Articles | Volume 15, issue 7
https://doi.org/10.5194/acp-15-3755-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-3755-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
07 Apr 2015
Research article |
| 07 Apr 2015
Monsoonal variations in aerosol optical properties and estimation of aerosol optical depth using ground-based meteorological and air quality data in Peninsular Malaysia
F. Tan
CORRESPONDING AUTHOR
School of Physics, Universiti Sains Malaysia, 11800 Penang, Malaysia
H. S. Lim
School of Physics, Universiti Sains Malaysia, 11800 Penang, Malaysia
K. Abdullah
School of Physics, Universiti Sains Malaysia, 11800 Penang, Malaysia
T. L. Yoon
School of Physics, Universiti Sains Malaysia, 11800 Penang, Malaysia
B. Holben
NASA Goddard Space Flight Center, Greenbelt, Maryland, USA
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This paper describes aspects of the 2012 7 Southeast Asian Studies (7SEAS) operations period, the largest within the Maritime Continent. Included were an enhanced deployment of Aerosol Robotic Network (AERONET) sun photometers, multiple lidars, and a Singapore supersite. Simultaneously, a ship was dispatched to the Palawan Archipelago and Sulu Sea of the Philippines for September 2012 to observe transported smoke and pollution as it entered the southwest monsoon trough.
Graydon Snider, Crystal L. Weagle, Kalaivani K. Murdymootoo, Amanda Ring, Yvonne Ritchie, Emily Stone, Ainsley Walsh, Clement Akoshile, Nguyen Xuan Anh, Rajasekhar Balasubramanian, Jeff Brook, Fatimah D. Qonitan, Jinlu Dong, Derek Griffith, Kebin He, Brent N. Holben, Ralph Kahn, Nofel Lagrosas, Puji Lestari, Zongwei Ma, Amit Misra, Leslie K. Norford, Eduardo J. Quel, Abdus Salam, Bret Schichtel, Lior Segev, Sachchida Tripathi, Chien Wang, Chao Yu, Qiang Zhang, Yuxuan Zhang, Michael Brauer, Aaron Cohen, Mark D. Gibson, Yang Liu, J. Vanderlei Martins, Yinon Rudich, and Randall V. Martin
Atmos. Chem. Phys., 16, 9629–9653, https://doi.org/10.5194/acp-16-9629-2016, https://doi.org/10.5194/acp-16-9629-2016, 2016
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We examine the chemical composition of fine particulate matter (PM2.5) collected on filters at traditionally undersampled, globally dispersed urban locations. Several PM2.5 chemical components (e.g. ammonium sulfate, ammonium nitrate, and black carbon) vary by more than an order of magnitude between sites while aerosol hygroscopicity varies by a factor of 2. Enhanced anthropogenic dust fractions in large urban areas are apparent from high Zn : Al ratios.
Makiko Nakata, Itaru Sano, Sonoyo Mukai, and Brent N. Holben
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-182, https://doi.org/10.5194/acp-2016-182, 2016
Revised manuscript not accepted
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We document the spatial and temporal variations of atmospheric aerosols in East Asia, specifically focusing on the NASA/AERONET-Osaka site in March 2012 during the AERONET “DRAGON-Japan” campaign. It has been shown that airborne pollutants can influence both the local atmosphere near to their source and relatively remote locations due to long-range transportation.
Myungje Choi, Jhoon Kim, Jaehwa Lee, Mijin Kim, Young-Je Park, Ukkyo Jeong, Woogyung Kim, Hyunkee Hong, Brent Holben, Thomas F. Eck, Chul H. Song, Jae-Hyun Lim, and Chang-Keun Song
Atmos. Meas. Tech., 9, 1377–1398, https://doi.org/10.5194/amt-9-1377-2016, https://doi.org/10.5194/amt-9-1377-2016, 2016
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The Geostationary Ocean Color Imager (GOCI) is the first ocean color sensor in geostationary orbit. It enables hourly aerosol optical properties to be observed in high spatial resolution. This study presents improvements of the GOCI Yonsei Aerosol Retrieval (YAER) algorithm and its validation results using ground-based and other satellite-based observation products during DRAGON-NE Asia 2012 Campaign. Retrieval errors are also analyzed according to various factors through the validation studies.
Anatoli Chaikovsky, Oleg Dubovik, Brent Holben, Andrey Bril, Philippe Goloub, Didier Tanré, Gelsomina Pappalardo, Ulla Wandinger, Ludmila Chaikovskaya, Sergey Denisov, Jan Grudo, Anton Lopatin, Yana Karol, Tatsiana Lapyonok, Vassilis Amiridis, Albert Ansmann, Arnoud Apituley, Lucas Allados-Arboledas, Ioannis Binietoglou, Antonella Boselli, Giuseppe D'Amico, Volker Freudenthaler, David Giles, María José Granados-Muñoz, Panayotis Kokkalis, Doina Nicolae, Sergey Oshchepkov, Alex Papayannis, Maria Rita Perrone, Alexander Pietruczuk, Francesc Rocadenbosch, Michaël Sicard, Ilya Slutsker, Camelia Talianu, Ferdinando De Tomasi, Alexandra Tsekeri, Janet Wagner, and Xuan Wang
Atmos. Meas. Tech., 9, 1181–1205, https://doi.org/10.5194/amt-9-1181-2016, https://doi.org/10.5194/amt-9-1181-2016, 2016
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This paper presents a detailed description of LIRIC (LIdar-Radiometer Inversion Code) algorithm for simultaneous processing of coincident lidar and radiometric observations for the retrieval of the aerosol concentrations. As the lidar/radiometric input data we use measurements from European Aerosol Research Lidar Network (EARLINET) lidars and collocated sun-photometers of Aerosol Robotic Network (AERONET). The LIRIC software package was implemented and tested at a number of EARLINET stations.
África Barreto, Emilio Cuevas, María-José Granados-Muñoz, Lucas Alados-Arboledas, Pedro M. Romero, Julian Gröbner, Natalia Kouremeti, Antonio F. Almansa, Tom Stone, Carlos Toledano, Roberto Román, Mikhail Sorokin, Brent Holben, Marius Canini, and Margarita Yela
Atmos. Meas. Tech., 9, 631–654, https://doi.org/10.5194/amt-9-631-2016, https://doi.org/10.5194/amt-9-631-2016, 2016
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This paper presents the new photometer CE318-T, able to perform daytime and
night-time photometric measurements using the sun and the moon as light
sources. This new device permits a complete cycle of diurnal aerosol and water vapour measurements to be extracted, valuable to enhance atmospheric monitoring. We have also highlighted the ability of this new device to capture short-term atmospheric variations, critical for climate studies.
M. Kim, J. Kim, U. Jeong, W. Kim, H. Hong, B. Holben, T. F. Eck, J. H. Lim, C. K. Song, S. Lee, and C.-Y. Chung
Atmos. Chem. Phys., 16, 1789–1808, https://doi.org/10.5194/acp-16-1789-2016, https://doi.org/10.5194/acp-16-1789-2016, 2016
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An aerosol model optimized for East Asia is improved by applying inversion data from the DRAGON-NE Asia 2012 campaign, and is applied to an AOD retrieval algorithm using single visible measurements from a GEO satellite. In sensitivity tests, a 4 % overestimation in SSA can cause an underestimation in AOD of over 20 %. In accordance with the test, the overestimating tendency of AOD was improved by 8 % after the modification of the aerosol model.
G. L. Schuster, O. Dubovik, A. Arola, T. F. Eck, and B. N. Holben
Atmos. Chem. Phys., 16, 1587–1602, https://doi.org/10.5194/acp-16-1587-2016, https://doi.org/10.5194/acp-16-1587-2016, 2016
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Some authors have recently suggested that the spectral dependence of aerosol absorption may be used to separate soot carbon absorption from the aerosol absorption associated with organic carbon and dust. We demonstrate that this approach is inconsistent with the underlying assumptions that are required to infer aerosol absorption through remote sensing techniques, and that carbonaceous aerosols can not be differentiated from dust by exclusively using spectral absorption signatures.
Q. Xiao, H. Zhang, M. Choi, S. Li, S. Kondragunta, J. Kim, B. Holben, R. C. Levy, and Y. Liu
Atmos. Chem. Phys., 16, 1255–1269, https://doi.org/10.5194/acp-16-1255-2016, https://doi.org/10.5194/acp-16-1255-2016, 2016
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Using ground AOD measurements from AERONET, DRAGON-Asia Campaign, and handheld sunphotometers, we evaluated emerging aerosol products from VIIRS, GOCI, and Terra and Aqua MODIS (Collection 6) in East Asia in 2012–2013. We found that satellite aerosol products performed better in tracking the day-to-day variability than the high-resolution spatial variability. VIIRS EDR and GOCI products provided the most accurate AOD retrievals, while VIIRS IP and MODIS C6 3 km products had positive biases.
U. Jeong, J. Kim, C. Ahn, O. Torres, X. Liu, P. K. Bhartia, R. J. D. Spurr, D. Haffner, K. Chance, and B. N. Holben
Atmos. Chem. Phys., 16, 177–193, https://doi.org/10.5194/acp-16-177-2016, https://doi.org/10.5194/acp-16-177-2016, 2016
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An aerosol retrieval and error analysis algorithm using OMI measurements based on an optimal-estimation method was developed in this study. The aerosol retrievals were validated using the DRAGON campaign products. The estimated errors of the retrievals represented the actual biases between retrieval and AERONET measurements well. The retrievals, with their estimated uncertainties, are expected to be valuable for relevant studies, such as trace gas retrieval and data assimilation.
D. Pérez-Ramírez, I. Veselovskii, D. N. Whiteman, A. Suvorina, M. Korenskiy, A. Kolgotin, B. Holben, O. Dubovik, A. Siniuk, and L. Alados-Arboledas
Atmos. Meas. Tech., 8, 3117–3133, https://doi.org/10.5194/amt-8-3117-2015, https://doi.org/10.5194/amt-8-3117-2015, 2015
H. Che, X.-Y. Zhang, X. Xia, P. Goloub, B. Holben, H. Zhao, Y. Wang, X.-C. Zhang, H. Wang, L. Blarel, B. Damiri, R. Zhang, X. Deng, Y. Ma, T. Wang, F. Geng, B. Qi, J. Zhu, J. Yu, Q. Chen, and G. Shi
Atmos. Chem. Phys., 15, 7619–7652, https://doi.org/10.5194/acp-15-7619-2015, https://doi.org/10.5194/acp-15-7619-2015, 2015
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This work studied more than 10 years of measurements of aerosol optical depths (AODs) made for 50 sites of CARSNET compiled into a climatology of aerosol optical properties for China. It lets us see a detailed full-scale description of AOD observations over China. The results would benefit us a lot in comprehending the temporal and special distribution aerosol optical property over China. Also the data would be valuable to communities of aerosol satellite retrieval, modelling, etc.
K. Knobelspiesse, B. van Diedenhoven, A. Marshak, S. Dunagan, B. Holben, and I. Slutsker
Atmos. Meas. Tech., 8, 1537–1554, https://doi.org/10.5194/amt-8-1537-2015, https://doi.org/10.5194/amt-8-1537-2015, 2015
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We test if ground-based sun photometers/radiometers like those in the Aerosol Robotic Network (AERONET) can use the polarization sensitivity of some instruments for improved cloud optical property retrieval. Our radiative transfer simulations show that the direction of linear polarization indicates cloud thermodynamic phase for optically thin clouds. In practice, data analysis shows a weak response with AERONET instruments, most likely due to noise and orientation/calibration ambiguity.
