate the impacts of this method on chemical transport. We find significant differences in sensitive regions of the stratosphere.
Min-Jee Kang, Hye-Yeong Chun, and Rolando R. Garcia
Atmos. Chem. Phys., 20, 14669–14693, https://doi.org/10.5194/acp-20-14669-2020, https://doi.org/10.5194/acp-20-14669-2020, 2020
Short summary
Short summary
In winter 2015/16, the descent of the westerly quasi-biennial oscillation (QBO) jet was interrupted by easterly winds. We find that Rossby–gravity and inertia–gravity waves weaken the jet core in early stages, and small-scale convective gravity waves, as well as horizontal and vertical components of Rossby waves, reverse the wind sign in later stages. The strong negative wave forcing in the tropics results from the enhanced convection, an anomalous wind profile, and barotropic instability.
Sabine Haase, Jaika Fricke, Tim Kruschke, Sebastian Wahl, and Katja Matthes
Atmos. Chem. Phys., 20, 14043–14061, https://doi.org/10.5194/acp-20-14043-2020, https://doi.org/10.5194/acp-20-14043-2020, 2020
Short summary
Short summary
Ozone depletion over Antarctica was shown to influence the tropospheric jet in the Southern Hemisphere. We investigate the atmospheric response to ozone depletion comparing climate model ensembles with interactive and prescribed ozone fields. We show that allowing feedbacks between ozone chemistry and model physics as well as including asymmetries in ozone leads to a strengthened ozone depletion signature in the stratosphere but does not significantly affect the tropospheric jet position.
Arata Amemiya and Kaoru Sato
Atmos. Chem. Phys., 20, 13857–13876, https://doi.org/10.5194/acp-20-13857-2020, https://doi.org/10.5194/acp-20-13857-2020, 2020
Short summary
Short summary
The spatial pattern of subseasonal variability of the Asian monsoon anticyclone (AMA) is analyzed using long-term reanalysis data, integrating two different views using potential vorticity and the geopotential height anomaly. This study provides a link between two existing description of the Asian monsoon anticyclone, which is important for the understanding of the whole life cycle of its characteristic subseasonal variability pattern.
Daniele Minganti, Simon Chabrillat, Yves Christophe, Quentin Errera, Marta Abalos, Maxime Prignon, Douglas E. Kinnison, and Emmanuel Mahieu
Atmos. Chem. Phys., 20, 12609–12631, https://doi.org/10.5194/acp-20-12609-2020, https://doi.org/10.5194/acp-20-12609-2020, 2020
Short summary
Short summary
The climatology of the N2O transport budget in the stratosphere is studied in the transformed Eulerian mean framework across a variety of datasets: a chemistry climate model, a chemistry transport model driven by four reanalyses and a chemical reanalysis. The impact of vertical advection on N2O agrees well in the datasets, but horizontal mixing presents large differences above the Antarctic and in the whole Northern Hemisphere.