J. S. Reid, N. D. Lagrosas, H. H. Jonsson, E. A. Reid, W. R. Sessions, J. B. Simpas, S. N. Uy, T. J. Boyd, S. A. Atwood, D. R. Blake, J. R. Campbell, S. S. Cliff, B. N. Holben, R. E. Holz, E. J. Hyer, P. Lynch, S. Meinardi, D. J. Posselt, K. A. Richardson, S. V. Salinas, A. Smirnov, Q. Wang, L. Yu, and J. Zhang
Atmos. Chem. Phys., 15, 1745–1768, https://doi.org/10.5194/acp-15-1745-2015, https://doi.org/10.5194/acp-15-1745-2015, 2015
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This paper reports on the first measurements of aerosol particles embedded in the convectively active southwest monsoonal flow of the South China Sea. The paper describes the research cruise and discusses how variability in aerosol characteristics relates to regional meteorological phenomena such as and the Madden Julian Oscillation, tropical cyclones, squall lines and the monsoonal flow itself. Of special interest is how aerosol transport relates to meteorological drivers of convective activity.
I. Veselovskii, D. N Whiteman, M. Korenskiy, A. Suvorina, A. Kolgotin, A. Lyapustin, Y. Wang, M. Chin, H. Bian, T. L. Kucsera, D. Pérez-Ramírez, and B. Holben
Atmos. Chem. Phys., 15, 1647–1660, https://doi.org/10.5194/acp-15-1647-2015, https://doi.org/10.5194/acp-15-1647-2015, 2015
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The multi-wavelength lidar technique was applied to the study of a smoke event near Washington, DC on 26-28 August 2013. Satellite observations combined with transport model predictions imply that the smoke plume originated mainly from Wyoming/Idaho forest fires. The NASA GSFC multi-wavelength Mie-Raman lidar was used to profile the smoke particle parameters such as volume density, effective radius and the real part of the refractive index.
G. Snider, C. L. Weagle, R. V. Martin, A. van Donkelaar, K. Conrad, D. Cunningham, C. Gordon, M. Zwicker, C. Akoshile, P. Artaxo, N. X. Anh, J. Brook, J. Dong, R. M. Garland, R. Greenwald, D. Griffith, K. He, B. N. Holben, R. Kahn, I. Koren, N. Lagrosas, P. Lestari, Z. Ma, J. Vanderlei Martins, E. J. Quel, Y. Rudich, A. Salam, S. N. Tripathi, C. Yu, Q. Zhang, Y. Zhang, M. Brauer, A. Cohen, M. D. Gibson, and Y. Liu
Atmos. Meas. Tech., 8, 505–521, https://doi.org/10.5194/amt-8-505-2015, https://doi.org/10.5194/amt-8-505-2015, 2015
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We have initiated a global network of ground-level monitoring stations to measure concentrations of fine aerosols in urban environments. Our findings include major ions species, total mass, and total scatter at three wavelengths. Results will be used to further evaluate and enhance satellite remote sensing estimates.
S. Seo, J. Kim, H. Lee, U. Jeong, W. Kim, B. N. Holben, S.-W. Kim, C. H. Song, and J. H. Lim
Atmos. Chem. Phys., 15, 319–334, https://doi.org/10.5194/acp-15-319-2015, https://doi.org/10.5194/acp-15-319-2015, 2015
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The estimation of PM10 from optical measurement of AERONET and MODIS by various empirical models was evaluated for the DRAGON-Asia campaign. The results showed the importance of boundary layer height (BLH) and effective radius (Reff) in estimating PM10. The highest correlation between the estimated and measured values was found to be 0.81 in winter due to the stagnant air mass and low BLH, while the poorest values were 0.54 in spring due to the influence of long-range transport above BLH.
T. F. Eck, B. N. Holben, J. S. Reid, A. Arola, R. A. Ferrare, C. A. Hostetler, S. N. Crumeyrolle, T. A. Berkoff, E. J. Welton, S. Lolli, A. Lyapustin, Y. Wang, J. S. Schafer, D. M. Giles, B. E. Anderson, K. L. Thornhill, P. Minnis, K. E. Pickering, C. P. Loughner, A. Smirnov, and A. Sinyuk
Atmos. Chem. Phys., 14, 11633–11656, https://doi.org/10.5194/acp-14-11633-2014, https://doi.org/10.5194/acp-14-11633-2014, 2014
A. M. Sayer, N. C. Hsu, T. F. Eck, A. Smirnov, and B. N. Holben
Atmos. Chem. Phys., 14, 11493–11523, https://doi.org/10.5194/acp-14-11493-2014, https://doi.org/10.5194/acp-14-11493-2014, 2014
P. Sawamura, D. Müller, R. M. Hoff, C. A. Hostetler, R. A. Ferrare, J. W. Hair, R. R. Rogers, B. E. Anderson, L. D. Ziemba, A. J. Beyersdorf, K. L. Thornhill, E. L. Winstead, and B. N. Holben
Atmos. Meas. Tech., 7, 3095–3112, https://doi.org/10.5194/amt-7-3095-2014, https://doi.org/10.5194/amt-7-3095-2014, 2014
R. P. Aryal, K. J. Voss, P. A. Terman, W. C. Keene, J. L. Moody, E. J. Welton, and B. N. Holben
Atmos. Chem. Phys., 14, 7617–7629, https://doi.org/10.5194/acp-14-7617-2014, https://doi.org/10.5194/acp-14-7617-2014, 2014
M. Chin, T. Diehl, Q. Tan, J. M. Prospero, R. A. Kahn, L. A. Remer, H. Yu, A. M. Sayer, H. Bian, I. V. Geogdzhayev, B. N. Holben, S. G. Howell, B. J. Huebert, N. C. Hsu, D. Kim, T. L. Kucsera, R. C. Levy, M. I. Mishchenko, X. Pan, P. K. Quinn, G. L. Schuster, D. G. Streets, S. A. Strode, O. Torres, and X.-P. Zhao
Atmos. Chem. Phys., 14, 3657–3690, https://doi.org/10.5194/acp-14-3657-2014, https://doi.org/10.5194/acp-14-3657-2014, 2014
H. Che, X. Xia, J. Zhu, Z. Li, O. Dubovik, B. Holben, P. Goloub, H. Chen, V. Estelles, E. Cuevas-Agulló, L. Blarel, H. Wang, H. Zhao, X. Zhang, Y. Wang, J. Sun, R. Tao, X. Zhang, and G. Shi
Atmos. Chem. Phys., 14, 2125–2138, https://doi.org/10.5194/acp-14-2125-2014, https://doi.org/10.5194/acp-14-2125-2014, 2014
M. E. Park, C. H. Song, R. S. Park, J. Lee, J. Kim, S. Lee, J.-H. Woo, G. R. Carmichael, T. F. Eck, B. N. Holben, S.-S. Lee, C. K. Song, and Y. D. Hong
Atmos. Chem. Phys., 14, 659–674, https://doi.org/10.5194/acp-14-659-2014, https://doi.org/10.5194/acp-14-659-2014, 2014
J. L. Moody, W. C. Keene, O. R. Cooper, K. J. Voss, R. Aryal, S. Eckhardt, B. Holben, J. R. Maben, M. A. Izaguirre, and J. N. Galloway
Atmos. Chem. Phys., 14, 691–717, https://doi.org/10.5194/acp-14-691-2014, https://doi.org/10.5194/acp-14-691-2014, 2014
Y. Choi, Y. S. Ghim, and B. N. Holben
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-13-26627-2013, https://doi.org/10.5194/acpd-13-26627-2013, 2013
Revised manuscript not accepted
L. A. Munchak, R. C. Levy, S. Mattoo, L. A. Remer, B. N. Holben, J. S. Schafer, C. A. Hostetler, and R. A. Ferrare
Atmos. Meas. Tech., 6, 1747–1759, https://doi.org/10.5194/amt-6-1747-2013, https://doi.org/10.5194/amt-6-1747-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Revealing dominant patterns of aerosol regimes in the lower troposphere and their evolution from preindustrial times to the future in global climate model simulations
Improving estimation of a record-breaking east Asian dust storm emission with lagged aerosol Ångström exponent observations
Impact of biomass burning aerosols (BBA) on the tropical African climate in an ocean–atmosphere–aerosol coupled climate model
Retrieval of refractive index and water content for the coating materials of aged black carbon aerosol based on optical properties: a theoretical analysis
Predicting hygroscopic growth of organosulfur aerosol particles using COSMOtherm
Dust aerosol from the Aralkum Desert influences the radiation budget and atmospheric dynamics of Central Asia
Global modeling of aerosol nucleation with a semi-explicit chemical mechanism for highly oxygenated organic molecules (HOMs)
Synergistic effects of the winter North Atlantic Oscillation (NAO) and El Niño–Southern Oscillation (ENSO) on dust activities in North China during the following spring
Aerosol composition, air quality, and boundary layer dynamics in the urban background of Stuttgart in winter
Measurement report: Source attribution and estimation of black carbon levels in an urban hotspot of the central Po Valley – an integrated approach combining high-resolution dispersion modelling and micro-aethalometers
Microphysical modelling of aerosol scavenging by different types of clouds: description and validation of the approach
Insights into the sources of ultrafine particle numbers at six European urban sites obtained by investigating COVID-19 lockdowns
In-plume and out-of-plume analysis of aerosol–cloud interactions derived from the 2014–2015 Holuhraun volcanic eruption
Impacts of atmospheric circulation patterns and cloud inhibition on aerosol radiative effect and boundary layer structure during winter air pollution in Sichuan Basin, China
Investigating the sign of stratocumulus adjustments to aerosols in the ICON global storm-resolving model
A model study investigating the sensitivity of aerosol forcing to the volatilities of semi-volatile organic compounds
Decomposing the effective radiative forcing of anthropogenic aerosols based on CMIP6 Earth system models
The role of interfacial tension in the size-dependent phase separation of atmospheric aerosol particles
Modeling impacts of dust mineralogy on fast climate response
Representation of iron aerosol size distributions is critical in evaluating atmospheric soluble iron input to the ocean
Uncertainties in laboratory-measured shortwave refractive indices of mineral dust aerosols and derived optical properties: a theoretical assessment
Diagnosing uncertainties in global biomass burning emission inventories and their impact on modeled air pollutants
Solar radiation estimation in West Africa: impact of dust conditions during 2021 dry season
Role of atmospheric aerosols in severe winter fog over the Indo-Gangetic Plain of India: a case study
Long-term variability in black carbon emissions constrained by gap-filled absorption aerosol optical depth and associated premature mortality in China
Intercomparison of aerosol optical depths from four reanalyses and their multi-reanalysis consensus
Global aviation contrail climate effects from 2019 to 2021
Multi-model effective radiative forcing of the 2020 sulphur cap for shipping
Rapid iodine oxoacid nucleation enhanced by dimethylamine in broad marine regions
Simulations of the impact of cloud condensation nuclei and ice-nucleating particles perturbations on the microphysics and radar reflectivity factor of stratiform mixed-phase clouds
Warming effects of reduced sulfur emissions from shipping
Aerosols in the central Arctic cryosphere: satellite and model integrated insights during Arctic spring and summer
Observationally constrained regional variations of shortwave absorption by iron oxides emphasize the cooling effect of dust
Droplet collection efficiencies inferred from satellite retrievals constrain effective radiative forcing of aerosol–cloud interactions
Global aerosol-type classification using a new hybrid algorithm and Aerosol Robotic Network data
Simulated phase state and viscosity of secondary organic aerosols over China
Comparing the simulated influence of biomass burning plumes on low-level clouds over the southeastern Atlantic under varying smoke conditions
A global dust emission dataset for estimating dust radiative forcings in climate models
Improved simulations of biomass burning aerosol optical properties and lifetimes in the NASA GEOS Model during the ORACLES-I campaign
Sharp increase in Saharan dust intrusions over the western Euro-Mediterranean in February–March 2020–2022 and associated atmospheric circulation
Temporal and spatial variations in dust activity in Australia based on remote sensing and reanalysis datasets
Sensitivity of global direct aerosol shortwave radiative forcing to uncertainties in aerosol optical properties
Molecular-level study on the role of methanesulfonic acid in iodine oxoacid nucleation
Regional to global distributions, trends, and drivers of biogenic volatile organic compound emission from 2001 to 2020
Impacts of ice-nucleating particles on cirrus clouds and radiation derived from global model simulations with MADE3 in EMAC
Seasonal characteristics of emission, distribution, and radiative effect of marine organic aerosols over the western Pacific Ocean: an investigation with a coupled regional climate aerosol model
Fire–precipitation interactions amplify the quasi-biennial variability in fires over southern Mexico and Central America
Improved estimates of smoke exposure during Australia fire seasons: importance of quantifying plume injection heights
New particle formation induced by anthropogenic–biogenic interactions on the southeastern Tibetan Plateau
Investigation of observed dust trends over the Middle East region in NASA Goddard Earth Observing System (GEOS) model simulations
Jingmin Li, Mattia Righi, Johannes Hendricks, Christof G. Beer, Ulrike Burkhardt, and Anja Schmidt
Atmos. Chem. Phys., 24, 12727–12747, https://doi.org/10.5194/acp-24-12727-2024, https://doi.org/10.5194/acp-24-12727-2024, 2024
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Aiming to understand underlying patterns and trends in aerosols, we characterize the spatial patterns and long-term evolution of lower tropospheric aerosols by clustering multiple aerosol properties from preindustrial times to the year 2050 under three Shared
Socioeconomic Pathway scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Socioeconomic Pathway scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Yueming Cheng, Tie Dai, Junji Cao, Daisuke Goto, Jianbing Jin, Teruyuki Nakajima, and Guangyu Shi
Atmos. Chem. Phys., 24, 12643–12659, https://doi.org/10.5194/acp-24-12643-2024, https://doi.org/10.5194/acp-24-12643-2024, 2024
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In March 2021, east Asia experienced an outbreak of severe dust storms after an absence of 1.5 decades. Here, we innovatively used the time-lagged ground-based aerosol size information with the fixed-lag ensemble Kalman smoother to optimize dust emission and reproduce the dust storm. This work is valuable for not only the quantification of health damage, aviation risks, and profound impacts on the Earth's system but also revealing the climatic driving force and the process of desertification.