Cited articles
Adcock, K. E., Fraser, P. J., Hall, B. D., Langenfelds, R. L., Lee, G., Montzka, S. A., Oram, D. E., Röckmann, T., Stroh, F., Sturges, W. T., Vogel, B., and Laube, J. C.:
Aircraft-Based Observations of Ozone-Depleting Substances in the Upper Troposphere and Lower Stratosphere in and Above the Asian Summer Monsoon,
J. Geophys. Res.-Atmos.,
126, e2020JD033137, https://doi.org/10.1029/2020JD033137, 2021. a
Andrews, A. E., Boering, K. A., Daube, B. C., Wofsy, S. C., Loewenstein, M., Jost, H., Podolske, J. R., Webster, C. R., Herman, R. L., Scott, D. C., Flesch, G. J., Moyer, E. J., Elkins, J. W., Dutton, G. S., Hurst, D. F., Moore, F. L., Ray, E. A., Romashkin, P. A., and Strahan, S. E.:
Mean ages of stratospheric air derived from in situ observations of CO2, CH4, and N2O,
J. Geophys. Res.-Atmos.,
106, 32295–32314, https://doi.org/10.1029/2001JD000465, 2001. a
Arfeuille, F., Luo, B. P., Heckendorn, P., Weisenstein, D., Sheng, J. X., Rozanov, E., Schraner, M., Brönnimann, S., Thomason, L. W., and Peter, T.: Modeling the stratospheric warming following the Mt. Pinatubo eruption: uncertainties in aerosol extinctions, Atmos. Chem. Phys., 13, 11221–11234, https://doi.org/10.5194/acp-13-11221-2013, 2013. a
Birner, T. and Bönisch, H.: Residual circulation trajectories and transit times into the extratropical lowermost stratosphere, Atmos. Chem. Phys., 11, 817–827, https://doi.org/10.5194/acp-11-817-2011, 2011. a
Bönisch, H., Engel, A., Birner, Th., Hoor, P., Tarasick, D. W., and Ray, E. A.: On the structural changes in the Brewer-Dobson circulation after 2000, Atmos. Chem. Phys., 11, 3937–3948, https://doi.org/10.5194/acp-11-3937-2011, 2011. a
Brasseur, G. and Solomon, S.:
Aeronomy of the middle atmosphere, 2 edn.,
Reidel, Dordrecht, The Netherlands, 1986. a
Brewer, A. W.:
Evidence for a world circulation provided by the measurements of helium and water vapour distribution in the stratosphere,
Q. J. Roy. Meteor. Soc.,
75, 351–363, https://doi.org/10.1002/qj.49707532603, 1949. a
Butchart, N. and Scaife, A. A.:
Removal of chlorofluorocarbons by increased mass exchange between the stratosphere and troposphere in a changing climate,
Nature,
410, 799–802, https://doi.org/10.1038/35071047, 2001. a
Butchart, N., Charlton-Perez, A. J., Cionni, I., Hardiman, S. C., Haynes, P. H., Krüger, K., Kushner, P. J., Newman, P. A., Osprey, S. M., Perlwitz, J., Sigmond, M., Wang, L., Akiyoshi, H., Austin, J., Bekki, S., Baumgaertner, A., Braesicke, P., Brühl, C., Chipperfield, M., Dameris, M., Dhomse, S., Eyring, V., Garcia, R., Garny, H., Jöckel, P., Lamarque, J.-F., Marchand, M., Michou, M., Morgenstern, O., Nakamura, T., Pawson, S., Plummer, D., Pyle, J., Rozanov, E., Scinocca, J., Shepherd, T. G., Shibata, K., Smale, D., Teyssèdre, H., Tian, W., Waugh, D., and Yamashita, Y.:
Multimodel climate and variability of the stratosphere,
J. Geophys. Res.-Atmos.,
116, D5, https://doi.org/10.1029/2010JD014995, 2011. a
Datskos, P., Carter, J., and Christophorou, L.:
Photodetachment of
Dee, D. P., Uppala, S. M., Simmons, A. J., Berrisford, P., Poli, P., Kobayashi, S., Andrae, U., Balmaseda, M. A., Balsamo, G., Bauer, P., Bechtold, P., Beljaars, A. C. M., van de Berg, L., Bidlot, J., Bormann, N., Delsol, C., Dragani, R., Fuentes, M., Geer, A. J., Haimberger, L., Healy, S. B., Hersbach, H., Hólm, E. V., Isaksen, L., Kållberg, P., Köhler, M., Matricardi, M., McNally, A. P., Monge-Sanz, B. M., Morcrette, J.-J., Park, B.-K., Peubey, C., de Rosnay, P., Tavolato, C., Thépaut, J.-N., and Vitart, F.:
The ERA-Interim reanalysis: Configuration and performance of the data assimilation system,
Q. J. Roy. Meteor. Soc.,
137, 553–597, https://doi.org/10.1002/qj.828, 2011. a, b
Dietmüller, S., Eichinger, R., Garny, H., Birner, T., Boenisch, H., Pitari, G., Mancini, E., Visioni, D., Stenke, A., Revell, L., Rozanov, E., Plummer, D. A., Scinocca, J., Jöckel, P., Oman, L., Deushi, M., Kiyotaka, S., Kinnison, D. E., Garcia, R., Morgenstern, O., Zeng, G., Stone, K. A., and Schofield, R.: Quantifying the effect of mixing on the mean age of air in CCMVal-2 and CCMI-1 models, Atmos. Chem. Phys., 18, 6699–6720, https://doi.org/10.5194/acp-18-6699-2018, 2018. a
Dietmüller, S., Garny, H., Eichinger, R., and Ball, W. T.: Analysis of recent lower-stratospheric ozone trends in chemistry climate models, Atmos. Chem. Phys., 21, 6811–6837, https://doi.org/10.5194/acp-21-6811-2021, 2021. a
Dlugokencky, E.:
Global Monitoring Laboratory – Carbon Cycle Greenhouse Gases – Trends in Atmospheric Sulpher Hexaflouride,
available at: https://www.esrl.noaa.gov/gmd/ccgg/trends_sf6/ (last access: 3 September 2020), 2005. a
Dobson, G. M. B. and Massey, H. S. W.:
Origin and distribution of the polyatomic molecules in the atmosphere,
P. R. Soc. Lond. A-Mat,
236, 187–193, https://doi.org/10.1098/rspa.1956.0127, 1956. a
Eichinger, R., Dietmüller, S., Garny, H., Šácha, P., Birner, T., Bönisch, H., Pitari, G., Visioni, D., Stenke, A., Rozanov, E., Revell, L., Plummer, D. A., Jöckel, P., Oman, L., Deushi, M., Kinnison, D. E., Garcia, R., Morgenstern, O., Zeng, G., Stone, K. A., and Schofield, R.: The influence of mixing on the stratospheric age of air changes in the 21st century, Atmos. Chem. Phys., 19, 921–940, https://doi.org/10.5194/acp-19-921-2019, 2019. a, b
Engel, A., Möbius, T., Bönisch, H., Schmidt, U., Heinz, R., Levin, I., Atlas, E., Aoki, S., Nakazawa, T., Sugawara, S., Moore, F., Hurst, D., Elkins, J., Schauffler, S., Andrews, A., and Boering, K.:
Age of stratospheric air unchanged within uncertainties over the past 30 years,
Nat. Geosci.,
2, 28–31, https://doi.org/10.1038/ngeo388, 2009. a, b, c, d, e, f, g, h, i, j, k, l, m, n, o, p, q
Eyring, V., Waugh, D. W., Bodeker, G. E., Cordero, E., Akiyoshi, H., Austin, J., Beagley, S. R., Boville, B. A., Braesicke, P., Brühl, C., Butchart, N., Chipperfield, M. P., Dameris, M., Deckert, R., Deushi, M., Frith, S. M., Garcia, R. R., Gettelman, A., Giorgetta, M. A., Kinnison, D. E., Mancini, E., Manzini, E., Marsh, D. R., Matthes, S., Nagashima, T., Newman, P. A., Nielsen, J. E., Pawson, S., Pitari, G., Plummer, D. A., Rozanov, E., Schraner, M., Scinocca, J. F., Semeniuk, K., Shepherd, T. G., Shibata, K., Steil, B., Stolarski, R. S., Tian, W., and Yoshiki, M.:
Multimodel projections of stratospheric ozone in the 21st century,
J. Geophys. Res.-Atmos.,
112, D16, https://doi.org/10.1029/2006JD008332, 2007. a
Garcia, R. and Randel, W.:
Acceleration of the Brewer-Dobson Circulation due to Increases in Greenhouse Gases,
J. Atmos. Sci.,
65, 2731–2739, https://doi.org/10.1175/2008JAS2712.1, 2008. a, b, c