Marc Mallet, Aurore Voldoire, Fabien Solmon, Pierre Nabat, Thomas Drugé, and Romain Roehrig
Atmos. Chem. Phys., 24, 12509–12535, https://doi.org/10.5194/acp-24-12509-2024, https://doi.org/10.5194/acp-24-12509-2024, 2024
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This study investigates the interactions between smoke aerosols and climate in tropical Africa using a coupled ocean–atmosphere–aerosol climate model. The work shows that smoke plumes have a significant impact by increasing the low-cloud fraction, decreasing the ocean and continental surface temperature and reducing the precipitation of coastal western Africa. It also highlights the role of the ocean temperature response and its feedbacks for the September–November season.
Jia Liu, Cancan Zhu, Donghui Zhou, and Jinbao Han
Atmos. Chem. Phys., 24, 12341–12354, https://doi.org/10.5194/acp-24-12341-2024, https://doi.org/10.5194/acp-24-12341-2024, 2024
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The hydrophilic coatings of aged black carbon (BC) particles absorb moisture during the hygroscopic growth process, but it is difficult to characterize how much water is absorbed under different relative humidities (RHs). In this study, we propose a method to obtain the water content in the coatings based on the equivalent complex refractive index retrieved from optical properties. This method is verified from a theoretical perspective, and it performs well for thickly coated BC at high RHs.
Zijun Li, Angela Buchholz, and Noora Hyttinen
Atmos. Chem. Phys., 24, 11717–11725, https://doi.org/10.5194/acp-24-11717-2024, https://doi.org/10.5194/acp-24-11717-2024, 2024
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Evaluating organosulfur (OS) hygroscopicity is important for assessing aerosol–cloud climate interactions in the post-fossil-fuel future, when SO2 emissions decrease and OS compounds become increasingly important. Here a state-of-the-art quantum-chemistry-based method was used to predict the hygroscopic growth factors (HGFs) of a group of atmospherically relevant OS compounds and their mixtures with (NH4)2SO4. A good agreement was observed between their model-estimated and experimental HGFs.
Jamie R. Banks, Bernd Heinold, and Kerstin Schepanski
Atmos. Chem. Phys., 24, 11451–11475, https://doi.org/10.5194/acp-24-11451-2024, https://doi.org/10.5194/acp-24-11451-2024, 2024
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The Aralkum is a new desert in Central Asia formed by the desiccation of the Aral Sea. This has created a source of atmospheric dust, with implications for the balance of solar and thermal radiation. Simulating these effects using a dust transport model, we find that Aralkum dust adds radiative cooling effects to the surface and atmosphere on average but also adds heating events. Increases in surface pressure due to Aralkum dust strengthen the Siberian High and weaken the summer Asian heat low.
Xinyue Shao, Minghuai Wang, Xinyi Dong, Yaman Liu, Wenxiang Shen, Stephen R. Arnold, Leighton A. Regayre, Meinrat O. Andreae, Mira L. Pöhlker, Duseong S. Jo, Man Yue, and Ken S. Carslaw
Atmos. Chem. Phys., 24, 11365–11389, https://doi.org/10.5194/acp-24-11365-2024, https://doi.org/10.5194/acp-24-11365-2024, 2024
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Highly oxygenated organic molecules (HOMs) play an important role in atmospheric new particle formation (NPF). By semi-explicitly coupling the chemical mechanism of HOMs and a comprehensive nucleation scheme in a global climate model, the updated model shows better agreement with measurements of nucleation rate, growth rate, and NPF event frequency. Our results reveal that HOM-driven NPF leads to a considerable increase in particle and cloud condensation nuclei burden globally.
Falei Xu, Shuang Wang, Yan Li, and Juan Feng
Atmos. Chem. Phys., 24, 10689–10705, https://doi.org/10.5194/acp-24-10689-2024, https://doi.org/10.5194/acp-24-10689-2024, 2024
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This study examines how the winter North Atlantic Oscillation (NAO) and El Niño–Southern Oscillation (ENSO) affect dust activities in North China during the following spring. The results show that the NAO and ENSO, particularly in their negative phases, greatly influence dust activities. When both are negative, their combined effect on dust activities is even greater. This research highlights the importance of these climate patterns in predicting spring dust activities in North China.
Hengheng Zhang, Wei Huang, Xiaoli Shen, Ramakrishna Ramisetty, Junwei Song, Olga Kiseleva, Christopher Claus Holst, Basit Khan, Thomas Leisner, and Harald Saathoff
Atmos. Chem. Phys., 24, 10617–10637, https://doi.org/10.5194/acp-24-10617-2024, https://doi.org/10.5194/acp-24-10617-2024, 2024
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Our study unravels how stagnant winter conditions elevate aerosol levels in Stuttgart. Cloud cover at night plays a pivotal role, impacting morning air quality. Validating a key model, our findings aid accurate air quality predictions, crucial for effective pollution mitigation in urban areas.
Giorgio Veratti, Alessandro Bigi, Michele Stortini, Sergio Teggi, and Grazia Ghermandi
Atmos. Chem. Phys., 24, 10475–10512, https://doi.org/10.5194/acp-24-10475-2024, https://doi.org/10.5194/acp-24-10475-2024, 2024
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In a study of two consecutive winter seasons, we used measurements and modelling tools to identify the levels and sources of black carbon pollution in a medium-sized urban area of the Po Valley, Italy. Our findings show that biomass burning and traffic-related emissions (especially from Euro 4 diesel cars) significantly contribute to BC concentrations. This research offers crucial insights for policymakers and urban planners aiming to improve air quality in cities.
Pascal Lemaitre, Arnaud Quérel, Alexis Dépée, Alice Guerra Devigne, Marie Monier, Thibault Hiron, Chloé Soto Minguez, Daniel Hardy, and Andrea Flossmann
Atmos. Chem. Phys., 24, 9713–9732, https://doi.org/10.5194/acp-24-9713-2024, https://doi.org/10.5194/acp-24-9713-2024, 2024
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A new in-cloud scavenging scheme is proposed. It is based on a microphysical model of cloud formation and may be applied to long-distance atmospheric transport models (> 100 km) and climatic models. This model is applied to the two most extreme precipitating cloud types in terms of both relative humidity and vertical extension: cumulonimbus and stratus.
Alex Rowell, James Brean, David C. S. Beddows, Tuukka Petäjä, Máté Vörösmarty, Imre Salma, Jarkko V. Niemi, Hanna E. Manninen, Dominik van Pinxteren, Thomas Tuch, Kay Weinhold, Zongbo Shi, and Roy M. Harrison
Atmos. Chem. Phys., 24, 9515–9531, https://doi.org/10.5194/acp-24-9515-2024, https://doi.org/10.5194/acp-24-9515-2024, 2024
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Different sources of airborne particles in the atmospheres of four European cities were distinguished by recognising their particle size distributions using a statistical procedure, positive matrix factorisation. The various sources responded differently to the changes in emissions associated with COVID-19 lockdowns, and the reasons are investigated. While traffic emissions generally decreased, particles formed from reactions of atmospheric gases decreased in some cities but increased in others.
Amy H. Peace, Ying Chen, George Jordan, Daniel G. Partridge, Florent Malavelle, Eliza Duncan, and Jim M. Haywood
Atmos. Chem. Phys., 24, 9533–9553, https://doi.org/10.5194/acp-24-9533-2024, https://doi.org/10.5194/acp-24-9533-2024, 2024
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Natural aerosols from volcanic eruptions can help us understand how anthropogenic aerosols modify climate. We use observations and model simulations of the 2014–2015 Holuhraun eruption plume to examine aerosol–cloud interactions in September 2014. We find a shift to clouds with smaller, more numerous cloud droplets in the first 2 weeks of the eruption. In the third week, the background meteorology and previous conditions experienced by air masses modulate the aerosol perturbation to clouds.
Hua Lu, Min Xie, Bingliang Zhuang, Danyang Ma, Bojun Liu, Yangzhihao Zhan, Tijian Wang, Shu Li, Mengmeng Li, and Kuanguang Zhu
Atmos. Chem. Phys., 24, 8963–8982, https://doi.org/10.5194/acp-24-8963-2024, https://doi.org/10.5194/acp-24-8963-2024, 2024
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To identify cloud, aerosol, and planetary boundary layer (PBL) interactions from an air quality perspective, we summarized two pollution patterns characterized by denser liquid cloud and by obvious cloud radiation interaction (CRI). Numerical simulation experiments showed CRI could cause a 50 % reduction in aerosol radiation interaction (ARI) under a low-trough system. The results emphasized the nonnegligible role of CRI and its inhibition of ARI under wet and cloudy pollution synoptic patterns.
Emilie Fons, Ann Kristin Naumann, David Neubauer, Theresa Lang, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 8653–8675, https://doi.org/10.5194/acp-24-8653-2024, https://doi.org/10.5194/acp-24-8653-2024, 2024
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Aerosols can modify the liquid water path (LWP) of stratocumulus and, thus, their radiative effect. We compare storm-resolving model and satellite data that disagree on the sign of LWP adjustments and diagnose this discrepancy with causal inference. We find that strong precipitation, the absence of wet scavenging, and cloud deepening under a weak inversion contribute to positive LWP adjustments to aerosols in the model, despite weak negative effects from cloud-top entrainment enhancement.
Muhammed Irfan, Thomas Kühn, Taina Yli-Juuti, Anton Laakso, Eemeli Holopainen, Douglas R. Worsnop, Annele Virtanen, and Harri Kokkola
Atmos. Chem. Phys., 24, 8489–8506, https://doi.org/10.5194/acp-24-8489-2024, https://doi.org/10.5194/acp-24-8489-2024, 2024
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The study examines how the volatility of semi-volatile organic compounds affects secondary organic aerosol (SOA) formation and climate. Our simulations show that uncertainties in these volatilities influence aerosol mass and climate impacts. Accurate representation of these compounds in climate models is crucial for predicting global climate patterns.
Alkiviadis Kalisoras, Aristeidis K. Georgoulias, Dimitris Akritidis, Robert J. Allen, Vaishali Naik, Chaincy Kuo, Sophie Szopa, Pierre Nabat, Dirk Olivié, Twan van Noije, Philippe Le Sager, David Neubauer, Naga Oshima, Jane Mulcahy, Larry W. Horowitz, and Prodromos Zanis
Atmos. Chem. Phys., 24, 7837–7872, https://doi.org/10.5194/acp-24-7837-2024, https://doi.org/10.5194/acp-24-7837-2024, 2024
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Effective radiative forcing (ERF) is a metric for estimating how human activities and natural agents change the energy flow into and out of the Earth’s climate system. We investigate the anthropogenic aerosol ERF, and we estimate the contribution of individual processes to the total ERF using simulations from Earth system models within the Coupled Model Intercomparison Project Phase 6 (CMIP6). Our findings highlight that aerosol–cloud interactions drive ERF variability during the last 150 years.
Ryan Schmedding and Andreas Zuend
EGUsphere, https://doi.org/10.5194/egusphere-2024-1690, https://doi.org/10.5194/egusphere-2024-1690, 2024
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Four different approaches for computing the interfacial tension between liquid phases in aerosol particles were tested for particles with diameters from 10 nm to more than 5 μm. Antonov's rule led to the strongest reductions in the onset relative humidity of liquid–liquid phase separation and reproduced measured interfacial tensions for highly immiscible systems. A modified form of the Butler equation was able to best reproduce measured interfacial tensions in more miscible systems.
Qianqian Song, Paul Ginoux, María Gonçalves Ageitos, Ron L. Miller, Vincenzo Obiso, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 7421–7446, https://doi.org/10.5194/acp-24-7421-2024, https://doi.org/10.5194/acp-24-7421-2024, 2024
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We implement and simulate the distribution of eight dust minerals in the GFDL AM4.0 model. We found that resolving the eight minerals reduces dust absorption compared to the homogeneous dust used in the standard GFDL AM4.0 model that assumes a globally uniform hematite content of 2.7 % by volume. Resolving dust mineralogy results in significant impacts on radiation, land surface temperature, surface winds, and precipitation over North Africa in summer.
Mingxu Liu, Hitoshi Matsui, Douglas Hamilton, Sagar Rathod, Kara Lamb, and Natalie Mahowald
EGUsphere, https://doi.org/10.5194/egusphere-2024-1454, https://doi.org/10.5194/egusphere-2024-1454, 2024
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Atmospheric aerosol deposition provides iron to promote marine primary production, yet its amount remains highly uncertain. This study demonstrates that iron-containing particle size at emission is a critical factor in regulating their input to open oceans by performing global aerosol simulations. Further observational constraints on this are needed to reduce modelling uncertainties.
Senyi Kong, Zheng Wang, and Lei Bi
Atmos. Chem. Phys., 24, 6911–6935, https://doi.org/10.5194/acp-24-6911-2024, https://doi.org/10.5194/acp-24-6911-2024, 2024
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The retrieval of refractive indices of dust aerosols from laboratory optical measurements is commonly done assuming spherical particles. This paper aims to investigate the uncertainties in the shortwave refractive indices and corresponding optical properties by considering non-spherical and inhomogeneous models for dust samples. The study emphasizes the significance of using non-spherical models for simulating dust aerosols.
Wenxuan Hua, Sijia Lou, Xin Huang, Lian Xue, Ke Ding, Zilin Wang, and Aijun Ding
Atmos. Chem. Phys., 24, 6787–6807, https://doi.org/10.5194/acp-24-6787-2024, https://doi.org/10.5194/acp-24-6787-2024, 2024
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In this study, we diagnose uncertainties in carbon monoxide and organic carbon emissions from four inventories for seven major wildfire-prone regions. Uncertainties in vegetation classification methods, fire detection products, and cloud obscuration effects lead to bias in these biomass burning (BB) emission inventories. By comparing simulations with measurements, we provide certain inventory recommendations. Our study has implications for reducing uncertainties in emissions in further studies.
Léo Clauzel, Sandrine Anquetin, Christophe Lavaysse, Gilles Bergametti, Christel Bouet, Guillaume Siour, Rémy Lapere, Béatrice Marticorena, and Jennie Thomas
EGUsphere, https://doi.org/10.5194/egusphere-2024-1604, https://doi.org/10.5194/egusphere-2024-1604, 2024
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Solar energy production in West Africa is set to rise, needing accurate solar radiation estimates, which is affected by desert dust. This work analyses a March 2021 dust event using a modelling strategy incorporating desert dust. Results show that considering desert dust cut errors in solar radiation estimates by 75 % and reduces surface solar radiation by 18 %. This highlights the importance of incorporating dust aerosols into solar forecasting for better accuracy.
Chandrakala Bharali, Mary Barth, Rajesh Kumar, Sachin D. Ghude, Vinayak Sinha, and Baerbel Sinha
Atmos. Chem. Phys., 24, 6635–6662, https://doi.org/10.5194/acp-24-6635-2024, https://doi.org/10.5194/acp-24-6635-2024, 2024
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This study examines the role of atmospheric aerosols in winter fog over the Indo-Gangetic Plains of India using WRF-Chem. The increase in RH with aerosol–radiation feedback (ARF) is found to be important for fog formation as it promotes the growth of aerosols in the polluted environment. Aqueous-phase chemistry in the fog increases PM2.5 concentration, further affecting ARF. ARF and aqueous-phase chemistry affect the fog intensity and the timing of fog formation by ~1–2 h.
Wenxin Zhao, Yu Zhao, Yu Zheng, Dong Chen, Jinyuan Xin, Kaitao Li, Huizheng Che, Zhengqiang Li, Mingrui Ma, and Yun Hang
Atmos. Chem. Phys., 24, 6593–6612, https://doi.org/10.5194/acp-24-6593-2024, https://doi.org/10.5194/acp-24-6593-2024, 2024
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We evaluate the long-term (2000–2020) variabilities of aerosol absorption optical depth, black carbon emissions, and associated health risks in China with an integrated framework that combines multiple observations and modeling techniques. We demonstrate the remarkable emission abatement resulting from the implementation of national pollution controls and show how human activities affected the emissions with a spatiotemporal heterogeneity, thus supporting differentiated policy-making by region.
Peng Xian, Jeffrey S. Reid, Melanie Ades, Angela Benedetti, Peter R. Colarco, Arlindo da Silva, Tom F. Eck, Johannes Flemming, Edward J. Hyer, Zak Kipling, Samuel Rémy, Tsuyoshi Thomas Sekiyama, Taichu Tanaka, Keiya Yumimoto, and Jianglong Zhang
Atmos. Chem. Phys., 24, 6385–6411, https://doi.org/10.5194/acp-24-6385-2024, https://doi.org/10.5194/acp-24-6385-2024, 2024
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The study compares and evaluates monthly AOD of four reanalyses (RA) and their consensus (i.e., ensemble mean). The basic verification characteristics of these RA versus both AERONET and MODIS retrievals are presented. The study discusses the strength of each RA and identifies regions where divergence and challenges are prominent. The RA consensus usually performs very well on a global scale in terms of how well it matches the observational data, making it a good choice for various applications.
Roger Teoh, Zebediah Engberg, Ulrich Schumann, Christiane Voigt, Marc Shapiro, Susanne Rohs, and Marc E. J. Stettler
Atmos. Chem. Phys., 24, 6071–6093, https://doi.org/10.5194/acp-24-6071-2024, https://doi.org/10.5194/acp-24-6071-2024, 2024
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The radiative forcing (RF) due to aviation contrails is comparable to that caused by CO2. We estimate that global contrail net RF in 2019 was 62.1 mW m−2. This is ~1/2 the previous best estimate for 2018. Contrail RF varies regionally due to differences in conditions required for persistent contrails. COVID-19 reduced contrail RF by 54% in 2020 relative to 2019. Globally, 2 % of all flights account for 80 % of the annual contrail energy forcing, suggesting a opportunity to mitigate contrail RF.
Ragnhild Bieltvedt Skeie, Rachael Byrom, Øivind Hodnebrog, Caroline Jouan, and Gunnar Myhre
EGUsphere, https://doi.org/10.5194/egusphere-2024-1394, https://doi.org/10.5194/egusphere-2024-1394, 2024
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In 2020 new regulations by the International Maritime Organization of sulphur emissions came into force that reduced emissions of SO2 from the shipping sector by approximately 80 %. In this study, we use multiple models to calculate by how much the Earth energy balance changed due to the emission reduction, the so called effective radiative forcing. The calculated effective radiative forcing is weak, comparable to the effect of the increase in CO2 over the last two to three years.
Haotian Zu, Biwu Chu, Yiqun Lu, Ling Liu, and Xiuhui Zhang
Atmos. Chem. Phys., 24, 5823–5835, https://doi.org/10.5194/acp-24-5823-2024, https://doi.org/10.5194/acp-24-5823-2024, 2024
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The nucleation of iodic acid (HIO3) and iodous acid (HIO2) was proven to be critical in marine areas. However, HIO3–HIO2 nucleation cannot effectively derive the rapid nucleation in some polluted coasts. We find a significant enhancement of dimethylamine (DMA) on the HIO3–HIO2 nucleation in marine and polar regions with abundant DMA sources, which may establish reasonable connections between the HIO3–HIO2 nucleation and the rapid formation of new particles in polluted marine and polar regions.