Garcia, R. R., Randel, W. J., and Kinnison, D. E.:
On the Determination of Age of Air Trends from Atmospheric Trace Species,
J. Atmos. Sci.,
68, 139–154, https://doi.org/10.1175/2010JAS3527.1, 2011. a, b
Garny, H., Birner, T., Bönisch, H., and Bunzel, F.:
The effects of mixing on age of air,
J. Geophys. Res.-Atmos.,
119, 7015–7034, https://doi.org/10.1002/2013JD021417, 2014. a
Haenel, F. J., Stiller, G. P., von Clarmann, T., Funke, B., Eckert, E., Glatthor, N., Grabowski, U., Kellmann, S., Kiefer, M., Linden, A., and Reddmann, T.: Reassessment of MIPAS age of air trends and variability, Atmos. Chem. Phys., 15, 13161–13176, https://doi.org/10.5194/acp-15-13161-2015, 2015. a, b, c, d, e, f, g, h, i, j, k, l, m, n, o
Hall, T. M. and Plumb, R. A.:
Age as a diagnostic of stratospheric transport,
J. Geophys. Res.-Atmos.,
99, 1059–1070, https://doi.org/10.1029/93JD03192, 1994. a, b, c, d
Hall, T. M. and Waugh, D. W.:
The influence of nonlocal chemistry on tracer distributions: Inferring the mean age of air from SF6,
J. Geophys. Res.,
103, 13327–13336, https://doi.org/10.1029/98JD00170, 1998. a
Harrison, J. J.:
New infrared absorption cross sections for the infrared limb sounding of sulfur hexafluoride (SF6),
J. Quant. Spectrosc. Ra.,
254, 107202, https://doi.org/10.1016/j.jqsrt.2020.107202, 2020. a, b
Huey, L. G., Hanson, D. R., and Howard, C. J.:
Reactions of SF6- and I- with Atmospheric Trace Gases,
J. Phys. Chem.,
99, 5001–5008, https://doi.org/10.1021/j100014a021, 1995. a
Jöckel, P., Sander, R., Kerkweg, A., Tost, H., and Lelieveld, J.: Technical Note: The Modular Earth Submodel System (MESSy) – a new approach towards Earth System Modeling, Atmos. Chem. Phys., 5, 433–444, https://doi.org/10.5194/acp-5-433-2005, 2005. a, b, c
Jöckel, P., Tost, H., Pozzer, A., Kunze, M., Kirner, O., Brenninkmeijer, C. A. M., Brinkop, S., Cai, D. S., Dyroff, C., Eckstein, J., Frank, F., Garny, H., Gottschaldt, K.-D., Graf, P., Grewe, V., Kerkweg, A., Kern, B., Matthes, S., Mertens, M., Meul, S., Neumaier, M., Nützel, M., Oberländer-Hayn, S., Ruhnke, R., Runde, T., Sander, R., Scharffe, D., and Zahn, A.: Earth System Chemistry integrated Modelling (ESCiMo) with the Modular Earth Submodel System (MESSy) version 2.51, Geosci. Model Dev., 9, 1153–1200, https://doi.org/10.5194/gmd-9-1153-2016, 2016. a, b, c, d, e, f, g, h, i, j, k, l
Kovács, T., Feng, W., Totterdill, A., Plane, J. M. C., Dhomse, S., Gómez-Martín, J. C., Stiller, G. P., Haenel, F. J., Smith, C., Forster, P. M., García, R. R., Marsh, D. R., and Chipperfield, M. P.: Determination of the atmospheric lifetime and global warming potential of sulfur hexafluoride using a three-dimensional model, Atmos. Chem. Phys., 17, 883–898, https://doi.org/10.5194/acp-17-883-2017, 2017. a, b, c
Leedham Elvidge, E., Bönisch, H., Brenninkmeijer, C. A. M., Engel, A., Fraser, P. J., Gallacher, E., Langenfelds, R., Mühle, J., Oram, D. E., Ray, E. A., Ridley, A. R., Röckmann, T., Sturges, W. T., Weiss, R. F., and Laube, J. C.: Evaluation of stratospheric age of air from CF4, C2F6, C3F8, CHF3, HFC-125, HFC-227ea and SF6; implications for the calculations of halocarbon lifetimes, fractional release factors and ozone depletion potentials, Atmos. Chem. Phys., 18, 3369–3385, https://doi.org/10.5194/acp-18-3369-2018, 2018. a, b