Junghwa Lee, Patric Seifert, Tempei Hashino, Maximilian Maahn, Fabian Senf, and Oswald Knoth
Atmos. Chem. Phys., 24, 5737–5756, https://doi.org/10.5194/acp-24-5737-2024, https://doi.org/10.5194/acp-24-5737-2024, 2024
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Spectral bin model simulations of an idealized supercooled stratiform cloud were performed with the AMPS model for variable CCN and INP concentrations. We performed radar forward simulations with PAMTRA to transfer the simulations into radar observational space. The derived radar reflectivity factors were compared to observational studies of stratiform mixed-phase clouds. These studies report a similar response of the radar reflectivity factor to aerosol perturbations as we found in our study.
Masaru Yoshioka, Daniel P. Grosvenor, Ben B. B. Booth, Colin P. Morice, and Kenneth S. Carslaw
EGUsphere, https://doi.org/10.5194/egusphere-2024-1428, https://doi.org/10.5194/egusphere-2024-1428, 2024
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Sulfur emissions from shipping has been reduced by about 80 % as a result of the new regulation introduced in 2020. This has reduced aerosol in the atmosphere and its cooling effect through interactions with clouds. As a result, our coupled climate model simulations predict a global warming of 0.04 K averaged over three decades, potentially surpassing the Paris target of 1.5 K or contributing to recent temperature spikes, particularly notable in the Arctic with a mean warming of 0.15 K.
Basudev Swain, Marco Vountas, Aishwarya Singh, Nidhi L. Anchan, Adrien Deroubaix, Luca Lelli, Yanick Ziegler, Sachin S. Gunthe, Hartmut Bösch, and John P. Burrows
Atmos. Chem. Phys., 24, 5671–5693, https://doi.org/10.5194/acp-24-5671-2024, https://doi.org/10.5194/acp-24-5671-2024, 2024
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Arctic amplification (AA) accelerates the warming of the central Arctic cryosphere and affects aerosol dynamics. Limited observations hinder a comprehensive analysis. This study uses AEROSNOW aerosol optical density (AOD) data and GEOS-Chem simulations to assess AOD variability. Discrepancies highlight the need for improved observational integration into models to refine our understanding of aerosol effects on cloud microphysics, ice nucleation, and radiative forcing under evolving AA.
Vincenzo Obiso, María Gonçalves Ageitos, Carlos Pérez García-Pando, Jan P. Perlwitz, Gregory L. Schuster, Susanne E. Bauer, Claudia Di Biagio, Paola Formenti, Kostas Tsigaridis, and Ron L. Miller
Atmos. Chem. Phys., 24, 5337–5367, https://doi.org/10.5194/acp-24-5337-2024, https://doi.org/10.5194/acp-24-5337-2024, 2024
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We calculate the dust direct radiative effect (DRE) in an Earth system model accounting for regionally varying soil mineralogy through a new observationally constrained method. Linking dust absorption at solar wavelengths to the varying amount of specific minerals (i.e., iron oxides) improves the modeled range of dust single scattering albedo compared to observations and increases the global cooling by dust. Our results may contribute to improved estimates of the dust DRE and its climate impact.
Charlotte M. Beall, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Adam Varble, Kentaroh Suzuki, and Takuro Michibata
Atmos. Chem. Phys., 24, 5287–5302, https://doi.org/10.5194/acp-24-5287-2024, https://doi.org/10.5194/acp-24-5287-2024, 2024
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Single-layer warm liquid clouds cover nearly one-third of the Earth's surface, and uncertainties regarding the impact of aerosols on their radiative properties pose a significant challenge to climate prediction. Here, we demonstrate how satellite observations can be used to constrain Earth system model estimates of the radiative forcing from the interactions of aerosols with clouds due to warm rain processes.
Xiaoli Wei, Qian Cui, Leiming Ma, Feng Zhang, Wenwen Li, and Peng Liu
Atmos. Chem. Phys., 24, 5025–5045, https://doi.org/10.5194/acp-24-5025-2024, https://doi.org/10.5194/acp-24-5025-2024, 2024
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A new aerosol-type classification algorithm has been proposed. It includes an optical database built by Mie scattering and a complex refractive index working as a baseline to identify different aerosol types. The new algorithm shows high accuracy and efficiency. Hence, a global map of aerosol types was generated to characterize aerosol types across the five continents. It will help improve the accuracy of aerosol inversion and determine the sources of aerosol pollution.
Zhiqiang Zhang, Ying Li, Haiyan Ran, Junling An, Yu Qu, Wei Zhou, Weiqi Xu, Weiwei Hu, Hongbin Xie, Zifa Wang, Yele Sun, and Manabu Shiraiwa
Atmos. Chem. Phys., 24, 4809–4826, https://doi.org/10.5194/acp-24-4809-2024, https://doi.org/10.5194/acp-24-4809-2024, 2024
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Secondary organic aerosols (SOAs) can exist in liquid, semi-solid, or amorphous solid states, which are rarely accounted for in current chemical transport models. We predict the phase state of SOA particles over China and find that in northwestern China SOA particles are mostly highly viscous or glassy solid. Our results indicate that the particle phase state should be considered in SOA formation in chemical transport models for more accurate prediction of SOA mass concentrations.
Alejandro Baró Pérez, Michael S. Diamond, Frida A.-M. Bender, Abhay Devasthale, Matthias Schwarz, Julien Savre, Juha Tonttila, Harri Kokkola, Hyunho Lee, David Painemal, and Annica M. L. Ekman
Atmos. Chem. Phys., 24, 4591–4610, https://doi.org/10.5194/acp-24-4591-2024, https://doi.org/10.5194/acp-24-4591-2024, 2024
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We use a numerical model to study interactions between humid light-absorbing aerosol plumes, clouds, and radiation over the southeast Atlantic. We find that the warming produced by the aerosols reduces cloud cover, especially in highly polluted situations. Aerosol impacts on drizzle play a minor role. However, aerosol effects on cloud reflectivity and moisture-induced changes in cloud cover dominate the climatic response and lead to an overall cooling by the biomass burning plumes.
Danny M. Leung, Jasper F. Kok, Longlei Li, David M. Lawrence, Natalie M. Mahowald, Simone Tilmes, and Erik Kluzek
EGUsphere, https://doi.org/10.5194/egusphere-2024-1124, https://doi.org/10.5194/egusphere-2024-1124, 2024
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This study derives a desert dust emission dataset for 1841–2000, by employing a combination of observed dust records from sedimentary cores as well as reanalyzed global dust cycle constraints. We evaluate the ability of global models to replicate the observed historical dust variability by using the emission dataset to force a historical simulation in an Earth system model. We show that prescribing our emissions forces the model to match better against observations than other mechanistic models.
Sampa Das, Peter R. Colarco, Huisheng Bian, and Santiago Gassó
Atmos. Chem. Phys., 24, 4421–4449, https://doi.org/10.5194/acp-24-4421-2024, https://doi.org/10.5194/acp-24-4421-2024, 2024
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The smoke aerosols emitted from vegetation burning can alter the regional energy budget via multiple pathways. We utilized detailed observations from the NASA ORACLES airborne campaign based in Namibia during September 2016 to improve the representation of smoke aerosol properties and lifetimes in our GEOS Earth system model. The improved model simulations are for the first time able to capture the observed changes in the smoke absorption during long-range plume transport.
Emilio Cuevas-Agulló, David Barriopedro, Rosa Delia García, Silvia Alonso-Pérez, Juan Jesús González-Alemán, Ernest Werner, David Suárez, Juan José Bustos, Gerardo García-Castrillo, Omaira García, África Barreto, and Sara Basart
Atmos. Chem. Phys., 24, 4083–4104, https://doi.org/10.5194/acp-24-4083-2024, https://doi.org/10.5194/acp-24-4083-2024, 2024
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During February–March (FM) 2020–2022, unusually intense dust storms from northern Africa hit the western Euro-Mediterranean (WEM). Using dust products from satellites and atmospheric reanalysis for 2003–2022, results show that cut-off lows and European blocking are key drivers of FM dust intrusions over the WEM. A higher frequency of cut-off lows associated with subtropical ridges is observed in the late 2020–2022 period.
Yahui Che, Bofu Yu, and Katherine Bracco
Atmos. Chem. Phys., 24, 4105–4128, https://doi.org/10.5194/acp-24-4105-2024, https://doi.org/10.5194/acp-24-4105-2024, 2024
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Dust events occur more frequently during the Austral spring and summer in dust regions, including central Australia, the southwest of Western Australia, and the northern and southern regions of eastern Australia using remote sensing and reanalysis datasets. High-concentration dust is distributed around central Australia and in the downwind northern and southern Australia. Typically, around 50 % of the dust lifted settles on Australian land, with the remaining half being deposited in the ocean.
Jonathan Elsey, Nicolas Bellouin, and Claire Ryder
Atmos. Chem. Phys., 24, 4065–4081, https://doi.org/10.5194/acp-24-4065-2024, https://doi.org/10.5194/acp-24-4065-2024, 2024
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Aerosols influence the Earth's energy balance. The uncertainty in this radiative forcing is large depending partly on uncertainty in measurements of aerosol optical properties. We have developed a freely available new framework of millions of radiative transfer simulations spanning aerosol uncertainty and assess the impact on radiative forcing uncertainty. We find that reducing these uncertainties would reduce radiative forcing uncertainty, but non-aerosol uncertainties must also be considered.
Jing Li, Nan Wu, Biwu Chu, An Ning, and Xiuhui Zhang
Atmos. Chem. Phys., 24, 3989–4000, https://doi.org/10.5194/acp-24-3989-2024, https://doi.org/10.5194/acp-24-3989-2024, 2024
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Iodic acid (HIO3) nucleates with iodous acid (HIO2) efficiently in marine areas; however, whether methanesulfonic acid (MSA) can synergistically participate in the HIO3–HIO2-based nucleation is unclear. We provide molecular-level evidence that MSA can efficiently promote the formation of HIO3–HIO2-based clusters using a theoretical approach. The proposed MSA-enhanced iodine nucleation mechanism may help us to deeply understand marine new particle formation events with bursts of iodine particles.
Hao Wang, Xiaohong Liu, Chenglai Wu, and Guangxing Lin
Atmos. Chem. Phys., 24, 3309–3328, https://doi.org/10.5194/acp-24-3309-2024, https://doi.org/10.5194/acp-24-3309-2024, 2024
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We quantified different global- and regional-scale drivers of biogenic volatile organic compound (BVOC) emission trends over the past 20 years. The results show that global greening trends significantly boost BVOC emissions and deforestation reduces BVOC emissions in South America and Southeast Asia. Elevated temperature in Europe and increased soil moisture in East and South Asia enhance BVOC emissions. The results deepen our understanding of long-term BVOC emission trends in hotspots.
Christof G. Beer, Johannes Hendricks, and Mattia Righi
Atmos. Chem. Phys., 24, 3217–3240, https://doi.org/10.5194/acp-24-3217-2024, https://doi.org/10.5194/acp-24-3217-2024, 2024
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Ice-nucleating particles (INPs) have important influences on cirrus clouds and the climate system; however, the understanding of their global impacts is still uncertain. We perform numerical simulations with a global aerosol–climate model to analyse INP-induced cirrus changes and the resulting climate impacts. We evaluate various sources of uncertainties, e.g. the ice-nucleating ability of INPs and the role of model dynamics, and provide a new estimate for the global INP–cirrus effect.
Jiawei Li, Zhiwei Han, Pingqing Fu, Xiaohong Yao, and Mingjie Liang
Atmos. Chem. Phys., 24, 3129–3161, https://doi.org/10.5194/acp-24-3129-2024, https://doi.org/10.5194/acp-24-3129-2024, 2024
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Organic aerosols of marine origin are important for aerosol climatic effects but are poorly understood. For the first time, an online coupled regional chemistry–climate model is applied to explore the characteristics of emission, distribution, and direct and indirect radiative effects of marine organic aerosols over the western Pacific, which reveals an important role of marine organic aerosols in perturbing cloud and radiation and promotes understanding of global aerosol climatic impact.
Yawen Liu, Yun Qian, Philip J. Rasch, Kai Zhang, Lai-yung Ruby Leung, Yuhang Wang, Minghuai Wang, Hailong Wang, Xin Huang, and Xiu-Qun Yang
Atmos. Chem. Phys., 24, 3115–3128, https://doi.org/10.5194/acp-24-3115-2024, https://doi.org/10.5194/acp-24-3115-2024, 2024
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Fire management has long been a challenge. Here we report that spring-peak fire activity over southern Mexico and Central America (SMCA) has a distinct quasi-biennial signal by measuring multiple fire metrics. This signal is initially driven by quasi-biennial variability in precipitation and is further amplified by positive feedback of fire–precipitation interaction at short timescales. This work highlights the importance of fire–climate interactions in shaping fires on an interannual scale.
Xu Feng, Loretta J. Mickley, Michelle L. Bell, Tianjia Liu, Jenny A. Fisher, and Maria Val Martin
Atmos. Chem. Phys., 24, 2985–3007, https://doi.org/10.5194/acp-24-2985-2024, https://doi.org/10.5194/acp-24-2985-2024, 2024
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During severe wildfire seasons, smoke can have a significant impact on air quality in Australia. Our study demonstrates that characterization of the smoke plume injection fractions greatly affects estimates of surface smoke PM2.5. Using the plume behavior predicted by the machine learning method leads to the best model agreement with observed surface PM2.5 in key cities across Australia, with smoke PM2.5 accounting for 5 %–52 % of total PM2.5 on average during fire seasons from 2009 to 2020.
Shiyi Lai, Ximeng Qi, Xin Huang, Sijia Lou, Xuguang Chi, Liangduo Chen, Chong Liu, Yuliang Liu, Chao Yan, Mengmeng Li, Tengyu Liu, Wei Nie, Veli-Matti Kerminen, Tuukka Petäjä, Markku Kulmala, and Aijun Ding
Atmos. Chem. Phys., 24, 2535–2553, https://doi.org/10.5194/acp-24-2535-2024, https://doi.org/10.5194/acp-24-2535-2024, 2024
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By combining in situ measurements and chemical transport modeling, this study investigates new particle formation (NPF) on the southeastern Tibetan Plateau. We found that the NPF was driven by the presence of biogenic gases and the transport of anthropogenic precursors. The NPF was vertically heterogeneous and shaped by the vertical mixing. This study highlights the importance of anthropogenic–biogenic interactions and meteorological dynamics in NPF in this climate-sensitive region.
Adriana Rocha-Lima, Peter R. Colarco, Anton S. Darmenov, Edward P. Nowottnick, Arlindo M. da Silva, and Luke D. Oman
Atmos. Chem. Phys., 24, 2443–2464, https://doi.org/10.5194/acp-24-2443-2024, https://doi.org/10.5194/acp-24-2443-2024, 2024
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Observations show an increasing aerosol optical depth trend in the Middle East between 2003–2012. We evaluate the NASA Goddard Earth Observing System (GEOS) model's ability to capture these trends and examine the meteorological and surface parameters driving dust emissions. Our results highlight the importance of data assimilation for long-term trends of atmospheric aerosols and support the hypothesis that vegetation cover loss may have contributed to increasing dust emissions in the period.
Cited articles
Ångström, A.: On the atmospheric transmission of sun radiation and on dust in the air, Geogr. Ann., 11, 156–166, 1929.
Arola, A., Eck, T. F., Huttunen, J., Lehtinen, K. E. J., Lindfors, A. V., Myhre, G., Smirnov, A., Tripathi, S. N., and Yu, H.: Influence of observed diurnal cycles of aerosol optical depth on aerosol direct radiative effect, Atmos. Chem. Phys., 13, 7895–7901, https://doi.org/10.5194/acp-13-7895-2013, 2013.
Awang, M. B., Jaafar, A. B., Abdullah, A. M., Ismail, M. B., Hassan, M. N., Abdullah, R., Johan, S., and Noor, H.: Air quality in Malaysia: impacts, management issues and future challenges, Respirology, 5, 183–196, 2000.
Barladeanu, R., Stefan, S., and Radulescu, R.: Correlation between the particulate matter (PM10) mass concentrations and aerosol optical depth in Bucharest, Romania, Romanian Reports in Physics, 64, 1085–1096, 2012.
Bäumer, D., Vogel, B., Versick, S., Rinke, R., Möhler, O., and Schnaiter, M.: Relationship of visibility, aerosol optical thickness and aerosol size distribution in an ageing air mass over South-West Germany, Atmos. Environ., 42, 989–998, https://doi.org/10.1016/j.atmosenv.2007.10.017, 2008.
Bougiatioti, A., Stavroulas, I., Kostenidou, E., Zarmpas, P., Theodosi, C., Kouvarakis, G., Canonaco, F., Prévôt, A. S. H., Nenes, A., Pandis, S. N., and Mihalopoulos, N.: Processing of biomass-burning aerosol in the eastern Mediterranean during summertime, Atmos. Chem. Phys., 14, 4793–4807, https://doi.org/10.5194/acp-14-4793-2014, 2014.
Campbell, J. R., Reid, J. S., Westphal, D. L., Zhang, J., Tackett, J. L., Chew, B. N., Welton, E. J., Shimizu, A., Sugimoto, N., Aoki, K., and Winker, D. M.: Characterizing the vertical profile of aerosol particle extinction and linear depolarization over Southeast Asia and the Maritime Continent: The 2007–2009 view from CALIOP, Atmos. Res., 122, 520–543, https://doi.org/10.1016/j.atmosres.2012.05.007, 2013.
Chen, B. B., Sverdlik, L. G., Imashev, S. A., Solomon, P. A., Lantz, J., Schauer, J. J., Shafer, M. M., Artamonova, M. S., and Carmichael, G.: Empirical relationship between particulate matter and aerosol optical depth over Northern Tien-Shan, Central Asia, Air Qual. Atmos. Health, 6, 385–396, 2013.
Chew, B. N., Campbell, J. R., Reid, J. S., Giles, D. M., Welton, E. J., Salinas, S. V., and Liew, S. C.: Tropical cirrus cloud contamination in sun photometer data, Atmos. Environ., 45, 6724–6731, 2011.
Chew, B. N., Campbell, J. R., Salinas, S. V., Chang, C. W., Reid, J. S., Welton, E. J., Holben, B. N., and Liew, S. C.: Aerosol particle vertical distributions and optical properties over Singapore, Atmos. Environ., 79, 599–613, 2013.
Cordero, L., Wu, Y., Gross, B. M., and Moshary, F.: Use of passive and active ground and satellite remote sensing to monitor fine particulate pollutants on regional scales, in: Advanced Environmental, Chemical, and Biological Sensing Technologies IX, Baltimore, MD, 2012.
de Meij, A., Pozzer, A., Pringle, K. J., Tost, H., and Lelieveld, J.: EMAC model evaluation and analysis of atmospheric aerosol properties and distribution with a focus on the Mediterranean region, Atmos. Res., 114–115, 38–69, 2012.
DOE: A Guide to Air Pollutant Index in Malaysia (API), 3rd Edn., D. O. Environment, Ed., Kuala Lumpur, Malaysia, 1–20, 1997.
DOE: Pollution sources inventory, in: Malaysia Environment Quality Report 2010, ch. 5, Department of Environment, Petaling Jaya, Malaysia, 2010.
Draxler, R. R. and Hess, G. D.: An overview of the HYSPLIT_4 modelling system for trajectories, dispersion and deposition, Aust. Meteorol. Mag., 47, 295–308, 1998.
Eck, T. F., Holben, B. N., Reid, J. S., Dubovik, O., Smirnov, A., O'Neill, N. T., Slutsker, I., and Kinne, S.: Wavelength dependence of the optical depth of biomass burning, urban, and desert dust aerosols, J. Geophys. Res.-Atmos., 104, 31333–31349, 1999.
Engling, G., He, J., Betha, R., and Balasubramanian, R.: Assessing the regional impact of indonesian biomass burning emissions based on organic molecular tracers and chemical mass balance modeling, Atmos. Chem. Phys., 14, 8043–8054, https://doi.org/10.5194/acp-14-8043-2014, 2014.
Fan, X., Chen, H., and Xia, X. A.: Progress in Observation Studies of Atmospheric Aerosol Radiative Properties in China, Chinese J. Atmos. Sci., 37, 477–498, https://doi.org/10.3878/j.issn.1006-9895.2012.12316, 2013.
Fernald, F. G.: Analysis of atmospheric lidar observations: some comments, Appl. Optics, 23, 652–653, 1984.
Field, R. D., van der Werf, G. R., and Shen, S. S. P.: Human amplification of drought-induced biomass burning in Indonesia since 1960, Nat. Geosci., 2, 185–188, 2009.
Gao, J. and Zha, Y.: Meteorological influence on predicting air pollution from MODIS-derived aerosol optical thickness: a case study in Nanjing, China, Remote Sens., 2, 2136–2147, 2010.
Gerasopoulos, E., Andreae, M. O., Zerefos, C. S., Andreae, T. W., Balis, D., Formenti, P., Merlet, P., Amiridis, V., and Papastefanou, C.: Climatological aspects of aerosol optical properties in Northern Greece, Atmos. Chem. Phys., 3, 2025–2041, https://doi.org/10.5194/acp-3-2025-2003, 2003.
Gupta, P., Khan, M. N., da Silva, A., and Patadia, F.: MODIS aerosol optical depth observations over urban areas in Pakistan: quantity and quality of the data for air quality monitoring, Atmos. Pollut. Res., 4, 43–52, 2013.
Hansen, J., Sato, M., and Ruedy, R.: Radiative forcing and climate response, J. Geophys. Res.-Atmos., 102, 6831–6864, https://doi.org/10.1029/96jd03436, 1997.
He, Q. S., Li, C. C., Mao, J. T., Lau, A. K. H., and Li, P. R.: A study on the aerosol extinction-to-backscatter ratio with combination of micro-pulse LIDAR and MODIS over Hong Kong, Atmos. Chem. Phys., 6, 3243–3256, https://doi.org/10.5194/acp-6-3243-2006, 2006.
Holben, B. N., Eck, T. F., Slutsker, I., Tanré, D., Buis, J. P., Setzer, A., Vermote, E., Reagan, J. A., Kaufman, Y. J., Nakajima, T., Lavenu, F., Jankowiak, I., and Smirnov, A.: AERONET – a federated instrument network and data archive for aerosol characterization, Remote Sens. Environ., 66, 1–16, https://doi.org/10.1016/s0034-4257(98)00031-5, 1998.