Marsh, D. R., Mills, M. J., Kinnison, D. E., Lamarque, J.-F., Calvo, N., and Polvani, L. M.:
Climate Change from 1850 to 2005 Simulated in CESM1(WACCM),
J. Climate,
26, 7372–7391, https://doi.org/10.1175/JCLI-D-12-00558.1, 2013. a
Morgenstern, O., Hegglin, M. I., Rozanov, E., O'Connor, F. M., Abraham, N. L., Akiyoshi, H., Archibald, A. T., Bekki, S., Butchart, N., Chipperfield, M. P., Deushi, M., Dhomse, S. S., Garcia, R. R., Hardiman, S. C., Horowitz, L. W., Jöckel, P., Josse, B., Kinnison, D., Lin, M., Mancini, E., Manyin, M. E., Marchand, M., Marécal, V., Michou, M., Oman, L. D., Pitari, G., Plummer, D. A., Revell, L. E., Saint-Martin, D., Schofield, R., Stenke, A., Stone, K., Sudo, K., Tanaka, T. Y., Tilmes, S., Yamashita, Y., Yoshida, K., and Zeng, G.: Review of the global models used within phase 1 of the Chemistry–Climate Model Initiative (CCMI), Geosci. Model Dev., 10, 639–671, https://doi.org/10.5194/gmd-10-639-2017, 2017. a
Ploeger, F., Abalos, M., Birner, T., Konopka, P., Legras, B., Müller, R., and Riese, M.:
Quantifying the effects of mixing and residual circulation on trends of stratospheric mean age of air,
Geophys. Res. Lett.,
42, 2047–2054, https://doi.org/10.1002/2014GL062927, 2014GL062927, 2015. a
Plumb, I. C., Vohralik, P. F., and Ryan, K. R.:
Normalization of correlations for atmospheric species with chemical loss,
J. Geophys. Res.-Atmos.,
104, 11723–11732, https://doi.org/10.1029/1999JD900014, 1999. a
Ravishankara, A. R., Solomon, S., Turnipseed, A. A., and Warren, R. F.:
Atmospheric lifetimes of long-lived halogenated species,
Science,
17, 194–199, https://doi.org/10.1126/science.259.5092.194, 1993. a, b, c
Ray, E. A., Moore, F. L., Rosenlof, K. H., Davis, S. M., Sweeney, C., Tans, P., Wang, T., Elkins, J. W., Bönisch, H., Engel, A., Sugawara, S., Nakazawa, T., and Aoki, S.:
Improving stratospheric transport trend analysis based on SF6 and CO2 measurements,
J. Geophys. Res.-Atmos.,
14, 110–128, https://doi.org/10.1002/2014JD021802, 2014. a, b, c
Ray, E. A., Moore, F., Elkins, J. W., Rosenlof, K., Laube, J., Röckmann, T., Marsh, D., and Andrews, A.:
Quantification of the SF6 lifetime based on mesospheric loss measured in the stratospheric polar vortex,
J. Geophys. Res.-Atmos.,
122, 4626–4638, https://doi.org/10.1002/2016JD026198, 2017. a, b, c, d, e, f, g
Roeckner, E., Bäuml, G., Bonaventura, L., Brokopf, R., Esch, M., Giorgetta, M., Hagemann, S., Kirchner, I., Kornblueh, L., Manzini, E., Rhodin, A., Schlese, U., Schulzweida, U., and Tompkins, A.:
The atmospheric general circulation model ECHAM 5. PART I: model description, Max Planck Institute for Meteorology Report,
Max Planck Institute for Meteorology, 349, 2003. a
Schoeberl, M. R., Sparling, L. C., Jackman, C. H., and Fleming, E. L.:
A Lagrangian view of stratospheric trace gas distributions,
J. Geophys. Res.-Atmos.,
105, 1537–1552, https://doi.org/10.1029/1999JD900787, 2000. a
SPARC:
SPARC CCMVal Report on the Evaluation of Chemistry-Climate Models, Tech. rep.,
SPARC, available at: http://www.sparc-climate.org/publications/sparc-reports/ (last access: 15 November 2021), 2010. a
Stiller, G., Harrison, J., Haenel, F., Glatthor, N., Kellmann, S., and von Clarmann, T.:
Improved global distributions of SF6 and mean age of stratospheric air by use of new spectroscopic data,