Holben, B. N., Tanré, D., Smirnov, A., Eck, T. F., Slutsker, I., Abuhassan, N., Newcomb, W. W., Schafer, J. S., Chatenet, B., Lavenu, F., Kaufman, Y. J., Vande Castle, J., Setzer, A., Markham, B., Clark, D., Frouin, R., Halthore, R., Karneli, A., O'Neill, N. T., Pietras, C., Pinker, R. T., Voss, K., and Zibordi, G.: An emerging ground-based aerosol climatology: aerosol optical depth from AERONET, J. Geophys. Res.-Atmos., 106, 12067–12097, 2001.
Horvath, H.: Estimation of the average visibility in Central Europe, Atmos. Environ., 29, 241–246, https://doi.org/10.1016/1352-2310(94)00236-e, 1995.
Hyer, E. J. and Chew, B. N.: Aerosol transport model evaluation of an extreme smoke episode in Southeast Asia, Atmos. Environ., 44, 1422–1427, https://doi.org/10.1016/j.atmosenv.2010.01.043, 2010.
Ichoku, C., Kaufman, Y. J., Remer, L. A., and Levy, R.: Global aerosol remote sensing from MODIS, Adv. Space Res., 34, 820–827, https://doi.org/10.1016/j.asr.2003.07.071, 2004.
IPCC: Climate Change 2007: The Physical Science Basis: Contribution of Working Group I to the Fourth Assessment Report of the Intergovernmental Panel on Climate Change, Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, 2007.
IPCC: Climate Change 2013: The Physical Science Basis: Contribution of Working Group I to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change, Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, 2013.
Jalal, K. A., Asmat, A., and Ahmad, N.: Retrievals of aerosol optical depth and angstrom exponent for identification of aerosols at Kuching, Sarawak, Trans Tech Publications Inc., Hohhot, China, 5734–5737, 2012.
Kaskaoutis, D. G., Kambezidis, H. D., Hatzianastassiou, N., Kosmopoulos, P. G., and Badarinath, K. V. S.: Aerosol climatology: on the discrimination of aerosol types over four AERONET sites, Atmos. Chem. Phys. Discuss., 7, 6357–6411, https://doi.org/10.5194/acpd-7-6357-2007, 2007.
Kaskaoutis, D. G. and Kambezidis, H. D.: The role of aerosol models of the SMARTS code in predicting the spectral direct-beam irradiance in an urban area, Renew. Energ., 33, 1532–1543, https://doi.org/10.1016/j.renene.2007.09.006, 2008.
Kaskaoutis, D. G., Kumar, S., Sharma, D., Singh, R. P., Kharol, S. K., Sharma, M., Singh, A. K., Singh, S., Singh, A., and Singh, D.: Effects of crop residue burning on aerosol properties, plume characteristics, and long-range transport over northern India, J. Geophys. Res.-Atmos., 119, 5424–5444, 2014.
Koschmieder, H.: Theorie der horizontalen Sichtweite, Beitr. Phvs. Freien. Atmos., 12, 33–55, 1924.
Krishna Moorthy, K., Suresh Babu, S., and Satheesh, S. K.: Temporal heterogeneity in aerosol characteristics and the resulting radiative impact at a tropical coastal station – Part 1: Microphysical and optical properties, Ann. Geophys., 25, 2293–2308, https://doi.org/10.5194/angeo-25-2293-2007, 2007.
Kumar, S. and Devara, P. C. S.: A long-term study of aerosol modulation of atmospheric and surface solar heating over Pune, India, Tellus B, 64, 18420, https://doi.org/10.3402/tellusb.v64i0.18420, 2012.
Lee, H. J., Coull, B. A., Bell, M. L., and Koutrakis, P.: Use of satellite-based aerosol optical depth and spatial clustering to predict ambient PM2.5 concentrations, Environ. Res., 118, 8–15, 2012.
Li, F. and Lu, D.: Features of aerosol optical depth with visibility grade over Beijing, Atmos. Environ., 31, 3413–3419, https://doi.org/10.1016/S1352-2310(97)83211-6, 1997.
Lin, J., van Donkelaar, A., Xin, J., Che, H., and Wang, Y.: Clear-sky aerosol optical depth over East China estimated from visibility measurements and chemical transport modeling, Atmos. Environ., 95, 258–267, 2014.
Lin, N.-H., Tsay, S.-C., Maring, H. B., Yen, M.-C., Sheu, G.-R., Wang, S.-H., Chi, K. H., Chuang, M.-T., Ou-Yang, C.-F., Fu, J. S., Reid, J. S., Lee, C.-T., Wang, L.-C., Wang, J.-L., Hsu, C. N., Sayer, A. M., Holben, B. N., Chu, Y.-C., Nguyen, X. A., Sopajaree, K., Chen, S.-J., Cheng, M.-T., Tsuang, B.-J., Tsai, C.-J., Peng, C.-M., Schnell, R. C., Conway, T., Chang, C.-T., Lin, K.-S., Tsai, Y. I., Lee, W.-J., Chang, S.-C., Liu, J.-J., Chiang, W.-L., Huang, S.-J., Lin, T.-H., and Liu, G.-R.: An overview of regional experiments on biomass burning aerosols and related pollutants in Southeast Asia: from BASE-ASIA and the Dongsha Experiment to 7-SEAS, Atmos. Environ., 78, 1–19, https://doi.org/10.1016/j.atmosenv.2013.04.066, 2013.
Lin, N. H., Sayer, A. M., Wang, S. H., Loftus, A. M., Hsiao, T. C., Sheu, G. R., Hsu, N. C., Tsay, S. C., and Chantara, S.: Interactions between biomass-burning aerosols and clouds over Southeast Asia: Current status, challenges, and perspectives, Environ. Pollut., 195, 292–307, https://doi.org/10.1016/j.envpol.2014.06.036, 2014.
Lo, C., Comstock, J. M., and Flynn, C.: An atmospheric radiation measurement value-added product to retrieve optically thin cloud visible optical depth using micropulse lidar, Rep. DOE/SC-ARM/TR-077, 13 pp., 2006.
Lopes, F. J. S., Mariano, G. L., Landulfo, E., and Mariano, E. V. C.: Chapter 9: Impacts of Biomass Burning in the Atmosphere of the Southeastern Region of Brazil Using Remote Sensing Systems, edited by: Abdul-Razzak, H., InTech, 247–272, 2012.
Mahowald, N. M., Ballantine, J. A., Feddema, J., and Ramankutty, N.: Global trends in visibility: implications for dust sources, Atmos. Chem. Phys., 7, 3309–3339, https://doi.org/10.5194/acp-7-3309-2007, 2007.
Mielonen, T., Portin, H., Komppula, M., Leskinen, A., Tamminen, J., Ialongo, I., Hakkarainen, J., Lehtinen, K. E. J., and Arola, A.: Biomass burning aerosols observed in Eastern Finland during the Russian wildfires in summer 2010 – Part 2: Remote sensing, Atmos. Environ., 47, 279–287, 2012.
Mishra, A. K., Srivastava, A., and Jain, V. K.: Spectral dependency of aerosol optical depth and derived aerosol size distribution over Delhi: An implication to pollution source, Sustain. Environ. Res., 23, 113–128, 2013.
Mogo, S., Cachorro, V. E., and de Frutos, A. M.: In situ UV-VIS-NIR absorbing properties of atmospheric aerosol particles: estimates of the imaginary refractive index and comparison with columnar values, J. Environ. Manage., 111, 267–271, 2012.
Müller, D., Lee, K. H., Gasteiger, J., Tesche, M., Weinzierl, B., Kandler, K., Müller, T., Toledano, C., Otto, S., Althausen, D., and Ansmann, A.: Comparison of optical and microphysical properties of pure Saharan mineral dust observed with AERONET Sun photometer, Raman lidar, and in situ instruments during SAMUM 2006, J. Geophys. Res.-Atmos., 117, D07211 https://doi.org/10.1029/2011JD016825, 2012.
Okulov, O., Ohvril, H., and Kivi, R.: Atmospheric precipitable water in Estonia, 1990–2001, Boreal Environ. Res., 7, 291–300, 2002.
Omar, A. H., Won, J.-G., Winker, D. M., Yoon, S.-C., Dubovik, O., and McCormick, M. P.: Development of global aerosol models using cluster analysis of Aerosol Robotic Network (AERONET) measurements, J. Geophys. Res.-Atmos., 110, D10S14, https://doi.org/10.1029/2004jd004874, 2005.
Pace, G., di Sarra, A., Meloni, D., Piacentino, S., and Chamard, P.: Aerosol optical properties at Lampedusa (Central Mediterranean). 1. Influence of transport and identification of different aerosol types, Atmos. Chem. Phys., 6, 697–713, https://doi.org/10.5194/acp-6-697-2006, 2006.
Pandithurai, G., Pinker, R. T., Devara, P. C. S., Takamura, T., and Dani, K. K.: Seasonal asymmetry in diurnal variation of aerosol optical characteristics over Pune, western India, J. Geophys. Res.-Atmos., 112, D08208, https://doi.org/10.1029/2006JD007803, 2007.
Peppler, R. A., Bahrmann, C. P., Barnard, J. C., Laulainen, N. S., Turner, D. D., Campbell, J. R., Hlavka, D. L., Cheng, M. D., Ferrare, R. A., Halthore, R. N., Heilman, L. A., Lin, C. J., Ogren, J. A., Poellot, M. R., Remer, L. A., Spinhirne, J. D., Sassen, K., and Splitt, M. E.: ARM Southern Great Plains site observations of the smoke pall associated with the 1998 Central American Fires, B. Am. Meteorol. Soc., 81, 2563–2591, https://doi.org/10.1175/1520-0477(2000)081< 2563:asgpso> 2.3.co;2, 2000.
Qin, S., Shi, G., Chen, L., Wang, B., Zhao, J., Yu, C., and Yang, S.: Long-term variation of aerosol optical depth in China based on meteorological horizontal visibility observations, Chin. J. Atmos. Sci, 34, 449–456, 2010.
Qiu, J. and Yang, L.: Variation characteristics of atmospheric aerosol optical depths and visibility in North China during 1980–1994, Atmos. Environ., 34, 603–609, 2000.
Ramachandran, S. and Srivastava, R.: Influences of external vs. core-shell mixing on aerosol optical properties at various relative humidities, Environ. Sci., 15, 1070–1077, 2013.
Reid, J. S., Hyer, E. J., Johnson, R. S., Holben, B. N., Yokelson, R. J., Zhang, J., Campbell, J. R., Christopher, S. A., Di Girolamo, L., Giglio, L., Holz, R. E., Kearney, C., Miettinen, J., Reid, E. A., Turk, F. J., Wang, J., Xian, P., Zhao, G., Balasubramanian, R., Chew, B. N., Janjai, S., Lagrosas, N., Lestari, P., Lin, N.-H., Mahmud, M., Nguyen, A. X., Norris, B., Oanh, N. T. K., Oo, M., Salinas, S. V., Welton, E. J., and Liew, S. C.: Observing and understanding the Southeast Asian aerosol system by remote sensing: An initial review and analysis for the Seven Southeast Asian Studies (7SEAS) program, Atmos. Res., 122, 403–468, https://doi.org/10.1016/j.atmosres.2012.06.005, 2013.