in: EGU General Assembly 2020, Online, 4–8 May 2020, EGU2020-2660, https://doi.org/10.5194/egusphere-egu2020-2660, 2020. a, b, c, d, e
Stiller, G. P., von Clarmann, T., Höpfner, M., Glatthor, N., Grabowski, U., Kellmann, S., Kleinert, A., Linden, A., Milz, M., Reddmann, T., Steck, T., Fischer, H., Funke, B., López-Puertas, M., and Engel, A.:
Global distribution of mean age of stratospheric air from MIPAS SF6 measurements, Atmos. Chem. Phys., 8, 677–695, https://doi.org/10.5194/acp-8-677-2008, 2008. a
Stiller, G. P., von Clarmann, T., Haenel, F., Funke, B., Glatthor, N., Grabowski, U., Kellmann, S., Kiefer, M., Linden, A., Lossow, S., and López-Puertas, M.: Observed temporal evolution of global mean age of stratospheric air for the 2002 to 2010 period, Atmos. Chem. Phys., 12, 3311–3331, https://doi.org/10.5194/acp-12-3311-2012, 2012. a, b, c, d, e, f, g
Stiller, G. P., Fierli, F., Ploeger, F., Cagnazzo, C., Funke, B., Haenel, F. J., Reddmann, T., Riese, M., and von Clarmann, T.: Shift of subtropical transport barriers explains observed hemispheric asymmetry of decadal trends of age of air, Atmos. Chem. Phys., 17, 11177–11192, https://doi.org/10.5194/acp-17-11177-2017, 2017. a, b
Stiller, G. P., Harrison, J. J., Haenel, F. J., Glatthor, N., and Kellmann, S.: Technical note: Improved global distributions of SF6 and mean age of stratospheric air by use of new spectroscopic data, Atmos. Chem. Phys. Discuss., in preparation, 2022. a
Totterdill, A., Kovács, T., Gómez Martín, J. C., Feng, W., and Plane, J. M. C.:
Mesospheric Removal of Very Long-Lived Greenhouse Gases SF6 and CFC-115 by Metal Reactions, Lyman-α Photolysis, and Electron Attachment,
J. Phys. Chem. A,
119, 2016–2025, https://doi.org/10.1021/jp5123344, pMID: 25647411, 2015. a
Volk, C. M., Elkins, J. W., Fahey, D. W., Dutton, G. S., Gilligan, J. M., Loewenstein, M., Podolske, J. R., Chan, K. R., and Gunson, M. R.:
Evaluation of source gas lifetimes from stratospheric observations,
J. Geophys. Res.-Atmos.,
102, 25543–25564, https://doi.org/10.1029/97JD02215, 1997. a
von Clarmann, T., Stiller, G., Grabowski, U., Eckert, E., and Orphal, J.: Technical Note: Trend estimation from irregularly sampled, correlated data, Atmos. Chem. Phys., 10, 6737–6747, https://doi.org/10.5194/acp-10-6737-2010, 2010. a
Waugh, D. and Hall, T.:
Age of stratospheric air: Theory, observations, and models,
Rev. Geophys.,
40, 1-1–1-26, https://doi.org/10.1029/2000RG000101, 2002. a, b
WMO:
Atmospheric ozone 1985 – volume I–III: assessment of our understanding of the processes controlling its present distribution and change,
World Meteorological Organization, 1986. a
Short summary
SF6-derived trends of stratospheric AoA from observations and model simulations disagree in sign. SF6 experiences chemical degradation, which we explicitly integrate in a global climate model. In our simulations, the AoA trend changes sign when SF6 sinks are considered; thus, the process has the potential to reconcile simulated with observed AoA trends. We show that the positive AoA trend is due to the SF6 sinks themselves and provide a first approach for a correction to account for SF6 loss.
SF6-derived trends of stratospheric AoA from observations and model simulations disagree in...
Altmetrics
Final-revised paper
Preprint