Retalis, A., Hadjimitsis, D. G., Michaelides, S., Tymvios, F., Chrysoulakis, N., Clayton, C. R. I., and Themistocleous, K.: Comparison of aerosol optical thickness with in situ visibility data over Cyprus, Nat. Hazards Earth Syst. Sci., 10, 421–428, https://doi.org/10.5194/nhess-10-421-2010, 2010.
Russell, P. B., Bergstrom, R. W., Shinozuka, Y., Clarke, A. D., DeCarlo, P. F., Jimenez, J. L., Livingston, J. M., Redemann, J., Dubovik, O., and Strawa, A.: Absorption Angstrom Exponent in AERONET and related data as an indicator of aerosol composition, Atmos. Chem. Phys., 10, 1155–1169, https://doi.org/10.5194/acp-10-1155-2010, 2010.
Salinas, S. V., Chew, B. N., and Liew, S. C.: Retrievals of aerosol optical depth and Ångström exponent from ground-based Sun-photometer data of Singapore, Appl. Optics, 48, 1473–1484, https://doi.org/10.1364/ao.48.001473, 2009.
Salinas, S. V., Chew, B. N., Miettinen, J., Campbell, J. R., Welton, E. J., Reid, J. S., Yu, L. E., and Liew, S. C.: Physical and optical characteristics of the October 2010 haze event over Singapore: A photometric and lidar analysis, Atmos. Res., 122, 555–570, https://doi.org/10.1016/j.atmosres.2012.05.021, 2013.
Singh, A. and Dey, S.: Influence of aerosol composition on visibility in megacity Delhi, Atmos. Environ., 62, 367–373, 2012.
Smirnov, A., Holben, B. N., Eck, T. F., Dubovik, O., and Slutsker, I.: Cloud-screening and quality control algorithms for the AERONET database, Remote Sens. Environ., 73, 337–349, https://doi.org/10.1016/S0034-4257(00)00109-7, 2000.
Smirnov, A., Holben, B. N., Dubovik, O., O'Neill, N. T., Eck, T. F., Westphal, D. L., Goroch, A. K., Pietras, C., and Slutsker, I.: Atmospheric aerosol optical properties in the Persian Gulf, J. Atmos. Sci., 59, 620–634, https://doi.org/10.1175/1520-0469(2002)059< 0620:aaopit> 2.0.co;2, 2002a.
Smirnov, A., Holben, B. N., Kaufman, Y. J., Dubovik, O., Eck, T. F., Slutsker, I., Pietras, C., and Halthore, R. N.: Optical properties of atmospheric aerosol in maritime environments, J. Atmos. Sci., 59, 501–523, https://doi.org/10.1175/1520-0469(2002)059< 0501:opoaai> 2.0.co;2, 2002b.
Smirnov, A., Holben, B. N., Dubovik, O., Frouin, R., Eck, T. F., and Slutsker, I.: Maritime component in aerosol optical models derived from Aerosol Robotic Network data, J. Geophys. Res.-Atmos., 108, 4033, https://doi.org/10.1029/2002jd002701, 2003.
Smirnov, A., Holben, B. N., Giles, D. M., Slutsker, I., O'Neill, N. T., Eck, T. F., Macke, A., Croot, P., Courcoux, Y., Sakerin, S. M., Smyth, T. J., Zielinski, T., Zibordi, G., Goes, J. I., Harvey, M. J., Quinn, P. K., Nelson, N. B., Radionov, V. F., Duarte, C. M., Losno, R., Sciare, J., Voss, K. J., Kinne, S., Nalli, N. R., Joseph, E., Krishna Moorthy, K., Covert, D. S., Gulev, S. K., Milinevsky, G., Larouche, P., Belanger, S., Horne, E., Chin, M., Remer, L. A., Kahn, R. A., Reid, J. S., Schulz, M., Heald, C. L., Zhang, J., Lapina, K., Kleidman, R. G., Griesfeller, J., Gaitley, B. J., Tan, Q., and Diehl, T. L.: Maritime aerosol network as a component of AERONET – first results and comparison with global aerosol models and satellite retrievals, Atmos. Meas. Tech., 4, 583–597, https://doi.org/10.5194/amt-4-583-2011, 2011.
Song, C., Zaveri, R. A., Alexander, M. L., Thornton, J. A., Madronich, S., Ortega, J. V., Zelenyuk, A., Yu, X.-Y., Laskin, A., and Maughan, D. A.: Effect of hydrophobic primary organic aerosols on secondary organic aerosol formation from ozonolysis of α-pinene, Geophys. Res. Lett., 34, L20803, https://doi.org/10.1029/2007gl030720, 2007.
Srivastava, A. K., Singh, S., Tiwari, S., and Bisht, D. S.: Contribution of anthropogenic aerosols in direct radiative forcing and atmospheric heating rate over Delhi in the Indo-Gangetic Basin, Environ. Sci. Pollut. R., 19, 1144–1158, 2012.
Stone, R. S.: Monitoring aerosol optical depth at Barrow, Alaska and South Pole; historical overview, recent results, and future goals, in: Proceedings of the 9th Workshop Italian Research on Antarctic Atmosphere, 22–24 October 2001, Rome, Italy, 123–144, 2002.
Suresh Babu, S., Krishna Moorthy, K., and Satheesh, S. K.: Temporal heterogeneity in aerosol characteristics and the resulting radiative impacts at a tropical coastal station – Part 2: Direct short wave radiative forcing, Ann. Geophys., 25, 2309–2320, https://doi.org/10.5194/angeo-25-2309-2007, 2007.
Tan, F., Abdullah, K., Lim, H. S., MatJafri, M. Z., Welton, E. J., and Lolli, S.: An initial assessment of ground based lidar backscattered signal in Penang Island, in: IEEE International Conference on Space Science and Communication (IconSpace) 2013, Melaka, Malaysia, 1–3 July 2013, 228–232, 2013.
Tan, F., Lim, H. S., Abdullah, K., Yoon, T. L., Matjafri, M. Z., and Holben, B.: Multiple regression method to determine aerosol optical depth in atmospheric column in Penang, Malaysia, IOP C. Ser. Earth Env., 18, 012081, https://doi.org/10.1088/1755-1315/18/1/012081, 2014a.
Tan, F., Lim, H. S., Abdullah, K., Yoon, T. L., Matjafri, M. Z., and Holben, B.: Manipulating API and AOD data to distinguish transportation of aerosol at high altitude in Penang, Malaysia, IOP C. Ser. Earth Env., 18, 012082, https://doi.org/10.1088/1755-1315/18/1/01208, 2014b.
Tan, F. Y., Hee, W. S., Hwee, S. L., Abdullah, K., Tiem, L. Y., Matjafri, M. Z., Lolli, S., Holben, B., and Welton, E. J.: Variation in daytime troposphereic aerosol via LIDAR and sunphotometer measurements in Penang, Malaysia, AIP Conference Proceedings, 1588, 286–292, https://doi.org/10.1063/1.4866962, 2014c.
Tang, I. N.: Chemical and size effects of hygroscopic aerosols on light scattering coefficients, J. Geophys. Res.-Atmos., 101, 19245–19250, https://doi.org/10.1029/96jd03003, 1996.
Tesche, M., Gross, S., Ansmann, A., MÜLler, D., Althausen, D., Freudenthaler, V., and Esselborn, M.: Profiling of Saharan dust and biomass-burning smoke with multiwavelength polarization Raman lidar at Cape Verde, Tellus B, 63, 649–676, https://doi.org/10.1111/j.1600-0889.2011.00548.x, 2011.
Toledano, C., Cachorro, V. E., Berjon, A., de Frutos, A. M., Sorribas, M., de la Morena, B. A., and Goloub, P.: Aerosol optical depth and Ångström exponent climatology at El Arenosillo AERONET site (Huelva, Spain), Q. J. Roy. Meteor. Soc., 133, 795–807, https://doi.org/10.1002/qj.54, 2007.
Toth, T. D., Zhang, J., Campbell, J. R., Hyer, E. J., Reid, J. S., Shi, Y., and Westphal, D. L.: Impact of data quality and surface-to-column representativeness on the PM2.5 / satellite AOD relationship for the contiguous United States, Atmos. Chem. Phys., 14, 6049–6062, https://doi.org/10.5194/acp-14-6049-2014, 2014.
Tripathi, S. N., Dey, Sagnik, Chandel, A., Srivastava, S., Singh, Ramesh P., and Holben, B. N.: Comparison of MODIS and AERONET derived aerosol optical depth over the Ganga Basin, India, Ann. Geophys., 23, 1093–1101, https://doi.org/10.5194/angeo-23-1093-2005, 2005.
van Beelen, A. J., Roelofs, G. J. H., Hasekamp, O. P., Henzing, J. S., and Röckmann, T.: Estimation of aerosol water and chemical composition from AERONET Sun–sky radiometer measurements at Cabauw, the Netherlands, Atmos. Chem. Phys., 14, 5969–5987, https://doi.org/10.5194/acp-14-5969-2014, 2014.
Wai, K. M., Wu, S., Kumar, A., and Liao, H.: Seasonal variability and long-term evolution of tropospheric composition in the tropics and Southern Hemisphere, Atmos. Chem. Phys., 14, 4859–4874, https://doi.org/10.5194/acp-14-4859-2014, 2014.
Wang, J. and Christopher, S. A.: Intercomparison between satellite-derived aerosol optical thickness and PM2.5 mass: implications for air quality studies, Geophys. Res. Lett., 30, 2095, https://doi.org/10.1029/2003gl018174, 2003.
Wang, K., Dickinson, R. E., and Liang, S.: Clear Sky Visibility Has Decreased over Land Globally from 1973 to 2007, Science, 323, 1468–1470, https://doi.org/10.1126/science.1167549, 2009.
Wang, Z. and Sassen, K.: Cloud type and macrophysical property retrieval using multiple remote sensors, J. Appl. Meteor., 40, 1665–1682, 2001.
Wang, Z., Liu, Y., Hu, M., Pan, X., Shi, J., Chen, F., He, K., Koutrakis, P., and Christiani, D. C.: Acute health impacts of airborne particles estimated from satellite remote sensing, Environ. Int., 51, 150–159, 2013.
Wardoyo, A. Y.: Biomass burning : particle emissions, characteristics, and airborne measurements PhD, Faculty of Science, Queensland University of Technology, Queensland University of Technology, 257 pp., 2007.
Xian, P., Reid, J. S., Atwood, S. A., Johnson, R. S., Hyer, E. J., Westphal, D. L., and Sessions, W.: Smoke aerosol transport patterns over the Maritime Continent, Atmos. Res., 122, 469–485, https://doi.org/10.1016/j.atmosres.2012.05.006, 2013.
Zhong, B., Liang, S., and Holben, B.: Validating a new algorithm for estimating aerosol optical depths over land from MODIS imagery, Int. J. Remote Sens., 28, 4207–4214, 2007.
Short summary
Southeast Asia stands out globally, as it hosts one of the most complex meteorological and environmental conditions, making remote sensing difficult both for AERONET and satellites. Cloud-cleared data leave gaps in our remote sensing data record, and conversely, residual cloud contamination of remotely sensed data causes challenging tasks for scientists studying aerosols. With the main motivation of overcoming this problem, an AOD-predicting model is proposed.
Southeast Asia stands out globally, as it hosts one of the most complex meteorological and...
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